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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 865 records · Page 48

Monolithic Photoelectrochemical CO 2 Reduction Producing Syngas at 10% Efficiency

We report increasing anthropogenic carbon dioxide emissions have prompted the search for photoelectrochemical (PEC) methods of converting CO 2 to useful commodity products, including fuels. Ideally, such PEC approaches will be sustained using only sunlight, water, and CO 2 as energetic and reactant inputs. However, low peak conversion efficiencies (< 5%) have made commercialization of fully-integrated PEC devices prohibitive. Here, a 4 cm 2 monolithic PEC device exceeding 10% solar-to-fuel efficiency with principal fuel products of carbon monoxide and hydrogen is reported. The corresponding solar-to-CO and solar-to-H 2 efficiencies are 7% and 3.5%, respectively. Screening of a range of operating conditions reveals a tunable product mixture of H 2 and CO using a gold electrocatalyst. Accordingly, it is shown that device optimization yields a H 2 -to-CO ratio of 1:2 commonly present in synthesis gas (syngas). Notably, the modularity and facile fabrication of this device permit the incorporation of a broad array of materials for various applications. For example, the electrocatalyst may easily be swapped to target a different set of products.

36 MATERIALS SCIENCE↗

Radiation Effects in Used Next Generation Nuclear Fuel Reprocessing Strategies

Given global commitments to significantly increase nuclear energy capacity, it is now more important than ever to develop efficient used nuclear fuel (UNF) management strategies to encourage widespread adoption of closed fuel cycles. To achieve this ambitious goal, a comprehensive understanding of radiation effects is essential for these next generation technologies, as radiolysis often limits longevity and performance. Here, we present new findings on: (i) the radiation robustness and performance of advanced sulfur chloride-based chlorination processes in the presence of nuclear materials (Fig. 1A); and (ii) the impacts of voloxidized uranium and rhenium complexation on monoamide-based UNF direct dissolution strategies (Fig 1B). These studies employed a combination of time-resolved electron pulse and dose accumulation gamma and electron beam irradiation techniques.

38 - RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCL↗

Emission FTIR analyses of thin microscopic patches of jet fuel residues deposited on heated metal surfaces

The relationship of fuel stability to fuel composition and the development of mechanisms for deposit formation were investigated. Fuel deposits reduce heat transfer efficiency and increase resistance to fuel flow and are highly detrimental to aircraft performance. Infrared emission Fourier transform spectroscopy was chosen as the primary method of analysis because it was sensitive enough to be used in-situ on tiny patches of monolayers or of only a few molecular layers of deposits which generally proved completely insoluble in any nondestructive solvents. Deposits of four base fuels were compared; dodecane, a dodecane/tetralin blend, commercial Jet A fuel, and a broadened-properties jet fuel particularly rich in polynuclear aromatics. Every fuel in turn was provided with and without small additions of such additives as thiophene, furan, pyrrole, and copper and iron naphthenates.

Lauer, J. L.↗

Application of Gas Analysis to Combustor Research

The performance of turbine-engine combustors usually is given in terms of operating limits and combustion efficiency. The latter property is determined most often by measuring the increase in enthalpy across the combustor through the use of thermocouples. This investigation was conducted to determine the ability of gas-analytical techniques to provide additional information about combustor performance. Gas samples were taken at the outlet and two upstream stations and their compositions determined. In addition to over-all combustion efficiency, estimates of local fuel-air ratios, local combustion efficiencies, and heat-release rates can be made. Conclusions can be drawn concerning the causes of combustion inefficiency and may permit corrective design changes to be made more intelligently. The purpose of this investigation was not to present data for a given combustor but rather to show the types and value of additional information that can be gained from gas-analytical data.

Hibbard, R. R.↗

Composition and Climate Impacts of Increasing Launches to Low Earth Orbit

We present simulations of an Earth system model in which launch vehicles inject gaseous and particulate combustion products into the stratosphere. We considered two plausible scenarios representative for the year 2050, one with 1000 launches per year and another with 10 times more, all of which assuming heavy lift (80 tons to low Earth orbit; LEO) launches using methane as a proxy for liquefied natural gas (LNG) fuel. An industry-standard plume flowfield model was used to predict emission of gaseous species including carbon monoxide, nitrogen oxides, and water vapor. Black carbon was introduced assuming vacuum emission equal 25% of equivalent kerosene engine. The gas emissions showed marginal or insignificant changes in atmospheric composition, while the black carbon emission was found to be the most influential component. Feedbacks involve tropopause and stratospheric warming, followed by a moistening of the stratosphere via tropospheric water vapor intrusions, together with a reduction in global albedo. The fact that LNG-fueled rockets could be a concern from aerosol emissions in our simulations, despite burning more efficiently than conventional fuels, underscores the need to better understand actual black carbon emissions from rocket engines in order to accurately predict the global impacts of launch vehicles on future climate.

Earth system model↗

Soot and Sulfuric Acid from Aircraft: Is There Enough to Cause Detrimental Environmental E-kCTSs?

Aerosol from aircraft can affect the environment in three ways: First, soot aerosol has been implicated to cause Icing-tern ozone depletion at mid-latitudes in the lower stratosphere at a rate of approx. 5% per decade. This effect is in addition and unrelated to the polar ozone holes which are strongly influenced by heterogeneous chemistry on polar stratospheric clouds. Second, the most obvious effect of jet aircraft is the formation of visible contrails in the upper troposphere. The Salt Lake City region experienced an 8% increase in cirrus cloud cover over a 15-year period which covariates with an increase in regional commercial air traffic. If soot particles act as freezing nuclei to cause contrail formation heterogeneously, they would be linked to a secondary effect to cloud modification that very likely is climatologically important. Third, a buildup of soot aerosol could reduce the single scatter albedo of stratospheric aerosol from 0.993+0.004 to 0.98, a critical value that has been postulated to separate stratospheric cooling from warming. Thus arises an important question: Do aircraft emit sufficient amounts of soot to have detrimental effects and warrant emission controls? During the 1996 SUCCESS field campaign, we sampled aerosols in the exhaust wake of a Boeing 757 aircraft and determined emission indices for sulfuric acid (EI(sub H2SO4) = 9.0E-2 and 5.0E-1 g/kg (sub FUEL) for 75 and 675 ppm fuel-sulfur, respectively) and soot aerosol (2.2E-3 less than EI(sub SOOT) = l.lE-2 g/kg (sub FUEL)). The soot particle analysis accounted for their fractal nature, determined electron-microscopically, which enhanced the surface area by a factor of 26 and the volume 11-fold over equivalent-volume spheres. The corresponding fuel-sulfur to H2SO4 conversion efficiency was 10% (for 675 ppmm fuel-S) and 37% (for 75 ppmm fuel-S). Applying the H2SO4 emission index to the 1990 fuel use by the worlds commercial fleets of 1.3E11 kg, a conversion efficiency of 30% of 500 ppmm fuel-S would have led to an annual contribution to the atmospheric sulfur budget by aircraft of 2.E7 kg H2SO4. This is about one part in 1.E4 of anthropogenic sulfate from other sources. The soot emission index given above yielded a 1990 injection of soot aerosol by aircraft of 1.E6 kg. Thus, soot amounts to only five percent of the aerosol generated by aircraft. Its reactivity with ozone would have to be 20 times that of sulfuric acid particles to make it chemically significant. Nevertheless, the findings, of stratospheric soot loadings commensurate with aircraft fuel consumption, based on the emission index given above and the assumption of stratospheric residence times of the order of one year implicate aircraft as stratospheric polluters. A trend similar to soot of H2SO4 aerosol loading could not be deciphered, neither from in situ measurements nor SAGE II satellite extinction, against the "noise" due to volcanic eruptions. Observation of soot particles at 20 km altitude which, if emitted by aircraft were generated at 10-12 km altitude, suggests a displacement of those particles against gravity. Because eddy mixing is virtually absent in the lower stratosphere and isentropic mixing explains lofting to only about 15 km, radiometric forces acting on morphologically and chemically asymmetric soot particles must be considered a possibility. The consequence could be an extended residence time of soot against that of sulfuric acid aerosol that would lower the single scatter albedo with time.

Pueschel, R. F.↗

Implementation of Triply Periodic Minimal Surfaces (TPMS) as surface objects in OpenMC

Triply Periodic Minimal Surfaces (TPMS) represent a promising geometry for future fuel designs due to their significant surface-to-volume ratio, which facilitates efficient cooling of nuclear fuel, a crucial factor for safety and efficiency. Demonstrating the remarkable capabilities of TPMS fuel requires initial modeling and simulation. This paper presents an implementation of TPMS in the Monte Carlo code OpenMC, enabling reactor physics modeling of TPMS. Here, the primary advantages over traditional methods using CAD files include reduced memory requirements for computations and high-fidelity implementation. This implementation has been tested against CAD files loaded in Serpent2, yielding promising results with low biases in the $k_{\textrm{eff}}$, comparable to biases in the material balance sheet. The implementation presented in this work will be used in future reactor physics computations related to new reactor designs involving TPMS-based fuels.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Backend Nuclear Fuel Cycle Radiation Chemistry

Given global commitments to significantly increase nuclear energy capacity, it is now more important than ever to develop efficient used nuclear fuel management strategies to improve resource utilization, energy security, and waste minimization. Here, an overview of nuclear energy, backend fuel cycle challenges, and advances in used nuclear fuel reprocessing radiation chemistry will be presented. More specifically, the use of electron pulse irradiation techniques to explore radiation-induced reaction mechanisms in actinide containing solutions and solvent systems.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

Enhancement of Mixing and Reaction in High-speed Combustor Flowfields

Research has been underway for a number of years, both in the United States and abroad, to develop advanced aerospace propulsion systems for use late in this century and beyond. One program is now underway at the NASA Langley Research Research has been underway for a number of years, both in the United States and abroad, to develop advanced aerospace propulsion systems for use late in this century and beyond. One program is now underway at the NASA Langley Research Center to develop a hydrogen-fueled supersonic combustion ramjet (scramjet) that is capable of propelling a vehicle at hypersonic speeds in the atmosphere. A part of that research has been directed toward the optimization of the scramjet combustor and, in particular, the efficiency of fuel-air mixing and reaction taking place in the engine. In the high-speed vehicle configurations currently being considered, achieving a high combustor efficiency becomes particularly difficult. With increasing combustor Mach number, the degree of fuel-air mixing that can be achieved through natural convective and diffusive processes is reduced leading to an overall decrease in combustion efficiency and thrust. Compressible shear layers and jets provide a good model for studying the physical processes occurring in high speed mixing and combustion in a scramjet. Mixing layers are characterized by large scale eddies that form due to the high shear that is present between the fuel and the air streams. These eddies entrain the fuel and air into the mixing region between the fluids leading to increased surface area and locally steep concentration gradients. Molecular diffusion then occurs across the strained interfaces. In an early study of high-speed mixing, Brown and Roshko show that the spreading rate of a supersonic mixing layer decreases with increasing Mach number, exhibiting a factor of three decrease in spread rate as compared with an incompressible mixing layer with the same density ratio. They conclude that the reduced spread rate is primarily due to compressibility. Papamoschou and Roshko also observe that the spreading rate of compressible mixing layers is significantly reduced over that of incompressible layers. To characterize the structure of the flow quantitatively, they define a convective Mach number. The reduction in mixing layer spreading rate is shown in these experiments to correlate well with increasing convective Mach number.

Drummond, J. Philip↗

Heating and Efficiency Comparison of a Fischer-Tropsch (FT) Fuel, JP-8+100, and Blends in a Three-Cup Combustor Sector

In order to realize alternative fueling for military and commercial use, the industry has set forth guidelines that must be met by each fuel. These aviation fueling requirements are outlined in MIL-DTL-83133F(2008) or ASTM D 7566-Annex standards and are classified as drop-in fuel replacements. This paper provides combustor performance data for synthetic-paraffinic-kerosene- (SPK-) type (Fisher-Tropsch (FT)) fuel and blends with JP-8+100, relative to JP-8+100 as baseline fueling. Data were taken at various nominal inlet conditions: 75 psia (0.52 MPa) at 500 aF (533 K), 125 psia (0.86 MPa) at 625 aF (603 K), 175 psia (1.21 MPa) at 725 aF (658 K), and 225 psia (1.55 MPa) at 790 aF (694 K). Combustor performance analysis assessments were made for the change in flame temperatures, combustor efficiency, wall temperatures, and exhaust plane temperatures at 3%, 4%, and 5% combustor pressure drop (% P) for fuel:air ratios (F/A) ranging from 0.010 to 0.025. Significant general trends show lower liner temperatures and higher flame and combustor outlet temperatures with increases in FT fueling relative to JP-8+100 fueling. The latter affects both turbine efficiency and blade/vane life. In general, 100% SPK-FT fuel and blends with JP-8+100 produce less particulates and less smoke and have lower thermal impact on combustor hardware.

Thomas, Anna E.↗

Experimental study of the impact of scavenging efficiency on diesel combustion in an opposed-piston two-stroke engine

The opposed-piston two-stroke (OP2S) engine is a promising alternative powertrain technology that can offer thermal and brake efficiency improvements over conventional four-stroke engines. In recent years, many of the technical barriers of the OP2S engine architecture have been overcome. However, there is still a need for fundamental studies to provide insight into the scavenging and combustion processes of the OP2S engine to help design and operate the most efficient combustion systems using this engine architecture. This work aims to provide such insights by analyzing experimental data collected on a 3-cylinder, 4.9 L OP2S engine. Specifically, a scavenging efficiency sweep, an engine speed sweep with a constant scavenging efficiency, and an engine speed with a constant pressure differential across the engine were studied in detail. It was found that in diesel combustion, as the scavenging efficiency decreased, the increase in temperature of the hot, internal residuals resulted in a significant increase in heat transfer. Despite lowering pumping losses, this resulted in an overall decrease in brake efficiency. When the bulk thermodynamic conditions of two different scavenging efficiency cases (67% and 72%) were matched at port closing, the lower scavenging efficiency case still displayed a 0.7 percentage point penalty in net thermal efficiency and an increase in engine-out indicated specific emissions of NOx of 18% due to residual stratification in the cylinder. The results presented in this work show that the optimal breathing strategy in diesel combustion on an OP2S engine architecture is one that results in a slightly under-scavenged environment at port closing. However, the results did show potential system-level efficiency benefits of decreasing scavenging efficiency, meaning that alternative fuels and combustion strategies without the constraints of diesel combustion could achieve system-level efficiency gains by running significantly under-scavenged.

Engineering↗

Two trillion gallons: Fuel savings from fuel economy improvements to US light-duty vehicles, 1975–2018

Since 1975, the fuel economy of new light-duty vehicles sold in the U.S. has almost doubled. Fuel economy improvements on laboratory tests gradually became real improvements on the road as newer, more efficient vehicles replaced older less efficient ones. Fleet-wide fuel economy gains produced large fuel savings. In this paper, we show that fuel economy gains measured on laboratory test cycles, adjusted for on-road conditions and weighted by the distribution of vehicles by age and their relative use, closely match estimates by the Federal Highway Administration based primarily on traffic counts and motor fuel tax records. Furthermore, adjusting for the rebound effect of fuel economy on vehicle miles traveled, we estimate the fuel savings, CO 2 emissions reductions and dollars saved on fuel due to fuel economy improvements over the past 43 years. Through the end of 2018, estimated cumulative fuel savings amount to approximately 2 trillion gallons of gasoline. We estimate that roughly one-fifth of the savings can be attributed to gasoline price increases over the period and four-fifths to fuel economy and greenhouse gas (ghg) standards.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗

Characterization Testing of the Teledyne Passive Breadboard Fuel Cell Powerplant

NASA's Exploration Technology Development Program (ETDP) is tasked with the development of enabling and enhancing technologies for NASA's exploration missions. As part of that initiative, the return to the Moon requires a reliable, efficient, and lightweight fuel cell powerplant system to provide power to the Altair Lunar Lander and for lunar surface systems. Fuel cell powerplants are made up of two basic parts; the fuel cell itself and the supporting ancillary subsystem. This subsystem is designed to deliver reactants to the fuel cell and remove product water and waste heat from the fuel cell. Typically, fuel cell powerplant ancillary subsystems rely upon pumps and active water separation techniques to accomplish these tasks for closed hydrogen/oxygen systems. In a typical system, these components are the largest contributors to the overall parasitic power load of the fuel cell powerplant. A potential step towards the development of an efficient lightweight power system is to maximize the use of "passive" or low-power ancillary components as a replacement to these high-power load components

Loyselle, Patricia↗

Life cycle analysis of gasification and Fischer-Tropsch conversion of municipal solid waste for transportation fuel production

Non-recyclable municipal solid waste (MSW) can be used as feedstock for liquid fuel production via gasification followed by Fischer-Tropsch (FT) processes. Given the heterogeneity of MSW material composition and variation in material properties, its convertibility to liquid hydrocarbon fuels could vary widely, affecting the sustainability of utilizing non-recyclable MSW for fuel production. This study evaluates the life cycle greenhouse gas (GHG) emissions (carbon intensities [CIs]) of FT fuels from non-recyclable MSW. Key issues that could greatly affect the CIs were examined, including fossil carbon content of the MSW, emission implications of diverting non-recyclable MSW from landfills to fuel production, and conversion efficiency. Results show that the CIs of fuels produced from various waste streams range 80–105 gCO2e/MJ, which may exceed the CI of petroleum fuels. Higher fossil carbon content in the MSW feedstock tends to incur higher GHG emissions as biogenic carbon emissions are considered carbon neutral. Meanwhile, diverting different fractions of non-recyclable MSW, such as food waste and low-quality paper, from landfills may result in GHG emissions that may include the potential avoidance of methane emissions and potential sequestration of biogenic carbon that is foregone. To reduce GHG emissions, a carbon capture and sequestration option in the fuel production stage is considered, which could reduce the CI by 53–64 gCO2e/MJ. Carbon fates of different non-recyclable MSW in landfills are further evaluated to determine how they vary and impact the CIs of MSW-derived fuels.

02 PETROLEUM↗

Energy conservation and air transportation

Air transportation demand and passenger energy demand are discussed, in relation to energy conservation. Alternatives to air travel are reviewed, along with airline advertising and ticket pricing. Cargo energy demand and airline systems efficiency are also examined, as well as fuel conservation techniques. Maximum efficiency of passenger aircraft, from B-747 to V/STOL to British Concorde, is compared.

Source record↗

Mixing and combustion enhancement in supersonic reacting flows

Research has been conducted for a number of years at the NASA Langley Research Center to develop a supersonic combustion ramjet (scramjet) capable of propelling a vehicle at hypersonic speeds in the atmosphere or beyond. Recently, that research has been directed toward the optimization of the scramjet combustor, and in particular the efficiency of fuel-air mixing and reaction in the engine. This paper describes a study of fuel-air mixing and reaction in a supersonic flow field, and discusses several techniques that were applied for enhancing the mixing processes and overal combustion efficiency in the flow. Based on the results of the study, an alternate fuel injector configuration was computationally designed, and that configuration significantly increased the amount of fuel-air mixing and combustion over a given combustor length that was achieved.

Drummond, J. Philip↗

Future of Fuel Savings

Using automation to free up controllers for more strategic management of air traffic is one approach being studied by NASA as it seeks to boost airspace system capacity and efficiency, thereby saving fuel. Heinz Erzberger, a NASA Ames Research Center senior scientist, says the Advanced Airspace Concept (AAC) has been studied for several years. It could increase efficiency 15% by providing optimal routes that cut airlines direct operating costs. A 25% increase in landings on existing runways could follow an important benefit. AAC is one of the efforts to be reviewed by the Joint Planning and Development Organization, an FAA-led initiative by six federal agencies to redesign the U.S. air transportation system by 2025. The main goal is to triple air traffic capacity within 20 years to avert the sort of gridlock that would make fuel consumption only one of many travel nightmares. The automated system approach would allow aircraft to fly optimal trajectories. A trajectory would be defined in the standard three dimensions and eventually include the fourth, time. The management of air traffic by the data-linked exchange of trajectories would start at high altitude and eventually move down to lower altitudes. The automated concept is an outgrowth of the type of tools developed by NASA for use by FAA controllers in managing traffic flows over the years, including ones that optimize routings for the best fuel burn. But AAC would push automation further to reduce workload so controllers can focus on "solving strategic control problems, managing traffic flow during changing weather and ... other unusal events." One key component, the automated trajectory server (ATS), is a ground systems that would rely on software to manage flight path requests from aircrews and controllers. But, Erzberger acknowledges, "The FAA's current plan for upgrades to air traffic services does not include [allowing] the future ground system to issue separation-critical clearances of trajectory changes autonomously to aircraft via data link without explicit approval of a controller," as the AAC proposes. The AAC enables pilots or controllers to data link requests for a trajectory change to the ATS for approval after they are deconflicted with the paths of other aircraft. To divert around storms, for example, pilots could data link their trajectory preference to the ATS. Since several aircraft might request similar routes, the computer would then have to suggest alternatives. This could be accomplished without pilot-controller radio calls, a big bottleneck now. The ATS would have a built-in conflict monitor to call for a resolution (turn, climb or descend), when loss of separation is likely in 1-20 min. The AAC system would reduce controller errors by 90%, according to NASA Ames estimates. The AAC would have a back-up program to assure separation-Tactical Separation Assurance (TSAFE). It s designed to detect short-term traffic conflicts within 3-4 min. of loss of separation. The last line of defense would still be provided by traffic alert & collision avoidance systems (TCAS).

Hughes, David↗

Flowsheet Development for the University of Tokyo YAYOI (UTY) Fuel

The Savannah River National Laboratory (SRNL) was requested by H-Canyon Engineering to determine the flowsheet parameters needed to dissolve and store the YAYOI Material Test Reactor (MTR) uranium fuel safely and efficiently. In response to this request, a literature review of existing SRNL MTR dissolution flowsheets and general fuel dissolution literature in the nuclear fuel processing industry was performed to evaluate chemical dissolution parameters required to dissolve the YAYOI fuel and the tin-plated carbon steel product cans (PC). Based on past dissolutions of similar fuel in the H-Canyon and open literature reviews on chemical dissolution of spent nuclear fuel (SNF), the following conclusions and flowsheet recommendations were made.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗