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At least 847 records · Page 47

Correlations Between Panoramic Imagery and Gamma-Ray Background in an Urban Area

When searching for radiological sources in an urban area, a vehicle-borne detector system will often measure complex, varying backgrounds primarily from natural gamma-ray sources. Much work has been focused on developing spectral algorithms that retain sensitivity and minimize the false-positive rate even in the presence of such spectral and temporal variability. However, information about the environment surrounding the detector system might also provide useful clues about the expected background, which if incorporated into an algorithm, could improve performance. Recent work has focused on extensive measuring and modeling of urban areas with the goal of understanding how these complex backgrounds arise. This work presents an analysis of panoramic video images and gamma-ray background data collected in Oakland, California, by the radiological multisensor analysis platform (RadMAP) vehicle. Features were extracted from the panoramic images by semantically labeling the images and then convolving the labeled regions with the detector response. A linear model was used to relate the image-derived features to gamma-ray spectral features obtained using nonnegative matrix factorization (NMF) under different regularizations. Here we find some gamma-ray background features correlate strongly with image-derived features that measure the response-adjusted solid angle subtended by sky and buildings, and we discuss the implications for the development of future, contextually aware detection algorithms.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Design and characterization of a new high-dose-rate brachytherapy Valencia applicator for larger skin lesions

Purpose: The aims of this study were (i) to design a new high-dose-rate (HDR) brachytherapy applicator for treating surface lesions with planning target volumes larger than 3 cm in diameter and up to 5 cm in size, using the microSelectron-HDR or Flexitron afterloader (Elekta Brachytherapy) with a {sup 192}Ir source; (ii) to calculate by means of the Monte Carlo (MC) method the dose distribution for the new applicator when it is placed against a water phantom; and (iii) to validate experimentally the dose distributions in water. Methods: The PENELOPE2008 MC code was used to optimize dwell positions and dwell times. Next, the dose distribution in a water phantom and the leakage dose distribution around the applicator were calculated. Finally, MC data were validated experimentally for a {sup 192}Ir mHDR-v2 source by measuring (i) dose distributions with radiochromic EBT3 films (ISP); (ii) percentage depth–dose (PDD) curve with the parallel-plate ionization chamber Advanced Markus (PTW); and (iii) absolute dose rate with EBT3 films and the PinPoint T31016 (PTW) ionization chamber. Results: The new applicator is made of tungsten alloy (Densimet) and consists of a set of interchangeable collimators. Three catheters are used to allocate the source at prefixed dwell positions with preset weights to produce a homogenous dose distribution at the typical prescription depth of 3 mm in water. The same plan is used for all available collimators. PDD, absolute dose rate per unit of air kerma strength, and off-axis profiles in a cylindrical water phantom are reported. These data can be used for treatment planning. Leakage around the applicator was also scored. The dose distributions, PDD, and absolute dose rate calculated agree within experimental uncertainties with the doses measured: differences of MC data with chamber measurements are up to 0.8% and with radiochromic films are up to 3.5%. Conclusions: The new applicator and the dosimetric data provided here will be a valuable tool in clinical practice, making treatment of large skin lesions simpler, faster, and safer. Also the dose to surrounding healthy tissues is minimal.

60 APPLIED LIFE SCIENCES↗

SU-F-J-75: Accuracy and Stability of Electron Density Measurements Across Patient Size Using Dual Energy CT

Purpose: Dual energy (DE) CT can be used to characterize tissue composition. One application of DE CT is to measure electron density (ED, rho) and atomic number (Z) for use in radiation therapy treatment planning. This work evaluated the accuracy and stability of ED estimation as patient size varied for both single-energy (SE) and DE CT. Methods: An ED phantom (CIRS) and four torso-shaped water tanks (lateral widths 15, 25, 35 and 45 cm) containing 8 tissue-simulating cylinders of known ED were scanned on a dual-source CT system (Siemens Somatom Force) in SE (120 kV) and DE (90/150Sn) modes. Additional scans were performed on the 15 and 25 cm water tanks using DE techniques of 70/150Sn and 80/150Sn, respectively. CTDIvol was matched for all SE and DE scans for a given phantom size. Images were reconstructed using quantitative kernels to preserve CT number accuracy. ED was estimated in each test cylinder and in solid and liquid water using calibration measurements acquired in the CIRS phantom (SE) and a Rho-Z algorithm (DE). Results: ED estimates showed good agreement with the nominal ED values when using Rho-Z (slope = 1.0051, R2 = 0.9982). Mean percent error was similar between SE (1.21%) and DE (1.28%). Mean deviation across patient size decreased 34% (1.43% with SE, 0.95% with DE). When compared to 90/150Sn, DE techniques of 70/150Sn and 80/150Sn showed mean differences in ED of 0.43% and 0.15%, respectively. Conclusion: While both DE Rho-Z and SE CT number calibration methods are both accurate for estimating ED, Rho-Z offers the advantages of having less variability across patient size, not requiring a phantom calibration, and being able to distinguish between materials of similar attenuation, but different chemical composition. Low kV DE pairs are an option in small patients due to lack of effect on ED accuracy. This research was supported by Siemens Healthcare.

60 APPLIED LIFE SCIENCES↗

Quantitative Correction of Ohmic Effects on Square Wave Voltammetry for High-Concentration Soluble-Soluble Redox Reactions in Molten Salts

Molten salts are of particular interest for a variety of industrial applications. As such, accurate characterization of species’ concentrations within the molten salt media is critical to ensure a well-controlled unit operation. Although electroanalytical tools are properly suited for precise in situ monitoring in these systems, uncompensated ohmic resistance R Ω can lead to erroneous, technique-dependent results. Using numerical simulations applied to a model system, this work will first illustrate then quantify the extent to which R Ω attenuates square wave voltammograms. This approach allows for post-experiment correction that leads to converging results across voltammetric techniques and facilitates accurate predictions of species’ concentrations.

Shaheen, Nora A. [Argonne National Laboratory (ANL↗

Lithium Vanadium Oxide (Li 1.1 V 3 O 8 ) Coated with Amorphous Lithium Phosphorous Oxynitride (LiPON): Role of Material Morphology and Interfacial Structure on Resulting Electrochemistry

In the present work, lithium vanadium oxide (Li 1.1 V 3 O 8 ) particles synthesized at two different temperatures were coated with an amorphous lithium phosphorous oxynitride (LiPON) film for the first time, and the effects of the LiPON coating on the electrochemistry of the Li 1.1 V 3 O 8 materials with different morphologies were systematically investigated by comparing uncoated Li 1.1 V 3 O 8 and Li 1.1 V 3 O 8 coated with LiPON of various thicknesses. Galvanostatic discharge-charge cycling revealed increased functional capacity for the LiPON-coated materials. Post-cycling electrochemical impedance spectroscopy showed that LiPON-coated Li 1.1 V 3 O 8 materials developed less interfacial resistance with extended cycling, rationalized by vanadium migration into the LiPON coating seen by electron energy loss spectra. Post-mortem quantitative analysis of the anodes revealed more severe vanadium dissolution for the more irregularly shaped Li 1.1 V 3 O 8 materials with less LiPON coverage. Thus, this study highlights the specific benefits and limitations of LiPON coatings for stabilizing a moderate voltage Li 1.1 V 3 O 8 cathode material under extended cycling in liquid electrolyte, and describes a generally applicable approach for comprehensive characterization of a composite electroactive material which can be used to understand interfacial transport properties in other functional systems.

25 ENERGY STORAGE↗

Scalable photonic integrated circuits for high-fidelity light control

Advances in laser technology have driven discoveries in atomic, molecular, and optical (AMO) physics and emerging applications, from quantum computers with cold atoms or ions, to quantum networks with solid-state color centers. This progress is motivating the development of a new generation of optical control systems that can manipulate the light field with high fidelity at wavelengths relevant for AMO applications. These systems are characterized by criteria: (C1) operation at a design wavelength of choice in the visible (VIS) or near-infrared (IR) spectrum, (C2) a scalable platform that can support large channel counts, (C3) high-intensity modulation extinction and (C4) repeatability compatible with low gate errors, and (C5) fast switching times. Here, we provide a pathway to address these challenges by introducing an atom control architecture based on VIS-IR photonic integrated circuit (PIC) technology. Based on a complementary metal–oxide–semiconductor fabrication process, this atom-control PIC (APIC) technology can meet system requirements (C1)–(C5). As a proof of concept, we demonstrate a 16-channel silicon-nitride-based APIC with (5.8±0.4)ns response times and >30dB extinction ratio at a wavelength of 780 nm.

Menssen, Adrian J.↗

Hardening of DOE UQ Codes for Ultra-Deep Proactive Geosteering in Oilfield Service

The primary objective of this project was to harden the DOE uncertainty quantification (UQ) code to solve the inverse problem for the geosteering service in the oilfield drilling and exploration. The primary focus is to verify the feasibility of using QUESO to solve geosteering inverse problems through statistical inversion. QUESO is a software library developed by QUEST, a DOE's Scientific Discovery through Advanced Computing (SciDAC) institute. In the process of drilling a borehole, geosteering is the act of adjusting the well trajectory on the fly to reach the geological targets or to keep the wellbore within desired formation. Geosteering inversion is to infer underground formation structure using measurements such as azimuthal resistivity logging data. The geosteering process relies on the real-time reconstruction of the subsurface earth model, and a robust and efficient inversion algorithm is always necessary to satisfy the job requirement. The new generation of azimuthal resistivity geosteering tool is capable of detecting multiple formation boundaries 20-100 ft away, and the corresponding geosteering inversion problem can be very challenging as many parameters need to be inverted within such a large depth of investigation. The success of the project will support US energy security by helping to advance subsurface modeling and characterization technologies in oilfield applications. An effective subsurface inversion algorithm and the implementation as a software package will promote the usage of ultra-deep azimuthal resistivity measurements, which can help well placement in complicated underground environments, reduce costs and risks of drilling, and increase oil and gas production. It will help medium and small size independent service companies and tool manufactures to enter the more advanced and lucrative directional drilling area. In addition, by hardening the QUESO code and building a transparent interface for easy manipulation of the QUESO functions, we provide a user-friendly tool for a larger scientific and industry communities that rely heavily on modeling and simulation tools for forecasting, parameter studies, design, and decision making. These are all activities that can strongly benefit from meaningful representations of modeling uncertainty supported by our product.

58 GEOSCIENCES↗

GADRAS-DRF 18.6 User's Manual

The Gamma Detector Response and Analysis Software–Detector Response Function (GADRAS-DRF) application computes the response of gamma-ray and neutron detectors to incoming radiation. This manual provides step-by-step procedures to acquaint new users with the use of the application. The capabilities include characterization of detector response parameters, plotting and viewing measured and computed spectra, analyzing spectra to identify isotopes, and estimating source energy distributions from measured spectra. GADRAS-DRF can compute and provide detector responses quickly and accurately, giving users the ability to obtain usable results in a timely manner (a matter of seconds or minutes).

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Investigation of Computational Corrections to X-Ray Computed Tomography for Dimensional Metrology of Complex Additively Manufactured Parts

X-ray computed tomography (CT) is a nondestructive evaluation technique that may be used to image complex internal features without the line-of-sight restrictions inherent in conventional optical and contact (stylus) metrology instrumentation. Applications of CT metrology include material defects (porosity), dimensions and surface texture. However, scan artifacts, such as streaking, caused primarily by beam hardening and scatter, limit the accuracy of CTbased metrology. Reduction of these artifacts would improve the accuracy material properties and dimensional metrology information. This paper reports on the development of additively manufactured (AM) Ti5553 and 316L measurement phantoms with integral lattice (lattice) structures specifically designed to exhibit these artifacts. The phantoms were scanned in three CT systems and a scanning-probe CMM measurement. Surfaces generated from uncorrected CT data exhibited “dimple” defects that are not present in the CMM measurement. Correction methods were developed in Livermore Tomography Tools (LTT) software and this paper reports on the successful correction of these artifacts. This work is expected to have application in areas where characterization of defects, dimensions and surface texture using CT are critical.

42 ENGINEERING↗

GADRAS-DRF Version 18 User's Manual

The Gamma Detector Response and Analysis Software Detector Response Function (GADRAS-DRF) application computes the response of gamma-ray and neutron detectors to incoming radiation and provides analysis on measured spectra. This manual provides step-by-step procedures to acquaint new users with the use of the application. The capabilities include characterization of detector response parameters, plotting and viewing measured and computed spectra, analyzing spectra to identify isotopes, estimating source energy distributions from measured spectra, and creating inject data. GADRAS-DRF can compute and provide detector responses quickly and accurately, giving users the ability to obtain usable results in a timely manner (a matter of seconds or minutes).

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Design and Validation of a Cryogenic Dilatometer

This project focuses on the design and development of a cryogenic dilatometer capable of measuring the thermal expansion of materials at extremely low temperatures. Understanding how materials change dimension with temperature is critical for applications involving cryogenic environments, particularly laminated systems housing superconducting magnets, where small dimensional changes can significantly affect performance and reliability. To address this, a dilatometer system was designed to operate within a liquid nitrogen environment while accurately measuring displacements caused by thermal contraction. The purpose of this device is to determine the coefficient of thermal expansion (CTE) of a material. The design process involved defining functional requirements, developing mechanical and thermal concepts for the measurement apparatus, selecting appropriate materials compatible with cryogenic temperatures, and integrating sensors capable of detecting small dimensional changes. The resulting system aims to provide a practical and repeatable method for evaluating material thermal expansion at cryogenic temperatures, supporting research into composite use in superconducting applications that require accurate characterization of material behavior in low-temperature environments.

Schmitt, Nicholas [Northern Illinois U.]↗

Scaling Sustainable Biochar Research & Commercialization for Agriculture & Conservation: A Summary from a Stakeholder Convening

Biochar is a carbon-rich substance with the potential to increase soil carbon sequestration, reduce greenhouse gas (GHG) emissions and improve soil health. When used as part of soil health management systems, biochar can provide multiple synergistic benefits for the agricultural sector and society, while also supporting the production of renewable, climate-neutral biofuels. Establishing a pyrolysis biochar bioenergy industry (PBBI) is necessary to harness the environmental benefits of biochar. To galvanize the necessary coordination to support a PBBI, the Foundation for Food & Agriculture Research (FFAR), the National Center for Appropriate Technology (NCAT), and American Farmland Trust (AFT) co-hosted a virtual convening event on biochar research and commercialization in March 2022. Participants represented a diverse set of stakeholders, including biochar producers, agricultural producers, and members of nonprofit, industry and government agencies. This whitepaper offers a summary of the convening, as well as insights from subsequent stakeholder engagement. Sustainably sourced, fit-for-purpose biochar can be a powerful tool in the soil health management systems and climate-smart toolbox, with decades of research supporting the soil, environment, production, and climate benefits. However, because biochar represents a range of feedstocks, processes and products, there is a critical need to: • Coordinate efforts to characterize and test the application of biochar types across locations with diverse soil and management conditions • Address research and decision-support gaps • Support the growing industry These objectives can be addressed or advanced through a coordinated strategy. To support establishment of this strategy, the convening participants identified key gaps in implementation and research. The experiences of foresters, ranchers, and farmers already using biochar, some of whom participated in the convening, helped inform priorities. Key gaps include: • Practical, applied on-farm research • Supporting management for agricultural productivity • Maximum benefits for conservation • Decision support • Life Cycle Assessment (LCA) • Quantification of climate mitigation potential Existing research gaps include: • Potential synergies among biochar, soil organic matter, and enhanced rock weathering • Development of new storage reservoirs for biochar in industrial products Convening participants further provided next steps for rapidly developing a PBBI to produce sustainable, fit-for-purpose biochars that increase soil health and mitigate climate change. Participants also stressed the need for actionable, coordinated, large-scale research relevant to commercial production in the next five years. To have a chance to reduce greenhouse gas emissions, we need an array of tools that would aid in mitigation; a coordinated strategy to enable biochar to be an effective tool in the climate-smart toolbox must be created; We cannot wait 50 years.

54 ENVIRONMENTAL SCIENCES↗

Characterization of High-Entropy Alloys for Accelerator Beam Window Applications

Particle production targets and accelerator beam windows receive millions of high-energy/intensity beam pulses throughout their service lifetime. For next-generation multi-MW accelerators, it is necessary for beam windows to be able to withstand higher levels of thermal shock and radiation damage, while also having good high-temperature mechanical properties. Novel High-Entropy Alloys (HEAs) that form a single-phase microstructure, have nanoscale precipitates, and are made from low-Z elements are good candidates for beam window materials. This is due to their high-temperature strength and high resistance to radiation-induced swelling and hardening, as well as their beam transparency, allowing for maximized particle production and a longer service lifetime.

Kidwell, Tristan [U. Chicago (main)] (ORCID:000900↗

Digital Miniature Cathode Ray Magnetometer

In this study, we introduce the concept and construction of an innovative Digital Miniature Cathode Ray Magnetometer designed for the precise detection of magnetic fields. This device addresses several limitations inherent to magnetic probes such as D.C. offset, nonlinearity, temperature drift, sensor aging, and the need for frequent recalibration, while capable of operating in a wide range of magnetic fields. The core principle of this device involves the utilization of a charged particle beam as the sensitivity medium. The system leverages the interaction of an electron beam with a scintillator material, which then emits visible light that is captured by an imager. The emitted scintillation light is captured by a CMOS sensor. This sensor not only records the scintillation light but also accurately determines the position of the electron beam, providing invaluable spatial information crucial for magnetic field mapping. The key innovation lies in the combination of electron beam projection, CMOS imager scintillation-based detection, and digital image signal processing. By employing this synergy, the magnetometer achieves remarkable accuracy, sensitivity and dynamic range. The precise position registration enabled by the CMOS sensor further enhances the device’s utility in capturing complex magnetic field patterns, allowing for 2D field mapping. In this work, the optimization of the probe’s performance is tailored for applications related to the characterization of insertion devices in light sources, including undulators.

Turqueti, Marcos↗

THE SOLAR NEIGHBORHOOD. XXXVII. THE MASS–LUMINOSITY RELATION FOR MAIN-SEQUENCE M DWARFS

We present a mass–luminosity relation (MLR) for red dwarfs spanning a range of masses from 0.62 M{sub ⊙} to the end of the stellar main sequence at 0.08 M{sub ⊙}. The relation is based on 47 stars for which dynamical masses have been determined, primarily using astrometric data from Fine Guidance Sensors (FGS) 3 and 1r, white-light interferometers on the Hubble Space Telescope (HST), and radial velocity data from McDonald Observatory. For our HST/FGS sample of 15 binaries, component mass errors range from 0.4% to 4.0% with a median error of 1.8%. With these and masses from other sources, we construct a V-band MLR for the lower main sequence with 47 stars and a K-band MLR with 45 stars with fit residuals half of those of the V band. We use GJ 831 AB as an example, obtaining an absolute trigonometric parallax, π {sub abs} = 125.3 ± 0.3 mas, with orbital elements yielding M{sub A}=0.270±0.004 M{sub ⊙} and M{sub B}=0.145±0.002 M{sub ⊙}. The mass precision rivals that derived for eclipsing binaries. A remaining major task is the interpretation of the intrinsic cosmic scatter in the observed MLR for low-mass stars in terms of physical effects. In the meantime, useful mass values can be estimated from the MLR for the ubiquitous red dwarfs that account for 75% of all stars, with applications ranging from the characterization of exoplanet host stars to the contribution of red dwarfs to the mass of the universe.

79 ASTRONOMY AND ASTROPHYSICS↗

Detecting Atmospheric Molecules of Nontransiting Temperate Terrestrial Exoplanets Using High-resolution Spectroscopy in the Mid-infrared Domain

Motivated by the development of high-dispersion spectrographs in the mid-infrared (MIR) range, we study their application to the atmospheric characterization of nearby nontransiting temperate terrestrial planets around M-type stars. We examine the detectability of CO{sub 2}, H{sub 2}O, N{sub 2}O, and O{sub 3 }features in high-resolution planetary thermal emission spectra at 12–18 μm assuming an Earth-like profile and a simplified thermal structure. The molecular line width of such planets can be comparable to or broader than the Doppler shift due to the planetary orbital motion. Given the likely difficulty in knowing the high-resolution MIR spectrum of the host star with sufficient accuracy, we propose observing the target system at two quadrature phases and extracting the differential spectra as the planetary signal. In this case, the signals can be substantially suppressed compared with the case where the host star spectrum is perfectly known, as some parts of the spectral features do not remain in the differential spectra. Despite this self-subtraction, the CO{sub 2} and H{sub 2}O features of nearby (≲5 pc) systems with mid-/late-M host stars would be feasible with a 6.5 m class cryogenic space telescope, and orbital inclination could also be constrained for some of them. For CO{sub 2} and N{sub 2}O in a 1 bar Earth-like atmosphere, this method would be sensitive when the mixing ratio is 1–10{sup 3} ppm. The detectability of molecules except O{sub 3} is not significantly improved when the spectral resolution is higher than R≳10,000, although the constraint on the orbital inclination is improved. This study provides some benchmark cases useful for assessing the value of MIR high-resolution spectroscopy in terms of characterization of potentially habitable planets.

47 OTHER INSTRUMENTATION↗

High Strain Rate Mechanical Characterization of Carbon Fiber Reinforced Polymer Composites Using Digital Image Correlations

We present that the introduction of carbon fiber reinforced polymer (CFRP) composites to structural components in lightweight automotive structures necessitates an assessment to evaluate that their crashworthiness dynamic response provides similar or higher levels of safety compared to conventional metallic structures. In order to develop, integrate and implement predictive computational models for CFRP composites that link the materials design, molding process and final performance requirements to enable optimal design and manufacturing vehicle systems for this study, the dynamic mechanical response of unidirectional (UD) and 2x2 twill weave CRFP composites was characterized at deformation rates applicable to crashworthiness performance. Non-standardized specimen geometries were tested on a standard uniaxial frame and an intermediate-to-high speed dynamic testing frame, equipped with high speed cameras for 3D digital image correlation (DIC). Specimen cross-sections, according to each fiber orientation tested, were consistent across strain rates to ensure results were comparable. Tensile strength and modulus were experimentally investigated over a wide range of strain rates (0.0001 to 200 s -1 ). DIC was used to estimate strain profiles on composites surfaces, and the modulus was calculated from those strain measurements. Experimental results demonstrated an increase in the tensile strength of UD CFRP composites in the longitudinal (0°) and transverse (90°) direction with increasing strain rates. In contrast, the tensile strength of 2x2 woven composites and the tensile modulus of the UD material were insensitive to increasing strain rates. Finally, comparison of failure modes provided insights on how loading rates influenced failure mechanisms.

36 MATERIALS SCIENCE↗