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NASA NTRS1994

Observations of lower-stratospheric ClONO2, HNO3, and aerosol by the UARS CLAES experiment between January 1992 and April 1993

This paper discusses simultaneous measurements of stratospheric ClONO2, HNO3, temperature, and aerosol extinction coefficient by the Cryogenic Limb Array Etalon Spectrometer (CLAES) on the NASA Upper Atmosphere Research Satellite (UARS), obtained over the period 9 January 1992 through 23 April 1993. The discussion concentrates on the stratosphere region near 21 km of particular interest to heterogeneously driven ozone depletion. For periods between 12 June and 1 September 1992 at latitudes poleward of about 60 deg S, when temperatures were below type I polar stratospheric cloud (PSC) formation thresholds throughout the lower stratosphere, CLAES observed high levels of PSCs coincident with highly depleted fields of both HNO3 and ClONO2. By 17 September, the incidence of PSCs had greatly diminished in the lower stratosphere, but both CLONO2 and HNO3 remained highly depleted. These observations are consistent with the removal of gaseous HNO3 through the formation of nitric acid trihydrate (NAT) particles and the removal of ClONO2 through heterogeneous reactions on the particle surfaces. They also suggest substantial denitrification of the lower Antarctic vortex through sedimentation of PSC particles. In the Northern Hemisphere winter of 1992/93 far fewer PSCs were observed in the Arctic lower-stratosphere vortex, which had shorter periods and more localized regions of cold temperatures. Both HNO3 and ClONO2 maintained much higher levels inside the Arctic vortex than seen in the Antarctic throughout the winter/spring period. Following 28 February 1993 when Arctic vortex temperatures rose above 195 K, ClONO2 was observed in large quantities (greater than 2.1 ppbv near 21 km) inside the vortex. The persistence of relatively high levels of HNO3 inside the Arctic spring vortex compared with the low levels seen in the Antarctic spring vortex suggest a much lower level of denitrification in the Arctic.

Roche, A. E.↗

NASA NTRS1988

In situ observations of ClO in the wintertime Northern Hemisphere: ER-2 aircraft results from 21 N to 61 N latitude

Measurements of lower stratospheric ClO taken during a NASA ER-2 flight between Moffett Field, CA (37 N, 122 W) and Great Slave Lake, Canada (61 N, 116 W) on 13 February 1988 are reported. Northbound, the aircraft was flown at about 20 km altitude from 39 N to 56 N, at 18 km from there to 58 N, in a descent to 15 km at 60 N, and in a rise and turn at the northernmost point. The southbound leg was flown in a gradual climb from 20 km to 21.5 km. On this day, the central position of the Arctic polar vortex, as determined by an NMC analysis of heights and temperatures at the 50 mb and 70 mb levels, was approximately 79 N, 100 W. Because the vortex was located on the North American side of the pole, the aircraft was able to reach a point slightly inside the maximum horizontal wind region where wind speeds were 80 to 90 knots. The general pattern for the observed ClO is that it increased with both latitude and altitude, and attained a maximum of about 55 pptv at 61 N latitude and 20.5 km altitude. This value is about 20 times smaller than the maxima observed over Antarctica, but is comparable to those seen just outside the chemical containment vessel located inside the Antarctic Polar vortex. On the other hand, in a comparison with northern midlatitude data taken on this and three other February flights, ClO mixing ratios observed north of 55 N latitude are 2 to 5 times larger at all flight altitudes (15 to 20 km). Possible reasons are discussed for this enhancement over midlatitude and the evidence is considered for whether or not the instruments sampled Arctic polar vortex air. A second feature of the data is the strong positive correlation between ClO and O3 during the entire flight.

Brune, W. H.↗

NASA NTRS1990

In situ observations of ClO in the Arctic Stratosphere - ER-2 aircraft results from 59 deg N to 80 deg N latitude

Large abundances of ClO were observed inside the Arctic polar vortex during 14 flights of the NASA ER-2 aircraft from Stavanger, Norway (59 deg N, 6 deg E) to 80 deg N latitude. Flights were conducted at altitudes between 14 and 20 km when the solar zenith angle was between 79 and 101 deg. Data are reported for three flights that represent the main features observed during the mission. These data, comparable to those obtained in the Antarctic ozone hole, indicate that the springtime Arctic polar vortex was extensively perturbed by heterogeneous chemistry and contained enough ClO to catalytically destroy ozone rapidly.

Brune, W. H.↗

NASA NTRS2006

EOS Microwave Limb Sounder Observations of 'Frozen-in' Anticyclonic Air in Arctic Summer

A previously unreported phenomenon, a 'frozen-in' anticyclone (FrIAC) after the 2005 Arctic spring vortex breakup, was discovered in Earth Observing System (EOS) Microwave Limb Sounder (MLS) long-lived trace gas data. A tongue of low-latitude (high-N2O, low-H2O) air was drawn into high latitudes and confined in a tight anticyclone, then advected intact in the summer easterlies through late August. A similar feature in O3 disappeared by early April as a result of chemical processes. The FrIAC was initially advected upright at nearly the same speed at all levels from approx.660 to 1300 K (approx.25-45 km); increasing vertical wind shear after early June tilted the FrIAC and weakened it at higher levels. The associated feature in PV disappeared by early June; transport calculations fail to reproduce the remarkable persistence of the FrIAC, suggesting deficiencies in summer high-latitude winds. The historical PV record suggests that this phenomenon may have occurred several times before. The lack of a persistent signature in O3 or PV, along with its small size and rapid motion, make it unlikely that a FrIAC could have been reliably identified without hemispheric daily longlived trace gas profiles such as those from EOS MLS.

Arctic vortex↗

NASA NTRS1990

A comparison of ER-2 measurements of stratospheric water vapor between the 1987 Antarctic and 1989 Arctic Airborne missions

Vertical profiles of water vapor inside the Antarctic vortex have been compared with those taken outside it over Punta Arenas (53 deg S, 71 deg W). A similar exercise was performed with Arctic vortex profiles and those taken over Stavanger (59 deg N, 6 deg E). Residual water, defined as the stratospheric water vapor mixing ratio with the contribution from methane oxidation subtracted, is also shown as profiles inside and outside the vortex for both missions. The Arctic and Antarctic profiles of water vapor and residual water are compared. Locally dehydrated air was evident both inside and outside the Antarctic vortex, but such dehydration was not evident in and around the Arctic vortex. Arctic profiles of residual water are consistent with nontropical entry for some air.

Kelly, K. K.↗

NASA NTRS2006

Chemical Observations of a Polar Vortex Intrusion

An intrusion of vortex edge air in D the interior of the Arctic polar vortex was observed on the January 31,2005 flight of the NASA DC-8 aircraft. This intrusion was identified as anomalously high values of ozone by the AROTAL and DIAL lidars. Our analysis shows that this intrusion formed when a blocking feature near Iceland collapsed, allowing edge air to sweep into the vortex interior. along the DC-8 flight track also shows the intrusion in both ozone and HNO3. Polar Stratospheric Clouds (PSCs) were observed by the DIAL lidar on the DC-8. The spatial variability of the PSCs can be explained using MLS HNO3 and H2O observations and meteorological analysis temperatures. We also estimate vortex denitrification using the relationship between N2O and HNO3. Reverse domain fill back trajectory calculations are used to focus on the features in the MLS data. The trajectory results improve the agreement between lidar measured ozone and MLS ozone and also improve the agreement between the HNO3 measurements PSC locations. The back trajectory calculations allow us to compute the local denitrification rate and reduction of HCl within the filament. We estimate a denitrification rate of about lO%/day after exposure to below PSC formation temperature. Analysis of Aura MLS observations made

Schoeberl, M. R.↗

NASA NTRS1995

Isentropic mixing in the Arctic stratosphere during the 1992-1993 and 1993-1994 winters

Dynamic isolation of the winter Arctic circumpolar vortex during 1992-1993 and 1993-1994 (the second and third northern hemisphere winters of the UARS mission) is studied using quasi-horizontal isentropic trajectories. Ejection of vortex air and entrainment of mid-latitude air into the vortex are quantified and compared with climatological values obtained from the analysis of 16 Arctic winters. A number of unusual features of both winters are discussed. The most notable features are the anomalous isolation experienced by the vortex during December 1992 and the unusual degree of isolation and persistence of the vortex during February and March of both years. the 1992-1993 winter season is the most consistently isolated vortex on record. Only during January 1993, when entrainment is large, is this pattern of extreme isolation broken.

Dahlberg, Steven P.↗

NASA NTRS1995

Interhemispheric differences in polar stratospheric HNO3, H2O, ClO, and O3

Simultaneous global measurements of nitric acid (HNO3), water (H2O), chlorine monoxide (ClO), and ozone (O3) in the stratosphere have been obtained over complete annual cycles in both hemispheres by the Microwave Limb Sounder on the Upper Atmosphere Research Satellite. A sizeable decrease in gas-phase HNO3 was evident in the lower stratospheric vortex over Antarctica by early June 1992, followed by a significant reduction in gas-phase H2O after mid-July. By mid-August, near the time of peak ClO, abundances of gas-phase HNO3 and H2O were extremely low. The concentrations of HNO3 and H2O over Antarctica remained depressed into November, well after temperatures in the lower stratosphere had risen above the evaporation threshold for polar stratospheric clouds, implying that denitrification and dehydration had occurred. No large decreases in either gas-phase HNO3 or H2O were observed in the 1992-1993 Arctic winter vortex. Although ClO was enhanced over the Arctic as it was over the Antarctic, Arctic O3 depletion was substantially smaller than that over Antarctica. A major factor currently limiting the formation of an Arctic ozone 'hole' is the lack of denitrification in the northern polar vortex, but future cooling of the lower stratosphere could lead to more intense denitrification and consequently larger losses of Arctic ozone.

Santee, M. L.↗

NASA NTRS1990

Aircraft deployment, and airborne arctic stratospheric expedition

The Airborne Arctic Stratospheric Expedition had two primary objectives: to study the production and loss mechanisms of ozone in the north polar stratosphere and to study the effect on ozone distribution of the Arctic Polar Vortex and of the cold temperatures associated with the formation of Polar Stratospheric Clouds. Two specially instrumented NASA aircraft were flown over the Arctic region. Each aircraft flew to acquire data on the meteorological, chemical and cloud physical phenomena that occur in the polar stratosphere during winter. The chemical processes which occur in the polar stratosphere during winter were also observed and studied. The data acquired are being analyzed.

Condon, Estelle↗

NASA NTRS1999

Polar Stratospheric Descent of NO(y) and CO and Arctic Denitrification During Winter 1992-1993

Observations inside the November 1994 Antarctic stratospheric vortex and inside the April 1993 remnant Arctic stratospheric vortex by the Atmospheric Trace Molecule Spectroscopy (ATMOS) Fourier transform spectrometer are reported. In both instances, elevated volume mixing ratios (VMRS) of carbon monoxide (CO) were measured. A peak Antarctic CO VMR of 60 ppbv (where 1 ppbv = 10(exp -9) per unit Volume) was measured at a potential temperature of 710 K (about 27 km), about 1 km below the altitude of a pocket of elevated NO(y) (total reactive nitrogen) at a deep minimum in N2O (<5 ppbv). The Arctic observations also show a region of elevated vortex CO with a peak VMR of 90 ppbv it 630-670 K (-25 km) but no corresponding enhancement in NO(sub y) perhaps because of stronger dynamical activity in the northern hemisphere polar winter and/or interannual variability in the production of mesospheric or lower thermospheric NO. By comparing vortex and extravortex observations of NO(y) obtained at the same N2O VMR, Arctic vortex denitrification of 5 +/- 2 ppbv at 470 K (at approximately 18 km) is inferred. We show that our conclusion of substantial Arctic winter 1992-1993 denitrification is robust by comparing our extravortex observations with previous polar measurements obtained over a wide range of winter conditions. Correlations of NO(y) with N2O measured at the same potential temperature by ATMOS in the Arctic vortex and at midlatitudes on board the ER-2 aircraft several weeks later lie along the same mixing line. The result demonstrates the consistency of the two data sets and confirms that the ER-2 sampled fragments of the denitrified Arctic vortex following its breakup. An analysis of the ATMOS Arctic measurements of total hydrogen shows no evidence for significant dehydration inside the vortex.

Rinsland, C. P.↗

NASA NTRS2015

Future Changes in Major Stratospheric Warmings in CCMI Models

Major stratospheric warmings (MSWs) are one of the most important phenomena of wintertime Arctic stratospheric variability. They consist of a warming of the Arctic stratosphere and a deceleration of the polar night jet, triggered by an anomalously high injection of tropospheric wave activity into the stratosphere. Due to the relevance and the impact of MSWs on the tropospheric circulation, several model studies have investigated their potential responses to climate change. However, a wide range of results has been obtained, extending from a future increase in the frequency of MSWs to a decrease. These discrepancies might be explained by different factors such as a competition of radiative and dynamical contributors with opposite effects on the Arctic polar vortex, biases of models to reproduce the related processes, or the metric chosen for the identification of MSWs. In this study, future changes in wintertime Arctic stratospheric variability are examined in order to obtaina more precise picture of future changes in the occurrence of MSWs. In particular, transient REFC2 simulations of different CCMs involved in the Chemistry Climate Model Initiative (CCMI) are used. These simulations extend from 1960 to 2100 and include forcings by halogens and greenhouse gases following the specifications of the CCMI-REF-C2 scenario. Sea surface temperatures (SSTs) and sea-ice distributions are either prescribed from coupled climate model integrations or calculated internally in the case of fully coupled atmosphere-ocean CCMs. Potential changes in the frequency and main characteristics of MSWs in the future are investigated with special focus on the dependence of the results on the criterion for the identification of MSWs and the tropospheric forcing of these phenomena.

Chemistry-Climate Modeling↗

NASA NTRS1993

In situ measurements of the ClO/HCl ratio: Heterogeneous processing on sulfate aerosols and polar stratospheric clouds

Simultaneous in situ measurements of stratospheric ClO and HCl have been made for the first time, during numerous flights of the ER-2 aircraft covering latitudes 24-90 deg N from October 1991 through March 1992. The ClO/HCl ratio is identified as a key indicator of heterogeneous processing both outside and within the Arctic polar vortex. For ClO mixing ratios below about 120 pptv, remarkably constant ClO/HCl values of about 15% characterize the lower stratosphere. The observed values are significantly higher than those derived from a 2-D model using either gas phase photochemistry alone (2%), or including heterogeneous sulfate chemistry (5-10%). During the Arctic early spring, after conversion of HCl into reactive chlorine has taken place, the vortex edge is poorly defined by ClO levels. Loss of HCl and its slow recovery following low-temperature polar heterogeneous chemistry distinguishes HCl as a new and unique dynamical tracer of polar stratospheric clouds (PSC)-processed air.

Webster, C. R.↗

NASA NTRS1993

In Situ Measurements of the ClO/HCl Ratio: Heterogeneous Processing on Sulfate Aerosols and Polar Stratospheric Clouds

Simultaneous in situ measurements of stratospheric ClO and HCl have been made for the first time, during numerous flights of the ER-2 aircraft covering latitudes 24-90 deg. N from October 1991 through March 1992. The ClO/HCl ratio is identified as a key indicator of heterogeneous processing both outside and within the Arctic polar vortex. For ClO mixing ratios below about 120 pptv, remarkably constant ClO/HCl values of about 15% characterize the lower stratosphere. The observed values are significantly higher than those derived from a 2-D model using either gas phase photochemistry alone (2%), or including heterogeneous sulfate chemistry (5-10%). During the Arctic early spring, after conversion of HCl into reactive chlorine has taken place, the vortex edge is poorly defined by ClO levels. Loss of HCl and its slow recovery following low-temperature polar heterogeneous chemistry distinguishes HCl as a new and unique dynamical tracer of PSC-processed air.

Webster, C. R.↗

NASA NTRS1993

In Situ Measurements of the ClO/HCl Ratio: Heterogeneous Processing on Sulfate Aerosols and Polar Stratospheric Clouds

Webster, C. R.↗

NASA NTRS2022

Seasonal Variability in the Mechanisms Behind the 2020 Siberian Heatwaves

Record-breaking heatwaves and wildfires immersed Siberia during the boreal spring of 2020 following an anomalously warm winter. Springtime heatwaves are becoming more common in the region, with statistically significant trends in the frequency, magnitude, and duration of heatwave events over the past four decades. Mechanisms by which the heatwaves occur and contributing factors differ by season. Winter heatwave frequency is correlated with the atmospheric circulation, particularly the Arctic Oscillation, while the frequency of heatwaves during the spring months is highly correlated with aspects of the land surface including snow cover, albedo, and latent heat flux. Idealized AMIP-style experiments are used to quantify the contribution of suppressed Arctic sea ice and snow cover over Siberia on the atmospheric circulation, surface energy budget, and surface air temperature in Siberia during the winter and spring of 2020. Sea ice concentration contributed to the strength of the stratospheric polar vortex and Arctic Oscillation during the winter months, thereby influencing the tropospheric circulation and surface air temperature over Siberia. Warm temperatures across the region resulted in an earlier-than-usual recession of the winter snowpack. The exposed land surface contributed to up to 20% of the temperature anomaly during the spring through the albedo feedback and changes in the ratio of the latent and sensible heat fluxes. This, in combination with favorable atmospheric circulation patterns, resulted in record-breaking heatwaves in Siberia in the spring of 2020.

Allison B. Marquardt Collow↗

NASA NTRS1994

Arctic chlorine monoxide observations during spring 1993 over Thule, Greenland, and implications for ozone depletion

We have determined the vertical distribution of chlorine monoxide (ClO), from measurements of pressure-broadened molecular-emission spectra made over Thule, Greenland, during the 1993 Arctic spring. The measurements show a weak lower stratospheric layer of chlorine monoxide inside the vortex in late February, which was, however, significantly greater in mixing ratio than that seen in observations we made in the spring of 1992. ClO was also observed in much smaller quantities in early to mid-March 1993 when Thule was outside the vortex. The amount of ClO within the vortex was severely reduced by the time it returned over Thule in late March. This reduction occurred several weeks earlier relative to the winter solstice than the decline of ClO inside the Antarctic vortex in 1993. The enhanced Arctic lower stratospheric layer seen in late February 1993 at a nearly equivalent photochemical period, and beyond. We have calculated daily ozone loss rates, due primarily to the dimer chlorine catalytic cycle, from both sets of measurements. The vertical integral of the Arctic daily percentage ozone loss when the largest ClO levels were present, at the end of February, is found to be approximately one quarter of that in the Antarctic at a photochemical period only 1 week later. The relative weakness of daily ozone depletion, combined with the early disappearance of ClO in the Arctic, suggests that hemispheric dilution by ozone-poor air from within the Arctic vortex is unlikely to be sufficient to explain the historically extreme loss of midlatitude northern hemisphere ozone which began in 1992 and persisted throughout 1993.

Shindell, D. T.↗

NASA NTRS2002

Dynamical and chemical contributions to variability in microwave limb sounder Arctic stratoshperic column ozone

Analyses of column ozone above 100 hPa (Col100) derived from Upper Atmosphere Research Satellite Microwave Limb Sounder (MLS) data in February/March 1992-1998 show that about half of the interannual variability in Col100 in the Arctic polar vortex in late winter results from interannual variability in chemical loss. A majority of the remainder results from interannual variability in day-to-day dynamical motions including adiabatic warming/cooling and poleward advection of underlying upper tropospheric subtropical air on short timescales, rather than from variations in descent rates and large-scale transport over the winters. The morphology of Col100 from MLS remains very similar to that in the dynamical models even in the years with most chemical ozone loss. The amount and character of day-to-day variability in dynamical models closely follows that in MLS Col100. Although the morphology of and day-to-day variability in Arctic column ozone are controlled by dynamical processes, chemical ozone loss was a major factor in producing both the low values of and the large interannual variability in Arctic column ozone observed during the 1990s.

Arctic ozone loss↗

NASA NTRS2000

What Controls the Temperature of the Arctic Stratosphere during the Spring?

Understanding the mechanisms that control the temperature of the polar lower stratosphere during spring is key to understanding ozone loss in the Arctic polar vortex. Spring ozone loss rates are directly tied to polar stratospheric temperatures by the formation of polar stratospheric clouds, and the conversion of chlorine species to reactive forms on these cloud particle surfaces. In this paper, we study those factors that control temperatures in the polar lower stratosphere. We use the National Centers for Environmental Prediction (NCEP)/NCAR reanalysis data covering the last two decades to investigate how planetary wave driving of the stratosphere is connected to polar temperatures. In particular, we show that planetary waves forced in the troposphere in mid- to late winter (January-February) are principally responsible for the mean polar temperature during the March period. These planetary waves are forced by both thermal and orographic processes in the troposphere, and propagate into the stratosphere in the mid and high latitudes. Strong mid-winter planetary wave forcing leads to a warmer Arctic lower stratosphere in early spring, while weak mid-winter forcing leads to cooler Arctic temperatures.

Newman, Paul A.↗