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At least 91 records · Page 5

Method for Evaluating Irradiation Effects on Flow Stress in Fe-9%Cr ODS Using TEM In Situ Cantilevers

Transmission electron microscopic (TEM) in situ mechanical testing has become a widely utilized tool for simultaneously measuring mechanical properties and understanding fundamental deformation mechanisms in irradiated and nuclear materials. Although tensile and compression specimen geometries are amongst the most common, opportunities remain for investigating alternative geometries that could provide unique insights into the plasticity of irradiated materials. This research demonstrates a new TEM in situ cantilever beam configuration. Cantilevers are produced from as-received and proton irradiated (1 dpa, 500°C) Fe-9%Cr oxide dispersion strengthened (ODS) steel. Flow stress is measured using a TEM in situ depth-sensing mechanical testing holder. A 200 MPa increase in flow stress is measured due to irradiation. Size effects arise when the intrinsic (i.e. microstructural) size approaches the extrinsic (i.e. external dimensions) size and can be described using a power law relationship as a function of the material microstructure and cantilever dimensions.

36 MATERIALS SCIENCE↗

Nucleonic shells and nuclear masses

The binding energy of an isotope is a sensitive indicator of the underlying shell structure as it reflects the net energy content of a nucleus. Since magic nuclei are significantly lighter, or more bound, compared to their neighbors, the presence of nucleonic shell structure makes an imprint on nuclear masses. In this study, using a carefully designed binding-energy indicator, we catalog the appearance of spherical and deformed shell and subshell closures throughout the nuclear landscape. After presenting experimental evidence for shell and subshell closures as seen through the lens of nuclear masses, we study the ability of global nuclear mass models to predict local binding-energy variations related to shell effects.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Limits on assigning a shape to a nucleus

The interpretation of nuclear observables in the laboratory frame in terms of the intrinsic deformation parameters β and γ is a classical theme in nuclear structure. Here we use the quadrupole invariants, calculated within the framework of the configuration-interaction shell model, to clarify the meaning and limitations of nuclear shapes. In this work we introduce a novel method that enables us to calculate accurately higher-order invariants and, therefore, the fluctuations in both β and γ. We find that the shape parameter β often has a non-negligible degree of softness and that the angle γ is usually characterized by large fluctuations, rendering its effective value not meaningful. Contrary to common belief, we conclude that doubly magic nuclei are not spherical, because the notion of a well-defined shape does not apply to them.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Progress in Constraining Nuclear Symmetry Energy Using Neutron Star Observables Since GW170817

The density dependence of nuclear symmetry energy is among the most uncertain parts of the Equation of State (EOS) of dense neutron-rich nuclear matter. It is currently poorly known especially at suprasaturation densities partially because of our poor knowledge about isovector nuclear interactions at short distances. Because of its broad impacts on many interesting issues, pinning down the density dependence of nuclear symmetry energy has been a longstanding and shared goal of both astrophysics and nuclear physics. New observational data of neutron stars including their masses, radii, and tidal deformations since GW170817 have helped improve our knowledge about nuclear symmetry energy, especially at high densities. Based on various model analyses of these new data by many people in the nuclear astrophysics community, while our brief review might be incomplete and biased unintentionally, we learned in particular the following: (1) The slope parameter L of nuclear symmetry energy at saturation density ρ0 of nuclear matter from 24 new analyses of neutron star observables was about L≈57.7±19 MeV at a 68% confidence level, consistent with its fiducial value from surveys of over 50 earlier analyses of both terrestrial and astrophysical data within error bars. (2) The curvature Ksym of nuclear symmetry energy at ρ0 from 16 new analyses of neutron star observables was about Ksym≈−107±88 MeV at a 68% confidence level, in very good agreement with the systematics of earlier analyses. (3) The magnitude of nuclear symmetry energy at 2ρ0, i.e., Esym(2ρ0)≈51±13 MeV at a 68% confidence level, was extracted from nine new analyses of neutron star observables, consistent with the results from earlier analyses of heavy-ion reactions and the latest predictions of the state-of-the-art nuclear many-body theories. (4) While the available data from canonical neutron stars did not provide tight constraints on nuclear symmetry energy at densities above about 2ρ0, the lower radius boundary R2.01=12.2 km from NICER’s very recent observation of PSR J0740+6620 of mass 2.08±0.07M⊙ and radius R=12.2–16.3 km at a 68% confidence level set a tight lower limit for nuclear symmetry energy at densities above 2ρ0. (5) Bayesian inferences of nuclear symmetry energy using models encapsulating a first-order hadron–quark phase transition from observables of canonical neutron stars indicated that the phase transition shifted appreciably both L and Ksym to higher values, but with larger uncertainties compared to analyses assuming no such phase transition. (6) The high-density behavior of nuclear symmetry energy significantly affected the minimum frequency necessary to rotationally support GW190814’s secondary component of mass (2.50–2.67) M⊙ as the fastest and most massive pulsar discovered so far. Overall, thanks to the hard work of many people in the astrophysics and nuclear physics community, new data of neutron star observations since the discovery of GW170817 have significantly enriched our knowledge about the symmetry energy of dense neutron-rich nuclear matter.

79 ASTRONOMY AND ASTROPHYSICS↗

Decay spectroscopy of 160 Eu: Quasiparticle configurations of excited states and structure of K π = 4 + bandheads in 160 Gd

Background: Detailed spectroscopy of neutron-rich, heavy, deformed nuclei is of broad interest for nuclear astrophysics and nuclear structure. Nuclei in the r-process path and following freeze-out region impact the resulting r-process abundance distribution, and the structure of nuclei midshell in both proton and neutron number helps to understand the evolution of subshell gaps and large deformation in these nuclei. Purpose: We aim to improve the understanding of the nuclear structure of 160 Gd, specifically the K π = 4 + bands, as well as study the β decay of 160 Eu into 160 Gd. Methods: High-statistics decay spectroscopy of 160 Gd resulting from the β-decay of 160 Eu was collected using the GRIFFIN spectrometer at the TRIUMF-ISAC facility. Results: Two new excited states and ten new transitions were observed in 160 Gd. The β-decaying half-lives of the low- and high-spin isomers in 160 Eu were determined, and the low-spin state's half-life was measured to be t 1/2 = 26.0 (8) s, ≈ 16% shorter than previous measurements. Lifetimes of the two K π = 4 + bandheads in 160 Gd were measured for the first time, as well as γ – γ angular correlations and mixing ratios of intense transitions out of those bandheads. Conclusions: Lifetimes and mixing ratios suggest that the hexadecapole phonon model of the K π = 4 + bandheads in 160 Gd is preferred over a simple two-state strong mixing scenario, although further theoretical calculations are needed to fully understand these states. Additionally, the 1999.0-keV state in 160 Gd heavily populated in β decay is shown to have positive parity, which raises questions regarding the structure of the high-spin β-decaying state in 160 Eu.

150 ≤ A ≤ 189↗

Properties of the neutron star crust: Quantifying and correlating uncertainties with improved nuclear physics

A compressible liquid-drop model (CLDM) is used to correlate uncertainties associated with the properties of the neutron star (NS) crust with theoretical estimates of the uncertainties associated with the equation of state (EOS) of homogeneous neutron and nuclear matter. For the latter, we employ recent calculations based on Hamiltonians constructed using chiral effective-field theory (χEFT). Fits to experimental nuclear masses are employed to constrain the CLDM further, and we find that they disfavor some of the χEFT Hamiltonians. The CLDM allows us to study the complex interplay between bulk, surface, curvature, and Coulomb contributions, and their impact on the NS crust. It also reveals how the curvature energy alters the correlation between the surface energy and the bulk symmetry energy. Here our analysis quantifies how the uncertainties associated with the EOS of homogeneous matter implies significant uncertainties for the composition of the crust, its proton fraction, and the volume fraction occupied by nuclei. We find that the finite-size effects impact the crust composition but have a negligible effect on the net isospin asymmetry of matter. The isospin asymmetry is largely determined by the bulk properties and the isospin dependence of the surface energy. The most significant uncertainties associated with matter properties in the densest regions of the crust, the precise location of the crust-core transition, are found to be strongly correlated with uncertainties associated with the Hamiltonians. By adopting a unified model to describe the crust and the core of NSs, we tighten the correlation between their global properties such as their mass-radius relationship, moment of inertia, crust thickness, and tidal deformability with uncertainties associated with the nuclear Hamiltonians.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

β -decay half-lives of 55 neutron-rich isotopes beyond the N = 82 shell gap

The β -decay half-lives of 55 neutron-rich nuclei Sn 134 - 139 , Sb 134 - 142 , Te 137 - 144 , I 140 - 146 , Xe 142 - 148 , Cs 145 - 151 , Ba 148 - 153 , and La 151 - 155 were measured at the Radioactive Isotope Beam Factory employing the projectile fission fragments of U 238 . The nuclear level structure, which relates to deformation, has a large effect on the half-lives. The impact of newly measured half-lives on modeling the astrophysical origin of the heavy elements is studied in the context of r process nucleosynthesis. For a wide variety of astrophysical conditions, including those in which fission recycling occurs, the half-lives have an important local impact on the second ( A ≈ 130) peak.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

A novel fiber-fretting test for tribological characterization of the fiber/matrix interface

Ceramic matrix composites exhibit excellent high temperature properties and are candidate materials for structural applications from jet engines to nuclear fuel cladding. The strength and deformation behavior of these composites are intrinsically tied to the properties of the fiber/matrix interface. This research introduces a novel technique to evaluate the fundamental friction and wear characteristics of these interfaces. A case study on SiC f /PyC/SiC m composites applies in situ fiber fretting to investigate the kinetic friction coefficient and cyclic wear characteristics of the interphase. The experimental methodology is presented in explicit detail to encourage other researchers to explore the capabilities of this technique. Additionally, testing was carried out as a function of fiber roughness, PyC thickness (≈10, 500, 1200 nm), cycle count (10, 100, 1000), and frequency (1, 5, and 10 Hz). The friction coefficient and wear behavior changed with cycle length due to a transition from adhesive to abrasive mechanisms. SEM fractography provided insights to tribological evolution from adhesive sliding to three-body abrasive wear. The structural disorder at the tribo-surface relating to graphitic content and dangling bond density was investigated using Raman spectroscopy. Properties are contextualized with comparison to uniaxial tensile behavior of the parent composite.

36 MATERIALS SCIENCE↗

Investigation of the excited states of 114 Sn using the GRIFFIN spectrometer at TRIUMF

The semi-magic 110-122 Sn isotopes display signs of shape coexistence in their excited 0 + states, which, in contrast to the spherical 0+ ground states, are deformed. Here, this paper investigates the nuclear structure of 114 Sn using the competing β + decay and electron capture of a radioactive beam of 114 Sb produced at the TRIUMF-ISAC facility using the GRIFFIN spectrometer. This study will allow for an in-depth understanding of the excited 0 + states in 114 Sn, by focusing on their decay patterns. In the present experiment, transitions at 856.2-keV and 1405.0-keV, which were observed in an earlier β + decay study but not placed in the 114 Sn level scheme, have been Physics, assigned to the level scheme in connection to the 0$^+_3$ level at 2156.0-keV. Properly assigning these transitions refines the level scheme and enhances our understanding of the nuclear structure in 114 Sn.

GRIFFIN↗

Accessing the shape of atomic nuclei with relativistic collisions of isobars

Nuclides sharing the same mass number (isobars) are observed ubiquitously along the stability line. While having nearly identical radii, stable isobars can differ in shape, and present different quadrupole deformations. We show that even small differences in these deformations can be probed by relativistic nuclear collisions experiments, where they manifest as deviations from unity in the ratios of elliptic flow coefficients taken between isobaric systems. Collider experiments with isobars represent, thus, a unique means to gain precise knowledge of the geometric shape of atomic nuclei.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Imaging nuclear shape through anisotropic and radial flow in high-energy heavy-ion collisions

Most atomic nuclei exhibit ellipsoidal shapes characterized by quadrupole deformation β 2 and triaxiality γ, and sometimes even a pear-like octupole deformation β 3 . The STAR experiment introduced a new ‘imaging-by-smashing’ technique to image the nuclear global shape by colliding nuclei at ultra-relativistic speeds and analyzing outgoing debris. Features of nuclear shape manifest in collective observables like anisotropic flow vn and radial flow via mean transverse momentum [p T ]. We present new measurements of the variances of v n (n = 2, 3, and 4) and [p T ], and the covariance of $v$$^{2}_{n}$ with [p T ], in collisions of highly deformed 238 U and nearly spherical 197 Au. Ratios of these observables between the two systems effectively suppress common final-state effects, isolating the strong impact of uranium’s deformation. By comparing results with state-of-the-art hydrodynamic model calculations, we extract β 2U and γ U values consistent with those deduced from low-energy nuclear structure measurements. Measurements of v 3 and its correlation with [p T ] also provide the first experimental suggestion of a possible octupole deformation for 238 U. These findings provide significant support for using high-energy collisions to explore nuclear shapes on femtosecond timescales, with implications for both nuclear structure and quark-gluon plasma studies.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Nuclear states projected from a pair condensate

Atomic nuclei exhibit deformation, pairing correlations, and rotational symmetries. To meet these competing demands in a computationally tractable formalism, we revisit the use of general pair condensates with good particle number as a trial wave function for even-even nuclei. After minimizing the energy of the condensate, allowing for general triaxial deformations, we project out states with good angular momentum with a fast projection technique. To show applicability, we present example calculations from pair condensates in several model spaces and compare against angular-momentum projected Hartree-Fock and full configuration-interaction shell-model calculations. This approach successfully generates spherical, vibrational, and rotational spectra, demonstrating potential for modeling medium- to heavy-mass nuclei.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Axially-deformed solution of the Skyrme-Hartree-Fock-Bogoliubov equations using the transformed harmonic oscillator basis (IV) HFBTHO (v4.0): A new version of the program

We describe the new version 4.0 of the code HFBTHO that solves the nuclear Hartree-Fock-Bogoliubov problem by using the deformed harmonic oscillator basis in cylindrical coordinates. In the new version, we have implemented the restoration of rotational, particle number, and reflection symmetry for even-even nuclei. The restoration of rotational symmetry does not require using bases closed under rotation. Furthermore, we added the SeaLL1 functional and improved the calculation of the Coulomb potential. Finally, we refactored the code to facilitate maintenance and future developments.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Large-scale calculations of 𝛽-decay rates and implications for 𝑟-process nucleosynthesis

Nuclear 𝛽 decay is a key element of the astrophysical rapid neutron capture process (𝑟 process). In this work, we present state-of-the-art global 𝛽-decay calculations based on the quantified relativistic nuclear energy density functional theory and the deformed proton-neutron quasiparticle random-phase approximation. Our analysis considers contributions from allowed and first-forbidden transitions. We used two point-coupling functionals with carefully calibrated time-odd terms and isoscalar pairing strength. The new calculations display consistent results for both employed functionals, especially near the neutron drip line, suggesting slower 𝛽 decays past the 𝑁=126 neutron shell closure than in commonly used 𝛽-decay models. The new rates, along with the existing rates based on the recent nonrelativistic global calculations, are found to slow down the synthesis of heavy elements in the 𝑟 process and significantly reduce the contribution of neutron-induced fission.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Effect of helium bubbles on the mobility of edge dislocations in copper

Abstract Helium bubbles can form in materials upon exposure to irradiation. It is well known that the presence of helium bubbles can cause changes in the mechanical behavior of materials. To improve the lifetime of nuclear components, it is important to understand deformation mechanisms in helium-containing materials. In this work, we investigate the interactions between edge dislocations and helium bubbles in copper using molecular dynamics (MD) simulations. We focus on the effect of helium bubble pressure (equivalently, the helium-to-vacancy ratio) on the obstacle strength of helium bubbles and their interaction with dislocations. Our simulations predict significant differences in the interaction mechanisms as a function of helium bubble pressure. Specifically, bubbles with high internal pressure are found to exhibit weaker obstacle strength as compared to low-pressure bubbles of the same size due to the formation of super-jogs in the dislocation. Activation energies and rate constants extracted from the MD data confirm this transition in mechanism and enable upscaling of these phenomena to higher length-scale models.

36 MATERIALS SCIENCE↗

Joint Inversion of Regional Waveform, First-Motion Polarity, and Synthetic Aperture Radar Surface Displacement for the Fourth and Sixth North Korean Declared Nuclear Explosions

Here, this study analyzed the Democratic People’s Republic of Korea’s (DPRK) fourth (DPRK4, 6 January 2016 M w 4.49) and sixth (DPRK6, 7 September 2017 M w 5.2) declared nuclear tests, employing a joint seismic and Interferometric Synthetic Aperture Radar (InSAR) inversion to improve understanding of these events and enhance moment tensor (MT) inversion capabilities. The recent efforts have focused on employing seismic waveform and InSAR geodetic deformation data separately to analyze these and the previous nuclear tests (e.g., Chiang et al., 2018; Myers et al., 2018; Wang et al., 2018). Building upon our previous work (Chi-Durán et al., 2021), we performed a joint regional waveform, first-motion (FM) polarity, and surface displacement inversion, which demonstrated improved source-type discrimination, a revised MT solution with reduced scalar moment uncertainty, and an independently constrained location. In this article, we build on the previous results for DPRK6 by including an analysis using a four-layered velocity model with free-surface topography to compute the near-source static deformation Green’s functions. The model consists of a 50 m basalt layer (⁠V P = 2.07 km/s, V S = 1.2 km/s⁠), a 250 m stratified volcanic deposit layer (⁠V P = 1.73 km/s, V S = 1.0 km/s⁠), a 700 m weathered granodiorite layer (⁠V P = 2.5 km/s, V S = 1.3 km/s⁠⁠), and a granodiorite half-space (⁠V P = 5.35 km/s, V S = 3.09 km/s⁠⁠). The half-space shares the velocity of the regional MDJ2 velocity model (Ford et al., 2010), which has proven effective for waveform inversion in the region. This model considers the range of reported values for various lithologies and weathering effects. Our findings show that using the layered velocity model enhances the recovery of source location and depth for both the explosions by improving fits and reducing uncertainties. The joint inversion also improves source-type discrimination and better constrains the scalar seismic moment necessary for downstream yield estimation.

58 GEOSCIENCES↗