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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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NASA NTRS2000

Coupling Satellite and Ground-Based Instruments to Map Climate Forcing by Anthropogenic Aerosols

Climate forcing by anthropogenic aerosols is a significant but highly uncertain factor in global climate change. Only satellites can offer the global coverage essential to reducing this uncertainty; however, satellite measurements must be coupled with correlative, in situ measurements both to constrain the aerosol optical properties required in satellite retrieval algorithms and to provide chemical identification of aerosol sources. This grant funded the first two years of a three-year project which seeks to develop methodologies for combining spaceborne lidar with in-situ aerosol data sets to improve estimates of direct aerosol climate forcing. Progress under this two-year grant consisted in the development and deployment of a new in-situ capability for measuring aerosol 180' backscatter and the extinction-to-backscatter ratio. This new measurement capacity allows definitive lidar/in-situ comparisons and improves our ability to interpret lidar data in terms of climatically relevant quantities such as the extinction coefficient and optical depth. Measurements were made along the coast of Washington State, in Central Illinois, over the Indian Ocean, and in the Central Pacific. Thus, this research, combined with previous measurements by others, is rapidly building toward a global data set of extinction-to-backscatter ratio for key aerosol types. Such information will be critical to interpreting lidar data from the upcoming PICASSO-CENA, or P-C, satellite mission. Another aspect of this project is to investigate innovative ways to couple the lidar-satellite signal with targeted in-situ measurements toward a direct determination of aerosol forcing. This aspect is progressing in collaboration with NASA Langley's P-C lidar simulator and radiative transfer modeling by the University of Lille, France.

Charlson, Robert J.↗
NASA NTRS2000

Coupling Satellite and Ground-Based Instruments to Map Climate Forcing by Anthropogenic Aerosol

Climate forcing by anthropogenic aerosols is a significant but highly uncertain factor in global climate change. Only satellites can offer the global coverage essential to reducing this uncertainty; however, satellite measurements must be coupled with correlative, in situ measurements both to constrain the aerosol optical properties required in satellite retrieval algorithms and to provide chemical identification of aerosol sources. This grant funded the third year of a three-year project which seeks to develop methodologies for combining spaceborne lidar with in-situ aerosol data sets to improve estimates of direct aerosol climate forcing. Progress under this one-year grant consisted in analysis and publication of field studies using a new in-situ capability for measuring aerosol 180 deg backscatter and the extinction-to-backscatter ratio. This new measurement capacity allows definitive lidar/in-situ comparisons and improves our ability to interpret lidar data in terms of climatically relevant quantities such as the extinction coefficient and optical depth. Analyzed data consisted of measurements made along the coast of Washington State, in Central Illinois, over the Indian Ocean, and in the Central Pacific. Thus, this research, combined with previous measurements by others, is rapidly building toward a global data set of extinction-to-backscatter ratio for key aerosol types. Such information will be critical to interpreting lidar data from the upcoming PICASSO-CENA, or P-C, satellite mission. Another aspect of this project is to investigate innovative ways to couple the lidar-satellite signal with target in-situ measurements toward a direct determination of aerosol forcing. This aspect is progressing in collaboration with NASA Langley's P-C lidar simulator.

Charlson, Robert J.↗
NASA NTRS2017

Take-off Engine Particle Emission Indices for In-Service Aircraft at Los Angeles International Airport

We present ground‐based, advected aircraft engine emissions from flights taking off at Los Angeles International Airport. 275 discrete engine take‐off plumes were observed on 18 and 25 May 2014 at a distance of 400 m downwind of the runway. CO2 measurements are used to convert the aerosol data into plume‐average emissions indices that are suitable for modelling aircraft emissions. Total and non‐volatile particle number EIs are of order 1016‐1017 kg‐1 and 1014‐1016 kg‐1, respectively. Black‐carbon‐equivalent particle mass EIs vary between 175‐941 mg kg‐1 (except for the GE GEnx engines at 46 mg kg‐1). Aircraft tail numbers recorded for each take‐off event are used to incorporate aircraft‐ and engine‐specific parameters into the data set. Data acquisition and processing follow standard methods for quality assurance. A unique aspect of the data set is the mapping of aerosol concentration time series to integrated plume EIs, aircraft and engine specifications, and manufacturer‐reported engine emissions certifications. The integrated data enable future studies seeking to understand and model aircraft emissions and their impact on air quality.

Richard H Moore↗
NASA NTRSDate not supplied

TPSAS-NF1676L-11598-DND

Satellite data show a strong summertime maximum in aerosol optical depth (AOD) over the Southeastern (SE) USA that can not be explained by anthropogenic sulfate or organic aerosols at the surface (Goldstein et al., 2009). The biogenic volatile organic compound (BVOC) emissions peak over the same region and models indicate a large source of secondary organic aerosols (SOA) here (van Donkelaar et al., 2007, Zhang et al., 2007, Liao et al., 2007). Aircraft measurements indicate dominance of organic aerosols over sulfates with altitude and models suggest most SOA production from isoprene oxidation takes place above the surface layers. Goldstein et al. (2009) hypothesized that these SOA drive the AOD maximum in summer with an altitude dependence. We examine the distributions of AOD and other optical properties over SE USA using height resolved aerosol data from CALIPSO. We also use AOD data from MODIS and OMI and UV aerosol index from OMI to characterize the aerosols over SE USA.

J Kar↗
NASA NTRS2002

Dynamics and Properties of Global Aerosol using MODIS, AERONET and GOCART Model

Recently produced daily Moderate Resolution Imaging Spectroradiometer (MODIS) aerosol data for the whole year of 2001 are used to show the concentration and dynamics of aerosol over ocean and large parts of the continents. The data were validated against the Aerosol Robotic Network (AERONET) measurements over land and ocean in a special issue in GRL now in press. Monthly averages and a movie based on the daily data are produced and used to demonstrate the spatial and temporal evolution of aerosol. The MODIS wide spectral range is used to distinguish fine smoke and pollution aerosol from coarse dust and salt. The aerosol is observed above ocean and land. The movie produced from the MODIS data provides a new dimension to aerosol observations by showing the dynamics of the system. For example in February smoke and dust emitted from the Sahel and West Africa is shown to travel to the North-East Atlantic. In April heavy dust and pollution from East Asia is shown to travel to North America. In May-June pollution and dust play a dynamical dance in the Arabian Sea and Bay of Bengal. In Aug-September smoke from South Africa and South America is shown to pulsate in tandem and to periodically to be transported to the otherwise pristine Southern part of the Southern Hemisphere. The MODIS data are compared with the Georgia Tech/Goddard Global Ozone Chemistry Aerosol Radiation Transport (GOCART) model to test and adjust source and sink strengths in the model and to study the effect of clouds on the representation of the satellite data.

Kaufman, Yoram↗
NASA NTRS2012

Vertical Profiles of Aerosol Optical Properties Over Central Illinois and Comparison with Surface and Satellite Measurements

Between June 2006 and September 2009, an instrumented light aircraft measured over 400 vertical profiles of aerosol and trace gas properties over eastern and central Illinois. The primary objectives of this program were to (1) measure the in situ aerosol properties and determine their vertical and temporal variability and (2) relate these aircraft measurements to concurrent surface and satellite measurements. Underflights of the CALIPSO satellite show reasonable agreement in a majority of retrieved profiles between aircraft-measured extinction at 532 nm (adjusted to ambient relative humidity) and CALIPSO-retrieved extinction, and suggest that routine aircraft profiling programs can be used to better understand and validate satellite retrieval algorithms. CALIPSO tended to overestimate the aerosol extinction at this location in some boundary layer flight segments when scattered or broken clouds were present, which could be related to problems with CALIPSO cloud screening methods. The in situ aircraft-collected aerosol data suggest extinction thresholds for the likelihood of aerosol layers being detected by the CALIOP lidar. These statistical data offer guidance as to the likelihood of CALIPSO's ability to retrieve aerosol extinction at various locations around the globe.

Sheridan P. J.↗
NASA NTRS2004

Characteristics and Global Impact of Aerosols from Southern Africa and Eastern Asia

Supported mainly by the NASA GACP and ACMAP, we have made significant progress in the global modeling of tropospheric aerosols and their precursors in the past few years, especially in the development of the GOCART model, simulation of anthropogenic and natural aerosols, data analysis of field observations and satellite retrievals, assessment of global and regional budgets, estimate of aerosol direct radiative forcing, and aerosol forecasting and data analysis for the ACE-Asia field experiment. Our results and findings are summarized in Chin et al. Model calculated multiple-year optical thickness for individual and total aerosols are at internet. These results have been frequently used by other groups, for example, to impose initial conditions for regional models, provide dust source functions for other global models, supply aerosol fields for chemistry and climate models, help data group interpret their measurements, select monitoring sites for ground observation network, and assist satellite retrievals.

Chin, Mian↗
NASA NTRS2002

MODIS and AERONET Characterization of the Global Aerosol

Recently produced daily MODIS aerosol data for the whole year of 2001 are used to show the concentration and dynamics of aerosol over ocean and large parts of the continents. The data were validated against the Aerosol Robotic Network (AERONET) measurements over land and ocean. Monthly averages and a movie based on the daily data are produced and used to demonstrate the spatial and temporal evolution of aerosol. The MODIS wide spectral range is used to distinguish fine smoke and pollution aerosol from coarse dust and salt. The movie produced from the MODIS data provides a new dimension to aerosol observations by showing the dynamics of the system. For example in February smoke and dust emitted from the Sahel and West Africa is shown to travel to the North-East Atlantic. In April heavy dust and pollution from East Asia is shown to travel to North America. In May-June pollution and dust play a dynamical dance in the Arabian Sea and Bay of Bengal. In Aug-September smoke from South Africa and South America is shown to pulsate in tandem and to periodically to be transported to the otherwise pristine Southern part of the Southern Hemisphere.

Kaufman, Yoram↗
NASA NTRS1982

Aerosol measurements from earth orbiting spacecraft

The global aerosol data base evolving from monitoring being done by Stratospheric Aerosol Measurement (SAM) II and Stratospheric Aerosol and Gas Experiment (SAGE) since the fall of 1978 is presented. Data reveal that polar stratospheric clouds (PSC) enhance extinction and optical depths by up to two orders of magnitude and an order of magnitude, respectively. These data are over background 1000 nm values of approximately 1.2 x 10 to the -4th per km, and 1.3 x 10 to the -3rd, respectively. SAGE has offered, for the first time, quantitative measurements of volcanic eruptions on a nearly global basis, and estimates are given for the amount of aerosol injected into the stratosphere from each volcano. For example, Northern Hemisphere aerosol was enhanced by more than 100% by the 1980 eruption of Mount St. Helens, which produced about 0.32 x 10 to the 6th metric tons of aerosol. A cirrus cloud data base is being developed which will be useful in earth radiation and water vapor budget studies. Cross-section, contour, and temperature variation diagrams are included.

Mccormick, M. P.↗
NASA NTRS1989

Global backscatter assessment

The focus of this effort is the development of a global-scale model of aerosol backscatter for laser atmospheric wind sounder (LAWS) design and performance studies. Background parameters are derived from aerosol data sets with global-scale spatial and/or temporal coverage, using objective statistical decomposition and/or a priori stratification based on supplementary data. Backscatter coefficients at the LAWS design wavelength are derived from background aerosol physical, chemical, and optical data, or from direct backscatter measurements at other wavelengths, using background conversion factors. Direct measurements of aerosol backscatter at 10.6 microns from the Royal Signals and Radar Establishment (RSRE) and the Wave Propagation Laboratory (WPL) were selected. The RSRE backscatter data processing code were optimized under low backscatter conditions, performed detailed analyses of collocated intercomparisons between the two lidars, and assisted in the analysis of the long-term backscatter climatologies from the two lidars. Timely presentation of global backscattering experiment (GLOBE) research results to the global geophysical community is required.

Bowdle, David A.↗
NASA NTRS1991

Tropospheric ozone and aerosols measured by airborne lidar during the 1988 Arctic boundary layer experiment

Ozone (O3) and aerosol distributions were measured from an aircraft using a differential absorption lidar (DIAL) system as part of the 1988 NASA Global Tropospheric Experiment - Arctic Boundary Layer Experiment (ABLE-3A) to study the sources and sinks of gases and aerosols over the tundra regions of Alaska during the summer. The tropospheric O3 budget over the Arctic was found to be strongly influenced by stratospheric intrusions. Regions of low aerosol scattering and enhanced O3 mixing ratios were usually correlated with descending air from the upper troposphere or lower stratosphere. Several cases of continental polar air masses were examined during the experiment. The aerosol scattering associated with these air masses was very low, and the atmospheric distribution of aerosols was quite homogeneous for those air masses that had been transported over the ice for greater than or = 3 days. The transition in O3 and aerosol distributions from tundra to marine conditions was examined several times. The aerosol data clearly show an abrupt change in aerosol scattering properties within the mixed layer from lower values over the tundra to generally higher values over the water. The distinct differences in the heights of the mixed layers in the two regions was also readily apparent. Several cases of enhanced O3 were observed during ABLE-3 in conjunction with enhanced aerosol scattering in layers in the free atmosphere. Examples are presented of the large scale variations of O3 and aerosols observed with the airborne lidar system from near the surface to above the tropopause over the Arctic during ABLE-3.

Browell, Edward V.↗
NASA NTRS2004

Multisensor Fire Observations

This DVD includes animations of multisensor fire observations from the following satellite sources: Landsat, GOES, TOMS, Terra, QuikSCAT, and TRMM. Some of the animations are included in multiple versions of a short video presentation on the DVD which focuses on the Hayman, Rodeo-Chediski, and Biscuit fires during the 2002 North American fire season. In one version of the presentation, MODIS, TRMM, GOES, and QuikSCAT data are incorporated into the animations of these wildfires. These data products provided rain, wind, cloud, and aerosol data on the fires, and monitored the smoke and destruction created by them. Another presentation on the DVD consists of a panel discussion, in which experts from academia, NASA, and the U.S. Forest Service answer questions on the role of NASA in fighting forest fires, the role of the Terra satellite and its instruments, including the Moderate Resolution Imaging Spectroradiometer (MODIS), in fire fighting decision making, and the role of fire in the Earth's climate. The third section of the DVD features several animations of fires over the years 2001-2003, including animations of global and North American fires, and specific fires from 2003 in California, Washington, Montana, and Arizona.

Boquist, C.↗
NASA NTRS2000

Preliminary Results from an Assimilation of TOMS Aerosol Observations Into the GOCART Model

At NASA Goddard we are developing a global aerosol data assimilation system that combines advances in remote sensing and modeling of atmospheric aerosols. The goal is to provide high resolution, 3-D aerosol distributions to the research community. Our first step is to develop a simple assimilation system for Saharan mineral aerosol. The Goddard Chemistry and Aerosol Radiation model (GOCART) provides accurate 3-D mineral aerosol size distributions that compare well with TOMS satellite observations. Surface, mobilization, wet and dry deposition, convective and long-range transport are all driven by assimilated fields from the Goddard Earth Observing System Data Assimilation System, GEOS-DAS. Our version of GOCART transports sizes from.08-10 microns and only simulates Saharan dust. TOMS radiance observations in the ultra violet provide information on the mineral and carbonaceous aerosol fields. We use two main observables in this study: the TOMS aerosol index (AI) which is directly related to the ratio of the 340 and 380 radiances and the 380 radiance. These are sensitive to the aerosol optical thickness, the single scattering albedo and the height of the aerosol layer. The Goddard Aerosol Assimilation System (GAAS) uses the Data Assimilation Office's Physical-space Statistical Analysis System (PSAS) to combine TOMS observations and GOCART model first guess fields. At this initial phase we only assimilate observations into the the GOCART model over regions of Africa and the Atlantic where mineral aerosols dominant and carbonaceous aerosols are minimal, Our preliminary results during summer show that the assimilation with TOMS data modifies both the aerosol mass loading and the single scattering albedo. Assimilated aerosol fields will be compared with assimilated aerosol fields from GOCART and AERONET observations over Cape Verde.

daSilva, Arlindo↗
NASA NTRS2016

An AERONET-Based Aerosol Classification Using the Mahalanobis Distance

We present an aerosol classification based on AERONET aerosol data from 1993 to 2012. We used the AERONET Level 2.0 almucantar aerosol retrieval products to define several reference aerosol clusters which are characteristic of the following general aerosol types: Urban-Industrial, Biomass Burning, Mixed Aerosol, Dust, and Maritime. The classification of a particular aerosol observation as one of these aerosol types is determined by its five-dimensional Mahalanobis distance to each reference cluster. We have calculated the fractional aerosol type distribution at 190 AERONET sites, as well as the monthly variation in aerosol type at those locations. The results are presented on a global map and individually in the supplementary material. Our aerosol typing is based on recognizing that different geographic regions exhibit characteristic aerosol types. To generate reference clusters we only keep data points that lie within a Mahalanobis distance of 2 from the centroid. Our aerosol characterization is based on the AERONET retrieved quantities, therefore it does not include low optical depth values. The analysis is based on point sources (the AERONET sites) rather than globally distributed values. The classifications obtained will be useful in interpreting aerosol retrievals from satellite borne instruments.

Hamill, Patrick↗
NASA NTRS2016

Retrieving the Height of Smoke and Dust Aerosols by Synergistic Use of Multiple Satellite Sensors

The Aerosol Single scattering albedo and Height Estimation (ASHE) algorithm was first introduced in Jeong and Hsu (2008) to provide aerosol layer height and single scattering albedo (SSA) for biomass burning smoke aerosols. By using multiple satellite sensors synergistically, ASHE can provide the height information over much broader areas than lidar observations alone. The complete ASHE algorithm uses aerosol data from MODIS or VIIRS, OMI or OMPS, and CALIOP. A simplified algorithm also exists that does not require CALIOP data as long as the SSA of the aerosol layer is provided by another source. Several updates have recently been made: inclusion of dust layers in the retrieval process, better determination of the input aerosol layer height from CALIOP, improvement in aerosol optical depth (AOD) for nonspherical dust, development of quality assurance (QA) procedure, etc.

satellite remote sensing↗
NASA NTRS2020

How Long Is Too Long? Variogram Analysis of AERONET Data to Aid Aerosol Validation and Intercomparison Studies

Geophysical data sets derived from satellite sensors, ground/airborne instrumentation, and computational models are often compared against each other. A common example is the validation of satellite aerosol optical depth (AOD) retrievals against measurements from Aerosol Robotic Network (AERONET) Sun photometers. Spatiotemporal mismatch between data set sampling means that uncaptured variation in the underlying geophysical field introduces apparent disagreement into such comparisons, known as representation or collocation matchup uncertainty. This study uses variogram analysis of AERONET data to estimate temporal mismatch uncertainties and decorrelation time scales for the global AERONET record. As well as total AOD, the fine‐ and coarse‐mode AODs, Ångström Exponent (AE), and fine‐mode fraction (FMF) of AOD are analyzed. Globally, a time difference of 30 min typically induces from 0.011–0.035 variation in AOD. For total, fine, and coarse AODs the typical time to decorrelation is around 2–10 days. For AE and FMF it is 3–33 days; that is, aerosol systems often persist significantly longer than individual events in them. Biomass burning regions tend to show the largest and fastest subdaily AOD variability and also longest times to decorrelation. Some sites show significant season‐to‐season variations in behavior. These results can be used to inform site‐specific time collocation thresholds for aerosol validation analyses and account for temporal variation when estimating data set uncertainty. They also have implications for comparisons between different satellite products or models, data aggregation, and time series analyses. Results are provided on a site‐by‐site basis to facilitate use by other researchers.

satellite↗
NASA NTRS2010

Understanding Aerosol Direct Radiative Forcing - How Satellites Fit In

The aerosol data products from the NASA Earth Observing System's MISR and MODIS instruments provide significant advances in regional and global aerosol optical depth (AOD) mapping, aerosol type measurement, and source plume characterization from space. Although these products have been and are being used for many applications, ranging from regional air quality assessment, to aerosol air mass type identification and evolution, to aerosol injection height and aerosol transport model validation, uncertainties still limit the quantitative constraints these satellite data place on global-scale direct aerosol radiative forcing. Some further refinement of the current aerosol products is possible, but a major advance in this area seems to require a different paradigm, involving the integration of satellite and suborbital data with models. This presentation will briefly summarize where we stand, and what incremental advances we can expect, with the current aerosol products, and will then elaborate on some initial steps aimed at the necessary integration of data from multiple sources and models.

Kahn, R. A.↗
NASA NTRS2009

A Critical Look at Deriving Monthly Aerosol Optical Depth from Satellite Data

Satellite-derived aerosol data sets, such as those provided by NASA's Moderate Resolution Imaging Spectroradiometer (MODIS) instruments, are greatly improving our understanding of global aerosol optical depth (AOD). Yet, there are sampling issues. MODIS specific orbital geometry, convolved with the need to avoid bright surfaces (glint, desert, clouds, etc.), means that AOD can be under- or over-sampled in places. When deriving downstream products, such as daily or monthly gridded AOD, one must consider the spatial and temporal density of the measurements relative to the gradients of the true AOD. Additionally, retrieval confidence criteria should be considered. Averaged products are highly dependent on choices made for data aggregation and weighting, and sampling errors can be further propagated when deriving regional or global mean AOD. Different choices for aggregation and weighting result in estimates of regional and global means varying by 30% or more. The impacts of a particular averaging algorithm vary by region and surface type and can be shown to represent different tolerance for clouds and retrieval confidence.

Levy, R. C.↗