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At least 811 records · Page 45
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

An overview of the ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) project: aerosol–cloud–radiation interactions in the southeast Atlantic basin

Southern Africa produces almost a third of the Earth's biomass burning (BB) aerosol particles, yet the fate of these particles and their influence on regional and global climate is poorly understood. ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) is a 5-year NASA EVS-2 (Earth Venture Suborbital-2) investigation with three intensive observation periods designed to study key atmospheric processes that determine the climate impacts of these aerosols. During the Southern Hemisphere winter and spring (June-October), aerosol particles reaching 3-5 km in altitude are transported westward over the southeast Atlantic, where they interact with one of the largest subtropical stratocumulus (Sc) cloud decks in the world. The representation of these interactions in climate models remains highly uncertain in part due to a scarcity of observational constraints on aerosol and cloud properties, as well as due to the parameterized treatment of physical processes. Three ORACLES deployments by the NASA P-3 aircraft in September 2016, August 2017, and October 2018 (totaling ~350 science flight hours), augmented by the deployment of the NASA ER-2 aircraft for remote sensing in September 2016 (totaling ~100 science flight hours), were intended to help fill this observational gap. ORACLES focuses on three fundamental science themes centered on the climate effects of African BB aerosols: (a) direct aerosol radiative effects, (b) effects of aerosol absorption on atmospheric circulation and clouds, and (c) aerosol–cloud microphysical interactions. This paper summarizes the ORACLES science objectives, describes the project implementation, provides an overview of the flights and measurements in each deployment, and highlights the integrative modeling efforts from cloud to global scales to address science objectives. Significant new findings on the vertical structure of BB aerosol physical and chemical properties, chemical aging, cloud condensation nuclei, rain and precipitation statistics, and aerosol indirect effects are emphasized, but their detailed descriptions are the subject of separate publications. The main purpose of this paper is to familiarize the broader scientific community with the ORACLES project and the dataset it produced.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1990

Comparison of cloud forcing derived from the Earth Radiation Budget Experiment with that simulated by the NCAR Community Climate Model

The cloud radiative forcing derived from the Earth Radiation Budget Experiment (ERBE) data was compared with cloud forcing simulated by a T42 version of the NCAR Community Climate Model (CCM). The comparison indicates a number of deficiencies in the CCM. Namely, it is shown that the model emits substantially more long-wave radiation than is observed by ERBE. This overestimation is attributed to two model characteristics: (1) the model is too dry and thus reduces the greenhouse longwave radiation effect of the atmosphere (permitting more longwave radiation to escape into space); and (2) the effective high cloud amount is quite small in the model.

Kiehl, J. T.↗
DOE OSTI2018

Understanding Global Model Systematic Shortwave Radiation Errors in Subtropical Marine Boundary Layer Cloud Regimes

Abstract Global numerical weather prediction and climate models are subject to long‐standing systematic shortwave radiation errors due to deficiencies in the representation of boundary layer clouds over the ocean. In the subtropics, clouds are typically too reflective in the cumulus regime and not reflective enough in the stratocumulus regime. Potential sources of error include cloud cover, liquid water path, effective radius, and subgrid heterogeneity, but diagnosing the absolute contributions of each to the radiation bias is hampered by uncertainties and sometimes contradictory information from different observational products. This paper draws on a set of ship‐based observations of boundary layer clouds obtained during the ARM MAGIC campaign along a northeast Pacific Ocean transect, crossing both stratocumulus and shallow cumulus cloud regimes. The surface‐based observations of cloud properties are compared with various satellite products, taking account of the diurnal cycle, to provide an improved quantitative assessment of the deficiencies in the European Centre for Medium‐Range Weather Forecasts global numerical weather prediction model. A series of off‐line radiation calculations are then performed to assess the impact on the shortwave radiation bias of correcting each of the model's deficiencies in cloud characteristics along the transect. A reduction in the bias is achieved by improving the agreement between modeled and observed in‐cloud liquid water path frequency distributions. In the cumulus regime, this is accomplished primarily by reducing the all‐sky water path, while for the stratocumulus regime, an underestimate of cloud cover and liquid water and an overestimate in effective radius and subgrid heterogeneity all contribute to a lack of reflected shortwave radiation.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1988

A 3-dimensional numerical simulation of the atmospheric injection of aerosols by a hypothetical basaltic fissure eruption

Researchers simulated the atmospheric response to a hypothetical basaltic fissure eruption using heating rates based on the Roza flow eruption. The simulation employs the Colorado State University Regional Atmospheric Model (RAMS) with scavenging effects. The numerical model is a three-dimensional non-hydrostatic time-split compressible cloud/mesoscale model. Explicit microphysics include prediction of cloud, rain, crystal, and hail precipitation types. Nucleation and phoretic scavenging are predicted assuming that the pollutant makes an effective cloud droplet nucleus. Smoke is carried as a passive tracer. Long and short wave radiation heating tendencies, including the effects of the smoke, are parameterized. The longwave emission by the lava surface is neglected in the parameterization and included as an explicit heating term instead. A regional scale domain of 100 x 100 km in the horizontal and 22 km high is used. The horizontal grid spacing is taken to be 2 km and the vertical spacing is taken to be 0.75 km. The initial atmospheric state is taken to be horizontally homogenous and based on the standard atmospheric sounding. The fissure is assumed to be 90 km long and oriented in a zig/zag pattern.

Tripoli, Gregory J.↗
NASA NTRS2008

Radiative Susceptibility of Cloudy Atmospheres to Droplet Number Perturbations: 2. Global analysis from MODIS

Global distributions of albedo susceptibility for areas covered by liquid clouds are presented for 4 months in 2005. The susceptibility estimates are based on expanded definitions presented in a companion paper and include relative cloud droplet number concentration (CDNC) changes, perturbations in cloud droplet asymmetry parameter and single-scattering albedo, atmospheric/surface effects, and incorporation of the full solar spectrum. The cloud properties (optical thickness and effective radius) used as input in the susceptibility calculations come from MODIS Terra and Aqua Collection 5 gridded data. Geographical distributions of susceptibility corresponding to absolute ( absolute cloud susceptibility ) and relative ( relative cloud susceptibility ) CDNC changes are markedly different indicating that the detailed nature of the cloud microphysical perturbation is important for determining the radiative forcing associated with the first indirect aerosol effect. However, both types of susceptibility exhibit common characteristics such as significant reductions when perturbations in single-scattering properties are omitted, significant increases when atmospheric absorption and surface albedo effects are ignored, and the tendency to decrease with latitude, to be higher over ocean than over land, and to be statistically similar between the morning and afternoon MODIS overpasses. The satellite-based susceptibility analysis helps elucidate the role of present-day cloud and land surface properties in indirect aerosol forcing responses. Our realistic yet moderate CDNC perturbations yield forcings on the order of 1-2 W/sq m for cloud optical property distributions and land surface spectral albedos observed by MODIS. Since susceptibilities can potentially be computed from model fields, these results have practical application in assessing the reasonableness of model-generated estimates of the aerosol indirect radiative forcing.

Oreopoulos, Lazaros↗
NASA NTRSDate not supplied

Evaluating Subgrid-Scale Properties of Low Clouds over the Beaufort Sea in Arctic System Reanalysis using ARISE Airborne In Situ Observations

Arctic low clouds influence the evolution of the Arctic system through their effects on radiative fluxes, boundary layer mixing, stability, turbulence, humidity, and precipitation. Unfortunately, atmospheric models and retrospective analysis (reanalysis) products struggle to accurately simulate the occurrence and properties of low clouds in the Arctic. To better understand the magnitude and possible causes of this problem, we analyze the disagreements between the Arctic System Reanalysis version 2 (ASR) and data taken during the September 2014 Arctic Radiation-IceBridge Sea and Ice Experiment (ARISE) airborne campaign conducted over the Beaufort Sea. Previous analysis of grid scale-averaged meteorological variables revealed a lack of cloud water produced in ASR, related to warm/dry biases, a failure to produce sufficient cloud water in conditions that are observed to be favorable for large cloud water values, and sampling issues with the ARISE flight paths. However, ARISE collected meteorological observations at one second intervals, offering spatial data resolution comparable to the subgrid scale of ASR. Subgrid scale properties and processes must be parameterized in conventional atmospheric models and reanalyses such as ASR, and often rely on assumed distributions of meteorological variables about the grid box mean state. To enable an examination of the realism of ASR’s subgrid scale properties, we use high resolution data from ARISE determine the “subgrid scale” distributions of cloud water and thermodynamic variables in the real atmosphere. Preliminary results show that the subgrid scale distribution of thermodynamic variables about the grid scale mean resembles the triangular distribution assumed in many bulk microphysical parameterization schemes, but also with tails resembling Gaussian distributions. The main goal is to understand the partitioning of the total available atmospheric water into water vapor and cloud water. Models typically covert some percentage of total water in a grid box to cloud water based on the estimated amount of supersaturation from the assumed vapor distribution. The ARISE measurements can reveal the relationship between subgrid scale supersaturation and the partition between cloud water and water vapor.

Jason Brant Dodson↗
NASA NTRSDate not supplied

A Path to Improving Simulated Properties of Low Clouds over the Beaufort Sea using Airborne In Situ Observations of Subgrid-Scale Variability

Arctic low clouds influence the evolution of the Arctic system through their effects on radiative fluxes, boundary layer mixing, stability, turbulence, humidity, and precipitation. Unfortunately, atmospheric models and retrospective analysis (reanalysis) products struggle to accurately simulate the occurrence and properties of low clouds in the Arctic. One of the main reasons for this problem are the possible unrealistic assumptions that models/reanalyses make about the subgrid-scale (SGS) variability of meteorological properties, as well as the relationship between SGS variability and grid-scale (GS) cloud properties. We utilize cloud and thermodynamic data of low level (primarily) liquid clouds collected from two aircraft campaigns conducted over the Beaufort Sea to better understand and characterize this problem. Examining data from the September 2014 Arctic Radiation-IceBridge Sea and Ice Experiment (ARISE) airborne campaign reveals that GS cloud water variability is closely related with SGS distribution of total water (i.e. water vapor + cloud water). Multiple models/reanalyses use SGS supersaturated total water (relative to GS saturation) as a threshold for partitioning available water for condensation, and indeed we find significant correlation between GS cloud water and SGS supersaturation. However, we also find that the assumption of a static threshold of 100% saturation to be unrealistic. Empirical calculations from the ARISE data show a large sensitivity of this threshold to GS relative humidity, and so a microphysical parameterization allowing the threshold to vary according to GS thermodynamic properties may result in more realistic GS cloud water values. Finally, to determine how sensitive the ARISE-derived results are to that particular campaign, we include additional data from the First International Satellite Cloud Climatology Project (ISCCP) Regional Experiment (FIRE)–Arctic Cloud Experiment (ACE) conducted in 1998. The inclusion of the second dataset will help with demonstrating the robustness of the results and their utility in improving the representation of Arctic clouds in models and reanalyses.

J Brant Dodson↗
NASA NTRSDate not supplied

A Path to Improving Simulated Properties of Low Clouds over the Beaufort Sea using Airborne In Situ Observations of Subgrid-Scale Variability

Arctic low clouds influence the evolution of the Arctic system through their effects on radiative fluxes, boundary layer mixing, stability, turbulence, humidity, and precipitation. Unfortunately, atmospheric models and retrospective analysis (reanalysis) products struggle to accurately simulate the occurrence and properties of low clouds in the Arctic. One of the main reasons for this problem are the possible unrealistic assumptions that models/reanalyses make about the subgrid-scale (SGS) variability of meteorological properties, as well as the relationship between SGS variability and grid-scale (GS) cloud properties. We utilize cloud and thermodynamic data of low level (primarily) liquid clouds collected from two aircraft campaigns conducted over the Beaufort Sea to better understand and characterize this problem. Examining data from the September 2014 Arctic Radiation-IceBridge Sea and Ice Experiment (ARISE) airborne campaign and the 1998 First International Satellite Cloud Climatology Project (ISCCP) Regional Experiment (FIRE)–Arctic Cloud Experiment (ACE) reveals that GS cloud water variability is closely related with SGS distribution of total water (i.e. water vapor + cloud water). We investigate two related approaches to prediction of GS cloud properties from SGS variability: the critical saturation ratio method, and the critical relative humidity method. We find significant correlation between GS cloud water and SGS supersaturation when the critical saturation ratio is set at 100%, as well as a notable relationship between GS cloud water and the width of the SGS total water distribution. Critical relative humidity also compares well with GS cloud water. However, we also find that the assumptions of a static critical saturation ratio of 100% to be unrealistic, as well as a fixed SGS distribution width. Empirical calculations from the ARISE data show a large sensitivity of these SGS variables to GS relative humidity, and so a SGS parameterization allowing them to vary according to GS thermodynamic properties may result in more realistic GS cloud water values.

J. Brant Dodson↗
NASA NTRS2013

The Role of Long-Lived Greenhouse Gases as Principal LW Control Knob that Governs the Global Surface Temperature for Past and Future Climate Change

The climate system of the Earth is endowed with a moderately strong greenhouse effect that is characterized by non-condensing greenhouse gases (GHGs) that provide the core radiative forcing. Of these, the most important is atmospheric CO2. There is a strong feedback contribution to the greenhouse effect by water vapor and clouds that is unique in the solar system, exceeding the core radiative forcing due to the non-condensing GHGs by a factor of three. The significance of the non-condensing GHGs is that once they have been injected into the atmosphere, they remain there virtually indefinitely because they do not condense and precipitate from the atmosphere, their chemical removal time ranging from decades to millennia. Water vapor and clouds have only a short lifespan, with their distribution determined by the locally prevailing meteorological conditions, subject to Clausius-Clapeyron constraint. Although solar irradiance is the ultimate energy source that powers the terrestrial greenhouse effect, there has been no discernible long-term trend in solar irradiance since precise monitoring began in the late 1970s. This leaves atmospheric CO2 as the effective control knob driving the current global warming trend. Over geological time scales, volcanoes are the principal source of atmospheric CO2, and the weathering of rocks is the principal sink, with the biosphere participating as both a source and a sink. The problem at hand is that human industrial activity is causing atmospheric CO2, to increase by 2 ppm per year, whereas the interglacial rate has been 0.005 ppm per year. This is a geologically unprecedented rate to turn the CO2 climate control knob. This is causing the global warming that threatens the global environment.

Greenhouse effect↗
DOE OSTI2015

Evaluation of high‐level clouds in cloud resolving model simulations with ARM and KWAJEX observations

Abstract In this study, we evaluate high‐level clouds in a cloud resolving model during two convective cases, ARM9707 and KWAJEX. The simulated joint histograms of cloud occurrence and radar reflectivity compare well with cloud radar and satellite observations when using a two‐moment microphysics scheme. However, simulations performed with a single moment microphysical scheme exhibit low biases of approximately 20 dB. During convective events, two‐moment microphysical overestimate the amount of high‐level cloud and one‐moment microphysics precipitate too readily and underestimate the amount and height of high‐level cloud. For ARM9707, persistent large positive biases in high‐level cloud are found, which are not sensitive to changes in ice particle fall velocity and ice nuclei number concentration in the two‐moment microphysics. These biases are caused by biases in large‐scale forcing and maintained by the periodic lateral boundary conditions. The combined effects include significant biases in high‐level cloud amount, radiation, and high sensitivity of cloud amount to nudging time scale in both convective cases. The high sensitivity of high‐level cloud amount to the thermodynamic nudging time scale suggests that thermodynamic nudging can be a powerful “tuning” parameter for the simulated cloud and radiation but should be applied with caution. The role of the periodic lateral boundary conditions in reinforcing the biases in cloud and radiation suggests that reducing the uncertainty in the large‐scale forcing in high levels is important for similar convective cases and has far reaching implications for simulating high‐level clouds in super‐parameterized global climate models such as the multiscale modeling framework.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2018

Simulated Global Climate Response to Tropospheric Ozone-Induced Changes in Plant Transpiration

Tropospheric ozone (O 3 ) pollution is known to damage vegetation, reducing photosynthesis and stomatal conductance, resulting in modified plant transpiration to the atmosphere. We use an Earth system model to show that global transpiration response to near-present-day surface tropospheric ozone results in large-scale global perturbations to net outgoing long-wave and incoming shortwave radiation. Our results suggest that the radiative effect is dominated by a reduction in shortwave cloud forcing in polluted regions, in response to ozone-induced reduction in land-atmosphere moisture flux and atmospheric humidity. We simulate a statistically significant response of annual surface air temperature of up to ~ +1.5 K due to this ozone effect in vegetated regions subjected to ozone pollution. This mechanism is expected to further increase the net warming resulting from historic and future increases in tropospheric ozone.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2018

Cloud Optical Properties Over West Antarctica From Shortwave Spectroradiometer Measurements During AWARE

A shortwave spectroradiometer was deployed on the West Antarctic Ice Sheet (WAIS) as part of the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) program ARM West Antarctic Radiation Experiment (AWARE). This instrument recorded 1-min averages of downwelling hemispheric spectral irradiance covering the wavelength range 350–2,200 nm with spectral resolution 3 and 10 nm for wavelengths shorter and longer than 1,000 nm, respectively. Using simultaneous micropulse lidar data to identify the thermodynamic phase of stratiform clouds, a radiative transfer algorithm is used here to retrieve optical depth and effective droplet (or particle) size for single-phase liquid water and ice water clouds. The AWARE campaign on the WAIS first sampled typical climatological conditions between 7 December 2015 and 9 January 2016 and then a much warmer air mass with more moisture associated with a surface melt event between 10 and 17 January 2016. Before the melt event most liquid cloud effective droplet radii were consistent with pristine polar maritime clouds (mode radius 13.5 μm) but showed a second local maximum in the distribution (at 8 μm) consistent with colder, moisture-limited conditions. Most ice clouds sampled occurred before the melt event (mode optical depth 4 and effective particle size 19 μm). During the melt event liquid water cloud optical depth nearly doubled (mode value increasing from 8 to 14). AWARE therefore sampled on the WAIS two cases relevant to climate model simulations: typical current climatological conditions, followed by warmer meteorology possibly consistent with future increasing surface melt scenarios.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Global organic and inorganic aerosol hygroscopicity and its effect on radiative forcing

The climate effects of atmospheric aerosol particles serving as cloud condensation nuclei (CCN) depend on chemical composition and hygroscopicity, which are highly variable on spatial and temporal scales. Here we present global CCN measurements, covering diverse environments from pristine to highly polluted conditions. We show that the effective aerosol hygroscopicity, κ, can be derived accurately from the fine aerosol mass fractions of organic particulate matter (ϵ org ) and inorganic ions (ϵ inorg ) through a linear combination, κ = ϵ org · κ org + ϵ inorg · κ inorg . In spite of the chemical complexity of organic matter, its hygroscopicity is well captured and represented by a global average value of κ org = 0.12 ± 0.02 with κinorg = 0.63 ± 0.01 as the corresponding value for inorganic ions. By showing that the sensitivity of global climate forcing to changes in κ org and κ inorg is small, we constrain a critically important aspect of global climate modelling.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2018

Improvement of the Simulation of Cloud Longwave Scattering in Broadband Radiative Transfer Models

Abstract Cloud longwave scattering is generally neglected in general circulation models (GCMs), but it plays a significant and highly uncertain role in the atmospheric energy budget as demonstrated in recent studies. To reduce the errors caused by neglecting cloud longwave scattering, two new radiance adjustment methods are developed that retain the computational efficiency of broadband radiative transfer simulations. In particular, two existing scaling methods and the two new adjustment methods are implemented in the Rapid Radiative Transfer Model (RRTM). The results are then compared with those based on the Discrete Ordinate Radiative Transfer model (DISORT) that explicitly accounts for multiple scattering by clouds. The two scaling methods are shown to improve the accuracy of radiative transfer simulations for optically thin clouds but not effectively for optically thick clouds. However, the adjustment methods reduce computational errors over a wide range, from optically thin to thick clouds. With the adjustment methods, the errors resulting from neglecting cloud longwave scattering are reduced to less than 2 W m−2 for the upward irradiance at the top of the atmosphere and less than 0.5 W m−2 for the surface downward irradiance. The adjustment schemes prove to be more accurate and efficient than a four-stream approximation that explicitly accounts for multiple scattering. The neglect of cloud longwave scattering results in an underestimate of the surface downward irradiance (cooling effect), but the errors are almost eliminated by the adjustment methods (warming effect).

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

A Process Model for ITCZ Narrowing under Warming Highlights Clear-Sky Water Vapor Feedbacks and Gross Moist Stability Changes in AMIP Models

Tropical areas with mean upward motion—and as such the zonal-mean intertropical convergence zone (ITCZ)—are projected to contract under global warming. To understand this process, a simple model based on dry static energy and moisture equations is introduced for zonally symmetric overturning driven by sea surface temperature (SST). Processes governing ascent area fraction and zonal mean precipitation are examined for insight into Atmospheric Model Intercomparison Project (AMIP) simulations. Bulk parameters governing radiative feedbacks and moist static energy transport in the simple model are estimated from the AMIP ensemble. Uniform warming in the simple model produces ascent area contraction and precipitation intensification—similar to observations and climate models. Contributing effects include stronger water vapor radiative feedbacks, weaker cloud-radiative feedbacks, stronger convection-circulation feedbacks, and greater poleward moisture export. The simple model identifies parameters consequential for the inter-AMIP-model spread; an ensemble generated by perturbing parameters governing shortwave water vapor feedbacks and gross moist stability changes under warming tracks inter-AMIP-model variations with a correlation coefficient ~0.46. Here, the simple model also predicts the multimodel mean changes in tropical ascent area and precipitation with reasonable accuracy. Furthermore, the simple model reproduces relationships among ascent area precipitation, ascent strength, and ascent area fraction observed in AMIP models. A substantial portion of the inter-AMIP-model spread is traced to the spread in how moist static energy and vertical velocity profiles change under warming, which in turn impact the gross moist stability in deep convective regions—highlighting the need for observational constraints on these quantities.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1974

Multiple scattering in cloud layers; some results

Theoretical methods are discussed for calculating radiative effects of aerosols. Experimental determination is emphasized for relevant aerosol parameters on a global basis to arrive at realistic estimates of heating and cooling. Internal radiation fields in very thin and very thick slabs are reviewed. Phase functions, polarization, emission by internal sources, and path length distribution are also considered.

Vandehulst, H. C.↗
NASA NTRS1991

Remote sensing cloud properties from simulated MODIS observations

One of the objectives of the MODIS program is to establish a global cloud climatology that can address the effects of cirrus and opaque clouds on the Earth Radiation Budget. The paper describes the cloud retrieval techniques developed for MODIS-N IR observations and presents results of a study of remote sensing cloud properties using simulated MODIS observations at different cirrus cloud conditions.

Menzel, W. P.↗