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NASA NTRS2001

Are Stronger North-Atlantic Southwesterlies the Forcing to the Late-Winter Warming in Europe?

We examine a possible mechanism leading to late-winter warming and thus to an early spring in Europe. From the NCEP Reanalysis, we extract for the years 1948-1999 ocean-surface winds over the eastern North Atlantic, and air temperatures at the surface, T(sub s), and at the 500 mb level, T(sub 500), in late-winter and spring. T(sub s) is extracted at six European locations, all at 50.5 N, ranging in longitude from 1.9 E (northeastern France) to 26.2 E (Ukraine). To quantify the advection of maritime air into Europe, we evaluate for 3-pentad groups the Index I(sub na) of the southwesterlies at 45 N; 20 W: I(sub na) is the average wind speed at this point if the direction is from the quadrant 180-270 deg (when the direction is different, the contribution counts as zero). In late winter correlations C(sub it) between the Index I(sub na) and the temperature T(sub s) are substantial, up to the 0.6 level, in western Europe (but weaker correlations for Poland and Ukraine). C(sub it) drops sharply by mid-March, taking occasionally negative values subsequently. This drop in C(sub it) indicates that maritime air advection is no longer associated closely with the surface-air warming, the role of immolation becomes important, and thus the drop in C(sub it) marks the arrival of spring. Correlations C(sub i delta) between I(sub na) and our lapse-rate parameter delta, the difference between T(sub s) and T(sub 500), indicate that the flow of warm maritime-air from the North Atlantic into this 'corridor' at 50.5 N is predominantly at low tropospheric level. By computing the best linear fit to I(sub na) and T(sub s), the trends for the period 1948-1999 are evaluated. The trends are appreciable in the second half of February and the first half of March. Our 3-pentad analysis points to the interval from mid-February to mid-March as the end-of-winter period in which the southwesterlies over the eastern North Atlantic become stronger and the surface-air temperatures in Europe rise markedly, the lapse rate becomes steeper, and concurrently the longitudinal temperature gradient between the Somme (France) and the Oder (Germany/Poland border) is reduced by 0.8 C, that is, by 20% of its 1948 value. Our thesis, that the observed late-winter warming and the corollary advancement of spring in Europe resulted at least in part from stronger southwesterlies over the North Atlantic, merits further investigations.

Otterman, J.↗

NASA NTRS2002

GCM Simulation of the Large-scale North American Monsoon Including Water Vapor Tracer Diagnostics

In this study, we have applied GCM water vapor tracers (WVT) to simulate the North American water cycle. WVTs allow quantitative computation of the geographical source of water for precipitation that occurs anywhere in the model simulation. This can be used to isolate the impact that local surface evaporation has on precipitation, compared to advection and convection. A 15 year 1 deg, 1.25 deg. simulation has been performed with 11 global and 11 North American regional WVTs. Figure 1 shows the source regions of the North American WVTs. When water evaporates from one of these predefined regions, its mass is used as the source for a distinct prognostic variable in the model. This prognostic variable allows the water to be transported and removed (precipitated) from the system in an identical way that occurs to the prognostic specific humidity. Details of the model are outlined by Bosilovich and Schubert (2002) and Bosilovich (2002). Here, we present results pertaining to the onset of the simulated North American monsoon.

Bosilovich, Michael G.↗

NASA NTRS2003

Satellite Detection of Precipitation over the North Pacific

Intense extratropical winter cyclones often impact the West Coast of North America with strong winds and heavy precipitation. Several times during a winter season, short-term forecasts (24 - 48 hours) of these storms are seriously deficient with central pressure errors in the 10's of hPa and surface low position errors in the 100's of km. For example, 48-hr sea level pressure errors (forecast - observation) at buoy 46005 off the Oregon coast for the 2001 - 2002 winter season is plotted. In addition, two times the standard deviation (determined from pressure errors from the last four winter seasons) are also shown. It is evident from this figure that large forecast errors (i.e. greater than 10 hPa) occurred about 10 times this past winter at buoy 46005 with three events where the errors were 20 hPa. Beside large forecast errors of sea level pressure, numerical forecasts of precipitation for land falling cyclones can also be flawed. This is due in large part to the lack of accurate precipitation information over the ocean. Therefore, remote sensing techniques are the only viable option for obtaining accurate information on the distribution and intensity of precipitation over the North Pacific. Due to the radiative characteristics of precipitation sized hydrometeors at microwave frequencies, microwave sensors are able to detect precipitation over oceanic regions. Past studies have demonstrated the utility of passive microwave rainrate data for locating intense rainfall in rapidly deepening cyclones, in detecting developing polar mesocyclones and in determining frontal bands. There are currently many sources of microwave rainrate data: the Special Sensor Microwave Imager (SSM/I) (currently flying on three platforms), the Advanced Microwave Sounding Unit (AMSU-B) (currently flying on NOAA-15, NOAA-16, and NOAA-17), and the Tropical Rainfall Measuring Mission Microwave Imager (TMI). Data will soon be available from the Advanced Microwave Radiometer-EOS (AMSR-E) on the Aqua platform. In this paper, we present a new technique for mapping rainrate distributions over the North Pacific utilizing rainrate estimates from several microwave sensors and upper-tropospheric winds derived from geosynchronous satellite IR data. The goal of this work is to develop a way to obtain high temporal and spatial rainfall information over the North Pacific. This information will be used to support the verification of model derived precipitation distributions and to support the analysis of in situ measurements of rainfall during the Improvement of Microphysical Parameterization through Observational Verification Experiment (IMPROVE) field campaigns.

Smith, Jeremy↗

NASA NTRS2002

The 1996-2002 Plunge in the North-Atlantic Oscillation Index Produces Cold Spring Temperatures in Central Europe

Surface-air temperatures in winter and spring in central Europe rose over the second half of the 20th century, reported for different data-spans, and by different approaches (Ross et al., 1996; Angell, 1999; Hansen et al., 1999; Demaree et al., 2002). Analysis with a finer temporal resolution shows that late-winter and early-spring (February and March) trends are much stronger than the 3-month season averages (Otterman et al., 2002a). Responding to this need for finer than 3- month resolution, observations at meteorological stations in central Europe are analyzed here for the years 1951-2002, computing six-pentad (5-day period) averages (effectively monthly averages for January, February, and March). The daily minimum surface-air temperature, T(sub min), and the daily maximum temperature, T(sub max), rose steeply in Berlin and Poznan' in the years 1951-1995. Based on sensitivity studies, the bulk of this sharp warming is due to stronger southwesterlies over the North Atlantic, with which the temperatures in Europe are strongly correlated (Otterman et al., 1999; 2002a). However, for the most recent seven years, a pronounced downturn of the warming is observed, which we attribute to the concurrent, 1996-2002, sharp downturn of the ocean-surface southwesterlies over the North Atlantic (Otterman et al., 2002b). Such changes in the ocean winds and variations in the storm tracks are associated with changes in the North Atlantic Oscillation, NAO (Rogers, 1997). The NAO index, the difference in the surface pressure between Iceland and Azores, constitutes a measure of the zonal winds over the eastern North Atlantic, and thus is a critically important factor influencing the flow of maritime air into Europe (but the temperature of the advected airmasses depends on the meridional component, as we discuss). The recent (1996-2002) downturn in this index resulted in much colder spring temperatures in Europe, with adverse significance for the growing season.

Atlas, Robert↗

NASA NTRS2003

Yearly Comparisons of the Mars North Polar Cap: 1999, 2001, and 2003 MOC Observations

The seasonal cycle of the martian north polar cap has been studied since the time of William Herschel, who published the first quantitative observations of the seasonal recession of the polar caps in 1784. Ground-based observations made after Herschel were summarized by Slipher in 1962. More recent ground-based observations of the north polar cap have been done by Iwasaki et al. Mariner 9 and Viking also made north polar observations. Cantor et al. used Hubble Space Telescope observations between 1990 and 1997 to determine several north polar recessions and Lambert albedos of the cap. Mars Global Surveyor went into orbit around Mars in September 1997. The wide-angle cameras on the Mars Orbiter Camera (MOC) acquire images of the entire planet every day at a resolution of approx. 7.5 km/pixel in both red (575 nm - 625 nm) and blue (400 nm - 450 nm) bandpasses (WAR and WAB). Some polar cap observations were acquired during the aerobraking (AB) and science phasing (SPO) of MGS before systematic mapping began in March, 1999 at Ls = 110 .

Benson, J. L.↗

NASA NTRS2007

Trans-Pacific Transport of Saharan Dust to Western North America: A Case Study

The first documented case of long range transport of Saharan dust over a pathway spanning Asia and the Pacific to Western North America is described. Crustal material generated by North African dust storms during the period 28 February - 3 March 2005 reached western Canada on 13-14 March 2005 and was observed by lidar and sunphotometer in the Vancouver region and by high altitude aerosol instrumentation at Whistler Peak. Global chemical models (GEOS-CHEM and NRL NAAPS) confirm the transport pathway and suggest source attribution was simplified in this case by the distinct, and somewhat unusual, lack of dust activity over Eurasia (Gobi and Takla Makan deserts) at this time. Over western North America, the dust layer, although subsiding close to the boundary layer, did not appear to contribute to boundary layer particulate matter concentrations. Furthermore, sunphotometer observations (and associated inversion products) suggest that the dust layer had only subtle optical impact (Aerosol Optical Thickness (Tau(sub a500)) and Angstrom exponent (Alpha(sub 440-870) were 0.1 and 1.2 respectively) and was dominated by fine particulate matter (modes in aerodynamic diameter at 0.3 and 2.5microns). High Altitude observations at Whistler BC, confirm the crustal origin of the layer (rich in Ca(++) ions) and the bi-modal size distribution. Although a weak event compared to the Asian Trans-Pacific dust events of 1998 and 2001, this novel case highlights the possibility that Saharan sources may contribute episodically to the aerosol burden in western North America.

Kendry, Ian G. M.↗

NASA NTRS2010

A Northward Shift of the North Atlantic Ocean Intertropical Convergence Zone in Response to Summertime Saharan Dust Outbreaks

The influence on the summertime North Atlantic Ocean inter-tropical convergence zone (ITCZ) of Saharan dust outbreaks is explored using nine years of continuous satellite observations and atmospheric reanalysis products. During dust outbreak events rainfall along the ITCZ shifts northward by 1 to 4 degrees latitude. Dust outbreaks coincide with warmer lower-tropospheric temperatures compared to low dust conditions, which is attributable to advection of the warm Saharan Air Layer, enhanced subtropical subsidence, and radiative heating of dust. The enhanced positive meridional temperature gradient coincident with dust outbreaks is accompanied by an acceleration of the easterly winds on the n011h side of the African Easterly Jet (AEJ). The center of the positive vorticity region south of the AEJ moves north drawing the center of low-level convergence and ITCZ rainfall northward with it. The enhanced precipitation on the north side of the ITCZ occurs in spite of widespread sea surface temperature cooling north of the ITCZ owing to reduced surface solar insolation by dust scattering.

Wilcox, Eric M.↗

NASA NTRS2012

On the Influence of North Pacific Sea Surface Temperature on the Arctic Winter Climate

Differences between two ensembles of Goddard Earth Observing System Chemistry-Climate Model simulations isolate the impact of North Pacific sea surface temperatures (SSTs) on the Arctic winter climate. One ensemble of extended winter season forecasts is forced by unusually high SSTs in the North Pacific, while in the second ensemble SSTs in the North Pacific are unusually low. High Low differences are consistent with a weakened Western Pacific atmospheric teleconnection pattern, and in particular, a weakening of the Aleutian low. This relative change in tropospheric circulation inhibits planetary wave propagation into the stratosphere, in turn reducing polar stratospheric temperature in mid- and late winter. The number of winters with sudden stratospheric warmings is approximately tripled in the Low ensemble as compared with the High ensemble. Enhanced North Pacific SSTs, and thus a more stable and persistent Arctic vortex, lead to a relative decrease in lower stratospheric ozone in late winter, affecting the April clear-sky UV index at Northern Hemisphere mid-latitudes.

Hurwitz, Margaret M.↗

NASA NTRS2012

Use of MODIS Snow-Cover Maps for Detecting Snowmelt Trends in North America

Research has shown that the snow season in the Northern Hemisphere has been getting shorter in recent decades, consistent with documented global temperature increases. Specifically, the snow is melting earlier in the spring allowing for a longer growing season and associated land-cover changes. Here we focus on North America. Using the Moderate-Resolution Imaging Radiometer (MODIS) cloud-gap-filled standard snow-cover data product we can detect a trend toward earlier spring snowmelt in the approx 12 years since the MODIS launch. However, not all areas in North America show earlier spring snowmelt over the study period. We show examples of springtime snowmelt over North America, beginning in March 2000 and extending through the winter of 2012 for all of North America, and for various specific areas such as the Wind River Range in Wyoming and in the Catskill Mountains in New York. We also compare our approx 12-year trends with trends derived from the Rutgers Global Snow Lab snow cover climate-data record.

Hall, Dorothy K.↗

NASA NTRS2013

The North-South Asymmetry of the Heliospheric Current Sheet: Results of an MHD Simulation

A displacement of the heliospheric current sheet (HCS) south of the helioequator by approx.10deg was proposed by Simpson et al. (1996) as a possible explanation of the north-south asymmetry in the galactic cosmic rays observed by Ulysses during its first fast transit in 1994-1995. The idea was not supported by magnetic field measurements on Ulysses and, on this ground, was dismissed by Simpson et al. (1996). In addition, Erdos & Balogh (1998) argued that any north-south symmetry was unlikely as there should be flux balance between the magnetic sectors of opposite polarity. Nonetheless, many in the scientific community have accepted the original suggestion of Simpson et al. (1996) that a displacement of the HCS was responsible for the cosmic ray asymmetry. In this paper, using a magnetohydrodynamic model of the solar corona and solar wind that includes both dipole and quadrupole magnetic source terms, we show that a north-south asymmetry of the magnetic field on the Sun does not give rise to a displacement of the HCS. The lack of displacement of the HCS results from a latitudinal redistribution of magnetic flux near the Sun where the plasma beta much < 1. The latitudinal redistribution is a direct consequence of the magnetic field gradient between pole and equator. Near the Sun, the latitudinal gradient in magnetic field generates meridional flows directed equatorward that tend to relax the gradient in the magnetic field (to make it more latitude-independent) as heliocentric distance increases. If there is an asymmetry between north and south magnetic field strength then the meridional flows are also asymmetric (i.e., stronger in the hemisphere of stronger magnetic field). Because the magnetic fluxes (positive and negative) in the hemispheres must be equal, the redistribution shifts the HCS into balance by approx. 16 R(solar mass). At larger distances, where the magnetic field is relatively weak (beta much > 1), the HCS can be displaced if there is a difference in total pressure between the hemispheres.

solar wind↗

NASA NTRS2014

Sources, Sinks, and Transatlantic Transport of North African Dust Aerosol: A Multimodel Analysis and Comparison With Remote Sensing Data

This study evaluates model-simulated dust aerosols over North Africa and the North Atlantic from five global models that participated in the Aerosol Comparison between Observations and Models phase II model experiments. The model results are compared with satellite aerosol optical depth (AOD) data from Moderate Resolution Imaging Spectroradiometer (MODIS), Multiangle Imaging Spectroradiometer (MISR), and Sea-viewing Wide Field-of-view Sensor, dust optical depth (DOD) derived from MODIS and MISR, AOD and coarse-mode AOD (as a proxy of DOD) from ground-based Aerosol Robotic Network Sun photometer measurements, and dust vertical distributions/centroid height from Cloud Aerosol Lidar with Orthogonal Polarization and Atmospheric Infrared Sounder satellite AOD retrievals. We examine the following quantities of AOD and DOD: (1) the magnitudes over land and over ocean in our study domain, (2) the longitudinal gradient from the dust source region over North Africa to the western North Atlantic, (3) seasonal variations at different locations, and (4) the dust vertical profile shape and the AOD centroid height (altitude above or below which half of the AOD is located). The different satellite data show consistent features in most of these aspects; however, the models display large diversity in all of them, with significant differences among the models and between models and observations. By examining dust emission, removal, and mass extinction efficiency in the five models, we also find remarkable differences among the models that all contribute to the discrepancies of model-simulated dust amount and distribution. This study highlights the challenges in simulating the dust physical and optical processes, even in the best known dust environment, and stresses the need for observable quantities to constrain the model processes.

Africa↗

NASA NTRS2014

Column Aerosol Optical Properties and Aerosol Radiative Forcing During a Serious Haze-Fog Month over North China Plain in 2013 Based on Ground-Based Sunphotometer Measurements

In January 2013, North China Plain experienced several serious haze events. Cimel sunphotometer measurements at seven sites over rural, suburban and urban regions of North China Plain from 1 to 30 January 2013 were used to further our understanding of spatial-temporal variation of aerosol optical parameters and aerosol radiative forcing (ARF). It was found that Aerosol Optical Depth at 500 nm (AOD500nm) during non-pollution periods at all stations was lower than 0.30 and increased significantly to greater than 1.00 as pollution events developed. The Angstrom exponent (Alpha) was larger than 0.80 for all stations most of the time. AOD500nm averages increased from north to south during both polluted and non-polluted periods on the three urban sites in Beijing. The fine mode AOD during pollution periods is about a factor of 2.5 times larger than that during the non-pollution period at urban sites but a factor of 5.0 at suburban and rural sites. The fine mode fraction of AOD675nm was higher than 80% for all sites during January 2013. The absorption AOD675nm at rural sites was only about 0.01 during pollution periods, while 0.03-0.07 and 0.01-0.03 during pollution and non-pollution periods at other sites, respectively. Single scattering albedo varied between 0.87 and 0.95 during January 2013 over North China Plain. The size distribution showed an obvious tri-peak pattern during the most serious period. The fine mode effective radius in the pollution period was about 0.01-0.08 microns larger than during nonpollution periods, while the coarse mode radius in pollution periods was about 0.06-0.38 microns less than that during nonpollution periods. The total, fine and coarse mode particle volumes varied by about 0.06-0.34 cu microns, 0.03-0.23 cu microns, and 0.03-0.10 cu microns, respectively, throughout January 2013. During the most intense period (1-16 January), ARF at the surface exceeded −50W/sq m, −180W/sq m, and −200W/sq m at rural, suburban, and urban sites, respectively. The ARF readings at the top of the atmosphere were approximately −30W/sq m in rural and −40-60W/sq m in urban areas.

Atmosphere↗

NASA NTRS2017

North American Drought and Links to Northern Eurasia: The Role of Stationary Rossby Waves

This chapter provides an overview of the role of stationary Rossby waves in the sub-seasonal development of warm season drought over North America and subsequent downstream development of climate anomalies over northern Eurasia. The results are based on a case study of a stationary Rossby wave event that developed during 20 May 15 June 1988. Simulations with the NASA Goddard Earth Observing System (GEOS-5) atmospheric general circulation model highlight the importance of the mean jet streams in guiding and constraining the path and speed of wave energy propagation. In particular, convective anomalies that developed over the western Pacific in late May (in the presence of the strong North Pacific jet) produce a predilection for persistent upper-level high anomalies over central North America about ten days later, leading to the rapid development of severe dry conditions there. There are indications of continued downstream wave energy propagation that reaches northern Eurasia about two weeks later, leading to the development of dry conditions over eastern Europe and western Russia, and cool and wet conditions over western Europe and central northern Eurasia. The results suggest that stationary Rossby waves can serve as a source of predictability for sub-seasonal development of droughts over North America and northern Eurasia.

GEOS-5↗

NASA NTRS2018

Simulation and Prediction of Warm Season Drought in North America

This presentation presents our recent work on model simulation and prediction of warm season drought in North America. The emphasis will be on the contribution from the leading modes of subseasonal atmospheric circulation variability, which are often present in the form of stationary Rossby waves. Here we take advantage of the results from observations, reanalyses, and simulations and reforecasts performed using the NASA Goddard Earth Observing System (GEOS-5) atmospheric and coupled General Circulation Model (GCM). Our results show that stationary Rossby waves play a key role in Northern Hemisphere (NH) atmospheric circulation and surface meteorology variability on subseasonal timescales. In particular, such waves have been crucial to the development of recent short-term warm season heat waves and droughts over North America (e.g. the 1988, 1998, and 2012 summer droughts) and northern Eurasia (e.g., the 2003 summer heat wave over Europe and the 2010 summer drought and heat wave over Russia). Through an investigation of the physical processes by which these waves lead to the development of warm season drought in North America, it is further found that these waves can serve as a potential source of drought predictability. In order to properly represent their effect and exploit this source of predictability, a model needs to correctly simulate the Northern Hemisphere (NH) mean jet streams and be able to predict the sources of these waves. Given the NASA GEOS-5 AGCM deficiency in simulating the NH jet streams and tropical convection during boreal summer, an approach has been developed to artificially remove much of model mean biases, which leads to considerable improvement in model simulation and prediction of stationary Rossby waves and drought development in North America. Our study points to the need to identify key model biases that limit model simulation and prediction of regional climate extremes, and diagnose the origin of these biases so as to inform modeling group for model improvement.

Rossby Waves↗

NASA NTRS2018

Understanding the Water Cycle Above the North Polar Cap on Mars Using MRO CRISM Retrievals of Water Vapor

The north polar cap (NPC) on Mars is the major reservoir of atmospheric water (H2O) currently on Mars. The retrieval and monitoring of atmospheric water vapor abundance are crucial for tracking the cycle of water above the NPC. The Compact Reconnaissance Imaging Spectrometer for Mars (CRISM) aboard the Mars Reconnaissance Orbiter (MRO) has provided a wealth of data that extend over 5 + Martian years, covering the time period between 2006 and 2016. CRISM is ideally suited for spring and summer observations of the north polar region (latitudes poleward of 60 °N). The retrievals of water vapor column abundances over this extended period of time were performed over both ice-free and water ice covered surfaces, extending the coverage of the water vapor maps to include the permanent cap, where a maximum value of 90 precipitable micrometers (pr–µm) is retrieved, as compared to 60 pr–µm over ice-free regions in the North Polar Region. Away from summertime maximum, modest interannual variability in the water vapor abundance is observed. Zonal averages over all the observed Martian years combined show a developing water front that shifts northward towards summer, before dissipating over the permanent cap during mid-summer. A prominent feature at latitudes around 75 °N shows large abundances of water vapor, indicating a water vapor annulus encircling the retreating edge of the seasonal polar cap during late spring. Meridional transport of water modeled here show that the annulus may be a result of the convergence of water vapor from both south and north along the retreating edge of the NPC.

Khayat, Alain S. J.↗

NASA NTRS2019

Coupled Modes of North Atlantic Ocean Atmosphere Variability and the Onset of the Little Ice Age

Hydroclimate extremes in North America, Europe, and the Mediterranean are linked to ocean and atmospheric circulation anomalies in the Atlantic, but the limited length of the instrumental record prevents complete identification and characterization of these patterns of covariability especially at decadal to centennial timescales. Here we analyze the coupled patterns of drought variability on either side of the North Atlantic Ocean basin using independent climate field reconstructions spanning the last millennium in order to detect and attribute epochs of coherent basin-wide moisture anomalies to ocean and atmosphere processes. A leading mode of broad-scale moisture variability is characterized by distinct patterns of North Atlantic atmosphere circulation and sea surface temperatures. We infer a negative phase of the North Atlantic Oscillation and colder Atlantic sea surface temperatures in the middle of the 15th century, coincident with weaker solar irradiance and prior to strong volcanic forcing associated with the early Little Ice Age.

Kevin J Anchukaitis↗

NASA NTRS2020

The Boreal Winter El Niño Precipitation Response over North America: Insights into Why January is More Difficult to Predict than February

This study examines the within−season monthly variation of the El Niño response over North America during December−March using the NASA/GEOS model. In agreement with previous studies, the skill of 1−month lead GEOS coupled model forecasts of precipitation over North America is largest (smallest) for February (January), with similar results in uncoupled mode. A key finding is that the relatively poor January skillis the result ofthe model placing the main circulation anomaly over the northeast Pacific slightly to the west of the observed, resulting inprecipitation anomalies that lie off the coast instead of over land as observed. In contrast, during February the observed circulation anomaly over the northeast Pacific shifts westward, lining up with the predicted anomaly which is essentially unchanged from January, resulting in both the observed and predicted precipitation anomalies remaining off the coast. Furthermore, the largest precipitation anomalies occur along the southern tier of states associated with an eastward extended jet–something that the models capture reasonably well. Simulations with a stationary wave model indicate that the placement of January El Niño response to the west of the observed over the northeast Pacificis the result of biases in the January climatological stationary waves, rather than errors in the tropical Pacific El Niño heating anomalies in January. Furthermore, evidence is provided that the relatively poor simulation of the observed January climatology, characterized by a strengthened North Pacific jet and enhanced ridge over western North America, can be traced back to biases in the January climatology heating over the Tibet region and the tropical western Pacific.

Young-kwon Lim↗

NASA NTRSDate not supplied

An Ensemble Investigation of the Causes for Regional Air-Quality Model Critical Load Exceedances Prediction Variability in European and North American Domains Using Diagnostics From Phase 4 of the Air Quality Model Evaluation International Initiative

We summarize tentative findings from multi air quality model ensembles for the years 2009 and 2010 in Europe (EU), and 2010 and 2016 in North America (NA), under AQMEII-4. The model predictions of sulphur and nitrogen deposition were used to estimate exceedances of critical loads for acidification and eutrophication, to show the extent to which the ensemble members agree in the magnitude and the trend of ecologically meaningful impacts. Model exceedance variability was analyzed using AQMEII-4 diagnostics. Evaluation against concentration and wet deposition observations, coupled with these diagnostics, identified specific process representations as the causes for variability between model predictions and for reduced model performance. All models predicted reductions in ecosystem acidification impacts in North America between the years 2010 and 2016, in accord with SO2 emissions reduction legislation which started in 2010 (SO2 SIP) However, all models in EU and NA domains had net negative biases for wet deposition of sulphur and nitrogen relative to observations. The wet S deposition average mean bias for the NA ensemble was -0.17 eq ha-1 d-1, and for the EU ensemble -1.15 eq ha-1 d-1. The NA daily wet deposition average mean bias for NH4+ was -0.37 eq ha-1d-1; EU -1.19 eq ha-1 d-1. The daily NA wet NO3- deposition average mean bias was -0.24 eq ha-1d-1; EU -0.69 eq ha-1 d-1. The members of the ensemble diverged (factor of 10) in their North American predictions for Ndep and consequently their eutrophication exceedances. The models with the highest eutrophication predictions also predicted the highest levels of gas-phase ammonia dry deposition (standard deviation of ammonia dry deposition flux across ensemble members was larger than the ensemble average). These models also had negative biases of predicted ammonia concentrations; average mean biases of -0.63 (satellite NH3) and -0.85 ppbv (surface NH3) compared to ensemble averages of -0.30 and -0.34 ppbv. Diagnostics showed that these differences resulted from the manner in which bidirectional ammonia fluxes were parameterized within these models. The second largest source of NA eutrophication prediction variability were models with positive biases in particulate ammonium and nitrate concentrations, and higher particle nitrogen deposition levels ( particle ammonium concentration bias +0.35 ug m-3; ensemble bias +0.15 ug m-3). We believe two factors may have led to these latter overestimates: higher levels of fine mode particle nitrate formation compared to other models (due to the use of an inorganic heterogeneous chemistry algorithm which did not take base cation chemistry into account), and updates to particle dry deposition velocities carried out in the absence of concurrent updates to wet scavenging algorithms. The relative importance of dry gas, dry particulate, and wet deposition towards total sulphur and nitrogen deposition totals differed between EU and North American domains, though all models had negative biases in wet deposition as noted above. Parallel and subsequent work suggests that multiphase hydrometeor scavenging may improve model wet deposition performance. An increased research focus is recommended for four model processes: multiphase hydrometeor scavenging, ammonia bidirectional fluxes, base cation chemistry and emissions, and particle dry deposition.

regional air-quality model↗