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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 91 records · Page 5
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

A compact neutron spectrometer system

A portable neutron spectrometer, nSpec, has been developed for passive interrogation of fast neutrons ( 1 MeV) from neutron sources. The design of the system includes four EJ-301 liquid scintillation cells, a custom stand, and tungsten caps for gamma-ray shielding. Data acquisition settings were optimized to provide a dynamic range of up to > 15 MeV neutron energy. Additionally, the detector response matrix was characterized using a time-of-flight method based on gamma-ray tagged neutron emission from 252 Cf. The spectrum unfolding was characterized using measured and simulated spectra of AmBe and 252 Cf with the GRAVEL and MLEM methods. Monte Carlo methods were used to examine the uncertainty propagation and determine sufficient counts for a measurement.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2023

Fission with Exotic Nuclei (Abbreviated Report)

Nuclear fission is a key mechanism involved in the synthesis of heavy elements in the Cosmos and is the primary explanation for the stability of superheavy elements. Nevertheless, our knowledge of fission remains extremely fragmented. Most experiments have been conducted only on a tiny number of stable actinide nuclei and are often incomplete, leading to gaps in our basic understanding of the process. For many radioactive isotopes, basic fission data such as the charge or mass distribution of the fragments is unknown. These gaps cannot always be filled by simulation alone. Common fission models contain too many free parameters and lack predictive power. In contrast, the fundamental theory of fission under development at LLNL is much more predictive, but its current computational cost is too high to be used extensively for data evaluations. A unique window of opportunity to resolve these limitations has recently opened: the U.S. nuclear science community is ramping up major experimental programs at the Facility for Rare Isotope Beams (FRIB, the DOE flagship facility in low-energy nuclear science), and techniques from machine learning have shown great potential to simplify the use of a fundamental, quantum-mechanical theory of fission. This project has two components. On the experimental side, we acquired and deployed at the HIGS facility a new dual Frisch-Grid ionization chamber to measure correlated fragment-mass, kinetic energy, and angular distributions of fission fragments from induced fission. This new device was used to perform measurements of charge, mass and total kinetic energy of fission fragments in the photofission of 238 U and eight gamma-ray beam energies between 6.2 and 13 MeV, which allowed extracting high-precision independent yields for this reaction. The device was also used to perform measurements of the same quantities in the neutron-induced fission of 234 U with monoenergetic beams of energy between 5 and 8 MeV. In parallel, we collaborated with a team at Commissariat à l’énergie atomique et aux énergies alternatives (CEA) to perform a series of measurements of fission yields in inverse kinematics for the two isotopes of 236 U and 240 Pu. The experiment took place at the Grand Accélérateur National d’Ions Lourds in France in June 2023. The deployment of the VAMOS spectrometer with a new array called PISTA allowed determining the excitation energy of the fissioning system within 1 Mega-electronvolts. The second component of the project involved using deep neural networks to build fast and reliable emulators of our current fission models. In an invited paper published in Frontier in Physics, we showed that autoencoders could successfully compress nuclear wavefunctions in nuclear density functional theory. We achieved a dimensionality reduction of the order of two orders of magnitude while keeping the error in the total energy to less than 0.01%. In a second paper submitted to Physical Review Letters in June 2023 with our collaborators at CEA, we showed that variational autoencoders can learn the collective degrees of freedom driving the fission process.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Fermi-LAT Gamma-Ray Emission Discovered from the Composite Supernova Remnant B0453-685 in the Large Magellanic Cloud

Abstract We report the second extragalactic pulsar wind nebula (PWN) to be detected in the megaelectronvolt–gigaelectronvolt band by the Fermi-LAT, located within the Large Magellanic Cloud. The only other known PWN to emit in the Fermi band outside of the Milky Way is N157B, which lies to the west of the newly detected gamma-ray emission at an angular distance of 4°. Faint, pointlike gamma-ray emission is discovered at the location of the composite supernova remnant (SNR) B0453-685 with a ∼4 σ significance with energies ranging from 300 MeV–2 TeV. We present the Fermi-LAT data analysis of the new gamma-ray source, coupled with a detailed multiwavelength investigation to understand the nature of the observed emission. Combining the observed characteristics of the SNR and the physical implications from broadband modeling, we argue it is unlikely that the SNR is responsible for the gamma-ray emission. While the gamma-ray emission is too faint for a pulsation search, we try to distinguish between any pulsar and PWN component of SNR B0453-685 that could be responsible for the observed gamma-ray emission using semi-analytic models. We determine the most likely scenario is that the old PWN ( τ ∼ 14,000 yr) within B0453-685 has been impacted by the return of the SNR reverse shock with a possible substantial pulsar component below 5 GeV.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2022

Fast neutron activation of ubiquitous materials

Nuclear explosions expose ubiquitous materials to large numbers of neutrons, producing a variety of radioactive isotopes. To simulate such phenomena from both fission and thermonuclear explosions, we irradiated 29 different targets with approximately 3 and 14 MeV neutrons and measured the beta-delayed gamma rays using germanium detectors. Therefore, for each neutron energy, the expected radioisotopes, half-lives, and gamma ray energies were deduced. From measurements of the ratios of activities of the radionuclides produced by neutron irradiations, we were able to identify several materials that are particularly sensitive to the neutron energy spectra.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

Gamma Radiation Monitoring Data

This dataset contains gamma-ray total counts in counts/minute (cpm), every 15-minutes, from the Gamma Radiation Monitoring campaign at the ENA site (Graciosa, Azores).

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2026

Evaluation of a deuterated detector for gamma-ray beam intensity measurements

Laser-Compton scattering sources of quasi-monochromatic γ-ray beams have been in operation for over 30 years, with new facilities being under construction or proposed. To sustain a high-quality experimental physics program, continuous monitoring of these beams is essential by measuring the spectral, temporal, and spatial characteristics. In this work, we introduce a new method for determining the γ-ray beam intensity by using photodisintegration of deuterons in an active target detector approach. Measurements were performed using deuterated liquid scintillator detectors at several incident gamma energies between 4 and 13 MeV at the High Intensity γ-ray Source, Durham, USA. The results demonstrate that an instrument based on a deuterated active detector can be used to monitor the intensity of the γ-ray beam with high efficiency and operational simplicity.

Compton scattering↗
DOE OSTI2021

Multi-pulse time resolved gamma ray spectroscopy of the advanced radiographic capability using gas Cherenkov diagnostics

The advanced radiographic capability located at the National Ignition Facility (NIF) uses high intensity, short pulse lasers to create bright photon sources for diagnosing high energy density experiments. There are radiographic needs for a multi-frame time-resolved MeV gamma diagnostic for experiments on the NIF with sub-nanosecond resolution. A series of experiments demonstrated measurements of MeV x-ray spectra resolved with a time separation of a few nanoseconds through the use of gas Cherenkov detectors. In this work, a two-pulse radiographic experiment found a 30% reduction in > 2.8 MeV photon flux compared to the first frame exposure.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2023

Testing shell-model interactions at high excitation energy and low spin: Nuclear resonance fluorescence in Ge 74

With their complex low-spin structure, the germanium isotopes have accrued a large number of experimental data which challenge nuclear models. The structure of the 74 Ge isotope is investigated here with nuclear resonance fluorescence as part of an extensive campaign of experimental tests of the shell model in the germanium isotopic chain using a number of complementary techniques. Levels were excited with 3.10 – 5.44 MeV photon beams provided by the High Intensity Gamma-Ray Source at TUNL. Many new levels were identified and their spins, parities, branching ratios, and associated scattering cross section values were determined. Large-scale shell-model calculations, which include jj44b and JUN45 effective interactions developed to describe nuclei in this mass region, predict the new data satisfactorily. Herein this study extends the validation of these two interactions, which are candidates for computation of matrix elements to be used in the interpretation of neutrinoless double-β decay experiments in 76 Ge, into the low-spin, high excitation energy domain.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

Exploring the MeV sky with a combined coded mask and Compton telescope: the Galactic Explorer with a Coded aperture mask Compton telescope (GECCO)

The sky at MeV energies is currently poorly explored. Here we present an innovative mission concept that builds upon the heritage of past and current missions improving the sensitivity and, very importantly, the angular resolution. This consists in combining a Compton telescope and a coded-mask telescope. We delineate the motivation for such a concept and we define the scientific goals for such a mission. The Galactic Explorer with a Coded Aperture Mask Compton Telescope (GECCO) is a novel concept for a next-generation telescope covering hard X-ray and soft gamma-ray energies. The potential and importance of this approach that bridges the observational gap in the MeV energy range are presented. With the unprecedented angular resolution of the coded mask telescope combined with the sensitive Compton telescope, a mission such as GECCO can disentangle the discrete sources from the truly diffuse emission. Individual Galactic and extragalactic sources are detected. This also allows to understand the gamma-ray Galactic center excess and the Fermi Bubbles, and to trace the low-energy cosmic rays, and their propagation in the Galaxy. Nuclear and annihilation lines are spatially and spectrally resolved from the continuum emission and from sources, addressing the role of low-energy cosmic rays in star formation and galaxy evolution, the origin of the 511 keV positron line, fundamental physics, and the chemical enrichment in the Galaxy. Such an instrument also detects explosive transient gamma-ray sources, which, in turn, enables identifying and studying the astrophysical objects that produce gravitational waves and neutrinos in a multi-messenger context. By looking at a poorly explored energy band it also allows discoveries of new astrophysical phenomena.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2022

Upgrades to the gamma ray imager on DIII-D enabling access to high flux hard x-ray measurements during the runaway electron plateau phase (invited)

The Gamma Ray Imager (GRI) is a pinhole camera providing 2D imaging of MeV hard x-ray (HXR) bremsstrahlung emission from runaway electrons (REs) over the poloidal cross section of the DIII-D tokamak. We report a series of upgrades to the GRI expanding the access to RE scenarios from the diagnosis of a trace amount of REs to high flux HXR measurements during the RE plateau phase. We present the implementation of novel gamma ray detectors based on LYSO and YAP crystals coupled to multi-pixel photon counters, enabling a count rate in excess of 1 MHz. Finally, we highlight new insights into the RE physics discovered during the current quench and RE plateau phase experiments as the result of these upgrades.

Lvovskiy, A. (ORCID:0000000236491169)↗
DOE OSTI2023

Radiation-induced alteration of sandstone concrete aggregate

This study investigates the alteration of felsic sandstone-type rock, which is used as a coarse aggregate in concrete, subject to the effects of gamma-ray and neutron irradiation. The effects of three gamma-ray doses (27, 55, and 108 MGy) and four neutron fluence levels (1.22, 2.19, 6.99, and 14.30 × 10 19 n/cm 2 , $E$ ≥ 0.01 MeV) were investigated. Quartz and albite were found to be the major rock-forming minerals, with microcline intermediates, chlorite, and muscovite as the minors. Gamma rays caused no significant changes to the physical properties of the sandstone aggregates, even at high doses (108 MGy). In contrast, neutron irradiation caused alterations that became more pronounced at higher neutron fluences. The solid was confirmed to expand through metamictization of the rock-forming minerals. Quartz and muscovite were the most affected phases, whereas albite and microcline intermediates were only slightly affected, and chlorite was almost unaffected. The decrease in density was measured by He and water pycnometry, and this value was almost reproduced by calculations using the rock-forming mineral composition of the pristine sample measured using X-ray powder diffraction/Rietveld analysis and the cell volume change of the major forming minerals. In addition, light optical microscopy and scanning electron microscopy images confirmed the presence of intergranular and intragranular cracks. Intergranular cracks appeared to have initiated from the quartz grains, which expanded significantly. The intragranular cracks were frequently observed in the albite and microcline intermediates. These cracks can be described as radial cracks starting from the expanding quartz, caused by enforced displacement for deformation consistency with quartz expansion. The crack area ratio quantified by SEM image analysis corresponds to the discrepancy of the volume expansion difference calculated by He or water pycnometry and dimensional change measurements. In conclusion, an evaluation of solid expansion and crack openings in aggregates is important to estimate concrete degradation.

36 MATERIALS SCIENCE↗
DOE OSTI2024

Optimization of the gamma reaction history diagnostic for double-shell pusher areal density and reaction history measurements on the National Ignition Facility

The double-shell inertial confinement fusion campaign, which consists of an aluminum ablator, a foam cushion, a high-Z pusher (tungsten or molybdenum), and liquid deuterium–tritium (DT) fuel, aims for its first DT filled implosions on the National Ignition Facility (NIF) in 2024. The high-Z, high density pusher does not allow x-rays to escape the double-shell capsule. Therefore, nuclear diagnostics such as the Gamma Reaction History (GRH) diagnostic on the NIF are crucial for understanding high-Z implosion performance. To optimize the GRH measurement of fusion reaction history and the pusher’s areal density, the MCNP6.3-based forward model of the detector was built. When calculating the neutron-induced inelastic gamma ray production, the interaction of neutrons with the compressed fuel was additionally included. By folding the calculated gamma ray spectrum output and the previously calibrated GRH detector responses, the optimum set of GRH energy thresholds for measuring the pusher areal density is determined to be 2.9 and 6.3 MeV for DT double-shell experiments. In addition, the effect of the down-scattering of neutrons on the gamma ray spectrum, the minimum required yield for measurements, and the attenuation of the gamma rays through the pusher are analyzed.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2025

First Event-by-Event Identification of Cherenkov Radiation from Sub-Mev Particles in Liquid Argon

This Letter reports the event-by-event observation of Cherenkov light from sub-MeV electrons in a high scintillation light-yield liquid argon detector by the coherent CAPTAIN-Mills (CCM) experiment. The CCM200 detector, located at Los Alamos National Laboratory, instruments seven tons (fiducial volume) of liquid argon with 200 eight-inch photomultiplier tubes, 80% of which are coated in a wavelength-shifting material and the remaining 20% are uncoated. In the prompt time region of an event, defined as - 6 ≤ t < 0 ns relative to the event start time t = 0 , the uncoated photomultiplier tubes are primarily sensitive to visible Cherenkov photons. Using gamma rays from a Na 22 source for production of sub-MeV electrons, we isolated prompt Cherenkov light with > 5 σ confidence and developed a selection to obtain a low-background electromagnetic sample. This is the first event-by-event observation of Cherenkov photons from sub-MeV electrons in a high-yield scintillator detector and represents a milestone in low-energy particle detector development.

Aguilar-Arevalo, A. A. [UNAM, Mexico]↗
DOE OSTI2020

Fermi Large Area Telescope Fourth Source Catalog

We present the fourth Fermi Large Area Telescope catalog (4FGL) of γ-ray sources. Based on the first eight years of science data from the Fermi Gamma-ray Space Telescope mission in the energy range from 50 MeV to 1 TeV, it is the deepest yet in this energy range. Relative to the 3FGL catalog, the 4FGL catalog has twice as much exposure as well as a number of analysis improvements, including an updated model for the Galactic diffuse γ-ray emission, and two sets of light curves (one-year and two-month intervals). The 4FGL catalog includes 5064 sources above 4σ significance, for which we provide localization and spectral properties. Seventy-five sources are modeled explicitly as spatially extended, and overall, 358 sources are considered as identified based on angular extent, periodicity, or correlated variability observed at other wavelengths. For 1336 sources, we have not found plausible counterparts at other wavelengths. More than 3130 of the identified or associated sources are active galaxies of the blazar class, and 239 are pulsars.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2024

Detection of uranium-photofission neutrons with a 4 He scintillation detector

The use of photon active interrogation to detect special nuclear material has held significant theoretical promise, as the interrogating source particles, photons, are fundamentally different from one of the main signatures of special nuclear material: neutrons produced in nuclear fission. However, neutrons produced by photonuclear reactions in the accelerator target, collimator, and environment can obscure the fission neutron signal. These (γ, n) neutrons could be discriminated from fission neutrons by their energy spectrum, but common detectors sensitive to the neutron spectrum, like organic scintillators, are typically hampered by the intense photon background characteristic of photon-based active interrogation. In contrast, high-pressure 4 ⁢He-based scintillation detectors are well-suited to photon active interrogation, as they are similarly sensitive to fast neutrons and can measure their spectrum, but show little response to gamma rays. Here, in this work, a photon active interrogation system utilizing a 4 ⁢He scintillation detector and a 9 MeV linac-bremsstrahlung x-ray source was experimentally evaluated. The detector was shown to be capable of operating in intense gamma-ray environments and detecting photofission neutrons from 238 ⁢U when interrogated by this x-ray source. The photofission neutrons show clear spectral separation from (γ, n) neutrons produced in lead, a common shielding material.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2023

Coexistence of single-particle and collective excitation in Ni 61

Here, the high-spin states in 61 Ni have been studied using the fusion evaporation reaction, 50 Ti( 14 C, 3n) 61 Ni at an incident beam energy of 40 MeV. A Compton suppressed multi-HPGe detector setup, consisting of six clover detectors and three single-crystal HPGe detectors, was used to detect the de-exciting $\gamma$ rays from the excited states. The level scheme has been extended up to an excitation energy of 12.8 MeV and a tentative J π =35/2 + . The low-lying negative parity levels are found to be generated by single-particle excitation within the fp shell and also excitations to the g 9/2 orbitals as explained well with shell model calculations using the GXPF1Br+V MU (modified) interaction. Two rotational structures of regular E2 sequences with small to moderate axial deformation have been established at higher excitation energy. Most interestingly, two sequences of M1 transitions are reported for the first time and described as magnetic rotational bands. The shears mechanism for both the bands can be described satisfactorily by the geometrical model. The shell model calculation involving the cross shell excitation beyond the fp shell well reproduce the M1 and E2 sequences. The shell model predicted B(M1) values for the magnetic rotational band B1 show the decreasing trend with spin as expected with closing of the shears.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2026

Measuring the neutrino-oxygen neutral current quasielastic cross section using the accelerator neutrino neutron interaction experiment

The Accelerator Neutrino Neutron Interaction Experiment (ANNIE) is a 26-ton gadolinium-doped water Cherenkov detector located on-axis to Fermilab’s Booster Neutrino Beam (BNB). ANNIE is uniquely positioned to perform high-statistics measurements of neutrino-nucleus interactions in water, benefiting from a large neutrino flux due to a short (100-meter) baseline. A central focus of ANNIE’s physics program is the measurement of both charged current (CC) and neutral current (NC) cross sections on water, including neutral current quasielastic (NCQE) and CC-inclusive channels. The NCQE measurement is particularly critical for constraining uncertainties in rare-event searches such as the Diffuse Supernova Neutrino Background (DSNB), where atmospheric $\nu$NCQE interactions constitute a significant and poorly constrained background. This dissertation presents a measurement of the flux-averaged neutrino-oxygen neutral current quasielastic ($\nu$NCQE) cross section using $2.573 \times 10^{20}$~POT of BNB exposure from the 2022 and 2023 beam years. The $\nu$NCQE interaction is identified through the primary $\gamma$-rays produced by nuclear de-excitation of the residual $^{15}$N$^*$ or $^{15}$O$^*$ nucleus following nucleon knockout from $^{16}$O. A dedicated Monte Carlo (MC) re-tuning campaign was conducted using an americium-beryllium (AmBe) calibration source, Michel electrons from stopped muons, and throughgoing dirt muons originating upstream of the detector. This multi-sample approach provided a wide-ranging $\mathcal{O}(\text{MeV})$--$\mathcal{O}(\text{GeV})$ dataset for tuning the simulated detector response, which was subsequently validated against AmBe neutron and Michel electron data for use in the $\nu$NCQE analysis. A dedicated laser calibration campaign was carried out to reduce timing uncertainties across the PMT system, enabling reconstruction of the BNB bunch substructure with sufficient resolution to serve as a background rejection tool. By selecting events in-time with individual neutrino bunches, beam-correlated $\nu$NCQE events are separated from diffuse and accelerator-induced backgrounds, notably skyshine neutrons and externally-originating events, that would otherwise dominate traditional charge-based selections within a small-scale, surface-level, short-baseline detector. A data-driven estimation of the skyshine neutron and external background rates was performed and incorporated into the systematic uncertainty budget. The flux-averaged $\nu$NCQE cross section on oxygen is measured to be $1.57 \pm 0.06\,(\text{stat.})$ $^{+0.91}_{-0.67}\,(\text{syst.})$ $\times 10^{-38}\ \text{cm}^{2}$. A full systematic budget is constructed by propagating uncertainties in the secondary hadronic interaction modeling, background cross section normalizations, detector response, neutrino flux, and the primary $\gamma$-ray emission probabilities from oxygen nuclear de-excitation. An idealized de-excitation model, constructed from existing measurements in the literature is developed to benchmark the predictions of the \textsc{GENIE} event generator. A comparison reveals that \textsc{GENIE} systematically overpredicts the primary $\gamma$-ray emission probability from oxygen de-excitation by a factor of $1.49\times$ for $E_\gamma > 6$~MeV and $3.07\times$ in the $3$--$6$~MeV band. This comparison motivates the dominant systematic uncertainty in this analysis, where a conservative uncertainty of $^{+39.9\%}_{-0\%}$ on the primary $\gamma$-ray signal prediction is assigned. The ANNIE result is consistent with and complementary to existing flux-averaged $\nu$NCQE cross section measurements from T2K and Super-Kamiokande, providing an independent measurement with a different detector, neutrino beam, and analysis methodology. Looking ahead, an upgrade to the ANNIE DAQ infrastructure enabling continuous extended readout will allow a complementary $\nu$NCQE neutron multiplicity measurement, directly relevant to constraining the NCQE background in DSNB searches, competitive with the recent T2K measurement at SK-Gd. The planned Super-SANDI upgrade, deploying a large Water-based Liquid Scintillator (WbLS) volume, will further extend ANNIE's reach to hadronic final states and exclusive NC channels, and enable joint measurements with liquid argon detectors sharing the BNB beamline ahead of DUNE and Hyper-Kamiokande.

Doran, Steven [Iowa State U.]↗
DOE OSTI2023

The Third Fermi Large Area Telescope Catalog of Gamma-Ray Pulsars

We present 294 pulsars found in GeV data from the Large Area Telescope (LAT) on the Fermi Gamma-ray Space Telescope. Another 33 millisecond pulsars (MSPs) discovered in deep radio searches of LAT sources will likely reveal pulsations once phase-connected rotation ephemerides are achieved. A further dozen optical and/or X-ray binary systems colocated with LAT sources also likely harbor gamma-ray MSPs. This catalog thus reports roughly 340 gamma-ray pulsars and candidates, 10% of all known pulsars, compared to ≤11 known before Fermi. Half of the gamma-ray pulsars are young. Of these, the half that are undetected in radio have a broader Galactic latitude distribution than the young radio-loud pulsars. The others are MSPs, with six undetected in radio. Overall, ≥236 are bright enough above 50 MeV to fit the pulse profile, the energy spectrum, or both. For the common two-peaked profiles, the gamma-ray peak closest to the magnetic pole crossing generally has a softer spectrum. The spectral energy distributions tend to narrow as the spindown power $\dot{E}$ decreases to its observed minimum near 10 33 erg s -1 , approaching the shape for synchrotron radiation from monoenergetic electrons. We calculate gamma-ray luminosities when distances are available. Our all-sky gamma-ray sensitivity map is useful for population syntheses. The electronic catalog version provides gamma-ray pulsar ephemerides, properties, and fit results to guide and be compared with modeling results.

79 ASTRONOMY AND ASTROPHYSICS↗