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Saha-Langmuir surface ionization relation.
Discrepancy between observed ion production rate in cesium thermionic converter and Saha-Langmuir equation prediction suggests locality of ion formation
Coherence mapping to identify the intermediates of multi-channel dissociative ionization
Identifying the short-lived intermediates and reaction mechanisms of multi-channel radical cation fragmentation processes remains a current and important challenge to understanding and predicting mass spectra. We find that coherent oscillations in the femtosecond time-dependent yields of several product ions following ultrafast strong-field ionization represent spectroscopic signatures that elucidate their mechanism of formation and identify the intermediate(s) they originate from. Experiments on endo-dicyclopentadiene show that vibrational frequencies from various intermediates are mapped onto their resulting products. Aided by ab initio methods, we identify the vibrational modes of both the cleaved and intact molecular ion intermediates. These results confirm stepwise and concerted fragmentation pathways of the dicyclopentadiene ion. This study highlights the power of tracking the femtosecond dynamics of all product ions simultaneously and sheds further light onto one of the fundamental reaction mechanisms in mass spectrometry, the retro-Diels Alder reaction.
Abrasion-ablation model for neutron production in heavy ion reactions
In heavy ion reactions, neutron production at forward angles is observed to occur with a Gaussian shape that is centered near the beam energy and extends to energies well above that of the beam. This paper presents an abrasion-ablation model for making quantitative predictions of the neutron spectrum. To describe neutrons produced from the abrasion step of the reaction where the projectile and target overlap, the authors use the Glauber model and include effects of final-state interactions. They then use the prefragment mass distribution from abrasion with a statistical evaporation model to estimate the neutron spectrum resulting from ablation. Measurements of neutron production from Ne and Nb beams are compared with calculations, and good agreement is found.
Role of Collective Effects in Dominance of Scattering Off Thermal Ions Over Langmuir Wave Decay: Analysis, Simulations, and Space Applications
Langmuir waves driven to high levels by beam instabilities are subject to nonlinear processes, including the closely related processes of scattering off thermal ions (STI) and a decay process in which the ion response is organized into a product ion acoustic wave. Calculations of the nonlinear growth rates predict that the decay process should always dominate STI, creating two paradoxes. The first is that three independent computer simulation studies show STI proceeding, with no evidence for the decay at all. The second is that observations in space of type 3 solar radio bursts and Earth's foreshock, which the simulations were intended to model, show evidence for the decay proceeding but no evidence for STI. Resolutions to these paradoxes follow from the realization that a nonlinear process cannot proceed when its growth rate exceeds the minimum frequency of the participating waves, since the required collective response cannot be maintained and the waves cannot respond appropriately, and that a significant number of e-foldings and wave periods must be contained in the time available. It is shown that application of these 'collective' and 'time scale' constraints to the simulations explains why the decay does not proceed in them, as well as why STI proceeds in specific simulations. This appears to be the first demonstration that collective constraints are important in understanding nonlinear phenomena. Furthermore, applying these constraints to space observations, it is predicted that the decay should proceed (and dominate STI) in type 3 sources and the high beam speed regions of Earth's foreshock for a specific range of wave levels, with a possible role for STI alone at slightly higher wave levels. Deeper in the foreshock, for slower beams and weaker wave levels, the decay and STI are predicted to become ineffective. Suggestions are given for future testing of the collective constraint and an explanation for why waves in space are usually much weaker than in the simulations.
Saha-Langmuir surface ionization relation
Ion production rate in cesium thermionic converter related to Saha-Langmuir surface ionization equation
Light Ion Double-Differential Cross Sections for Space Radiation
Neutrons and light ions have been shown to make large contributions to space radiation dose equivalent for realistic shielding scenarios. However, there are considerable uncertainties in the calculation of light ion production. Efficient and accurate calculation of light ion double-differential cross sections are required for input into space radiation transport codes. A thermal proton cross section model is developed which includes proton production from the 3 sources of projectile, central fireball, and target. It is shown that this 3-source model is able to explain the low-momentum, small-angle shoulder seen in proton spectra. Using the coalescence model, the thermal proton model is used to calculate light ion double-differential cross sections for use in space radiation transport codes. The 3-source model is also seen to be essential to explain the light ion shoulders, which are even more pronounced than the proton shoulders. Extensive comparisons between models and experimental measurements are shown and necessary future work is discussed.
Ionization probability of iron particles at meteoritic velocities
Ion production for ablation of micron size iron particles moving at supersonic speed in air and argon
Performance of the CELSS Antarctic Analog Project (CAAP) Crop Production System
Regenerative life support systems potentially offer a level of self-sufficiency and a concomitant decrease in logistics and associated costs in support of space exploration and habitation missions. Current state-of-the-art in plant based, regenerative life support requires resources in excess of resource allocations proposed for candidate mission scenarios. Feasibility thresholds have been identified for candidate exploration missions. The goal of this paper is to review recent advances in performance achieved in the CELSS Antarctic Analog Project (CAAP) in light of likely resource constraints. A prototype CAAP crop production chamber has been constructed and operated at the Ames Research Center. The chamber includes a number of unique hardware and software components focused on attempts to increase production efficiency, increase energy efficiency, and control the flow of energy and mass through the system to achieve enhanced performance efficiency. Both single crop, batch production, and continuous cultivation of mixed crops Product ion scenarios have been completed. The crop productivity as well as engineering performance of the chamber will be described. For each scenario, energy required and partitioned for lighting, cooling, pumps, fans, etc. is quantified. Crop production and the resulting lighting efficiency and energy conversion efficiencies are presented. In the mixed-crop scenario, with up to 25 different crops under cultivation, 17 sq m of crop area provided a mean of 515 g edible biomass per day (83% of the approximately 620 g required for one person). Lighting efficiency (moles on photons kWh-1) approached 4 and the conversion efficiency of light energy to biomass was greatly enhanced compared with conventional growing systems. Engineering and biological performance achieved place plant-based life support systems at the threshold of feasibility.
Ion cyclotron resonance study of the secondary ion-molecule reactions in hexafluoroethane.
Secondary ion production in electron impact decomposition of hexafluoroethane, using ion cyclotron double resonance techniques
Star of Condor - A strontium critical velocity experiment, Peru, 1983
'Star of Condor' was a critical velocity experiment using Sr vapor produced in a radial shaped charge, which was carried to 571.11 km altitude on a Taurus-Tomahawk rocket launched from Punto Lobos, Peru, and detonated in the plane of the magnetic field lines so that all ranges of pitch angles from parallel to B to perpendicular to B were covered. Sr has a critical velocity of 3.3 km/s, and from observation, 42.5 percent of the neutral Sr gas had a velocity component perpendicular to B exceeding that value. No Sr ion emissions were detected shortly after the burst with usual TV integration times. However, about 10 min after the detonation a faint field-aligned streak was discovered with long TV integration times. The brightness is estimated as 5 R, which, combined with the streak geometry, implies an ion production of 2.4 x 10 to the 19th ions. This is only 0.0036 percent ionization of the Sr vapor. All the ions could easily have been produced by thermal ionization from the original detonation thermal distribution. The breakup of the Sr gas into small bloblike structures may have allowed the high-energy electrons to escape before an ionization cascade could be produced. For whatever reason, the Alfven mechanism proposed for space plasmas in the absence of laboratory walls did not produce an ionization cascade in the experiment.
Characteristics of ring-cusp discharge chambers
Measurements have been obtained for the operating characteristics of a 30 cm diameter ring-cusp ion thruster (RCIT), quantitatively comparing its performance parameters to those of a divergent-field J-series cluster of the same size. The high level of performance established for the RCIT is due to its maintenance of both a higher primary-electron population and Maxwellian-electron temperature, as the beam-ion production cost is reduced to its baseline value. Ion losses to the discharge-chamber walls can be reduced by an applied electrostatic field.
Ion Storage Tests with the High Performance Antimatter Trap (HiPAT)
The NASA/Marshall Space Flight Centers (NASA/MSFC) Propulsion Research Center (PRC) is evaluating an antiproton storage system, referred to as the High Performance Antiproton Trap (HiPAT). This interest stems from the sheer energy represented by matter/antimatter annihilation process with has an energy density approximately 10 order of magnitude above that of chemical propellants. In other terms, one gram of antiprotons contains the equivalent energy of approximately 23 space shuttle external tanks or ET's (each ET contains roughly 740,000 kgs of fuel and oxidizer). This incredible source of stored energy, if harnessed, would be an enabling technology for deep space mission where both spacecraft weight and propulsion performance are key to satisfying aggressive mission requirements. The HiPAT hardware consists of a 4 Tesla superconductor system, an ultra high vacuum test section (vacuum approaching 10(exp -12) torr), and a high voltage confinement electrode system (up to 20 kvolts operation). The current laboratory layout is illustrated. The HiPAT designed objectives included storage of up to 1 trillion antiprotons with corresponding lifetimes approaching 18 days. To date, testing has centered on the storage of positive hydrogen ions produced in situ by a stream of high-energy electrons that passes through the trapping region. However, due to space charge issues and electron beam compression as it passes through the HiPAT central field, current ion production is limited to less then 50,000 ions. Ion lifetime was determined by counting particle populations at the end of various storage time intervals. Particle detection was accomplished by destructively expelling the ions against a micro-channel plate located just outside the traps magnetic field. The effect of radio frequency (RF) stabilization on the lifetime of trapped particles was also examined. This technique, referred to as a rotating wall, made use of a segmented electrode located near the center of the trap on which various phases of a particular frequency were applied. Various experiments were performed illustrating the ability of an RF drive to both prolong and reduced the lifetimes of various ion species depending on the selected frequency. HiPAT is now being reconfigured for testing with an ion source that will provide both positive and negative hydrogen ions from an external source. This ion system shall provide higher fill capacity (order of million of ions per shot), stacking of multiple shots, and injection schemes typical of a realistic antiproton delivery system.
Overview of the High Performance Antiproton Trap (HiPAT) Experiment
A general overview of the High Performance Antiproton Trap (HiPAT) Experiment is presented. The topics include: 1) Why Antimatter? 2) HiPAT Applicability; 3) Approach-Goals; 4) HiPAT General Layout; 5) Sizing For Containment; 6) Laboratory Operations; 7) Vacuum System Cleaning; 8) Ion Production Via Electron Gun; 9) Particle Capture Via Ion Sources; 10) Ion Beam Steering/Focusing; 11) Ideal Ion Stacking Sequence; 12) Setup For Dynamic Capture; 13) Dynamic Capture of H(+) Ions; 14) Dynamic Capture; 15) Radio Frequency Particle Detection; 16) Radio Frequency Antenna Modeling; and 17) R.F. Stabilization-Low Frequencies. A short presentation of propulsion applications of Antimatter is also given. This paper is in viewgraph form.
Association reactions at low pressure. 5: The CH3(+)/HCN system. A final word?
The reaction of the methyl cation with hydrogen cyanide is revisited. We have confidence that we have resolved a long standing apparent contradiction of experimental results. A literature history is presented along with one new experiment and a re-examination of an old experiment. In this present work it is shown that all of the previous studies had made consistent observations. Yet, each of the previous studies failed to observe all of the information present. The methyl cation does react with HCN by radiative association, a fact which had been in doubt. The product ions formed in the two-body and three-body processes react differently with HCN. The collisionally stabilized association product formed by a three-body mechanism, does not react with HCN and is readily detected in the experiments. The radiatively stabilized association product, formed by a slow two-body reaction, is not detected because it reacts with HCN by a fast proton transfer reaction forming the protonated HCN ion. Previous studies either 'lost' this product in the extremely large protonated HCN signal that is always present when HCN is used, or discounted it for various reasons. We have been able to show by ion cyclotron resonance (ICR) techniques (both FT-ICR and tandem ICR-dempster-ICR) that the radiative association product does react with the HCN to form the protonated HCN ion.
Ion flow experiments in a multipole discharge chamber
It has been customary to assume that ions flow nearly equally in all directions from the ion production region within an electron-bombardment discharge chamber. Ion flow measurements in a multipole discharge chamber have shown that this assumption is not true. In general, the electron current through a magnetic field can alter the electron density, and hence the ion density, in such a way that ions tend to be directed away from the region bounded by the magnetic field. When this mechanism is understood, it becomes evident that many past discharge chamber designs have operated with a preferentially directed flow of ions.
Ion Mobility Drift Spectrometer (IMDS) as a flight analytical instrument technique
A detailed knowledge of the history and abundances of the biogenic elements and their compounds throughout the solar system can provide the exobiologists with a basis for understanding the conditions necessary for chemical evolution and the origin of life. The Ion Mobility Drift Spectrometer is an ion molecule reactor coupled with an ion drift spectrometer. Sample molecules are ionized to form product ions in the reactant region. An electric field moves the ions through a drift region against the flow of a drift gas where they are separated according to their size and structure producing an ion mobility spectrum. These spectra provide the IMDS with virtually universal sample identification capability. To conform to the rigid limits of weight, volume and consumables placed on flight instrumentation, several aspects of the IMDS must be studied and redesigned for flight use. In addition to miniaturization of the instrument, a reduction in the high flow rates used for the drift gas is an obvious necessary consideration. The effect of drastically reduced drift flow rates on IMDS spectra was investigated by lowering flow rates from 500ml/min to 50ml/min. Changes in peak shape, drift time and total spectra were studied at each flow rate.
Advanced electric propulsion research, 1989
Results of an experimental study of the characteristics of ion thruster hollow cathodes operating at high discharge currents (up to 60 A) are presented in a companion report. This work shows that ions produced near the cathode orifice can acquire sufficient energy to induce the high sputter erosion rates on cathode potential surfaces that have been observed in ion thrusters. A mechanism by which these ions could be produced is also described. A second, brief study showing how a discharge chamber model developed previously can be applied to determine optimal values for one or more discharge chamber design parameters is presented. The experimental approach being used to study the plasma potential field and charge-exchange ion production rate downstream of the accelerator grid of an ion thruster is discussed and preliminary results are presented.