Search NASA⌕ Search

SEARCH · Search NASA

Results for “nuclear shell model”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.

At least 793 records · Page 44
All sourcesNASA NTRSDOE OSTI
NASA NTRS2007

Coupled Groups of g-Modes in a Sun with Mixed Core

Groups of linear g-modes can sum to create long-lived nonlinear oscillations in small "hot volumes" very deep in the Sun that help drive the modes. In these volumes (dimensions -10 Mm), the time average rate of He-3 burning doubles as temperature fluctuations exceed 10% and rises by an order of magnitude for fluctuations of 25%. To be consistent with locally large motions, we impose a mixed shell on an otherwise standard solar model before computing g-mode solutions. Mixing in the assumed shell r = (0.10+/-0.03) R(sub sun) is rapid (<<10(exp 6) yr) with slower mixing somewhat beyond. If l is the principal spherical harmonic index, a set of g-modes for any single l less than or equal to 15 with five consecutive radial harmonics can be excited with nearly linear thermal amplitudes, A(sub T) less than or equal to 0.053, throughout the star and a fractional temperature fluctuation in its hot volume of (Delta)T/T less than or equal to 0.18. These thresholds for excitation will become smaller when sets for several values of l are computed simultaneously. There is some evidence for the rotation of g-mode sets in the long solar activity record and g-mode upward wave flux has been suggested to explain the 1.3 yr reversing flows tentatively detected below the Sun's convective envelope (CE). The large local amplitudes needed for excitation implies that g-modes may transport a non-negligible fraction of the solar luminosity, yet their near linear amplitudes outside the hot volume suggests amplitudes over most of the solar surface that would be barely detectable for l > 3. A formalism is presented for summing the g-modes and estimating growth rates under the approximation that modes are strictly linear except in a hot volume which holds only a few percent of mode kinetic energy. Finally over the range 2 less than or equal to l less than or equal to 30, we summed all zonal harmonics, m, for a given l and computed the relative angular orientations that would release the most nuclear energy. This should be close to the physically preferred angular state of such a family and a few examples were displayed.

Wolff, Charles L.↗
DOE OSTI2024

Measurements of dense fuel hydrodynamics in the NIF burning plasma experiments using backscattered neutron spectroscopy

The hydrodynamics of the dense confining fuel shell is of great importance in defining the behavior of the burning plasma and burn propagation regimes of inertial confinement fusion experiments. However, it is difficult to probe due to its low emissivity in comparison with the central fusion core. In this work, we utilize the backscattered neutron spectroscopy technique to directly measure the hydrodynamic conditions of the dense fuel during fusion burn. Experimental data are fit to obtain dense fuel velocities and apparent ion temperatures. Trends of these inferred parameters with yield and velocity of the burning plasma are used to investigate their dependence on alpha heating and low mode drive asymmetry. It is shown that the dense fuel layer has an increased outward radial velocity as yield increases, showing that burn has continued into re-expansion, a key signature of hotspot ignition. A comparison with analytic and simulation models shows that the observed dense fuel parameters are displaying signatures of burn propagation into the dense fuel layer, including a rapid increase in dense fuel apparent ion temperature with neutron yield.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2024

New isomeric transition in Mg 36 : Bridging the N = 20 and N = 28 islands of inversion

Here, we observed a new isomeric γ transition at 168 keV in 36 Mg, with a half-life of T1/2=90⁢($^{+410}_{-50}$) ns. We propose that the observed transition deexcites a new 0 + isomeric state at 833 keV and populates the previously known first 2 + state. The existence of this isomer is consistent with the predictions of the large-scale shell-model calculations of 36 Mg using the sdpf-u-mix interaction. The observed excitation energy of the second 0 + state is caused by the small energy separation between two prolate-deformed configurations where the intruder configuration corresponds to two-neutron excitations from the sd to the pf shell. Within this interpretation, 36 Mg becomes the crossing point between nuclei in which ground state deformed/superdeformed configurations are caused by the dominance of N=20 intruders ( 32,34 Mg) and nuclei where deformed configurations are associated with the breaking of the N=28 closure and a large occupancy of the 1⁢p 3/2 neutron orbit ( 38 Mg and beyond). We found the lack of three-body monopole corrections in other effective interactions results in a predominance of N=20 intruder configurations past 38 Mg incompatible with our observation. We conclude that 36 Mg bridges the N=20 and N=28 islands of inversion, forming the so-called big island of deformation.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2017

The effects of convergence ratio on the implosion behavior of DT layered inertial confinement fusion capsules

The wetted foam capsule design for inertial confinement fusion capsules, which includes a foam layer wetted with deuterium-tritium liquid, enables layered capsule implosions with a wide range of hot-spot convergence ratios (CR) on the National Ignition Facility. In this paper, we present a full-scale wetted foam capsule design that demonstrates high gain in one-dimensional simulations. In these simulations, increasing the convergence ratio leads to an improved capsule yield due to higher hot-spot temperatures and increased fuel areal density. High-resolution two-dimensional simulations of this design are presented with detailed and well resolved models for the capsule fill tube, support tent, surface roughness, and predicted asymmetries in the x-ray drive. Our modeling of these asymmetries is validated by comparisons with available experimental data. In 2D simulations of the full-scale wetted foam capsule design, jetting caused by the fill tube is prevented by the expansion of the tungsten-doped shell layer due to preheat. While the impacts of surface roughness and predicted asymmetries in the x-ray drive are enhanced by convergence effects, likely underpredicted in 2D at high CR, simulations predict that the capsule is robust to these features. Nevertheless, the design is highly susceptible to the effects of the capsule support tent, which negates all of the one-dimensional benefits of increasing the convergence ratio. Indeed, when the support tent is included in simulations, the yield decreases as the convergence ratio is increased for CR > 20. Finally and nevertheless, the results suggest that the full-scale wetted foam design has the potential to outperform ice layer capsules given currently achievable levels of asymmetries when fielded at low convergence ratios (CR < 20).

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2017

Using FENOSOL{sup TM} Phenolic Foam as a Shock Absorber for Type B Packaging - 17256

Type B and fissile material transportation packages are designed to withstand deformation from dynamic forces experienced during impacts in hypothetical accident conditions. A critical aspect is to ensure the containment system is not breached. The package design normally includes impact limiters made up of a shell filled with energy-absorbing material. Various types of materials are used as energy absorbers, including wood, foam, and honeycomb structures. Synthetic foam is an ideal material for impact limiters; it has isotropic material properties, it acts as a heat insulator during fire conditions, and it maintains structural integrity at high temperatures. In addition, the density of the foam may be controlled during the manufacturing process, allowing the cask designer flexibility to select the right density for each application. The foam properties can be used as inputs for numerical simulations of dynamic impacts. These simulations are a key component of the safety analysis report for Type B transportation casks. Robatel has recently invested in equipment to produce FENOSOL{sup TM} phenolic foam in our factory for use in our cask designs. This acquisition was made jointly between Robatel and the CEA, with Robatel ensuring the industrialization of the product. In the past decade, this foam was successfully integrated into more than 10 European cask designs, and there has been extensive in-laboratory characterization of its properties. FENOSOL{sup TM} has already been accepted by the French Nuclear Safety Authority (ASN) as a shock absorbing material for use in cask designs. Since the acquisition of the phenolic foam production process by Robatel, a new research and development program has been launched to provide more accurate information to our clients, extend the range of application of this foam, and to improve its properties. Robatel has built an extensive database of material characteristics through the use of a universal mechanical tester, a scanning electron microscope, and a nuclear magnetic resonance spectrometer. In addition, Robatel has successfully implemented FENOSOL{sup TM} in two recent cask designs. This included scale model drop testing of a 9 meter drop in three orientations, and a pin puncture drop test. Robatel is in the process of producing FENOSOL{sup TM} samples for testing according to ASTM standards. Various densities will be included in the study. The testing will include duro-meter hardness, specific heat, thermal conductivity, compressive strength and modulus, and tensile strength. Once the testing is complete, Robatel will compile the data in the form of product specification sheets for each density. These information sheets and test reports will be used to validate FENOSOL{sup TM} for use in future impact limiters for the North American Type B cask market. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
DOE OSTI2017

Indirect study of the stellar Ar 34 ( α , p ) K 37 reaction rate through Ca 40 ( p , t ) Ca 38 reaction measurements

The 34 Ar(α,p) 37 K reaction is believed to be one of the last in a sequence of (α,p) and (p,γ) reactions within the T z = -1 , sd-shell nuclei, known as the αp-process. This process is expected to influence the shape and rise times of luminosity curves coming from type I x-ray bursts (XRBs). With very little experimental information known on many of the reactions within the αp-process, stellar rates are calculated using a statistical model, such as Hauser-Feshbach. Questions on the applicability of a Hauser-Feshbach model for the 34 Ar (α,p) 37 K reaction arise due to level density considerations in the compound nucleus, 38 Ca . We have performed high energy-resolution forward-angle 40 Ca (p,t) 38 Ca measurements with the K = 600 spectrograph at iThemba LABS in order to identify levels above the α-threshold in 38 Ca . States identified in this work were then used to determine the 34 Ar (α,p) 37 K reaction rate based on a narrow-resonance formalism. Comparisons are made to two standard Hauser-Feshbach model predicted rates at XRB temperatures.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2025

Valence 1⁢𝑠−0⁢𝑑 proton vacancy of the 32 Si ground state

The 32 Si( 3 He,d) 33 P reaction was studied in inverse kinematics at 6.3 MeV/u. States in 33 P corresponding to the proton 1s-0d single-particle orbitals were identified up to ≈ 4.5 MeV in excitation energy. The ( 3 He,d) spectroscopic factors were determined from distorted-wave Born approximation calculations. When combined with complementary neutron-adding data, the 1s-0d proton vacancies in the 32 Si ground state were extracted. In conjunction with a reanalysis of data from previous single-particle measurements, the trends in proton and neutron vacancy were explored across the 28,30,32,34 Si isotopes. Both proton and neutron vacancy data show gradual changes in their occupancies. The proton 1s 1/2 orbitals in 32 Si and 34 Si are both consistent with being empty. In conclusion, the ground-state nucleon distributions are described by shell-model calculations constrained to the 1s-0d model space.

Watwood, N. [Argonne National Laboratory (ANL), Ar↗
DOE OSTI2018

Microscopically based energy density functionals for nuclei using the density matrix expansion. II. Full optimization and validation

Background: Energy density functional methods provide a generic framework to compute properties of atomic nuclei starting from models of nuclear potentials and the rules of quantum mechanics. Until now, the overwhelming majority of functionals have been constructed either from empirical nuclear potentials such as the Skyrme or Gogny forces, or from systematic gradient-like expansions in the spirit of the density functional theory for atoms. Purpose: In this study, we seek to obtain a usable form of the nuclear energy density functional that is rooted in the modern theory of nuclear forces. We thus consider a functional obtained from the density matrix expansion of local nuclear potentials from chiral effective field theory. We propose a parametrization of this functional carefully calibrated and validated on selected ground-state properties that is suitable for large-scale calculations of nuclear properties. Methods: Our energy functional comprises two main components. The first component is a non-local functional of the density and corresponds to the direct part (Hartree term) of the expectation value of local chiral potentials on a Slater determinant. Contributions to the mean field and the energy of this term are computed by expanding the spatial, finite-range components of the chiral potential onto Gaussian functions. The second component is a local functional of the density and is obtained by applying the density matrix expansion to the exchange part (Fock term) of the expectation value of the local chiral potential. We apply the UNEDF2 optimization protocol to determine the coupling constants of this energy functional. Results: We obtain a set of microscopically constrained functionals for local chiral potentials from leading order up to next-to-next-to-leading order with and without three-body forces and contributions from Δ excitations. These functionals are validated on the calculation of nuclear and neutron matter, nuclear mass tables, single-particle shell structure in closed-shell nuclei, and the fission barrier of 240 Pu . Quantitatively, they perform noticeably better than the more phenomenological Skyrme functionals. Conclusions: The inclusion of higher-order terms in the chiral perturbation expansion seems to produce a systematic improvement in predicting nuclear binding energies while the impact on other observables is not really significant. In conclusion, this result is especially promising since all the fits have been performed at the single-reference level of the energy density functional approach, where important collective correlations such as center-of-mass correction, rotational correction, or zero-point vibrational energies have not been taken into account yet.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2017

High-spin structures in Xe 132 and Xe 133 and evidence for isomers along the N = 79 isotones

In this study, the transitional nuclei 132 Xe and 133 Xe are investigated after multinucleon-transfer (MNT) and fusion-evaporation reactions. Both nuclei are populated (i) in 136 Xe + 208 Pb MNT reactions employing the high-resolution Advanced GAmma Tracking Array (AGATA) coupled to the magnetic spectrometer PRISMA, (ii) in the 136 Xe + 198 Pt MNT reaction employing the GAMMASPHERE spectrometer in combination with the gas-detector array CHICO, and (iii) as an evaporation residue after a 130 Te (α,xn) 134-xn Xe fusion-evaporation reaction employing the HORUS γ -ray array at the University of Cologne. The high-spin level schemes are considerably extended above the J π = (7 - ) and (10 + ) isomers in 132 Xe and above the 11/2 - isomer in 133 Xe. The results are compared to the high-spin systematics of the Z = 54 as well as the N = 78 and N = 79 chains. Furthermore, evidence is found for a long-lived (T 1/ 2 » 1 μs) isomer in 133 Xe which closes a gap along the N = 79 isotones. Finally, shell-model calculations employing the SN100PN and PQM130 effective interactions reproduce the experimental findings and provide guidance to the interpretation of the observed high-spin features.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

A database and meta-analysis on the performance of exploding pusher implosions conducted at OMEGA

A database of 222 exploding pusher implosions conducted at the OMEGA Laser Facility is presented. The dataset consists of glass-shell capsules filled with varying pressures of D 2 , T 2 , and 3 He, which were imploded using square laser pulses with intensities ranging from 1 to 1 × 10 15 W/cm 2 . The database includes measurements of bang times, ion temperatures, and yields from the DD, D 3 He, and DT fusion reactions. A semi-analytic exploding pusher model is introduced, which effectively captures the observed trends in the data. This model predicts that the measurements scale according to a power-law relation based on the initial capsule and laser conditions. A generalized power-law scaling relation is directly fit to each dataset, providing a useful interpolation of the entire database. Overall, the database provides a valuable resource to estimating bang times, temperatures, and yields for the design of future experiments. Additionally, it provides a diverse set of data for validating more advanced implosion physics models.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2020

CISME report on experiments with HMX powder, PBX 9501 prills, and heated PBX 9501

The ability to predict post-ignition explosive response is relevant to explosives safety, particularly weapons assembly/disassembly operations that must operate under a sufficiently conservative safety basis to meet risk mitigation criteria for inadvertent nuclear detonation (IND). In particular, hazard determinations hinge on whether the PBX 9501 main charge can ultimately attain detonation from an initial, non-shock, ignition stimulus. The CISME experiment uses a spherical explosive charge, which is thermally ignited in the center using a fiber-delivered infrared laser pulse. This ignition mechanism - i.e. a localized thermal hotspot - is representative of the ignition-causing insults typical in accident scenarios, including low-velocity impact, drop, skid, and punch events. In fiscal year 2018 CISME experiments were conducted with pristine PBX 9501 spheres, confined and unconfined. Sub-detonative, low-violence reactions were observed. Here we report experiments conducted since 2018. The explosive charge was varied: experiments were conducted with room temperature pour-density HMX powder and prills of PBX 9501, and heated, thermally damaged PBX 9501. Experiments were conducted in a confined configuration, with two 4 mm-thick stainless-steel hemispherical shells bolted around the sphere. Detonation, via DDT (deflagration-to-detonation transition) was observed in the 3-inch diameter powdered HMX and the 6-inch diameter heated and thermally-damaged PBX 9501 tests. No transition to DDT was observed in smaller diameters for those configurations, and no DDT was observed for pour-density prills of PBX 9501 of any diameter. The original test series demonstrated that the response of pristine, undamaged PBX 9501 to a central ignition is relatively benign. This new test series shows that increased porosity, lack of polymer binders and thermal damage can greatly increase the violence of the post-ignition response, up to and including detonation. These results bridge the explosive response of PBX 9501 from sub-detonative through detonation as a function of diameter and provide valuable test cases for modeling efforts that strive to capture the DDT threshold. By exploring explosive response in a more representative 3D geometry, we can also benchmark these new results to more plentiful DDT datasets generated from testing in 1D tube confinement (the historical test configuration)–the configuration upon which almost all DDT models were developed.

42 ENGINEERING↗
DOE OSTI2017

Electronic Structure and Properties of Berkelium Iodates

The reaction of 249 Bk(OH) 4 with iodate under hydrothermal conditions results in the formation of Bk(IO 3 ) 3 as the major product with trace amounts of Bk(IO 3 ) 4 also crystallizing from the reaction mixture. The structure of Bk(IO 3 ) 3 consists of nine-coordinate Bk III cations that are bridged by iodate anions to yield layers that are isomorphous with those found for Am III , Cf III , and with lanthanides that possess similar ionic radii. Bk(IO 3 ) 4 was expected to adopt the same structure as M(IO 3 ) 4 (M = Ce, Np, Pu), but instead parallels the structural chemistry of the smaller Zr IV cation. Bk III –O and Bk IV –O bond lengths are shorter than anticipated and provide further support for a postcurium break in the actinide series. Photoluminescence and absorption spectra collected from single crystals of Bk(IO 3 ) 4 show evidence for doping with Bk III in these crystals. In addition to luminescence from Bk III in the Bk(IO 3 ) 4 crystals, a broad-band absorption feature is initially present that is similar to features observed in systems with intervalence charge transfer. However, the high-specific activity of 249 Bk ( t 1/2 = 320 d) causes oxidation of Bk III and only Bk IV is present after a few days with concomitant loss of both the BkIII luminescence and the broadband feature. The electronic structure of Bk(IO 3 ) 3 and Bk(IO 3 ) 4 were examined using a range of computational methods that include density functional theory both on clusters and on periodic structures, relativistic ab initio wave function calculations that incorporate spin–orbit coupling (CASSCF), and by a full-model Hamiltonian with spin–orbit coupling and Slater–Condon parameters (CONDON). Some of these methods provide evidence for an asymmetric ground state present in Bk IV that does not strictly adhere to Russel–Saunders coupling and Hund’s Rule even though it possesses a half-filled 5 f 7 shell. Multiple factors contribute to the asymmetry that include 5 f electrons being present in microstates that are not solely spin up, spin–orbit coupling induced mixing of low-lying excited states with the ground state, and covalency in the Bk IV –O bonds that distributes the 5f electrons onto the ligands. These factors are absent or diminished in other f 7 ions such as Gd III or Cm III .

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2017

Isomers and high-spin structures in the N = 81 isotones Xe 135 and Ba 137

In this study, the high-spin structures and isomers of the N=81 isotones 135 Xe and 137 Ba are investigated after multinucleon-transfer (MNT) and fusion-evaporation reactions. Both nuclei are populated (i) in 136 Xe + 238 U and (ii) 136 Xe+ 208 Pb MNT reactions employing the high-resolution Advanced Gamma Tracking Array (AGATA) coupled to the magnetic spectrometer PRISMA, (iii) in the 136 Xe+ 198 Pt MNT reaction employing the γ-ray array GAMMASPHERE in combination with the gas-detector array CHICO, and (iv) via a 11 B+ 130 Te fusion-evaporation reaction with the HORUS γ-ray array at the University of Cologne. The high-spin level schemesof 135 Xe and 137 Ba are considerably extended to higher energies. The 2058-keV (19/2 - ) state in 135 Xe is identified as an isomer, closing a gap in the systematics along the N=81 isotones. Its half-life is measured to be 9.0(9) ns, corresponding to a reduced transition probability of B(E2,19/2 - →15/2 - )=0.52(6) W.u. The experimentally deduced reduced transition probabilities of the isomeric states are compared to shell-model predictions. Finally, latest shell-model calculations reproduce the experimental findings generally well and provide guidance to the interpretation of the new levels.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Neutron-proton pairing correction in the extended isovector and isoscalar pairing model

An extended O ST (8) model with multi j-orbits is constructed based on the angular momentum decomposition with “pseudo”-spin S for valence nucleons in a j-orbit. It is shown that the isovector S = 0 and T=1 pairs are exactly the J=0 and T=1 pairs in a given j-orbit, while the isoscalar S = 1 pairs are linear combinations of J=odd pairs, with which the pairing Hamiltonian can be used to estimate isovector and isoscalar pairing interactions. As an example of the model application, some low-lying J = 0 + level energies of even-even and odd-odd A=18 – 28 nuclei up to the half-filling in the ds-shell above the 16 O core are fit by the model and compared with the fitting results of the same Hamiltonian in the O LST (8) form. It has been verified from the fitting of both the models that the isoscalar pairing interaction can be neglected in the lower energy part of the spectra of these ds-shell nuclei as far as binding energies and a few J=0 + excited levels of these nuclei are concerned. With the mean-field plus isovector pairing interaction only, neutron-neutron, proton-proton, and neutron-proton pairing contributions at the ground or the lowest J=0 + state of these nuclei are estimated. It is shown that the isovector np-pairing contribution to the binding in the odd-odd N=Z nuclei is systematically larger than that in the even-even nuclei. Furthermore, the isoscalar np-pair content at the lowest J=0+ state of these nuclei is also estimated. In both the O ST (8) and O LST (8) models, it is clearly shown that the isoscalar-pair content in the lowest J=0 + state of the N=Z and N=Z±2 nuclei increases with increasing of the valence nucleons, especially in those even-even nuclei, which indicates the isoscalar pairing correlation to be of importance at low-lying states of N=Z and N=Z±2 nuclei, especially in those even-even nuclei with more valence nucleons up to the half-filling, even though the isoscalar pairing interaction is negligible.

20 ≤ A ≤ 38↗
DOE OSTI2018

Hypernuclear no-core shell model

We extend the No-Core Shell Model (NCSM) methodology to incorporate strangeness degrees of freedom and apply it to single-Λ hypernuclei. After discussing the transformation of the hyperon-nucleon (YN) interaction into Harmonic-Oscillator (HO) basis and the Similarity Renormalization Group transformation applied to it to improve model-space convergence, we introduce two complementary formulations of the NCSM, one that uses relative Jacobi coordinates and symmetry-adapted basis states to fully exploit the symmetries of the hypernuclear Hamiltonian, and one working in a Slater determinant basis of HO states where antisymmetrization and computation of matrix elements is simple and to which an importance-truncation scheme can be applied. For the Jacobi-coordinate formulation, we give an iterative procedure for the construction of the antisymmetric basis for arbitrary particle number and present the formulae used to embed two- and three-baryon interactions into the many-body space. For the Slater-determinant formulation, we report on the conversion of the YN interaction matrix elements from relative to single-particle coordinates, the importance-truncation scheme that tailors the model space to the description of the low-lying spectrum, and the role of the redundant center-of-mass degrees of freedom. We end with a confirmation of both formulations in the four-body system, giving converged ground-state energies for a chiral Hamiltonian, and present a short survey of the A ≤ 7 hyper-helium isotopes.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2019

Novel Zoned Waste-forms for High-Priority Radionuclide Waste Streams

This report describes the potential of a novel class of materials—α-ZrW 2 O 8 , Zr 2 WP 2 O 12 , and related compounds that contract upon amorphization as possible radionuclide waste-forms. The proposed ceramic waste-forms would consist of zoned grains, or sintered ceramics with center- loaded radionuclides and barren shells. Radiation-induced amorphization would result in core shrinkage but would not fracture the shells or overgrowths, maintaining isolation of the radionuclide. In this report, we have described synthesis techniques to produce phase-pure forms of the materials, and how to fully densify those materials. Structural models for the materials were developed and validated using DFPT approaches, and radionuclide substitution was evaluated; U(IV), Pu(IV), Tc(IV) and Tc(VII) all readily substitute into the material structures. MD modeling indicated that strain associated with radiation-induced amorphization would not affect the integrity of surrounding crystalline materials, and these results were validated via ion beam experimental studies. Finally, we have evaluated the leach rates of the barren materials, as determined by batch and flow-through reactor experiments. ZrW 2 O 8 leaches rapidly, releasing tungstate while Zr is retained as a solid oxide or hydroxide. Tungsten release rates remain elevated over time and are highly sensitive to contact times, suggesting that this material will not be an effective waste-form. Conversely, tungsten releases rates from Zr 2 WP 2 O 12 rapidly drop, show little dependence on short-term changes in fluid contact time, and in over time, become tied to P release rates. The results presented here suggest that this material may be a viable waste-form for some hard-to-handle radionuclides such as Pu and Tc.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
DOE OSTI2016

Remarks on the fission barriers of super-heavy nuclei

Shell-correction energies of super-heavy nuclei are approximated by using QαQα values of measured decay chains. Five decay chains were analyzed, which start at the isotopes 285 Fl, 294 118, 291 Lv, 292 Lv and 293 Lv. The data are compared with predictions of macroscopic-microscopic models. Fission barriers are estimated that can be used to eliminate uncertainties in partial fission half-lives and in calculations of evaporation-residue cross-sections. In that calculations, fission probability of the compound nucleus is a major factor contributing to the total cross-section. The data also provide constraints on the cross-sections of capture and quasi-fission in the entrance channel of the fusion reaction. Here, arguments are presented that fusion reactions for synthesis of isotopes of elements 118 and 120 may have higher cross-sections than assumed so far.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗
DOE OSTI2016

Symmetry tuning of a near one-dimensional 2-shock platform for code validation at the National Ignition Facility

Here, we introduce a new quasi 1-D implosion experimental platform at the National Ignition Facility designed to validate physics models as well as to study various Inertial Confinement Fusion aspects such as implosion symmetry, convergence, hydrodynamic instabilities, and shock timing. The platform has been developed to maintain shell sphericity throughout the compression phase and produce a round hot core at stagnation. This platform utilizes a 2-shock 1 MJ pulse with 340 TW peak power in a near-vacuum AuHohlraum and a CH ablator capsule uniformly doped with 1% Si. We also performed several inflight radiography, symmetry capsule, and shock timing experiments in order to tune the symmetry of the capsule to near round throughout several epochs of the implosion. Finally, adjusting the relative powers of the inner and outer cones of beams has allowed us to control the drive at the poles and equator of the capsule, thus providing the mechanism to achieve a spherical capsule convergence. Details and results of the tuning experiments are described.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗