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Progress on Long-Term Objectives for the Development of Advanced Reactor Mechanistic Source Term Modeling and Simulation Tools

To assist both the advanced reactor industry and U.S. Nuclear Regulatory Commission (NRC) in the pursuit of reactor design and licensing, the U.S. Department of Energy (DOE) Nuclear Energy Advanced Modeling and Simulation (NEAMS) program has established a mechanistic source term (MST) research project under the auspices of the Multiphysics Applications technical area. MST analysis is central to the reactor licensing process and a focus of the NRC regarding their mission to provide reasonable assurance of adequate protection of public health and safety and environment. The MST research project is a collaboration between Argonne National Laboratory (Argonne) and Sandia National Laboratories (SNL) with a high-level objective to coordinate the development of comprehensive advanced reactor MST mod/sim capabilities to support risk-informed design and licensing decisions. As part of this effort, an MST mod/sim development pathway was developed in FY21, which outlines the high-level objectives and near-term tasks necessary to achieve the project objectives. Since publication of the development pathway, Argonne and SNL have focused initial efforts on addressing the “near-term tasks” outlined in the report, and the current work provides a status update of the progress achieved in FY22. This report is a progress update on 6 tasks supporting molten salt reactor (MSR) and sodium fast reactor (SFR) MST analyses which were initiated in FY22 as recommended high priority near-term tasks. These tasks were continued into FY23 as they also support previously recommended long-term development objectives to advance MST analyses for these advanced reactors.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Advanced Reactor Designs Security Analysis, Risk, and Recommendations: Risks, Consequences, and Possible by-Design Mitigation Approaches Associated with Select Advanced Reactors

Next-generation advanced reactors (ARs) incorporate enhanced safety systems, have smaller source terms, and feature compact modular designs, which should lessen their collective risk profiles. However, to fully evaluate risk, security needs to be a part of the equation. Without taking security into consideration, safety systems and components in the new ARs may be vulnerable to sabotage. These base attributes, coupled with enhanced security features specific to AR design through sound engineering and security-by-design (SeBD), should provide developers and operators with lower inherent security risk profiles. Building security early into the AR design may remove or passively secure potential critical targets from an adversary’s reach , thereby increasing overall safety and security. An integrated approach and diverse design team that includes engineering, operations, and security experts are fundamental to building security into the design without sacrificing fundamental operational efficiencies and principles. The objective of this project was to evaluate the security and safety interfaces for five classes of reactors, identify potential security vulnerabilities of structures, systems, and components (SSC), and underscore the need to consider security alongside safety in the design o f these concepts. The five reactor classes evaluated in this project and presented in this report are molten-salt reactors (MSR), high temperature gas reactors (HTGR), sodium-fast reactors (SFR), advanced light-water reactors (ALWR), and microreactors. These designs were selected because they reflect the concepts that are closest to market deployment and have received significant resource investments from the public and private sector. This project assesses the inherent security risks posed by common classes of ARs, provides a methodology and framework to assess security along with safety, and offers an analysis of potential mitigation strategies that could be incorporated. For each AR technology, the SSCs that relate to radionuclide source safety functions are discussed to understand the SSC contribution to safety and relative importance in the protective strategy for the design. The assumptions that went into evaluating each reactor concept originated from generic publicly available nonproprietary information and should not directly be used to qualify an absolute risk profile nor to rank specific AR designs. Instead, the purpose of the analysis is to understand and compare the generic inherent security risks of different AR technologies.

98 - NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL↗

Large Language Model for Validation, Optical Calibration, and Learning (VOCAL) Distributed Temperature Sensing Interface

Distributed temperature sensing (DTS) using fiber optic sensors (FOS) offers a promising method for temperature measurements in advanced reactors, such as sodium fast reactors and molten salt cooled reactors. To support the calibration and validation of DTS measurements, Argonne National Laboratory developed the Validation, Optical Calibration, and Learning (VOCAL) software package. This report describes the integration of a local large language model (LLM) with a retrieval-augmented generation (RAG) system into the VOCAL interface to serve as an interactive user assistant. The LLM framework enhances the VOCAL platform’s accessibility to users by explaining interface components, clarifying inputs and outputs, and answering user queries dynamically in real-time. The accuracy of the LLM assistant performance was evaluated with 20 queries regarding the interface and its parameters using experimental data from the Thermal Hydraulic Experimental Test Article (THETA) facility. Results demonstrate that the LLM achieved a 95% accuracy rate, with a BERTScore of 0.8816 and SBERT value of 0.7417. Furthermore, validation of the RAG system within the LLM framework showed optimal accuracy with k-values between 1 and 2 using the k-refinement convergence test. The prompt perturbation analysis demonstrated good initial consistency for the RAG system, exhibiting the highest accuracy under punctuation variations and the greatest sensitivity under query reordering. Notably, the model’s errors were limited to data retrieval failures rather than factual hallucinations, reinforcing its baseline reliability. The integration of LLM provides a highly accurate, userfriendly enhancement to the VOCAL platform without disrupting its core computational capabilities for FOS calibration and validation.

Hong, Evan↗

Progress Towards Developing Neutron Tolerant Magnetostrictive and Piezoelectric Transducers

Current generation light water reactors (LWRs), sodium cooled fast reactors (SFRs), small modular reactors (SMRs), and next generation nuclear plants (NGNPs) produce harsh environments in and near the reactor core that can severely tax material performance and limit component operational life. To address this issue, several Department of Energy Office of Nuclear Energy (DOE-NE) research programs are evaluating the long duration irradiation performance of fuel and structural materials used in existing and new reactors. In order to maximize the amount of information obtained from Material Testing Reactor (MTR) irradiations, DOE is also funding development of enhanced instrumentation that will be able to obtain in-situ, real-time data on key material characteristics and properties, with unprecedented accuracy and resolution. Such data are required to validate new multi-scale, multi-physics modeling tools under development as part of a science-based, engineering driven approach to reactor development. It is not feasible to obtain high resolution/microscale data with the current state of instrumentation technology. However, ultrasound-based sensors offer the ability to obtain such data if it is demonstrated that these sensors and their associated transducers are resistant to high neutron flux, high gamma radiation, and high temperature. To address this need, the Advanced Test Reactor National Scientific User Facility (ATR-NSUF) is funding an irradiation, led by PSU, at the Massachusetts Institute of Technology Research Reactor to test the survivability of ultrasound transducers. As part of this effort, PSU and collaborators have designed, fabricated, and provided piezoelectric and magnetostrictive transducers that are optimized to perform in harsh, high flux, environments. Four piezoelectric transducers were fabricated with either aluminum nitride, zinc oxide, or bismuth titanate as the active element that were coupled to either Kovar or aluminum waveguides and two magnetostrictive transducers were fabricated with Remendur or Galfenol as the active elements. Pulse-echo ultrasonic measurements of these transducers are made in-situ. This paper will present an overview of the test design including selection criteria for candidate materials and optimization of test assembly parameters, data obtained from both out-of-pile and in-pile testing at elevated temperatures, and an assessment based on initial data of the expected performance of ultrasonic devices in irradiation conditions

Reinhardt1, Brian↗

Neutron initiation probability in fast burst reactor

Based on the probability balance of neutron random events in multiply system, the four random process of neutron in prompt super-critical is described and then the equation of neutron initiation probability W(r,E,{Omega},t) is deduced. On the assumption of static, slightly prompt super-critical and the two factorial approximation, the formula of the average probability of 'one' neutron is derived which is the same with the result derived from the point model. The MC simulation using point model is applied in Godiva- II and CFBR-II, and the simulation result of one neutron initiation is well consistent with the theory that the initiation probability of Godiva- II inverted commas CFBR-II burst reactor are 0.00032, 0.00027 respectively on the ordinary burst operation. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

On the effect of different placing ZrH moderator material on the performance of a SFR core

This study describes the development of a sodium fast reactor fuel assembly design with reduced void reactivity coefficient, achieved through the use of the ZrH moderating material. In the study the sodium void effect, as well as the major feedback coefficients are analyzed. Besides the feedback coefficients, the influence on the operational parameters like neutron flux distribution, power distribution, and burnup distribution is investigated for the different possibilities of arranging the moderating material in the fuel assembly. Additionally, the fuel cycle parameters - breeding and minor actinide production - are analyzed. For a first evaluation of the behavior during transients the influence of temperature changes in the ZrH is studied. (authors)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Summary of the Advanced Reactor Design Criteria (ARDC) Phase 2 Activities

This report provides an end-of-year summary reflecting the progress and status of proposed regulatory design criteria for advanced non-LWR designs in accordance with the Level 3 milestone in M3AT-15IN2001017 in work package AT-15IN200101. These criteria have been designated as ARDC, and they provide guidance to future applicants for addressing the GDC that are currently applied specifically to LWR designs. The report provides a summary of Phase 2 activities related to the various tasks associated with ARDC development and the subsequent development of example adaptations of ARDC for Sodium Fast Reactor (SFR) and modular High Temperature Gas-cooled Reactor (HTGR) designs.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Proven Uranium Recovery Solutions for the Nuclear Fuel Manufacturing Market - 16060

During the Nuclear Fuel Manufacturing process a number of by-products and residues are generated from various sources. In recent years, Westinghouse has characterised and processed around 50,000 drums of residue comprising of numerous different types generated over 60 years from the manufacture of numerous types of fuel for greater than 50 reactors. These include, AGR, Magnox (uranium metal fuel), PWR, fast reactors and various test reactors. Different organisations have different definitions and names for each of these categories but essentially they fall into one of the following categories: Clean Scrap (U{sub 3}O{sub 8}, UO{sub 2}, UO{sub 3}, UF{sub 4}, powders, pellets), Dirty Scrap (U{sub 3}O{sub 8}, UO{sub 2}, UO{sub 3}, UF{sub 4}, powders, pellets), Gd Contaminated Scrap (U{sub 3}O{sub 8}, UO{sub 2}, powders, pellets), Ash, Sludge, Combustible / soft residues (e.g. ventilation filters, gloves, plastic bags), Contaminated metals (including contaminated scrap zirconium tubes), Materials arising from decommissioning. Routes have been developed across the industry for a number of the categories listed above, however in numerous examples, routes have not been established and materials have been stored creating a significant legacy. Westinghouse understands the issues regarding legacy uranic material and the financial and regulatory impact of storage. Interim storage of materials may seem like a low cost option in the short term; however ongoing costs for facilities, manpower and equipment, without a permanent and final solution can result in significant lifetime material management costs. Recovery of uranium and sending materials for safe disposal of enriched uranium residues is not easy because of the criticality risk both during processing and at a disposal site. Therefore quantities of materials than can be sent via permitted disposal routes are very limited The development of regulations often means that finding solutions is becoming more difficult. It is believed that timely resolution is ultimately the most cost effective solution. In addition, the intrinsic value of recycling this material is also high and in some cases can mitigate the cost of processing. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Development of Innovative Measurement Techniques for Fission Product Transport Quantification

This document provides the progress of a research project at Texas A&M University (TAMU), led by Idaho National Laboratory (INL), in support of the Versatile Test Reactor (VTR) program and work scope area of gas-cooled fast reactors. The VTR TAMU INL project started in October 2018. The document includes the main objectives of the project, scaling analysis applied to the experimental facilities, experimental methodology including instrumentation and techniques applied, and up-to-date results from the experimental and numerical studies.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Evaluation on double-wall-tube residual stress distribution of sodium-heated steam generator by neutron diffraction and numerical analysis

A double-wall-tube is nominated for the steam generator heat transfer tube of future sodium fast reactors (SFRs) in Japan, to decrease the possibility of sodium/water reaction. The double-wall-tube consists of an inner tube and an outer tube, and they are mechanically contacted to keep the heat transfer of the interface between the inner and outer tubes by their residual stress. During long term SG operation, the contact stress at the interface gradually falls down due to stress relaxation. This phenomenon might increase the thermal resistance of the interface and degrade the tube heat transfer performance. The contact stress relaxation can be predicted by numerical analysis, and the analysis requires the data of the initial residual stress distributions in the tubes. However, unclear initial residual stress distributions prevent precious relaxation evaluation. In order to resolve this issue, a neutron diffraction method was employed to reveal the tri-axial (radius, hoop and longitudinal) initial residual stress distributions in the double-wall-tube. Strain gauges also were used to evaluate the contact stress. The measurement results were analyzed using a JAEA's structural computer code to determine the initial residual stress distributions. Based on the stress distributions, the structural computer code has predicted the transition of the relaxation and the decrease of the contact stress. The radial and longitudinal temperature distributions in the tubes were input to the structural analysis model. Since the radial thermal expansion difference between the inner (colder) and outer (hotter) tube reduces the contact stress and the tube inside steam pressure contributes to increasing it, the analytical model also took these effects into consideration. It has been conduced that the inner and outer tubes are contacted with sufficient stresses during the plant life time, and that effective heat transfer degradation dose not occur in the double-wall-tube SG. (authors)

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Nuclear data uncertainty propagation applied to the versatile test reactor conceptual design

We report the Versatile Test Reactor (VTR) currently under development is a 300 MWth sodium-cooled fast reactor (SFR) fueled with ternary metal alloy fuel, which aims to accelerate the testing of advanced nuclear fuels, materials, instrumentation, and sensors in high flux environments that are necessary to license the next generation of advanced reactor concepts. To support the VTR design process, uncertainties associated with the nuclear data has been propagated through the reactor core neutronics calculation to global parameters of interest, such as the core multiplication factor, kinetic parameters, and various reactivity feedback coefficients, following the sensitivity based uncertainty propagation approach. By folding the sensitivity coefficients, separately computed by the generalized perturbation theory code PERSENT and Monte Carlo code Serpent 2, with the variance-covariance matrices from COMMARA-2.0, we obtain the reaction-wise, isotope-wise, and overall uncertainties for each response of interest due to nuclear data uncertainty. With Serpent 2, the statistical error of the uncertainty is obtained by propagating the statistical error of the sensitivity coefficients through the same process using a newly developed uncertainty propagation method. From both codes, the overall top uncertainty contributors are found to be the cross section of Fe-56 elastic scattering, Na-23 elastic scattering, and U 238 inelastic scattering. The large contributions of the Fe-56 elastic scattering cross sections to global parameters are due to its relatively large relative uncertainty of 5–10% in nuclear data and the large volume of Fe-containing reflector assemblies in the fairly compact VTR core design. Both codes agreed well for the overall uncertainty estimates of all responses of interest, except the delayed neutron fraction, prompt neutron generation time, and the coolant density feedback coefficient, where Serpent 2 yielded a much larger value than PERSENT due to the large statistical error of sensitivity coefficients. The calculated uncertainties are also compared to those associated with other SFR cores. Another outcome of this study is a variance-covariance matrix of reactivity coefficients, which can be used in the subsequent uncertainty propagation to the system level to investigate the impact of identified uncertainties on system responses in the safety analysis.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Numerical Simulation of Twin Jets using LES with the Nek5000 Code

The twin jet activity, a joint effort between Texas A and M University, University of Tennessee - Knoxville, and Argonne National Laboratory, is being used to analyze the performance of various computational fluid dynamics (CFD) code packages. The twin jet water facility (TJWF) is based off a semi-classical problem of combining planar turbulent jets in a large free-shear environment or enclosure. The problem is similar to physics seen in advanced reactor designs such as in the large upper plena of a sodium fast reactor. Utilizing the experimental data sets created using laser Doppler velocimetry (LDV) and particle image velocimetry (PIV), the Nek5000 code, among others, is qualitatively compared to the experimental work. This effort is a starting point for determining the appropriate simulation techniques needed for resolving the twin jet physics.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

A Summary of the Department of Energy’s Advanced Demonstration and Test Reactor Options Study

An assessment of advanced reactor technology options was conducted to provide a sound comparative technical context for future decisions by the U.S. Department of Energy (DOE) concerning these technologies. Strategic objectives were established that span a wide variety of important missions, and advanced reactor technology needs were identified based on recent DOE and international studies. A broad team of stakeholders from industry, academia, and government was assembled to develop a comprehensive set of goals, criteria, and metrics to evaluate advanced irradiation test and demonstration reactor concepts. Point designs of a select number of concepts were commissioned to provide a deeper technical basis for evaluation. The technology options were compared on the bases of technical readiness and the ability to meet the different strategic objectives. Using the study's evaluation criteria and metrics, an independent group of experts from industry, universities, and national laboratories scored each of the point designs. Pathways to deployment for concepts of varying technical maturities were estimated for the different demonstration systems with regard to cost, schedule, and possible licensing approaches. This study also presents the trade-offs that exist among the different irradiation test reactor options in terms of the ability to conduct irradiations in support of advanced reactor research and development and to serve potential secondary missions. The main findings of the study indicate the following: (1) for industrial process heat supply, a high-temperature gas-cooled reactor is the best choice because of the high outlet temperature of the reactor and its strong passive and inherent safety characteristics; (2) for resource utilization and waste management, a sodium-cooled fast reactor (SFR) is best because of the use of a fast flux to destroy actinides; (3) to realize the advantages of a promising but less-mature technology, a fluoride salt-cooled high-temperature reactor and a lead-cooled fast reactor fare about the same; (4) for fulfilling the needs of a materials test reactor, a SFR is considered best because of its ability to produce high fast flux, incorporate test loops, and provide additional large volumes for testing.

Advanced reactors↗