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At least 883 records · Page 49

Large-Eddy Simulations of Marine Boundary Layer Clouds Associated with Cold-Air Outbreaks during the ACTIVATE Campaign. Part I: Case Setup and Sensitivities to Large-Scale Forcings

Large-eddy simulation (LES) is able to capture key boundary layer (BL) turbulence and cloud processes. Yet, large-scale forcing and surface turbulent fluxes of sensible and latent heat are often poorly prescribed for LESs. We derive these quantities from measurements and reanalysis obtained for two cold-air outbreak (CAO) events during Phase I of the Aerosol Cloud Meteorology Interactions over the Western Atlantic Experiment (ACTIVATE) in February–March 2020. We study the two contrasting CAO cases by performing LES and test the sensitivity of BL structure and clouds to large-scale forcings and turbulent heat fluxes. Profiles of atmospheric state and large-scale divergence and surface turbulent heat fluxes obtained from ERA5 data agree reasonably well with those derived from ACTIVATE field measurements for both cases at the sampling time and location. Therefore, we adopt the time-evolving heat fluxes, wind, and advective tendencies profiles from ERA5 data to drive the LES. We find that large-scale thermodynamic advective tendencies and wind relaxations are important for the LES to capture the evolving observed BL meteorological states characterized by the hourly ERA5 data and validated by the observations. We show that the divergence (or vertical velocity) is important in regulating the BL growth driven by surface heat fluxes in LESs. The evolution of liquid water path is largely affected by the evolution of surface heat fluxes. The liquid water path simulated in LES agrees reasonably well with the ACTIVATE measurements. This study paves the path to investigate aerosol–cloud–meteorology interactions using LES informed and evaluated by ACTIVATE field measurements.

54 ENVIRONMENTAL SCIENCES↗

The temporal structure of RF radiation from lightning

Radiation from lightning in the RF band from 3-300 MHz has been examined. Simultaneous measurements were made of the RF radiation from lightning together with records of fast and slow field changes. Continuous analogue recordings were made with a system having 300 kHz of bandwidth in the RF channels. The temporal history of RF radiation of these frequencies consists of a sequence of discrete pulses. The data reveal a distinct pattern in the radiation which is independent of frequency and depends on the type of lightning flash: Cloud-to-ground flashes are characterized by an abrupt beginning associated with the stepped leader, whereas cloud-to-cloud flashes begin with a slower train of noise pulses more typical of the end of both types of flash. An exception to this pattern is cloud-to-ground flashes preceded by a breakdown phase, in which case the radiation begins like a cloud-to-cloud flash.

Levine, D. M.↗

Case study of a low-reflectivity pulsating microburst - Numerical simulation of the Denver, 8 July 1989, storm

An intense, low-reflectivity, and pulsating microburst event, detected on July 8, 1989 by the Low-Level Windshear Alert System north of Denver Stapleton Airport is described using a Terminal Area Simulation System (TASS) model (Proctor, 1987). This 3d nonhydrostatic cloud model includes parametrizations for both liquid- and ice-phase microphysics. Simulation results show that the dissipating cloud induces a type-1 pulsating microburst event, with at least three distinct microburst pulses over a period of 20 min. Virga from the dissipating cloud continued to maintain hazardous windshear for a period much longer than the typical lifetime of a single microburst.

Proctor, Fred H.↗

Large-Eddy Simulations of Marine Boundary-Layer Clouds Associated With Cold Air Outbreaks During the Activate Campaign – Part 1: Case Setup and Sensitivities to Large-Scale Forcings

Large-eddy simulation (LES) is able to capture key boundary-layer (BL) turbulence and cloud processes. Yet, large-scale forcing and surface turbulent fluxes of sensible and latent heat are often poorly prescribed for LES simulations. We derive these quantities from measurements and reanalysis obtained for two cold air outbreak (CAO) events during Phase I of the Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment (ACTIVATE) in February-March 2020. We study the two contrasting CAO cases by performing LES and test the sensitivity of BL structure and clouds to large-scale forcings and turbulent heat fluxes. Profiles of atmospheric state and large-scale divergence and surface turbulent heat fluxes obtained from the reanalysis data ERA5 agree reasonablywell with those derived fromACTIVATE field measurements for both cases at the sampling time and location. Therefore, we adopt the time evolving heat fluxes, wind and advective tendencies profiles from ERA5 reanalysis data to drive the LES.We find that large-scale thermodynamic advective tendencies and wind relaxations are important for the LES to capture the evolving observed BL meteorological states characterized by the hourly ERA5 reanalysis data and validated by the observations. We show that the divergence (or vertical velocity) is important in regulating the BL growth driven by surface heat fluxes in LES simulations. The evolution of liquid water path is largely affected by the evolution of surface heat fluxes. The liquid water path imulated in LES agrees reasonably well with the ACTIVATE measurements. This study paves the path to investigate aerosol-cloud-meteorology interactions using LES informed and evaluated by ACTIVATE field measurements.

Large-eddy simulation↗

Retrieval of Boundary Layer 3D Cloud Properties Using Scanning Cloud Radar and 3D Radiative Transfer

Retrievals of cloud optical and microphysical properties for boundary layer clouds, including those widely used by ASR investigators, frequently assume that clouds are sufficiently horizontally homogeneous that scattering and absorption (at all wavelengths) can be treated using one dimensional (1D) radiative transfer, and that differences in the field-of-view of different sensors are unimportant. Unfortunately, most boundary layer clouds are far from horizontally homogeneous, and numerous theoretical and observational studies show that the assumption of horizontal homogeneity leads to significant errors. The introduction of scanning cloud and precipitation radars at the U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) program sites presents opportunities to move beyond the horizontally homogeneous assumption. The primary objective of this project was to develop a 3D retrieval for warm-phase (liquid only) boundary layer cloud microphysical properties, and to assess errors in current 1D (non-scanning) approaches. Specific research activities also involved examination of the diurnal cycle of hydrometeors as viewed by ARM cloud radar, and continued assessment of precipitation impacts on retrievals of cloud liquid water path using passive microwaves.

54 ENVIRONMENTAL SCIENCES↗

Equatorial response to northeasterly cold surges as inferred from satellite cloud imagery

Daily convective activity in equatorial regions during Dec.-Jan., 1974-1975 was estimated from NOAA satellite data and composited in relation to the phase of cold surge episodes which then occured. Eastward and westward propagating cloud clusters displayed phase speeds of about 5 and 10 m/sec, respectively, and were generated near southwestern Borneo after a cold surge. Kelvin wave responses were indicated by confinement of the eastward-moving components to the equatorial region. Further, an analysis of symmetric and asymmetric characteristics showed that components symmetric with respect to the equator displayed a larger response amplitude, which was taken to mean that strongly trapped waves were generated from heat sources near the equator.

Lau, K.-M.↗

Quasar Rain: The Broad Emission Line Region as Condensations in the Warm Accretion Disk Wind

The origin of the broad emission line region (BELR) in quasars and active galactic nuclei is still unclear. I propose that condensations form in the warm, radiation-pressure-driven, accretion disk wind of quasars creating the BEL clouds and uniting them with the other two manifestations of cool (∼10{sup 4} K) gas in quasars, the low ionization phase of the warm absorbers (WAs) and the clouds causing X-ray eclipses. The cool clouds will condense quickly (days to years), before the WA outflows reach escape velocity (which takes months to centuries). Cool clouds form in equilibrium with the warm phase of the wind because the rapidly varying X-ray quasar continuum changes the force multiplier, causing pressure waves to move gas into stable locations in pressure–temperature space. The narrow range of two-phase equilibrium densities may explain the (luminosity){sup 1/2} scaling of the BELR size, while the scaling of cloud formation timescales could produce the Baldwin effect. These dense clouds have force multipliers of order unity and so cannot be accelerated to escape velocity. They fall back on a dynamical timescale (months to centuries), producing an inflow that rains down toward the central black hole. As they soon move at Mach ∼10–100 with respect to the WA outflow, these “raindrops” will be rapidly destroyed within months. This rain of clouds may produce the elliptical BELR orbits implied by velocity-resolved reverberation mapping in some objects and can explain the opening angle and destruction timescale of the narrow “cometary” tails of the clouds seen in X-ray eclipse observations. Some consequences and challenges of this “quasar rain” model are presented, along with several avenues for theoretical investigation.

79 ASTRONOMY AND ASTROPHYSICS↗

Clouds and their effects on spectroscopic observations

Data on spectroscopic phase curves of near IR CO2 is reviewed. The composition of the Venusian clouds is discussed. Some recent calculations on the variations in line profiles with different scattering and reflecting models are presented.

Young, L. D. G.↗

The Contribution of Water Ice Clouds to the Water Cycle in the North Polar Region of Mars: Preliminary Analysis

While it has long been known that Mars' north residual polar cap and the Martian regolith are significant sources of atmospheric water vapor, the amount of water vapor observed in the northern spring season by the Viking Mars Atmospheric Water Detector instrument (MAWD) cannot be attributed to cap and regolith sources alone. Kahn suggested that ice hazes may be the mechanism by which additional water is supplied to the Martian atmosphere. Additionally, a significant decrease in atmospheric water vapor was observed in the late northern summer that could not be correlated with the return of the cold seasonal C02 ice. While the detection of water ice clouds on Mars indicate that water exists in Mars' atmosphere in several different phases, the extent to which water ice clouds play a role in moving water through the Martian atmosphere remains uncertain. Work by Bass et. al. suggested that the time dependence of water ice cap seasonal variability and the increase in atmospheric water vapor depended on the polar cap center reaching 200K, the night time saturation temperature. Additionally, they demonstrated that a decrease in atmospheric water vapor may be attributed to deposition of water ice onto the surface of the polar cap; temperatures were still too warm at this time in the summer for the deposition of carbon dioxide. However, whether water ice clouds contribute significantly to this variability is unknown. Additional information is contained in original extended abstract.

Bass, D. S.↗

DEEPLY EMBEDDED PROTOSTELLAR POPULATION IN THE 20 km s{sup −1} CLOUD OF THE CENTRAL MOLECULAR ZONE

We report the discovery of a population of deeply embedded protostellar candidates in the 20 km s{sup −1} cloud, one of the massive molecular clouds in the Central Molecular Zone (CMZ) of the Milky Way, using interferometric submillimeter continuum and H{sub 2}O maser observations. The submillimeter continuum emission shows five 1 pc scale clumps, each of which further fragments into several 0.1 pc scale cores. We identify 17 dense cores, among which 12 are gravitationally bound. Among the 18 H{sub 2}O masers detected, 13 coincide with the cores and probably trace outflows emanating from the protostars. There are also 5 gravitationally bound dense cores without H{sub 2}O maser detection. In total, the 13 masers and 5 cores may represent 18 protostars with spectral types later than B1 or potentially growing more massive stars at earlier evolutionary stages, given the non-detection in the centimeter radio continuum. In combination with previous studies of CH{sub 3}OH masers, we conclude that the star formation in this cloud is at an early evolutionary phase, before the presence of any significant ionizing or heating sources. Our findings indicate that star formation in this cloud may be triggered by a tidal compression as it approaches pericenter, similar to the case of G0.253+0.016 but with a higher star formation rate, and demonstrate that high angular resolution, high-sensitivity maser, and submillimeter observations are promising techniques to unveil deeply embedded star formation in the CMZ.

79 ASTRONOMY AND ASTROPHYSICS↗

Use of Collocated KWAJEX Satellite, Aircraft, and Ground Measurements for Understanding Ambiguities in TRMM Radiometer Rain Profile Algorithm

Coordinated ground, aircraft, and satellite observations are analyzed from the 1999 TRMM Kwajalein Atoll field experiment (KWAJEX) to better understand the relationships between cloud microphysical processes and microwave radiation intensities in the context of physical evaluation of the Level 2 TRMM radiometer rain profile algorithm and uncertainties with its assumed microphysics-radiation relationships. This talk focuses on the results of a multi-dataset analysis based on measurements from KWAJEX surface, air, and satellite platforms to test the hypothesis that uncertainties in the passive microwave radiometer algorithm (TMI 2a12 in the nomenclature of TRMM) are systematically coupled and correlated with the magnitudes of deviation of the assumed 3-dimensional microphysical properties from observed microphysical properties. Re-stated, this study focuses on identifying the weaknesses in the operational TRMM 2a12 radiometer algorithm based on observed microphysics and radiation data in terms of over-simplifications used in its theoretical microphysical underpinnings. The analysis makes use of a common transform coordinate system derived from the measuring capabilities of the aircraft radiometer used to survey the experimental study area, i.e., the 4-channel AMPR radiometer flown on the NASA DC-8 aircraft. Normalized emission and scattering indices derived from radiometer brightness temperatures at the four measuring frequencies enable a 2-dimensional coordinate system that facilities compositing of Kwajalein S-band ground radar reflectivities, ARMAR Ku-band aircraft radar reflectivities, TMI spacecraft radiometer brightness temperatures, PR Ku-band spacecraft radar reflectivities, bulk microphysical parameters derived from the aircraft-mounted cloud microphysics laser probes (including liquid/ice water contents, effective liquid/ice hydrometeor radii, and effective liquid/ice hydrometeor variances), and rainrates derived from any of the individual ground, aircraft, or satellite algorithms applied to the radar or radiometer measurements, or their combination. The results support the study's underlying hypothesis, particularly in context of ice phase processes, in that the cloud regions where the 2a12 algorithm's microphysical database most misrepresents the microphysical conditions as determined by the laser probes, are where retrieved surface rainrates are most erroneous relative to other reference rainrates as determined by ground and aircraft radar. In reaching these conclusions, TMI and PR brightness temperatures and reflectivities have been synthesized from the aircraft AMPR and ARMAR measurements with the analysis conducted in a composite framework to eliminate measurement noise associated with the case study approach and single element volumes obfuscated by heterogeneous beam filling effects. In diagnosing the performance of the 2a12 algorithm, weaknesses have been found in the cloud-radiation database used to provide microphysical guidance to the algorithm for upper cloud ice microphysics. It is also necessary to adjust a fractional convective rainfall factor within the algorithm somewhat arbitrarily to achieve satisfactory algorithm accuracy.

Smith, Eric A.↗

Biogenic, urban, and wildfire influences on the molecular composition of dissolved organic compounds in cloud water

Organic aerosol formation and transformation occurs within aqueous aerosol and cloud droplets, yet little is known about the composition of high molecular weight organic compounds in cloud water. Cloud water samples collected at Whiteface Mountain, New York, during August-September 2014 were analyzed by ultra-high-resolution mass spectrometry to investigate the molecular composition of dissolved organic carbon, with a focus on sulfur- and nitrogen-containing compounds. Organic molecular composition was evaluated in the context of cloud water inorganic ion concentrations, pH, and total organic carbon concentrations to gain insights into the sources and aqueous-phase processes of the observed high molecular weight organic compounds. Cloud water acidity was positively correlated with the average oxygen : carbon ratio of the organic constituents, suggesting the possibility for aqueous acid-catalyzed (prior to cloud droplet activation or during/after cloud droplet evaporation) and/or radical (within cloud droplets) oxidation processes. Many tracer compounds recently identified in laboratory studies of bulk aqueous-phase reactions were identified in the cloud water. Organosulfate compounds, with both biogenic and anthropogenic volatile organic compound precursors, were detected for cloud water samples influenced by air masses that had traveled over forested and populated areas. Oxidation products of long-chain (C 10-12 ) alkane precursors were detected during urban influence. Influence of Canadian wildfires resulted in increased numbers of identified sulfur-containing compounds and oligomeric species, including those formed through aqueous-phase reactions involving methylglyoxal. Light-absorbing aqueous-phase products of syringol and guaiacol oxidation were observed in the wildfire-influenced samples, and dinitroaromatic compounds were observed in all cloud water samples (wildfire, biogenic, and urban-influenced). Overall, the cloud water molecular composition depended on air mass source influence and reflected aqueous-phase reactions involving biogenic, urban, and biomass burning precursors.

54 ENVIRONMENTAL SCIENCES↗

Chemical Imaging of Atmospheric Organic Particles in the Southern Great Plains Field Campaign Report

The main goal of this field project was to characterize the chemical and physical properties of atmospheric particles representative of the Southern Great Plains (SGP) environment to establish a relationship between the composition of aerosol particles and their atmospheric impacts. The specific research efforts were focused on in-depth microscopy studies of chemical and physical properties of atmospheric organic particles collected at the U.S. Department of Energy’s Atmospheric Radiation Measurement (ARM) SGP observatory. An array of novel molecular-level characterization and chemical imaging approaches were used to characterize chemical composition of particles and elucidate fundamental processes governing their atmospheric aging, evolution of chemical composition, optical properties, cloud formation ability, and implications for particle-cloud interactions – the most challenging problems relevant to predictive understanding of aerosol effects on climate.(1, 2) Atmospheric particles consist of a complex mixture of organic compounds with a wide range of molecular structures, morphologies, physical properties, and chemical reactivity. The chemical composition, morphology, and phase state of atmospheric particles are of crucial importance for understanding the formation and reaction mechanisms of particles, their atmospheric evolution, and their impact on climate. It is of great interest to understand how the chemical and morphological particle microstructure affects their physicochemical properties such as chemical reactivity, thermodynamics of gas-particle partitioning, phase separations inside individual particles, hygroscopicity, optical properties, and ability to form liquid droplets (cloud condensation nuclei) and ice crystals (ice nuclei) in clouds. The phase state of organic particles, which yet remains poorly understood, plays a key role in their physicochemical properties and has important implications in various atmospheric processes. Fundamental understanding of these physicochemical properties and their possible evolution in time requires advanced analytical approaches for chemical imaging of particles with a resolution on the scale of 10-100 nm.(3) Comprehensive characterization of the size-dependent chemical composition of individual particles collected at the site was carried out using advanced molecular-level characterization and imaging approaches to identify their possible sources and to correlate to their climatic properties.

Southern Great Plains, aerosols, HI-SCALE field ca↗

Cloud Shortwave Optical Properties

The data set consists of calibrated zenith shortwave spectral radiances (400-950 nm and 940-1665 nm) and cloud optical depth (COD) retrievals every 2 seconds. The field of view is 0.5 degree. Retrievals of cloud droplet effective radius and thermodynamic phase are currently experimental and done offline. Effective radius and phase are not in this data set.

54 ENVIRONMENTAL SCIENCES↗

STUDYING ATMOSPHERE-DOMINATED HOT JUPITER KEPLER PHASE CURVES: EVIDENCE THAT INHOMOGENEOUS ATMOSPHERIC REFLECTION IS COMMON

We identify three Kepler transiting planets, Kepler-7b, Kepler-12b, and Kepler-41b, whose orbital phase-folded light curves are dominated by planetary atmospheric processes including thermal emission and reflected light, while the impact of non-atmospheric (i.e., gravitational) processes, including beaming (Doppler boosting) and tidal ellipsoidal distortion, is negligible. Therefore, those systems allow a direct view of their atmospheres without being hampered by the approximations used in the inclusion of both atmospheric and non-atmospheric processes when modeling the phase-curve shape. We present here the analysis of Kepler-12b and Kepler-41b atmosphere based on their Kepler phase curve, while the analysis of Kepler-7b was already presented elsewhere. The model we used efficiently computes reflection and thermal emission contributions to the phase curve, including inhomogeneous atmospheric reflection due to longitudinally varying cloud coverage. We confirm Kepler-12b and Kepler-41b show a westward phase shift between the brightest region on the planetary surface and the substellar point, similar to Kepler-7b. We find that reflective clouds located on the west side of the substellar point can explain the phase shift. The existence of inhomogeneous atmospheric reflection in all three of our targets, selected due to their atmosphere-dominated Kepler phase curve, suggests this phenomenon is common. Therefore, it is also likely to be present in planetary phase curves that do not allow a direct view of the planetary atmosphere as they contain additional orbital processes. We discuss the implications of a bright-spot shift on the analysis of phase curves where both atmospheric and gravitational processes appear, including the mass discrepancy seen in some cases between the companion’s mass derived from the beaming and ellipsoidal photometric amplitudes. Finally, we discuss the potential detection of non-transiting but otherwise similar planets, whose mass is too small to show a gravitational photometric signal, but their atmosphere is reflective enough to show detectable phase modulations.

79 ASTRONOMY AND ASTROPHYSICS↗

Examining the Impacts of Microphysical-Dynamical Feedbacks on Convective Clouds in Different Aerosol Environments Using Enhanced Observational and Modeling Strategies

This project investigated how microphysical–dynamical feedbacks influence deep convective clouds across a range of aerosol conditions, storm lifecycles, and meteorological regimes, and how these sensitivities depend on the modeling framework used to represent convection and microphysics. Using the Aerosol, Cloud, Precipitation, and Climate (ACPC) Working Group model intercomparison simulations of isolated deep convection in the Houston region, we found a robust warm-phase aerosol response in most cloud-resolving models. Increased aerosol loading tended to suppress warm-rain production, increase cloud water, and reduce surface rainfall and near-surface evaporation. These impacts were typically strongest early in the convective lifecycle, with the largest aerosol-driven differences occurring during the first half of storm evolution. The ice-phase response, on the other hand, varied widely across modeling frameworks, and differed in sign, timing, and vertical structure. Ice microphysical pathways and parameterizations are therefore leading sources of uncertainty in aerosol–deep convection interactions. Theoretical analyses further suggested that aerosol-driven invigoration through cold-phase processes was much weaker than previously hypothesized for cold-based storms, and in warm-based storms could even reduce updraft strength. These results imply that any invigoration signal is more likely linked to warm-phase processes and peaks early in storm development.

54 ENVIRONMENTAL SCIENCES↗

Particle Cloud Combustion Experiment

Preparation of flight experiment designs is supported by experimental studies of acoustically induced mixing process, optical transmissivities of particle cloud distributions, wall saturation effects and their control through the use of electrically neutral flame tube materials and surfaces, and the pyrolysis-vaporization kinetics of selected organic particulates. Drop tower tests of stabilized particle cloud flames have allowed valuable comparison of g = 0 and g = 1 (upwards and downwards) stabilized flame propagation. These stabilized flame data will be valuable assists in dealing with the freely propagating particle cloud flame data anticipated through Space Shuttle experimentation. Supporting theoretical studies emphasize comprehensive flame propagation and extinction relations among premixed single phase (gaseous) flames and premixed particle cloud flames, for both stabilized and freely propagating flames.

Berlad, A. L.↗