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Final Design for Additional Thermal/Epithermal eXperiments (TEX) with Sodium Chloride Absorbers to Provide Validation Benchmarks for TerraPower

The first set of Thermal/Epithermal eXperiments (TEX) with chlorine absorbers (TEX-Cl) were executed in Q4FY24 and are in the process of being benchmarked for the ICSBEP. TEX-Cl builds upon the TEX-HEU baseline cases that were published in the 2022 International Criticality Safety Benchmark Evaluation Project (ICSBEP) Handbook. TEX-HEU, like TEX-Pu, was designed to be modular to allow for the incorporation of various absorbers and reflectors to test nuclear data and application case needs. For example, TEX-HEU with hafnium (TEX-Hf) utilizes hafnium plates as both absorbers and reflectors, depending on the tested configuration. A second set of chlorine experiments, dubbed More TEX-Cl, are laid out in this report to meet the needs of TerraPower for chlorine validation for their Molten Chloride Fast Reactor (MCFR) systems. TerraPower’s Molten Chloride Reactor Experiment (MCRE) and MCFR are fast molten salt reactors that utilize sodium chloride (NaCl) salt eutectics as the fuel and coolant. The MCRE eutectic is a mixture of NaCl and uranium trichloride (UCl 3 ). An abundant need for chlorine absorption validation has been expressed by multiple members of the community, including Y-12 (whose needs were addressed with the first set of experiments), LANL (whose needs were addressed with the Chlorine Worth Study (CWS)), TerraPower, institute de radioprotection et de sûreté nucléaire (IRSN), Savannah River Nuclear Solutions (SNRS), and others. Of the members who have expressed interest in this validation, most are interested in the fast neutron energy region, where the 35 Cl(n,p) reaction is most prominent. New 35 Cl(n,p) differential cross section measurements performed by LANL at LANCSE show substantial changes to the cross sections (Figure 1) and may be validated through these experiments as some configurations are optimally sensitive to this cross section.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Hydrochlorination of Uranium Dioxide in a Molten Salt Mixture- Phase 2: Sparged Benchtop Reaction Vessel Experiment

In 2023, Metatomic® Inc., a South Carolina based company, was awarded a Gateway for Advanced Innovation in Nuclear (GAIN) research voucher for a proposed series of experiments aimed at demonstrating the viability of a spent nuclear fuel (SNF) recycling process patented by Metatomic Inc. For the GAIN voucher, Metatomic Inc. selected Savannah River National Laboratory (SRNL) as a partner in executing the proposed proof-of-concept experiments. This report outlines the proof-of-concept experiments performed by SRNL for Metatomic Inc. during Phase 2 (of 2) experimentation. Though Phase 1 provided evidence of successful hydrochlorination, Phase 2 highlighted the nuances and challenges associated with scaling the reaction. The target UCl 4 species generated by the hydrochlorination of UO 2 generates water, which consumes UCl 4 . Compared to the single datapoint obtained at the end of the Phase 1 experiments, data collected at multiple timepoints during Phase 2 experiments indicated a presumed maximum percent conversion of 23% for this system that is likely influenced by water generation. Engineering improvements might be able to increase the percent conversion, but not likely to the degree needed for successful implementation of the technology. Moisture also presents an issue for the Hastelloy C276 reaction vessel. Eventually, corrosion will compromise the integrity of the reaction vessel, and the corrosion products could potentially affect the hydrochlorination chemistry. The presence of corrosion products, which were not produced in the Phase 1 alumina crucible, can and have created challenges when analyzing samples.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Design and test of a special magnet for the Mu2e experiment

The Mu2e experiment (Muon-to-Electron Conversion Experiment) is looking for evidence that a muon can change into an electron without the emission of neutrinos. The experiment will search for the charged-lepton flavor violating (CLFV) neutrino-less conversion of a negative muon into an electron in the field of a nucleus. The conversion process results in a monochromatic electron with an energy of 104.97 MeV, slightly below the muon rest mass. The goal of the experiment is to improve the previous upper limit by four orders of magnitude and reach a SES (single event sensitivity) of 3 × 10 -17 on the conversion rate, a 90% CL of 8 × 10 -17 , and a 5σ discovery reach at 2 × 10 -16 . The experiment will use an intense pulsed negative muon beam, which is essential to reducing backgrounds. The other essential element is a sophisticated magnetic system composed of three consecutive solenoids (figure 1) that form the muon beam.

43 PARTICLE ACCELERATORS↗

Measuring the muon precession frequency in the E989 Fermilab g-2 experiment

Since more than 50 years the electron and muon anomalies, $a_e$ and $a_\mu$, defined in terms of the gyromagnetic factor $g_i$ for particle $i$ as $a_i=(g_i-2)/2$, have provided a deep insight into the quantum structure of elementary particles.They have been, and continue to be, a milestone for the development of the Standard Model of Particle Physics against which all new theories have to be compared.For almost 20 years, the experimental value of $a_\mu$ has shown a tantalizing discrepancy of more than $3 \sigma$ from the theoretical prediction making it mandatory for experimentalists to improve the current result, dominated by the E821 experiment at BNL\cite{BNL}. The Muon $g-2$ E989 experiment at Fermilab will use the same storage ring technique used at BNL, and previously in the CERN-III experiment, with the goal of decreasing by a factor of 4 the current error on $a_\mu$, which will allow for a finer comparison with the theoretical prediction. E989 started collecting data in winter 2018 accumulating, in the period April-July 2018 (Run1) almost twice the statistics of the previous experiment (before application of data quality cuts). In this document, the experiment will be briefly described, underlying the improvements which will allow to reduce the systematic error, and some preliminary result will be shown.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Relationship between Telework Experience and Presenteeism during COVID-19 Pandemic, United States, March–November 2020

Persons with COVID-19–like illnesses are advised to stay home to reduce the spread of SARS-CoV-2. We assessed relationships between telework experience and COVID-19 illness with work attendance when ill. Adults experiencing fever, cough, or loss of taste or smell who sought healthcare or COVID-19 testing in the United States during March–November 2020 were enrolled. Adults with telework experience before illness were more likely to work at all (onsite or remotely) during illness (87.8%) than those with no telework experience (49.9%) (adjusted odds ratio 5.48, 95% CI 3.40–8.83). COVID-19 case-patients were less likely to work onsite (22.1%) than were persons with other acute respiratory illnesses (37.3%) (adjusted odds ratio 0.36, 95% CI 0.24–0.53). Among COVID-19 case-patients with telework experience, only 6.5% worked onsite during illness. Telework experience before illness gave mildly ill workers the option to work and improved compliance with public health recommendations to stay home during illness.

60 APPLIED LIFE SCIENCES↗

HighNESS conceptual design report: Volume II. The NNBAR experiment.

A key aim of the HighNESS project for the European Spallation Source is to enable cutting-edge particle physics experiments. This volume presents a conceptual design report for the NNBAR experiment. NNBAR would exploit a new cold lower moderator to make the first search in over thirty years for free neutrons converting to anti-neutrons. The observation of such a baryon-number-violating signature would be of fundamental significance and tackle open questions in modern physics, including the origin of the matter-antimatter asymmetry. This report shows the design of the beamline, supermirror focusing system, magnetic and radiation shielding, and anti-neutron detector necessary for the experiment. A range of simulation programs are employed to quantify the performance of the experiment and show how background can be suppressed. For a search with full background suppression, a sensitivity improvement of three orders of magnitude is expected, as compared with the previous search. Civil engineering studies for the NNBAR beamline are also shown, as is a costing model for the experiment.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

A Possible Neutron-Antineutron Oscillation Experiment at PF1B at the Institut Laue Langevin

We consider a possible neutron–antineutron ($n-\overline{n}$) oscillation experiment at the PF1B instrument at Institut Laue Langevin. It can improve the best existing constraint on the transition rate and also allow the testing of the methods and instrumentation which would be needed for a later larger-scale experiment at ESS. The main gain factors over the most competitive experiment, performed earlier at PF1 instrument at ILL, are: a more intense neutron beam and a new operating mode based on coherent n and $\overline{n}$ mirror reflections. The installation of such an experiment would need a temporary replacement of the existing ballistic neutron guide by a specially designed n/$\overline{n}$ guide with a gradually increasing cross section and a specially selected coating as well as the development and construction of an advanced $\overline{n}$ annihilation detector with a high efficiency and low background. The overall gain factor could reach up to an order of magnitude and depends on the chosen experiment configuration.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Opportunistic experiments to constrain aerosol effective radiative forcing

Aerosol–cloud interactions (ACIs) are considered to be the most uncertain driver of present-day radiative forcing due to human activities. The nonlinearity of cloud-state changes to aerosol perturbations make it challenging to attribute causality in observed relationships of aerosol radiative forcing. Using correlations to infer causality can be challenging when meteorological variability also drives both aerosol and cloud changes independently. Natural and anthropogenic aerosol perturbations from well-defined sources provide “opportunistic experiments” (also known as natural experiments) to investigate ACI in cases where causality may be more confidently inferred. These perturbations cover a wide range of locations and spatiotemporal scales, including point sources such as volcanic eruptions or industrial sources, plumes from biomass burning or forest fires, and tracks from individual ships or shipping corridors. We review the different experimental conditions and conduct a synthesis of the available satellite datasets and field campaigns to place these opportunistic experiments on a common footing, facilitating new insights and a clearer understanding of key uncertainties in aerosol radiative forcing. Cloud albedo perturbations are strongly sensitive to background meteorological conditions. Strong liquid water path increases due to aerosol perturbations are largely ruled out by averaging across experiments. Opportunistic experiments have significantly improved process-level understanding of ACI, but it remains unclear how reliably the relationships found can be scaled to the global level, thus demonstrating a need for deeper investigation in order to improve assessments of aerosol radiative forcing and climate change.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

An overview of cloud–radiation denial experiments for the Energy Exascale Earth System Model version 1

Abstract. The interaction between clouds and radiation is a key process within the climate system, and assessing the impacts of that interaction provides valuable insights into both the present-day climate and future projections. Many modeling experiments have been designed over the years to probe the impact of the cloud radiative effect (CRE) on the climate, including those that seek to disrupt the mean CRE effect and those that only disrupt the covariance of the CRE with the circulation. Seven such experimental designs have been added to the Energy Exascale Earth System Model version 1 (E3SMv1) of the US Department of Energy. These experiments include both the first and second iterations of the Clouds On/Off Klimate Intercomparison Experiment (COOKIE) experimental design, as well as the cloud-locking method. This paper documents the code changes necessary to implement such experiments and also provides detailed instructions for how to run them. Analyses across experiment types provide valuable insights and confirm the findings of prior studies, including the role of cloud radiative heating toward intensifying the monsoon, intensifying rain rates, and poleward expansion of the general circulation owing to cloud feedbacks.

Harrop, Bryce E. (ORCID:0000000339524525)↗

Vegetation Warming Experiment: Environmental Conditions, Utqiagvik (Barrow), Alaska, 2018

Environmental conditions measured in five warming chambers and paired ambient control plots located on the Barrow Environmental Observatory (BEO), Utqiagvik, Alaska from 16 June - 24 September, 2018. These data were recorded in support of the Zero Power Warming (ZPW) vegetation warming experiment, a series of single season vegetation warming treatments conducted over four years from 2017-2021 (no experiment in 2020). Air temperature and humidity, infrared surface (canopy) temperature, soil temperature, soil moisture, NDVI (normalized difference vegetation index), PRI (photochemical reflectance index), solar radiation and chamber venting were recorded in each chamber at 1 minute intervals. Ambient air temperature, humidity, solar radiation and uplooking PRI and NDVI were measured at a centrally located meteorology station. Vapor pressure deficit (VPD) was calculated and included in the final processed data products. Data has undergone full QA/QC and is presented as 1 minute data, and hourly and daily aggregate data products. This data package includes unprocessed raw data (*.dat files), processed data (*.csv) and metadata including a full description of sensors, calculations and processing (*.csv, *.pdf). See related NGEE-Arctic "Vegetation Warming Experiment" data packages for leaf-level gas exchange and other leaf trait data; chamber, plot and landscape phenocamera images; thaw depth, and GPS locations of chambers and ambient plots.The Next-Generation Ecosystem Experiments: Arctic (NGEE Arctic), was a 15-year research effort (2012-2027) to reduce uncertainty in Earth System Models by developing a predictive understanding of carbon-rich Arctic ecosystems and feedbacks to climate. NGEE Arctic was supported by the Department of Energy's Office of Biological and Environmental Research. The NGEE Arctic project had two field research sites: 1) located within the Arctic polygonal tundra coastal region on the Barrow Environmental Observatory (BEO) and the North Slope near Utqiagvik (Barrow), Alaska and 2) multiple areas on the discontinuous permafrost region of the Seward Peninsula north of Nome, Alaska. Through observations, experiments, and synthesis with existing datasets, NGEE Arctic provided an enhanced knowledge base for multi-scale modeling and contributed to improved process representation at global pan-Arctic scales within the Department of Energy's Earth system Model (the Energy Exascale Earth System Model, or E3SM), and specifically within the E3SM Land Model component (ELM).

54 ENVIRONMENTAL SCIENCES↗

Vegetation Warming Experiment: Environmental conditions, Utqiagvik (Barrow), Alaska, 2019

Environmental conditions measured in five warming chambers and paired ambient control plots located on the Barrow Environmental Observatory (BEO), Utqiagvik, Alaska from 19 June – 25 September, 2019. These data were recorded in support of the Zero Power Warming (ZPW) vegetation warming experiment, a series of single season vegetation warming treatments conducted over four years from 2017–2021 (no experiment in 2020). Air temperature and humidity, infrared surface (canopy) temperature, soil temperature, soil moisture, NDVI (normalized difference vegetation index), PRI (photochemical reflectance index), solar radiation and chamber venting were recorded in each chamber at 1 minute intervals. Ambient air temperature, humidity, solar radiation and uplooking PRI and NDVI were measured at a centrally located meteorology station. Vapor pressure deficit (VPD) was calculated and included in the final processed data products. Data has undergone full QA/QC and is presented as 1 minute data, and hourly and daily aggregate data products. This data package includes unprocessed raw data (*.dat files), processed data (*.csv) and metadata including a full description of sensors, calculations and processing (*.csv, *.pdf). See related NGEE-Arctic "Vegetation Warming Experiment" data packages for leaf-level gas exchange and other leaf trait data; chamber, plot and landscape phenocamera images; thaw depth, and GPS locations of chambers and ambient plots.The Next-Generation Ecosystem Experiments: Arctic (NGEE Arctic), was a 15-year research effort (2012-2027) to reduce uncertainty in Earth System Models by developing a predictive understanding of carbon-rich Arctic ecosystems and feedbacks to climate. NGEE Arctic was supported by the Department of Energy's Office of Biological and Environmental Research. The NGEE Arctic project had two field research sites: 1) located within the Arctic polygonal tundra coastal region on the Barrow Environmental Observatory (BEO) and the North Slope near Utqiagvik (Barrow), Alaska and 2) multiple areas on the discontinuous permafrost region of the Seward Peninsula north of Nome, Alaska. Through observations, experiments, and synthesis with existing datasets, NGEE Arctic provided an enhanced knowledge base for multi-scale modeling and contributed to improved process representation at global pan-Arctic scales within the Department of Energy's Earth system Model (the Energy Exascale Earth System Model, or E3SM), and specifically within the E3SM Land Model component (ELM).

54 ENVIRONMENTAL SCIENCES↗

Vegetation Warming Experiment: Environmental Conditions, Utqiagvik (Barrow), Alaska, 2017

Environmental conditions measured in five warming chambers and paired ambient control plots located on the Barrow Environmental Observatory (BEO), Utqiagvik, Alaska from 22 June - 17 September, 2017. These data were recorded in support of the Zero Power Warming (ZPW) vegetation warming experiment, a series of single season vegetation warming treatments conducted over four years from 2017-2021 (no experiment in 2020). Air temperature and humidity, infrared surface (canopy) temperature, soil temperature, soil moisture, NDVI (normalized difference vegetation index), PRI (photochemical reflectance index), solar radiation and chamber venting were recorded in each chamber at 1 minute intervals. Ambient air temperature, humidity, solar radiation and uplooking PRI and NDVI were measured at a centrally located meteorology station. Vapor pressure deficit (VPD) was calculated and included in the final processed data products. Data has undergone full QA/QC and is presented as 1 minute data, and hourly and daily aggregate data products. This data package includes unprocessed raw data (*.dat files), processed data (*.csv) and metadata including a full description of sensors, calculations and processing (*.csv, *.pdf). See related NGEE-Arctic Vegetation Warming Experiment data packages for leaf-level gas exchange and other leaf trait data; chamber, plot and landscape phenocamera images; thaw depth, and GPS locations of chambers and ambient plots. The Next-Generation Ecosystem Experiments: Arctic (NGEE Arctic), was a research effort to reduce uncertainty in Earth System Models by developing a predictive understanding of carbon-rich Arctic ecosystems and feedbacks to climate. NGEE Arctic was supported by the Department of Energy's Office of Biological and Environmental Research.The NGEE Arctic project had two field research sites: 1) located within the Arctic polygonal tundra coastal region on the Barrow Environmental Observatory (BEO) and the North Slope near Utqiagvik (Barrow), Alaska and 2) multiple areas on the discontinuous permafrost region of the Seward Peninsula north of Nome, Alaska.Through observations, experiments, and synthesis with existing datasets, NGEE Arctic provided an enhanced knowledge base for multi-scale modeling and contributed to improved process representation at global pan-Arctic scales within the Department of Energy's Earth system Model (the Energy Exascale Earth System Model, or E3SM), and specifically within the E3SM Land Model component (ELM).

54 ENVIRONMENTAL SCIENCES↗

Vegetation Warming Experiment: Environmental conditions, Utqiagvik (Barrow), Alaska, 2021

Environmental conditions measured in five warming chambers and paired ambient control plots located on the Barrow Environmental Observatory (BEO), Utqiagvik, Alaska from 19 June - 17 September, 2021. These data were recorded in support of the Zero Power Warming (ZPW) vegetation warming experiment, a series of single season vegetation warming treatments conducted over four years from 2017-2021 (no experiment in 2020). Air temperature and humidity, infrared surface (canopy) temperature, soil temperature, soil moisture, NDVI (normalized difference vegetation index), PRI (photochemical reflectance index), solar radiation and chamber venting were recorded in each chamber at 1 minute intervals. Ambient air temperature, humidity, solar radiation and uplooking PRI and NDVI were measured at a centrally located meteorology station. Vapor pressure deficit (VPD) was calculated and included in the final processed data products. Data has undergone full QA/QC and is presented as 1 minute data, and hourly and daily aggregate data products. This data package includes unprocessed raw data (*.dat files), processed data (*.csv) and metadata including a full description of sensors, calculations and processing (*.csv, *.pdf). See related NGEE-Arctic "Vegetation Warming Experiment" data packages for leaf-level gas exchange and other leaf trait data; chamber, plot and landscape phenocamera images; thaw depth, and GPS locations of chambers and ambient plots. The Next-Generation Ecosystem Experiments: Arctic (NGEE Arctic), was a research effort to reduce uncertainty in Earth System Models by developing a predictive understanding of carbon-rich Arctic ecosystems and feedbacks to climate. NGEE Arctic was supported by the Department of Energy's Office of Biological and Environmental Research. The NGEE Arctic project had two field research sites: 1) located within the Arctic polygonal tundra coastal region on the Barrow Environmental Observatory (BEO) and the North Slope near Utqiagvik (Barrow), Alaska and 2) multiple areas on the discontinuous permafrost region of the Seward Peninsula north of Nome, Alaska. Through observations, experiments, and synthesis with existing datasets, NGEE Arctic provided an enhanced knowledge base for multi-scale modeling and contributed to improved process representation at global pan-Arctic scales within the Department of Energy's Earth system Model (the Energy Exascale Earth System Model, or E3SM), and specifically within the E3SM Land Model component (ELM).

54 ENVIRONMENTAL SCIENCES↗

The spacecraft radiation experiments

The radiation experiments on the Telstar spacecraft were designed to measure the electron and proton particle distributions in the region of space explored by the satellite orbit and to give information on the integral semiconductor radiation damage produced by these particles. A solar aspect experiment is included with the radiation experiments because of its direct importance to solar cell damage results. The design and the hardware for these experiments are described in the present paper. Results of the experiments are included in a companion paper in this issue.

TELSTAR SATELLITE↗

Heat flow experiment

The heat flow experiment installed on the lunar surface during the Apollo 15 flight is described. Subjects discussed are: (1) the experiment concept and design, (2) the operations of the experiment, (3) the employment of the experiment on the lunar surface at Hadley Rille site, (4) subsurface lunar temperatures, and (5) extrapolation of sensor temperatures to equilibrium values. Graphs of the data obtained from the experiment are provided.

Langseth, M. G., Jr.↗

A preliminary investigation of the environmental Control and Life Support Subsystems (EC/LSS) for animal and plant experiment payloads

A preliminary study of the environmental control and life support subsystems (EC/LSS) necessary for an earth orbital spacecraft to conduct biological experiments is presented. The primary spacecraft models available for conducting these biological experiments are the space shuttle and modular space station. The experiments would be housed in a separate module that would be contained in either the shuttle payload bay or attached to the modular space station. This module would be manned only for experiment-related tasks, and would contain a separate EC/LSS for the crew and animals. Metabolic data were tabulated on various animals that are considered useful for a typical experiment program. The minimum payload for the 30-day space shuttle module was found to require about the equivalent of a one-man EC/LSS; however, the selected two-man shuttle assemblies will give a growth and contingency factor of about 50 percent. The maximum payloads for the space station mission will require at least a seven-man EC/LSS for the laboratory colony and a nine-man EC/LSS for the centrifuge colony. There is practically no room for growth or contingencies in these areas.

Wells, H. B.↗

Space science experiments aboard ATS-F.

The Environmental Measurements Experiment (EME) package is mounted on the ATS-F spacecraft to a structure that is located on top of the 30-foot parabolic reflector hub. The eight experiments of the EME package are designed to study the environment in space at synchronous altitude and to obtain information on electromagnetic-ionospheric interactions. Six of these experiments will obtain data on charged particles of several different types. A seventh experiment is to provide magnetic field data. The eighth experiment is concerned with solar cell degradation studies.

Wales, R.↗

Feasibility study of a zero-gravity (orbital) atmospheric cloud physics experiments laboratory

A feasibility and concepts study for a zero-gravity (orbital) atmospheric cloud physics experiment laboratory is discussed. The primary objective was to define a set of cloud physics experiments which will benefit from the near zero-gravity environment of an orbiting spacecraft, identify merits of this environment relative to those of groundbased laboratory facilities, and identify conceptual approaches for the accomplishment of the experiments in an orbiting spacecraft. Solicitation, classification and review of cloud physics experiments for which the advantages of a near zero-gravity environment are evident are described. Identification of experiments for potential early flight opportunities is provided. Several significant accomplishments achieved during the course of this study are presented.

Hollinden, A. B.↗