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At least 865 records · Page 48

Modeling the Lunar Wake Response to a CME Using a Hybrid PIC Model

In the solar wind, a low-density wake region forms downstream of the nightside lunar surface. In this study, we use a series of 3D hybrid particle-in-cell simulations to model the response of the lunar wake to a passing coronal mass ejection (CME). Average plasma parameters are derived from the Wind spacecraft located at 1 au during three distinct phases of a passing halo (Earth-directed) CME on 2015 June 22. Each set of plasma parameters, representing the shock/plasma sheath, a magnetic cloud, and plasma conditions we call the mid-CME phase, are used as the time-static upstream boundary conditions for three separate simulations. These simulation results are then compared with results that use nominal solar wind conditions. Results show a shortened plasma void compared to nominal conditions and a distinctive rarefaction cone originating from the terminator during the CME's plasma sheath phase, while a highly elongated plasma void reforms during the magnetic cloud and mid-CME phases. Developments of electric and magnetic field intensification are also observed during the plasma sheath phase along the central wake, while electrostatic turbulence dominates along the plasma void boundaries and 2–3 lunar radii RM downstream in the central wake during the magnetic cloud and mid-CME phases. The simulations demonstrate that the lunar wake responds in a dynamic way with the changes in the upstream solar wind during a CME.

Anthony P. Rasca↗

On the Retrieval of Ice Cloud Particle Shapes from POLDER Measurements

Shapes of ice crystals can significantly affect the radiative transfer in ice clouds. The angular distribution of the polarized reflectance over ice clouds strongly depends on ice crystal shapes. Although the angular-distribution features of the total or polarized reflectance over ice clouds implies a possibility of retrieving ice cloud particle shapes by use of remote sensing data, the accuracy of the retrieval must be evaluated. In this study, a technique, which applies single ice crystal habit and multidirectional polarized radiance to retrieve ice cloud particle shapes, is assessed. Our sensitivity studies show that the retrieved particle shapes &om this algorithm can be considered good approximations to those in actual clouds in calculation of the phase matrix elements. Although a fractal poly-crystal shape or an inhomogeneous hexagonal column may also produce this type of phase functions, more representative single-scattering properties from combinations of natural particle shapes and size distributions may still be necessary in accurate retrieval of other cloud properties such as optical thickness and particle size.

Sun, W.↗

Hydrogen chloride measurements in the Space Shuttle exhaust cloud - First launch, April 12, 1981

Partitioning of hydrogen chloride between the aerosol and gaseous phases in the first Space Shuttle exhaust cloud was experimentally investigated as the exhaust cloud was diluted with ambient air. Airborne measurements were obtained of gaseous hydrogen chloride (HCl), total HCl, relative humidity, and temperature to determine the conditions controlling HCl aerosol formation in the Shuttle exhaust cloud. Two segments of the cloud, each at a significantly different relative humidity, were monitored. Equilibrium predictions of HCl aerosol formation agreed with the measured HCl partitioning at the higher and lower relative humidity conditions, but do not agree at the aerosol formation threshold region. Measurements were taken in the Shuttle exhaust cloud from 8.6 min until 2 h and 8 min after launch. HCl concentrations ranged from 17.5 to 0.9 ppm and relative humidity from 86% to less than 10%.

Sebacher, D. I.↗

Evidence for interstellar H2O in the Orion molecular cloud

A search for interstellar gas phase H2O in the infrared spectrum of the BN object in Orion is reported. There is absorption (S/N = 2-4) at the position of the nu3 1(01)-2(02) line of H2O at 3801.42/cm, the strongest expected H2O line. Statistical analysis of the spectrum provides corroborating evidence for other H2O lines. With an assumed H2O excitation temperature of 150 K, N(H2O) of 2.3 x 10 to the 17th/sq cm or less toward the BN object is derived. The H2O column density implies abundance ratios of (H2O)/(CO) = 0.01-0.08 or less and (HDO)/(H2O) = 0.8-3.0 x 10 to the -3rd or more. The gas-to-ice ratio is (H2O gas)/(H2O ice) = 0.06 with an estimated uncertainty of a factor of 5.

Knacke, R. F.↗

Uncertainties in Ice-Sheet Altimetry from a Spaceborne 1064-nm Single-Channel Lidar Due to Undetected Thin Clouds

In support of the Ice, Cloud, and land Elevation Satellite (ICESat)-II mission, this paper studies the bias in surface-elevation measurements caused by undetected thin clouds. The ICESat-II satellite may only have a 1064-nm single-channel lidar onboard. Less sensitive to clouds than the 532-nm channel, the 1064-nm channel tends to miss thin clouds. Previous studies have demonstrated that scattering by cloud particles increases the photon-path length, thus resulting in biases in ice-sheet-elevation measurements from spaceborne lidars. This effect is referred to as atmospheric path delay. This paper complements previous studies in the following ways: First, atmospheric path delay is estimated over the ice sheets based on cloud statistics from the Geoscience Laser Altimeter System onboard ICESat and the Moderate Resolution Imaging Spectroradiometer (MODIS) onboard Terra and Aqua. Second, the effect of cloud particle size and shape is studied with the state-of-the-art phase functions developed for MODIS cirrus- cloud microphysical model. Third, the contribution of various orders of scattering events to the path delay is studied, and an analytical model of the first-order scattering contribution is developed. This paper focuses on the path delay as a function of telescope field of view (FOV). The results show that reducing telescope FOV can significantly reduce the expected path delay. As an example, the average path delays for FOV = 167 microrad (a 100-m-diameter circle on the surface) caused by thin undetected clouds by the 1064-nm channel over Greenland and East Antarctica are illustrated.

Yang, Yuekui↗

Application of the CALIOP Layer Product to Evaluate the Vertical Distribution of Aerosols Estimated by Global Models: AeroCom Phase I Results

The CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) layer product is used for a multimodel evaluation of the vertical distribution of aerosols. Annual and seasonal aerosol extinction profiles are analyzed over 13 sub-continental regions representative of industrial, dust, and biomass burning pollution, from CALIOP 2007-2009 observations and from AeroCom (Aerosol Comparisons between Observations and Models) 2000 simulations. An extinction mean height diagnostic (Z-alpha) is defined to quantitatively assess the models' performance. It is calculated over the 0-6 km and 0-10 km altitude ranges by weighting the altitude of each 100 m altitude layer by its aerosol extinction coefficient. The mean extinction profiles derived from CALIOP layer products provide consistent regional and seasonal specificities and a low inter-annual variability. While the outputs from most models are significantly correlated with the observed Z-alpha climatologies, some do better than others, and 2 of the 12 models perform particularly well in all seasons. Over industrial and maritime regions, most models show higher Z-alpha than observed by CALIOP, whereas over the African and Chinese dust source regions, Z-alpha is underestimated during Northern Hemisphere Spring and Summer. The positive model bias in Z-alpha is mainly due to an overestimate of the extinction above 6 km. Potential CALIOP and model limitations, and methodological factors that might contribute to the differences are discussed.

Aerosols and particles↗

The Chemistry and Excitation of Water in Molecular Clouds

We model the chemistry and thermal balance of opaque molecular clouds exposed to an external flux of ultraviolet photons. We include the processes of gas phase and grain surface chemical reactions; in particular we examine closely the freezing of atoms and molecules onto grain surfaces and the desorption of molecules from grain surfaces as a function of depth into a molecular cloud. We find that on the surface of a molecular cloud the gas phase water abundances are low because of photodissociation, and the grain phase water (ice) abundance is low because of photodesorption of water from the grain surfaces. Deeper into the cloud, at A(sub v) less than or approximately 2-8 depending on the strength of the external ultraviolet flux, the gas phase water abundance increases with depth as the photodissociation rates decline due to dust attenuation of the ultraviolet field. However, beyond A(sub v) less than or approximately 2-8 the gas phase water abundance declines because the water freezes as water ice on the grains, and photodesorption is no longer effective in clearing the ice. A peak water abundance of about 10(exp -6) to 10(exp -7) occurs at about A(sub v) approximately 2-8, relatively independent of the gas density and the ultraviolet field. We show that such a model matches very closely the observations of the Submillimeter Wave Astronomical Satellite (SWAS), a NASA Small Explorer Mission. The model elucidates several mechanisms that have been recently invoked to understand gas phase chemistry in clouds, including-the freeze-out of molecules onto grain surface, the desorption of these molecules from the surfaces, and the abundance gradients of molecules as functions of depth into molecular clouds.

Hollenbach, David↗

EPCAPE-PT-LANL Measurements: Humidified Cavity Attenuated Phase Shift Spectroscopy

Coastal cities offer a unique environment for studying aerosol-cloud interactions and the effects of urban emissions on cloud properties. As part of the Eastern Pacific Cloud Aerosol Precipitation Experiment (EPCAPE), the Partitioning Thrust by Los Alamos National Laboratory (EPCAPE-PT-LANL) was conducted. Our campaign focused on measuring the optical and chemical properties of aerosols and their interactions within marine stratocumulus clouds in La Jolla, California. EPCAPE-PT-LANL enhances the primary goals of EPCAPE through innovative observations of vapor-phase transitions between aerosols and cloud droplets, the impact of black carbon on aerosol-cloud dynamics, and the effects of cloud processing on aerosol optical properties. Instrument: Humidified Cavity Attenuated Phase Shift Particulate Matter Single Scattering Albedo (H-CAPS-PMSSA, Aerodyne Inc) Data Notes: The scattering truncation correction was not applied to Bsca. The Bext needs no correction. Files: data_10sec_CAPS.csv, data_10min_CAPS.csv Header: - Bext_wet_CAPS_450nm[1/Mm]: Wet aerosol extinction coefficient measured at 450 nm by the CAPS, in inverse megameters (Mm⁻¹). - Bsca_wet_CAPS_450nm[1/Mm]: Wet aerosol scattering coefficient measured at 450 nm by the CAPS, in inverse megameters (Mm⁻¹). - Temp_wet_CAPS[K]: Temperature inside the wet CAPS measurement chamber, in Kelvin. - Bext_dry_CAPS_450nm[1/Mm]: Dry aerosol extinction coefficient measured at 450 nm by the CAPS, in inverse megameters (Mm⁻¹). - Bsca_dry_CAPS_450nm[1/Mm]: Dry aerosol scattering coefficient measured at 450 nm by the CAPS, in inverse megameters (Mm⁻¹). - Temp_dry_CAPS[K]: Temperature inside the dry CAPS measurement chamber, in Kelvin. - Wet_RH_preCAPS[%]: Relative humidity before entering the wet CAPS, in percent. - Wet_RH_postCAPS[%]: Relative humidity after exiting the wet CAPS, in percent. - Humidifier_RH_CAPS[%]: Relative humidity inside the humidifier used with the CAPS, in percent. - dualCAPS_inlet_RH[%]: Relative humidity at the inlet of the dual (wet/dry) CAPS setup, in percent. - Wet_Temp_preCAPS[C]: Temperature before entering the wet CAPS, in degrees Celsius. - Wet_Temp_postCAPS[C]: Temperature after exiting the wet CAPS, in degrees Celsius. - Humidifier_Temp[C]: Temperature inside the humidifier used with the CAPS, in degrees Celsius. - dualCAPS_inlet_Temp[C]: Temperature at the inlet of the dual (wet/dry) CAPS setup, in degrees Celsius. - Zero_dry_CAPS: 1 is a calibration check for the dry CAPS to ensure zero reading under filter air conditions. - Zero_wet_CAPS: 1 is a calibration check for the wet CAPS to ensure zero reading under filter air conditions. - CVI_Flag[bool]: A boolean flag indicating whether the Counterflow Virtual Impactor (CVI) was active (true) or inactive (false) during the measurement.

54 ENVIRONMENTAL SCIENCES↗

Protostellar formation in rotating interstellar clouds. II - Axially symmetric collapse

A two spatial dimension gravitational hydrodynamics code has been used to calculate the initial isothermal dynamic collapse phase of axially symmetric, rotating interstellar clouds. The Eulerian code has been constructed so as to conserve angular momentum both locally (approximately) and globally (exactly). An axially symmetric, rotating cloud collapses to form a rotating, near-equilibrium ring. The rings so formed are compared with those found previously by Black and Bodenheimer, and Bodenheimer and Tscharnuter, and found to agree in structure fairly well. Numerical tests with the code, as well as an analytic calculation of the collapse of a pressureless, rotating, axially symmetric cloud in a fixed gravitational potential, support the assertion that the observed ring formation is physically realistic.

Boss, A. P.↗

Better Constraining Supercooled Clouds Could Reduce Projected Warming Spread

The increase of climate sensitivity to rising greenhouse gas concentrations in the coupled model intercomparison project phase 6 (CMIP6) Earth system models (ESMs) compared to CMIP5 ESMs is primarily attributed to a larger extratropical cloud response to climate change, referred to as cloud feedback. The ratio of supercooled liquid cloud water relative to all cloud water, termed liquid phase ratio (LPR), which has also notably increased in many recent ESMs, is thought to be a primary driver of the extratropical cloud feedback increase. Unlike the preponderance of previous studies that compare native model LPR directly with observations, here we evaluate LPR over three ESM generations against Cloud–Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) using an instrument simulator approach, which mimics instrument limitations and uses consistent cloud definitions and resolutions. We find that current coupled model intercomparison project (CMIP) ESMs collectively simulate greater LPR than previous CMIP generations and overestimate LPR compared to observations, contrary to previous findings, likely driven by past inconsistent comparisons of ESM outputs with CALIPSO observations. We further show that greater LPR in ESM present-day climate is unexpectedly correlated with a smaller extratropical cloud feedback, attributable to a decrease of cloud amount exceeding the increase of cloud optical depth. Finally, our results suggest that improving constraints on model LPR using our evaluation framework would likely reduce the spread in CMIP6 climate sensitivities, owing to its effect on extratropical cloud feedback from supercooled clouds.

greenhouse gas concentrations↗

Water vapor in the Orion Molecular Cloud

Infrared observations of interstellar gas-phase H2O in the spectrum of the BN object in Orion are reported. There are absorptions (S/N = 2-5) at the positions of four of the strong lines in the 000-001 nu3 vibration-rotation band. With an estimated excitation temperature of 150 K, the column density of gaseous H2O toward BN in the OMC-1 cloud is (2 + or - 1) x 10 to the 17th/sq cm. The intensities of the lines imply an ortho/para ratio of 1 + or - 0.5 indicating recent sublimation of H2O from low-temperature grains. The results give gas-phase abundance ratios of H2O/CO roughly 0.03 + or - 0.02 and HDO/H2O = 0.001-0.0001 toward BN. The velocities of the H2O absorptions agree with those of the ridge source and CO outflow, but the position along the line of sight is not well constrained. The gas/solid ratio is H2O(gas)/H20(ice) = 0.05 or less. Less than 1 percent of the oxygen is in H2O gas (assuming total cosmic abundance). Most of the H2O in the line of sight to BN, and by inference in quiescent regions of molecular clouds generally, is frozen on grains.

Knacke, R. F.↗

The 1980 eruptions of Mount St. Helens - Physical and chemical processes in the stratospheric clouds

The large and diverse set of observational data collected in the high-altitude plumes of the May 18, May 25, and June 13, 1980 eruptions is organized and analyzed with a view to discerning the processes at work. The data serve to guide and constrain detailed model simulations of the volcanic clouds. For this purpose, use is made of a comprehensive one-dimensional model of stratospheric sulfate aerosols, sulfur precursor gases, and volcanic ash and dust. The model takes into account gas-phase and condensed-phase (heterogeneous) chemistry in the clouds, aerosol nucleation and growth, and cloud expansion. Computational results are presented for the time histories of the gaseous species concentrations, aerosol size distributions, and ash burdens of the eruption clouds. Also investigated are the long-term buildup of stratospheric aerosols in the Northern Hemisphere and the persistent effects of injected chlorine and water vapor on stratospheric ozone. It is concluded that SO2, water vapor, and ash were probably the most important substances injected into the stratosphere by the Mount St. Helens volcano, both with respect to their widespread effects on composition and their effect on climate.

Turco, R. P.↗

Optical and morphological properties of Cirrus clouds determined by the high spectral resolution lidar during FIRE

Cirrus clouds reflect incoming solar radiation and trap outgoing terrestrial radiation; therefore, accurate estimation of the global energy balance depends upon knowledge of the optical and physical properties of these clouds. Scattering and absorption by cirrus clouds affect measurements made by many satellite-borne and ground based remote sensors. Scattering of ambient light by the cloud, and thermal emissions from the cloud can increase measurement background noise. Multiple scattering processes can adversely affect the divergence of optical beams propagating through these clouds. Determination of the optical thickness and the vertical and horizontal extent of cirrus clouds is necessary to the evaluation of all of these effects. Lidar can be an effective tool for investigating these properties. During the FIRE cirrus IFO in Oct. to Nov. 1986, the High Spectral Resolution Lidar (HSRL) was operated from a rooftop site on the campus of the University of Wisconsin at Madison, Wisconsin. Approximately 124 hours of fall season data were acquired under a variety of cloud optical thickness conditions. Since the IFO, the HSRL data set was expanded by more than 63.5 hours of additional data acquired during all seasons. Measurements are presented for the range in optical thickness and backscattering phase function of the cirrus clouds, as well as contour maps of extinction corrected backscatter cross sections indicating cloud morphology. Color enhanced images of range-time indicator (RTI) displays a variety of cirrus clouds with approximately 30 sec time resolution are presented. The importance of extinction correction on the interpretation of cloud height and structure from lidar observations of optically thick cirrus are demonstrated.

Grund, Christian John↗

Interstellar O2. I - Abundance, excitation, and prospects for detection of O-16O-18 at radio frequencies

Molecular oxygen, O2, is predicted to be an important constituent of the interstellar gas, but it has not yet been detected in interstellar clouds. In this paper, the gas phase production and destruction of O2 are reconsidered, a non-LTE calculation of level populations at cloud temperatures is presented, and O2 column densities in diffuse and dark clouds are predicted. Ground-based detection of the 234 GHz line of O-16O-18 is shown to be feasible; if CO and O2 are comparable in abundance in clouds similar to the Taurus molecular cloud or in giant molecular clouds, the brightness temperature is predicted to be 0.1 K.

Black, J. H.↗

The Performance of Current Atmospheric Radiation Codes in Phase I of CIRC

The Continual Intercomparison of Radiation Codes (CIRC) is intended as an evolving and regularly updated reference source for evaluation of radiative transfer (RT) codes used in Global Climate Models and other atmospheric applications. In our presentation we will discuss our evaluation of the performance of 13 shortwave and 11 longwave RT codes that participated in Phase I of CIRC. CIRC differs from previous intercomparisons in that it relies on an observationally validated catalogue of cases. The seven CIRC Phase I baseline cases, five cloud-free, and two with overcast liquid clouds, are built around observations by the Atmospheric Radiation Measurements (ARM) program that satisfy the goals .of Phase I, namely to examine RT model performance in realistic, yet not overly complex, atmospheric conditions. Besides the seven baseline cases, additional idealized "subcases" are also examined to facilitate interpretation of model errors. We will quantify individual model performance with respect to reference line-by-line calculations, and will also highlight RT code behavior for conditions of doubled CO2 , aspects of utilizing a spectral specification of surface albedo, and the impact of the inclusion of scattering in the thermal infrared. Our analysis suggests that RT codes should work towards improving their calculation of diffuse shortwave flux, shortwave absorption, treatment of spectral surface albedo, and shortwave CO2 forcing. Despite practical difficulties in comparing our results to previous results by the Intercomparison of Radiation Codes in Climate Models (ICRCCM) conducted about 20 years ago, it appears that the current generation of RT codes do indeed perform better than the codes of the ICRCCM era. By enhancing the range of conditions under which participating codes are tested, future CIRC phases will hopefully allow even more rigorous examination of RT code performance.

Oreopoulos, L.↗

Comparison of the MODIS Collection 5 Multilayer Cloud Detection Product with CALIPSO

CALIPSO, launched in June 2006, provides global active remote sensing measurements of clouds and aerosols that can be used for validation of a variety of passive imager retrievals derived from instruments flying on the Aqua spacecraft and other A-Train platforms. The most recent processing effort for the MODIS Atmosphere Team, referred to as the Collection 5 scream, includes a research-level multilayer cloud detection algorithm that uses both thermodynamic phase information derived from a combination of solar and thermal emission bands to discriminate layers of different phases, as well as true layer separation discrimination using a moderately absorbing water vapor band. The multilayer detection algorithm is designed to provide a means of assessing the applicability of 1D cloud models used in the MODIS cloud optical and microphysical product retrieval, which are generated at a 1 km resolution. Using pixel-level collocations of MODIS Aqua, CALIOP, we investigate the global performance of multilayer cloud detection algorithms (and thermodynamic phase).

Platnick, Steven↗

The Big Plunge at Venus: The DAVINCI Descent Phase

DAVINCI (Deep Atmosphere Venus Investigation of Noble gases, Chemistry, and Imaging) was selected as one of two new Discovery missions in summer of 2021 with the primary goals are to study how the Venus atmosphere formed and changed over time. DAVINCI does this by making in situ measurements of the atmosphere and taking images below the cloud layer during the descent phase. The probe is neither designed nor required to land on the surface so all critical science data must be taken and transmitted to a relay spacecraft prior to impact. This architecture drives the mission to a carefully-crafted concept of operations; deployments, instrument operations, and communications are choreographed to ensure the right data is gathered at the right altitude given the uncertainties in the trajectory and timeline. A complex flow of analyses and tests throughout development will validate the system’s ability to execute the mission goals. In the end, DAVINCI will be ready for the one opportunity at one hour of descent time to meet its driving science goals.

DAVINCI↗