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DOE OSTI2022

Compton Polarimetry for Neutral Weak Form Factor Measurements in 208Pb and 48Ca

Atomic nuclei contain a number of protons and neutrons. Most heavy nuclei contain more neutrons than protons in order to remain stable. The nuclear proton distribution can be measured via elastic scattering of charged particles, but the neutron distribution remains poorly constrained. Nuclear structure theory also predicts a "neutron skin" ?Rnp where the mean radii of neutrons in the nucleus exceeds that of protons. Two experiments were run in 2019 and 2020 to measure the neutron skin in two different nuclei. The first experiment, PREX-II, was designed to measure the neutron skin in 208Pb, while the second experiment, CREX, was designed to measure the neutron skin in 48Ca. Both experiments employed the parity-violating electron scattering (PVES) technique in which longitudinally spin-polarized electrons are scattered off an unpolarized target.

Zec, Allison↗
DOE OSTI2022

Whitepaper submitted to Snowmass21: Advanced accelerator linear collider demonstration facility at intermediate energy

It is widely accepted that the next lepton collider beyond a Higgs factory would require center-of-mass energy of the order of up to 15 TeV. Since, given reasonable space and cost restrictions, conventional accelerator technology reaches its limits near this energy, high-gradient advanced acceleration concepts are attractive. Advanced and novel accelerators (ANAs) are leading candidates due to their ability to produce acceleration gradients on the order of 1--100~GV/m, leading to compact acceleration structures. Over the last 10-15 years significant progress has been achieved in accelerating electron beams by ANAs. For example, the demonstration of several-GeV electron beams from laser-powered capillary discharge waveguides, as well as the proof-of-principle coupling of two accelerating structures powered by different laser pulses, has increased interest in ANAs as a viable technology to be considered for a compact, TeV-class, lepton linear collider. However, intermediate facilities are required to test the technology and demonstrate key subsystems. A 20-100 GeV center-of-mass energy ANA-based lepton collider can be a possible candidate for an intermediate facility. Apart from being a test beam facility for accelerator and detector studies, this collider will provide opportunities to study muon and proton beam acceleration, investigate charged particle interactions with extreme electromagnetic fields (relevant for beam delivery system designs and to study the physics at the interaction point), as well as precision Quantum Chromodynamics and Beyond the Standard Model physics measurements. Possible applications of this collider include the studies of $\gamma\gamma$ and $e$-ion collider designs.

43 PARTICLE ACCELERATORS↗
DOE OSTI2022

Accelerator and Beam Physics: Grand Challenges and Research Opportunities

Accelerator and beam physics (ABP) is the science of the motion, generation, acceleration, manipulation, prediction, observation and use of charged particle beams. It focuses on fundamental long-term accelerator and beam physics research and development. Accelerator and beam physics research has resulted in important advances in accelerator science, yet support for this research is declining. NSF has terminated its program in accelerator Science and funding by DOE through GARD and Accelerator Stewardship has been steady or declining. The declining support for accelerator research will slow advances and threaten student training and work-force development in accelerator science. We propose a robust and scientifically challenging program in accelerator and beam physics, which will position the field of US High Energy Physics to be productive and competitive for decades to come.

43 PARTICLE ACCELERATORS↗
DOE OSTI2022

Harmonic combiner and divider

The harmonic combiner and divider efficiently combines multiple harmonic signals onto a common transmission line. Combined harmonic signals can be used to generate fast, high-fidelity arbitrary waveforms by superimposing the harmonics described in their Fourier series. Fast arbitrary waveforms have applications in communications, radar, and can be used for manipulating and controlling charged particle beams. The harmonic combiner and divider also efficiently divides fast arbitrary waveforms into their constituent harmonics and provides an efficient mechanism for waveform analysis and for multi-channel communications.

Roberts, Brock Franklin↗
DOE OSTI2022

Rare Higgs Processes at CMS and Precision Timing Detector Studies for HL-LHC CMS Upgrade

This thesis describes the search for two rare Higgs processes. The first analysis describes the CMS Run 2 search for $H$ $\rightarrow$ $\mu$$\mu$ decays, with 137.3 fb$^{-1}$ of data at $\sqrt{s}$ = 13 TeV. The analysis targeted four different Higgs production modes: the gluon fusion (ggH), the vector boson fusion (VBF), the Higgs-strahlung process (VH), and the production in association with a pair of top quarks (ttH). Each category used a dedicated machine learning based classifier to separate the signal from the background processes. A combined fit from all these categories saw a slight excess in the data corresponding to 3.0 standard deviations at $M$$_{H}$ = 125.38 GeV, and gave the first evidence for the Higgs boson decay to second-generation fermions. The best-fit signal strength and the corresponding 68% CL interval was found to be +0.17?????? = 1.19 $_{-0.39}^{+0.41}$ (stat)$_{-0.16}^{+0.17}$(syst) at $M$$_{H}$ = 125.38 GeV. The second analysis describes the CMS Run 2 search for 𝐻𝐻 → 𝑏𝑏𝑏𝑏 with highly boosted Higgs bosons. This analysis used a dedicated jet identification algorithm based on graph neural networks (ParticleNet) to identify boosted H→ bb jets. This search targeted the gluon fusion and the vector boson fusion HH production modes, and put constraints on the allowed values of the various Higgs couplings as: 𝜅𝜆 ∈ [−9.9, 16.9] when 𝜅𝑉 = 1, 𝜅2𝑉 = 1; 𝜅𝑉 ∈ [−1.17, −0.79] ∪ [0.81, 1.18] when 𝜅𝜆 = 1, 𝜅2𝑉 = 1; 𝜅2𝑉 ∈ [0.62, 1.41] when 𝜅𝜆 = 1, 𝜅𝑉 = 1. A scenario with 𝜅2𝑉 = 0 was excluded with a significance of 6.3 standard deviations for the first time, when other H couplings are fixed to their SM values. The combined observed (expected) 95% upper limit on the HH production cross section was found to be 9.9 (5.1) × SM. Finally, this thesis also discusses the planned MIP Timing Detector (MTD) upgrade for CMS at the HL-LHC. The MTD will be a time-of-flight (TOF) detector, designed to provide a precision timing information for charged particles using SiPMs + LYSO scintillating crystals, with a time resolution of ∼30 ps. This thesis describes several R&D tests that have been performed for characterizing the sensor properties (time resolution, light yield, etc.) and optimizing the sensor design geometry. This thesis also contains a description of mock test setups for cooling the sensors, since it is known to be an effective way of mitigating the increased dark current rates in the sensors due to radiation damage.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2023

Compact Multicell Superconducting Crab Cavity for ILC

We propose a novel design of a crab cavity (CC) for the ILC project with low parasitic High Order Modes (HOM) losses and preserving the beam emittance, which is critical for operation with high beam current intensity. Multiple electrodes immersed in the hollow waveguide form a trapped-mode resonator. The transverse components of the electromagnetic field of the trapped dipole mode induce a transverse kick and efficiently deflect charged particles passing through the cavity. We present a scalable design of a superconducting Quasi-waveguide Multicell Resonator (QMiR) seamlessly connected with a beam vacuum chamber. The cavity is completely open at both ends, which significantly reduces the maximum loaded quality factor of the higher order modes (HOM), avoids complex HOM couplers, and thus simplifies the mechanical design of the cavity. The same port is used to feed RF power to the operating mode and to extract the same order modes (SOM). Finally, we estimate the expected cryogenic losses, HOM impedance limits, RF input power required, and frequency tuning for a QMiR cavity designed to operate at 2.6 GHz.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2023

Flash radiotherapy accelerator

Methods, devices and systems for ultra-high dose radiotherapy are disclosed. The described techniques rely in-part on active switching control of a photoconductive switch during the time the accelerator is accelerating charged particles to produce the output radiation at the desired dose rates. One flash radiotherapy system includes an induction accelerator, and a controllable switch coupled to the induction accelerator. The switch is operable to produce a plurality of voltage pulses to drive the induction accelerator. The radiotherapy system also includes a radiation measurement device to measure output radiation produced by the radiotherapy system and provide feedback to the controllable switch. The controllable switch is operable to, based on the received feedback, modify an amplitude, shape, spacing, number or width of the voltage pulses that are supplied to the particle accelerator to deliver the desired output radiation.

Sampayan, Stephen E.↗
DOE OSTI2022

High-order diamond differencing schemes for the Boltzmann Fokker-Planck equation in 3D Cartesian geometries

The Boltzmann Fokker-Planck, an approximate form of the linear Boltzmann equation is commonly used to treat efficiently the transport of charged particles in matter. This paper introduces the application of high-order diamond differencing schemes (HODD), specifically the DD1 and DD2 schemes which are 4- and 6-order accurate respectively, to handle the spatial discretization of that equation in 3D Cartesian geometries. The energy deposition solutions for the coupled transport of electrons and photons presented in this work shows that HODD, compared to classical DD scheme, provides correction to the oscillations and a reduced propensity to yield negative fluxes. They are useful tools to minimize local error, notably in regions with abrupt variations of the flux solution. They also can be used to reduced execution time by decreasing the needed number of voxels to obtain a fixed accuracy. On the tested benchmarks, the DD1 scheme is 87%- 92%-91% more accurate than the classical DD scheme for total, mean per-voxels and maximum deviation of energy deposition values respectively. For comparison, a calculation with 8 times more voxels, requiring roughly 2.5 times more time to execute, is 92%-90%-77% more accurate. (authors)

97 MATHEMATICS AND COMPUTING↗
DOE OSTI2024

Probing the Isospin Composition of Short-Range Correlated Pairs at Jefferson Lab Hall B

Nucleons in short-range correlated (SRC) pairs, due to their close proximity and high relative momentum, can provide insight into the short-range part of the strong nuclear interaction. In particular, the prevalence of np pairs is due to the dominance of a tensor term for correlated nucleons with momenta of approximately 400?600 MeV/c. This dissertation comprises two studies advancing the community?s understanding of the isospin composition of SRC pairs. First, I performed a study of proton and neutron knockout from initially low-momentum and high-momentum states in 3He. Previous work has shown that protons are disproportionately represented in high-momentum states in neutron-rich nuclei. I demonstrate that spectral functions for the proton-rich nucleus 3He predict, in agreement with data, that neutrons are disproportionately represented in high-momentum states, but that 3He does not display the same strong prevalence of np pairs that is observed in larger nuclei. Second, Generalized Contact Formalism (GCF), a well-supported theory for predicting SRC behavior, predicts the transition from an isospin-dependent, tensor-dominant interaction at intermediate distances to a scalar-dominant, isospin-independent interaction at very short distances. This dissertation uses data from the CLAS12 Nuclear Targets Experiments in Hall B at Jefferson Lab to measure the relative abundances of pp and pn pairs for increasing relative momentum and decreasing separation. I provide an independent confirmation of the previously-observed increase in pp pairs at increasing momentum of the struck nucleon. I also contribute to the application of the new CLAS12 Central Neutron Detector by precisely measuring the neutron detection efficiency and developing a machine learning model for rejecting charged particle background.

Seroka, Erin↗
DOE OSTI2025

Analysis and Validation of PMT s Waveforms in ICARUS LArTPC Using Monte Carlo Simulations

ICARUS (Imaging Cosmic and Rare Underground Signals) serves as the Far Detector in the Short Baseline Neutrino (SBN) program at Fermilab, playing a central role in investigating the potential existence of sterile neutrinos in the eV squared mass range. The detector consists of two large Liquid Argon Time Projection Chambers (LArTPCs) with a total capacity of 760 tons of liquid Argon. A key component of the system is its array of 360 Photo-Multiplier Tubes (PMTs), which detect the scintillation light produced by charged particles in liquid Argon; the fast scintillation signal enables accurate event timing, triggering, and reconstruction. Together with the TPC and CRT systems, the PMTs ensure precise interaction time measurements, which are crucial for distinguishing neutrino interactions from cosmic-ray backgrounds. ICARUS uses Hamamatsu R5912-MOD PMTs, optimized for cryogenic temperatures, with high quantum efficiency, excellent timing resolution, low dark current (around 10 nA at 1500 V), and broad spectral sensitivity (300–650 nm). These characteristics are crucial for the efficient detection of scintillation light. Analyzing the waveforms of PMT signals allows for a detailed comparison between experimental data and Monte Carlo simulations. This analysis is fundamental for improving the accuracy of neutrino event reconstruction, enhancing detector calibration, and optimizing the detector's performance for current and future operations.

Brio, V. [Catania U.] (ORCID:0009000088807391)↗
DOE OSTI2025

First Measurement of $π^+$-Ar and $p$-Ar Total Inelastic Cross Sections in the Sub-GeV Energy Regime with ProtoDUNE-SP Data

The ProtoDUNE-SP detector, a kiloton-scale prototype for the Deep Underground Neutrino Experiment (DUNE), is the largest liquid argon time projection chamber built to date. Operated at CERN from 2018 to 2020, it collected both cosmic-ray data and a beam consisting of positively-charged particles with discrete momentum settings across a range of 0.3 GeV/$c$ to 7 GeV/$c$. In this letter, we report the total inelastic cross section measurements for $π^+$-Ar and $p$-Ar interactions using selected $π^+$ and proton samples from the 1 GeV/$c$ beam data. These results provide the first measurement of the total inelastic cross sections for $π^+$-Ar in the 500-900 MeV kinetic energy range and for $p$-Ar below 450 MeV, both of which are directly relevant to the DUNE energy range. The measured cross sections are consistent with predictions and provide a dataset that was previously unavailable for argon targets. These measurements are essential for constraining neutrino-argon interaction models, which are crucial for the precision physics goals of the upcoming DUNE experiment.

Abbaslu, Saeed [IPM, Tehran] (ORCID:00000003356771↗
DOE OSTI2026

Experimental Studies of Nonlinear Integrable Optics with Elliptic Potentials

The stable transport of charged particle beams is the core challenge in designing and operating accelerators. The current paradigm for transverse focusing is based on quadrupole and dipole elements, described as a linear integrable Hamiltonian by Courant and Snyder. The operational limits of high intensity accelerators are often determined by collective instabilities within the beam. Nonlinear elements may be added to suppress certain forms of these collective effects, but restrict the range of stable trajectories. These shortcomings motivate extending to a nonlinear integrable system which can offer the benefits of suppressing collective instabilities without limiting the stable trajectories. Danilov and Nagaitsev proposed a novel nonlinear integrable system with elliptical potentials, which could be implemented as magnetic elements in an accelerator. Such a system has been implemented for practical verification in the integrable optics test accelerator (IOTA), a small storage ring constructed for beam dynamics studies. Electron beam studies in IOTA treat the low-emittance beam as a macroparticle for detailed probing of the expected single particle dynamics. This dissertation details new measurements of the nonlinear integrable system relevant for practical implementation. Turn-by-turn measurements of the kicked beam responses are used for phase space reconstruction and analysis of the predicted nonlinear dynamics. The stability and aperture for various nonlinear configurations are measured with beam losses. Amplitude dependent detuning, a core figure of merit for suppressing instabilities, is measured and compared with high fidelity particle tracking simulations. The synchrotron radiation images of circulating beam allow direct measurements of the topology and lifetime in configurations where nonlinear focusing terms dominate.

Wieland, John [Michigan U.] (ORCID:000000028971852↗
DOE OSTI2026

Neutrino beam bunch structure reconstruction with precision timing in the ICARUS liquid argon time projection chamber

The ICARUS detector has been operating smoothly since 2021 as the far detector in the Short Baseline Neutrino (SBN) program at Fermilab, collecting neutrino interactions from both the Booster Neutrino Beam (BNB) and off-axis from the Neutrinos at the Main Injector (NuMI) beam. Analysis of neutrino interactions in ICARUS requires mitigation of substantial cosmogenic backgrounds. This is achieved by using an external Cosmic Ray Tagger (CRT) and a Photomultiplier Tube (PMT) system embedded in the liquid argon. The intrinsic neutrino beam bunch structure, inherited time structure from the Radio Frequency (RF) system used to accelerate the protons, can be resolved at the ICARUS detector using precise timing information. Located at shallow depth, ICARUS is exposed to a high flux of cosmic rays that can be mistaken for neutrino interactions. To mitigate this background, the CRT and a 3-meter-thick concrete overburden were installed. To better model backgrounds, ICARUS makes use of an overlay technique where simulated neutrino events are superimposed on detector beam-off data. PMTs installed within a Time Projection Chamber detect argon scintillation light emitted by high energy charged particles passing through the chamber and provide the event timing of neutrino interactions. The nanosecond-level beam bunch structure is reconstructed with the PMT system and can be used to further understand backgrounds and enhance neutrino physics capabilities. In this thesis, I will discuss background mitigation techniques using precision timing and present a novel technique to select neutrino events from our unbiased data stream using the beam bunch structure.

Heggestuen, Anna [Colorado State U.] (ORCID:000000↗
DOE OSTI2026

Longitudinal Phase Space Tomography for the Booster Synchrotron

Efforts in the study of the longitudinal behavior of charged particles in the Fermilab Booster can be catalyzed with an image of the two-dimensional phase space distribution. In the past, tomography had been employed in the reconstruction of the phase space in accelerators such as the Recycler at Fermilab and the Proton Synchrotron Booster at CERN. However, such a capability had yet to realize for the Fermilab Booster synchrotron. In this work, the first successful tomographic phase space reconstruction of a low-energy Booster bunch is presented along with validation metrics. A numerical turn-by-turn model of the longitudinal particle dynamics in the Booster has been implemented, which utilizes a fast, map-based particle transport algorithm. Using a sinogram generated from the Wall Current Monitor signal, the iterative reconstruction algorithm recovers a discretized image of the original phase space distribution at variable resolution. The reconstruction result shows low root-mean-square error and a rapid convergence toward the solution, providing strong evidence of accuracy. Future and ongoing work includes modeling high-energy bunches above transition and using tomography to infer certain machine parameters such as synchronous phase, peak gap voltage, and synchronous energy in addition to the phase space distribution.

Ebeid, Safi [Unlisted; Fermilab]↗
DOE OSTI2026

Characterizing the Electromagnetic Response of the NOvA Detectors

The NOvA Test Beam Program was commissioned to complement the full-scale NOvA experiment in its goal of measuring neutrino oscillations. The NOvA Experiment consists of a 300-ton Near Detector and a 14-kton Far Detector, both exposed to the same beam, which can be operated in neutrino or antineutrino mode from Fermilab at an off-axis angle of 14.6~mrad. These detectors can discriminate between $\nu_\mu$-CC and $\nu_e$-CC neutrino (or corresponding antineutrino) events, enabling appearance and disappearance measurements of these flavors across the \SI{810}{\kilo\meter} near-to-far detector baseline. From these measurements, the underlying parameters of the three-flavor PMNS oscillations framework are measured. The NOvA Test Beam uses identical technology to the full-scale detectors, but scaled down to 30~tons. It is exposed to a beam of charged particles closely matched to the daughter products of NOvA (anti)neutrino interactions in both energy and species. An instrumented beamline determines both particle momentum and species upstream of the NOvA detector, allowing for a crisp measurement of the NOvA detector response to these known inputs. This dissertation presents an analysis of the electromagnetic response of the NOvA hardware and establishes a framework for incorporating these results to enhance the physics reach of the experiment. Prior to this work, the electromagnetic energy response of the NOvA detector relied primarily on simulation-driven calibration together with a globally applied energy scale uncertainty. The measurements presented here provide direct test beam constraints on the detector response, enabling particle-dependent and potentially energy-dependent uncertainty models derived from controlled electromagnetic inputs.

Myers, Dalton Grant [U. Texas, Austin (main)] (ORC↗
DOE OSTI2022

Nanoscale Measurements of Charge Transfer at Cocatalyst/Semiconductor Interfaces in BiVO 4 Particle Photocatalysts

Semiconductor photocatalyst particles convert solar energy to fuels like H 2 . The particles are often assumed to provide crystalline-facet-dependent electron-hole separation. A common strategy is to deposit HER electrocatalyst on electron-selective facets and OER electrocatalyst on hole-selective facets. A precise understanding of how charge-carrier-selective contacts emerges and how they rationally designed, however, is missing. Using a combination of ex-situ and in-situ conducting-AFM experiments and new ionomer/catalyst-semiconductor test structures, we show how heterogeneity in charge-carrier selectivity can be measured at the nanoscale. We discover that the presence of interface water/electrolyte is critical to induce hole selectivity between the CoO x water-oxidation catalyst and the BiVO 4 light absorber. pH-dependent measurements suggest that negative surface charge on the semiconductor is central to inducing hole selectivity. Furthermore, the work also demonstrates a new approach to control local pH and introduce water using thin-film ionomers compatible with conductive-AFM measurements.

14 SOLAR ENERGY↗
DOE OSTI2024

Colloidal Stability of PFSA-Ionomer Dispersions. Part I. Single-Ion Electrostatic Interaction Potential Energies

Charged colloidal particles neutralized by a single counterion are increasingly important for many emerging technologies. Attention here is paid specifically to hydrogen fuel cells and water electrolyzers whose catalyst layers are manufactured from a perfluorinated sulfonic acid polymer (PFSA) suspended in aqueous/alcohol solutions. Partially dissolved PFSA aggregates, known collectively as ionomers, are stabilized by the electrostatic repulsion of overlapping diffuse double layers consisting of only protons dissociated from the suspended polymer. We denote such double layers containing no added electrolyte as "single ion". Size-distribution predictions build upon interparticle interaction potential energies from the Derjaguin-Landau-Verwey-Overbeek (DLVO) formalism. However, when only a single counterion is present in solution, classical DLVO electrostatic potential energies no longer apply. Accordingly, here a new formulation is proposed to describe how single-counterion diffuse double layers interact in colloidal suspensions. Part II (Srivastav, H.; Weber, A. Z.; Radke, C. J. Langmuir 2024 DOI: 10.1021/acs.langmuir.3c03904) of this contribution uses the new single-ion interaction energies to predict aggregated size distributions and the resulting solution pH of PFSA in mixtures of n-propanol and water. A single-counterion diffuse layer cannot reach an electrically neutral concentration far from a charged particle. Consequently, nowhere in the dispersion is the solvent neutral, and the diffuse layer emanating from one particle always experiences the presence of other particles (or walls). Thus, in addition to an intervening interparticle repulsive force, a backside osmotic force is always present. With this new construction, we establish that single-ion repulsive pair interaction energies are much larger than those of classical DLVO electrostatic potentials. The proposed single-ion electrostatic pair potential governs dramatic new dispersion behavior, including dispersions that are stable at a low volume fraction but unstable at a high volume fraction and finite volume-fraction dispersions that are unstable with fine particles but stable with coarse particles. Finally, the proposed single-counterion electrostatic pair potential provides a general expression for predicting colloidal behavior for any charged particle dispersion in ionizing solvents with no added electrolyte.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2021

Automated microbial detection and quantification

A method for automated microbial detection includes collecting air particles into a solid-state sampler, the air particles including microbes, charging the air particles using a plasma field generated by propulsion electrodes, focusing the charged air particles toward a sample well of a microfluidic testing cartridge, tagging the charged air particles with a fluorescence marker, and detecting a quantity of the microbes using a fluorescence detector.

Gilbert, James H.↗