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At least 91 records · Page 5

IER 489: Critical Unresolved Region Integral Experiment (CURIE) CEDT Phase-2 Final Design

The final design for the CURIE integral benchmark experiment is presented in this report. Measurements will be performed on the Comet vertical assembly machine and include various critical configurations consisting of High Enriched Uranium (HEU) metal plates and Teflon moderator plates surrounded by a thick copper reflector. The various configurations with different Teflon plate thickness planned allow for complimentary measurements with differing nuclear data sensitivity in the Unresolved Resonance Region (URR). Similar to previously performed Zeus experiments, the proposed work will serve to validate vital nuclear data quantities and uncertainties and identify deficiencies in current radiation transport codes. Additionally, it will assess the applicability of optimization approaches to nuclear critical experiment design. The final experiment design is detailed in this report and includes design, optimization, uncertainty and continuous-energy nuclear data sensitivity analysis for the final experimental configurations that will provide the basis for a future benchmark evaluation intended for submission to the International Criticality Safety Benchmark Evaluation Project (ICSBEP) Handbook [1]. This document discusses the method, approach, considerations and final design chosen with conclusions. It also includes cost and schedule. The basis and principles of this document come from the preliminary design report [2]. Section 2 discusses the content and potential impact; section 3 gives an overview of the nuclear data and unresolved resonance region; section 4 gives a summary of the work done during the preliminary design; section 5 discusses the machine learning method and principles used for final design; section 6 summaries the results from final design; section 7 provides conclusions and the range of configurations chosen to carry forward to experiment execution; and section 8 includes a summary of costs.

42 ENGINEERING↗

Bayesian Optimization Framework for Imperfect Data or Models

Conventional Bayesian optimization methods implicitly assume that the data and model being optimized are “perfect.” This assumption leads to inaccurate posterior probability distribution functions (PDFs) when applied to “imperfect” data or models. The new Bayesian optimization framework presented in this report provides a way to parameterize the effect of imperfections usually encountered in a prior PDF of generalized data or a model on the posterior PDF. The effects of imperfections are parameterized by a set of constraints imposed on the posterior expectation values of deviations between the data and the model and on their covariance matrix elements. A particular set of values for these constraints conveys an evaluator’s best estimate of the effect of imperfections on the corresponding posterior expectation values. When a prior PDF of generalized data is assumed to be normal, an expression for a posterior PDF satisfying an arbitrary set of constraints is derived analytically for linear models. An analogous iterative algorithm is given for nonlinear models. The corresponding posterior PDF should be used to estimate any posterior expectation values in the presence of imperfections parameterized by that set of constraints. A posterior PDF of a conventional Bayesian optimization method is recovered analytically when all evaluator-specified constraints are set to zero (i.e., in the absence of any imperfections). The analytical expressions derived in this report for normal PDFs and linear models were verified numerically by a Metropolis–Hastings Monte Carlo method. The methods presented herein could be applied to any kind of data or models, including differential cross-section data or integral benchmark experiments.

97 MATHEMATICS AND COMPUTING↗

Updates and Validation for the n+ 63,65 Cu Cross Sections [Slides]

The RRR and URR parameters for 63,65 Cu have been optimized to transmission and capture data. Several data sets have been newly incorporated in this evaluation. The angular distribution parameters have been adopted from differential measurements, as was done in ENDF/B-V. The performance of this evaluation in the integral benchmark calculations is favorable, and the validation is ongoing.

07 ISOTOPE AND RADIATION SOURCES↗

Review of SCALE Validations Applicable to Spent Nuclear Fuel Shielding Calculations

This report presents a review of publicly available documents providing validations of SCALE code system capabilities for depletion and shielding calculations. The validation studies primarily used information available in the Spent Fuel Isotopic Composition Database, the Shielding Integral Benchmark Archive and Database, and the International Criticality Safety Benchmark Evaluation Project Handbook. Validation results based on radiochemical assay data and shielding benchmark experiments relevant to spent nuclear fuel shielding applications are summarized in this report. The information summarized in this report supports pressurized water reactor and boiling water reactor spent fuel storage and transportation safety analyses.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Integral Experiment Final Design for Thermal/Epithermal eXperiments with 233U3O8 ZPR Fuel Elements and Polyethylene (IER-329 CED-2 Report)

This report documents the integral experiment final design for IER-329, Thermal/Epithermal eXperiments (TEX) with 233 U 3 O 8 Zero Power Reactor (ZPR) Fuel Elements and Polyethylene. IER-329 (TEX-23) is the third baseline design in the Thermal/Epithermal eXperiments (TEX) series led by Lawrence Livermore National Laboratory (LLNL) and funded by the DOE’s Nuclear Criticality Safety Program. This experiment was designed to address the existing 233U integral benchmark experiments over prediction in k eff by up to 2% for thermal systems and under-prediction in k eff by up to 4% for intermediate systems. The TEX-23 design utilizes assemblies of 233 U 3 O 8 Zero Power Reactor (ZPR) fuel elements moderated and reflected by high-density polyethylene. This design is similar to the existing TEX-Pu and TEX-HEU designs, utilizing an adjustable moderator to tune the neutron energy spectra and modular layers for the incorporation of diluent materials.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Integral Experiment Validation of Hafnium with TEX-HEU and TEX-Hf [Slides]

Lead by Lawrence Livermore National Laboratory under the U.S. Department of Energy's Nuclear Criticality Safety Program. The goal of TEX is to provide integral benchmark experiments than span the entire neutron energy spectrum and incorporate high-priority materials. TEX includes two test bed configurations providing a baseline for comparison to better understand the contribution of additional materials

Highly Enriched Uranium↗

ORNL FY2024 Nuclear Data Evaluation Contributions: Cu, La, N, and Ta [Slides]

63,65 Cu angular distributions resolved for ENDF/B-VIII.1, consistent with both differential data and integral benchmark performance. 139 La RRR and URR evaluations will be merged with the LANL high energy evaluation, and to be submitted to the future ENDF-B release (post-VIII.1). 14 N RRR evaluation is planned to produce n+ 14 N, p+ 14 C, and a+ 11 B contributions to be submitted to the future ENDF-B release (post-VIII.1). 181 Ta covariances repaired and reported as intended in an errata to ENDF/B-VIII.1.

139-La↗

NCSP supports 240 Pu prompt fission neutron spectrum (PFNS) evaluation

A new 240 Pu PFNS evaluation was recently undertaken at LANL as a strategic priority. It truly is an NCSP end-to-end product. It factors in a new differential experiment funded by NCSP, builds on theoretical work coming out of a previous NCSP nuclear data evaluation milestone and was validated with an NCERC experiment that was recently evaluated as an integral benchmark with NCSP funds.

240Pu↗

Advancing Inverse Sensitivity/Uncertainty Methods for Nuclear Fuel Cycle Applications

The inverse sensitivity/uncertainty quantification (IS/UQ) method has recently been implemented in the Inverse Sensitivity/UnceRtainty Estimiator (INSURE) module of the AMPX system [1]. The IS/UQ method aims to quantify and prioritize the cross section measurements along with uncertainties needed to yield a given nuclear application(s) target response uncertainty, and doing this at a minimum cost. Since in some cases the extant uncertainties of the differential cross section data are already near the limits of the present-day state-of-the-art measurements, requiring significantly smaller uncertainties may be unrealistic. Therefore we have incorporated integral benchmark experiments (IBEs) data into the IS/UQ method using the generalized linear least-squares method, and have implemented it in the INSURE module. We show how the IS/UQ method could be applied to systematic and statistical uncertainties in a self-consistent way. We show how the IS/UQ method could be used to optimize uncertainties of IBEs and differential cross section data simultaneously.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Finalizing the 63 Cu and 65 Cu Resonance Evaluations for the ENDF/B-VIII Release

The resolved resonance region evaluation for the only two natural isotopes of copper ( 63 Cu and 65 Cu) was carried out at the Oak Ridge National Laboratory (ORNL) in support of the US Department of Energy (DOE) Nuclear Criticality Safety Program (NCSP). The particular interest in the isotope of copper arose because it was linked with poor performance of the Zeus series of integral benchmarks from the International Criticality Safety Benchmark Evaluation Project (ICSBEP). Good agreement between the calculated and experimentally measured values for the ICSBEP benchmarks is essential to the NCSP because the ICSBEP benchmarks are used for validation purposes of criticality safety calculations.

07 ISOTOPE AND RADIATION SOURCES↗

Modernization efforts for the R -Matrix code SAMMY [Abstract]

The R-Matrix code SAMMY is a widely used nuclear data evaluation code focused on the resolved range, which includes corrections for experimental effects. The code is still mostly written in Fortran 77, and uses a memory management system suitable for the time of its initial writing (1984). A modernization effort is under way to bring the code in-line with modern software development practices. A continuous-integration testing framework was added, automating the large existing set of test cases. It is run on every commit. The memory management was updated to current standard practices suitable for modern software analysis tools. The code can be obtained from https://code.ornl.gov/RNSD/SAMMY. The resonance parameters and covariance information are now stored in C++ objects shared by SAMMY and AMPX, the processing code that generates nuclear data libraries for SCALE. This allows for easier maintenance and access to the resonance parameters inside and outside of SAMMY. This feature is already used by accessing and changing parameters in memory in the Bayesian Monte Carlo Evaluation Framework for Cross Sections Nuclear Data and Integral Benchmark Experiments project, Further plans include the switch to the ENDF reading and writing routines in AMPX, as these routines are more robust, easier to maintain, and support more features. Of note here is support for the new GNDS format. Previously it wasn’t easy to share the full covariance matrix for evaluations containing more than one isotope due to limitations on the ENDF format; this is now supported in GNDS. The data are currently available in a binary SAMMY format and can be exported to GNDS to make them more widely available and sharable. The next step will be to use the same resonance processing code at 0K in AMPX and SAMMY as one of the available Reich-Moore R-Matrix formalism. The first step toward this goal is to isolate the reconstruction into a module that takes resonance parameters as its input and does not depend on SAMMY global parameters. This goal has been achieved and it should now be possible to more easily change the resonance formalism and add enhancements as the Phenomenological R-Matrix parameterization of direct, doorway, and compound nuclear reactions discussed elsewhere on this conference. This concerted modernization and enhancement effort provides multiple advantages to the nuclear data community. It will allow parameter optimization using enhanced formalisms, including experimental effects, that better match complex experimental data. Then those evaluated parameters can immediately be passed off to AMPX to be reconstructed with the exact same cross section model and be put into a data library for subsequent testing using SCALE and the Valid Benchmark suite or other suitable benchmark suites.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Neutron Noise Analysis of the Neptunium Subcritical Observation (NESO) Experiment

The Neptunium Subcritical Observation (NeSO) experiment was a subcritical integral benchmark experiment. This experiment was designed in 2017-2018 and was performed at the National Criticality Experiments Research Center (NCERC) in 2019. Eight different subcritical configurations were measured with varying Nickel reflector thickness. For all configurations, a 3 He detection system was used to record neutron events. The focus of this work is to share neutron noise results of the measured data.

3-Helium↗

Advancing the Theory of Nuclear Data Evaluations [Abstract]

We present recent advances in the R-matrix formalism as well as the Bayesian evaluation framework for improved nuclear data evaluations. The advances in the R matrix formalism include: 1) direct processes, 2) doorway, as well as multistep, processes, and 3) various forms of the Reich-Moore approximation for eliminated capture channels. Furthermore, to address unreasonably small posterior uncertainties often encountered in nuclear data evaluations of large data sets using the conventional form of the Bayes’ theorem, we introduce imperfections (of the data or the model) as a formal evaluation tool for taming the evaluated uncertainties in harmony with Bayes’ theorem. These theoretical advances were motivated by the nuclear data evaluations of differential resolved resonance cross section data using the code SAMMY, as well as the integral benchmark experiments using the SCALE code system, being performed at Oak Ridge National Laboratory for the Nuclear Criticality Safety Program. Some pedagogical applications of the new formalism, as well as a snapshot of the SAMMY modernization efforts, will be presented.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Chlorine Worth Study Nuclear Data

The Chlorine Worth Study (CWS) was a series of experiments that took place at the National Criticality Experiments Research Center (NCERC), operated by Los Alamos National Laboratory (LANL). The focus of the experiments was to develop new integral benchmarks for the International Criticality Safety Benchmark Evaluation Project (ICSBEP) Handbook with high sensitivity to chlorine in the thermal neutron energy region and which match sensitivities of aqueous chloride operations at LANL. This work discusses the experiment and how the experimental and simulated results using different nuclear data libraries compare to each other.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

IER-517: Molybdenum Optimized Benchmark System Demonstrating Integral Correlations (MOBY DICK)

Nuclear criticality experiments are essential to the validation of nuclear data used in simulation software. The quality of nuclear data becomes paramount as simulation software becomes more relied upon for criticality safety studies and designs of nuclear systems. To improve the quality of nuclear data, experimenters can design critical experiments that are sensitive to isotope reaction pairs in materials of interest. The efforts conducted by the Organisation for Economic Co-operation and Development - Nuclear Energy Agency (OECD-NEA) Working Party on Nuclear Criticality Safety (WPNCS) Subgroup 8: Preservation of Expert Knowledge and Judgement Applied to Criticality Benchmarks (SG8) to categorize benchmarks according to their usefulness for nuclear data validation have been of great importance. Based on the OECD studies benchmark experiments included in the International Criticality Safety Benchmark Evaluation Project (ICSBEP) Handbook are concisely used by nuclear data evaluators, criticality safety engineers and others to validate nuclear data and simulation results. A lack of benchmarks sensitive to molybdenum in the (ICSBEP), particularly in the intermediate range, was noted by Los Alamos National Laboratory (LANL), the French Institut de Radioprotection et de Sûreté Nucléaire (IRSN), and Y-12 National Security Site prompting them to submit a joint integral experiment request to the Nuclear Criticality Safety Program (NCSP) in 2019. The request included both HEU and Plutonium systems in order to validate differential nuclear data focusing on the intermediate energy range but also includes thermal and fast configurations. This document represents the preliminary design work for a series of molybdenum integral experiments known as Molybdenum Optimized Benchmark System Demonstrating Integral Correlations (MOBY DICK).

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

‘Wasteaware’ benchmark indicators for integrated sustainable waste management in cities

Highlights: • Solid waste management (SWM) is a key utility service, but data is often lacking. • Measuring their SWM performance helps a city establish priorities for action. • The Wasteaware benchmark indicators: measure both technical and governance aspects. • Have been developed over 5 years and tested in more than 50 cities on 6 continents. • Enable consistent comparison between cities and countries and monitoring progress. - Abstract: This paper addresses a major problem in international solid waste management, which is twofold: a lack of data, and a lack of consistent data to allow comparison between cities. The paper presents an indicator set for integrated sustainable waste management (ISWM) in cities both North and South, to allow benchmarking of a city’s performance, comparing cities and monitoring developments over time. It builds on pioneering work for UN-Habitat’s solid waste management in the World’s cities. The comprehensive analytical framework of a city’s solid waste management system is divided into two overlapping ‘triangles’ – one comprising the three physical components, i.e. collection, recycling, and disposal, and the other comprising three governance aspects, i.e. inclusivity; financial sustainability; and sound institutions and proactive policies. The indicator set includes essential quantitative indicators as well as qualitative composite indicators. This updated and revised ‘Wasteaware’ set of ISWM benchmark indicators is the cumulative result of testing various prototypes in more than 50 cities around the world. This experience confirms the utility of indicators in allowing comprehensive performance measurement and comparison of both ‘hard’ physical components and ‘soft’ governance aspects; and in prioritising ‘next steps’ in developing a city’s solid waste management system, by identifying both local strengths that can be built on and weak points to be addressed. The Wasteaware ISWM indicators are applicable to a broad range of cities with very different levels of income and solid waste management practices. Their wide application as a standard methodology will help to fill the historical data gap.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

ORNL Testing of Multiple Graphite Benchmarks [Slides]

Integral criticality safety and reactor physics benchmark experiments from the International Handbook of Evaluated Criticality Safety Benchmark Experiments (ICSBEP Handbook) and the International Handbook of Reactor Physics Experiments (IRPhE Handbook) are essential for nuclear data validation and testing

ENDF↗