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NASA NTRSDate not supplied

Spaceborne Passive-Microwave Hail Detection: Global Climatologies, Validation, and Challenges Going Forward

In addition to the myriad threats that severe hailstorms pose to society, infrastructure and agriculture, severe hail is difficult to measure in situ, and surface-based hail reporting and detection methods are inconsistent and vulnerable to nonmeteorological biases. This motivates the use of spaceborne remote-sensing platforms to retrieve hail and construct climatologies in a globally uniform way. We have developed a hail detection algorithm that leverages the sensitivity of spaceborne passive-microwave radiometers to scattering by hail, particularly in the channels from 10 to 89 GHz. We use this retrieval to construct global passive-microwave climatologies of severe hail using the Tropical Rainfall Measuring Mission (TRMM) Microwave Imager (TMI), Global Precipitation Measurement Mission (GPM) Microwave Imager, Advanced Microwave Scanning Radiometer for EOS (AMSR-E), and Advanced Microwave Scanning Radiometer 2 (AMSR2) sensors and are working to extend into the pre-TRMM era to the Special Sensor Microwave Imager/Sounder (SSMI/(S)) data. Using coincident Global Precipitation Measurement (GPM) Ku-band precipitation radar, we assessed this retrieval and several others in the literature for their effectiveness and regional variability. We find that this retrieval, which leverages a signature in the Minimum 19-GHz polarization corrected temperature (PCT) combined with the 37-GHz PCT depression normalized by tropopause height constrains the radar reflectivity most tightly, and gives the least appearance of regional biases compared to other passive-microwave approaches in the literature. Satellite platforms offer consistent observations, even in remote, data-sparse, and oceanic regions that ground-based networks exclude. There are, however, potential disconnects between the processes identified aloft by the satellite and the resultant weather at the ground, leading to uncertainties in the retrievals that may propagate into satellite-based climatologies, particularly in the Tropics, where there are abundant strong - but not necessarily hailing - storms that are strongly represented in the current satellite climatologies. We will discuss ongoing efforts to assess and mitigate the contributing factors to these uncertainties, chiefly among them the effects of non-uniform beam filling in the passive-microwave footprint, and the relationships between the size distributions of hailstones aloft and the dynamic processes and environments with which they interact throughout their trajectories.

Sarah D. Bang↗

NASA NTRS2022

Highly Supercooled Riming and Unusual Triple-Frequency Radar Signatures Over McMurdo Station, Antarctica

Riming of ice crystals by supercooled water droplets is an efficient ice growth process, but its basic properties are still poorly known. While it has been shown to contribute significantly to surface precipitation at mid-latitudes, little is known about its occurrence at high latitudes. In Antarctica, two competing effects can influence the occurrence of riming: (i) the scarcity of supercooled liquid water clouds due to the extremely low tropospheric temperatures and (ii) the low aerosol concentration, which may lead to the formation of fewer and larger supercooled drops potentially resulting in an enhanced riming efficiency. In this work, by exploiting the deployment of an unprecedented number of multiwavelength remote sensing systems (including triple-frequency radar measurements) in West Antarctica, during the Atmospheric Radiation Measurements West Antarctic Radiation Experiment (AWARE) field campaign, we evaluate the riming incidence at McMurdo Station and find that riming occurs at much lower temperatures when compared to previous results in the mid-latitudes. This suggests the possible occurrence of a common atmospheric state over Antarctica that includes a rather stable atmosphere inhibiting turbulent mixing, and a high riming efficiency driven by large cloud droplets. We then focus on a peculiar case study featuring a persistent layer with a particularly pronounced riming signature in triple-frequency radar data but only a relatively modest amount of supercooled liquid water. In-depth analysis of the radar observations suggests that such signatures can only be explained by the combined effects of moderately rimed aggregates or similarly shaped florid polycrystals and a narrow particle size distribution (PSD). Simulations of this case study performed with a one-dimensional bin model indicate that similar triple-frequency radar observations can be reproduced when narrow PSDs are simulated. Such narrow PSDs can in turn be explained by two key factors: (i) the presence of a shallow homogeneous droplet or humidified aerosol freezing layer aloft seeding an underlying supercooled liquid layer, and (ii) the absence of turbulent mixing throughout a stable polar atmosphere that sustains narrow PSDs, as hydrometeors grow from the nucleation region aloft to ice particles of several millimeters in size, by vapor deposition and then riming.

Riming↗

NASA NTRSDate not supplied

Detecting Hail from Space: Algorithms, Climatologies, and Challenges Going Forward

In addition to the myriad threats that severe hailstorms pose to society, infrastructure and agriculture, severe hail is difficult to measure in situ, and surface-based hail reporting and detection methods are inconsistent and subject to geographical or societal biases. This motivates the use of spaceborne remote-sensing platforms to retrieve hail and construct climatologies in a globally uniform way. We have developed a hail detection algorithm that leverages the sensitivity of spaceborne passive-microwave radiometers to scattering by hail, particularly in the channels from 10 to 89 GHz. We use this retrieval to construct global climatologies of severe hail using several different spaceborne sensors: the Tropical Rainfall Measuring Mission (TRMM) Microwave Imager (TMI), Global Precipitation Measurement Mission (GPM) Microwave Imager, Advanced Microwave Scanning Radiometer for EOS (AMSR-E), and Advanced Microwave Scanning Radiometer 2 (AMSR2) sensors and are working to extend into the late 1980’s using the Special Sensor Microwave Imager/Sounder (SSMI/(S)) data. Using coincident Global Precipitation Measurement (GPM) Ku-band precipitation radar, we assessed this retrieval and several others in the literature for their effectiveness and regional variability. We developed a passive-microwave algorithm that corresponds tightly to radar reflectivity and gives the least appearance of regional biases compared to other passive-microwave approaches in the literature. Satellite platforms offer consistent observations, even in remote, data-sparse, and oceanic regions that ground-based networks exclude. There are, however, potential disconnects between the processes identified aloft by the satellite and the resultant weather at the ground, leading to uncertainties in the retrievals that may propagate into satellite-based climatologies, particularly in the Tropics, where there are abundant strong - but not necessarily hailing - storms that are strongly represented in the current satellite climatologies. We will discuss ongoing efforts to assess and mitigate the contributing factors to these uncertainties, chiefly among them the effects of non-uniform beam filling in the passive-microwave footprint, and the relationships between the size distributions of hailstones aloft and the dynamic processes and environments with which they interact throughout their trajectories.

Sarah D Bang↗

NASA NTRSDate not supplied

Remote Sensing of Hail from Space: Retrievals, Climatologies, and Challenges Going Forward

In addition to the myriad threats that severe hailstorms pose to society, infrastructure and agriculture, severe hail is difficult to measure in situ, and surface-based hail reporting and detection methods are inconsistent and subject to geographical or societal biases. This motivates the use of spaceborne remote-sensing platforms to retrieve hail and construct climatologies in the most globally consistent way. Passive-microwave algorithms leverage the sensitivity of spaceborne passive-microwave radiometers to scattering by hail, particularly in the channels from 10 to 89 GHz. These retrievals are used to construct global climatologies of severe hail. The Bang and Cecil (2019) retrievals has been applied to several different spaceborne sensors: the Tropical Rainfall Measuring Mission (TRMM) Microwave Imager (TMI), Global Precipitation Measurement Mission (GPM) Microwave Imager, Advanced Microwave Scanning Radiometer for EOS (AMSR-E), and Advanced Microwave Scanning Radiometer 2 (AMSR2) sensors and used to construct [near] global climatologies of severe hail. This retrieval, and others, have been tested using Global Precipitation Measurement (GPM) Ku-band precipitation radar, to assess their effectiveness and regional variability. A successful retrieval and climatology are those that correspond tightly to radar reflectivity and give minimal appearance of regional biases, especially with latitude. Satellite platforms offer consistent observations, even in remote, data-sparse, and oceanic regions that ground-based networks exclude. There are, however, potential disconnects between the processes identified aloft by the satellite and the resultant weather at the ground, leading to uncertainties in the retrievals that may propagate into satellite-based climatologies, particularly in the Tropics, where there are abundant strong - but not necessarily hailing - storms that are strongly represented in the current satellite climatologies. There are ongoing efforts to assess and mitigate the contributing factors to these uncertainties, chiefly among them the effects of non-uniform beam filling in the passive-microwave footprint, and the relationships between the size distributions of hailstones aloft and the dynamic processes and environments with which they interact throughout their trajectories.

Sarah D Bang↗

NASA NTRSDate not supplied

Spaceborne Remote Sensing of Hail: Retrievals, Climatologies, and Challenges Going Forward

In addition to the myriad threats that severe hailstorms pose to society, infrastructure and agriculture, severe hail is difficult to measure in situ, and surface-based hail reporting and detection methods are inconsistent and subject to geographical or societal biases. This motivates the use of spaceborne remote-sensing platforms to retrieve hail and construct climatologies in the most globally consistent way. Passive-microwave algorithms leverage the sensitivity of spaceborne passive-microwave radiometers to scattering by hail, particularly in the channels from 10 to 89 GHz. These retrievals are used to construct global climatologies of severe hail. The Bang and Cecil (2019) retrievals has been applied to several different spaceborne sensors: the Tropical Rainfall Measuring Mission (TRMM) Microwave Imager (TMI), Global Precipitation Measurement Mission (GPM) Microwave Imager, Advanced Microwave Scanning Radiometer for EOS (AMSR-E), and Advanced Microwave Scanning Radiometer 2 (AMSR2) sensors and used to construct [near] global climatologies of severe hail. This retrieval, and others, have been tested using Global Precipitation Measurement (GPM) Ku-band precipitation radar, to assess their effectiveness and regional variability. A successful retrieval and climatology are those that correspond tightly to radar reflectivity and give minimal appearance of regional biases, especially with latitude. Satellite platforms offer consistent observations, even in remote, data-sparse, and oceanic regions that ground-based networks exclude. There are, however, potential disconnects between the processes identified aloft by the satellite and the resultant weather at the ground, leading to uncertainties in the retrievals that may propagate into satellite-based climatologies, particularly in the Tropics, where there are abundant strong - but not necessarily hailing - storms that are strongly represented in the current satellite climatologies. There are ongoing efforts to assess and mitigate the contributing factors to these uncertainties, chiefly among them the effects of non-uniform beam filling in the passive-microwave footprint, and the relationships between the size distributions of hailstones aloft and the dynamic processes and environments with which they interact throughout their trajectories.

Sarah D Bang↗

NASA NTRSDate not supplied

Geophysical Retrievals and Cloud Analyses from Merged Airborne Radiometer Datasets Covering 10–684 GHz

Airborne microwave radiometers provide insight about numerous aspects of Earth’s atmosphere and yield critical validation datasets for spaceborne radiometers. Three radiometers that are important to NASA’s airborne remote-sensing arsenal include: the Advanced Microwave Precipitation Radiometer (AMPR), covering 10–85 GHz; the Conical Scanning Millimeter-wave Imaging Radiometer (CoSMIR), covering 50–183 GHz; and the Compact Scanning Submillimeter-wave Imaging Radiometer (CoSSIR), covering 170–684 GHz. The NASA field campaigns of interest to this study include: the Integrated Precipitation and Hydrology Experiment (IPHEx) in 2014, the Olympic Mountains Experiment and Radar Definition Experiment (OLYMPEX/RADEX) in 2015–2016, the Investigation of Microphysics and Precipitation for Atlantic Coast-Threatening Snowstorms (IMPACTS) in 2020–2023, and the Airborne Lightning Observatory for FEGS and TGFs (ALOFT) in 2023. To provide a more comprehensive perspective on clouds and precipitation observed during these airborne field campaigns, AMPR data were merged spatiotemporally with CoSMIR data for IPHEx, OLYMPEX/RADEX, and IMPACTS (2020 and 2022), while considering differences in instrument characteristics and operations, providing brightness temperature (Tb) values from 10–183 GHz in a common background grid throughout each flight. AMPR and CoSSIR data were similarly merged for IMPACTS (2023) and ALOFT, providing a common background grid with Tb values covering 10–684 GHz throughout each flight. These merged Tb data were employed in geophysical retrievals using the Community Radiative Transfer Model (CRTM), an Eddington radiative transfer model, and a one-dimensional variational (1DVAR) inversion method. Retrievals of cloud liquid water path were of primary interest. This presentation will include an overview of the methods for the radiometer data mergers, the radiative transfer methods, the geophysical retrievals, and detailed results from examining trends in Tb and cloud liquid water path in clouds, precipitation, and cloud-to-precipitation transition zones.

Corey G Amiot↗

NASA NTRS2024

Global Influence of Organic Aerosol Volatility on Aerosol Microphysical Processes: Composition and Number

We present MATRIX-VBS, a new aerosol scheme that simulates organic partitioning in an aerosol microphysics model, as part of the NASA GISS ModelE Earth System Model. MATRIX-VBS builds on its predecessor aerosol microphysics model MATRIX (Bauer et al., 2008, https://doi.org/10.5194/acp-8-6003-2008) and was developed in the box model framework (Gao et al., 2017, https://doi.org/10.5194/gmd-10-751-2017). The scheme features the inclusion of organic partitioning between the gas and particle phases and the photochemical aging process using the volatility-basis set (Donahue et al., 2006, https://doi.org/10.1021/es052297c). To assess the performance of the new model, we compared its mass concentration, number concentration, and activated number concentration to the original scheme MATRIX, and evaluated its mass concentrations in four seasons against data from the NASA Atmospheric Tomography Mission (ATom) aircraft campaign. Results from MATRIX-VBS show that organics are transported further away from their source, and their mass concentration increases aloft and decreases at the surface compared to those in MATRIX. The mass concentration of organics at the surface agrees well with measurements, and there are discrepancies for vertical profiles aloft. In the new scheme, the global mass load of organic aerosols increased by 50%, there is also an increased number of particles at the surface and fewer activated ones in most regions. The new scheme presents advanced and more comprehensive capability in simulating aerosol processes.

aerosol modeling↗

NASA NTRSDate not supplied

Hunting Energetic Radiation from Thunderstorms

The true nature and mechanisms of terrestrial gamma-ray flashes (TGFs) have remained mysterious since their discovery in the 1990s. Despite decades of detections, their violent origins and irregularity make them particularly difficult to observe directly. Combined with the wide range of measured characteristics, this has kept the details of these energetic events in the dark. The recent ALOFT (Airborne Lightning Observatory for FEGS and TGFs) campaign has undertaken the challenge of hunting these elusive flashes from an airborne platform. This was performed by the NASA ER-2 aircraft in July 2023 equipped with a host of meteorological, electric field, and gamma-ray instruments to study intense tropical thunderstorms and their connection to gamma-ray production. Here we present on the campaign's success alongside some of its exciting preliminary results.

Lightning↗

DOE OSTI2022

Mesoscale evaluation of AMPS using AWARE radar observations of a wind and precipitation event over the Ross Island region of Antarctica

Surface, upper-air, and radar observations are used to assess the performance of the Antarctic Mesoscale Prediction System (AMPS) in simulating the mesoscale aspects of a wind and precipitation event over the Ross Island region of Antarctica that spanned January 16–20, 2016. The observations, collected during the Atmospheric Radiation Measurement (ARM) West Antarctic Radiation Experiment (AWARE), provide a unique dataset for evaluating AMPS, especially the radar observations that facilitate a three-dimensional depiction of winds and precipitation. Comparisons of AMPS forecast data with surface meteorology, balloon-sounding, and profiling radar observations at and above sites near McMurdo Station reveal a mixture of similarities and differences. A generally southerly flow is evident at low levels in both the AMPS simulations and observed Doppler radial velocities. AMPS winds are comparable to those observed at the surface and aloft in terms of magnitude, direction, and timing but the strongest simulated southerly flow is displaced eastward relative to the observations. AMPS-simulated reflectivity over the broader Ross Island region is more limited in areal extent and smaller in magnitude than observed by a scanning Doppler radar. Three episodes of surface precipitation are observed near McMurdo Station over the five-day event with peak rates of ~3 mm h -1 and a total accumulation of ~22 mm. However, AMPS produces no surface precipitation at that location over the five-day event due to a low-level dry bias in the forecasts. Herein, the results show the first observationally based three-dimensional understanding of meteorology in the Ross Island region.

AMPS↗

DOE OSTI2023

New insights on wind turbine wakes from large‐eddy simulation: Wake contraction, dual nature, and temperature effects

Abstract Large‐eddy simulation (LES) has been adopted to study wind turbine wakes because it can capture fine‐scale details of turbulent wind flows and interactions with wind turbines. Here, we use the LES version of the Weather Research and Forecasting (WRF) model with an actuator disk model to gain insights on several wake effects that have been traditionally difficult to measure. The first finding is that the wake has a “dual nature,” meaning that the wind speed deficit behaves differently from the added turbulent kinetic energy (TKE) and the two are not co‐located in space. For example, the wind speed deficit peaks at hub height and reaches the ground within 8D (D is the rotor diameter), but added TKE peaks near the rotor tip and generally remains aloft. Second, temperature changes near the ground are driven by the added TKE in the rotor area and by atmospheric stability. The combination of these two factors determines the sign and intensity of the vertical heat flux divergence below the rotor, with convergence and warming associated with stable conditions and weak divergence and modest cooling with unstable conditions. Third, wakes do not expand indefinitely, as suggested by similarity theory applied to the wind speed deficit, but eventually stop expanding and actually contract, at different rates depending on atmospheric stability. The implication of these findings is that, in order to study wakes, it is not sufficient to focus on wind speed deficit alone, because TKE is also important and yet behaves differently from the wind speed deficit.

17 WIND ENERGY↗

DOE OSTI2024

Overview of the Alaskan Layered Pollution and Chemical Analysis (ALPACA) Field Experiment

The Alaskan Layered Pollution And Chemical Analysis (ALPACA) field experiment was a collaborative study designed to improve understanding of pollution sources and chemical processes during winter (cold climate and low-photochemical activity), to investigate indoor pollution, and to study dispersion of pollution as affected by frequent temperature inversions. A number of the research goals were motivated by questions raised by residents of Fairbanks, Alaska, where the study was held. This paper describes the measurement strategies and the conditions encountered during the January and February 2022 field experiment, and reports early examples of how the measurements addressed research goals, particularly those of interest to the residents. Outdoor air measurements showed high concentrations of particulate matter and pollutant gases including volatile organic carbon species. During pollution events, low winds and extremely stable atmospheric conditions trapped pollution below 73 m, an extremely shallow vertical scale. Tethered-balloon-based measurements intercepted plumes aloft, which were associated with power plant point sources through transport modeling. Because cold climate residents spend much of their time indoors, the study included an indoor air quality component, where measurements were made inside and outside a house to study infiltration and indoor sources. In the absence of indoor activities such as cooking and/or heating with a pellet stove, indoor particulate matter concentrations were lower than outdoors; however, cooking and pellet stove burns often caused higher indoor particulate matter concentrations than outdoors. The mass-normalized particulate matter oxidative potential, a health-relevant property measured here by the reactivity with dithiothreiol, of indoor particles varied by source, with cooking particles having less oxidative potential per mass than pellet stove particles.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2025

Advancing Aerosol Chemical Characterization and Vertical Profiling over the Southern Great Plains Using Uncrewed Aerial Sampling and Offline Aerosol Mass Spectrometry

Recent advancements in uncrewed aerial systems (UASs) and particulate matter (PM) analytical techniques have provided opportunities for atmospheric research. In this study, we deployed the Department of Energy’s fixed-wing ArcticShark UAS to examine PM 2.5 composition at varying altitudes─within and above the planetary boundary layer (PBL)─over the Southern Great Plains atmospheric observatory (SGP). A total of 22 flights were conducted across March, June, and August 2023. Composite filter samples were collected during each flight and analyzed with offline aerosol mass spectrometry (AMS), complemented by on-board real-time sensors and ground-based instrumentation, to provide a comprehensive view of regional aerosol characteristics. Results show clear vertical and seasonal differences in the aerosol composition. Relative to ground-level measurements, aloft samples exhibited shifts in the distribution of organic and inorganic PM, with the organic composition varying distinctly across seasons. Particulate organic nitrogen (ON) was elevated, with bulk compositions similar in March and June but strongly altered in August, likely driven by biomass burning and enhanced photochemical activity. Combined AMS and chemical ionization mass spectrometry analyses detected amines, amides, and amino acids. PM above the planetary boundary layer was enriched in oxidized organic aerosols, while ground-level PM contained higher nitrate and sulfate. Seasonal differences in aqueous-phase processing were also observed, which were strongest in March during persistent cloud cover and weaker in the drier August period, suggesting a shift from aqueous- to gas-phase SOA formation. In conclusion, these findings highlight the value of UAS in advancing PM measurements and vertical profiling of aerosol composition.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2021

Atmospheric Transport of North African Dust-Bearing Supermicron Freshwater Diatoms to South America: Implications for Iron Transport to the Equatorial North Atlantic Ocean

The equatorial North Atlantic Ocean (NAO) is a nutrient-limited ecosystem that relies on the deposition of long-range transported iron (Fe)-containing aerosols to stimulate primary productivity. Using microscopy, we characterized supermicron and supercoarse mode African aerosols transported to the western NAO in boreal winter/spring. In this work, we detected three particle types including African dust, primary biological aerosol particles, and freshwater diatoms (FDs). FDs contained 4% Fe by weight due to surficial dust inclusions that may be susceptible to chemical processing and dissolution. FDs were typically larger than dust particles and comprised 38% of particles between 10 and 18 μm in diameter. The low density, high surface-area-to-volume ratio, and large aspect ratios of FD particles suggest a mechanism by which they can be carried great distances aloft. These same properties likely increase the residence time of FDs in surface waters thereby increasing the time for Fe dissolution and their potential impact on marine biogeochemical cycles.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2020

Impacts of Latent Energy and Snow Fall Speed on a Wintertime Midlatitude Cyclone

This study aimed to understand the impacts of latent energy as well as snow fall speeds on precipitation properties and synoptic-scale storm characteristics of a wintertime midlatitude cyclone. Simulations of a potent winter storm that impacted the Rocky Mountains and northern Great Plains of the United States in February 2017 were performed using the Weather Research and Forecasting model with latent heating or cooling from individual microphysical processes systematically turned off and fall speeds adjusted by ±50%. Results indicated substantial impacts on the microphysical characteristics of the simulated storm to fall speed, cooling from sublimation, and warming from deposition. The impacts of cooling and warming were manifested as differences in accumulated snowfall. Increased (decreased) fall speeds led to smaller (larger) ice crystals and total mass, resulting in offsetting effects on the precipitation flux, and thus minimal impacts on snowfall and large-scale characteristics of the storm. Warming and cooling associated with deposition and sublimation, respectively, impacted the synoptic-scale dynamics, whereby removing warming from deposition resulted in an increased meridional temperature gradient near the jet stream, thus increasing the jet strength and causing it to be more westerly with less curvature aloft. This in turn limited upper-level divergence, creating a weaker surface low and shifting the precipitation shield southward. The opposite occurred with the removal of latent cooling due to sublimation. This study highlights the potential importance of latent energy associated with ice sublimation and deposition and fall speeds in the larger-scale characteristics of winter storms.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2022

Assessing Physical Relationships Between Atmospheric State, Fluxes, and Boundary Layer Stability at McMurdo Station, Antarctica

Observations at McMurdo Station, Antarctica from 24 November 2015 through 3 January 2017 were used to characterize the physical relationships between boundary layer stability and atmospheric state and fluxes. The basis of this analysis was self-organizing maps (SOMs), a neural network algorithm, used to identify the range of potential temperature profiles present in the twice-daily radiosonde data during the ARM (Atmospheric Radiation Measurement) West Antarctic Radiation Experiment (AWARE) campaign. The SOM identified profiles ranging from strongly stable to weakly stable regimes over the lowest 500 m of the atmosphere. It was found that in the winter (MJJA), moderate and strongly stable regimes occur most frequently (61%), while weakly stable regimes dominate in the summer (DJ, 83.4%). The mechanisms responsible for the dominance of different stability regimes in each season were analyzed to determine why these regimes occur with varying frequency throughout the year. This analysis found that wind speed variations and radiative cooling are responsible for the stability observed in the winter, radiative warming, as well as weaker wind speeds, are responsible for summer weak stability, and stability variations in the transition seasons (FMA, SON) are characterized by a change in sign of net radiation with increasing stability, as wind speed changes little across stability regimes. Low-level jets were observed to occur about 50% of the time below areas of enhanced stability aloft and were observed most frequently in the transition seasons. The boundary layer depth, as determined by the Bulk Richardson number, was found to decrease with increasing stability.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2022

Turbulent Flux Measurements of the Near‐Surface and Residual‐Layer Small Particle Events

Abstract According to recent field studies, almost half of the New Particle Formation (NPF) events occur aloft, in a residual layer, near the top of the boundary layer. Therefore, measurements of the meteorological parameters, precursor gas concentrations, and aerosol loadings conducted at the ground level are often not representative of the conditions where the NPFs take place. This paper presents new measurements obtained during the Turbulent Flux Measurements of the Residual Layer Nucleation Particles, conducted at the Southern Great Plains research site. Vertical turbulent fluxes of 3–10 nm‐sized particles were measured using a sonic anemometer and two condensation particle counters with nominal cutoff diameters of 3 nm and 10 nm mounted at the top of the 10‐m telescoping tower. Aerosol number size distribution (5–300 nm) was determined through the ground‐based Scanning Mobility Particle Sizers. The size selected (15–50 nm) particle hygroscopicity was derived with the Humidified Tandem Differential Mobility Analyzer. The ground level observations were supplemented by vertically‐resolved measurements of horizontal and vertical wind speeds and aerosol backscatter. The data analysis suggests that (a) turbulent flux measurements of 3–10 nm particles can distinguish between near‐surface and residual‐layer small particle events; (b) sub‐50 nm particles had a hygroscopicity value of 0.2, suggesting that organic compounds dominate atmospheric nanoparticle chemical composition at the site; and (c) current methodologies are inadequate for estimating the dry deposition velocity of sub‐10 nm particles because it is not feasible to measure particle concentration very near the surface, in the diffusion sublayer.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2023

Simulating the Transport and Rupture of Pollen in the Atmosphere

Pollen, one type of primary biological aerosol particle (PBAP), is emitted from the terrestrial biosphere and can undergo physical changes in the atmosphere via particle rupture. To examine the fate of pollen and its atmospheric processing, a pollen emission and transport scheme is coupled to the Weather Research and Forecasting Model with Chemistry (WRF-Chem). We simulate the emission of pollen and its impacts on the cloud properties and precipitation in the Southern Great Plains from 12 to 19 April 2013, a period with both high pollen emissions and convective activity. We conduct a suite of ensemble runs that simulate primary pollen and three different pollen rupture mechanisms that generate subpollen particles, including (a) high humidity-induced surface rupture, (b) high humidity-induced in-atmosphere plus surface rupture, and (c) lightning-induced rupture, where in-cloud and cloud-to-ground lightning strikes trigger pollen rupture events. When relative humidity is high (>80%), coarse primary pollen (~1 μg m –3 ) is converted into fine subpollen particles (~1.2e –4 μg m –3 ), which produces 80% more subpollen particles than lightning-induced rupture. The in-atmosphere humidity-driven rupture predominantly produces subpollen particles, which is further enhanced during a frontal thunderstorm. During strong convection, vertical updrafts lift primary pollen and subpollen particles (~0.5e –4 μg m –3 ) to the upper troposphere (~12 km) and laterally transports the ruptured pollen in the anvil top outflow. In regions of high pollen and strong convection, ruptured pollen can influence warm cloud formation by decreasing low cloud (<4 km) cloud water mixing ratios and increasing ice phase hydrometeors aloft (>10 km)

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2024

The Role of Non-Local Effects on Surface Sensible Heat Flux Under Different Types of Thermal Structures Over the Arctic Sea-Ice Surface

The effects of atmospheric thermal structure on the surface energy flux are poorly understood over the Arctic sea-ice surface. Here, we explore the mechanism of sensible heat exchange under different types of thermal structures over the Arctic sea-ice surface by using data collected during the Multidisciplinary drifting Observatory for the Study of Arctic Climate expedition. The quadrant analysis indicates that strong surface temperature inversions below 100 m enhance non-local effects on the positive (upward) sensible heat flux ($\overline{w'θ'}$) through entrainment of large eddies from the convective boundary layer aloft. However, strong surface inversions restrict the contributions of large eddies to the negative (downward) $\overline{w'θ'}$ due to intensified surface stability. By inspecting the existing parameterization schemes, we found that the European Center for Medium-Range Weather Forecasts Integrated Forecasting System scheme fails to predict the impacts of non-local processes on the positive $\overline{w'θ'}$, and an adjustment term to correct the bias of parameterized $\overline{w'θ'}$ is proposed.

54 ENVIRONMENTAL SCIENCES↗