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At least 883 records · Page 49

Biological particles and aerosol-cloud interactions in the Southern Great Plains

The United States Southern Great Plains (SGP) is the genesis for much of the warm season precipitation in the central and eastern United States. While atmospheric thermodynamics and large-scale dynamics play an important role in formation of precipitation, precipitation mechanisms are also sensitive to aerosols. Aerosols can suppress precipitation as cloud condensation nuclei (CCN) or act as ice nucleating particles (INP) in deep convective clouds. This project focused on understanding the role of primary biological aerosol particles (PBAP) in the region and its influence on cloud formation. Specifically, we focused on biological aerosol in the form of pollen, one type of PBAP that is emitted in large yet variable quantities from vegetation in the mid latitudes. Field observations provide evidence of pollen in the planetary boundary layer and pollen components in cloud droplets and fine particulate matter. Further, pollen grains can easily rupture when wet, forming smaller, sub pollen particles with sizes less than one micron. We evaluated the potential for PBAP events at the Department of Energy (DoE) SGP Atmospheric Radiation Measurement (ARM) research facility due to the rich dataset available. We also developed model simulations that accounted for pollen emission and the generation of sub pollen particles, which have been shown to be both cloud condensation nuclei and ice nucleating particles. The proposed work was designed to address the following questions: 1. What are the physical and chemical signatures of biological aerosol such as pollen in SGP ARM measurements? 2. What is the role of pollen-derived particles on deep convection and precipitation in the Central US? Using measurements from the DoE SGP ARM site and recent airborne campaigns, we evaluated the signatures of pollen and pollen-derived aerosols on optical properties, cloud properties and precipitation (Subba et al., 2021). We identified pollen-driven events over the data record and used the Weather Research and Forecasting Model with fully coupled chemistry (WRF-Chem) to conduct chemically realistic simulations of aerosols during and summer mesoscale convective events in the Southern Great Plains (Subba et al., in review). This work improved our understanding of the role of biological aerosol on clouds and precipitation in the Central United States and placed these results in context with anthropogenically-driven processes.

54 ENVIRONMENTAL SCIENCES↗

Smoke and Pollution Aerosol Effect on Cloud Cover

Pollution and smoke aerosols can increase or decrease the cloud cover. This duality in the effects of aerosols forms one of the largest uncertainties in climate research. Using solar measurements from Aerosol Robotic Network sites around the globe, we show an increase in cloud cover with an increase in the aerosol column concentration and an inverse dependence on the aerosol absorption of sunlight. The emerging rule appears to be independent of geographical location or aerosol type, thus increasing our confidence in the understanding of these aerosol effects on the clouds and climate. Preliminary estimates suggest an increase of 5% in cloud cover.

Kaufman, Yoram J.↗

Boundary conditions for the paleoenvironment: Chemical and physical processes in the pre-solar nebula

The first interstellar hydrocarbon ring, cyclopropenylidene (C3H2) is being studied. Both a survey of galactic sources in several C3H2 transitions and a more detailed study of a subset of these sources are under way. In the latter category is a study of the nearby cold dark cloud TMC-1, which is a potential formation site for solar type stars. A spectra is shown of seven rotational transitions which have been observed at the Five College Radio Astronomy Observatory. Three of these were detected for the first time in any astronomical source: the 3 sub 30 to 2 sub 21 transition at 216 GHz, the 2 sub 21 to 1 sub 10 transition at 122 GHz, and the 1 sub 11 to 0 sub 00 transition at 52 GHz. From the data it is apparent that C3H2 is quite spacially extended in typical interstellar molecular clouds, and that at least in TMC-1 it is one of the most abundant organic molecules.

Irvine, W. M.↗

Solar activity, magnetic clouds, and geomagnetic storms

Associational aspects of magnetic clouds and solar activity, and of magnetic clouds and geomagentic storms are described. For example, recent research has shown associations to exist between the launch of magnetic clouds directed Earthward from the Sun and, in particular, two forms of solar activity: flare-related, type II metric radio bursts and disappearing filaments (prominences). Furthermore, recent research has shown an association to exist between the onset of magnetic clouds on Earth and the initiation of geomagnetic storms. Based on these findings, STIP Intervals XV-XIX are examined for possible occurrences of Earthward-directed magnetic clouds.

Wilson, Robert M.↗

The unusual supernova SN1993J in the galaxy M81

Supernova 1993J in the galaxy M81 is the second-brightest type II supernova observed this century, surpassed only by SN1987A in the Large Magellanic Cloud. Here we report the evolution of the photometric and spectral properties of SN1993J for the first 50 d following its discovery. The behavior of this supernova is unusual, showing features typical of type II supernovae near the initial maximum, but with the strong helium lines characteristic of type Ib supernovae at later times. This implies that the progenitor star had an unusually thin hydrogen envelope (compared to normal type II progenitors), suggesting that significant mass loss had taken place before the explosion. Application of an expanding photosphere model to our data provides an estimate of the distance to the supernova of 2.6 +/- 0.4 Mpc, broadly consistent with the distance to M81 determined using Cepheid variable stars. Supernova models that more closely match the atypical spectral features of SN1993J may change the inferred distance, and should provide better constraints on the structure of the progenitor.

Schmidt, Brian P.↗

The Aerosol/Cloud/Ecosystems Mission (ACE)

The goals and measurement strategy of the Aerosol/Cloud/Ecosystems Mission (ACE) are described. ACE will help to answer fundamental science questions associated with aerosols, clouds, air quality and global ocean ecosystems. Specifically, the goals of ACE are: 1) to quantify aerosol-cloud interactions and to assess the impact of aerosols on the hydrological cycle and 2) determine Ocean Carbon Cycling and other ocean biological processes. It is expected that ACE will: narrow the uncertainty in aerosol-cloud-precipitation interaction and quantify the role of aerosols in climate change; measure the ocean ecosystem changes and precisely quantify ocean carbon uptake; and, improve air quality forecasting by determining the height and type of aerosols being transported long distances. Overviews are provided of the aerosol-cloud community measurement strategy, aerosol and cloud observations over South Asia, and ocean biology research goals. Instruments used in the measurement strategy of the ACE mission are also highlighted, including: multi-beam lidar, multiwavelength high spectra resolution lidar, the ocean color instrument (ORCA)--a spectroradiometer for ocean remote sensing, dual frequency cloud radar and high- and low-frequency micron-wave radiometer. Future steps for the ACE mission include refining measurement requirements and carrying out additional instrument and payload studies.

Schoeberl, Mark↗

Distribution functions of intergalactic clouds

Width spectrum data derived from high-redshift QSO Ly-alpha absorption lines are used to study the statistical properties of intergalactic clouds. Several theoretical distribution functions for size and density are derived and tested against observational data for two types of line broadening: thermal and cosmological. Good agreement was found between the theoretical distribution functions and the observational data when the clouds were thermally broadened, and when distribution functions for both cloud size and width have a nonzero width. Attempts to fit the data with a single radius or density distribution function were unsuccessful.

Sherman, R. D.↗

Magnetic cloud passage at Earth and associated substorm activity

An approach to the study of the solar wind-magnetosphere interaction by signal type, that is, by examining the effect in the magnetosphere of well defined interplanetary structures, is presented. Focus is on the response of the magnetosphere to interplanetary magnetic clouds. Among their properties are: the slow and smooth variation of the magnetic field vector, with fluctuation level well below common interplanetary values; the similarly well behaved bulk flow; the wide range of field and flow parameters; and the longevity of passage (1 to 2 days). If the magnetic cloud is oriented such that a long period of uninterruptedly northward pointing field is followed by a long interval of continuously southward pointing field, then the transition of the magnetosphere from a quiescent state (the 'ground state') to a very active state can be studied, the latter being sustained by continued forcing from the magnetic cloud. A synopsis of the main findings of a recent study in such an interaction is given, concentrating on the substorm activity attending the second part of cloud passage.

Farrugia, C. J.↗

Raindrop Size Spectrum in Deep Convective Regions of the Americas

This study compared drop size distribution (DSD) measurements on the surfaces, the corresponding properties, and the precipitation modes among three deep convective regions within the Americas. The measurement compilation corresponded to two sites in the midlatitudes: the U.S. Southern Great Plains and Córdoba Province in subtropical South America, as well as to one site in the tropics: Manacapuru in central Amazonia; these are all areas where intense rain-producing systems contribute to the majority of rainfall in the Americas’ largest river basins. This compilation included two types of disdrometers (Parsivel and 2D-Video Disdrometer) that were used at the midlatitude sites and one type of disdrometer (Parsivel) that was deployed at the tropical site. The distributions of physical parameters (such as rain rate R, mass-weighted mean diameter D m , and normalized droplet concentration N w ) for the raindrop spectra without rainfall mode classification seemed similar, except for the much broader N w distributions in Córdoba. The raindrop spectra were then classified into a light precipitation mode and a precipitation mode by using a cutoff at 0.5 mm h -1 based on previous studies that characterized the full drop size spectra. These segregated rain modes are potentially unique relative to previously studied terrain-influenced sites. In the light precipitation and precipitation modes, the dominant higher frequency observed in a broad distribution of N w in both types of disdrometers and the identification of shallow light precipitation in vertically pointing cloud radar data represent unique characteristics of the Córdoba site relative to the others. As a result, the co-variability between the physical parameters of the DSD indicates that the precipitation observed in Córdoba may confound existing methods of determining the rain type by using the drop size distribution.

54 ENVIRONMENTAL SCIENCES↗

Toward Exploring the Synergy Between Cloud Radar Polarimetry and Doppler Spectral Analysis in Deep Cold Precipitating Systems in the Arctic

The study of Arctic ice and mixed-phase clouds, which are characterized by a variety of ice particle types in the same cloudy volume, is challenging research. This study illustrates a new approach to qualitative and quantitative analysis of the complexity of ice and mixed-phase microphysical processes in Arctic deep precipitating systems using the combination of Ka-band zenith-pointing radar Doppler spectra and quasi-vertical profiles of polarimetric radar variables measured by a Ka/W-band scanning radar. The results illustrate the frequent occurrence of multimodal Doppler spectra in the dendritic/planar growth layer, where locally generated, slower-falling particle populations are well separated from faster-falling populations in terms of Doppler velocity. The slower-falling particle populations contribute to an increase of differential reflectivity (Z DR ), while an enhanced specific differential phase (K DP ) in this dendritic growth temperature range is caused by both the slower and faster-falling particle populations. Another area with frequent occurrence of multimodal Doppler spectra is in mixed-phase layers, where both populations produce Z DR and K DP values close to 0, suggesting the occurrence of a riming process. A Joint analysis of the Doppler spectra and the polarimetric radar variables provides important insight into the microphysics of snow formation and allows the separation of the contributions of ice of different habits to the values of reflectivity and Z DR .

54 ENVIRONMENTAL SCIENCES↗

High Semi-Volatile Organic Aerosol Contributions Associated with Ammonium Nitrate in the Coastal Urban Environment

Organic components often contribute 50% or more of the submicron aerosol mass in coastal urban environments, but their partitioning between the gas and particle phases is controlled by a complex mixture of unidentified organic compounds that are poorly constrained by observations. This study compares daily filter organic functional groups (OFG) with online organic mass fragments from La Jolla, California, as part of the Eastern Pacific Cloud Aerosol Precipitation Experiment (EPCAPE), quantifying the contributions of four types of non-volatile (NV) organic emission sources to the submicron composition. Daily filters retained only 0.79–0.98 µg/m3 NV submicron organic mass concentration, even though 1.8–1.9 µg/m3 non-refractory (NR) submicron organic mass concentration was measured online. The 62–64% of measured NR submicron organic mass concentration that exceeded what remained on the filters after 23-hr sampling is interpreted as semi-volatile, consistent with the moderate correlation of the NR NV difference to NR ammonium, NR nitrate, and biomass burning-related NV and NR organic factors. The association between semi-volatile organic components and ammonium nitrate likely results from both co-emission and co-evaporation. Size-resolved filter analysis showed that NV organic mass concentration accounts for 68% of NR organic mass concentration for 0.5–1 µm dry diameter but account for 9.0% for 0.18–0.5 µm dry diameter showing the differences in volatility between particle modes. Importantly, volatility of organic components was size-dependent Information Classification: General and associated with ammonium nitrate and biomass burning, providing guidance for constraining atmospheric aerosol properties in global models.

Pelayo, Christian↗

Revealing the Drag Instability in One-fluid Nonideal Magnetohydrodynamic Simulations of a 1D Isothermal C-shock

C-type shocks are believed to be ubiquitous in turbulent molecular clouds thanks to ambipolar diffusion. We investigate whether the drag instability in 1D isothermal C-shocks, inferred from the local linear theory of Gu & Chen, can appear in nonideal magnetohydrodynamic simulations. Two C-shock models (with narrow and broad steady-state shock widths) are considered to represent the typical environment of star-forming clouds. The ionization-recombination equilibrium is adopted for the one-fluid approach. In the 1D simulation, the inflow gas is continuously perturbed by a sinusoidal density fluctuation with a constant frequency. The perturbations clearly grow after entering the C-shock region until they start being damped at the transition to the post-shock region. We show that the profiles of a predominant Fourier mode extracted locally from the simulated growing perturbation match those of the growing mode derived from the linear analysis. Moreover, the local growth rate and wave frequency derived from the predominant mode generally agree with those from the linear theory. Therefore, we confirm the presence of the drag instability in simulated 1D isothermal C-shocks. We also explore the nonlinear behavior of the instability by imposing larger-amplitude perturbations to the simulation. We find that the drag instability is subject to wave steepening, leading to saturated perturbation growth. Issues concerning local analysis, nonlinear effects, one-fluid approach, and astrophysical applications are discussed.

79 ASTRONOMY AND ASTROPHYSICS↗

Activation of intact bacteria and bacterial fragments mixed with agar as cloud droplets and ice crystals in cloud chamber experiments

Biological particles, including bacteria and bacterial fragments, have beenof much interest due to the special ability of some to nucleate ice atmodestly supercooled temperatures. This paper presents results from a recentstudy conducted on two strains of cultivated bacteria which suggest thatbacterial fragments mixed with agar, and not whole bacterial cells, serve ascloud condensation nuclei (CCN). Due to the absence of whole bacteria cellsin droplets, they are unable to serve as ice nucleating particles (INPs) inthe immersion mode under the experimental conditions. Experiments wereconducted at the Aerosol Interaction and Dynamics in the Atmosphere (AIDA)cloud chamber at the Karlsruhe Institute of Technology (KIT) by injectingbacteria-containing aerosol samples into the cloud chamber and inducing cloudformation by expansion over a temperature range of -5 to -12 ° C.Cloud droplets and ice crystals were sampled through a pumped counterflowvirtual impactor inlet (PCVI) and their residuals were characterized with asingle particle mass spectrometer (miniSPLAT). The size distribution of theoverall aerosol was bimodal, with a large particle mode composed of intactbacteria and a mode of smaller particles composed of bacterial fragmentsmixed with agar that were present in higher concentrations. Results fromthree expansions with two bacterial strains indicate that the cloud dropletresiduals had virtually the same size distribution as the smaller particlesize mode and had mass spectra that closely matched those of bacterialfragments mixed with agar. The characterization of ice residuals that weresampled through an ice-selecting PCVI (IS-PCVI) also shows that the sameparticles that activate to form cloud droplets, bacteria fragments mixed withagar, were the only particle type observed in ice residuals. These resultsindicate that the unavoidable presence of agar or other growth media inall laboratory studies conducted on cultivated bacteria can greatlyaffect the results and needs to be considered when interpreting CCN and INactivation data.

54 ENVIRONMENTAL SCIENCES↗

The significant impact of aerosol vertical structure on lower atmosphere stability and its critical role in aerosol–planetary boundary layer (PBL) interactions

The aerosol–planetary boundary layer (PBL) interaction was proposed as an important mechanism to stabilize the atmosphere and exacerbate surface air pollution. Despite the tremendous progress made in understanding this process, its magnitude and significance still have large uncertainties and vary largely with aerosol distribution and meteorological conditions. In this study, we focus on the role of aerosol vertical distribution in thermodynamic stability and PBL development by jointly using micropulse lidar, sun photometer, and radiosonde measurements taken in Beijing. Despite the complexity of aerosol vertical distributions, cloud-free aerosol structures can be largely classified into three types: well-mixed, decreasing with height, and inverse structures. The aerosol–PBL relationship and diurnal cycles of the PBL height and PM 2.5 associated with these different aerosol vertical structures show distinct characteristics. The vertical distribution of aerosol radiative forcing differs drastically among the three types, with strong heating in the lower, middle, and upper PBL, respectively. Such a discrepancy in the heating rate affects the atmospheric buoyancy and stability differently in the three distinct aerosol structures. Absorbing aerosols have a weaker effect of stabilizing the lower atmosphere under the decreasing structure than under the inverse structure. As a result, the aerosol–PBL interaction can be strengthened by the inverse aerosol structure and can be potentially neutralized by the decreasing structure. Moreover, aerosols can both enhance and suppress PBL stability, leading to both positive and negative feedback loops. This study attempts to improve our understanding of the aerosol–PBL interaction, showing the importance of the observational constraint of aerosol vertical distribution for simulating this interaction and consequent feedbacks.

54 ENVIRONMENTAL SCIENCES↗

Mini-Micropulse Lidar data from TAMU TRACER campaign in the Houston TX region from July to September 2022

During TRACER, the Texas A&M Rapid Onsite Atmospheric Measurements Van (ROAM-V) was deployed to capture airmasses behind (maritime) and ahead (continental) of the passage of the sea-breeze front through Houston. On select sampling days, ROAM-V sampled in the morning/mid-day on the coast and then transited to a second inland site for the afternoon/evening. The suite of instruments deployed on ROAM-V included a Condensation Particle Counter (CPC; GRIMM Model 5.403 CPC), Scanning Mobility Particle Sizer (SMPS; TSI 3750 detector, TSI 3082 classifier, TSI 3088 neutralizer, TSI 3081A Differential Mobility Analyzer), Cloud Condensation Nuclei counter (Droplet Measurement Technologies CCN Counter), micro pulse lidar (Droplet Measurement Technologies Micro Pulse LiDAR (mini-MPL)), and a Davis Rotating Uniform size-cut Monitor (DRUM; DRUMAir 4-DRUM). Before sampling at each location, the latitude and longitude were recorded using the GPS on the phone application “My Altitude”. The mini-MPL deployed with ROAM-V is a 532 nm elastic and polarization lidar. The mini-MPL outputs normalized relative backscatter (NRB) derived from raw signal after after-pulse, overlap, and dead-time correction calibration. The depolarization ratio is calculated from the co-polarized and cross-polarized NRB (Flynna et al., 2007). The NRB and depolarization ratio data are resampled from the original data at 1-minute intervals. The vertical resolution of the mini-MPL data is 15 meters. The mini-MPL data can be used to determine the boundary layer, cloud top, and cloud bottom height and can be used to retrieve aerosol type and concentration profile. This data was collected for ARM Field Campaign AFC07055 and supported by DOE ASR grant DE-SC0021047. For any further questions, please feel free to contact the instrument PI, Sarah D. Brooks, sbrooks@tamu.edu . Flynna, C. J., Mendozaa, A., Zhengb, Y., & Mathurb, S. (2007). Novel polarization-sensitive micropulse lidar measurement technique. Optics express, 15(6), 2785-2790.

54 ENVIRONMENTAL SCIENCES↗

The supernova trigger for formation of the solar system

It is suggested that the explosion of a Type II supernova triggered the collapse of a nearby interstellar cloud and led to the formation of the solar system. Estimates of the abundances resulting from nuclear processing of the supernova ejecta are presented. It appears promising that nucleosynthesis in this single supernova event can account for most isotopic anomalies and traces of extinct radioactivities in solar-system material.

Cameron, A. G. W.↗

Vertical profiles of condensation nuclei

Condensation nuclei measurements using a low supersaturation (about 10%) thermal gradient diffusion cloud chamber (TGDCC) and a high supersaturation (about 200%) expansion type instrument were compared on a series of three balloon flights over Laramie, Wyoming. In general, the two instruments produced similar vertical profiles but some discrepancies remain unexplained. Agreement between the two would indicate that the low supersaturations used in the TGDCC were still large enough to cause the instrument to count essentially all of the particles present. The TGDCC condensation nuclei (CN) counter was flown at several sites in both the Northern and Southern Hemispheres. The results indicate the existence of a relative maximum in the CN mixing ratio associated with the upper equatorial troposphere and what appears to be a worldwide constant mixing ratio of CN above 20-25 km.

Rosen, J. M.↗

Heat Capacity Mapping Mission (HCMM): Interpretation of imagery over Canada

Visual analysis of HCMM images acquired over two sites in Canada and supporting aircraft and ground data obtained at a smaller subsite in Alberta show that nightime surface temperature distribution is primarily related to the near-surface air temperature; the effects of topography, wind, and land cover were low or indirect through air temperature. Surface cover and large altitudinal differences were important parameters influencing daytime apparent temperature values. A quantitative analysis of the relationship between the antecedent precipitation index and the satellite thermal IR measurements did not yield statistically significant correlation coefficients, but the correlations had a definite temporal trend which could be related to the increasing uniformity of vegetation cover. The large pixel size (resulting in a mixture of cover types and soil/canopy temperatures measured by the satellite) and high cloud cover frequency found in images covering both Canadian sites and northern U.S. were considered the main deficiencies of the thermal satellite data.

Cihlar, J.↗