Search NASA⌕ Search

SEARCH · Search NASA

Results for “Atmospheric composition”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.

At least 811 records · Page 45

Retrievals of Aerosol Optical and Microphysical Properties from Imaging Polar Nephelometer Scattering Measurements

A method for the retrieval of aerosol optical and microphysical properties from in situ light-scattering measurements is presented and the results are compared with existing measurement techniques. The Generalized Retrieval of Aerosol and Surface Properties (GRASP) is applied to airborne and laboratory measurements made by a novel polar nephelometer. This instrument, the Polarized Imaging Nephelometer (PI-Neph), is capable of making high-accuracy field measurements of phase function and degree of linear polarization, at three visible wavelengths, over a wide angular range of 3 to 177°. The resulting retrieval produces particle size distributions (PSDs) that agree, within experimental error, with measurements made by commercial optical particle counters (OPCs). Additionally, the retrieved real part of the refractive index is generally found to be within the predicted error of 0.02 from the expected values for three species of humidified salt particles, with a refractive index that is well established. The airborne measurements used in this work were made aboard the NASA DC-8 aircraft during the Studies of Emissions and Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys (SEAC4RS) field campaign, and the inversion of this data represents the first aerosol retrievals of airborne polar nephelometer data. The results provide confidence in the real refractive index product, as well as in the retrieval's ability to accurately determine PSD, without assumptions about refractive index that are required by the majority of OPCs.

Espinosa, W. Reed↗

Supporting NASA Science with High-Altitude Long-Endurance Aircraft

NASA Earth Science and Aeronautics researchers have been involved in development and use of High Altitude Long Endurance (HALE) unmanned aircraft systems (UAS) since the 1990's. The NASA Environmental Research Aircraft Sensor and Technology Program (ERAST) demonstrated the promise of HALE aircraft for providing observations while also proving the importance of triple-redundant avionics to improve system reliability for large unmanned aircraft. Early efforts to develop an operational HALE capability for earth observations languished for nearly two decades owing to insufficient solar panel efficiency, battery power density, and light-weight, yet strong, materials. During this time NASA researchers focused on using the Global Hawk to demonstrate the utility of providing diurnal measurements over severe storms (ie. HS3) and to track stratospheric water vapor transport (ATTREX). Recent significant commercial investments are now leading to the realization of a long-held goal of week- to month-long sustained observations and measurements from the stratosphere. In addition to a historical review of NASA use and interest in HALE aircraft, this paper will present current concepts for exploiting current and planned HALE aircraft capabilities including in situ characterization of atmospheric composition and dynamics as well as imagery collection. NASA researchers anticipate HALE will provide a useful means to test smallsat instruments and components. Observations from HALE-based instruments might also provide useful gap-filler observations to flagship satellite missions where the repeat time doesn't allow for measurements of quickly changing phenomenon. HALE will likely also provide measurements and communications relay to facilitate other aircraft in multi-aircraft campaigns. We will also report on progress towards a NASA-funded flight test planned for summer 2019 of a solar-electric vehicle designed to carry 7kg (15lbs) for 30 days at 20km altitude.

earth observations↗

Abundance Measurements of Titan's Stratospheric HCN, HC3N, C3H4, and CH3CN from ALMA Observations

Previous investigations have employed more than 100 close observations of Titan by the Cassini orbiter to elucidate connections between the production and distribution of Titan's vast, organic-rich chemical inventory and its atmospheric dynamics. However, as Titan transitions into northern summer, the lack of incoming data from the Cassini orbiter presents a potential barrier to the continued study of seasonal changes in Titan's atmosphere. In our previous work, we demonstrated that the Atacama Large Millimeter/submillimeter Array (ALMA) is well suited for measurements of Titan's atmosphere in the stratosphere and lower mesosphere (~100 - 500 km) through the use of spatially resolved (beam sizes <1") flux calibration observations of Titan. Here, we derive vertical abundance profiles of four of Titan's trace atmospheric species from the same 3 independent spatial regions across Titan's disk during the same epoch (2012-2015): HCN, HC3N, C3H4, and CH3CN. We find that Titan's minor constituents exhibit large latitudinal variations, with enhanced abundances at high latitudes compared to equatorial measurements; this includes CH3CN, which eluded previous detection by Cassini in the stratosphere, and thus spatially resolved abundance measurements were unattainable. Even over the short 3-year period, vertical profiles and integrated emission maps of these molecules allow us to observe temporal changes in Titan's atmospheric circulation during northern spring. Our derived abundance profiles are comparable to contemporary measurements from Cassini infrared observations, and we find additional evidence for subsidence of enriched air onto Titan's south pole during this time period. Continued observations of Titan with ALMA beyond the summer solstice will enable further study of how Titan's atmospheric composition and dynamics respond to seasonal changes.

Thelen, Alexander E.↗

Chapter 6: Sulfur on Mars from the Atmosphere to the Core

Observations of the martian surface from orbiting spacecraft and in situ landers and rovers, as well as analyses of martian meteorites in terrestrial laboratories, have consistently indicated that Mars is a sulfur-rich planet. The global inventory of sulfur, from the atmosphere to the core, carries widespread implications of potential geophysical, geochemical, climatological, and astrobiological significance. For example, the sulfur content of the core carries implications for core density; the speciation of igneous sulfur minerals reflects the oxidation state of the magma from which they formed; sulfur-bearing gases may have exerted control on the temperatures at the surface of early Mars; and the widespread availability of sulfur on Mars would have provided an abundant source for energy and nutrients to fuel sulfur-metabolizing microbes, such as those that arose during the emergence of primitive life on Earth. Here we provide an overview of martian sulfur and its relevance to these areas of interest, including a discussion of analytical techniques and results acquired by space missions and meteorite analyses to date. We review current studies modeling the potential effects of sulfur-bearing gases on the past martian climate and possible constraints on atmospheric composition implied by sulfur isotopic data. We also explore the importance of sulfur to the search for extinct or extant life on Mars. Finally, we summarize a few areas of interest to future work, including advances in space exploration technology and preparation for Mars sample return.

Climate↗

File Specification for GEOS-CF Products

The NASA Global Earth Observing System (GEOS) model has been expanded to provide global near-real-time forecasts of atmospheric composition at a horizontal resolution of 0.25 degrees (about 25 km). This GEOS Composition Forecast (GEOS-CF) system combines the GEOS weather analysis and forecasting system with the state-of-the-science GEOS-Chem chemistry module (Bey et al., 2001; Keller et al., 2014; Long et al., 2015) to provide detailed chemical analysis of a wide range of air pollutants including ozone, carbon monoxide, nitrogen oxides, and fine particulate matter (PM2.5).

Knowland, Katherine E.↗

Demonstrating Next Generation High-Altitude, Long Endurance Aircraft for Earth Science

This paper will address NASA activities to monitor and study Earth processes from long-duration unmanned aircraft systems (UAS). NASA is currently supporting both large and small UAS development and demonstration. In a follow-on to previous work, NASA Armstrong Flight Research Center is hosting test flights of a large AeroVironment solar-powered aircraft, while NASA Ames Research Center is supporting the demonstration of a light-weight solar powered aircraft by Swift Engineering. Both are designed for long duration, multi-day flight. NASA Earth Science and Aeronautics researchers have been involved in the development and use of High Altitude Long Endurance (HALE) UAS since the 1990's. The NASA Environmental Research Aircraft Sensor and Technology Program (ERAST) demonstrated the promise of HALE aircraft for providing observations while also proving the importance of triple-redundant avionics to improve system reliability for large unmanned aircraft. Early efforts to develop an operational HALE capability for earth observations languished for nearly two decades owing to insufficient solar panel efficiency, battery power density, and light-weight, yet strong, materials. During this time NASA researchers focused on using the Global Hawk to demonstrate the utility of providing diurnal measurements over severe storms (i.e. HS3) and to track stratospheric water vapor transport (ATTREX). Recent significant commercial investments are now leading to the realization of a long-held goal of week- to month-long sustained observations and measurements from the stratosphere. In addition to a historical review of NASA use and interest in HALE aircraft, this paper will present current concepts for exploiting current and planned HALE aircraft capabilities including in situ characterization of atmospheric composition and dynamics as well as imagery collection and internet connectivity. NASA researchers anticipate HALE will also provide a useful means to test smallsat instruments and components. Observations from HALE-based instruments might also provide useful gap-filler observations to flagship satellite missions where the repeat time doesn't allow for measurements of quickly changing phenomenon. HALE will likely also provide measurements and communications relay to facilitate other aircraft in multi-aircraft campaigns. We will also report on progress towards a NASA-supported flight tests solar electric vehicles planned for 2019. One is the Swift Engineering UAS designed to carry 7kg (15lbs) for 30 days at 20km altitude. The other is the AeroVironment Hawk 30, also designed for multi-day flight.

high-altitude↗

NASA Global Satellite and Model Data Products and Services for Tropical Cyclone Research

The lack of observations over vast tropical oceans is a major challenge for tropical cyclone research. Satellite observations and model reanalysis data play an important role in filling these- gaps. Established in the mid-1980's, the Goddard Earth Sciences Data and Information Services Center (GES DISC), as one of the 12 NASA data centers, archives and distributes data from several Earth science disciplines such as precipitation, atmospheric dynamics, atmospheric composition, hydrology, including well-known NASA satellite missions (e.g. TRMM, GPM) and model assimilation projects (MERRA-2). Acquiring datasets suitable for tropical cyclone research in a large data archive is a challenge for many, especially for those who are not familiar with satellite or model data. Over the years, the GES DISC has developed user-friendly data services. For example, Giovanni is an online visualization and analysis tool, allowing users to visualize and analyze over 2000 satellite- and model-based variables with a Web browser, without downloading data and software. In this chapter, we will describe data and services at the GES DISC with emphasis on tropical cyclone research. We will also present two case studies and discuss future plans.

Liu, Zhong↗

TPSAS-NF1676L-18612-DND

Can a space-based elastic backscatter lidar and coincident infrared radiometer recognize the varied microphysical properties observed by aircraft-based cloud probes in cirrus clouds? If so, then the global and continuous coverage provided by the satellite instruments can extend the knowledge about cirrus cloud properties gained from intensive aircraft field campaigns. The recent Studies of Emissions and Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys (SEAC4RS) aircraft field mission that occurred during August and September, 2013 is an ideal data set to use to test whether this is possible. During SEAC4RS there was extensive sampling of cirrus clouds occurring in widely varied conditions, including the North American Monsoon, forest fires, midlatitude frontal convection and tropical convection. Aircraft cloud probe sampling (2D-S, FCDP or FSSP, CPI) was performed from three airplanes, often coordinated with remote sensing by an aircraft-based elastic backscatter lidar (CPL). During the mission the CALIPSO satellite also observed these clouds from space with a similar elastic backscatter lidar (CALIOP) and an infrared radiometer (IIR). There are several cases where the airplanes sampled directly along the satellite track, but also many overpasses of the region and these features that were not coincident with the aircraft-based sampling. This presentation seeks to address the question of whether relationships between the cloud particle size distribution measurements and habits observed by the SPEC cloud probes and CPL aircraft lidar parameters can be up-scaled to classify the CALIPSO satellite observations from this region and time period. The lidar can also provide cloud top information and evidence of whether there was irreversible transport of ice and aerosols into the UT/LS.

Melody Avery↗

TPSAS-NF1676L-23428-DND

Recent theoretical advances now enable accurate characterization of both the single scattering and multiple scattering contributions to the lidar backscatter signals obtained from opaque water clouds (Hu et al., 2006). As a consequence, lidar measurements of opaque water clouds have increasingly broad applications, especially for space-based polarization-sensitive lidars such as CALIOP. Among the most prominent and useful of these are (1) calibration and assessments of calibration accuracy (e.g., O'Connor et al., 2004; Hu et al., 2006); (2) accurate estimates of extrinsic (e.g., optical depths) and intrinsic (e.g., extinction-to-backscatter ratios) optical properties of clouds and aerosol layers lying above opaque water clouds (Hu et al., 2007; Liu et al., 2015); and (3) retrievals of water cloud microphysical properties such as cloud droplet number concentrations (Hu et al., 2007; Li et al., 2011; Zeng et al., 2014). In the first part of this presentation we give an overview of the recent advances in this subject area. The second part introduces several new studies of water clouds using the multi-wavelength depolarization measurement capabilities of NASA's airborne high spectral resolution lidars (HSRL). We use these measurements to assess existing theory, validate the measurement concept and explore several new application concepts. The third part discusses changes in Arctic water clouds using CALIOP measurements. The HSRL water cloud study is supported by NASA's atmospheric composition program.

Y Hu↗

Description and Evaluation of the Specified-Dynamics Experiment in the Chemistry-Climate Model Initiative

We provide an overview of the REF-C1SD specified-dynamics experiment that was conducted as part of phase 1 of the Chemistry-Climate Model Initiative (CCMI). The REF-C1SD experiment, which consisted of mainly nudged general circulation models (GCMs) constrained with (re)analysis fields, was designed to examine the influence of the large-scale circulation on past trends in atmospheric composition. The REF-C1SD simulations were produced across various model frameworks and are evaluated in terms of how well they represent different measures of the dynamical and transport circulations. In the troposphere there are large (~40 %) differences in the climatological mean distributions, seasonal cycle amplitude, and trends of the meridional and vertical winds. In the stratosphere there are similarly large (~50 %) differences in the magnitude, trends and seasonal cycle amplitude of the transformed Eulerian mean circulation and among various chemical and idealized tracers. At the same time, interannual variations in nearly all quantities are very well represented, compared to the underlying reanalyses. We show that the differences in magnitude, trends and seasonal cycle are not related to the use of different reanalysis products; rather, we show they are associated with how the simulations were implemented, by which we refer both to how the large-scale flow was prescribed and to biases in the underlying free-running models. In most cases these differences are shown to be as large or even larger than the differences exhibited by free-running simulations produced using the exact same models, which are also shown to be more dynamically consistent. Overall, our results suggest that care must be taken when using specified-dynamics simulations to examine the influence of large-scale dynamics on composition.

Clara Orbe↗

TRAPPIST-1 Habitable Atmosphere Intercomparison (THAI): motivations and protocol version 1.0

Upcoming telescopes such as the James Webb Space Telescope (JWST), the European Extremely Large Telescope (E-ELT), the Thirty Meter Telescope (TMT) or the Giant Magellan Telescope (GMT) may soon be able to characterize, through transmission, emission or reflection spectroscopy, the atmospheres of rocky exoplanets orbiting nearby M dwarfs. One of the most promising candidates is the late M-dwarf system TRAPPIST-1, which has seven known transiting planets for which transit timing variation (TTV) measurements suggest that they are terrestrial in nature, with a possible enrichment in volatiles. Among these seven planets, TRAPPIST-1e seems to be the most promising candidate to have habitable surface conditions, receiving ∼66 % of the Earth's incident radiation and thus needing only modest greenhouse gas inventories to raise surface temperatures to allow surface liquid water to exist. TRAPPIST-1e is, therefore, one of the prime targets for the JWST atmospheric characterization. In this context, the modeling of its potential atmosphere is an essential step prior to observation. Global climate models (GCMs) offer the most detailed way to simulate planetary atmospheres. However, intrinsic differences exist between GCMs which can lead to different climate prediction and thus observability of gas and/or cloud features in transmission and thermal emission spectra. Such differences should preferably be known prior to observations. In this paper we present a protocol to intercompare planetary GCMs. Four testing cases are considered for TRAPPIST-1e, but the methodology is applicable to other rocky exoplanets in the habitable zone. The four test cases included two land planets composed of modern-Earth and pure-CO2 atmospheres and two aqua planets with the same atmospheric compositions. Currently, there are four participating models (LMDG, ROCKE-3D, ExoCAM, UM); however, this protocol is intended to let other teams participate as well.

Thomas Jean Daniel Fauchez↗

Historical (1850‐2014) Aerosol Evolution and Role on Climate Forcing Using the GISS Modele2.1 Contribution to CMIP6

The Earth’s climate is rapidly changing. Over the past centuries, aerosols, via their ability to absorb or scatter solar radiation and alter clouds, played an important role in counterbalancing some of the greenhouse gas (GHG) caused global warming. The multi-century anthropogenic aerosol cooling effect prevented present-day climate from reaching even higher surface air temperatures and subsequent more dramatic climate impacts. Trends in aerosol concentrations and optical depth show that in many polluted regions such as Europe and the United States of America, aerosol precursor emissions decreased back to levels of the 1950s. More recent polluting countries such as China may have reached a turning point in recent years as well, while India still follows an upward trend. Here we study aerosol trends in the CMIP6 simulations of the GISS ModelE2.1 climate model using a fully coupled atmosphere composition onfiguration, including interactive gas-phase chemistry, and either an aerosol microphysical (MATRIX) or a mass-based (OMA) aerosol module. Results show that whether global aerosol radiative forcing is already declining depends on the aerosol scheme used. Using the aerosol microphysical scheme, where the aerosol system reacts more strongly to the trend in sulfur dioxide (SO2) emissions, global peak direct aerosol forcing was reached in the 1980’s, whereas the mass-based scheme simulates peak direct aerosol forcing around 2010.

Aerosol forcing↗

Studying the 2019 Australian Bushfires Disaster using NASA Data: A Data-Driven Storytelling Approach

The 2019-2020 Australian fire season was particularly devastating, with millions of acres of land burned and impacts affecting Australian ecology, local populations and air quality, and the atmosphere. Australia saw unprecedented heat waves, with temperatures reaching 120 F (49.1 C) in January across central and eastern Australia. The fires gave rise to a host of atmospheric phenomenon, including smoke transport and lofting generated by storm-induced by fires, known as pyrocumulonimbus, reaching the stratosphere. NASA’s satellites not only tracked the event in real time, but also gathered data to further inform forecasting and response methods in the future. To better assist the public in understanding the lead up, impacts, and aftermath effects of these fires, the Science Outreach Team at NASA Langley Research Center’s Atmospheric Science Data Center (ASDC) Distributed Active Archive Center (DAAC) used Esri’s storymap tool to guide users through understanding relevant phenomenon, contributing factors, the effects this event has had on global atmospheric composition, and the science behind researching the tie between disasters and public health. The storymap uses data from the ASDC-supported NASA missions Measurements Of Pollution In The Troposphere (MOPITT), Cloud-Aerosol and Infrared Pathfinder Satellite Observation (CALIPSO), Clouds and the Earth’s Radiant Energy System (CERES), the Stratospheric Aerosol and Gas Experiment (SAGE III), and Multi-angle Imaging SpectroRadiometer (MISR). By using data-driven storytelling to communicate impacts of a large fire event, we hope to provide an accessible, engaging science outreach tool format.

Sanjana Paul↗

Challenges of Operations in a Dynamic Environment: A Three-Year Perspective of SAGE III

The Stratospheric Aerosol and Gas Experiment~III on the International Space Station (SAGE III/ISS) was delivered to the International Space Station (ISS) on 23 February 2017. The SAGE III/ISS payload was robotically installed external to the ISS and began acquiring science measurements on 17 March 2017. The SAGE III/ISS instrument retrieves vertical profiles of atmospheric ozone, multi-wavelength aerosol extinctions, and other gaseous species. This paper will focus on the improvements made to the operations of the SAGE III/ISS payload. A key focus of the operations team following commissioning was to create robust tools that aide in the operations of the payload. A close collaboration with the SAGE III/ISS ground systems team allowed for the development of web-based tools to continuously monitor the health of the instrument. The mission operations team also worked with the SAGE III/ISS science team to gain a better sense of how the instrument works to maximize the quality and quantity of the science data collected. Another unique aspect of the SAGE III/ISS payload, that will be discussed, is the challenges of operating a hosted payload on the ISS; an active platform that has frequent attitude maneuvers, dockings, and EVA's. This active environment increases the need for the SAGE III/ISS operations team command the payload. Through coordination and teamwork, SAGE III/ISS mission has developed an operations team that has successfully managed the instrument around ISS activities and recovered from multiple instrument upsets. This has led the SAGE III/ISS payload to successfully surpass the acquisition metrics set forth prior to launch, allowing for the continued contribution to studying the atmospheric composition of the stratosphere and how it plays a role in earth’s climate.

SAGE III↗

Studying the 2019-2020 Australian Bushfires Using NASA Data

The 2019-2020 season has been one of the worst fire seasons on record. Australia has seen unprecedented heat waves, with temperatures reaching 120 F (49.1 C) in January across central and eastern Australia. NASA's satellites not only tracked the event in real time, using resources such as the Global Actives Fires and Hotspots Dashboard you see below, but also collected large volumes of rich data that scientists and researchers can use to study the event and the regional and global effects of the disaster. In this Esri StoryMap, we will guide you through the factors leading up to the 2019-2020 Australian bushfires disaster, the effect this event has had on air quality and global atmospheric composition, and the science behind researching the tie between disasters and public health. This story map will use data from ASDC-supported NASA missions such as the Measurements Of Pollution In The Troposphere (MOPITT), Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO), Clouds and the Earth’s Radiant Energy System (CERES), Stratospheric Aerosol and Gas Experiment (SAGE III) on the International Space Station (ISS), and Multi-angle Imaging SpectroRadiometer (MISR).

Sanjana Paul↗

Earth system modeling: can we stay ahead of what's actually happening?

Over the last forty years, Earth System Models have become more and more comprehensive and detailed. They have assimilated previously independent modeling efforts in ocean circulation, atmospheric composition, the stratosphere, land surface, and the cryosphere, and are today demonstrably more skillful than earlier efforts. Yet the structural uncertainty in the latest model projections is actually increasing. Meanwhile, impacts of climate change on, for instance, wildfires, tropical cyclones and sea level, appear to be increasing faster than we have been able to predict. I will address some of the current issues at the bleeding edges of model development and the continuing importance of model evaluation.

Gavin A Schmidt↗

Operations Challenges in a Dynamic Environment: A Three-Year Perspective of SAGE III

The Stratospheric Aerosol and Gas Experiment III on the International Space Station (SAGE III/ISS) was delivered to the International Space Station (ISS) on 23 February 2017. The SAGE III/ISS payload was robotically installed external to the ISS and began acquiring science measurements on 17 March 2017. The SAGE III/ISS instrument retrieves vertical profiles of atmospheric ozone, multi-wavelength aerosol extinctions, and other gaseous species. This paper will focus on the improvements made to the operations of the SAGE III/ISS payload. A key focus of the operations team following commissioning was to create robust tools that aid in the operations of the payload. A close collaboration with the SAGE III/ISS ground systems team allowed for the development of web-based tools to continuously monitor the health of the payload. The mission operations team also worked with the SAGE III/ISS science team to gain a better sense of how the instrument works to maximize the quality and quantity of the science data collected. Another unique aspect of the SAGE III/ISS payload, that will be discussed, is the challenges of operating a hosted payload on the ISS; an active platform that has frequent attitude maneuvers, dockings, and EVAs. This active environment increases the need for the SAGE III/ISS operations team command to the payload. Through coordination and teamwork, SAGE III/ISS mission has developed an operations team, tool, and procedures that have successfully managed the payload around ISS activities and recovered from multiple instrument upsets. This has led the SAGE III/ISS payload to successfully surpass the acquisition metrics set forth prior to launch, allowing for the continued contribution to studying the atmospheric composition of the stratosphere and how it plays a role in Earth’s climate.

SAGE III↗

The Climate Response to Emissions Reductions due to COVID-19: Initial Results from CovidMIP

Many nations responded to the COVID-19 pandemic by restricting travel and other activities during 2020, resulting in temporarily reduced emissions of CO2, other greenhouse gases and ozone and aerosol precursors. We present the initial results from a coordinated Intercomparison, CovidMIP, of Earth system model simulations which assess the impact on climate of these emissions reductions. Twelve models performed multiple initial-condition ensembles to produce over 300 simulations spanning both initial condition and model structural uncertainty. We find model consensus on reduced aerosol amounts (particularly over southern and eastern Asia) and associated increases in surface shortwave radiation levels. However, any impact on near-surface temperature or rainfall during 2020-2024 is extremely small and is not detectable in this initial analysis. Regional analyses on a finer scale, and closer attention to extremes (especially linked to changes in atmospheric composition and air quality) are required to test the impact of COVID- 19-related emission reductions on near-term climate.

Chris D. Jones↗