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Neutron Absorber Plate Characterization Plan for Criticality Experiments Design [Slides]

The goal of this presentation is to show the feasibility of performing a critical experiment with a B 4 C/Aluminum alloy neutron absorber plate. The motivation of this experiment is to provide integral data on modern neutron absorber product “Boralcan” by Rio Tinto. In 2020, used in about 20% of spent fuel pools in the US, and in casks for storage and transportation in the US and in Europe. The added value of this experiment: Neutron absorber plate modeling method verification: homogeneous or not, a lot of potential savings by relaxing boron loading credit limits. No available critical benchmark involving Boralcan, other boron-related experiments are relatively old. Nuclear data validation for B, C, and Al in the form of B 4 C in Al matrix.

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Field Test Report Neutron Scintillator Array Dry Storage Cask Scanner FY2024

During two weeks of Field Testing at the Idaho National Laboratory INTEC Cask Farm in July and August 2024, the LLNL Dry Storage Cask Scanner Array was lifted on top of an MC-10 dry storage fuel cask and operated to acquire neutron and gamma-ray data from the 24 fuel bundle positions. Neutron and gamma-ray data acquisition scans across the top of the cask of varying dwell times were performed July 15-18, 2024 and August 19-22, 2024 to evaluate the ability of the scanner data to reveal asymmetries in the fuel positions that reflect asymmetries in the MC-10 cask fuel bundle loading. The MC-10 cask 24 position fuel bundle loading at the INTEC Cask Farm is well documented, including the locations of six empty fuel bundle positions. This loading presents an opportunity to test the ability of the scanner system to detect diversion of spent fuel bundles as well as to validate the MC-10 cask MCNP modeling. The cask scanner array consists of six Stilbene crystal scintillator detectors and a linear actuator frame that moves the six detectors across the MC-10 dry storage cask to obtain data above each of the 24 fuel bundle positions. The detectors are connected to a pulse-shape discrimination data acquisition system capable of generating separate neutron and gamma-ray spectra for each detector and for each scan position. From the prior single detector Field Test in 2021 and iteration with MCNP modeling, the neutron and gamma-ray data were analyzed in multiple energy regions to identify an analysis method that would provide the strongest and most consistent signature of the asymmetric MC-10 cask fuel loading1 . From both the 2021 Field Test and the current Field Test results, the neutron capture gamma-ray count rate around 2.2 MeV provides the strongest signature of the asymmetric MC-10 cask fuel loading and has qualitative agreement with MCNP calculations. Counting all gamma-rays produces a similar signature. Neutrons emerging from the cask top are moderated and captured by the hydrogen in the polyethylene moderator and scintillator detector, producing a 2.2 MeV gamma ray which is seen in the scintillator gamma-ray spectrum. The count rate in the 2.2 MeV gamma-ray region is ~50 c/s, which is ~1000x higher than the ~0.05 n/s rate in the > 4MeV neutron region, and ~50x greater than the ~1 n/s rate in the neutrons > 500 keV region. Analysis of the 2.2 MeV neutron-capture Compton-scattered gamma-rays produces a statistically significant signature of the INTEC Cask Farm MC-10 asymmetric fuel loading. MCNP simulations indicate that the average neutron energy spectrum offers the potential to detect a large asymmetry from several missing bundles as well as individual missing fuel bundles. Testing this feature will require measurements on a cask with single missing elements.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Metallographic examinations and hydrogen measurements of high-burnup spent nuclear fuel cladding

In the US, commercial spent nuclear fuel (SNF) is transferred to interim dry storage casks where it will be stored for decades awaiting transport to a consolidated interim storage facility or a geologic repository. Because the fuel rod cladding is the first barrier against any radioactive material release, understanding the behavior of SNF cladding, particularly at high burnup (HBU), in dry storage conditions is crucial to safely store and transport the spent fuel. In this study, a series of metallographic examinations and cladding hydrogen measurements were conducted on HBU SNF cladding at Oak Ridge National Laboratory as a part of the High Burnup Spent Fuel Data Project, which is sponsored by the US Department of Energy (DOE) Office of Nuclear Energy (NE). Here, t o investigate the effect of simulated drying conditions on the cladding, three as-received fuel rods with different cladding materials—M5, ZIRLO, and Zircaloy-4—were heated to 400°C and then slow-cooled to room temperature. The pellet and cladding were then qualitatively and quantitatively analyzed and compared in terms of pellet crack morphology, HBU rim, waterside oxide, cladding H, and cladding hydride morphologies. This paper presents and discusses the results of these analyses in detail.

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Non-destructive evaluation and machine learning methods for inspection of spent nuclear fuel canisters: A state-of-the-art review

Nuclear energy is among the cleanest and most efficient energy sources currently available. The operation of nuclear power plants (NPPs) produces large amounts of high-level radioactive waste known as spent nuclear fuel (SNF). Currently, large amounts of SNF is stored in dry cask storage systems (DCSSs) for extended interim storage until a permanent disposal solution becomes available. During the extended interim storage, the DCSS, particularly the SNF canisters, may degrade and abnormal conditions may occur. Therefore, non-destructive evaluation (NDE) and machine learning (ML) approaches are necessary for inspection of SNF canisters. This paper presents a state-of-the-art review of literature by summarizing recent progress made on the applications of NDE and ML for inspection of SNF canisters. Sixteen NDE methods are examined and compared: visual inspection, ultrasonic guided waves (UGWs), laser-based approaches, acoustic emission (AE), eddy current testing (ECT), non-invasive acoustic sensing, dynamic modal testing, cosmic ray muons tomography, neutron imaging, gamma rays detection, fiber optical sensors, through-wall communications, X-ray computed tomography (CT), vibrothermography, monoenergetic photon sources, and surface acoustic wave (SAW) sensors. The technology readiness level (TRL) for each method is assessed and compared. Recent publications on ML-enhanced visual inspection, AE, non-invasive acoustic sensing, dynamic modal testing, and neutron imaging for SNF canisters are summarized and future research needs are identified. In conclusion, this review article provides a convenient reference on the state-of-the-art applications of NDE and ML methods for inspection of SNF canisters.

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Skyshine Calculations for a Large Spent Nuclear Fuel Storage Facility with SCALE 6.2.3

The SCALE code system developed at Oak Ridge National Laboratory includes state-of-the-art capabilities for radiation source term and radiation transport simulations that can be used in numerous applications, including dose rate analyses of complex consolidated interim storage facilities (CISFs). A licensed CISF could be used to store tens of thousands of tonnes of spent nuclear fuel discharged from commercial power reactors using various cask and storage pad designs. A CISF design must comply with the regulatory requirements provided in 10 CFR Part 72, including requirements related to annual dose limits applicable to real individuals located beyond the area controlled by the licensee. Therefore, calculating a dose to the public is a necessary part of the licensing process for the construction of a CISF. These calculations are very challenging because of the complexity of the CISF design and the low magnitude of dose rate at large distances from the facility. This paper describes detailed far-field dose rate calculations performed for a proposed CISF using MAVRIC, the Monte Carlo radiation shielding sequence in SCALE 6.2.3, with automated variance reduction based on discrete ordinates calculations. The method presented in this paper uses a detailed Monte Carlo radiation transport simulation in one step from source to dose rate. A series of independent simulations was made using the complete site geometry (all casks present), but with only one cask containing radiation sources to obtain the dose rate maps produced by each storage cask. The CISF dose rate map was obtained by adding the dose rate maps produced by the independent individual cask simulations. Ample volumes of air and soil extending beyond the location of interest for dose rate calculation were included in the calculation model to properly simulate important radiation attenuation and scattering events that affect far-field dose rates. Furthermore, a comprehensive sensitivity study is included in this paper to illustrate the importance of selecting appropriate air volume, mass density, and composition for CISF skyshine dose rate calculations. Dry soil and soil containing water were analyzed to determine their effects on groundshine radiation.

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Modeling and Analysis for Spent Nuclear Fuel Seismic Testing

Note: This is the final public release version of PNNL-31671 Draft, which was previously released to the sponsor for review. The intent is the public release version will be PNNL-31671. There are no significant changes from the earlier draft version. This unlimited distribution report is the deliverable for M3SF-21PN010202014: Modeling and Analysis for Spent Nuclear Fuel Seismic Testing. This report summarizes the modeling, analysis, and test plan support completed by Pacific Northwest National Laboratory for the spent nuclear fuel dry storage system seismic test plan through May of 2021. Test plan preparation is planned to continue until the seismic test is completed in July of 2022. This report covers preliminary structural dynamic model development and computer-aided design of test hardware. Based on preliminary modeling, the strongest earthquakes under consideration in this test program provide mechanical loading on the spent nuclear fuel that is comparable to the 30 cm cask drop scenario, although the loads do not appear to be strong enough to cause significant permanent deformation of the fuel assembly spacer grids. The potential for grid deformation during the test will be assessed when the proposed shake table motion becomes available. The weakest earthquakes considered in this test are expected to be comparable to the mechanical loads witnessed in the multimodal transportation test of 2017. The horizontal canister system is predicted to provide nearly-uniform loading condition on the fuel assemblies it contains, while the vertical cask system is predicted to cause non-uniform dynamic loads on the fuel assemblies. In the horizontal case, gravity keeps the fuel assemblies in contact with one basket wall surface unless the loads are strong enough to cause a separation. In the vertical case, the fuel assemblies are relatively long and slender, and seismic motion in the anticipated test range is predicted to cause the assemblies to lean, tilt, and impact the basket walls throughout the seismic event. These gap closures are a nonlinear force transmission condition, so the vertical system is expected to have more variation and variability than the horizontal system. While the horizontal system is expected to have a relatively more linear response than the vertical system, there is still the potential for nonlinear behavior in the horizontal system because the fuel assemblies are free to slide, bounce, and impact the basket walls if the seismic loads are strong enough. One major conclusion of this study is that the use of mixed fuel assemblies in the canister will be acceptable. There are differences in overall system response when the mass, center of gravity, or gaps are changed, but the changes in response are within the bounds of a system that contains completely homogeneous fuel assemblies. One important observation is that the loading for each individual fuel assembly within the vertical canister is expected to be different from that of the others because of nonlinearities in the system. The horizontal canister system is expected to have a more uniform and more predictable response than the vertical canister, making variations in fuel assembly characteristics easier to account for. One important recommendation that comes from this modeling work is to repeat some of the strongest shake tests at different angles, particularly for the vertical cask system. Modeling predicts that strong seismic motion will cause the fuel assemblies to close initial gaps and impact the fuel basket walls when the canister is in the vertical cask configuration. Each shake test will impose a pre-defined three-dimensional time history on the cask system.

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Coupling SCALE with DAKOTA for Axial Burnup Profiles Assessment in Burnup Credit

This paper presents a computational study that demonstrates the application of the SCALE code system in conjunction with the Design Analysis Kit for Optimization and Terascale Applications (DAKOTA) for the analysis of key factors influencing the evaluation of burnup credit (BUC) in pressurized water reactors (PWRs). The primary objective of this analysis is to characterize the model by utilizing parameterization, uncertainty quantification, and optimization studies. Using this approach, we can comprehensively assess the system and conduct informed predictive studies. This study highlights the effectiveness of the SCALE code system integrated within the DAKOTA framework in terms of efficiency and capability. With the coupling of the burnup code ORIGAMI with the CSAS or TSUNAMI-3D sequence embedded in a DAKOTA analysis, we can characterize the factors that influence the k eff of PWR 17x17 spent nuclear fuel (SNF) in the GBC-32 computational benchmark cask for the assessment of BUC in criticality safety analysis. The coupling methodology used in this study is not exclusive to BUC analysis. However, the choice to apply this methodology to the BUC problem is particularly significant because of the diverse range of aspects it encompasses in nuclear criticality safety analyses. This problem presents a unique opportunity to explore and address multiple facets of such analyses related to BUC and illustrates the capability of the SCALE code system with DAKOTA. This analysis makes use of historical reference data for the axial burnup profile, where the entire space within the bounds is considered. Both SCALE and DAKOTA are currently integrated in the Nuclear Energy Advanced Modeling Simulation (NEAMS) Workbench code system, which has a user-friendly graphical interface that simplifies the setup of simulations and configuration of input parameters as well as the visualization of simulation results.

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Next Generation System Analysis Model: Recently Added Features and Future Plans

To better enable informed decision-making regarding the back-end of the nuclear fuel cycle, the Integrated Waste Management System (IWMS) program within the U.S. Department of Energy, Office of Nuclear Energy (DOE-NE) has been sponsoring the development and application of system analysis tools capable of analyzing various system options for the management of spent nuclear fuel (SNF) and high-level radioactive waste (HLW).With these tools, IWMS architecture analyses are being conducted to support the future deployment of a comprehensive nuclear waste management system that considers all major back-end aspects of the nuclear fuel cycle (i.e., transportation, storage, and disposal). The Next Generation System Analysis Model (NGSAM) is an agent-based simulation software tool expressly designed to be capable of modeling features within various IWMS architectures. NGSAM imports data from Oak Ridge National Laboratory (ORNL)’s unified database (e.g., historic assembly information, thermal profiles for assembly heat, and at-reactor dry storage loadings) to ensure that each simulation initializes with a realistic representation of the state of commercial SNF in the U.S. Recent major enhancements implemented into NGSAM in the period since NGSAM was last presented at the WM2019 conference include: • Tracking of railroad escort car acquisition and buffer car acquisition • The addition of heavy haul truck (HHT) and barge routes for some sites, as well as support for user-defined inter-modal routes • Updates to the logic that checks the transportation cask thermal limit maps prior to package transport • An allocation method that predicts when reactor sites would pack assemblies from their spent fuel pools for dry storage, and prioritizes shipments directly from the pools of those reactor sites in the preceding periods (before the predicted loadings to dry storage), thus reducing the number of casks loaded into dry storage at reactor sites • The addition of “reactor site family” operational limits to restrict the number of loads of SNF taken from the pool and from dry storage at a given reactor site each year • Added support for multiple canister loading map options and packages with multiple compatible transportation overpacks • Updates to the handling of non-commercial SNF, including a new database that contains data to support the updates • Updates to allow analysis of hypothetical scenarios which include repackaging at reactor sites, e.g., for possible comparative analysis with other scenarios • Implementation of additional output reports, or modification of existing ones • The ability to generate and implement user edits via the NGSAM website • The ability to model loading SNF from pool storage at an interim storage facility (ISF) into dry storage at the ISF • The ability to model consolidating SNF from different existing storage containers at a DOE site into the same DOE standard canister • The ability to model transferring SNF casks from one transportation mode to another, e.g., from HHT to rail, referred to as transloading. These new features have improved NGSAM capabilities and users’ experience with the model. Preliminary NGSAM requirements for modeling advanced reactor fuels, reprocessing, treatment, and conditioning were considered, and this paper describes them at a high level. Other nuclear fuel cycle system analysis tools developed under sponsorship of DOE-NE, like the VISION code developed at Idaho National Laboratory, might be better suited for initial high-level analysis of those technologies and advanced fuel cycles. As technologies are developed and system concepts evolve, NGSAM could provide value by providing more detailed modeling of transport, storage, and disposal of spent fuel and wastes from advanced reactors and advanced fuel cycles at the fuel element and waste container level.

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Investigation of Cold Spray as a Dry Storage Canister Repair and Mitigation Tool

The lack of a permanent spent nuclear fuel repository means utilities are faced with extending licenses for dry cask storage systems (DCSS) canisters far beyond their original 20-year license period. DCSS canisters are made from austenitic stainless steels (SSs) and fabricated using fusion welds. High heat input and melting associated with fabrication welds causes material around the weld to be susceptible to chloride-induced stress corrosion cracking (CISCC). The purpose of the work reported here is to investigate the use of cold spray for repair and mitigation of CISCC in DCSS canisters to ensure integrity far beyond their original license period. This report presents an analysis of cold spray for canister life extension, a summary of related efforts, relevant technology down selections, work accomplished, and future efforts relative to use of cold spray for repair and mitigation of CISCC in DCSS canisters.

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Code of Record: DOE Standard Canister (DOESC)

The United States Department of Energy (DOE) Spent Nuclear Fuel (SNF) Packaging Demonstration seeks to develop and demonstrate the designs, technology, processes, and regulatory framework for packaging DOE SNF for road-ready dry storage (RRDS); and establish the processes that will be used in a future production facility. The Packaging Demonstration will utilize the DOE Standard Canister (DOESC) for packaging select DOE-managed SNF types for interim storage, transportation and disposal as part of RRDS. Placing DOE-managed SNF into RRDS is part of the strategic framework for SNF on the Idaho National Laboratory (INL) site. To comply with DOE, INL and Nuclear Regulatory Commission (NRC) requirements, this Code of Record establishes the American Society of Mechanical Engineers (ASME) Boiler and Pressure Vessel Code (BPVC), Section III, Division 3 as the Code that will govern DOESC and internal support structure constructioni, with certain clarifications. This Code of Record establishes a rationale for proceeding without construction certification of the DOESC (i.e., “N-stamping) and the extent to which a Registered Professional Engineer is required for the DOE Spent Fuel Packaging Demonstration. Given the (i) standard industry practice to pursue independent licensure of commercial storage casks and transportation packages by the NRC in lieu of ASME certification and (ii) guidance provided by 10 CFR 830, DOESC construction activities need not be certified (i.e., “stamped”) to the ASME BPVC. However, additional quality assurance requirements will apply as outlined in this Code of Record.

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Seismic response of vertical dry storage casks under three-dimensional earthquake motions

Ensuring the long-term seismic safety of dry storage casks (DSCs) is becoming increasingly critical as these systems evolve from temporary to de facto permanent repositories for spent nuclear fuels. Traditional seismic soil–structure interaction (SSI) assessment methods use one-dimensional deconvolution or simplified boundary conditions to model incident waves. Although computationally appealing, simplifying assumptions may alter the seismic risk by neglecting the full complexity of three-dimensional (3D) wave propagation effects. To address this challenge, this paper introduces a novel high-fidelity computational framework that leverages the Domain Reduction Method (DRM) with perfectly matched layers (PML) to accurately transfer complex, 3D seismic wavefields from regional-scale fault-rupture simulations into local-scale finite element models of DSCs. Using broadband, physics-based ground motions from a generic M w 7.0 strike-slip event, both single-cask and multi-cask configurations were investigated under near- and far-field conditions. Emphasis is placed on capturing complex SSI, spatial variability in the ground motion, and nonlinear phenomena such as cask rocking and sliding. Numerical results demonstrate that near-field conditions, where forward directivity and fling-step effects dominate, lead to significantly higher DSC rocking and sliding. Far-field cases, by contrast, generally exhibit modest responses. Incorporating SSI tends to amplify or alter DSC response spectra and introduce response variability, which underscores the need for site-specific evaluations and robust modeling approaches to ensure the seismic integrity of DSCs in interim spent fuel storage installations.

Das, Tonmoy↗

Using temperature and flow fields to detect gas leakage from canisters containing spent nuclear fuel: Applications to RAMM-TM

The multi-physics STAR-CCM+ code has been used to simulate the temperature and flow fields in canister gas leakage experiments conducted by using a 1/4.5-scale model storage cask. The simulations were conducted at Argonne National Laboratory’s Laboratory Computing Resource Center, utilizing high-performance computing resources. Development of STAR-CCM+ simulation models for the 1/4.5-scale model cask is described herein, followed by validation of the simulation results against experimental data. Canister depressurization and thermal response during gas leakage are discussed, along with analyses of the leakage path and allowable leakage rate. The insights gained from the STAR-CCM+ simulations and leakage analyses will help guide future experiments and actual industry applications of Argonne’s Remote Area Modular Monitoring system for canister surface temperature measurement (RAMM-TM) to enable effective aging management of spent fuel during extended dry storage, as well as help reduce risks to public safety and health and protect the environment.

Canister gas leakage↗

Drop impact tester development for spent nuclear fuel vibration integrity study

The accumulated damage of SNF rod is defined as the integrated damage induced by the SNF assembly harmonic vibrations and SNF assembly & cask system contact interactions induced transient shocks, experienced by SNF rods during normal conditions of transportation (NCT). The CIRFT technology has provided means to resolve/understand the SNF rod harmonic vibration reliability issues associated with maximum axial clad tubing stress induced by SNF inertia related dynamic bending loading. However, the SNF rod integrity in association with the transient shock loads during NCT through dynamic contact interactions among SNF assembly cannot be investigated systematically through CIRFT technology alone. Thus, the proposed drop impact tester development become a viable tool for SNF system transient shock effect investigation. Furthermore, the transient shocks induced loading mode is normally perpendicular to the SNF rod axial orientation, i.e., in a transverse orientation to the SNF rod. To proceed with such loading mode investigation, a new device, “SNF Drop Impact Tester” that provides the transverse impact shock load onto a SNF rod through a free-drop projectile was developed in FY20 for SNF System Vibration Reliability Investigation; where the SNF system contact impact intensity can be calibrated accordingly with projectile weight and projectile head geometry. This newly developed research tool can further provide a detailed understanding about the effect of dynamic contact-interaction loadings; and combined harmonic vibration and transient shock loading modes on the fatigue damage evolution of the HBU SNF under NCT.

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Preliminary Evaluation of Removing SNF from Nuclear Power Plant Sites - Pilgrim Site Visit - 20048

The U.S. Department of Energy Office of Integrated Waste Management (DOE-IWM)a conducted an evaluation of removing spent nuclear fuel (SNF) from the Pilgrim site on November 4-8, 2019. The Pilgrim site is located on the western shore of Cape Cod Bay in the Town of Plymouth, Massachusetts, about 61 km southeast of Boston and 71 km east of Providence, Rhode Island. Participants in the site visit included the U.S. Department of Energy, Oak Ridge National Laboratory, Pacific Northwest National Laboratory, the state of Massachusetts, the Federal Railroad Administration, the U.S. Coast Guard, the U.S. Army Corps of Engineers, the Mashpee Wampanoag Tribe, the Consolidated Group of Tribes and Organizations, the Council of State Governments-Eastern Regional Conference, the Pilgrim Nuclear Decommissioning Citizens Advisory Panel, and the Massachusetts Coastal Railroad. The Pilgrim site was found to have two transportation mode options for the removal of SNF, offsite rail access and onsite barge access. Two offsite heavy haul truck to rail transload locations were evaluated, one in Middleborough, Massachusetts, about 35-47 km from the Pilgrim site, and a second location in Middleborough about 36-43 km from the Pilgrim site. A passenger railroad terminates in Plymouth, Massachusetts, about 11 km from the Pilgrim site; however, this location is not suitable for freight rail involving large SNF transportation casks. There is also an onsite barge facility located on the Pilgrim site that was used during construction and would require refurbishment to be used. (authors)

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Estimation of Respirable Aerosol Release Fractions through Stress Corrosion Crack-Like Geometries

The formation of a stress corrosion crack (SCC) in the canister wall of a dry cask storage system (DCSS) has been identified as a potential issue for the long-term storage of spent nuclear fuel. The presence of an SCC in a storage system could represent a through-wall flow path from the canister interior to the environment. Modern, vertical DCSSs are of particular interest due to the significant backfill pressurization of the canister, up to approximately 800 kPa. This pressure differential offers a relatively high driving potential for blowdown of any particulates that might be present in the canister. In this study, the carrier gas flow rates and aerosol transmission properties were evaluated for an engineered microchannel with characteristic dimensions similar to those of an SCC. The microchannel was formed by mating two gage blocks with a slot orifice measuring 28.9 μm (0.0011 in.) tall by 12.7 mm (0.500 in.) wide by 8.86 mm (0.349 in.) long (flow length). Surrogate aerosols of cerium oxide, Ce0 2 , were seeded and mixed inside a pressurized tank. The aerosol characteristics were measured immediately upstream and downstream of the simulated SCC at elevated and ambient pressures, respectively. These data sets are intended to demonstrate a new capability to characterize SCCs under well-controlled boundary conditions. Separate modeling efforts are also underway that will be validated using these data. The test apparatus and procedures developed in this study can be easily modified for the evaluation of more complex SCC-like geometries including laboratory-grown SCC samples.

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Continued Investigations of Respirable Release Fractions for Stress Corrosion Crack-Like Geometries

The formation of a stress corrosion crack (SCC) in the canister wall of a dry cask storage system (DCSS) has been identified as a potential issue for the long-term storage of spent nuclear fuel. The presence of an SCC in a storage system could represent a through-wall flow path from the canister interior to the environment. Modern, vertical DCSSs are of particular interest due to the commercial practice of using relatively high backfill pressures (up to approximately 800 kPa) in the canister to enhance internal natural convection. This pressure differential offers a comparatively high driving potential for blowdown of any particulates that might be present in the canister. In this study, the rates of gas flow and aerosol transmission of a spent fuel surrogate through an engineered microchannel with dimensions representative of an SCC were evaluated experimentally using coupled mass flow and aerosol analyzers. The microchannel was formed by mating two gage blocks with a linearly tapering slot orifice nominally 13 μm (0.005 in.) tall on the upstream side and 25 μm (0.0010 in.) tall on the downstream side. The orifice is 12.7 mm (0.500 in.) wide by 8.89 mm (0.350 in.) long (flow length). Surrogate aerosols of cerium oxide, CeO 2 , were seeded and mixed with either helium or air inside a pressurized tank. The aerosol characteristics were measured immediately upstream and downstream of the simulated SCC at elevated and ambient pressures, respectively. These data sets are intended to demonstrate a new capability to characterize SCCs under well-controlled boundary conditions. Modeling efforts were also initiated that evaluate the depletion of aerosols in a commercial dry storage canister. These preliminary modeling and ongoing testing efforts are focused on understanding the evolution in both size and quantity of a hypothetical release of aerosolized spent fuel particles from failed fuel to the canister interior and ultimately through an SCC.

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Quantification of Aerosol Transmission through Stress Corrosion Crack-Like Geometries

The formation of a stress corrosion crack (SCC) in the canister wall of a dry cask storage system (DCSS) has been identified as a potential issue for the long-term storage of spent nuclear fuel. The presence of an SCC in a storage system could represent a through-wall flow path from the canister interior to the environment. Modern, vertical DCSSs are of particular interest due to the commercial practice of using more significant backfill pressures in the canister, up to approximately 800 kPa. This pressure differential offers a relatively high driving potential for blowdown of any particulates that might be present in the canister. In this study, the rates of gas flow and aerosol transmission of a spent fuel surrogate through an engineered microchannel with dimensions representative of an SCC were evaluated experimentally using coupled mass flow and aerosol analyzers. The microchannel was formed by mating two gage blocks with a linearly tapering slot orifice nominally 13 μm (0.005 in.) tall on the upstream side and 25 μm (0.0010 in.) tall on the downstream side. The orifice is 12.7 mm (0.500 in.) wide by 8.86 mm (0.349 in.) long (flow length). Surrogate aerosols of cerium oxide, CeO 2 , were seeded and mixed with either helium or air inside a pressurized tank. The aerosol characteristics were measured immediately upstream and downstream of the simulated SCC at elevated and ambient pressures, respectively. These data sets are intended to add to previous testing that characterized SCCs under well-controlled boundary conditions through the inclusion of testing improvements that establish initial conditions in a more consistent way. These ongoing testing efforts are focused on understanding the evolution in both size and quantity of a hypothetical release of aerosolized spent fuel particles from failed fuel to the canister interior and ultimately through an SCC.

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