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DOE OSTI2023

Feebly-interacting particles: FIPs 2022 Workshop Report

Particle physics today faces the challenge of explaining the mystery of dark matter, the origin of matter over anti-matter in the Universe, the origin of the neutrino masses, the apparent fine-tuning of the electro-weak scale, and many other aspects of fundamental physics. Perhaps the most striking frontier to emerge in the search for answers involves new physics at mass scales comparable to familiar matter, below the GeV-scale, or even radically below, down to sub-eV scales, and with very feeble interaction strength. New theoretical ideas to address dark matter and other fundamental questions predict such feebly interacting particles (FIPs) at these scales, and indeed, existing data provide numerous hints for such possibility. A vibrant experimental program to discover such physics is under way, guided by a systematic theoretical approach firmly grounded on the underlying principles of the Standard Model. This document represents the report of the FIPs 2022 workshop, held at CERN between the 17 and 21 October 2022 and aims to give an overview of these efforts, their motivations, and the decadal goals that animate the community involved in the search for FIPs.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2023

Feebly-Interacting Particles: FIPs 2022 Workshop Report

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2024

Solvent-Dependent Dynamics of Cellulose Nanocrystals in Process-Relevant Flow Fields

Flow-assisted alignment of anisotropic nanoparticles is a promising route for the bottom-up assembly of advanced materials with tunable properties. While aligning processes could be optimized by controlling factors such as solvent viscosity, flow deformation, and the structure of the particles themselves, it is necessary to understand the relationship between these factors and their effect on the final orientation. In this study, we investigated the flow of surface-charged cellulose nanocrystals (CNCs) with the shape of a rigid rod dispersed in water and propylene glycol (PG) in an isotropic tactoid state. In situ scanning small-angle X-ray scattering (SAXS) and rheo-optical flow-stop experiments were used to quantify the dynamics, orientation, and structure of the assigned system at the nanometer scale. The effects of both shear and extensional flow fields were revealed in a single experiment by using a flow-focusing channel geometry, which was used as a model flow for nanomaterial assembly. Due to the higher solvent viscosity, CNCs in PG showed much slower Brownian dynamics than CNCs in water and thus could be aligned at lower deformation rates. Moreover, CNCs in PG also formed a characteristic tactoid structure but with less ordering than CNCs in water owing to weaker electrostatic interactions. The results indicate that CNCs in water stay assembled in the mesoscale structure at moderate deformation rates but are broken up at higher flow rates, enhancing rotary diffusion and leading to lower overall alignment. Albeit being a study of cellulose nanoparticles, the fundamental interplay between imposed flow fields, Brownian motion, and electrostatic interactions likely apply to many other anisotropic colloidal systems.

36 MATERIALS SCIENCE↗

DOE OSTI2019

Probing the Fundamental Nature of Dark Matter with the Large Synoptic Survey Telescope

Astrophysical and cosmological observations currently provide the only robust, empirical measurements of dark matter. Future observations with Large Synoptic Survey Telescope (LSST) will provide necessary guidance for the experimental dark matter program. This white paper represents a community effort to summarize the science case for studying the fundamental physics of dark matter with LSST. We discuss how LSST will inform our understanding of the fundamental properties of dark matter, such as particle mass, self-interaction strength, non-gravitational couplings to the Standard Model, and compact object abundances. Additionally, we discuss the ways that LSST will complement other experiments to strengthen our understanding of the fundamental characteristics of dark matter. More information on the LSST dark matter effort can be found at https://lsstdarkmatter.github.io/ .

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2019

Light-Ferroic Interaction in Hybrid Organic–Inorganic Perovskites

Given the remarkable performance of hybrid organic–inorganic perovskites (HOIPs) in solar cells, light emitters, and photodetectors, the quest to advance the fundamental understanding of the photophysical properties in this class of materials remains highly relevant. Recently, the discovery of ferroic twin domains in HOIPs has renewed the debate of the ferroic effects on optoelectric processes. This work explores the interaction between light and ferroic twin domains in CH 3 NH 3 PbI 3 . Due to strain and chemical inhomogeneities, photogenerated electrons and holes show a preferential motion in the ferroelastic twin domains. Density functional theory (DFT) shows that electrons and holes result in lattice expansion in CH 3 NH 3 PbI 3 differently. Hence, light generates strain in the ferroelastic domains due to preferential photocarrier motion, leading to a screening of strain variation. X-ray diffraction studies verify the DFT simulations and reveal that the photoinduced strain is light intensity dependent, and the photoexcitation is a prerequisite of inducing strain by light. This work extends the fundamental understanding of light-ferroic interaction and offers guidance for developing functional devices.

36 MATERIALS SCIENCE↗

DOE OSTI2022

CoSyR: A novel beam dynamics code for the modeling of synchrotron radiation effects

The self-consistent nonlinear dynamics of a relativistic charged particle beam interacting with its complete self-fields is a fundamental problem underpinning many of the accelerator design issues in high brightness beam applications, as well as the development of advanced accelerators. Particularly, synchrotron radiation induced effects in a magnetic dispersive beamline element can lead to collective beam instabilities and emittance growth. A novel beam dynamics code is developed based on a Lagrangian method for the calculation of the particles’ radiation near-fields using wavefront/wavelet meshes via the Green’s function of the Maxwell equations. These fields are then interpolated onto a moving mesh for dynamic update of the beam. This method allows radiation co-propagation and self-consistent interaction with the beam in 2D/3D simulations at greatly reduced numerical errors. Multiple levels of parallelisms are inherent in this method and implemented in our code CoSyR to enable at-scale simulations of nonlinear beam dynamics on modern computing platforms using MPI, multi-threading, and GPUs. Here, the current 2D implementation of CoSyR has been used to evaluate the transverse and longitudinal coherent radiation effects on the beam and to investigate beam optics designs proposed for mitigation of beam brightness degradation in a magnetic bunch compressor. In this paper, the design of CoSyR, as well as the benchmark with other coherent synchrotron radiation models, are described and discussed. Extension of the core algorithms to 3D is possible and planned.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DOE OSTI2015

Catalysis applications of size-selected cluster deposition

In this Perspective, we review recent studies of size-selected cluster deposition for catalysis applications performed at the U.S. DOE National Laboratories, with emphasis on work at Argonne National Laboratory (ANL) and Brookhaven National Laboratory (BNL). The focus is on the preparation of model supported catalysts in which the number of atoms in the deposited clusters is precisely controlled using a combination of gas-phase cluster ion sources, mass spectrometry, and soft-landing techniques. This approach is particularly effective for investigations of small nanoclusters, 0.5-2 nm (<200 atoms), where the rapid evolution of the atomic and electronic structure makes it essential to have precise control over cluster size. Cluster deposition allows for independent control of cluster size, coverage, and stoichiometry (e.g., the metal-to-oxygen ratio in an oxide cluster) and can be used to deposit on any substrate without constraints of nucleation and growth. Examples are presented for metal, metal oxide, and metal sulfide cluster deposition on a variety of supports (metals, oxides, carbon/diamond) where the reactivity, cluster-support electronic interactions, and cluster stability and morphology are investigated. Both UHV and in situ/operando studies are presented that also make use of surface-sensitive X-ray characterization tools from synchrotron radiation facilities. Novel applications of cluster deposition to electrochemistry and batteries are also presented. This review also highlights the application of modern ab initio electronic structure calculations (density functional theory), which can essentially model the exact experimental system used in the laboratory (i.e., cluster and support) to provide insight on atomic and electronic structure, reaction energetics, and mechanisms. As amply demonstrated in this review, the powerful combination of atomically precise cluster deposition and theory is able to address fundamental aspects of size-effects, cluster-support interactions, and reaction mechanisms of cluster materials that are central to how catalysts function. Lastly, the insight gained from such studies can be used to further the development of novel nanostructured catalysts with high activity and selectivity.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2021

Near-field imaging of plasmonic nanopatch antennas with integrated semiconductor quantum dots

Plasmonic nanopatch antennas that incorporate dielectric gaps hundreds of picometers to several nanometers thick have drawn increasing attention over the past decade because they confine electromagnetic fields to grossly sub-diffraction-limited volumes. Substantial control over the optical properties of excitons and color centers confined within these plasmonic cavities has already been demonstrated with far-field optical spectroscopies, but near-field optical spectroscopies are essential for an improved understanding of the plasmon–emitter interaction at the nanoscale. Here, we characterize the intensity and phase-resolved plasmonic response of isolated nanopatch antennas by cathodoluminescence microscopy. Furthermore, we explore the distinction between optical and electron beam spectroscopies of coupled plasmon–exciton heterostructures to identify constraints and opportunities for future nanoscale characterization and control of hybrid nanophotonic structures. While we observe substantial Purcell enhancement in time-resolved photoluminescence spectroscopies, negligible Purcell enhancement is observed in cathodoluminescence spectroscopies of hybrid nanophotonic structures. The substantial differences in measured Purcell enhancement for electron beam and laser excitation can be understood as a result of the different selection rules for these complementary experiments. Overall, these results provide a fundamentally new understanding of near-field plasmon–exciton interactions in nanopatch antennas, which is essential for myriad emerging quantum photonic devices.

36 MATERIALS SCIENCE↗

DOE OSTI2016

Matter power spectrum in hidden neutrino interacting dark matter models: a closer look at the collision term

Dark Matter (DM) models providing possible alternative solutions to the small-scale crisis of the standard cosmology are nowadays of growing interest. We consider DM interacting with light hidden fermions via well-motivated fundamental operators showing the resultant matter power spectrum is suppressed on subgalactic scales within a plausible parameter region. Our basic description of the evolution of cosmological perturbations relies on a fully consistent first principles derivation of a perturbed Fokker-Planck type equation, generalizing existing literature. The cosmological perturbation of the Fokker-Planck equation is presented for the first time in two different gauges, where the results transform into each other according to the rules of gauge transformation. Furthermore, our focus lies on a derivation of a broadly applicable and easily computable collision term showing important phenomenological differences to other existing approximations. As one of the main results and concerning the small-scale crisis, we show the equal importance of vector and scalar boson mediated interactions between the DM and the light fermions.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2015

Binding the diproton in stars: anthropic limits on the strength of gravity

We calculate the properties and investigate the stability of stars that burn via strong (and electromagnetic) interactions, and compare their properties with those that, as in our Universe, include a rate-limiting weak interaction. It has been suggested that, if the diproton were bound, stars would burn ∼10{sup 18} times brighter and faster via strong interactions, resulting in a universe that would fail to support life. By considering the representative case of a star in our Universe with initially equal numbers of protons and deuterons, we find that stable, 'strong-burning' stars adjust their central densities and temperatures to have familiar surface temperatures, luminosities and lifetimes. There is no 'diproton disaster'. In addition, strong-burning stars are stable in a much larger region of the parameter space of fundamental constants, specifically the strength of electromagnetism and gravity. The strongest anthropic bound on stars in such universes is not their stability, as is the case for stars limited by the weak interaction, but rather their lifetime. Regardless of the strength of electromagnetism, all stars burn out in mere millions of years unless the gravitational coupling constant is extremely small, α{sub G}∼< 10{sup −30}.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2017

PERIOD–COLOR AND AMPLITUDE–COLOR RELATIONS AT MAXIMUM AND MINIMUM LIGHT FOR RR LYRAE STARS IN THE SDSS STRIPE 82 REGION

Investigation of period–color (PC) and amplitude–color (AC) relations at the maximum and minimum light can be used to probe the interaction of the hydrogen ionization front (HIF) with the photosphere and the radiation hydrodynamics of the outer envelopes of Cepheids and RR Lyraes. For example, theoretical calculations indicated that such interactions would occur at minimum light for RR Lyrae and result in a flatter PC relation. In the past, the PC and AC relations have been investigated by using either the ( V − R ){sub MACHO} or ( V − I ) colors. In this work, we extend previous work to other bands by analyzing the RR Lyraes in the Sloan Digital Sky Survey Stripe 82 Region. Multi-epoch data are available for RR Lyraes located within the footprint of the Stripe 82 Region in five ( ugriz ) bands. We present the PC and AC relations at maximum and minimum light in four colors: ( u − g ){sub 0}, ( g − r ){sub 0}, ( r − i ){sub 0}, and ( i − z ){sub 0}, after they are corrected for extinction. We found that the PC and AC relations for this sample of RR Lyraes show a complex nature in the form of flat, linear or quadratic relations. Furthermore, the PC relations at minimum light for fundamental mode RR Lyrae stars are separated according to the Oosterhoff type, especially in the ( g − r ){sub 0} and ( r − i ){sub 0} colors. If only considering the results from linear regressions, our results are quantitatively consistent with the theory of HIF-photosphere interaction for both fundamental and first overtone RR Lyraes.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2014

Solving The Long-Standing Problem Of Nuclear Reactions At The Highest Microscopic Level: Annual Continuation And Progress Report

The aim of this project is to develop a comprehensive framework that will lead to a fundamental description of both structural properties and reactions of light nuclei in terms of constituent protons and neutrons interacting through nucleon-nucleon (NN) and three-nucleon (NNN) forces. This project will provide the research community with the theoretical and computational tools that will enable: (1) an accurate prediction for fusion reactions that power stars and Earth-based fusion facilities; (2) an improved description of the spectroscopy of exotic nuclei, including light Borromean systems; and (3) a fundamental understanding of the three-nucleon force in nuclear reactions and nuclei at the drip line. To achieve this goal, we build upon a promising technique emerged recently as a candidate to reach a fundamental description of low-energy binary reactions between light ions, that is the ab initio no-core shell model combined with the resonating-group method (NCSM/RGM). This approach has demonstrated the capability to describe binary reactions below the three-body breakup threshold based, up to now, on similarity-renormalization-group (SRG) 5 evolved NN only potentials. To advance the understanding of nuclear reactions at low energies and light exotic nuclei, this project aims at extending the NCSM/RGM approach to include the full range of NNN interactions as well as the treatment of three-cluster bound and continuum states. Three-nucleon interactions are unavoidable components of a fundamental nuclear Hamiltonian obtained in a low-energy effective theory. In addition, three-nucleon force terms are induced by the SRG procedure and have to be taken into account for such a transformation to be unitary in many-body calculations. At the same time, the introduction of three-body cluster states is key to achieve a microscopic description of Borromean systems as well as three-body breakup reactions. This project will both enhance the fundamentality and enlarge the scope of our microscopic description of nuclear properties. A successful completion of this project will result in improved accuracy of the 3 He( 3 He,2p) 4 He and 3 He(α,γ) 7 Be reaction rates and consequently, in enhancement of the predictive capability of the standard solar model. In addition, we will study also the mirror reactions 3 H( 3 H,2n) 4 He and 3 H(α,γ) 7 Li (a key reaction for the production of 7 Li in the standard big-bang nucleosynthesis), and the spectroscopy of the 6 He, 6 Be, and 11 Li nuclei.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2023

Exchange-Driven Intermixing of Bulk and Topological Surface States by Chiral Excitons in Bi 2 Se 3

Topological surface states (TSS) in the prototypical topological insulator (TI) Bi 2 Se 3 are frequently characterized using optical probes, but electron-hole interactions and their effect on surface localization and optical response of the TSS remain unexplored. Here, we use ab initio calculations to understand excitonic effects in the bulk and surface of Bi 2 Se 3 . We identify multiple series of chiral excitons that exhibit both bulk and TSS character, due to exchange-driven mixing. Further, our results address fundamental questions about the degree to which electron-hole interactions can relax the topological protection of surface states and dipole selection rules for circularly polarized light in TIs by elucidating the complex intermixture of bulk and surface states excited in optical measurements and their coupling to light.

42 ENGINEERING↗

DOE OSTI2017

A Laboratory Astrophysical Jet to Study Canonical Flux Tubes

Understanding the interaction between plasma flows and magnetic fields remains a fundamental problem in plasma physics, with important applications to astrophysics, fusion energy, and advanced space propulsion. For example, flows are of primary importance in astrophysical jets even if it is not fully understood how jets become so long without becoming unstable. Theories for the origin of magnetic fields in the cosmos rely on flowing charged fluids that should generate magnetic fields, yet this remains to be demonstrated experimentally. Fusion energy reactors can be made smaller with flows that improve stability and confinement. Advanced space propulsion could be more efficient with collimated and stable plasma flows through magnetic nozzles but must eventually detach from the nozzle. In all these cases, there appears to be a spontaneous emergence of flowing and/or magnetic structures, suggesting a form of self-organization in plasmas. Beyond satisfying simple intellectual curiosity, understanding plasma self-organization could enable the development of methods to control plasma structures for fusion energy, space propulsion, and other applications. The research project has therefore built a theory and an experiment to investigate the interaction between magnetic fields and plasma flows. The theory is called canonical field theory for short, and the experiment is called Mochi after a rice cake filled with surprising, yet delicious fillings.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2020

Design of High-Performance Photon-Number-Resolving Photodetectors Based on Coherently Interacting Nanoscale Elements

A number of applications in basic science and technology would benefit from high-fidelity photon-number-resolving photodetectors. While some recent experimental progress has been made in this direction, the requirements for true photon number resolution are stringent, and no design currently exists that achieves this goal. Here we employ techniques from fundamental quantum optics to demonstrate that detectors composed of subwavelength elements interacting collectively with the photon field can achieve high-performance photon number resolution. We propose a new design that simultaneously achieves photon number resolution, high efficiency, low jitter, low dark counts, and high count rate. Finally, we discuss specific systems that satisfy the design requirements, pointing to the important role of nanoscale device elements.

47 OTHER INSTRUMENTATION↗

DOE OSTI2014

MO-E-18C-02: Hands-On Monte Carlo Project Assignment as a Method to Teach Radiation Physics

Purpose: To present a hands-on project on Monte Carlo methods (MC) recently added to the curriculum and to discuss the students' appreciation. Methods: Since 2012, a 1.5 hour lecture dedicated to MC fundamentals follows the detailed presentation of photon and electron interactions. Students also program all sampling steps (interaction length and type, scattering angle, energy deposit) of a MC photon transport code. A handout structured in a step-by-step fashion guides student in conducting consistency checks. For extra points, students can code a fully working MC simulation, that simulates a dose distribution for 50 keV photons. A kerma approximation to dose deposition is assumed. A survey was conducted to which 10 out of the 14 attending students responded. It compared MC knowledge prior to and after the project, questioned the usefulness of radiation physics teaching through MC and surveyed possible project improvements. Results: According to the survey, 76% of students had no or a basic knowledge of MC methods before the class and 65% estimate to have a good to very good understanding of MC methods after attending the class. 80% of students feel that the MC project helped them significantly to understand simulations of dose distributions. On average, students dedicated 12.5 hours to the project and appreciated the balance between hand-holding and questions/implications. Conclusion: A lecture on MC methods with a hands-on MC programming project requiring about 14 hours was added to the graduate study curriculum since 2012. MC methods produce “gold standard” dose distributions and slowly enter routine clinical work and a fundamental understanding of MC methods should be a requirement for future students. Overall, the lecture and project helped students relate crosssections to dose depositions and presented numerical sampling methods behind the simulation of these dose distributions. Research funding from governments of Canada and Quebec. PP acknowledges partial support by the CREATE Medical Physics Research Training Network grant of the Natural Sciences and Engineering Research Council (Grant number: 432290)

07 ISOTOPE AND RADIATION SOURCES↗

DOE OSTI2026

ELECTRON SHOWER RECONSTRUCTION IN THE ICARUS EXPERIMENT

This dissertation presents a study in the field of neutrino physics. Neutrinos are fundamental particles that are electrically neutral and have extremely small mass, allowing them to traverse matter with very little interaction. Because of this property, neutrinos are exceptionally difficult to detect. Nevertheless, understanding their behavior is essential for addressing fundamental questions about the origin of the Universe and the properties of matter. This work focuses on the reconstruction of electron showers produced by interactions of electron neutrinos (𝜈𝑒) in the ICARUS experiment, located at the Fermi National Accelerator Laboratory in the United States. ICARUS employs a liquid argon time projection chamber detector, which is capable of recording with high precision the tracks left by particles produced in neutrino interactions. The main objective of this research is to improve the reconstruction algorithms and techniques used to identify and characterize these electron showers, enhancing metrics such as completeness, defined as the fraction of correctly reconstructed signals, and purity, which quantifies how much of the reconstructed signal truly belongs to the candidate event. These improvements are crucial for reducing false positives and increasing the accuracy of electron photon discrimination. Consequently, this work directly contributes to improved neutrino oscillation analyses and to a deeper understanding of neutrino properties.

Salmoria, Gabrieli [Parana Tech. Fed. U., Toledo]↗

DOE OSTI2026

Cooperative spin coupling in PrFeO3

A transition from crystal-field to spin wave excitations has been experimentally observed in PrFeO3 using inelastic neutron scattering. Theoretical modeling with density functional theory and the mean field random phase approximation successfully reproduces the experimental observations and allows extraction of the values for the various exchange interactions. The study reveals that the strong coupling between the two magnetic sublattices of Pr and Fe is the fundamental mechanism underlying the low-temperature Pr magnetism. This coupling, analogous to the Dicke cooperative interaction between atoms and photons, polarizes the Pr moments, enhances the Pr-Pr interactions, and contributes to the formation of a quasidoublet, leading to the transition from single-particle to collective excitations within the Pr sublattice. Furthermore, this coupling induces spin reorientation on the Fe sublattice. The manipulation of magnetic moments via spin waves is achievable through the coupling between different magnetic sublattices in a bulk material containing multiple magnetic ions.

Garlea, Vasile [ORNL] (ORCID:0000000253227271)↗