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At least 91 records · Page 5

Study of excitation transfer in a flowing helium afterglow pumped with a tuneable dye laser. 1: Measurement of the rate coefficient for selected quenching reactions involving he(5 3P)

A system is described for the measurement of excited state reaction times in the nanosecond range. A flowing afterglow produces large populations of chemically unstable species, and a pulsed, tuneable dye laser is used to selectively pump these into the reacting excited state. The transient fluorescence from the populations of reactants and end products is used to determine reaction lifetimes and yields. This radiatron is collected with a photon counting system which logs arrival times of spectrally dispersed photons with 10 nanosecond resolution.

Collins, C. B.↗

Study of excitation transfer in flowing helium afterglow pumped with a tuneable dye laser. 2: Measurement of the rate coefficient for the rotational relaxation of He2(3p (3 Pi g))

The rotational relaxation of the He2(3p(3pi g)) state is examined by optically pumping a flowing helium afterglow with a tuneable dye laser. The population of the J = 8 rotational state is enhanced by optically saturating the R sub 7 component of the transition connecting this state with the metastable He2(2s (3 Sigma u +)) molecular state. From the lifetime and yield of the Q sub 7 component, the rate coefficient for the rotational relaxation via the forbidden delta J = 1 channel is determined to be of the order of 2 x 10 to the minus 11th power cm3/sec. It is found that this represents about half of the total rate of rotational relaxation in this state.

Collins, C. B.↗

The air afterglow revisited

The air afterglow, 0 + NO2 chemiluminescence, is discussed in terms of fluorescence, photodissociation, and quantum theoretical calculations of NO2. The experimental results presented include pressure dependence, M-dependence, spectral dependence of P and M, temperature dependence, and infrared measurements. The NO2 energy transfer model is also discussed.

Kaufman, F.↗

Time-resolved double-probe study in a He-Hg afterglow plasma

An experimental double-probe technique is described which allows the He(+) ion density to be measured directly as a function of time in the afterglow of a helium-metal-vapor discharge. As an application example, two CW laser transitions of the He-Hg(+) laser at 6150 and 7944 A are considered which both arise from excited 7p (2) P terms of Hg II. The time-resolved double-probe technique is used to measure the destruction rate of the He(+) ion density, which is then compared with the spontaneous-emission decay rate for 7p (2) P terms of Hg II. The results obtained show unambiguously and directly that the dominant excitation process for the two transitions considered is a charge-transfer collisional reaction of the form He(+) plus Hg yields He plus metastable Hg(+) plus the energy defect for this reaction. It is noted that the time-resolved double-probe technique may provide a simple method for measuring ion mobilities in a multi-ion plasma.

Shay, T.↗

Theoretical study of the A prime 5Sigma(+)g and C double prime 5Pi u states of N2 - Implications for the N2 afterglow

Theoretical spectroscopic constants are reported for the A prime 5Sigma(+)g and C double prime 5Pi u states of N2 based on CASSCF/MRCI calculations using large ANO Gaussian basis sets. The calculated A prime Sigma(+)g potential differs qualitatively from previous calculations in that the inner well is significantly deeper (De = 3450/cm). This deeper well provides considerable support for the suggestion of Berkowitz et al. (1956) that A prime 5Sigma(+)g is the primary precursor state involved in the yellow Lewis-Rayleigh afterglow of N2.

Partridge, Harry↗

Decrease in the etch rate of polymers in the oxygen afterglow with increasing gas flow rate

This paper reports the variation of the etch rate of polymers in the afterglow of a radio frequency discharge in oxygen as a function of total flow rate in the range 2-10 cu cm (STP)/min. The measurements were made at ambient temperature with the O(P-3) concentration held essentially constant. Results are reported on three polymers: cis-polybutadiene, a polybutadiene with 33 percent 1,2 double bonds, and a polybutadiene with 40 percent 1,2 double bonds. It has been observed that the etch rate of these polymers decreases significantly with increasing flow rate, strongly suggesting that the vapor-phase products of polymer degradation contribute to the degradation process.

Lerner, N. R.↗

Polymer etching in the oxygen afterglow - Increased etch rates with increased reactor loading

Reactor loading has an effect on the etch rate (rate of decrease of film thickness) of films of polyvinylfluoride (Tedlar) and polyethylene exposed in the afterglow of an RF discharge in oxygen. The etch rate is found to increase with the total surface area of the polymer exposed in the reactor. The etch rates of polypyromellitimide (Kapton H) and polystyrene under these conditions are very low. However, the etch rate of these polymers is greatly enhanced by adding either Tedlar or polyethylene to the reactor. A kinetic model is proposed based on the premise that the oxygen atoms produced by the RF discharge react with Tedlar or polyethylene to produce a much more reactive species, which dominates the etching of the polymers studied.

Lerner, N. R.↗

The influence of flowing afterglow exposure on the degradation of various polymeric materials

Changes in polymer properties which result after exposure to an atomic oxygen-rich environment of a flowing afterglow are presented. Dynamic mechanical and Fourier Transform Infrared (FTIR) spectra as well as scanning electron microscopy micrographs were employed to monitor variations in mechanical properties and chemical and physical structure. Polymers analyzed include polystyrene, PEKK, and a polyester.

Letton, Alan↗

Gamma-ray line afterglow from burst environments

We consider photoerosion and direct pair production in a medium surrounding a gamma-ray burst. The resulting secondary gamma-rays may provide diagnostic tools of these environments and, in turn, of the nature of the bursters themselves. In some instances short-lived nuclides are formed; the beta-delayed gamma-rays produced from their decays provide the signatures of the photoerosion. In addition, annihilation radiation produced from positrons resulting from direct pair production is related to the plasma conditions in the medium. We investigate the plausibility of detecting the various radiations. Under extremely favorable conditions, the photoerosion afterglow might be detectable with the present generation of detectors. However, the positron annihilation line should be detectable under a fairly wide range in the conditions of the medium.

Fencl, H. S.↗

Recombination of H3(+) and D3(+) Ions in a Flowing Afterglow Plasma

The analysis of flowing afterglow plasmas containing H3(+) or D3(+) ions indicates that the de-ionization of such plasmas does not occur by simple dissociative recombination of ions with electrons. An alternative model of de-ionization is proposed in which electrons are captured into H3(**) auto-ionization Rydberg states that are stabilized by collisional mixing of the Rydberg molecules' angular momenta. The proposed mechanism would enable de-ionization to occur without the need for dissociative recombination by the mechanisms of potential-surface crossings.

Gougousi, T.↗

Langmuir-Probe Measurements in Flowing-Afterglow Plasmas

The validity of the orbital-motion theory for cylindrical Langmuir probes immersed in flowing- afterglow plasmas is investigated experimentally. It is found that the probe currents scale linearly with probe area only for electron-collecting but not for ion-collecting probes. In general, no agreement is found between the ion and electron densities derived from the probe currents. Measurements in recombining plasmas support the conclusion that only the electron densities derived from probe measurements can be trusted to be of acceptable accuracy. This paper also includes a brief derivation of the orbital-motion theory, a discussion of perturbations of the plasma by the probe current, and the interpretation of plasma velocities obtained from probe measurements.

Johnsen, R.↗

Electron-Ion Recombination Rate Coefficient Measurements in a Flowing Afterglow Plasma

The flowing-afterglow technique in conjunction with computer modeling of the flowing plasma has been used to determine accurate dissociative-recombination rate coefficients alpha for the ions O2(+), HCO(+), CH5(+), C2H5(+), H3O(+), CO2(+), HCO2(+), HN2O(+), and N2O(+) at 295 K. We find that the simple form of data analysis that was employed in earlier experiments was adequate and we largely confirm earlier results. In the case of HCO(+) ions, published coefficients range from 1.1 X 10(exp -7) to 2.8 x 10(exp -7) cu cm/S, while our measurements give a value of 1.9 x 10(exp -7) cu cm/S.

Gougousi, Theodosia↗

The Discovery and Broadband Follow-Up of the Transient Afterglow of GRB 980703

We report on the discovery of the radio, infrared, and optical transient coincident with an X-ray transient proposed to be the afterglow of GRB 980703. At later times when the transient has faded below detection, we see an underlying galaxy with R = 22.6; this galaxy is the brightest host galaxy (by nearly 2 mag) of any cosmological gamma-ray burst (GRB) thus far. In keeping with an established trend, the GRB is not significantly offset from the host galaxy. Interpreting the multiwavelength data in the framework of the popular fireball model requires that the synchrotron cooling break was between the optical and X-ray bands on 1998 July 8.5 UT and that the intrinsic extinction of the transient is A(sub v) = 0.9. This is somewhat higher than the extinction for the galaxy as a whole, as estimated from spectroscopy.

Bloom, J. S.↗

Discovery of an Afterglow Extension of the Prompt Phase of Two Gamma Ray Bursts Observed by Swift

Contemporaneous BAT and XRT observations of two recent well-covered GRBs observed by Swift, GRB 050315 and GRB 050319, show clearly a prompt component of the afterglow emission. The rapid slewing capability of the spacecraft enables X-ray observations immediately after the burst, typically approximately 100 s following the initiation of the prompt gamma-ray phase. By fitting a power law form to the gamma-ray spectrum, we extrapolate the time dependent fluxes measured by the BAT, in the energy band 15 - 350 keV, into the spectral regime observed by the XRT, 0.2 - 10 keV, and examine the functional form of the rate of decay of the two light curves. We find that the BAT and XRT light curves merge to form a unified curve. There is a period of steep decay up to approximately 300 s, followed by a flatter decay. The duration of the steep decay, approximately 100 s in the source frame after correcting for cosmological time dilation, agrees with a theoretical estimate for the deceleration time of the relativistic ejecta as it interacts with circumstellar material. For GRB 050315, the steep decay can be characterized by an exponential form, where T(sub e),(BAT)approximately equal to 24 plus or minus 2 s, and T(sub e)(XRT) approximately equal to 35 plus or minus 2 s. For GRB 050319 a power law decay -d lnf/d lnt = n, where n approximately equal to 3, provides a reasonable fit. The early time X-ray fluxes are consistent with representing the lower energy tail of the prompt emission, and provide our first quantitative measure of the decay of the prompt gamma-ray emission over a large dynamic range. The initial steep decay is expected from the high latitude emission from a curved shell of relativistic plasma illuminated only for a short interval. The overall conclusion is that the prompt phase of GRBs lasts for hundreds of seconds longer than previously thought.

Barthelmy, S. D.↗

Discovery of an Afterglow Extension of the Prompt Phase of Two Gamma Ray Bursts Observed by Swift

Contemporaneous BAT and XRT observations of two recent well-covered GRBs observed by Swift, GRB 050315 and GRB 050319, show clearly a prompt component joining the onset of the afterglow emission. The rapid slewing capability of the spacecraft enables X-ray observations immediately after the burst, typically ~ 100 s following the initiation of the prompt y-ray phase. By fitting a power law form to the y-ray spectrum, we extrapolate the time dependent fluxes measured by the BAT, in the energy band 15 - 350 keV, into the spectral regime observed by the XRT 0.2 - 10 keV, and examine the functional form of the rate of decay of the two light curves. We find that the BAT and XRT light curves merge to form a unified curve. There is a period of steep decay up to ~ 300 s, followed by a flatter decay. The duration of the steep decay, ~ 100 s in the source frame after correcting for cosmological time dilation, agrees roughly with a theoretical estimate for the deceleration time of the relativistic ejecta as it interacts with circumstellar material. For GRB 050315, the steep decay can be characterized by an exponential form, where one e-folding decay time Te (BAT)~ = 24 f 2 s, and Te,(XRT)~ = 35 f 2 s. For GRB 050319, a power law decay - d l n f / d l n t = n, where n approx. ~ = 3, provides a reasonable fit. The early time X-ray fluxes are consistent with representing the lower energy tail of the prompt emission, and provide our first quantitative measure of the decay of the prompt y-ray emission over a large dynamic range in flux. The initial steep decay is expected due to the delayed high latitude photons from a curved shell of relativistic plasma illuminated only for a short interval. The overall conclusion is that the prompt phase of GRBs remains observable for hundreds of seconds longer than previously thought.

Bathelmy, S. D.↗

Rapid Identification of GRB Afterglows with Swift/UVOT

As part of the automated response to a new gamma-ray burst (GRB), the Ultraviolet and Optical Telescope (UVOT) instrument on Swift starts a 200-second exposure with the V filter within approximately 100 seconds of the BAT burst trigger. The instrument searches for sources in a 8' x 8' region, and sends the list of sources and a 160" x 160" sub-image centered on the burst position to the ground via Tracking and Data Relay Satellite System (TDRSS). These raw products and additional products calculated on the ground are then distributed through the GCN within a few minutes of the trigger. We describe the sensitivity of these data for detecting afterglows, summarize current results, and outline plans for rapidly distributing future detections.

Marshall, F. E.↗

Prompt and Afterglow Emission Properties of Gamma-Ray Bursts with Spectroscopically Identified Supernovae

We present a detailed spectral analysis of the prompt and afterglow emission of four nearby GRBs (GRBs 980425, 030329, 031203, and 060218) that were spectroscopically found to be associated with type Ib/c supernovae. For each event, we investigated its spectral and luminosity evolution and estimated the total energy budget based on the broadband observations. We discuss the properties of the four events in comparison to general burst population, and infer the physical parameters involved in creation of these nearby GRB-SN events

Kaneko, Yuki↗

Prompt and Afterglow Emmision Properties of Gamma-ray Bursts with Spectroscopically Identified Supernovae

We present a detailed spectral analysis of the prompt and afterglow emission of four nearby long-soft gamma-ray bursts (GRBs 980425,030329,031203, and 060218) that were spectroscopically found to be associated with Type IC supernovae and compare them to the general GRB population. For each event, we investigate the spectral and luminosity evolution and estimate the total energy budget based on broadband observations. The observational inventory for these events has become rich enough to allow estimates of their energy content in relativistic and subrelativistic form. The result is a global portrait of the effects of the physical processes responsible for producing long-soft GRBs. In particular, we find that the values of the energy released in mildly relativistic out8ows appears to have a sigruficantly smaller scatter than those found in highly relativistic ejecta. This is consistent with a picture in which the energy released inside the progenitor star is roughly standard, while the fracti

Kaneko, Yuki↗