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ORNL Package Testing Program Software Quality Assurance Plan

The Oak Ridge National Laboratory (ORNL) Package Testing Program (PTP) uses commercial off-the-shelf (COTS) software in performing data collection of thermal test results for package designs that contain radioactive materials. Specifically, this software is used to collect temperature data from the furnace, packages, and ambient air to prepare and execute the thermal test specified in 10 CFR 71.73, “Thermal Test.” This software quality assurance (SQA) plan sets forth the guidelines, standards, and procedures that shall be used to provide SQA for PTP software applications. This is a living document that will be maintained for the lifecycle of the PTP program. The SQA plan follows the requirements set forth in ORNL Standards Based Management System (SBMS): Information Technology; Subject Area: Software Quality Assurance. When applicable to the requirements as described in ORNL SBMS, Software Quality Assurance, the software shall be listed in the ORNL Software Registration System (SRS). Exemptions to this SBMS are COTS and firmware that are not modified; spreadsheet applications and personal productivity tools that do not have a utility or safety application, research applications, legacy software, system software, vendor-supplied software used to interface with the vendor’s services, software used within the organization to facilitate processing or management of information, and software developed for applications not specific to the US Department of Energy (DOE).

97 MATHEMATICS AND COMPUTING

PNNL-Sequim Campus Radionuclide Air Emissions Report for Calendar Year 2024

The U.S. Department of Energy Office of Science’s Pacific Northwest Site Office has oversight and stewardship duties associated with the Pacific Northwest National Laboratory (PNNL) Sequim campus. Facility operations include radiological operations with the potential to emit low levels of radioactive materials.

54 ENVIRONMENTAL SCIENCES

Test Report for the Regulatory Testing of the Welded Isotek-SFC-W-3 Special Form Capsule

Two prototypes the welded ISOTEK-SFC-W-3 special form capsules (SFCs) of the same design were evaluated to determine if the requirements of Title 49, Code of Federal Regulations (CFR), Part 173.469, Tests for Special Form Class 7 (Radioactive) Materials, were met. The results of the special form tests are documented in this test report. This report describes the special form testing activities performed on the two welded ISOTEK-SFC-W-3 capsules. The test units were designated as TU-1 and TU-2. TU-1 was subjected to leak testing, percussion testing, and impact testing. TU-1 was leak tested using the leak rate test specified in 49 CFR 173.469(a)(4)(i). The impact test on TU-1 was conducted according to the requirements in 49 CFR 173.469 (b)(1). The percussion test that was carried out on TU-1 was conducted in accordance with 49 CFR 173.469 (b)(2). TU-2 was subjected to a leak rate test as specified in 173.469(a)(4)(i) and a heat test as specified in 49 CFR 173.469(b)(4). Each test unit was leak tested before and after these respective tests. The leak rate tests performed were helium back-pressure tests and bubble tests, as specified in American National Standards Institute (ANSI) N14.5-2014. The measured leak rates were converted to standard condition leak rates as specified in American Society for Testing and Measurement (ASTM) E 493. The determined standardized leak rates obtained from the test and the calculations for all the test units met the requirements for special form certification. The testing was performed under the direction of the Oak Ridge National Laboratory (ORNL) Package Testing Program (PTP).

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS

Evaluation of Cease Fire CFP 640 for Use in Gloveboxes (Final Report)

A Los Alamos National Laboratory (LANL) task group was established to discuss and evaluate a candidate fire suppression system (FSS) for gloveboxes (GB) and dropboxes (DB, for brevity, this report will simply refer to gloveboxes). Suitability criteria include compliance, compatibility, and capability. LANL contracted with New Mexico Tech (NMT) to quantitatively evaluate the perfor mance of one of those systems including its ability to extinguish GB fires, limit over-pressurization of the GB, etc. Additionally, the results of these experiments provide data points that could be used when fire hazard evaluations (FHEs) are conducted for determining when to require a fire suppres sion system installation within a GB (as required by NFPA 801, Standard for Facilities Handling Radioactive Materials, DOE Standard 1066-2012 Fire Protection, and AGS-G010-2011 Standard of Practice for Glovebox Fire Protection).

42 ENGINEERING

Progress on the US-Japan Source Term Benchmark Analysis Collaboration

There has been a resurgence in global interest in advanced reactor technology, with a variety of innovative concepts being proposed and developed. Sodium-cooled Fast Reactors (SFRs) have garnered considerable attention given their beneficial characteristics and extensive historical development programs and operating experience. Central to the licensing of non-light water reactor (non-LWR) technology is the characterization of the safety case. At its basics, reactor safety focuses on the prevention and mitigation of the release of radioactive material to the environment.

22 GENERAL STUDIES OF NUCLEAR REACTORS

Automated Systems for Solvent Extraction

An automated solvent extraction system for the eventual handling of radioactive materials has been designed and procured for rapid, efficient and safe liquid-liquid extraction processes. This system will be configured to carry out liquid-liquid separations from beginning to end, automating tedious and time-consuming tasks such as organic/aqueous phase prep, pH checks, phase separation, and metal ion analysis. The system features advanced liquid handling capabilities, a robotic arm for precise sample transfer, and sophisticated analytical tools including UV-VIS spectrophotometry for real-time monitoring. Additionally, it incorporates automated capping of vials, vortex mixing, and centrifugation to ensure thorough mixing and phase separation. This report provides an overview of the system and general capabilities as well as initial efforts to develop an automated workflow for liquid-liquid separations.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA

In-Plane Liftout and Push-to-Pull for In Situ Mechanical Testing of Irradiated Inconel X-750

A streamlined sample preparation method for nanomechanical testing is needed to improve the quality of specimens, reduce the cost, and increase the versatility of specimen fabrication. This work outlines an in-plane liftout focused ion beam (FIB) fabrication procedure to prepare electron-transparent specimens for in situ transmission electron microscopy (TEM) nanomechanical testing. Ion etching and electron backscatter diffraction (EBSD) techniques were used to lift out a [110] oriented grain from a neutron-irradiated bulk X-750 alloy. Careful control of voltages and currents ensured precision. Top surface thinning sweeps prevented resurfacing and redeposition while dog-bone geometries were shaped with a 1:4 gauge width-to-milling pattern diameter ratio. Nanotensile testing in the TEM with a picoindenter allowed for the estimation of an ultimate tensile strength of 2.41 GPa, and inspection revealed a high density of bubbles in the X-750 matrix. The proposed fabrication procedure is significant for preparing samples from radioactive materials, studying complex structures that are orientation-dependent, and analyzing desired planar areas.

36 MATERIALS SCIENCE

Radiological safety handbook

Radiation hazard handbook supplement - persons exposed to ionizing radiation or radioactive materials

RADIATION HAZARD

Safe atmosphere entry of an isotope heat source with a single stable trim attitude at hypersonic speeds

A theoretical investigation has been made to design an isotope heat source capable of satisfying the conflicting thermal requirements of steady-state operation and atmosphere entry. The isotope heat source must transfer heat efficiently to a heat exchange during normal operation with a power system in space, and in the event of a mission abort, it must survive the thermal environment of atmosphere entry and ground impact without releasing radioactive material. A successful design requires a compatible integration of the internal components of the heat source with the external aerodynamic shape. To this end, configurational, aerodynamic, motion, and thermal analyses were coupled and iterated during atmosphere entries at suborbital through superorbital velocities at very shallow and very steep entry angles. Results indicate that both thermal requirements can be satisfied by a heat source which has a single stable aerodynamic orientation at hypersonic speeds. For such a design, the insulation material required to adequately protect the isotope fuel from entry heating need extend only half way around the fuel capsule on the aerodynamically stable (wind-ward) side of the heat source. Thus, a low-thermal-resistance, conducting heat path is provided on the opposite side of the heat source through which heat can be transferred to an adjacent heat exchanger during normal operation without exceeding specified temperature limits.

Levy, L. L., Jr.

Approximations for neutron emission spectra from proton collisions between 20 and 500 MeV on nuclei of A greater than or equal to 12

When high energy protons from solar proton events or trapped radiation belts impinge on spacecraft structures, secondary particles are emitted. The most pernicious secondaries, from either a biological or physical standpoint, are the cascade and evaporation neutrons because of their reaction with matter leading to radioactive materials in the spacecraft structures. Empirically determined cascade and evaporation neutron emission spectra for protons of energy between 20 and 500 MeV incident on all materials at or above carbon in mass number are presented.

Burrell, M. O.

The Satellite Nuclear Power Station - An option for future power generation.

A new concept in nuclear power generation is being explored which essentially eliminates major objections to nuclear power. The Satellite Nuclear Power Station, remotely operated in synchronous orbit, would transmit power safely to the ground by a microwave beam. Fuel reprocessing would take place in space and no radioactive materials would ever be returned to earth. Even the worst possible accident to such a plant should have negligible effect on the earth. An exploratory study of a satellite nuclear power station to provide 10,000 MWe to the earth has shown that the system could weigh about 20 million pounds and cost less than $1000/KWe. An advanced breeder reactor operating with an MHD power cycle could achieve an efficiency of about 50% with a 1100 K radiator temperature. If a hydrogen moderated gas core reactor is used, its breeding ratio of 1.10 would result in a fuel doubling time of a few years. A rotating fluidized bed or NERVA type reactor might also be used. The efficiency of power transmission from synchronous orbit would range from 70% to 80%.

Williams, J. R.

Introduction

The accomplishments of the Apollo 17 flight are briefly described. The characteristics of the Taurus-Littrow region landing site are analyzed. The experiments conducted to analyze the composition of the lunar surface are reported. The extent to which the results of the Apollo 17 experiments confirmed theories concerning lunar seismology, thermal characteristics, presence of radioactive materials, and origin of the moon is developed.

Calio, A. J.

Satellite nuclear power station: An engineering analysis

A nuclear-MHD power plant system which uses a compact non-breeder reactor to produce power in the multimegawatt range is analyzed. It is shown that, operated in synchronous orbit, the plant would transmit power safely to the ground by a microwave beam. Fuel reprocessing would take place in space, and no radioactive material would be returned to earth. Even the effect of a disastrous accident would have negligible effect on earth. A hydrogen moderated gas core reactor, or a colloid-core, or NERVA type reactor could also be used. The system is shown to approach closely the ideal of economical power without pollution.

Williams, J. R.

Dynamo generation in Mercury

Models of the interior and thermal evolution of Mercury calculated by Siegfried and Solomon (1974) using Lewis' (1972) cosmochemical calculations to constrain the composition are tested for four necessary conditions for MHD dynamo generation. It is shown that dynamo generation requires at least a partially fluid interior, an energy source that drives a flow of core fluid relative to the rigidly rotating planet, a magnetic-field diffusion time in excess of the characteristic fluid-flow time scale, and a fluid flow of sufficient complexity to satisfy Cowling's (1934) theorem. It is concluded that a literal interpretation of Lewis' calculations implies that dynamo generation in Mercury is improbable. Generation would be possible only if the metallic core were contaminated with substantial amounts of radioactive material.

Stevenson, D. J.

Release of radiogenic gases from the moon

The rate of escape of Ar-40 from the moon is calculated from mass-spectrometer data obtained at the Apollo-17 landing site. It is shown that the rate of loss of Ar from the moon varies significantly over periods the order of one lunation and that the average loss rate is about 3 t/a, corresponding to about 6% of the present rate of Ar production by K decay within the moon. These features of the Ar loss-rate data are interpreted as evidence that this gas originates in the partially molten asthenosphere, which in turn requires that early differentiation only affected the outer 600 to 1,000 km of the moon, trapping significant amounts of radioactive materials in the present asthenosphere. The relationship between the venting of Ar and other radiogenic gases in the lunar atmosphere is discussed.

Hodges, R. R., Jr.