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Electron temperature dependence of molecular neon ions recombination with electrons using microwave afterglow/mass spectrometer, obtaining recombination coefficient
D region electron density rocket measurements implying recombination coefficient
Lower E region recombination coefficients from electron density and flux measurements in glow aurora by Nike-Apache rocket
The growth over sunrise of the C and D layers of the ionosphere is investigated. The model which is analyzed includes the negative ion species O(-), O2(-), O3(-), O4(-), NO3(-), CO3(-), and CO4(-). Ionization sources due to galactic cosmic rays, precipitated electrons, ionization of NO by scattered Lyman alpha radiation, and the direct solar radiation ionization are also included. The photodetachment of most of the negative ions is discussed, as well as the time variation of these parameters. The time variations of the electron, negative ion, and positive ion densities are calculated over sunrise. From these data, the mesospheric C and D layer development is plotted. Several model parameters are varied until the best agreement with experimentally determined electron densities is obtained. The results are discussed in light of several atmospheric parameters including the O and NO concentrations and the electron-ion recombination coefficient.
Recombination coefficients of electrons with ions of the hydrated hydronium ion series (H3O(+))(H2O)n, where n = 0, 1, 2, 3, 4, 5, 6, were determined with a microwave afterglow/mass spectrometer apparatus. Afterglow measurements of electron density decays in helium-water vapor mixtures are correlated with the decay of mass-identified ion currents to the wall of the microwave cavity. By varying the temperature of the gas and the partial pressure of the water vapor in the mixture, different groups of hydronium series ions are made to dominate the afterglow.
Demonstration that, during the process of dielectronic recombination, the energy of a recombined ion after a resonance capture and subsequent stabilization may still be higher than the first ionization limit. If that happens, a secondary autoionization can take place and reduce the recombination coefficient. The importance of this effect is considered for iron ions Fe(9+) to Fe(13+).
Semi-empirical potentials are constructed that have eigenvalues close in magnitude to the binding energies of the valence electron in lithium. The potentials include the long range polarization force between the electron and the core. The corresponding eigenfunctions are used to calculate dynamic polarizabilities, discrete oscillator strengths, photoionization cross sections and radiative recombination coefficients. A consistent application of the theory imposes a modification on the transition operator, but its effects are small for lithium. The method presented can be regarded as a numerical generalization of the widely used Coulomb approximation.
A theoretical and experimental demonstration is presented which shows that under suitable conditions the volume recombination coefficient can be determined by measuring the heat transfer rate into the wall of a cylinder through which a dissociated stream is passing. The experimental results obtained are in agreement with those of other investigators.
Microwave discharge plasmas take place within heated zone. Changes in weight of specimens in plasma as well as temperature of sample and plasma can be obtained, facilitating determinations of reaction rates and recombination coefficients.
An apparatus is described which is used for the controlled production, characterization, and study of dissociated gases in a microwave discharge at elevated temperatures. A unique feature is the ability to produce and study a microwave discharge plasma in the heated zone. This allows elevated temperature reactions to be studied in high concentrations of dissociated gases. Further, the system permits weight change measurements of specimens in the plasma, thus facilitating reaction rate determinations. Included is a description of a cavity for use on a 50-mm diameter cylindrical reactor. The effects of flow rate, pressure, temperature, power, metal sample, and sampling position on dissociation percentage of oxygen in the apparatus are described as well as a technique for sample temperature measurements in the plasma which permits determination of high temperature recombination coefficients and reaction rates.
Results of the study of Chatanika incoherent scatter radar data and Lockheed Palo Alto Research Laboratory satellite data are reported. Specific topics covered include: determination of the effective recombination coefficient in the auroral E region; determination of the location of the auroral oval; auroral boundary characteristics; and the relationship of auroral current systems, particle precipitation, visual aurora, and radar aurora.
Low latitude middle atmosphere ionization was studied with data obtained from three blunt conductivity probes and one Gerdien condenser. An investigation was conducted into the effects of various ionization sources in the 40 to 65 Km altitude range. An observed enhancement of positive ion conductivity taking place during the night can be explained by an atmsopheric effect, with cosmic rays being the only source of ionization only if the ion-ion recombination coefficient (alpha sub i) is small(10 to the -7 power cu cm/s) and varies greatly with altitude. More generally accepted values of alpha sub i ( approximately equal to 3x10 to the -7 power cu cm/s) require an additional source of ionization peaking at about 65 Km, and corresponding approximately to the integrated effect of an X-ray flux measured on a rocket flown in conjunction with the ionization measurements. The reasonable assumption of an alpha sub i which does not vary with altitude in the 50-70 Km range implies an even greater value alpha sub i and a more intense and harder X-ray spectrum.
Electron density measurements made with the partial reflections technique above Urbana, Illinois (44 deg 10 min N, 88 deg 10 min W) were analyzed for day-to-day variations, seasonal variations, magnetic storm aftereffects, and stratosphere-ionosphere coupling effects. As well as showing a winter anomaly, the electron densities near 76 km were significantly lower in fall than in spring. Magnetic storm aftereffects of the type predicted by models of energetic electron precipitation at middle latitudes were observed. No strong correlations were found between stratospheric and D-region time series, or between the occurrence of stratospheric warmings and D-region changes. It is likely that most of the electron density variation was due to variations in the transport of minor neutral constituents. The spring-fall differences were also probably caused by differences in minor constituent concentrations rather than the effect of temperature changes on the recombination coefficient.
A rocket-borne spectrometer measured the weak UV nightglow from 1240 to 1670 A in the altitude range 180-345 km above White Sands, New Mexico. Detection of nightglow emissions at the atomic oxygen lines (1304 and 1356 A) confirmed the existence of a weak midlatitude oxygen nightglow similar to the tropical airglow. Radiative recombination appeared to be the principal cause of the peak observed intensities of the atomic oxygen line emissions, though a maximum 25% contribution from mutual neutralization of O(+) and O(-) could also be contemplated. Partial radiative recombination coefficients are derived from the data.
Recent laboratory measurements have shown that N(2P) atoms, and thus probably hot N(2D) atoms, will recombine with atomic oxygen via an associative ionization process at the gas kinetic rate. In the present paper the likelihood of the associative ionization of N(2D) and O playing a significant role in the normal ionosphere is investigated in the light of several recent studies. It is concluded that the associative ionization process is not an important factor and that a more probable cause for disagreements in the various determinations of the recombination coefficient, is the difference in excited states of the ions in the various experiments.
A microwave afterglow mass spectrometer apparatus is used to determine the dependence on electron temperature T sub e of the recombination coefficients alpha sub n of the dimer and trimer ions of the series CO+.(CO) sub n. It is found that alpha sub 1 = (1.3 + or - 0.3)x 0.000001 (T sub e(K)/300) to the -0.34; and alpha sub 2 = (1.9 + or - 0.4)x 0.000001 (T sub e(K)/300) to the -0.33 cu cm/sec. These dependences on T sub e are quite different from those obtained previously for polar-cluster ions of the hydronium and ammonium series but are similar to that for simple diatomic ions.
Efficient ionization has been observed when an atomic vapor of strontium, barium or calcium was illuminated with a long pulse tunable laser at the frequency of the atomic resonance line. The variation in the degree of ionization with neutral density and laser intensity has been measured using the 'hook' method. The maximum ionization observed was 94%. Excited state populations were measured yielding an excitation temperature (depending on exact experimental conditions) in the region of 0.4 eV. The decay of ion density after the laser pulse was monitored and the recombination coefficients determined. The results are interpreted in terms of an electron heating model.
Temperature-dependent catalytic recombination coefficients are used to calculate the heat flux to the Space Shuttle Orbiter. With variable entropy boundary-layer edge properties obtained from a reacting inviscid flow-field calculation, the reacting boundary-layer equations are solved along the forward 50 percent of the windward centerline using the boundary-layer integral matrix procedure. The results are compared with fully catalytic and noncatalytic reacting solutions, with equilibrium solutions, and with the Orbiter-design heating rates. The fully catalytic heat fluxes are about equal to the equilibrium predictions; whereas, the finite catalytic results are about 12 to 27 percent lower than the fully catalytic results (approaching the noncatalytic results downstream) and as much as 30 to 50 percent lower than design predictions away from the nose area.