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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 91 records · Page 5
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

Development of an accelerator-based neutron source to prototype Mo-99 production, Part II: A liquid LBE loop under a high vacuum

To provide US domestic supply of Mo-99 without using high-enriched uranium (HEU), a subcritical uranium target assembly (UTA) is irradiated by an accelerator-based neutron source to create Mo-99 through fission. Part I of this work discusses the design of a liquid lead–bismuth eutectic (LBE) windowless target for an accelerator-based neutron source development. Part II discusses how to couple this windowless target to an accelerator operating at an ultra-high vacuum and the subcritical UTA cooled by water at room temperature. Due to the windowless design of the target, the liquid LBE flow shares an ultra-high vacuum (<1.3 × 10 -7 Pa or 10 -9 Torr) space with the accelerator. As a result of this shared vacuum space, the LBE system must operate at a high vacuum (10 -3 ~10 -6 Pa or 10 -5 ~10 -8 Torr). A magnetic rotary motion feedthrough unit utilizes magnetic fluid to allow rotation of the pump while maintaining a high vacuum environment. Prior to testing the LBE system under vacuum, a pump curve measurement is performed to estimate flowrate in the system. This measurement also generates data on orifice loss coefficients, which are compared to correlations in literature. The second experiment investigates vacuum level in the LBE system during operation. High vacuum is maintained (10 -3 ~10 -5 Pa or 10 -5 ~10 -7 Torr) during system operation, and a residual gas analyzer (RGA) scan shows that partial pressures of residual gases in the LBE system lower over the duration of LBE system operations. The third experiment investigates the gravity driven liquid LBE flowing out of the target chamber in the return line, which is partially full. If the liquid LBE is not drained quickly enough, flooding in the target chamber could occur. The coefficient n in the Manning equation is found to be around 0.008 s/m 1/3 . The last experiment performed is a demonstration that a vacuum jacket could provide sufficient thermal insulation to allow coupling between 300 °C LBE loop and a water tank at room temperature. In conclusion, the results from these experiments have influenced the development of the neutron source for the future commercial scale Mo-99 production system.

43 PARTICLE ACCELERATORS↗
DOE OSTI2020

Design and Analysis of a Double Wall, Water Cooled Window for Accelerator Based Mo-99 Production

The electron accelerator based Mo-99 production technique requires the use of Rhodotrons to generate 38 MeV, 6.32 mA pulsed electron beams. The introduction of the pulsed beam structure has introduced fatigue concerns in the vacuum-helium windows that did not exist previously for electron beam production via linear accelerators. Previous analysis has shown that temperature fluctuations of approximately 100°C above and below the steady state operating temperature of ~500°C will occur within the windows. A water cooled window will eliminate this concern by reducing the primary mechanical stress due to the 300-psig helium pressure load as well as the secondary thermally induced stress. Although a water cooled window was considered years ago, the complexities of adding an additional water line was unattractive until now. A double wall, water cooled window has been designed and analyzed for this reason. The water cooled window design is shown to decrease the helium-side window temperature to as low as 125°C, while the vacuum-side window is maintained at 161°C at a water flow rate of 3.2 GPM. These low steady state temperatures reduce the thermal stress of the helium-side window significantly. Also, the primary mechanical stress has been reduced by roughly 50% due to the reduced pressure gradient across the helium-side window (150-psig water and 300-psig helium). Considering a Mo-99 production loss of roughly 1%, the water cooled window is a drastic improvement over the previous helium cooled designs and should be greatly considered for future upgrades and redesign.

43 PARTICLE ACCELERATORS↗
DOE OSTI2020

Northstar Mo100 Target Beam Spot Size Sensitivity Study

Northstar Mo100 target for production of the medical isotope Mo99 is particularly sensitive to beam over focusing because of the intended high power density. At 38 MeV and 6.32 mA (240 kW beam power, nominally 160 kW th in the target), small deviation from the nominal 12 mm FWHM beam can significantly increase the target disk temperatures and more importantly the load bearing target window temperature. A rhodotron will be the source of the electron beam to be used in the isotope production. This machine operates in a pulsed beam mode, currently expected to be at 50 Hz, which results in a 100 C temperature oscillation above and below the steady state temperature that is the focus of this study. This must be considered in the determination of minimum beam spot size that can be accepted by the target without risk of failure. In addition to the nominal beam spot size of 12 mm, the analysis of 10, 11 and 14.5 mm beam spot sizes are analyzed. The primary conclusion is that an over focused beam to just 11 mm FWHM is the minimum beam spot allowable, based on window temperature and the Ultimate Tensile Stress (UTS) of the window material Inconel 718 as a function of temperature. In contrast an under focused beam of 14.5 mm FWHM has much reduced target and window temperatures, but there is a resulting 6% drop in isotope production, all other factor staying the same. These results are presented herein.

07 ISOTOPE AND RADIATION SOURCES↗
DOE OSTI2024

Photoelectron spectroscopy of CsK2Sb photocathode at Synchrotron Radiation Facility using vacuum transport system

As accelerators and electron microscopes become more advanced, high-performance photocathodes are required. In particular, Cesium potassium antimonide (CsK 2 Sb) photocathode is of interest because of its low emittance, excitability in visible light, and high quantum efficiency (QE). The challenge is its high susceptibility to environment that lead to low operating vacuum pressure and short lifetime/low extraction charge. To resolve these issues, it is necessary to understand the molecular structure of the cathode and its degradation mechanism. In this study, we transported CsK 2 Sb photocathode to a beamline of synchrotron radiation facility using a vacuum transport system for molecular structure analysis. Specifically, the cathode was deposited in an evaporation system at Nagoya University. We transported it to Aichi Synchrotron Radiation Center (Aichi SR) located 15 km away, and analyzed it in the depth direction by X-ray photoelectron spectroscopy (XPS) at BL7U. Based on the results, we quantitatively evaluated the composition ratios and stoichiometry of the cathode elements (Sb, K, Cs). A Cs ex-cess state of surface was observed at the surface, and it is consistent with previous studies. The intended atomic structure of CsK 2 Sb was formed only at a few nanometres of the surface on the Mo substrate. On the other hand, the CsK 2 Sb cathode structure on the graphene substrate was preserved further in the depth direction.

47 OTHER INSTRUMENTATION↗
DOE OSTI2025

Post-DTL Beam Delivery

Ensuring that the beam delivered from the upgraded Front-End (FE) meets the Key Performance Parameters (KPPs) at each user facility is critical to the success of the LANSCE Accelerator Modernization Project (LAMP). For a high-intensity, multi-user facility like LANSCE, compliance with beam loss and radiation thresholds is as important as the charge delivered to each target. While early LAMPF/LANSCE operations relied on iterative tuning to minimize losses from beam halo and tail particles, the new FE may introduce different beam distributions and loss modes—making predictive modeling essential. To manage this, the F2E (Front-End to End) effort is developing detailed particle-tracking models that reflect realistic beamline conditions, including halo formation and expected diagnostic readings. These "snapshot" simulations aim to benchmark live machine performance at a given moment. This will help quantify how beam quality from the new FE will propagate downstream through the facility. Only by validating these models can we confidently assess and mitigate the potential impacts of the LAMP FE on beam delivery. Post-DTL, the beam splits to serve five major user facilities. Historically, low-energy beam transport has been modeled using TRACE, and higher-energy sections with TRANSPORT. These have now been unified into MAD-X format and validated with codes such as Elegant, pyOrbit, XSuite, Impact-Z, and HPSim. The primary focus now is on accurate modeling of full particle distributions (including beam halo) as they traverse the accelerator and beamlines to each experimental station. All models are at various stages of validation with empirical data.

43 PARTICLE ACCELERATORS↗
DOE OSTI2018

Review of Heavy Charged Particle Transport in MCNP6.2

The release of version 6.2 of the MCNP6 radiation transport code is imminent. To complement the newest release, a summary of the heavy charged particle physics models used in the 1 MeV to 1 GeV energy regime is presented. Several changes have been introduced into the charged particle physics models since the merger of the MCNP5 and MCNPX codes into MCNP6. Here, this article discusses the default models used in MCNP6 for continuous energy loss, energy straggling, and angular scattering of heavy charged particles. Explanations of the physics models’ theories are included as well.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2018

Physics design of the next-generation spallation neutron target-moderator-reflector-shield assembly at LANSCE

Here, we discuss the physics design of the next-generation spallation neutron target-moderator-reflector-shield (TMRS) assembly for the Manuel Lujan Jr. Neutron Scattering Center (Lujan Center) at the Los Alamos Neutron Science Center (LANSCE). We developed this TMRS to improve the neutronic performance of the Lujan Center in the intermediate energy range (keV–MeV) enabling a variety of new nuclear physics experiments, as well as increasing the quality of the ongoing experiments. The results of our Monte Carlo optimization study indicate that the new TMRS will generate keV–MeV neutrons with higher intensity and improved time resolution. At the same time, the new design largely maintains its current performance in the cold and thermal ranges supporting materials research. In this article we show that the new TMRS has the potential to enhance the Lujan Center’s experimental capability in a wider interval of energies – cold to intermediate – after its scheduled installation in 2020.

43 PARTICLE ACCELERATORS↗
DOE OSTI2018

Experimental improvement of 750-keV H - beam transport at LANSCE Accelerator Facility

The 750-keV low-energy beam transport of the Los Alamos Neutron Science Center (LANSCE) linac consists of two independent beam lines that facilitate simultaneous injection of H + and H - beams into the linear accelerator. The efficiency of beam transport within this structure is largely controlled by the effects of space-charge neutralization. In this study, we report a series of experiments that were performed to determine the level, as well as the required timescale for the onset of beam space charge neutralization. Measurements performed along the structure indicate significant variation of neutralized space charge beam dynamics in the beamline, and the corresponding results have been used to substantially improve beam transport with diminished beam losses. Finally, the analysis of experimental and theoretical data employed in optimization of beam performance in the transport line is discussed.

43 PARTICLE ACCELERATORS↗
DOE OSTI2019

Divergence study and emittance measurements for the electron beam emitted from a diamond pyramid

This paper reports the results of a divergence study and emittance measurements for an electron beam emitted from a single diamond pyramid in a sparse diamond field-emitter array (DFEA) cathode. DFEA cathodes are arrays of micrometer scale diamond pyramids with nanometer scale tips. A single diamond pyramid produces currents as high as 10 μA from a small surface area. DFEA cathodes are expected to be a good beam source for compact dielectric laser accelerators. For the electron beam divergence experiment, we have designed and assembled a test stand consisting of a DFEA cathode, a mesh anode, and a screen. We measured current and the size of the beam on the screen as functions of the distance between the cathode and the anode, the size of a pyramid’s base, and applied voltage on the cathode. In order to perform beam emittance measurements, we designed and fabricated a magnetic lens to be placed between the mesh and the screen. By measuring the size of the beam for different distances between the lens and the screen, we estimate the beam’s emittance. Here, we also simulated the electron beam dynamics with Computer Simulation Technology Studio and General Particle Tracer codes. Experimentally measured divergence angles and normalized transverse emittance show good agreement with simulations.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2021

Six-dimensional matching of intense beam with linear accelerating structure

Beam matching is a common technique that is routinely employed in accelerator design with the aim of minimizing beam losses and preservation of beam brightness. Despite being widely used, a full theoretical understanding of beam matching in 6D remains elusive. In this work, we present an analytical treatment of 6D beam matching of a high-intensity beam onto an RF structure. We begin our analysis within the framework of a linear model, and apply the averaging method to a set of 3D beam envelope equations. Accordingly, we obtain a matched solution that is comprised of smoothed envelopes and periodic terms, describing envelope oscillations with the period of the focusing structure. We then consider the nonlinear regime, where the beam size is comparable with the separatrix size. Stating with a Hamiltonian analysis in 6D phase space, we attain a self-consistent beam profile and show that it is significantly different from the commonly used ellipsoidal shape. Subsequently, we analyze the special case of an equilibrium with equal space charge depression between all degrees of freedom. Comparison of beam dynamics for equipartitioned, equal space charge depression, and equal emittances beams is given. Finally, we present experimental results on beam matching in the LANSCE linac.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2024

Innovative approaches to neutron beam optimization: A case study of FP14 at LANSCE

This paper describes an experimental method to acquire high resolution energy- and spatially- resolved neutron beam spots using the time-gated neutron imaging system with Teledyne Pi-MAX4 camera. These experimental data offer a unique opportunity for benchmarking beam spot simulations. High-quality simulations depend significantly on a high-fidelity geometry model, which can be challenging for legacy facilities. We informed our MCNPX geometry model by latest metrology survey employing Leica laser tracker ATS600. It gave us a high fidelity description of our facility geometry. Such a robust integration of novel tools and methods yields a previously unattainable level of accuracy in both predicting and capturing neutron beam spots, marking a notable advancement over traditional methods reliant on static image plates. Here, to demonstrate the practical application of these tools, we are showing a non-uniform beam spot challenge at our Flight Path 14 (FP14) at the Los Alamos Neutron Science Center (LANSCE). Our precise MCNPX prediction of beam spot shifting as function of neutron energy was confirmed by experimental beam spot measured with extremely high level of detail. Results of this research demonstrate a significant leap in neutron beam optimization at LANSCE and set a new benchmark in beam spot characterization. The advanced methods presented here have potential for adoption at similar research facilities worldwide, aiming at substantial improvement in neutron beam delivery for experiments.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2019

Application of a radial radio-frequency electron gun to waste treatment

Electron-beam irradiation has been shown to be a clean, efficient, and effective technique for treating a variety of contaminants in a variety of media. In particular, the ionizing radiation produced by an electron beam can effectively decontaminate wastewater and aid in removing harmful chemicals from industrial flue gas. In this paper, we investigate a novel technique for waste treatment using an electron-beam system in which an (approximately) annular beam converges radially into the treatment volume. We provide preliminary system-level analysis of the design of a radial electron gun, and we discuss hypothetical system constructs in which a radial electron gun is used for treatment of flue gas and wastewater. We derive dose uniformity, throughput rates, and other important treatment parameters for each application. Our results suggest that a lower-energy system with a large-radius cylindrical treatment volume is preferable for flue gas treatment, whereas a higher-energy system with an annular treatment volume is better-suited for wastewater treatment.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗
DOE OSTI2018

Observation of multipath effects in the detection of RF-modulated x-rays

As part of the Air Force Research Laboratory’s ongoing research in particle accelerators and beams, we recently began investigating the interaction of RF-modulated x-ray beams with RF structures. Additionally, these bremsstrahlung x-rays, produced using an S-band RF electron linac and tungsten foil, were able to drive RF signals at the linac frequency and its integer harmonics in an S-band waveguide. This was interpreted as a result of secondary electron production inside the waveguide by the modulated x-ray beam and implied that the primary electron beam RF modulation was preserved, to at least some degree, through both the processes of x-ray and secondary electron production. The strength of these signals induced on the waveguide varied as the distance of the waveguide from the tungsten foil changed, with the nature of these changes suggesting the existence of an interference process resulting from multipath propagation of the modulated x-rays. Here, we report on our initial attempt to verify this multipath propagation by altering the configuration of shielding and reflective masses in the environment of the waveguide. Finally, these measurements support the existence of a multipath propagation effect and further indicate that the RF modulation of the x-rays is preserved as they undergo scattering events inside the accelerator vault.

43 PARTICLE ACCELERATORS↗
DOE OSTI2018

Hot filament performance in a Freeman ion source

Here, we report on the simulation results of the hot tungsten filament behavior in a Freeman ions source installed in the LANL electro-magnetic isotope separator (EMIS). The Freeman source enables us to ionize and extract high intensity single-charge ion beams from different gases as well as from various solid materials in order to purify the content of a selected isotope. We have modified our LANSCE H– Ion Source Filament Model to calculate the ion source working parameters during a beam production cycle and estimate the ion source filament lifetime. Two main mass erosion processes of the hot cathode in a Freeman ion source are included: thermal evaporation and plasma sputtering. The initial working temperature of the ion source filament was estimated to be in range of 2400 to 2500 K. The filament model shows that the plasma sputtering rate is several magnitude of order higher than the thermal evaporation rate. The results of ion source modeling were compared with recorded data during the EMIS beam production runs using krypton noble gas.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2018

Multi-plate interceptive electron beam energy diagnostic—Implementation and validation

A previous publication [P. D. McChesney, “Multi-plate interceptive electron beam energy diagnostic—Theoretical design,” AIP Adv. (submitted)] reported a new interceptive electron beam kinetic energy measurement technique based on the beam penetration depth within a stack of conductive plates and gave results on the theoretical design of such a device. This paper expands on this and gives further results on the actual implementation of the diagnostic. The device geometry and measurement electronics system are described in detail. A prototype version of the multi-plate diagnostic was fabricated and tested using an electron linear accelerator at the Idaho Accelerator Center (IAC). A high-precision magnetic spectrometer system was designed and built for the purpose of validating the multi-plate diagnostic’s energy measurement capabilities. It was found that the diagnostic provides electron beam energy estimates that are accurate to better than the 10% level.

43 PARTICLE ACCELERATORS↗
DOE OSTI2019

Theory of electron transport and emission from a semiconductor nanotip

An sufficient mass based model accounting for the conduction band quantization in a high aspect ratio semiconductor nanotip is developed to describe injected electron transport and subsequent electron emission from the nanotip. A transfer matrix formalism is used to treat electron scattering induced by the variation in the tip diameter and in the electron emission. Numerical assessment of the scattering and emission probabilities is performed for the diamond parametrized nanotip model. Our scattering and emission models are further combined with a Monte Carlo (MC) approach to simulate electron transport through the nanotip. The MC simulations, additionally accounting for the electron-phonon scattering and externally applied electric field, are performed for a minimal nanotip model and an equivalent width diamond slab. An effect of the level quantization, electron scattering due to the nanotip diameter variation, and electron-phonon scattering on the nanotip emission properties are identified and compared with the case of a bulk slab.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2021

Systematic evaluation of magnetic sensitivities of anisotropic magnetoresistive sensors at liquid helium temperature for superconducting cavities

Trapped magnetic flux in bulk superconductors reduces the quality factor Q in superconducting radio-frequency (SRF) cavities. However, the mechanisms underlying flux trapping and radio-frequency loss are not well understood. Detailed observation of the magnetic distributions is important for understanding such phenomena. Magnetic field mapping is useful for observing the magnetic field distribution around SRF cavities. Measuring the change in the magnetic field around the cavity elucidates the flux trapping behavior. Anisotropic magnetoresistive (AMR) sensors are inexpensive and small devices that can detect magnetic flux density. The magnetic sensitivities of AMR sensors need to be evaluated at liquid helium temperature for the magnetic field mapping of SRF cavities. In this study, a test stand was constructed to calibrate the magnetic sensitivities of AMR sensors in liquid helium, and 110 AMR sensors were tested using this stand. The magnetic sensitivities were evaluated systematically. A solenoid coil was used to control the uniform external magnetic field and to measure the magnetic sensitivity at low temperatures. All AMR sensors exhibited suitable sensitivities to the magnetic field around the SRF cavity. The variation in these sensitivities in all AMR sensors was ~1%. Further, the AMR sensors were found to have sufficient sensitivity for mapping the magnetic field around the exterior surface of the SRF cavity.

43 PARTICLE ACCELERATORS↗