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A Global Climatology of Tropospheric and Stratospheric Ozone Derived from Aura OMI and MLS Measurements

A global climatology of tropospheric and stratospheric column ozone is derived by combining six years of Aura Ozone Monitoring Instrument (OMI) and Microwave Limb Sounder (MLS) ozone measurements for the period October 2004 through December 2010. The OMI/MLS tropospheric ozone climatology exhibits large temporal and spatial variability which includes ozone accumulation zones in the tropical south Atlantic year-round and in the subtropical Mediterranean! Asia region in summer months. High levels of tropospheric ozone in the northern hemisphere also persist in mid-latitudes over the eastern North American and Asian continents extending eastward over the Pacific Ocean. For stratospheric ozone climatology from MLS, largest ozone abundance lies in the northern hemisphere in the latitude range 70degN-80degN in February-April and in the southern hemisphere around 40degS-50degS during months August-October. The largest stratospheric ozone abundances in the northern hemisphere lie over North America and eastern Asia extending eastward across the Pacific Ocean and in the southern hemisphere south of Australia extending eastward across the dateline. With the advent of many newly developing 3D chemistry and transport models it is advantageous to have such a dataset for evaluating the performance of the models in relation to dynamical and photochemical processes controlling the ozone distributions in the troposphere and stratosphere.

Ziemke, J.R.↗

File Specification for MERRA-2 Stratospheric Composition Reanalysis of Aura MLS (M2-SCREAM)

This document provides a brief description of the output collections from the MERRA-2 Stratospheric Composition Reanalysis of the Aura Microwave Limb Sounder (M2-SCREAM) produced at NASA’s Global Modeling and Assimilation Office. These data are generated by assimilating retrievals from the Microwave Limb Sounder (MLS) and the Ozone Monitoring Instrument (OMI) into the Global Earth Observing System (GEOS) Constituent Data Assimilation System (CoDAS) driven by meteorological fields from MERRA-2. M2-SCREAM assimilates hydrochloric acid (HCl), nitric acid (HNO3), stratospheric water vapor (H2O), nitrous oxide (N2O) and ozone with a system equipped with a version of the GEOS general circulation model and a stratospheric chemistry model, StratChem. Assimilated fields are provided globally at 0.5° by 0.625° resolution at three-hourly frequencies from 2004/09/01 to 2021. Assimilation uncertainties for each of the assimilated constituents are calculated from the CoDAS statistical output (Wargan et al., 2022) and provided as global full-resolution three-dimensional monthly files.

Krzysztof Wargan↗

A Golden Era of PSC Observations From the A-Train By CALIOP and MLS

The fundamental role of polar stratospheric clouds (PSCs) in the depletion of stratospheric ozone is well established. Heterogeneous reactions on PSCs convert the stable chlorine reservoirs HCl and ClONO2 to chlorine radicals that destroy ozone catalytically. PSCs also prolong ozone depletion by delaying chlorine deactivation through the removal of gas-phase HNO3 and H2O by sedimentation of large PSC particles. There has been substantial recent progress in our understanding of PSC processes due to the long-term, vortex-wide observations from the CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) lidar on the CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations) satellite and the MLS (Microwave Limb Sounder) on the Aura satellite. The CALIOP observations provide unprecedented high spatial resolution information on particulate aerosol/PSC morphology and composition, while MLS provides complementary collocated measurements of gas-phase HNO3 and H2O, the major constituents of all PSC particles. The combined analyses of these datasets have enabled better PSC composition discrimination and provided valuable new insight into PSC formation processes and particle growth kinetics. The more than 17 years of CALIOP and MLS data have uniquely captured the primary aspects of the seasonal and multi-year variability of PSCs in the Arctic and Antarctic, enabling the development of a state-of-the-art reference PSC data record and climatology. In this presentation, we highlight the significant advances in our understanding achieved during this golden era of spaceborne PSC observations and identify remaining gaps in our knowledge that future spaceborne lidar missions may help resolve.

polar stratospheric clouds↗

Mesospheric Temperature Inversion Layers: Recent Observations from UARS ISAMS and MLS

This paper presents an observational study of the mesospheric temperature inversion layer with Upper Atmosphere Research Satellite (UARS) Improved Stratospheric and Mesospheric Sounder (ISAMS) and Microwave Limb Sounder (MLS). The satellite data show that the temperature inversion layer can be generated from deep penetration of planetary waves in the mesosphere.

mesospheric temperature inversion layers UARS ISAM↗

Monitoring and Assimilation of MLS Measurements in the DAO Ozone Data Assimilation System

Since 1999 the DAO (Data Assimilation Office) at NASA Goddard has operationally assimilated ozone measurements in near real time. Currently, the assimilation system analyzes SBUV profile and total column measurements using an off line CTM with parameterized chemistry within the 3D-PSAS algorithm. During the last year the assimilation system was modified to either monitor or actively assimilate MLS (Microwave Limb Sounder) measurements in conjunction with the active assimilation of TOMS total column and SBUV profiles. It is expected that the active assimilation of MLS profiles will improve analysis results in two ways. First, there should be an improvement in the vertical resolution. Second, there should be an improvement in regions where SBUV measurements do not exist (such as in the polar night). A series of experiments using UARS (Upper Atmospheric Research Satellite) MLS data from December 1991 to March 1992 were run. In these experiments MLS data was either monitored in conjunction with active assimilation of the SBUV profile and TOMS total column measurements, or some combination of MLS, TOMS, and SBUV observations was actively assimilated. Monitoring of MLS data indicated that the MLS observations contain verifiable information that should improve the vertical structure of the analysis results, especially below the ozone peak and above the tropopause. The monitoring also substantiated the potential to improve the assimilation in the polar night. Active assimilation of MLS data does indeed improve the analysis results in these two ways, although the quality of the improvements is not uniform. This suggests that refinement of the specification of the error covariances might be needed to optimize the system. In addition it may be necessary to account for biases between the different sources of ozone information.

Atlas, Robert↗

MLS and CALIOP Cloud Ice Measurements in the Upper Troposphere: A Constraint from Microwave on Cloud Microphysics

This study examines the consistency and microphysics assumptions among satellite ice water content (IWC) retrievals in the upper troposphere with collocated A-Train radiances from Microwave Limb Sounder (MLS) and lidar backscatters from Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP). For the cases in which IWC values are small (less than 10mg m(exp-23)), the cloud ice retrievals are constrained by both MLS 240- and 640- GHz radiances and CALIOP 532-nm backscatter beta(532). From the observed relationships between MLS cloud-induced radiance T(sub cir) and the CALIOP backscatter integrated gamma532 along the MLS line of sight, an empirical linear relation between cloud ice and the lidar backscatter is found: IWC/beta532=0.58+/-0.11. This lidar cloud ice relation is required to satisfy the cloud ice emission signals simultaneously observed at microwave frequencies, in which ice permittivity is relatively well known. This empirical relationship also produces IWC values that agree well with the CALIOP, version 3.0, retrieval at values, less than 10mg m(exp-3). Because the microphysics assumption is critical in satellite cloud ice retrievals, the agreement found in the IWC-beta532 relationships increase fidelity of the assumptions used by the lidar and microwave techniques for upper-tropospheric clouds.

ice water content↗

Calibration of the Microwave Limb Sounder on the Upper Atmosphere Research Satellite

This paper describes pre-launch radiometric and spectral calibrations of the Microwave Limb Sounder (MLS) on the Upper Atmosphere Research Satellite (UARS). Use of in-flight data for validation or refinement of calibration is described. The estimated uncertaint in calibrated radiance from pre-launch radiometric and spectral calibration data is better than 2% in most bands.

Microwave Limb Sounder↗

Processing EOS MLS Level-2 Data

A computer program performs level-2 processing of thermal-microwave-radiance data from observations of the limb of the Earth by the Earth Observing System (EOS) Microwave Limb Sounder (MLS). The purpose of the processing is to estimate the composition and temperature of the atmosphere versus altitude from .8 to .90 km. "Level-2" as used here is a specialists f term signifying both vertical profiles of geophysical parameters along the measurement track of the instrument and processing performed by this or other software to generate such profiles. Designed to be flexible, the program is controlled via a configuration file that defines all aspects of processing, including contents of state and measurement vectors, configurations of forward models, measurement and calibration data to be read, and the manner of inverting the models to obtain the desired estimates. The program can operate in a parallel form in which one instance of the program acts a master, coordinating the work of multiple slave instances on a cluster of computers, each slave operating on a portion of the data. Optionally, the configuration file can be made to instruct the software to produce files of simulated radiances based on state vectors formed from sets of geophysical data-product files taken as input.

Snyder, W. Van↗

Aura Atmospheric Data Products and Their Availability from NASA Goddard Earth Sciences DAAC

NASA's EOS-Aura spacecraft was launched successfully on July 15, 2004. The four instruments onboard the spacecraft are the Microwave Limb Sounder (MLS), the Ozone Monitoring Instrument (OMI), the Tropospheric Emission Spectrometer (TES), and the High Resolution Dynamics Limb Sounder (HBDLS). The Aura instruments are designed to gather earth sciences measurements across the ultraviolet, visible, infra-red, thermal and microwave regions of the electromagnetic spectrum. Aura will provide over 70 distinct standard atmospheric data products for use in ozone layer and surface UV-B monitoring, air quality forecast, and atmospheric chemistry and climate change studies (http://eosaura.gsfc.nasa.gov/). These products include earth-atmosphere radiances and solar spectral irradiances; total column, tropospheric, and profiles of ozone and other trace gases, surface W-B flux; clouds and aerosol characteristics; and temperature, geopotential height, and water vapor profiles. The MLS, OMI, and HIRDLS data products will be archived at the NASA Goddard Earth Sciences (GES) Distributed Active Archive Center (DAAC), while data from TES will be archived at NASA Langley Research Center DAAC. Some of the standard products which have gone through quick preliminary checks are already archived at the GES DAAC (http://daac.nsfc.nasa.gov/) and are available to the Aura science team and data validation team members for data validation; and to the application and visualization software developers, for testing their application modules. Once data are corrected for obvious calibration problems and partially validated using in-situ observations, they would be made available to the broader user community. This presentation will provide details of the whole suite of Aura atmospheric data products, and the time line of the availability of the rest of the preliminary products and of the partially validated provisional products. Software and took available for data access, visualization, and data mining will also be discussed.

Ahmad, S.↗

Five-Year (2004-2009)Observations of Upper Tropospheric Water Vapor and Cloud Ice from MLS and Comparisons with GEOS-5 Analyses

This paper gives an overview of August 2004 through July 2009 upper tropospheric (UT) water vapor (H2O) and ice water content (IWC) from the Aura Microwave Limb Sounder (MLS) and comparisons with outputs from the NASA Goddard Earth Observing System Version 5 (GEOS-5) data assimilation system. Both MLS and GEOS-5 show that high values of H2O and IWC at 215 to 147 hPa are associated with areas of deep convection. They exhibit good (within approximately 15%) agreement in IWC at these altitudes, but GEOS-5 H2O is approximately 50% (215 hPa) to approximately 30% (147 hPa) larger than MLS, possibility due to its higher temperatures at these altitudes. GOES-5 produces a weaker intertropical convergence zone than MLS, while a seasonally-migrating band of tropical deep convection is clearly evident in both the MLS and GEOS-5 UT H2O and IWC. MLS and GEOS-5 both show spatial anti-correlation between IWC and H2O at 100 hPa, where less H2O is associated with low temperatures in regions of tropical convection. At 100 hPa, GEOS-5 produces 50% less IWC and 15% less H2O in the tropics, and approximately 20% more H2O in the extra-tropics, than does MLS. Behavior of the 100 hPa H2O, which exhibits a quasi-biennial oscillation, appears consistent with it being controlled by temperature. The seasonal cycle in the vertical transport of tropical mean H2O from approximately 147 hPa to approximately 10 hPa appears much stronger in MLS than in GEOS-5. The UT IWC and H2O interannual variations, from both MLS and GEOS-5, show clear imprints of the El Nino-Southern Oscillation.

Jiang, Jonathan H.↗

Climatology 2011: An MLS and Sonde Derived Ozone Climatology for Satellite Retrieval Algorithms

The ozone climatology used as the a priori for the version 8 Solar Backscatter Ultraviolet (SBUV) retrieval algorithms has been updated. The Microwave Limb Sounder (MLS) instrument on Aura has excellent latitude coverage and measures ozone daily from the upper troposphere to the lower mesosphere. The new climatology consists of monthly average ozone profiles for ten degree latitude zones covering pressure altitudes from 0 to 65 km. The climatology was formed by combining data from Aura MLS (2004-2010) with data from balloon sondes (1988-2010). Ozone below 8 km (below 12 km at high latitudes) is based on balloons sondes, while ozone above 16 km (21 km at high latitudes) is based on MLS measurements. Sonde and MLS data are blended in the transition region. Ozone accuracy in the upper troposphere is greatly improved because of the near uniform coverage by Aura MLS, while the addition of a large number of balloon sonde measurements improves the accuracy in the lower troposphere, in the tropics and southern hemisphere in particular. The addition of MLS data also improves the accuracy of climatology in the upper stratosphere and lower mesosphere. The revised climatology has been used for the latest reprocessing of SBUV and TOMS satellite ozone data.

McPeters, Richard D.↗

Evaluation of UTLS Carbon Monoxide Simulations in GMI and GEOS-Chem Chemical Transport Models using Aura MLS Observations

This study evaluates the distribution and variation of carbon monoxide (CO) in the upper troposphere and lower stratosphere (UTLS) during 2004-2012 as simulated by two chemical transport models, using the latest version of Aura Microwave Limb Sounder (MLS) observations. The simulated spatial distributions, temporal variations and vertical transport of CO in the UTLS region are compared with those observed by MLS. We also investigate the impact of surface emissions and deep convection on CO concentrations in the UTLS over different regions, using both model simulations and MLS observations. Global Modeling Initiative (GMI) and GEOS-Chem simulations of UTLS CO both show similar spatial distributions to observations. The global mean CO values simulated by both models agree with MLS observations at 215 and 147 hPa, but are significantly underestimated by more than 40% at 100 hPa. In addition, the models underestimate the peak CO values by up to 70% at 100 hPa, 60% at 147 hPa and 40% at 215 hPa, with GEOS-Chem generally simulating more CO at 100 hPa and less CO at 215 hPa than GMI. The seasonal distributions of CO simulated by both models are in better agreement with MLS in the Southern Hemisphere (SH) than in the Northern Hemisphere (NH), with disagreements between model and observations over enhanced CO regions such as southern Africa. The simulated vertical transport of CO shows better agreement with MLS in the tropics and the SH subtropics than the NH subtropics. We also examine regional variations in the relationships among surface CO emission, convection and UTLS CO concentrations. The two models exhibit emission-convection- CO relationships similar to those observed by MLS over the tropics and some regions with enhanced UTLS CO.

spatial distribution↗

Validation of UARS Microwave Limb Sounder Temperature and Pressure Measurements

The accuracy and precision of the Upper Atmosphere Research Satellite (UARS) Microwave Limb Sounder (MLS) atmospheric temperature and tangent-point pressure measurements are described. Temperatures and tangent-point pressure are retrieved from a 15-channel 63-GHz radiometer measuring O 2 microwave emissions from the stratosphere and mesosphere.

atmospheric↗

EOS MLS Level 1B Data Processing, Version 2.2

A computer program performs level- 1B processing (the term 1B is explained below) of data from observations of the limb of the Earth by the Earth Observing System (EOS) Microwave Limb Sounder (MLS), which is an instrument aboard the Aura spacecraft. This software accepts, as input, the raw EOS MLS scientific and engineering data and the Aura spacecraft ephemeris and attitude data. Its output consists of calibrated instrument radiances and associated engineering and diagnostic data. [This software is one of several computer programs, denoted product generation executives (PGEs), for processing EOS MLS data. Starting from level 0 (representing the aforementioned raw data, the PGEs and their data products are denoted by alphanumeric labels (e.g., 1B and 2) that signify the successive stages of processing.] At the time of this reporting, this software is at version 2.2 and incorporates improvements over a prior version that make the code more robust, improve calibration, provide more diagnostic outputs, improve the interface with the Level 2 PGE, and effect a 15-percent reduction in file sizes by use of data compression.

Perun, Vincent↗

Dynamical Analysis of MLS and ISAMS Data from the Upper Atmosphere Research Satellite

The primary goal of this project is to investigate two aspects of upper stratosphere and mesosphere circulation dynamics using data from the Upper Atmosphere Research Satellite's (UARS) Microwave Limb Sounder (MLS) and Improved Stratospheric and Mesospheric Sounder (ISAMS) instruments. The first aspect involves observational analyses and comparison with model predictions for the polar night "4-day wave". The second project focus is the distribution of carbon monoxide (CO) in the middle atmosphere and circulation features that can be deduced from analyses of such a tracer and comparison with atmospheric circulation models.

Stanford, John L.↗

Solar Occultation Satellite Data and Derived Meteorological Products: Sampling Issues and Comparisons with Aura MLS

Derived Meteorological Products (DMPs, including potential temperature (theta), potential vorticity, equivalent latitude (EqL), horizontal winds and tropopause locations) have been produced for the locations and times of measurements by several solar occultation (SO) instruments and the Aura Microwave Limb Sounder (MLS). DMPs are calculated from several meteorological analyses for the Atmospheric Chemistry Experiment-Fourier Transform Spectrometer, Stratospheric Aerosol and Gas Experiment II and III, Halogen Occultation Experiment, and Polar Ozone and Aerosol Measurement II and III SO instruments and MLS. Time-series comparisons of MLS version 1.5 and SO data using DMPs show good qualitative agreement in time evolution of O3, N2O, H20, CO, HNO3, HCl and temperature; quantitative agreement is good in most cases. EqL-coordinate comparisons of MLS version 2.2 and SO data show good quantitative agreement throughout the stratosphere for most of these species, with significant biases for a few species in localized regions. Comparisons in EqL coordinates of MLS and SO data, and of SO data with geographically coincident MLS data provide insight into where and how sampling effects are important in interpretation of the sparse SO data, thus assisting in fully utilizing the SO data in scientific studies and comparisons with other sparse datasets. The DMPs are valuable for scientific studies and to facilitate validation of non-coincident measurements.

Manney, Gloria↗

Learning from GES DISC's MLS and OMI Data Users: Metrics Matter

It has been over 15 years since Aura research satellite launched in 2004 to observe the Earth's ozone layer, air quality, and climate from four different instruments - the High Resolution Dynamics Limb Sounder (HIRDLS), the Microwave Limb Sounder (MLS), the Ozone Monitoring Instrument (OMI), and the Tropospheric Emission Spectrometer (TES). Observations from the Aura mission have established a concrete understanding of the changing chemistry of our atmosphere.The NASA Goddard Earth Sciences Data and Information Services Center (GES DISC) is the official archive and distribution center for the HIRDLS, MLS, and OMI instruments. This presentation will report metrics of data usage and services on these instruments. Key to GES DISC's mission to provide better data support is gaining a better understanding of our users' needs and behaviors as they discover, access and utilize these data. We will summarize the users' needs from these instruments based on user inquiry information collected over the Aura mission lifetime and present findings from this ensemble metrics.

Metrics↗