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Research and Test Reactor Fuels

PRO-RR is the research reactor focused program element of the broader Proliferation Resistance Optimization program (PRO-X) under the National Nuclear Safety Administration (NNSA) in the U.S. Department of Energy (DOE). PRO-X provides a framework for integrating proliferation resistance in nuclear system designs to minimize weapons usable nuclear materials (WUNM) production and diversion pathways while optimizing systems performance for peaceful use missions. PRO-RR applies the PRO-X mission objectives to research reactor system design. This document serves as one of the foundational documents for the PRO-RR-Fuel System Design technical team by documenting current research reactor fuels usage. The PRO-RR-Fuel System Design technical team consists of subject matter experts from Argonne National Laboratory (Argonne) and Savannah River National Laboratory (SRNL). In order to determine the preferred fuel of use in upcoming research and test reactors to optimize proliferation resistance, performance, and safety, it is useful to assess the fuels that have been used in the past, or are currently in use. This report reviews the historical and current fuels used in research and test reactors to inform future fuel selection. Chapter 2 discusses the low-enriched uranium (LEU) fuels currently in use in terms of thermal power level and utilization of the reactor. Chapter 3 summarizes the fabrication processes for common fuel types. Chapter 4 discusses in detail the fuel types in use in research and test reactors. A review of the cladding types in use is presented in Chapter 5, and a historical review of research and test reactor fuel fabricators is presented in Chapter 6. The data collection strategy used the International Atomic Energy Agency (IAEA) research reactor database [1] as a starting point. Information on the fuel used was gathered on research reactors (other than critical assemblies) that were listed as operational, planned, or in temporary shutdown in the IAEA database. Data on the fuel type, geometry, enrichment, uranium loading, cladding type, and fabricator were collected for each of the reactors available in the public domain. Sources of data included conference papers, journal articles, and facility and fabricator websites. Data on research reactors operating on LEU fuels are presented in Appendix A, while Appendix B presents data collected on all reactors at the time of publication of this report. Appendix C presents data collected on reactors that were part of the M3 research and test reactor conversion program.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Baseline Fuel Fabrication Facility

PRO-RR is the research reactor focused program element of the broader Proliferation Resistance Optimization program (PRO-X) under the National Nuclear Safety Administration (NNSA) in the U.S. Department of Energy (DOE). PRO-X provides a framework for integrating proliferation resistance in nuclear system designs to minimize weapons usable nuclear materials (WUNM) production and diversion pathways while optimizing systems performance for peaceful use missions. PRO-RR applies the PRO-X mission objectives to research reactor system design. This document serves as one of the foundational documents for the PRO-RR-Fuel System Design technical team by documenting a baseline fuel fabrication facility to be used for further optimization studies. The PRO-RR-Fuel System Design technical team consists of subject matter experts from Argonne National Laboratory (Argonne) and Savannah River National Laboratory (SRNL). In order to develop specific strategies for fuel fabrication facilities to optimize proliferation resistance, performance, and safety, a baseline fuel fabrication facility design basis was developed. Having a baseline design basis allows for the qualitative and quantitative comparison of design choices in the optimization process. This report describes the baseline fuel fabrication facility and general optimization strategy. Chapter 2 describes the fuel system selected for examination, the fabrication process used as the baseline, a description of the model developed to track uranium utilization, and a generic floorplan of the fabrication facility. Chapter 3 describes the overarching optimization strategy that could be implemented for a fabrication facility.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Fuel Fabrication Capability Assessment in Support of Advanced Reactor Deployments

More than 30 U.S. companies are designing a variety of advanced reactor concepts, and several companies are planning to demonstrate their reactor designs in the mid-2020s to late 2030s time frame. In 2020, the U.S. Department of Energy (DOE) announced a series of awards under the Advanced Reactor Demonstration Program (ARDP) to accelerate the successful deployment of 10 of these reactors under three pathways. TerraPower and X-energy were awarded grants under the Advanced Reactor Demonstration Program to deploy their respective Natrium reactor and Xe-100 reactor designs in the next 7–10 years. These demonstrations are in addition to several parallel programs, including the U.S. Department of Defense’s (DoD’s) interest in the development of microreactors, and interest of the National Aeronautics and Space Administration in space nuclear power and propulsion. The National Reactor Innovation Center’s (NRIC’s) mission is to accelerate the demonstration and deployment of advanced reactors; NRIC is partnering with several reactor developers and harnessing the world-class capabilities of the U.S. National Laboratory system to deliver on its mission. Several of these reactor designs will require advanced fuel forms that are not commercially available today, including metal fuel, molten salt fuel, TRi-structural ISOtropic (TRISO) particle fuel, and uranium nitride fuel. Recognizing that there may be potential gaps in the laboratory-scale process development and pilot-scale first-of-a-kind (FOAK) production of these fuel forms leading to delivery of the FOAK cores, NRIC commissioned this study to look at the challenges that need to be overcome for successful deliveries, including the evaluation of existing facilities and the potential need for a new fuel fabrication facility.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Physics Division Strategic Plan: Science Drivers

The Physics Division Science Drivers articulate the overarching scientific objectives that we seek to address and that form the lifeblood of our Division. While many physics subfields are represented in the Physics Division’s scientific portfolio, we strive to maintain or achieve excellence and international leadership in only a few areas. While diversity of science and engineering efforts is strongly supported and provides the fertile soil for innovation, there are dominating areas in which we must excel to accomplish our mission that is stated as: “We design, execute and analyze experiments that challenge, improve and validate our understanding of fundamental physics underpinning LANL’s national security mission.”

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

The Interstellar Mapping And Acceleration Probe High Energy (IMAP-Hi) Neutral Atom Imager

The IMAP-Hi Energetic Neutral Atom (ENA) Imager on NASA’s Interstellar Mapping and Acceleration Probe (IMAP) mission (McComas et al. 2018a, 2025) is designed to measure ENAs from the global interaction between the heliosphere and the local interstellar medium (LISM). These ENAs are initially plasma ions of solar wind origin that are neutralized by charge exchange with the cold neutral atoms of LISM that freely flow through the heliosphere-LISM interaction region. IMAP-Hi consists of two identical single-pixel sensors, each covering the ENA spectral range from 0.44 keV to 15.6 keV over nine contiguous energy passbands and having an approximately conical field-of-view (FOV) of 4.1o full width at half maximum (FWHM). The Hi-45 sensor points 45o relative to the spacecraft spin axis from the antisunward direction; each spacecraft spin, it measures ENA intensity over a circular swath with half-cone angle 45o centered on the ecliptic plane. The Hi-90 sensor points 90o relative to the spin axis; each spacecraft spin, it measures ENA intensity over a great circle in the sky, sampling both the north and south ecliptic poles. As the IMAP spin vector is re-pointed daily toward the Sun, the ecliptic longitude of the swaths moves daily by ∼1o such that a full sky map is acquired by Hi-90 every six months and a complete low latitude (−45o to +45o) map is acquired by Hi-45 annually. The IMAP-Hi sensor design has direct heritage from the IBEX-Hi imager on the Interstellar Boundary Explorer (IBEX) mission, with substantial improvements in energy range, energy resolution, angular resolution, signal-to-noise ratio, and, for ecliptic latitudes within ±45o, temporal resolution and exposure time. The global ENA maps acquired by IMAP-Hi partially overlap in energy and viewing with the ENA maps acquired by the IMAP-Lo and IMAP-Ultra ENA imagers, which we combine to answer fundamental questions about the structure and dynamics of the interaction of the heliosphere and the LISM.

79 ASTRONOMY AND ASTROPHYSICS↗

Technical Resilience Navigator

The Technical Resilience Navigator (TRN) is a systematic approach to identifying vulnerabilities with energy and water systems, and prioritizing solutions that reduce risk. The ultimate outcome of the TRN is a set of actionable resilience solutions that address the site's most important gaps in resilience and enhance the ability to maintain mission continuity. The TRN is designed to step users through this planning process, providing a framework to: assign roles and responsibilities; collect and document information and data; document key inputs and outputs for each of the TRN modules (Site Level Planning, Baseline Development, Risk Assessment, Solution Development, and Solution Prioritization); document prioritized list of resilience solutions; and track progress through the entire process. Currently "software as a service" at the listed website.

Rotondo, Julia↗

Earth as an Exoplanet. I. Time Variable Thermal Emission Using Spatially Resolved Moderate Imaging Spectroradiometer Data

Among the more than 4000 exoplanets known today, some terrestrial planets have been detected in the so-called habitable zone of their host stars and their number is expected to increase in the near future, energizing a drive to understand and interpret the eagerly awaited wealth of data to identify signs of life beyond our solar system. So far, Earth remains the best and only example of a habitable (and inhabited) world. Although, it seems extremely unlikely that any other exoplanets will be true Earth twins, it is important to explore and understand the full range of spectral signatures and variability of Earth in order to inform the design of future instruments and missions, and understand their diagnostic power as well as potential limitations. In this work we use Earth observation data collected by the MODIS instrument aboard the Aqua satellite. The complete data set comprises 15 years of thermal emission observations in the 3.66–14.40 μm range for five different locations on Earth (Amazon Rainforest, Antarctica, Arctic, Indian Ocean, and the Sahara Desert). We then determine flux levels and variations as a function of wavelength and surface type (i.e., climate zone and surface thermal properties) and investigate whether periodic signals indicating Earth’s tilted rotation axis can be detected. Our findings suggest that (1) viewing geometry plays an important role when thermal emission data is analyzed as Earth’s spectrum varies by a factor of three and more depending on the dominant surface type underneath; (2) typically strong absorption bands from CO 2 (15 μm) and O 3 (9.65 μm) are significantly less pronounced and partially absent in data from the polar regions implying that estimating correct abundance levels for these molecules might be challenging in these cases; and (3) the time-resolved thermal emission spectrum encodes information about seasons/planetary obliquity, but the significance depends on the viewing geometry and spectral band considered.

79 ASTRONOMY AND ASTROPHYSICS↗

X-ray characterization of fully-depleted p-channel Skipper-CCDs for the DarkNESS mission

The Dark matter Nanosatellite Equipped with Skipper Sensors (DarkNESS) mission is a 6U CubeSat designed to search for X-ray lines from decaying dark matter using Skipper-CCDs. Thick, fully-depleted p-channel Skipper-CCDs provide low readout noise and high quantum efficiency for 1-10 keV X-rays, but their X-ray performance has not yet been demonstrated in the space environment. DarkNESS will operate in low-Earth orbit, where trapped protons induce displacement damage in the sensor that increases charge-transfer inefficiency and degrades the X-ray energy resolution. This work measures the X-ray line response of Skipper-CCDs before and after proton irradiation and quantifies the associated degradation. A sensor was exposed to 217 MeV protons at a fluence of 8.4 x 10^10 protons cm^-2, corresponding to a displacement-damage dose more than an order of magnitude above the three-year expectation for representative mid-inclination and Sun-synchronous low-Earth orbits. A 55Fe source was used to compare the energy resolution of the beam-exposed quadrant to adjacent unexposed quadrants and a non-irradiated reference sensor. These measurements provide a quantitative assessment of radiation-induced spectral degradation in Skipper-CCDs and enable an estimate of the end-of-life X-ray energy resolution expected for DarkNESS operation in low-Earth orbit.

Alpine, Phoenix [Illinois U., Urbana] (ORCID:00090↗

Effects of Hydrogen Redistribution at High Temperatures in Yttrium Hydride Moderator Material

We report advanced materials development, manufacturing, and modeling capabilities for innovative reactor designs support nuclear security and mission-focused science through enhanced technology for safer and more efficient and secure production of nuclear energy. The high temperature moderator material yttrium hydride poses a significant enhancement in small reactor design by thermalizing (slowing down) neutrons and decreasing the required fuel mass for a system. The research presented here supports understanding hydrogen distribution in yttrium hydride through: (1) the development of neutron-based hydrogen imaging and crystallographic characterization that allows us to understand fundamental diffraction behaviors and to observe changes in hydrogen distribution as a function of temperature and (2) subsequent neutron multiplication (reactivity) effects of changes in hydrogen distribution using measurement-based cross sections in a sample microreactor design. The main conclusions from the work are that: (1) hydrogen does not redistribute significantly below temperatures of 800°C in yttrium hydride and (2) hydrogen redistribution affects the reactivity slightly but not significantly.

36 MATERIALS SCIENCE↗

LANL Weapons Physics Directorate: Mission Scope and Opportunities [Slides]

The Weapons Physics Directorate stewards a number of critical capabilities to meet the LANL mission. To execute our mission, ALDX develops and applies cutting-edge theory, computational models and multi-physics simulation codes, and designs, executes, and analyzes complex experiments. Our mission is to sustain the current stockpile, provide future stockpile options, and help shape a globalized nuclear world.

45 MILITARY TECHNOLOGY, WEAPONRY, AND NATIONAL DEF↗

Evaluation of Low Dose Silicon Carbide Temperature Monitors

Thermocouples are generally used to provide real-time temperature indications in instrumented tests performed at materials and test reactors. Melt wires or paint spots are often included in such tests as an independent technique of detecting peak temperatures incurred during irradiation. In addition, less expensive static capsule tests, which have no leads attached for real-time data transmission, often rely on melt wires and paint spots as a post-irradiation technique for peak temperature indication. Unfortunately, these techniques are limited in that they can only detect whether a single temperature is or is not exceeded. Silicon carbide (SiC) monitors are advantageous because a single monitor can be used to determine the peak temperature reached within a relatively broad range (200 – 800°C). Although the use of SiC monitors was proposed more than five decades ago, the ultimate performance limits of this technique are not fully understood. The Nuclear Science User Facilities (NSUF) is the United States Department of Energy Office of Nuclear Energy's only designated nuclear energy user facility. Its mission is to provide nuclear energy researchers access to world-class capabilities and to facilitate the advancement of nuclear science and technology. This mission is supported by providing access to state-of-the-art experimental irradiation testing, post irradiation examination facilities, and high performance computing capabilities as well as technical and scientific assistance for the design and execution of projects. As part of an NSUF project, low dose silicon carbide monitors were irradiated in the Belgian Reactor 2 and were then evaluated both at the SCK•CEN and at Idaho National Laboratory's High Temperature Test Laboratory to determine their peak temperature achieved during irradiation. The technical significance of this work was that the monitors were irradiated to a dose that was significantly less than recommended in published literature. This paper will discuss the evaluation process, the irradiation test, and the performance of the low dose silicon carbide temperature monitors.

36 MATERIALS SCIENCE↗

NSUF Melt Wire Evaluations for BSU 8242 and GE Hitachi-10393 Irradiation Experiments

The Nuclear Science User Facilities (NSUF) is the United States Department of Energy Office of Nuclear Energy's only designated nuclear energy user facility. Its mission is to provide nuclear energy researchers access to world-class capabilities and to facilitate the advancement of nuclear science and technology. This mission is supported by providing access to state-of-the-art experimental irradiation testing, post-irradiation examination facilities, and high-performance computing capabilities as well as technical and scientific assistance for the design and execution of projects. Two NSUF irradiation experiments, Boise State University-8242 and General Electric Hitachi, used melt wire packs to determine peak temperatures reached during irradiation testing. This report will discuss the temperature evaluation process and present the associated data.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Key Design Trades for a Near-term Lunar Fission Surface Power System

NASA and DOE have been developing concepts for lunar and Mars Fission Surface Power (FSP) systems for decades and have considered many different technologies and system variations. In 2023, three contractor teams completed Phase 1 conceptual design studies on a 40 kWe lunar FSP system in response to a modest set of NASA requirements and goals. A government team consisting of NASA Glenn Research Center (GRC), Los Alamos National Laboratory (LANL), and Idaho National Laboratory (INL) was formed to develop an independent design approach that adhered to the same requirements and goals posed to the contractor teams. GRC provided expertise, analysis, and design decisions for the power conversion, heat rejection, power management & distribution (PMAD), and mission integration. LANL and INL provided expertise, analysis, and design decisions for the reactor and shielding. The goal of the government study was to develop representative concepts that could be used in NASA architecture studies, guide government technology investments, and inform Phase 2 requirements definition. This paper provides a summary of the key technology options, system-level trades, and mission-level concept-of-operations.

99 - GENERAL AND MISCELLANEOUS↗

Final Design of the Material Plasma Exposure eXperiment

The Material Plasma Exposure eXperiment (MPEX) has completed its design phase. MPEX will be a unique facility to investigate plasma material interactions (PMIs) under fusion prototypic divertor conditions in steady state. This includes plasma exposure conditions expected in a fusion reactor divertor. Materials to be investigated will include solids, liquids, and neutron pre-irradiated materials. Electron and ion heating will allow for a large operational domain ranging from erosion-dominated PMI conditions to deposition-dominated PMI conditions. An overview of the final design for all MPEX systems is given. Here, in particular, it is shown how mission-driven project requirements have led to detailed design choices with innovative solutions. Examples are the water-cooled helicon window, the electron cyclotron heating launcher, the target holder and manipulator, and the autonomous decouplers.

Fusion reactor↗

Radiation tolerance of the PNI RM3100 magnetometer for a Europa lander mission

The results of two radiation test campaigns on a low-cost commercial off-the-shelf magnetometer are presented. The test setup and the total ionization dose (TID) levels studied were designed to meet the requirements of a mission to land on Europa. Based on the Europa Lander Science Definition Team report, instruments inside an aluminum vault at the surface of Europa would need to withstand TID of up to 300 krad(SI). In order to evaluate the performance of the PNI RM3100 magnetometer, nine separate sensors were irradiated at two different facilities during two separate campaigns and under different configurations, including passive and active tests. Of the nine sensors, seven survived the TID of 300 krad(SI) while the other two sensors started presenting failures after reaching 150 krad(SI). Post-irradiation tests showed that eight of the nine sensors continued to work without appreciable degradation after stopping exposure, while one sensor stopped working altogether.

58 GEOSCIENCES↗

Decentralized modular hybrid supervisory control for the formation of unmanned helicopters

Abstract Formation control of Unmanned Aerial Vehicles (UAVs) requires them to tightly cooperate to reach and keep the formation, while avoiding collision. This paper proposes a novel decentralized hybrid supervisory control approach for the formation control of multiple UAVs. This is achieved by developing a symbolic motion planning technique to polarly partition the motion space resulting in a finite state discrete event model for the motion dynamics of each UAV. Then, a modular discrete supervisor is designed for different components of the formation mission including reaching the formation, keeping the formation, and collision avoidance. Further, for the collision avoidance mechanism, a novel top‐down decomposition‐based approach is developed to design local supervisors decentralizedly. It is formally proved that with the proposed top‐down decomposition‐based approach, the (locally) supervised UAVs, as a whole, can cooperatively satisfy the desired (global) collision avoidance specification. The proposed decentralized supervisory control algorithm is also verified through a hardware‐in‐the‐loop simulator for the formation control of unmanned helicopters.

Karimoddini, Ali↗

Quantum surrogate models for uncertainty quantification

Surrogate models are a critical ingredient to computation-based design and validation of many DOE mission-relevant physical systems. When first-principles computation of properties of a physical systems becomes pro hibitive, surrogate models are the only path towards achieving tasks such as uncertainty quantification (UQ), exploration of design space, and validation of design choices. In this project we have developed and demonstrated a new surro gate modeling paradigm for complex models that is data-driven, non-intrusive, and has the potential to be versatile and equipped with performance guaran tees. This combination of features is absent in existing surrogate modeling tools. The framework we have developed in this project exploits a quantum-classical correspondence to establish a quantum system that mimics the dynamics of the classical Hamiltonian system from which data in the form of temporal snapshots is provided. Since quantum dynamics propagates distributions over observables, the framework is naturally suited to propagation of epistemic uncertainties in the form of distributions over initial state and parametric uncertainties. In this project, we take the first step in establishing this novel framework by deriving a quantization and de-quantization procedure, demonstrating the accuracy of the quantum surrogate models these define using two model systems, and defining the next steps in maturing the framework towards a tool applicable to Sandia mission-relevant problems.

97 MATHEMATICS AND COMPUTING↗