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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 91 records · Page 5
All sourcesNASA NTRSDOE OSTI
DOE OSTI2019

HPCAT: A Static Compression Science Sector at the Advance Photon Source

Static compression is a useful tool to investigate the materials properties and phase behavior both under uniaxial stress and hydrostatic pressure. From evaluation of the equation of state (P-V-T relationship) to a discovery of near-room temperature superconductivity, the use of diamond anvil cells (DAC) and large-volume presses (LVP) as devices for static compression experiments that couple with synchrotron-based x-ray diffraction, spectroscopy, and imaging techniques achieved pioneering, paradigm defining scientific advancements in multidisciplinary fields for the past two decades. High-Pressure Collaborative Access Team (HPCAT) is a sector at the Advanced Photon Source dedicated to developing multiple synchrotron-based x-ray techniques to maximize the utility of DAC and portable-LVP techniques to advance compression science. The beamlines are optimized to adapt various sample environments under extreme P-T conditions. HPCAT is comprised of two insertion device beamlines, one for diffraction and the other for spectroscopy, and two bending magnet beamlines, one for general purpose and the other for white-beam application, respectively. As a result, each beamline’s specification and applications are introduced.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Beamline Spectroscopy of Integrated Circuits With Hard X-Ray Transition Edge Sensors at the Advanced Photon Source

At Argonne National Laboratory, we are developing hard X-ray (2 to 20 keV) Transition Edge Sensor (TES) arrays for beamline science. The significantly improved energy resolution provided by superconducting detectors compared to semiconductor-based energy-dispersive detectors, but with better collection efficiency than wavelength-dispersive instruments, will enable greatly improved X-ray emission and absorption spectroscopic measurements. Additionally, a prototype instrument with 24 microwave-frequency multiplexed pixels is now in testing at the Advanced Photon Source (APS) 1-BM beamline. Initial measurements show an energy resolution ten times better (150 eV compared to < 15 eV) than the silicon-drift detectors currently available to APS beamline users, and in particular demonstrate the ability to resolve closely-spaced emission lines in samples containing multiple transition metal elements, such as integrated circuits. Comparing fluorescence spectra of integrated circuits measured with our TESs at the beamline to those measured with silicon detectors, we find emission lines and elements largely hidden (e.g. Hf alongside Cu) from a semiconductor-based detector but well resolved by a TES. This directly shows the strengths of TES-based instruments in fluorescence mapping.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2019

Methods for operando coherent X-ray diffraction of battery materials at the Advanced Photon Source

Bragg coherent X-ray diffraction imaging has become valuable for visualization of the structural, morphological and strain evolution of crystals in operando electrode materials. As the electrode material particles (either in a single-crystal form or an aggregation form of single crystals) are evenly dispersed and randomly oriented in the electrode laminate, the submicrometer-sized coherent X-ray beam can be used to probe the local properties of electrode material crystals using two approaches. Coherent multi-crystal diffraction provides collective structural information of phase transitions in tens of crystals simultaneously as well as the individual behavior from single crystals, which are oriented at the Bragg condition in the X-ray illumination volume. Bragg coherent diffractive imaging enables one to monitor the evolution of the morphology and strain in individual crystals. This work explores and highlights the Bragg coherent X-ray diffraction measurements of battery electrode materials in operando conditions at the 34-ID-C beamline at the Advanced Photon Source. The experiment is demonstrated with NaNi 1/3 Fe 1/3 Mn 1/3 O 2 , a sodium-ion cathode material loaded in a half cell. Furthermore, the paper will discuss, in detail, the beamline setup, sample mounting and handling, alignment strategies and the data acquisition protocols.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2016

2D/3D cryo x-ray fluorescence imaging at the bionanoprobe at the advanced photon source

Trace elements, particularly metals, play very important roles in biological systems. Synchrotron-based hard X-ray fluorescence microscopy offers the most suitable capabilities to quantitatively study trace metals in thick biological samples, such as whole cells and tissues. In this manuscript, we have demonstrated X-ray fluorescence imaging of frozen-hydrated whole cells using the recent developed Bionanoprobe (BNP). The BNP provides spatial resolution down to 30 nm and cryogenic capabilities. Frozen-hydrated biological cells have been directly examined on a sub-cellular level at liquid nitrogen temperatures with minimal sample preparation.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2019

Data Management at the Advanced Photon Source

Data are crucial to the scientific discoveries enabled by experiments performed at the APS. Presently the APS generates approximately 10 PB of raw experimental data per year from its sixty-six operating beamlines that house over 100 unique instruments. This data is generated as a part of over 6,000 annual experiments performed by over 5,500 facility users each year. Similar to other synchrotrons, the amount of data generated at the APS continues to quickly increase due to beamline advances, such as new measurement techniques, technological advances in detectors, high-throughput instrumentation, multi-modal instruments that can acquire several measurements in a single experiment, and advanced data processing algorithms. This trend is expected to continue in the future. The revolutionized high-energy synchrotron facility proposed in the APS-U project will increase brightness and coherence, leading to further increases in data rates. Successful management of data is of vital importance to the current and future scientific productivity of the APS.

96 KNOWLEDGE MANAGEMENT AND PRESERVATION↗
DOE OSTI2025

SEM/EBSD Characterization of Baffle-Former Bolts Designated for High Energy X-ray Microscopy Studies at the Advanced Photon Source

This report documents the microstructural and surface characterization of two high-fluence baffle-former bolts (BFBs) harvested from a commercial pressurized water reactor (PWR) after nearly four decades of service. These bolts experienced extreme conditions including high neutron fluence, elevated temperatures, corrosive primary water, and sustained mechanical loads, all of which contribute to degradation mechanisms such as irradiation-assisted stress corrosion cracking (IASCC). Using scanning electron microscopy (SEM) and electron backscatter diffraction (EBSD), the study assessed bulk and near-surface microstructures, grain boundary characteristics, and in-service oxide layers. The results revealed significant differences between bolts exposed to 41 dpa and 29 dpa, including differences in recrystallization extent, deformation structures, and oxidation morphology. These findings establish critical baseline data for integration with advanced synchrotron-based high-energy X-ray microscopy (HEXM) and computational crystal plasticity models. Ultimately, the work supports improved mechanistic understanding and predictive capability regarding the long-term performance of reactor core internal components.

Lach, Tim [Oak Ridge National Laboratory (ORNL), O↗
DOE OSTI2018

High-Energy-Resolution Resonant Inelastic (Hard) X-ray Scattering (RIXS) at the Advanced Photon Source

Resonant Inelastic X-ray Scattering (RIXS) is a powerful technique for studying electronic excitations in a wide variety of complex materials and environments with momentum-, energy- and potentially polarization resolution. Since its inception, the development of RIXS instrumentation and scientific subjects of study have benefited from a closely intertwined evolution; improvements in energy resolution and throughput, spurred by specific scientific cases, have in turn made new subjects of study feasible. Early RIXS work in the late 1990s was aimed at the study of charge transfer excitations in transition metal oxides (TMO), including the high-Tc superconducting Cuprates, the Nickelates and Manganites, in which the lowest lying excitations across the optical gap at a few eV from the elastic line could be accessed. As the understanding of strongly correlated electron systems progressed, scientific inquiries were directed towards the orbital degrees of freedom: in many Mott insulators the crystal field splits the degeneracy of the active d-orbitals, and the transitions between levels, the dd excitations, generate spectral features at energy losses of <2 eV. These features could reliably be observed with the state-of-the-art resolution at the time of 100-200 meV. In 2008, a ground-breaking paper appeared, that established RIXS as a probe of magnetic excitations. Magnetism and magnetic ordering are central questions in the study of correlated electron systems, however associated spectral features (“magnons”) lie at a fraction of an eV or even in the sub-10meV regime. A significant advance in energy resolution was necessary to study pressing scientific subjects, including magnetic excitations, in the newly discovered Iridate systems. Also, in 2011 a comprehensive review of the RIXS technique was published, which coined the terms “direct RIXS" and “indirect RIXS" and suggested that, for transition metal compounds, RIXS is most productive when employed at L-absorption edges. Thus, research assignments were divided between the soft- x-ray and hard x-ray communities according to L-edge energies: compounds with 3-d elements to the soft, compounds with 5-d elements to the hard x-ray side and other elements somewhere in-between.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2017

Materials Research with X-ray Micro-beams at the Advanced Photon Source

X-ray scattering has had a rich and prominent place in the history of materials research. For samples that are large single crystals, X-ray diffraction provides very detailed, high-quality information about the atomic structure of almost every kind. However, most engineering materials are not a large single crystal, but mixtures of materials or a poly-crystalline material. Still, X-ray diffraction using X-ray beams significantly larger than the structures being investigated has produced much excellent information. Examples of this are powder diffraction, texture analysis, strain analysis, etc. While these types of analyses have been very useful in providing a microscopic understanding, they do not provide the microscopic information that we really want. What we really want to have is this useful X-ray diffraction information for every volume element in our sample; not just the diffraction information about small volume elements, but all of the volume elements, exactly where they are in our sample, and how each one diffracts. Furthermore this detailed spatial and structural information is what is needed for a full understanding of the source of the properties that we find in engineering materials.

36 MATERIALS SCIENCE↗