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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 847 records · Page 47
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DOE OSTI2019

Efficient Quaternary Organic Solar Cells with Parallel‐Alloy Morphology

Abstract Two compatible donors (PBDB‐T and PTB7‐Th) and two miscible acceptors (ITIC and FOIC) are employed to deliver a parallel‐alloy morphology model in non‐fullerene‐based quaternary organic solar cells. PBDB‐T and PTB7‐Th form a parallel link with a slight adjustment of molecular packing into enhanced face‐on crystallites while ITIC disperses into discontinuous FOIC microcrystal regions to form continuous and ordered alloy‐like acceptor phases. Characterization of blend morphology highlights the parallel‐alloy model—enabled by the introduction of PBDB‐T and ITIC, which contributes to improved molecular packing and reduced domain size resulting in efficient charge generation and consistent transport channels. This successful parallel‐alloy quaternary blend morphology demonstrates an enhanced optical absorption, optimized domain size, and nanostructures toward simultaneous improvement in charge transfer and transport. Therefore, a power conversion efficiency of 12.52% is realized for a quaternary device which is 6% higher than the ternary device (PBDB‐T:PTB7‐Th:FOIC) and 12% higher than the binary device (PTB7‐Th:FOIC). Domination of quaternary devices over ternary and binary blends, which is another feasible way to realize highly efficient devices through further investigation of quaternary OSCs, is presented.

Bi, Zhaozhao↗
DOE OSTI2010

VLBI OBSERVATIONS OF THE TYPE I b/c SUPERNOVA 2009bb

We report on VLBI as well as Very Large Array radio observations of the Type I b/c supernova 2009bb. The high radio luminosity of this supernova seems to require relativistic outflow, implying that the early radio emission was 'engine-driven', that is, driven by collimated outflow from a compact object, even though no gamma-ray emission was seen. The radio light curve shows a general decline, with a 'bump' near t = 52 d, seen most prominently at 5 GHz. The light-curve bump could be either engine-driven or it might represent the turn-on of the normal radio emission from a supernova, driven by interaction with the circumstellar material rather than by the engine. We undertook VLBI observations to resolve SN 2009bb's relativistic outflow. Our observations constrain the angular outer radius at an age of 85 d to be <0.64 mas, corresponding to <4 x 10{sup 17} cm and an average apparent expansion speed of <1.74 c. This result is consistent with the moderately relativistic ejecta speeds implied by the radio luminosity and spectrum.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2011

NON-RELATIVISTIC RADIATION-MEDIATED SHOCK BREAKOUTS. I. EXACT BOLOMETRIC PLANAR BREAKOUT SOLUTIONS

The problem of a non-steady planar radiation-mediated shock (RMS) breaking out from a surface with a power-law density profile, {rho}{proportional_to}x{sup n} , is numerically solved in the approximation of diffusion with constant opacity. For an appropriate choice of time, length, and energy scales, determined by the breakout opacity, velocity, and density, the solution is universal, i.e., depends only on the density power-law index n. The resulting luminosity depends weakly on the value of n. An approximate analytic solution, based on the self-similar hydrodynamic solutions and on the steady RMS solutions, is constructed and shown to agree with the numerical solutions as long as the shock is far from the surface, {tau} >> c/v{sub sh}. Approximate analytic expressions, calibrated based on the exact solutions, are provided, which describe the escaping luminosity as a function of time. These results can be used to calculate the bolometric properties of the bursts of radiation produced during supernova shock breakouts. For completeness, we also use the exact breakout solutions to provide an analytic approximation for the maximum surface temperature for fast (v{sub sh} {approx}> 0.1) non-thermal breakouts and show that it is a few times smaller than inferred based on steady state RMS solutions.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2011

COSMOLOGICAL-MODEL-INDEPENDENT TESTS FOR THE DISTANCE-DUALITY RELATION FROM GALAXY CLUSTERS AND TYPE Ia SUPERNOVA

We perform a cosmological-model-independent test for the distance-duality (DD) relation {eta}(z) = D{sub L} (z)(1 + z){sup -2}/D{sub A} (z), where D{sub L} and D{sub A} are the luminosity distance and angular diameter distance, respectively, with a combination of observational data for D{sub L} taken from the latest Union2 SNe Ia and that for D{sub A} provided by two galaxy cluster samples compiled by De Filippis et al. and Bonamente et al. Two parameterizations for {eta}(z), i.e., {eta}(z) = 1 + {eta}{sub 0} z and {eta}(z) = 1 + {eta}{sub 0} z/(1 + z), are used. We find that the DD relation can be accommodated at 1{sigma} confidence level (CL) for the De Filippis et al. sample and at 3{sigma} CL for the Bonamente et al. sample. We also examine the DD relation by postulating two more general parameterizations: {eta}(z) = {eta}{sub 0} + {eta}{sub 1} z and {eta}(z) = {eta}{sub 0} + {eta}{sub 1} z/(1 + z), and find that the DD relation is compatible with the results from the De Filippis et al. and the Bonamente et al. samples at 1{sigma} and 2{sigma} CLs, respectively. Thus, we conclude that the DD relation is compatible with present observations.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2011

ON THE MASS-LOSS RATE OF MASSIVE STARS IN THE LOW-METALLICITY GALAXIES IC 1613, WLM, AND NGC 3109

We present a spectroscopic analysis of Very Large Telescope/X-Shooter observations of six O-type stars in the low-metallicity (Z {approx} 1/7 Z {sub sun}) galaxies IC 1613, WLM, and NGC 3109. The stellar and wind parameters of these sources allow us, for the first time, to probe the mass loss versus metallicity dependence of stellar winds at metallicities below that of the Small Magellanic Cloud (at Z {approx} 1/5 Z {sub sun}) by means of a modified wind momentum versus luminosity diagram. The wind strengths that we obtain for the objects in WLM and NGC 3109 are unexpectedly high and do not agree with theoretical predictions. The objects in IC 1613 tend toward a higher than expected mass-loss rate, but remain consistent with predictions within their error bars. We discuss potential systematic uncertainties in the mass-loss determinations to explain our results. However, if further scrutinization of these findings point towards an intrinsic cause for this unexpected sub-SMC mass-loss behavior, implications would include a higher than anticipated number of Wolf-Rayet stars and Ib/Ic supernovae in low-metallicity environments, but a reduced number of long-duration gamma-ray bursts produced through a single-star evolutionary channel.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2024

Probing the origin of the two-component structure of broad-line region by reverberation mapping of an extremely variable quasar

ABSTRACT The physical origins of quasar components, such as the broad-line region (BLR) and dust torus, remain under debate. To gain insights into them, we focused on changing-state quasars (CSQs) which provide a unique perspective through structural changes associated with accretion disc state transitions. We targeted SDSS J125809.31+351943.0, an extremely variable CSQ, to study its central core structure and kinematics. We conducted reverberation mapping with optical spectroscopy to explore the structure of the BLR and estimate the black hole mass. The results from Hβ reverberation mapping indicated a black hole mass of $10^{9.64^{+0.11}_{-0.20}}\rm {M_\odot }$. Additionally, we analysed variations in the optical to X-ray spectral indices, αox, before and after the state transition, to investigate the accretion disc. These variations in αox and the Eddington ratio (from 0.4 per cent to 2.4 per cent) exhibitied behaviour similar to state transitions observed in X-ray binary systems. Spectral analysis of Hβ revealed a predominantly double-peaked profile during dim periods, transitioning to include a single-peaked component as the quasar brightened, suggesting that Hβ contains a mixture of two components. Each of these components has its distinct characteristics: the first is a double-peaked profile that remains stable despite changes in the accretion rate, while the second is a variable single-peaked profile. Using time-lags from reverberation mapping, we estimated the spatial relationships between these BLR components, the accretion disc, and the dust torus. Our results suggest that the BLR consists of two distinct components, each differing in location and origin.

Nagoshi, Shumpei (ORCID:0000000326504322)↗
DOE OSTI2018

Absolute Dimensions and Evolutionary Status of the Semi-detached Algol W Ursae Minoris

Double-lined eclipsing binaries allow accurate and direct determination of fundamental parameters such as mass and radius for each component, and they provide important constraints on the stellar structure and evolution models. In this study, we aim to determine a unique set of binary parameters for the Algol system W UMi and to examine its evolutionary status. New high-resolution time-series spectroscopic observations were carried out during 14 nights from 2008 April to 2011 March, and a total of 37 spectra were obtained using the Bohyunsan Optical Echelle Spectrograph. We measured the radial velocities (RVs) for both components, and the effective temperature of the primary star was found to be T {sub eff,1} = 9310 ± 90 K by a comparison of the observed spectra and the Kurucz models. The physical parameters of W UMi were derived by an analysis of our RV data together with the multi-band light curves of Devinney et al. The individual masses, radii, and luminosities of both components are M {sub 1} = 3.68 ± 0.10 M {sub ⊙} and M {sub 2} = 1.47 ± 0.04 M {sub ⊙}, R {sub 1} = 3.88 ± 0.03 R {sub ⊙} and R {sub 2} = 3.13 ± 0.03 R {sub ⊙}, and L {sub 1} = 102 ± 1 L {sub ⊙} and L {sub 2} = 7.3 ± 0.1 L {sub ⊙}, respectively. A comparison of these parameters with theoretical stellar models showed that the primary component lies in the main-sequence band, while the less massive secondary is noticeably evolved. The results indicate that the initially more massive star became the present secondary by losing most of its own mass via mass transfer to the companion (present primary).

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

Synthesis of Bi{sub 2}S{sub 3} with different sulfur content by conventional high temperature solid state solvothermal route

Bismuth sulfide (Bi{sub 2}S{sub 3}) is a binary chalcogenide compound material belonging to V-VI group of semiconductors. Because of its direct band gap of 1.3 eV and high figure of merit (ZT) value, it is widely used as a thermo electronic-cooling material based on the Peltier effect. The electrical and optical property of Bi{sub 2}S{sub 3} material is strongly dependent on stoichiometric composition, defect chemistry and structure. In this study, we have synthesized Bi{sub 2}S{sub x} (x = 3.15, 3.30, 3.45) compound material with different sulfur content by conventional high temperature solid state solvothermal reaction of bismuth and sulfur. X-ray diffraction (XRD), scanning electron microscopy (SEM) and energy dispersive x-ray spectroscopy (EDXS) analysis of synthesized compound materials were carried out to observe crystallinity, surface morphology and composition of elements in the compound. The optical analysis revealed that energy band gap decreases with increase of sulfur content.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2014

A BLUE POINT SOURCE AT THE LOCATION OF SUPERNOVA 2011DH

We present Hubble Space Telescope (HST) observations of the field of the Type IIb supernova (SN) 2011dh in M51 performed at ≈1161 rest-frame days after explosion using the Wide Field Camera 3 and near-UV filters F225W and F336W. A star-like object is detected in both bands and the photometry indicates it has negative (F225W – F336W) color. The observed object is compatible with the companion of the now-vanished yellow supergiant progenitor predicted in interacting binary models. We consider it unlikely that the SN is undergoing strong interaction and thus estimate that it makes a small contribution to the observed flux. The possibilities of having detected an unresolved light echo or an unrelated object are briefly discussed and judged unlikely. Adopting a possible range of extinction by dust, we constrain parameters of the proposed binary system. In particular, the efficiency of mass accretion onto the binary companion must be below 50%, if no significant extinction is produced by newly formed dust. Further multiband observations are required in order to confirm the identification of the object as the companion star. If confirmed, the companion star would already be dominant in the UV-optical regime, so it would readily provide a unique opportunity to perform a detailed study of its properties.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2019

Ground-based Spectroscopy of the Exoplanet XO-2b Using a Systematic Wavelength Calibration

Exoplanets orbiting close to their host star are expected to support a large ionosphere, which extends to larger pressures than witnessed in our solar system. These ionospheres can be investigated with ground-based transit observations of the optical signatures of alkali metals, which are the source of the ions. However, most ground-based transit spectra do not systematically resolve the wings of the features and continuum, as needed to constrain the alkali abundances. Here we present new observations and analyses of optical transit spectra that cover the Na doublet in the atmosphere of the exoplanet XO-2b. To assess the consistency of our results, observations were obtained from two separate platforms: Gemini/GMOS and Mayall/KOSMOS. To mitigate the systematic errors, we chose XO-2, because it has a binary companion of the same brightness and stellar type, which provides an ideal reference star to model Earth’s atmospheric effects. We find that interpretation of the data is highly sensitive to time-varying translations along the detector, which change according to wavelength and differ between the target and reference star. It was necessary to employ a time-dependent cross-correlation to align our wavelength bins and correct for atmospheric differential refraction. This approach allows us to resolve the wings of the Na line across five wavelength bins at a resolution of ∼1.6 nm and limit the abundance of Na. We obtain consistent results from each telescope with an Na amplitude of 521 ± 161 and 403 ± 186 ppm for GMOS and KOSMOS, respectively. The results are analyzed with a radiative transfer model that includes the effects of ionization. The data are consistent with a clear atmosphere between ∼1 and 100 mbar that establishes a lower limit on Na at 0.4{sub −0.3}{sup +2} ppm ([Na/H] = −0.64{sub −0.6}{sup +0.78}), consistent with solar. However, we cannot rule out the presence of clouds at ∼10 mbar that allow for higher Na abundances, which would be consistent with the stellar metallicity measured for the host star ([Na/H] = 0.485 ± 0.043).

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2017

A gravitational-wave standard siren measurement of the Hubble constant

On 17 August 2017, the Advanced LIGO and Virgo detectors observed the gravitational-wave event GW170817—a strong signal from the merger of a binary neutron-star system. Less than two seconds after the merger, a γ-ray burst (GRB 170817A) was detected within a region of the sky consistent with the LIGO–Virgo-derived location of the gravitational-wave source. This sky region was subsequently observed by optical astronomy facilities, resulting in the identificationof an optical transient signal within about ten arcseconds of the galaxy NGC 4993. This detection of GW170817 in both gravitational waves and electromagnetic waves represents the first ‘multi-messenger’ astronomical observation. Such observations enable GW170817 to be used as a ‘standard siren’ (meaning that the absolute distance to the source can be determined directly from the gravitational-wave measurements) to measure the Hubble constant. This quantity represents the local expansion rate of the Universe, sets the overall scale of the Universe and is of fundamental importance to cosmology. Here we report a measurement of the Hubble constant that combines the distance to the source inferred purely from the gravitational-wave signal with the recession velocity inferred from measurements of the redshift using the electromagnetic data. In contrast to previous measurements, ours does not require the use of a cosmic ‘distance ladder’: the gravitational-wave analysis can be used to estimate the luminosity distance out to cosmological scales directly, without the use of intermediate astronomical distance measurements. We determine the Hubble constant to be about 70 kilometres per second per megaparsec. Furthermore, this value is consistent with existing measurements, while being completely independent of them. Additional standard siren measurements from future gravitational-wave sources will enable the Hubble constant to be constrained to high precision.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

Spectral anomalies of the effect of light-induced drift of caesium atoms caused by the velocity dependence of transport collision frequencies

The spectral features of the light-induced drift (LID) velocity of caesium atoms in inert buffer gases are studied theoretically. A strong temperature dependence of the spectral LID line shape of Cs atoms in Ar or Kr atmosphere in the vicinity of T ∼ 1000 K is predicted. It is shown that the anomalous LID of Cs atoms in binary buffer mixtures of two different inert gases can be observed at virtually any (including ambient) temperature, depending on the content of the components in these mixtures. The results obtained make it possible to precisely test the interatomic interaction potentials in the experiments on the anomalous LID. (quantum optics)

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2015

Liquid crystal mesophases beyond commensurate four-layer periodicity

For more than one decade, SMC* d4 , SmC* d3 , and SmC* A were the only three confirmed commensurate SmC* variant phases with periodicities less than or equal four layers. In 2006, employing ellipsometry and resonant X-ray diffraction (RXRD), our research team first discovered a new liquid crystal mesophase having a six-layer periodicity in one ternary mixture which includes one sulfur-containing compound. From our ellipsometric results, this phase showed antiferroelectric-like optical response. This novel discovery inspired renewed interest to search for liquid crystal mesophases with commensurate periodicities greater than four layers. Soon after, another mesophase having a six-layer structure and showing a ferrielectric-like dielectric response, instead, was uncovered by RXRD measurements on a different binary mixture which has one bromine-containing compound. Meanwhile mesophases having a 5-, 8-, 12- or 15-layer periodicity were reported. However, numerous questions remain to be addressed associated with these unusual reported phases. Theoretical models giving rise to mesophases with periodicities greater than four layers have been developed; but, to date, none of them have provided satisfactory explanations of all the physical phenomena related to the mesophases exhibiting a six-layer structure. Moreover, the question “what is the source of long-range interactions between liquid-like smectic layers, which are responsible for establishing mesophases with long periodicities and mean-field behavior of the smectic-A–smectic-C transition?” remains unanswered for more than three decades.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2011

EFFECTS OF ROTATION ON STOCHASTICITY OF GRAVITATIONAL WAVES IN THE NONLINEAR PHASE OF CORE-COLLAPSE SUPERNOVAE

By performing three-dimensional (3D) simulations that demonstrate the neutrino-driven core-collapse supernovae aided by the standing accretion shock instability (SASI), we study how the spiral modes of the SASI can impact the properties of the gravitational-wave (GW) emission. To see the effects of rotation in the nonlinear postbounce phase, we give a uniform rotation on the flow advecting from the outer boundary of the iron core, the specific angular momentum of which is assumed to agree with recent stellar evolution models. We compute fifteen 3D models in which the initial angular momentum and the input neutrino luminosities from the protoneutron star are changed in a systematic manner. By performing a ray-tracing analysis, we accurately estimate the GW amplitudes generated by anisotropic neutrino emission. Our results show that the gravitational waveforms from neutrinos in models that include rotation exhibit a common feature; otherwise, they vary much more stochastically in the absence of rotation. The breaking of the stochasticity stems from the excess of the neutrino emission parallel to the spin axis. This is because the compression of matter is more enhanced in the vicinity of the equatorial plane due to the growth of the spiral SASI modes, leading to the formation of the spiral flows circulating around the spin axis with higher temperatures. We point out that recently proposed future space interferometers like Fabry-Perot-type DECIGO would permit the detection of these signals for a Galactic supernova.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2019

Lessons from the light of a neutron star merger

The discovery by Advanced LIGO/Virgo of gravitational waves from the binary neutron star merger GW170817, and subsequently by astronomers of transient emission across the electromagnetic spectrum, has initiated a new era of multi-messenger gravitational wave astronomy. Here I summarize the electromagnetic discoveries in the context of theoretical counterpart models and present personal views on the major take-away lessons and outstanding new questions from this watershed event, focused on the implications for nuclear physics. The luminosity and colors of the early optical emission discovered within a day of the merger agree well with predictions for “kilonova” emission, powered by the radioactive decay of light r-process nuclei (atomic mass number A≲140). The transition of the spectral energy distribution to near-infrared wavelengths on timescales of days indicates that inner portions of the ejecta contain heavy r-process nuclei with high UV/optical opacity due to the presence of at least some lanthanide elements (A≳140). The “blue” and “red” ejecta components likely possess distinct origins (e.g. dynamical ejecta, magnetar-powered wind, or accretion disk outflow), with implications for the merger process (e.g. the lifetime of the remnant prior to black hole formation) and fundamental properties of neutron stars. I outline the predicted diversity in the electromagnetic emission of future mergers−observed with different ingoing binary masses and/or viewing angles−discovered in the years ahead as LIGO/Virgo reach design sensitivity.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

TRACING THE REVERBERATION LAG IN THE HARD STATE OF BLACK HOLE X-RAY BINARIES

We report results obtained from a systematic analysis of X-ray lags in a sample of black hole X-ray binaries, with the aim of assessing the presence of reverberation lags and studying their evolution during outburst. We used XMM-Newton and simultaneous Rossi X-ray Timing Explorer (RXTE) observations to obtain broadband energy coverage of both the disk and the hard X-ray Comptonization components. In most cases the detection of reverberation lags is hampered by low levels of variability-power signal-to-noise ratio (typically when the source is in a soft state) and/or short exposure times. The most detailed study was possible for GX 339-4 in the hard state, which allowed us to characterize the evolution of X-ray lags as a function of luminosity in a single source. Over all the sampled frequencies (∼0.05–9 Hz), we observe the hard lags intrinsic to the power-law component, already well known from previous RXTE studies. The XMM-Newton soft X-ray response allows us to detail the disk variability. At low frequencies (long timescales) the disk component always leads the power-law component. On the other hand, a soft reverberation lag (ascribable to thermal reprocessing) is always detected at high frequencies (short timescales). The intrinsic amplitude of the reverberation lag decreases as the source luminosity and the disk fraction increase. This suggests that the distance between the X-ray source and the region of the optically thick disk where reprocessing occurs gradually decreases as GX 339-4 rises in luminosity through the hard state, possibly as a consequence of reduced disk truncation.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2013

BRIGHT BROADBAND AFTERGLOWS OF GRAVITATIONAL WAVE BURSTS FROM MERGERS OF BINARY NEUTRON STARS

If double neutron star mergers leave behind a massive magnetar rather than a black hole, then a bright early afterglow can follow the gravitational wave burst (GWB) even if there is no short gamma-ray burst (SGRB)-GWB association or if there is an association but the SGRB does not beam toward Earth. Besides directly dissipating the proto-magnetar wind, as suggested by Zhang, here we suggest that the magnetar wind could push the ejecta launched during the merger process and, under certain conditions, would reach a relativistic speed. Such a magnetar-powered ejecta, when interacting with the ambient medium, would develop a bright broadband afterglow due to synchrotron radiation. We study this physical scenario in detail and present the predicted X-ray, optical, and radio light curves for a range of magnetar and ejecta parameters. We show that the X-ray and optical light curves usually peak around the magnetar spin-down timescale ({approx}10{sup 3}-10{sup 5} s), reaching brightnesses readily detectable by wide-field X-ray and optical telescopes, and remain detectable for an extended period. The radio afterglow peaks later, but is much brighter than the case without a magnetar energy injection. Therefore, such bright broadband afterglows, if detected and combined with GWBs in the future, would be a probe of massive millisecond magnetars and stiff equations of state for nuclear matter.

79 ASTRONOMY AND ASTROPHYSICS↗