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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 91 records · Page 5
All sourcesNASA NTRSDOE OSTI
DOE OSTI2017

Noble metal free photocatalytic H 2 generation on black TiO 2 : On the influence of crystal facets vs. crystal damage

In this study, we investigate noble metal free photocatalytic water splitting on natural anatase single crystal facets and on wafer slices of the [001] plane before and after these surfaces have been modified by high pressure hydrogenation and hydrogen ion-implantation. Here, we find that on the natural, intact low index planes, photocatalytic H 2 evolution (in the absence of a noble metal co-catalyst) can only be achieved when the hydrogenation treatment is accompanied by the introduction of crystal damage, such as simple scratching and miscut in the crystal, or by implantation damage. X-ray reflectivity, Raman, and optical reflection measurements show that plain hydrogenation leads to a ≈ 1 nm thick black titania surface layer without activity, while a colorless, density modified, and ≈7 nm thick layer with broken crystal symmetry is present on the ion implanted surface. These results demonstrate that (i) the H-treatment of an intact anatase surface needs to be combined with defect formation for catalytic activation and (ii) activation does not necessarily coincide with the presence of black color.

36 MATERIALS SCIENCE↗
DOE OSTI2017

Ab initio studies of structural, electronic, optical, elastic and thermal properties of CuGaTe{sub 2}

We have performed ab initio calculations for the structural, electronic, optical, elastic and thermal properties of CuGaTe{sub 2}. In this study, we used an accurate full potential linearized augmented plane wave (FP-LAPW) method to find the equilibrium structural parameters and to compute the full elastic tensors. We report electronic and optical properties with the recently developed density functional of Tran and Blaha. Furthermore, optical features such as dielectric functions, refractive indices, extinction coefficient, optical reflectivity, absorption coefficients, optical conductivities, were calculated for photon energies up to 30 eV. The thermodynamical properties such as Debye temperature, entropy and Gruneisen parameter, bulk modulus and hardness were calculated employing the quasi-harmonic Debye model at different temperatures (0–1000 K) and pressures (0–8 GPa) and the silent results were interpreted. Most of the investigated parameters are reported for the first time.

36 MATERIALS SCIENCE↗
DOE OSTI2015

Preablation electron and lattice dynamics on the silicon surface excited by a femtosecond laser pulse

The study of the time-resolved optical reflection from the silicon surface excited by single femtosecond laser pulses below and near the melting threshold reveals fast (less than 10 ps) Auger recombination of a photogenerated electron–hole plasma with simultaneous energy transfer to the lattice. The acoustic relaxation of the excited surface layer indicates (according to reported data) a characteristic depth of 150 nm of the introduction of the laser radiation energy, which is related to direct linear laser radiation absorption in the photoexcited material due to a decrease in the energy bandgap. The surface temperature, which is probed at a time delay of about 100 ps from the reflection thermomodulation of probe radiation and the integrated continuous thermal emission from the surface, increases with the laser fluence and, thus, favors a nonlinear increase in the fluorescence of sublimated silicon atoms. The surface temperature estimated near the picosecond melting threshold demonstrates a substantial (20%) overheating of the material with respect to the equilibrium melting temperature. Above the melting threshold, the delay of formation of the material melt decreases rapidly (from several tens of picoseconds to several fractions of a picosecond) when the laser fluence and, correspondingly, the surface temperature increase. In the times of acoustic relaxation of the absorbing layer and even later, the time modulation of the optical reflectivity of the material demonstrates acoustic reverberations with an increasing period, which are related to the formation of melt nuclei in the material.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2016

Transparency of the strong shock-compressed diamond for 532 nm laser light

An optical reflectivity and transmissivity model for the shock-compressed diamond is established and used to calculate the optical reflectivity and transmissivity of the diamond under different shock compressions. The simulated results indicate that the reflection occurs at the shock front and does not depend on the thickness of the compressed diamond, but the transmissivity decreases with the thickness. The simulated reflectivity is consistent with the experimental results in the literature, which validates the model. It is shown that the diamond keeps transparent when the shock pressure is lower than 2.00 Mbar, and becomes opaque but does not reflect the probe laser as the shock pressure increases from 2.00 Mbar to 4.60 Mbar and reflects the probe laser markedly when the shock pressure is higher than 4.60 Mbar.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2019

Dynamic power and chirp measurements of amplified 19 ps pulses in traveling-wave and reflective semiconductor optical amplifiers using a linear pulse characterization technique

The dynamic chirp and power of amplified pulses in semiconductor optical amplifiers is of importance in the application of these devices as conventional amplifiers and in optical signal processing. Non-linear measurement techniques are appropriate for pulsewidths less than 5 ps but have low sensitivity for wider pulsewidths commonly present in moderate bit rate optical systems. Typical measurements of chirp and power of 20 GHz repetition rate amplified 19 ps pulsewidth pulses in traveling-wave and reflective SOAs are obtained using a linear characterization technique based on small-signal sinusoidal modulation at half the pulse stream repetition rate and post-processing of the resulting optical spectrums. The results show that the amplified pulse dynamic power and chirp can have a complex structure and thereby pulse spectrum, which in turn can influence pulse propagation in optical fiber.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2016

HYBRID simulations of diffraction-limited focusing with Kirkpatrick-Baez mirrors for a next-generation In Situ hard X-ray nanoprobe

Next-generation hard X-ray nanoprobe beamlines such as the In Situ Nanoprobe (ISN) beamline being planned at the Advanced Photon Source aim at providing very high spatial resolution while also enabling very high focused flux, to study complex materials and devices using fast, multidimensional imaging across many length scales. The ISN will use diffractive optics to focus X-rays with a bandpass of ΔE/E = 10 –4 into a focal spot of 20 nm or below. Reflective optics in Kirkpatrick-Baez geometry will be used to focus X-rays with a bandpass as large as ΔE/E = 10 –2 into a focal spot of 50 nm. Diffraction-limited focusing with reflective optics is achieved by spatial filtering and use of a very long, vertically focusing mirror. Furthermore, to quantify the performance of the ISN beamline, we have simulated the propagation of both partially and fully coherent wavefronts from the undulator source, through the ISN beamline and into the mirror-based focal spot. Simulations were carried out using the recently developed software “HYBRID.”

43 PARTICLE ACCELERATORS↗
NASA NTRS1998

Holographic Airborne Rotating Lidar Instrument Experiment (HARLIE)

Scanning holographic lidar receivers are currently in use in two operational lidar systems, PHASERS (Prototype Holographic Atmospheric Scanner for Environmental Remote Sensing) and now HARLIE (Holographic Airborne Rotating Lidar Instrument Experiment). These systems are based on volume phase holograms made in dichromated gelatin (DCG) sandwiched between 2 layers of high quality float glass. They have demonstrated the practical application of this technology to compact scanning lidar systems at 532 and 1064 nm wavelengths, the ability to withstand moderately high laser power and energy loading, sufficient optical quality for most direct detection systems, overall efficiencies rivaling conventional receivers, and the stability to last several years under typical lidar system environments. Their size and weight are approximately half of similar performing scanning systems using reflective optics. The cost of holographic systems will eventually be lower than the reflective optical systems depending on their degree of commercialization. There are a number of applications that require or can greatly benefit from a scanning capability. Several of these are airborne systems, which either use focal plane scanning, as in the Laser Vegetation Imaging System or use primary aperture scanning, as in the Airborne Oceanographic Lidar or the Large Aperture Scanning Airborne Lidar. The latter class requires a large clear aperture opening or window in the aircraft. This type of system can greatly benefit from the use of scanning transmission holograms of the HARLIE type because the clear aperture required is only about 25% larger than the collecting aperture as opposed to 200-300% larger for scan angles of 45 degrees off nadir.

Schwemmer, Geary K.↗
DOE OSTI2019

Breakdown of Fermi Degeneracy in the Simplest Liquid Metal

We are reporting the observation of the breakdown of electrons’ degeneracy and emergence of classical statistics in the simplest element: metallic deuterium. We have studied the optical reflectance, shock velocity and temperature of dynamically compressed liquid deuterium up to its Fermi temperature, TF. Above the insulator–metal transition, the optical reflectance shows the distinctive temperature-independent resistivity saturation, which is prescribed by the Mott-Ioffe-Regel minimum metallic limit, in agreement with previous experiments. At T > 0.4 T F , however, the reflectance of metallic deuterium starts to rise with a temperature-dependent slope, consistent with the breakdown of the Fermi surface. The experimentally inferred collisional time in this region exhibits the characteristic temperature dependence expected for a classical Landau-Spitzer plasma. Our observation of electron degeneracy lifting extends studies of degeneracy to new fermionic species, electron Fermi systems and offers an invaluable benchmark for quantum statistical models of Coulomb systems over a wide range of temperatures relevant to dense astrophysical objects and ignition physics.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
NASA NTRS2015

Solar Lyman-Alpha Polarization Observation of the Chromosphere and Transition Region by the Sounding Rocket Experiment CLASP

We are planning an international rocket experiment Chromospheric Lyman-Alpha Spectro-Polarimeter (CLASP) is (2015 planned) that Lyman α line (Ly(alpha) line) polarization spectroscopic observations from the sun. The purpose of this experiment, detected with high accuracy of the linear polarization of the Ly(alpha) lines to 0.1% by using a Hanle effect is to measure the magnetic field of the chromosphere-transition layer directly. For polarization photometric accuracy achieved that approx. 0.1% required for CLASP, it is necessary to realize the monitoring device with a high throughput. On the other hand, Ly(alpha) line (vacuum ultraviolet rays) have a sensitive characteristics that is absorbed by the material. We therefore set the optical system of the reflection system (transmission only the wavelength plate), each of the mirrors, subjected to high efficiency of the multilayer coating in accordance with the role. Primary mirror diameter of CLASP is about 30 cm, the amount of heat about 30,000 J is about 5 minutes of observation time is coming mainly in the visible light to the telescope. In addition, total flux of the sun visible light overwhelmingly large and about 200 000 times the Ly(alpha) line wavelength region. Therefore, in terms of thermal management and 0.1% of the photometric measurement accuracy achieved telescope, elimination of the visible light is essential. We therefore, has a high reflectivity (> 50%) in Lyα line, visible light is a multilayer coating be kept to a low reflectance (<5%) (cold mirror coating) was applied to the primary mirror. On the other hand, the efficiency of the polarization analyzer required chromospheric magnetic field measurement (the amount of light) Conventional (magnesium fluoride has long been known as a material for vacuum ultraviolet (MgF2) manufactured ellipsometer; Rs = 22%) about increased to 2.5 times were high efficiency reflective polarizing element analysis. This device, Bridou et al. (2011) is proposed "that is coated with a thin film of the substrate MgF2 and SiO2 fused silica." As a result of the measurement, Rs = 54.5%, to achieve a Rp = 0.3%, high efficiency, of course, capable of taking out only about s-polarized light. Other reflective optical elements (the secondary mirror, the diffraction gratingcollector mirror), subjected to high-reflection coating of Al + MgF2 (reflectance of about 80%), less than 5% in the entire optical system by these (CCD Science was achieved a high throughput as a device for a vacuum ultraviolet ray of the entire system less than 5% (CCD of QE is not included).

Narukage, Noriyuki↗
NASA NTRS1991

Displacement response, detection limit, and dynamic range of fiber-optic lever sensors

The authors present the evaluation of the displacement response, detection limit, and dynamic range of fiber-optic lever sensors in a general format to establish their dependence on fiber sizes, optoelectronic detector specifications, input power, and other relevant parameters. The formations for the normalized reflected optical power change are derived for the evaluation of the optimal sensor response, the linearity range, and the minimum detectable displacement. The theoretical models are verified by an experiment which determines sensor response, modulation index, reflected optical power change, and linear response range through dynamic measurement. The application of this theoretical model to the study of a fiber-optic microphone for acoustic pressure detection is considered.

He, Gang↗
DOE OSTI2018

Plasmon-Excitonic Polaritons in Metal-Semiconductor Nanostructures with Quantum Wells

A theory of plasmon-exciton coupling and its spectroscopy is developed for metal-semiconductor nanostructures. Considered as a model is a periodic superlattice with cells consisting of a quantum well and a layer of metal nanoparticles. The problem is solved self-consistently using the electrodynamic Green’s functions taking account of resonant polarization. Coulomb plasmon-exciton interaction is associated with the dipole surface plasmons of particles and their image charges due to excitonic polarization of neighboring quantum well. Optical reflection spectra are numerically investigated for superlattices with GaAs/AlGaAs quantum wells and silver nanoparticles. Superradiant regime caused by one-dimensional Bragg diffraction is studied for plasmonic, excitonic and plasmon-excitonic polaritons depending on the number of supercells. The plasmon-excitonic Rabi splitting is shown to occur in reflectivity spectra of resonant Bragg structures.

36 MATERIALS SCIENCE↗
NASA NTRSDate not supplied

Characterization of Novel Spacecraft Materials aboard the Materials International Space Station Experiment-Flight Facility (Preliminary Results)

This work will encompass the preflight characterization of 15 novel and heritage materials currently under observation on the Materials International Space Station Experiment-Flight Facility (MISSE-FF). MISSE-FF has been upgraded to perform active reflectance measurements of the materials. Images taken in RGB/IR colors are compared to results from an extensive ground testing campaign to obtain quantitative on-orbit material evolution data. Identical materials samples are to be flown on the ram, wake, and zenith faces of MISSE-FF, enabling deconvolution of the energetic electron, proton, atomic oxygen, and ultraviolet damage pathways. Energy deposition from the space environment leads to chemical changes in the material that in turn alter the optical properties. The same chemical damage that manifests as changes in optical reflectance and absorptance also leads to changes in myriad physical properties such as mechanical strength, electrical conductivity, and chemical reactivity. Therefore, flight materials are able to be characterized based on their unique reflectance spectra by comparing on-orbit measurements of optical reflectance with extensive terrestrial experiments, which help to correlate changes in reflectance with respect to changes in other material properties. The MISSE program has been a part of the International Space Station National Laboratory for many years and has been instrumental in understanding space weather modification of material properties. However, MISSE-FF has been limited to passive experiments with only pre/post flight material studies possible. In advance of the MISSE-16 experiment, the flight facility has received a major upgrade to provide daily spectral observations by way of a RGB/IR camera and a tunable light source. The MISSE-16 mission launched in February 2022 and carries 15 material samples for 6 months of the low Earth orbital exposure. Identical materials samples are to be flown on the ram, wake, and zenith faces of MISSE-FF, enabling deconvolution of the energetic electron, proton, atomic oxygen, and ultraviolet damage pathways. This paper discusses the MISSE-16 experiment, highlights the first use of the facility upgrades, and presents results from the extensive preflight material characterization that includes directional hemispherical reflectance, bidirectional reflectance, AFM, SEM, and electrical conductivity. Additionally, data showing the modification of these properties by ground-based exposure to space-like electron and atomic oxygen flux will be discussed. Finally, updates on deployment and initial check-out of the experiment on MISSE-FF will be presented. It is the ultimate goal of this program to provide validation for the development of ground based space weather simulation facilities and techniques.

Ryan Hoffman↗
NASA NTRS1992

Geometric-optical bidirectional reflectance modeling of the discrete crown vegetation canopy - Effect of crown shape and mutual shadowing

Many natural vegetation covers can be regarded as assemblages of plant crowns, on a background, which interact with light as discrete objects. On this basis, geometric optics furnish an approach to the modeling of vegetation canopies that captures the most important features of such growths' bidirectional measurements. Attention is presently given to models which approximate these phenomena and relate the size, shape, and count density of plant crowns to viewing and illumination positions and to crown-background reflectance contrasts.

Li, Xiaowen↗
DOE OSTI2018

Reflection Spectra of Microarrays of Silicon Nanopillars

The optical-reflection spectra of microarrays of silicon nanopillars are studied in the visible and near-IR regions. The microarrays of silicon nanopillars are formed by electron-beam lithography and reactive ion etching. The reflection spectra of nanopillar arrays with pitches of 400, 600, 800, and 1000 nm are measured. The height of nanopillars in the array is 0.5 μm, and the diameter varies from 150 to 240 nm. It is noted that the spectral features of the reflection are caused by increased absorption of individual nanopillars and interference effects inside the array. A relation between the geometric parameters of nanopillars and the resonance reflection characteristics is determined taking into account the influence of the substrate.

77 NANOSCIENCE AND NANOTECHNOLOGY↗
NASA NTRS1989

Experimental results of a high Q quasioptical reflection cavity

A quasi-optical reflection cavity intended to be used as the resonant load of a submillimeter wavelength oscillator has been designed, constructed, and tested. The resonator consists of three elements in cascade: a high Q, high finesse folded Fabry-Perot resonator, a lower Q, low finesse Fabry-Perot resonator, and a Littrow mounted diffraction grating. The resonator exhibits a Q of 6600 and 2.5 dB of loss at 63 GHz. The design can be scaled to 1 THz, where waveguide structures become impractical, to serve as the resonator for high frequency quantum well resonant tunneling device oscillators.

Lee, Karen A.↗
DOE OSTI2019

Simultaneous scanning near-field optical and X-ray diffraction microscopy for correlative nanoscale structure-property characterization

A multimodal imaging instrument has been developed that integrates scanning near-field optical microscopy with nanofocused synchrotron X-ray diffraction imaging. The instrument allows for the simultaneous nanoscale characterization of electronic/near-field optical properties of materials together with their crystallographic structure, facilitating the investigation of local structure–property relationships. The design, implementation and operating procedures of this instrument are reported. The scientific capabilities are demonstrated in a proof-of-principle study of the insulator–metal phase transition in samarium sulfide (SmS) single crystals induced by applying mechanical pressure via a scanning tip. The multimodal imaging of an in situ tip-written region shows that the near-field optical reflectivity can be correlated with the heterogeneously transformed structure of the near-surface region of the crystal.

insulator–metal transitions↗
NASA NTRS2001

A Multi-Band Analytical Algorithm for Deriving Absorption and Backscattering Coefficients from Remote-Sensing Reflectance of Optically Deep Waters

A multi-band analytical (MBA) algorithm is developed to retrieve absorption and backscattering coefficients for optically deep waters, which can be applied to data from past and current satellite sensors, as well as data from hyperspectral sensors. This MBA algorithm applies a remote-sensing reflectance model derived from the Radiative Transfer Equation, and values of absorption and backscattering coefficients are analytically calculated from values of remote-sensing reflectance. There are only limited empirical relationships involved in the algorithm, which implies that this MBA algorithm could be applied to a wide dynamic range of waters. Applying the algorithm to a simulated non-"Case 1" data set, which has no relation to the development of the algorithm, the percentage error for the total absorption coefficient at 440 nm a (sub 440) is approximately 12% for a range of 0.012 - 2.1 per meter (approximately 6% for a (sub 440) less than approximately 0.3 per meter), while a traditional band-ratio approach returns a percentage error of approximately 30%. Applying it to a field data set ranging from 0.025 to 2.0 per meter, the result for a (sub 440) is very close to that using a full spectrum optimization technique (9.6% difference). Compared to the optimization approach, the MBA algorithm cuts the computation time dramatically with only a small sacrifice in accuracy, making it suitable for processing large data sets such as satellite images. Significant improvements over empirical algorithms have also been achieved in retrieving the optical properties of optically deep waters.

Lee, Zhong-Ping↗
DOE OSTI2016

Summary Report: NMSBA CY 2016 - AEgis Technologies Group Inc. #12458.

AEgis requires large area partial mirror optics consisting of partially reflecting optical coatings on large dimension substrates for high energy laser (HEL) applications. The partial mirrors should transmit nearly the same small fraction of HEL radiation incident from a wide range of angles of incidence (AOIs), and the laser-induced damage threshold (LIDT) of the coatings should be high enough for them to be able to withstand direct exposure to near infrared CW HEL radiation at multi-kilowatt/cm2 power levels. The transmitted fraction of incident HEL radiation should reach an array of detectors at power levels high enough for reliable detection but low enough to not damage the detectors. The reflected fraction of incident HEL radiation should scatter into a divergent pattern so as to be eye safe at a distance of ~ 200 m from the mirror in the case of 100 kilowatt incident laser power. The detector array together with the partial mirror optic and possible additional optics that provide divergent scattering of reflected HEL radiation constitute what AEgis refers to as a target board. The target board use environment may vary from benign, indoor laboratory conditions to harsh, outdoor conditions in tests on the ground as well as in air. Under this NMSBA project, Sandia agreed to apply its extensive expertise and capability in the design and production of high LIDT coatings on large dimension optics for high power pulsed laser radiation to advise and assist AEgis in the design and development of high LIDT coatings for the partial mirror optic. Sandia and AEgis met several times to discuss the partial mirror and target board requirements, and Sandia was guided in its work by these discussions as well as by the partial mirror and target board requirement summaries of Tables 1 and 2, respectively, that were provided by AEgis.

47 OTHER INSTRUMENTATION↗