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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 811 records · Page 45
All sourcesNASA NTRSDOE OSTI
DOE OSTI2017

Final Scientific/Technical Report of Gas Hydrate Dynamics on the Alaskan Beaufort Continental Slope: Modeling and Field Characterization

Methane Hydrates, a solid form of methane and water, exist at high pressures and low temperatures, occurs on every continental margin on Earth, represents one of the largest reservoirs of carbon on the planet, and, if destabilized, may play an important role in both slope stability and climate change. For decades, researchers have studied methane hydrates with the hope of determining if methane hydrates are destabilizing, and if so, how this destabilization might impact slope stability and ocean/atmosphere carbon budgets. In the past ~5 years, it has become well established that the upper “feather-edge” of methane hydrate stability (intermediate water depths of ~200-500 meters below sea level) represents an important frontier for methane hydrates stability research, as this zone is most susceptible to destabilization due to minor fluctuations in ocean temperature in space and time. The Arctic Ocean—one of the fastest warming regions on Earth—is perhaps the best place to study possible changes to methane hydrate stability due to ocean warming. To address the stability of methane hydrates at intermediate ocean depths, Southern Methodist University in partnership with Oregon State University and The United State Geological Survey at Woods Hole began investigating methane hydrate stability in intermediate water depths below both the US Beaufort Sea and the Atlantic Margin, from 2012-2017. The work was funded by the Department of Energy’s (DOE) National Energy Technology Laboratory (NETL). The key goal of the SMU component of this study was to collect the first ever heat flow data in the Beaufort Sea and compare measured shallow (probe-based1) heat flow values with deeper (BSR-derived2) heat flow values, and from this, determine whether hydrates were in thermal equilibrium. In September 2016, SMU/OSU collected the first ever heat flow measurements in the US Beaufort Sea. Despite poor weather and rough seas, the cruise was a success, with 116 heat flow measurements acquired across the margin, spanning 4 transects separated by more than 400 km. Useable heat flow data exists for 97% (113) of probe heat flow measurements, revealing a clear picture of regional heat flow across the basin. During the past 8 months since the cruise, SMU researchers have processed the heat flow and thermal conductivity measurements and compared results to deeper heat flow estimates obtained from seismic data. The analysis reveals clear, consistent trends: All probe heat flow measurements in depths greater than 800 mbsl are consistent with BSR-derived values; heat flow measurements obtained in water depths between ~250-750 mbsl are systematically lower than those estimated from BSRs; and heat flow estimates in water depths shallower than ~250 mbsl are systematically warmer than deeper estimates. The consistency between shallow (probe) and deep (BSR) heat flow measurements at depths greater than ~750 m where ocean temperature changes are minimal supports the premise that the hydrates consist primarily of methane and represent a valuable tool for estimating heat flow. The anomalous cooling trend observed in the upper 250 m is consistent with expected seasonal effects observed in shallow ocean buoy measurements in the arctic, when cold, less dense melting sea ice cools the upper 200 m of the ocean during the summer as ice melting occurs. The discrepancy in heat flow at intermediate water depths is best explained via recent intermediate ocean temperature warming, where long-term (annual or longer) warming intermediate ocean bottom waters result in an anomalously low heat flow in shallow heat flow measurements. Using the characteristic 1D time-length scale for diffusion, we estimate that ocean temperature warming began no later than ~1200 years ago but arguably much more recently as results are limited by seismic resolution. More importantly, our analysis indicates methane hydrate is destabilizing not only in the upper feather edge (200-500 mbsl) but at depths as great as 750 mbsl. The intermediate ocean warming rate supports previous studies suggesting geologically rapid warming (>0.1 deg C/decade) at intermediate ocean depths in the Beaufort Sea. Assuming no further changes or additional warming, our analysis indicates methane hydrates will destabilize at seafloor depths shallower than 750 mbsl in the Beaufort Sea within the next ~3000 years. 1 Probe outfitted with sensors inserted into the seafloor sediment 2 Bottom-simulating reflector (BSR) seismic data indicates presence of hydrate deposits

58 GEOSCIENCES↗
DOE OSTI2016

A NUMERICAL MODEL OF PARSEC-SCALE SSC MORPHOLOGIES AND THEIR RADIO EMISSION

In current models for jets of active galactic nuclei and their emission a shortcoming in the description and understanding of the connection between the largest and smallest scales exists. In this work we present a spatially resolved synchrotron self-Compton model extended to parsec scales, which opens the possibility of probing the connections between the radio and high-energy properties. We simulate an environment that leads to Fermi-I acceleration of leptonic particles and includes the full time dependence of this process. Omitting the restriction of a finite downstream region, we find that the spectral energy distribution produced by the accelerated particles strongly depends on their radial confinement behind the shock. The requirement, for both the restriction of high-energy emission to a small region around the shock and the production of a flat radio spectrum, is an initial linear increase of the radius immediately behind the shock, which then slows down with increasing distance from the shock. A good representation of the data for the blazar Mrk 501 is achieved by a parameterized log function. The prediction for the shape of the radio blob is given by the flux distribution with respect to shock distance.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2017

The Re-Acceleration of Galactic Electrons at the Heliospheric Termination Shock

Observations by the Voyager spacecraft in the outer heliosphere presented several challenges for the paradigm of diffusive shock acceleration (DSA) at the solar wind termination shock (TS). In this study, the viability of DSA as a re-acceleration mechanism for galactic electrons is investigated using a comprehensive cosmic-ray modulation model. The results demonstrate that the efficiency of DSA depends strongly on the shape of the electron spectra incident at the TS, which in turn depends on the features of the local interstellar spectrum. Modulation processes such as drifts therefore also influence the re-acceleration process. It is found that re-accelerated electrons make appreciable contributions to intensities in the heliosphere and that increases caused by DSA at the TS are comparable to intensity enhancements observed by Voyager 1 ahead of the TS crossing. The modeling results are interpreted as support for DSA as a re-acceleration mechanism for galactic electrons at the TS.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2018

A Fundamental Test for Galaxy Formation Models: Matching the Lyman- α Absorption Profiles of Galactic Halos Over Three Decades in Distance

Galaxy formation depends critically on the physical state of gas in the circumgalactic medium (CGM) and its interface with the intergalactic medium (IGM), determined by the complex interplay between inflow from the IGM and outflows from supernovae and/or AGN feedback. The average Lyα absorption profile around galactic halos represents a powerful tool to probe their gaseous environments. We compare predictions from Illustris and Nyx hydrodynamical simulations with the observed absorption around foreground quasars, damped Lyα systems, and Lyman-break galaxies. We show how large-scale BOSS and small-scale quasar pair measurements can be combined to precisely constrain the absorption profile over three decades in transverse distance 20 kpc ≲ b ≲ 20 Mpc. Far from galaxies, ≲ 2 Mpc, the simulations converge to the same profile and provide a reasonable match to the observations. This asymptotic agreement arises because the ΛCDM model successfully describes the ambient IGM and represents a critical advantage of studying the mean absorption profile. However, significant differences between the simulations, and between simulations and observations, are present on scales 20 kpc ≲ b ≲ 20 Mpc, illustrating the challenges of accurately modeling and resolving galaxy formation physics. It is noteworthy that these differences are observed as far out as ~2 Mpc, indicating that the "sphere of influence" of galaxies could extend to approximately ~7 times the halo virial radius. Current observations are very precise on these scales and can thus strongly discriminate between different galaxy formation models. We demonstrate that the Lyα absorption profile is primarily sensitive to the underlying temperature-density relationship of diffuse gas around galaxies, and argue that it thus provides a fundamental test of galaxy formation models.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS1975

Test evaluation of potential heat shield contamination of an Outer Planet Probe's atmospheric sampling system

An Outer Planets Probe which retains the charred heatshield during atmospheric descent must deploy a sampling tube through the heatshield to extract atmospheric samples for analysis. Once the sampling tube is deployed, the atmospheric samples ingested must be free of contaminant gases generated by the heatshield. Outgassing products such as methane and water vapor are present in planetary atmospheres and hence, ingestion of such species would result in gas analyzer measurement uncertainties. This paper evaluates the potential for, and design impact of, the extracted atmospheric samples being contaminated by heatshield outgassing products. Flight trajectory data for Jupiter, Saturn and Uranus entries are analyzed to define the conditions resulting in the greatest potential for outgassing products being ingested into the probe's sampling system. An experimental program is defined and described which simulates the key flow field features for a planetary flight in a ground-based test facility. The primary parameters varied in the test include: sampling tube length, injectant mass flow rate and angle of attack. Measured contaminant levels predict the critical sampling tube length for contamination avoidance. Thus, the study demonstrates the compatibility of a retained heatshield concept and high quality atmospheric trace species measurements.

Kessler, W. C.↗
NASA NTRS1983

Global empirical model of the Venus thermosphere

Direct measurements of neutral CO2, O, CO, N2, He, and N densities from the Pioneer Venus Orbiter Neutral Mass Spectrometer are described in terms of a spherical harmonic representation (latitude and local time coordinates) of exospheric temperature and number densities at 150 km, using modified Bates temperature profiles. The exospheric temperatures are determined from the altitude variations of atomic oxygen. A global average temperature of 228 K is derived with a first harmonic variation of 5%. The altitude profiles are extended downward to 100 km by using empirical formulas to provide a transition through the turbopause region (simulating the effect of eddy diffusion and vertical flows) and matching entry probe density data. The model reflects the observed variations of temperature and density with the 10.7 cm radio flux index. For a given change in flux at the planet, the exospheric temperature on Venus changes by only 10% of the change seen in the terrestrial thermosphere.

Hedin, A. E.↗
NASA NTRS1998

Nanoscale Etching and Indentation of Silicon Surfaces with Carbon Nanotubes

The possibility of nanolithography of silicon and germanium surfaces with bare carbon nanotube tips of scanning probe microscopy devices is considered with large scale classical molecular dynamics (MD) simulations employing Tersoff's reactive many-body potential for heteroatomic C/Si/Ge system. Lithography plays a key role in semiconductor manufacturing, and it is expected that future molecular and quantum electronic devices will be fabricated with nanolithographic and nanodeposition techniques. Carbon nanotubes, rolled up sheets of graphene made of carbon, are excellent candidates for use in nanolithography because they are extremely strong along axial direction and yet extremely elastic along radial direction. In the simulations, the interaction of a carbon nanotube tip with silicon surfaces is explored in two regimes. In the first scenario, the nanotubes barely touch the surface, while in the second they are pushed into the surface to make "nano holes". The first - gentle scenario mimics the nanotube-surface chemical reaction induced by the vertical mechanical manipulation of the nanotube. The second -digging - scenario intends to study the indentation profiles. The following results are reported in the two cases. In the first regime, depending on the surface impact site, two major outcomes outcomes are the selective removal of either a single surface atom or a surface dimer off the silicon surface. In the second regime, the indentation of a silicon substrate by the nanotube is observed. Upon the nanotube withdrawal, several surface silicon atoms are adsorbed at the tip of the nanotube causing significant rearrangements of atoms comprising the surface layer of the silicon substrate. The results are explained in terms of relative strength of C-C, C-Si, and Si-Si bonds. The proposed method is very robust and does not require applied voltage between the nanotube tips and the surface. The implications of the reported controllable etching and hole-creating for nanolithography on silicon are discussed in detail.

Dzegilenko, Fedor N.↗
NASA NTRS2003

Implicit Spacecraft Gyro Calibration

This paper presents an implicit algorithm for spacecraft onboard instrument calibration, particularly to onboard gyro calibration. This work is an extension of previous work that was done where an explicit gyro calibration algorithm was applied to the AQUA spacecraft gyros. The algorithm presented in this paper was tested using simulated data and real data that were downloaded from the Microwave Anisotropy Probe (MAP) spacecraft. The calibration tests gave very good results. A comparison between the use of the implicit calibration algorithm used here with the explicit algorithm used for AQUA spacecraft indicates that both provide an excellent estimation of the gyro calibration parameters with similar accuracies.

Harman, Richard↗
NASA NTRS2019

Glenn Extreme Environment Rig (GEER)

Visions and Voyages for Planetary Science in the Decade 2013-2022[1] identified the goal of understanding the origin, evolution, and processes that control climate on terrestrial planets,with direct interest in Venus. The Glenn Extreme Environment Rig (GEER), located at NASA Glenn Research Center, was developed to address a community need for a facility which could simulate the extreme environments of the Venus surface. It actively supports science investigations and technical development activities of research institutions and industry partners. It is uniquely suited for studying the interactions between Venus' substantial atmosphere, its surface, and exploration components. Ongoing facility enhancements will provide significant additional value to the research community and maintain GEERs status as a world-class Venus simulation facility.

probe↗
NASA NTRS2023

RF Metrology of Lunar Highlands Regolith Simulant NU-LHT-2M

Understanding the electrical properties of lunar regolith is vital to modeling radiofrequency(RF) propagation on the lunar surface a fundamental step in planning lunar surface missions. Near the lunar south pole, the regolith has yet to be directly sampled and thus there remains uncertainty in the electrical properties of the regolith. The regolith simulant NU-LHT-2M is a highlands simulant that is representative of the expected chemical composition of the regolith near the lunar south pole. Previous studies have investigated properties of NU-LHT at UHF and S-band[1]. Future missions to the lunar south pole are expected to utilize X and Ka-band for direct-to-Earth links and UHF, S-band, C-band, and Ka-band for lunar surface communication[2]. As a result, it is necessary to electrically characterize the lunar regolith at these frequencies. In this paper, coaxial impedance dielectric reflectometry is performed on the NU-LHT-2M simulant using a commercially available soil permittivity measurement device. This study serves as a preliminary measurement of the simulant and may lead to enhanced efficacy of the measurement hardware for future applications.

simulant↗
NASA NTRSDate not supplied

RF Metrology of Lunar Highlands Regolith Simulant NU-LHT-2M

*Presentation for the publication* Understanding the electrical properties of lunar regolith is vital to modeling radiofrequency (RF) propagation on the lunar surface, a fundamental step in planning lunar surface missions. Near the lunar south pole, the regolith has yet to be directly sampled and thus there remains uncertainty in the electrical properties of the regolith. The regolith simulant NU-LHT-2M is a highlands simulant that is representative of the expected chemical composition of the regolith near the lunar south pole. Previous studies have investigated properties of NU-LHT at UHF and S-band[1]. Future missions to the lunar south pole are expected to utilize X and Ka-band for direct-to-Earth links and UHF, S-band, C-band, and Ka-band for lunar surface communication [2]. As a result, it is necessary to electrically characterize the lunar regolith at these frequencies. In this paper, coaxial impedance dielectric reflectometry is performed on the NU-LHT-2M simulant using a commercially available soil permittivity measurement device. This study serves as a preliminary measurement of the simulant and may lead to enhanced efficacy of the measurement hardware for future applications.

simulant↗
DOE OSTI2019

Pump-probe ghost imaging with SASE FELs

In this paper we propose a new approach to measuring ultrafast dynamics with free-electron lasers (FELs). Ultrafast experiments are among the most promising avenues of research at x-ray FELs, with potential to reveal the chemical dynamics of charge separation, conical intersection crossing, and biologically mediated reactions. Pump-probe scanning is the standard approach to measure dynamics at x-ray FELs, but at the shortest time scales, and particularly for x-ray pump, x-ray probe experiments, the scans require challenging beam setups and can introduce systematic errors. Here we propose an alternative approach using the randomness of the self-amplified spontaneous emission (SASE) process to drive many simultaneous pump-probe experiments on each shot. Measuring the fluctuations in the incident beam’s time profile on a shot-to-shot basis enables reconstruction of ultrafast dynamics down to the coherence length of the FEL without the need for pump-probe scans. Due to similarity to ghost imaging, in which spatial properties are reconstructed by measuring the incident probe’s transverse properties, we call this ``pump-probe ghost imaging" (PPGI). In this paper we describe the method and simulate an example experiment. We also describe an alternative implementation that uses only spectral measurements, avoiding the need for direct time-domain diagnostics, and extending the method to the attosecond regime.

Ratner, Daniel Fried↗
DOE OSTI2024

Confinement Effects on Proton Transfer in TiO 2 Nanopores from Machine Learning Potential Molecular Dynamics Simulations

Improved understanding of proton transfer in nanopores is critical for a wide range of emerging applications, yet experimentally probing mechanisms and energetics of this process remains a significant challenge. To help reveal details of this process, we developed and applied a machine learning potential derived from first-principles calculations to examine water reactivity and proton transfer in TiO 2 slit-pores. Here, we find that confinement of water within pores smaller than 0.5 nm imposes strong and complex effects on water reactivity and proton transfer. Although the proton transfer mechanism is similar to that at a TiO 2 interface with bulk water, confinement reduces the activation energy of this process, leading to more frequent proton transfer events. This enhanced proton transfer stems from the contraction of oxygen–oxygen distances dictated by the interplay between confinement and hydrophilic interactions. Our simulations also highlight the importance of the surface topology, where faster proton transport is found in the direction where a unique arrangement of surface oxygens enables the formation of an ordered water chain. In a broader context, our study demonstrates that proton transfer in hydrophilic nanopores can be enhanced by controlling pore size, surface chemistry, and topology.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Water, Ion, and Proton Dynamics and Interactions in Nanoconfined Systems

The research was directed at understanding the role that nanoconfinement has on the dynamics and structure of liquids confined in nanometer size structures. Experiments were conducted using ultrafast infrared methods. The methods were two dimensional infrared (2D IR) spectroscopy and polarization pump-probe (PSPP) experiments. In addition FT-IR spectroscopy was used. To augment the experimental work, high level molecular dynamics simulations of the systems were conducted. The system used for confinement were nanoporous silica with essentially monodispersed pores. Pores of different diameters were studies, i.e., 2.5 nm to 8 nm. Water and organic liquids were investigated. The experiments were performed on a vibrational probe molecule, i.e., the CN stretch of the anion SeCN-. The 2D IR experiments measured spectral diffusion, which directly reported on the structural dynamics of the confined liquids. 2D IR was also used to perform chemical exchange measurements, which observed the formation and dissociation of molecular complexes with surface silanols. The PSPP experiments measured orientational relaxation of the probe molecule as well as it vibrational lifetime. All of the observables depended on the diameter of the pores and the type of liquid. The simulations of the observables provided detailed structural information on the structure of the confined liquids and there interactions with the surfaces. In addition to the study of the confinement in nanopores, water in hydrogels was also studied. The same experimental methods were used along with MD simulations. It was found the influence of hydrogels on water did not come from confinement of the water in the hydrogel polymer network, but rather from the interactions of the water with the individual monomers that compose the polymer. In addition, the temperature dependence of a polymer/water system was tracked from below to above the lower critical solution temperature to observe the nature of the phase separated polymer and how water responded to the phase separation.

36 MATERIALS SCIENCE↗
NASA NTRSDate not supplied

On Characterization of Flow Disturbances in Arc-Jet Testing

This paper reports computational simulations and analysis of flow characterization tests in high enthalpy arc-jet facilities at NASA Ames Research Center. Flow disturbances and their characterization are presented through case studies, and their implications for testing are discussed. The case studies include free-jet test configurations from three different arc heaters and nozzles: the 60-MW IHF 30-inch conical nozzle, the 10-MW TP3 15-inch conical nozzle, and the 20-MW AHF 12-inch conical nozzle. For all cases, test articles are placed in the jet exiting the conical nozzle, and the existence of a flow disturbance is confirmed through flow survey data using pitot pressure and heat flux probes and accompanying analysis. The paper focuses on cases where the effects of the disturbances on test article surface quantities are important. The present analysis comprises computational fluid dynamics simulations of the nonequilibrium flowfield in the facility nozzles and test box, including the models tested. Comparisons of computations with the experimental measurements are presented. The computations that reproduce the probe sweep data approximately are essential to interpret the arc-jet test data accurately, while providing insights into several observed calorimeter anomalies caused by flow disturbances.

Arc-jet testing↗
NASA NTRSDate not supplied

On Characterization of Flow Disturbances in Arc-Jet Testing

This paper reports computational simulations and analysis of flow characterization tests in high enthalpy arc-jet facilities at NASA Ames Research Center. Flow disturbances and their characterization are presented through case studies, and their implications for testing are discussed. The case studies include free-jet test configurations from three different arc heaters and nozzles: the 60-MW IHF 30-inch conical nozzle, the 10-MW TP3 15-inch conical nozzle, and the 20-MW AHF 12-inch conical nozzle. For all cases, test articles are placed in the jet exiting the conical nozzle, and the existence of a flow disturbance is confirmed through flow survey data using pitot pressure and heat flux probes and accompanying analysis. The paper focuses on cases where the effects of the disturbances on test article surface quantities are important. The present analysis comprises computational fluid dynamics simulations of the nonequilibrium flowfield in the facility nozzles and test box, including the models tested. Comparisons of computations with the experimental measurements are presented. The computations that reproduce the probe sweep data approximately are essential to interpret the arc-jet test data accurately, while providing insights into several observed calorimeter anomalies caused by flow disturbances.

Arc-jet testing↗