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At least 91 records · Page 5

Backscatter laser depolarization studies of simulated stratospheric aerosols - Crystallized sulfuric acid droplets

The optical depolarizing properties of simulated stratospheric aerosols were studied in laboratory laser (0.633 micrometer) backscattering experiments for application to polarization lidar observations. Clouds composed of sulfuric acid solution droplets, some treated with ammonia gas, were observed during evaporation. The results indicate that the formation of minute ammonium sulfate particles from the evaporation of acid droplets produces linear depolarization ratios of beta equivalent to 0.02, but beta equivalent to 0.10 to 0.15 are generated from aged acid cloud aerosols and acid droplet crystalization effects following the introduction of ammonia gas into the chamber. It is concluded that partially crystallized sulfuric acid droplets are a likely candidate for explaining the lidar beta equivalent to 0.10 values that have been observed in the lower stratosphere in the absence of the relatively strong backscattering from homogeneous sulfuric acid droplet (beta equivalent to 0) or ice crystal (beta equivalent to 0.5) clouds.

Sassen, Kenneth↗

Low-pressure electrical discharge experiment to simulate high-altitude lightning above thunderclouds

Recently, extremely interesting high-altitude cloud-ionosphere electrical discharges, like lightning above thunderstorms, have been observed from NASA's space shuttle missions and during airborne and ground-based experiments. To understand these discharges, a new experiment was conceived to simulate a thundercloud in a vacuum chamber using a dielectric in particulate form into which electrodes were inserted to create charge centers analogous to those in an electrified cloud. To represent the ionosphere, a conducting medium (metallic plate) was introduced at the top of the chamber. It was found that for different pressures between approximately 1 and 300 mb, corresponding to various upper atmospheric altitudes, different discharges occurred above the simulated thundercloud, and these bore a remarkable similarity to the observed atmospheric phenomena. At pressures greater than 300 mb, these discharges were rare and only discharges within the simulated thundercloud were observed. Use of a particulate dielectric was critical for the successful simulation of the high-altitude lightning.

Jarzembski, M. A.↗

Lyophilized spore dispenser

A lyophilized spore dispenser is provided which produces a finely divided, monoparticulate cloud of bacterial spores. The spores are contained within a tightly sealed chamber, and a turbulator orifice connected to an air supply source provides a jet of air which stirs up the spores and causes the spores to be suspended in eddy currents within the chamber. This air jet also produces a positive pressure within the chamber which forces the spores out of an injection orifice.

Jessup, A. D.↗

The Chemical Evolution of Cosmic Dust: From Gas-Phase Precursors to Solid Grains - Laboratory Studies with the COSmIC Facility

Cosmic dust in in its gas phase and solid phase components plays an essential role in the chemical and physical evolution of the universe. Our understanding of cosmic dust properties relies on a combination of astronomical observations, astrophysical modeling and laboratory studies of realistic analogs of cosmic dust being gas-phase molecules and/or solid grains. The COSmIC facility was developed at NASA Ames to study the evolution of cosmic carbon from circumstellar outflows to interstellar clouds to planetary atmospheres in the laboratory. COSmIC stands for “Cosmic Simulation Chamber” and is dedicated to the study of neutral and ionized molecules and grain particles under the low temperature and density conditions that are required to simulate space environments. It integrates a variety of instruments that allow generating, processing, and monitoring simulated space conditions in the laboratory. It is composed of a Pulsed Discharge Nozzle (PDN) expansion that generates a plasma in a free supersonic jet expansion, coupled to high-sensitivity, complementary in situ diagnostic tools used for the detection and characterization of the species present in the expansion: Cavity Ring Down Spectroscopy (CRDS) and fluorescence spectroscopy systems for photonic detection and an orthogonal Reflectron Time-Of-Flight Mass Spectrometer (oReTOF-MS) for mass detection. Recent advances achieved using COSmIC’s laboratory data in synergy with observational data will be presented. These results include the formation of dust grains and aerosols from gas-phase molecular precursors in environments as varied as circumstellar outflows of late AGB stars and planetary atmospheres [4] and the evolution of our understanding of the diffuse interstellar bands (DIBs) with applications to the ESO Diffuse Interstellar Bands Large Exploration Survey (EDIBLES). Plans for future laboratory developments and techniques to study the evolution of cosmic carbon molecules and grains (including NIR-MIR CRDS, laser induced fluorescence (LIF) and incandescence (LII)) will also be addressed as well as their astronomical applications.

Farid Salama↗

The Chemical Evolution of Cosmic Carbon: Laboratory Studies with the COSmIC Facility

Cosmic dust plays an essential role in our understanding of the chemical and physical evolution of the universe. Our understanding of cosmic dust relies on a combination of astronomical observations (either remote or on extraterrestrial dust samples), astrophysical modeling and laboratory studies of realistic analogs of cosmic dust grains. The COSmIC facility was developed at NASA Ames to study the evolution of cosmic carbon from circumstellar outflows to interstellar clouds to planetary atmospheres in the laboratory [1]. COSmIC stands for “Cosmic Simulation Chamber” and is dedicated to the study of neutral and ionized molecules and grain particles under the low temperature and density conditions that are required to simulate space environments. COSmIC integrates a variety of instruments that allow generating, processing, and monitoring simulated space conditions in the laboratory. It is composed of a Pulsed Discharge Nozzle (PDN) expansion that generates a plasma in a free supersonic jet expansion, coupled to high-sensitivity, complementary in situ diagnostic tools used for the detection and characterization of the species present in the expansion: Cavity Ring Down Spectroscopy (CRDS) and fluorescence spectroscopy systems for photonic detection and an orthogonal Reflectron Time-Of-Flight Mass Spectrometer (oReTOF-MS) for mass detection. Recent advances achieved in laboratory astrophysics using COSmIC’s laboratory data in synergy with observational data will be presented. These results include the formation of dust grains and aerosols from gas-phase molecular precursors in environments as varied as circumstellar outflows of late AGB stars [2] and planetary atmospheres [3] and the evolution of our understanding of the diffuse interstellar bands (DIBs) with applications to the ESO Diffuse Interstellar Bands Large Exploration Survey (EDIBLES [4, 5]). Plans for future laboratory developments and techniques to study the evolution of cosmic carbon molecules and grains (including NIR-MIR CRDS, laser induced fluorescence (LIF) and incandescence (LII)) will also be addressed as well as their astronomical applications.

Salama, F.↗

The Chemical Evolution of Cosmic Dust: From Gas-Phase Precursors to Solid Grains - Laboratory Studies with the COSmIC Facility

Cosmic dust in in its gas phase and solid phase components plays an essential role in the chemical and physical evolution of the universe. Our understanding of cosmic dust properties relies on a combination of astronomical observations, astrophysical modeling and laboratory studies of realistic analogs of cosmic dust being gas-phase molecules and/or solid grains. The COSmIC facility was developed at NASA Ames to study the evolution of cosmic carbon from circumstellar outflows to interstellar clouds to planetary atmospheres in the laboratory [1]. COSmIC stands for “Cosmic Simulation Chamber” and is dedicated to the study of neutral and ionized molecules and grain particles under the low temperature and density conditions that are required to simulate space environments. It integrates a variety of instruments that allow generating, processing, and monitoring simulated space conditions in the laboratory. It is composed of a Pulsed Discharge Nozzle (PDN) expansion that generates a plasma in a free supersonic jet expansion, coupled to high-sensitivity, complementary in situ diagnostic tools used for the detection and characterization of the species present in the expansion: Cavity Ring Down Spectroscopy (CRDS) and fluorescence spectroscopy systems for photonic detection and an orthogonal Reflectron Time-Of-Flight Mass Spectrometer (oReTOF-MS) for mass detection. Recent advances achieved using COSmIC’s laboratory data in synergy with observational data will be presented. These results include the formation of dust grains and aerosols from gas-phase molecular precursors in environments as varied as circumstellar outflows of late AGB stars [2, 3] and planetary atmospheres [4] and the evolution of our understanding of the diffuse interstellar bands (DIBs) with applications to the ESO Diffuse Interstellar Bands Large Exploration Survey (EDIBLES [5, 6]). Plans for future laboratory developments and techniques to study the evolution of cosmic carbon molecules and grains (including NIR-MIR CRDS, laser induced fluorescence (LIF) and incandescence (LII)) will also be addressed as well as their astronomical applications.

Planetary↗

A cloud condensation nucleus spectrometer designed for airborne measurements

The spectrometer is a simple extension of the continuous flow diffusion chamber (CFDC) operated in the vertical mode. The principal new design features of the instrument are its rapid time response and ability to rapidly measure the CCN activity spectrum. The activity spectrum of CCN in an air sample is measured by simultaneously operating the spectrometer at four supersaturations. The CCN spectrometer consists of four essentially indepenent CFDC's in a parallel array. Each CFDC is 61 cm long, 10 cm wide, and consists of two vertical parallel plates 1 cm apart, maintained at different temperatures. Each CFDC has a single particle optical counter located at the center of its base.

Radke, L. F.↗

Project S'COOL

The Students Clouds Observations On-Line or S'COOL project was piloted in 1997. It was created with the idea of using students to serve as one component of the validation for the Clouds and the Earth's Radiant Energy System (CERES) instrument which was launched with the Tropical Rainfall Measuring Mission (TRMM) in November, 1997. As part of NASA's Earth Science Enterprise CERES is interested in the role clouds play in regulating our climate. Over thirty schools became involved in the initial thrust of the project. The CERES instrument detects the location of clouds and identifies their physical properties. S'COOL students coordinate their ground truth observations with the exact overpass of the satellite at their location. Their findings regarding cloud type, height, fraction and opacity as well as surface conditions are then reported to the NASA Langley Distributed Active Archive Center (DAAC). The data is then accessible to both the CERES team for validation and to schools for educational application via the Internet. By March of 1998 ninety-three schools, in nine countries had enrolled in the S'COOL project. Joining the United States participants were from schools in Australia, Canada, France, Germany, Norway, Spain, Sweden, and Switzerland. The project is gradually becoming the global project envisioned by the project s creators. As students obtain the requested data useful for the scientists, it was hoped that students with guidance from their instructors would have opportunity and motivation to learn more about clouds and atmospheric science as well.

Green, Carolyn J.↗

Atmospheric scavenging of hydrochloric acid

The scavenging of hydrogen chloride from a solid rocket exhaust cloud was investigated. Water drops were caused to fall through a confined exhaust cloud and then analyzed to determine the amount of HCl captured during fall. Bubblers were used to measure HCl concentration within the chamber. The measured chamber HCl concentration, together with the measured HCl deposition on the chamber walls, accounted for 81 to 94% of the theoretical HCl. It was found that the amount of HCl captured was approximately one-half of that predicted by the Frossling correlation. No effect of humidity was detected through a range of 69-98% R.H.. The scavenging of HCl from a solid rocket exhaust cloud was calculated using an idealized Kennedy Space Center rain cycle. Results indicate that this cycle would reduce the cloud HCl concentration to 20.6% if its value in the absence of rain.

Knutson, E. O.↗

Modification of the continuous flow diffusion chamber for use in zero-gravity

The design philosophy and performance characteristics of the continuous flow diffusion chamber developed for use in ground-based simulation of some of the experiments planned for the atmospheric cloud physics laboratory during the first Spacelab flight are discussed. Topics covered include principle of operation, thermal control, temperature measurement, tem-powered heat exchangers, wettable metal surfaces, sample injection system, and control electronics.

Keyser, G.↗

A Balloon-Borne Cloud Condensation Nuclei Counter

A balloon-borne instrument was constructed for observations of vertical profiles of cloud condensation nucleus (CCN) concentrations, active at 1% supersaturation. Droplet concentration in the static thermal-gradient diffusion chamber is deduced from the amount of scattered laser light detected by a photodetector. The photodetector is calibrated using a video camera and computer system to count the number of droplets produced from NaCl aerosol. Preliminary data are available from nine early morning profiles obtained at Laramie, Wyoming, between June 1995 and January 1997. To complement the CCN measurements, instruments that measure condensation nuclei (CN) and aerosols with diameter greater than 0.30 micrometers (D(sub 0.3) were also included on the balloon package. CCN concentrations exhibited a general decrease from the surface to the top of the boundary layers, were generally uniform through well-mixed layers, and show variability above well-mixed layers. In general, the structure of the CCN profile appears to be closely related to the structure in the CN and D(sub 0.3) profiles. Summer profiles generally have CCN concentration greater than 200/cu cm up to 500 mbar, whereas winter profiles are less than 200/cu cm at all levels.

Delene, David J.↗

Warm/cold cloud processes

Final development of a gravimetric test for performance evaluation of a precision saturator is described. The design and development of a prototype droplet levitation chamber is discussed. Technical assistance to the MSFC Airborne Laser Doppler Program is reported.

Davis, M. H.↗

Ice nucleus concentrations measured during the 1975 Florida Area Cumulus Experiment /FACE/

Ice nuclei measurements were made aboard a cloud-base aircraft during the 1975 Florida Area Cumulus Experiment. Two techniques were used to obtain the ice nuclei concentrations; membranes were collected and analyzed using the NCAR membrane development chamber and continuous ice nuclei concentrations were obtained using the NCAR acoustical counter. Results showed that the membrane technique failed to effectively detect ice nuclei in this maritime tropical area. However, the concentrations recorded by the acoustical counter showed natural afternoon diurnal increases which may have ramifications on cloud development and seeding potential within the particular study area.

Wisniewski, J.↗

Estimates of the Lightning NOx Profile in the Vicinity of the North Alabama Lightning Mapping Array

The NASA Marshall Space Flight Center Lightning Nitrogen Oxides Model (LNOM) is applied to August 2006 North Alabama Lightning Mapping Array (LMA) data to estimate the raw (i.e., unmixed and otherwise environmentally unmodified) vertical profile of lightning nitrogen oxides, NOx = NO + NO 2 . This is part of a larger effort aimed at building a more realistic lightning NOx emissions inventory for use by the U.S. Environmental Protection Agency (EPA) Community Multiscale Air Quality (CMAQ) modeling system. Data from the National Lightning Detection Network TM (NLDN) is also employed. Overall, special attention is given to several important lightning variables including: the frequency and geographical distribution of lightning in the vicinity of the LMA network, lightning type (ground or cloud flash), lightning channel length, channel altitude, channel peak current, and the number of strokes per flash. Laboratory spark chamber results from the literature are used to convert 1-meter channel segments (that are located at a particular known altitude; i.e., air density) to NOx concentration. The resulting raw NOx profiles are discussed.

Koshak, William J.↗

Estimates of the Lightning NOx Profile in the Vicinity of the North Alabama Lightning Mapping Array

The NASA Marshall Space Flight Center Lightning Nitrogen Oxides Model (LNOM) is applied to August 2006 North Alabama Lightning Mapping Array (NALMA) data to estimate the (unmixed and otherwise environmentally unmodified) vertical source profile of lightning nitrogen oxides, NOx = NO + NO2. Data from the National Lightning Detection Network (Trademark) (NLDN) is also employed. This is part of a larger effort aimed at building a more realistic lightning NOx emissions inventory for use by the U.S. Environmental Protection Agency (EPA) Community Multiscale Air Quality (CMAQ) modeling system. Overall, special attention is given to several important lightning variables including: the frequency and geographical distribution of lightning in the vicinity of the NALMA network, lightning type (ground or cloud flash), lightning channel length, channel altitude, channel peak current, and the number of strokes per flash. Laboratory spark chamber results from the literature are used to convert 1-meter channel segments (that are located at a particular known altitude; i.e., air density) to NOx concentration. The resulting lightning NOx source profiles are discussed.

Koshak, William J.↗

Students as Ground Observers for Satellite Cloud Retrieval Validation

The Students' Cloud Observations On-Line (S'COOL) Project was initiated in 1997 to obtain student observations of clouds coinciding with the overpass of the Clouds and the Earth's Radiant Energy System (CERES) instruments on NASA's Earth Observing System satellites. Over the past seven years we have accumulated more than 9,000 cases worldwide where student observations are available within 15 minutes of a CERES observation. This paper reports on comparisons between the student and satellite data as one facet of the validation of the CERES cloud retrievals. Available comparisons include cloud cover, cloud height, cloud layering, and cloud visual opacity. The large volume of comparisons allows some assessment of the impact of surface cover, such as snow and ice, reported by the students. The S'COOL observation database, accessible via the Internet at http://scool.larc.nasa.gov, contains over 32,000 student observations and is growing by over 700 observations each month. Some of these observations may be useful for assessment of other satellite cloud products. In particular, some observing sites have been making hourly observations of clouds during the school day to learn about the diurnal cycle of cloudiness.

Chambers, Lin H.↗

Zinc Nucleation and Growth in Microgravity

We report our experiences with zinc nucleation in a microgravity environment aboard NASA's Reduced Gravity Research Facility. Zinc vapor is produced by a heater in a vacuum chamber containing argon gas. Nucleation is induced by cooling and its onset is easily detected visually by the appearance of a cloud of solid, at least partially crystalline zinc particles. Size distribution of these particles is monitored in situ by photon correlation spectroscopy. Samples of particles are also extracted for later analysis by SEM. The initially rapid increase in particle size is followed by a slower period of growth. We apply Scaled Nucleation Theory to our data and find that the derived critical temperature of zinc, the critical cluster size at nucleation, and the surface tension values are all in reasonably good agreement with their accepted literature values.

Michael, B. Patrick↗

Optical properties of CO2 ice and CO2 snow from ultraviolet to infrared: Application to frost deposits and clouds on Mars

Researchers found that it is possible to grow large clear samples of CO2 ice at Mars-like temperatures of 150-170K if a temperature controlled refrigerator is connected to an isolated two-phase pure CO2 system. They designed a chamber for transmission measurements whose optical path between the 13mm diameter window is adjustable from 1.6mm to 107mm. This will allow measurements of linear absorption down to less than 0.01 cm (exp -1). A preliminary transmission spectrum of a thick sample of CO2 ice in the near infrared was obtained. Once revised optical constants have been determined as a function of wavelength and temperature, they can be applied to spectral reflectance/emissivity models for CO2 snow surfaces, both pure and contaminated with dust and water ice, using previously established approaches. It will be useful, also, to develop an infrared scattering-emission cloud radiance model (especially as viewed from near the limb) in order to develop a strategy for the identification of CO2 cloud layers by the atmospheric infrared radiometer instrument on the Mars Observer.

Hansen, Gary B.↗