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At least 793 records · Page 44

A methodology for domain overlapping coupling of thermal-hydraulic systems

Multi-scale coupling has increasingly drawn attention as a promising approach for modeling thermal systems. Traditional system codes provide fast and robust predictions at the plant scale, while high-fidelity computational fluid dynamics (CFD)-based tools resolve localized flow and heat transfer phenomena with greater accuracy. By combining these complementary strengths, co-simulations enable multi-scale analysis that would otherwise be computationally prohibitive for a standalone CFD code. Here, this work introduces a robust and problem-agnostic domain overlapping (DO) coupling between the system thermal-hydraulic (STH) code System Analysis Module (SAM) and the coarse-mesh CFD code Pronghorn. Both applications belong to the Comprehensive Reactor Analysis Bundle (BlueCRAB) code suite, a code suite in active development at the Idaho National Laboratory (INL), tailored for multi-physics analysis of advanced reactors. Unlike previous approaches, BlueCRAB supports an agnostic interface between codes based on different fidelity, while its coupling formulation can address arbitrary flow geometries with multiple inlets and outlets in coupled components. The implemented method leads to consistent pressure drops, enthalpies, and scalar concentrations between coupled SAM and Pronghorn simulations. The methodology is demonstrated through two verification tests, which ensure the numerical consistency and conservation across the codes, and through one validation test against experimental data. The proposed problems explore different physical aspects inherent to thermal systems, with particular attention given to nuclear reactor analysis. These include buoyancy-driven flows, complex flow patterns, and setups with multiple inlets and outlets, representing challenges in advanced reactor applications.

22 - GENERAL STUDIES OF NUCLEAR REACTORS↗

Multifidelity uncertainty quantification with models based on dissimilar parameters

Multifidelity uncertainty quantification (MF UQ) sampling approaches have been shown to significantly reduce the variance of statistical estimators while preserving the bias of the highest-fidelity model, provided that the low-fidelity models are well correlated. However, maintaining a high level of correlation can be challenging, especially when models depend on different input uncertain parameters, which drastically reduces the correlation. Existing MF UQ approaches do not adequately address this issue. In this work, we propose a new sampling strategy that exploits a shared space to improve the correlation among models with dissimilar parameterization. We achieve this by transforming the original coordinates onto an auxiliary manifold using the adaptive basis (AB) method (Tipireddy and Ghanem, 2014). The AB method has two main benefits: (1) it provides an effective tool to identify the low-dimensional manifold on which each model can be represented, and (2) it enables easy transformation of polynomial chaos representations from high- to low-dimensional spaces. This latter feature is used to identify a shared manifold among models without requiring additional evaluations. Here we present two algorithmic flavors of the new estimator to cover different analysis scenarios, including those with legacy and non-legacy high-fidelity (HF) data. We provide numerical results for analytical examples, a direct field acoustic test, and a finite element model of a nuclear fuel assembly. For all examples, we compare the proposed strategy against both single-fidelity and MF estimators based on the original model parameterization.

42 ENGINEERING↗

{sup 1}H relaxation enhancement induced by nanoparticles in solutions: Influence of magnetic properties and diffusion

Magnetic nanoparticles that induce nuclear relaxation are the most promising materials to enhance the sensitivity in Magnetic Resonance Imaging. In order to provide a comprehensive understanding of the magnetic field dependence of the relaxation enhancement in solutions, Nuclear Magnetic Resonance {sup 1}H spin-lattice relaxation for decalin and toluene solutions of various Fe{sub 2}O{sub 3} nanoparticles was investigated. The relaxation experiments were performed in a frequency range of 10 kHz–20 MHz by applying Field Cycling method, and in the temperature range of 257–298 K, using nanoparticles differing in size and shape: spherical – 5 nm diameter, cubic – 6.5 nm diameter, and cubic – 9 nm diameter. The relaxation dispersion data were interpreted in terms of a theory of nuclear relaxation induced by magnetic crystals in solution. The approach was tested with respect to its applicability depending on the magnetic characteristics of the nanocrystals and the time-scale of translational diffusion of the solvent. The role of Curie relaxation and the contributions to the overall {sup 1}H spin-lattice relaxation associated with the electronic spin-lattice and spin-spin relaxation was thoroughly discussed. It was demonstrated that the approach leads to consistent results providing information on the magnetic (electronic) properties of the nanocrystals, i.e., effective electron spin and relaxation times. In addition, features of the {sup 1}H spin-lattice relaxation resulting from the electronic properties of the crystals and the solvent diffusion were explained.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

One-proton and one-neutron knockout reactions from N = Z = 28 56 Ni to the A = 55 mirror pair 55 Co and 55 Ni

Here, we present a high-resolution in-beamγ-ray spectroscopy study of excited states in the mirror nuclei 55 Co and 55 Ni following one-nucleon knockout from a projectile beam of 56 Ni. The newly determined partial cross sections and theγ-decay properties of excited states provide a test of state-of-the-art nuclear structure models and probe mirror symmetry in unique ways. The new experimental data are compared to large-scale shell-model calculations in the full pf space and including charge-dependent contributions. A mirror asymmetry for the partial cross sections leading to the two lowest 3/2 – states in the A = 55 mirror pair was identified as well as a significant difference in the E 1 decays from the 1/2 + 1 state to the same two 3/2 – states. The mirror asymmetry in the partial cross sections cannot be reconciled with the present shell-model picture or small mixing introduced in a two-state model. The observed mirror asymmetry in theE1 decay pattern, however,points at stronger mixing between the two lowest 3/2 – states in 55 Co than in its mirror 55 Ni.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

The propagation of seismic waves, misinformation, and disinformation from the 2024-10-05 M 4.5 Iran earthquake

The 2024-10-05 Iran M 4.5 earthquake took place at a time of heightened tensions in the Middle East. We perform a discrimination and moment tensor analysis and identify a shallow-dipping, reverse fault source commensurate with the compressional setting of the Iranian interior. Nonetheless, the event's aftermath saw widespread dissemination of misinformation, and potentially active disinformation, concluding that it was in fact a test of an Iranian nuclear weapon. The 'evidence' for many of these claims was based on inaccurate interpretation of seismic data. In this paper, we analyze how geophysical 'fake news' propagated through social media (mainly Twitter/X) following this event, eventually gaining traction in mainstream, earned media. This event is an illustrative warning of how seismic data can be misinterpreted and/or manipulated in public discourse.

58 GEOSCIENCES↗

Early User Test: BISON for Fission Gas Release Modeling

As a test to develop an understanding of the capabilities and input of the nuclear fuel performance code BISON, we modeled the fission gas release of the Oconee rod 15309 as there is benchmark data available for comparison. BISON has two fission gas models available, the Forsber-Massih model and the Simple Integrated Fission Gas Release and Swelling [sifgrs] model. Due to time constraints and availability of model parameters [we did not have all of the parameters for the sifgrs model already in hand] we only tested the Forsberg-Massih model. The Oconee rod test has been used in a number of benchmark studies including the integral assessment of FRAPCON 3.4. The Oconee Rod test is a 5-cycle test bundle with an average burnup of 50GWd/MTU. The FRAPCON assessment predicted that Oconee Rod15309 Test case would release 1.25% of all fission gas produced, while experimentally only 0.8% was released at EOL. Other studies using BISON with the sifgrs model have under predicted EOL fission gas release [FGR].

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Non-Destructive Evaluation of Polyolefin Thermal Aging Using Infrared Spectroscopy

Fourier transform infrared (FTIR) spectroscopy is an information-rich method that reveals chemical bonding near the surface of polymer composites. FTIR can be used to verify composite composition, identify chemical contaminants and expose composite moisture content. Polymer matrix changes due to thermal exposure including loss of additives, chain scission, oxidation and changes in crystallinity may also be determined using FTIR spectra. Portable handheld instruments using non-contact reflectance or surface contact attenuated total reflectance (ATR) may be used for non-destructive evaluation (NDE) of thermal aging in polymer and composite materials of in-service components. We report the use of ATR FTIR to track oxidative thermal aging in ethylene-propylene rubber (EPR) and chlorinated polyethylene (CPE) materials used in medium voltage nuclear power plant electrical cable insulation and jacketing. Mechanical property changes of the EPR and CPE materials with thermal degradation for correlation with FTIR data are tracked using indenter modulus (IM) testing. IM is often used as a local NDE metric of cable jacket health. The FTIR-determined carbonyl index was found to increase with IM and may be a valuable NDE metric with advantages over IM for assessing cable remaining useful life.

aging↗

Sister Rod Destructive Examinations (FY23) Appendix I: SNF Aerosols Released During Rod Fracture

This report documents work performed under the Spent Fuel and Waste Disposition’s Spent Fuel and Waste Science and Technology program for the US Department of Energy (DOE) Office of Nuclear Energy (NE). This work was performed to fulfill Level 3 Milestone M3SF-23OR010201026, “FY23 M3 draft report on results from testing in FY23,” within work package SF-23OR01020102 and is an updated to the work reported in M2SF-23OR010201024, M2SF-22OR010201047, M2SF-21OR010201032, M2SF-19ORO010201026, and M2SF-19OR010201028. As a part of the DOE NE High Burnup Spent Fuel Data Project, Oak Ridge National Laboratory (ORNL) is performing destructive examinations (DEs) of high burnup (HBU) (>45 GWd/MTU) spent nuclear fuel (SNF) rods from the North Anna Nuclear Power Station operated by Dominion Energy. The SNF rods, called sister rods or sibling rods, are all HBU and include four different kinds of fuel rod cladding: standard Zircaloy-4 (Zirc-4), low-tin Zirc-4, ZIRLO, and M5. The DEs are being conducted to obtain a baseline of the HBU rods’ condition before dry storage and are focused on understanding overall SNF rod strength and durability. Fuel rods and defueled cladding will be tested to derive material properties. Although the data generated can be used for multiple purposes, one primary goal for obtaining the post-irradiation examination data and the associated measured mechanical properties is to support SNF dry storage licensing and relicensing activities by (1) addressing identified knowledge gaps and (2) enhancing the technical basis for post-storage transportation, handling, and subsequent disposition.This report documents the status of the ORNL Phase 1 DE activities related to the collection of SNF aerosol particles released during fuel rod fracture in 4-point bending in Phase 1 of the sister rod test program.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

AGR Irradiated Specimen Air/Moisture Heating Test Plan

The Advanced Gas Reactor (AGR) program has a need to perform high-temperature oxidation testing of tristructural isotropic (TRISO)-coated particle fuel and reactor core materials to evaluate their performance under conditions relevant to air- and moisture-ingress events in high-temperature gas-cooled reactors (HTGRs). The objectives of these tests are to assess the impact of oxidizing environments on fission product release from exposed fuel kernels, compact matrix, and nuclear grade graphite, and to determine the impact of oxidizing environments on TRISO coating integrity. The program is currently developing a capability for testing irradiated fuel, matrix, and graphite specimens inside a hot cell. The Air/Moisture Ingress Experiment (AMIX) system will be capable of temperatures up to 1650°C in atmospheres containing oxygen or moisture with varying concentrations. The system will be capable of collecting fission gases as well as condensable fission products, in order to quantify total released inventory from the heated specimens. A basis for establishing experimental test matrices, and the test matrices themselves, are presented in this document. This includes considerations on specific objectives for the tests, types of oxidizing environments that should be tested, and the expected availability of irradiated specimens from the various AGR program irradiation experiments. This document only briefly discusses post-test analysis of the heated specimens, and it is recognized that in many cases the post-test analysis may be extensive. It is expected that this will be a “living” document, subject to revision as data are collected and scoping calculations are performed.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

US-ROK Action Sheet 34: Safeguards Application of a Hand-held Mechanically Cooled Germanium Spectrometer

This report summarizes results of Action Sheet 34 - for the cooperative efforts on the field testing and evaluation of a high-resolution, hand-held, gamma-ray spectrometer, known as SPG (Spectroscopic Planar Germanium), for safeguards application such as short notice inspections, UF6 analysis, enrichment determination, and other potential applications. The Spectroscopic Planar Germanium (SPG) has been demonstrated IAEA Physical Inventory Verification (PIV) in South Korea. This field test was a success and the feedback provided by KINAC, IAEA, and national laboratory staff was used to direct efforts to improve the instrument this year. Key points in this report include measurement results from PIV, analysis of spectra with commercially available Ortec U235 and PC-FRAM, and completion of tripod and tungsten collimator and integration of user feedback.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Frequency spectrum analysis code for nuclear noise based on improved wavelet algorithm - 337

The core of the narrow flow channel generally faced the problem of local bubble boiling with the temperature rise of the nuclear fuel element, it is necessary and meaningful to answer and deal with the problem on the technical level. Reactor noise analysis begins with the study of the physical characteristics of the core, after nearly 30 years of research and development it has become a powerful tool in the auxiliary monitoring of the power reactor operating. By using this noise frequency spectrum analysis technology, the reactor dynamic parameter such as prompt neutron decay constant can be measured. Also, through such system, the frequency characteristics of reactor can be real-time monitored, which is helpful for safety operation and fault diagnosis. Spectrum analysis technology in the Fourier analysis era is now barely available, the reason is that the local spectral characteristics of this technology are not obvious, but this defect can be greatly improved by wavelet analysis technique, however, the traditional wavelet analysis will introduce the problem of spectral confusion. To solve the problem, based on the improved wavelet algorithm, frequency spectrum analysis code for nuclear noise is developed,from the perspective of fine spectral analysis, the local boiling accident of the coolant can be prejudged and avoid. Based on the analysis and test of experimental data,The results show that the calculation ability of the code is in accordance with the expected, it can be applied in the operation of research reactor. (authors)

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Predictive based monitoring of nuclear plant component degradation using support vector regression

Nuclear power plants (NPPs) are large installations comprised of many active and passive assets. Degradation monitoring of all these assets is expensive (labor cost) and highly demanding task. In this paper a framework based on Support Vector Regression (SVR) for online surveillance of critical parameter degradation of NPP components is proposed. In this case, on time replacement or maintenance of components will prevent potential plant malfunctions, and reduce the overall operational cost. In the current work, we apply SVR equipped with a Gaussian kernel function to monitor components. Monitoring includes the one-step-ahead prediction of the component’s respective operational quantity using the SVR model, while the SVR model is trained using a set of previous recorded degradation histories of similar components. Predictive capability of the model is evaluated upon arrival of a sensor measurement, which is compared to the component failure threshold. A maintenance decision is based on a fuzzy inference system that utilizes three parameters: (i) prediction evaluation in the previous steps, (ii) predicted value of the current step, (iii) and difference of current predicted value with components failure thresholds. The proposed framework will be tested on turbine blade degradation data.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Bayesian Exploration of Phenomenological EoS of Neutron/Hybrid Stars with Recent Observations

The description of the stellar interior of compact stars remains as a big challenge for the nuclear astrophysics community. The consolidated knowledge is restricted to density regions around the saturation of hadronic matter ρ 0 =2.8 × 10 14 g cm -3 , regimes where our nuclear models are successfully applied. As one moves towards higher densities and extreme conditions up to the quark/gluons deconfinement, little can be said about the microphysics of the equation of state (EoS). Here, we employ a Markov Chain Monte Carlo (MCMC) strategy to access the variability at high density regions of polytropic piecewise models for neutron star (NS) EoS or possible hybrid stars, i.e., a NS with a small quark-matter core. With a fixed description of the hadronic matter for low density, below the nuclear saturation density, we explore a variety of models for the high density regimes leading to stellar masses near to 2.5 M ⊙ , in accordance with the observations of massive pulsars. The models are constrained, including the observation of the merger of neutrons stars from VIRGO-LIGO and with the pulsar observed by NICER. In addition, we also discuss the possibility of the use of a Bayesian power regression model with heteroscedastic error. The set of EoS from the Laser Interferometer Gravitational-Wave Observatory (LIGO) was used as input and treated as the data set for the testing case.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Fire-Induced Pressure Response and Failure Characterization of PCV/SCV/3013 Containers - Phase 3

Several Department of Energy (DOE) facilities have materials stored in robust, welded, stainless - steel containers with presumed fire - induced pressure response behaviors. Lack of test data related to fire exposure requires conservative safety analysis assumptions for container response at these facilities. This conservatism can in turn result in the implementation of challenging operational restrictions with costly nuclear safety controls. To help address this issue for sites that store DOE 3013 stainless - steel containers, a series of ten tests were undertaken at Sandia National Laboratories. The goal of this test series was to obtain the response behavior for various configurations of DOE 3013 containers with various payload compositions when exposed to one of two ASTM fire conditions. Key parameters measured in the test series included identification of failure - specific characteristics such as pressure, temperature, and whether or not a vessel was breached during a test . Numerous failure - specific characteristics were identified from the ten tests. This report describes the implementation and execution of the test series performed to identify these failure - specific characteristics. Discussions on the test configurations, payload compositions, thermal insults, and experimental setups are presented. Test results in terms of pressurization and vessel breach (or no - breach) are presented along with corresponding discussions for each test.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Modeling Astrophysical Explosions and the Nucleosynthesis of the Heavy Elements

The heavier elements in the Universe were created and dispersed in the supernova explosions of stars. These events involve a fascinating interplay of nuclear physics, gravity, hydrodynamics, neutrino and photon transport, and radioactive decay, all occurring under extreme conditions. Astronomical experiments provide a rich and constraining data set, but our theoretical understanding of supernovae remains incomplete. The goal of this project is to advance numerical models of astrophysical explosions and use them to connect the nuclear theory of supernovae to current observational and experimental programs. Our contributions focus on one important aspect of the problem --modeling the transport of radiation (both neutrino and electromagnetic) which is essential to understanding the supernova explosion mechanism, the resulting nucleosynthesis, and the observable spectra and light curves. We will exploit recent advances in high performance computing to improve 3-dimensional simulations of core collapse supernovae and neutron star mergers. The benefits include: 1) Further defining the explosive astrophysical environments that govern the nucleosynthesis of r-process nuclei. 2) Preparing the way for more realistic treatments of neutrino interactions, with the ultimate goal of making supernovae a testing ground for probing fundamental neutrino physics, e.g., unknown mixing angles and new aspects of the MSW mechanism. 3) Providing a means for testing explosion simulations and nucleosynthesis calculations against data from optical and x-ray telescopes, thereby permitting the experimental validation or falsification of supernova models. 4) Helping position nuclear physics, through the development of new algorithms of the type incorporated in our simulation codes, to play a leading role in DOE large scale computing.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

SNM Radiation Signature Classification Using Different Semi-Supervised Machine Learning Models

The timely detection of special nuclear material (SNM) transfers between nuclear facilities is an important monitoring objective in nuclear nonproliferation. Persistent monitoring enabled by successful detection and characterization of radiological material movements could greatly enhance the nuclear nonproliferation mission in a range of applications. Supervised machine learning can be used to signal detections when material is present if a model is trained on sufficient volumes of labeled measurements. However, the nuclear monitoring data needed to train robust machine learning models can be costly to label since radiation spectra may require strict scrutiny for characterization. Therefore, this work investigates the application of semi-supervised learning to utilize both labeled and unlabeled data. As a demonstration experiment, radiation measurements from sodium iodide (NaI) detectors are provided by the Multi-Informatics for Nuclear Operating Scenarios (MINOS) venture at Oak Ridge National Laboratory (ORNL) as sample data. Anomalous measurements are identified using a method of statistical hypothesis testing. After background estimation, an energy-dependent spectroscopic analysis is used to characterize an anomaly based on its radiation signatures. In the absence of ground-truth information, a labeling heuristic provides data necessary for training and testing machine learning models. Supervised logistic regression serves as a baseline to compare three semi-supervised machine learning models: co-training, label propagation, and a convolutional neural network (CNN). In each case, the semi-supervised models outperform logistic regression, suggesting that unlabeled data can be valuable when training and demonstrating value in semi-supervised nonproliferation implementations.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

Advanced Multiphysics Code Coupling for Cladding Surface Thermocouples During Two-Phase Heat Transfer from Nuclear Fuel

Transient testing of nuclear fuel involves the evaluation of fuel performance under off-normal and accident conditions and is essential for proving design performance. Instrumentation included in such experiments commonly includes thermocouples attached to the outer surface of the cladding to provide temperature measurements throughout the transient. However, the presence of thermocouples on the cladding surface can alter the local heat transfer characteristics with the surrounding coolant. These localized effects can influence the temperature of the nearby cladding surface and introduce uncertainties in interpreting the thermocouple data. Understanding the impact of thermocouples attached to the outer surface of the cladding is crucial for accurate data interpretation as well as its effect on the thermomechanical behavior of the cladding. This paper presents a novel methodology for simulating the impact of outer cladding thermocouples during transient testing of nuclear fuels. The simulation framework leverages the thermal-hydraulic capabilities of RELAP5-3D coupled to the BISON fuel performance code through the RELAPCouplingApp interface. The methodology is compared against Accident Tolerant Fuel Reactivity Initiated Accident-1-E experiment performed at Idaho National Laboratory. The results reveal approximately 100°C difference between thermocouple-altered temperature and virgin cladding surface. The model overpredicts surface rewet time due to conservative correlations.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Data Evaluation of Actinide Cross Sections: 240 Am, 241 Am, and 242 Am

Evaluations for neutron-induced reactions on the isotopes 240 Am, 241 Am, and 242 Am were per formed by optimizing reaction-model calculations based on existing experimental data from both direct measurements and surrogate reactions. The evaluated data were based on results obtained from the LLNL reaction codes YAHFC and FRESCO using up-to-date nuclear models; including an improvement upon some previous treatments for inelastic processes. Nuclear reaction codes generated data for all relevant reaction channels, which were then translated into Generalized Nu clear Data Structure and LLNL’s Evaluated Neutron Data Libraries (ENDL). These data libraries were tested for potential errors and applied to verification and validation (V&V) tests suites where applicable for comparisons.

42 ENGINEERING↗