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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 91 records · Page 5
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Ultrafast optical modulation of vibrational strong coupling in ReCl(CO) 3 (2,2-bipyridine)

Polaritons – hybrid light-matter states formed from the strong coupling of a bright molecular transition with a confined photonic mode – may offer new opportunities for optical control of molecular behavior. Vibrational strong coupling (VSC) has been reported to impact ground-state chemical reactivity, but its influence on electronic excited-state dynamics remains unexplored. Here, we take a first step towards excited-state VSC by demonstrating optical modulation of the ReCl(CO) 3 (bpy), (bpy = 2,2-bipyridine) complex under VSC using femtosecond ultraviolet (UV)-pump/infrared (IR)-probe spectroscopy. We establish ground-state VSC of ReCl(CO) 3 (bpy) in a microfluidic Fabry-Pérot cavity equipped with indium tin oxide (ITO)-coated mirrors. ITO is effectively dichroic as it is reflective in the IR and transmissive in the UV-visible and therefore minimizes optical interference. Excitation with UV pump light drives ReCl(CO) 3 (bpy) into a manifold of electronic excited states that subsequently undergo non-radiative relaxation dynamics. We probe the transient response of the strongly-coupled system in the mid-IR, observing both Rabi contraction and cavity-filtered excited-state absorption signatures. We reconstruct the intrinsic response of intracavity molecules from the transient cavity transmission spectra to enable quantitative comparison with extracavity control experiments. We report no changes in the excited-state dynamics of ReCl(CO) 3 (bpy) under ground-state VSC. However, we do observe significant amplification of transient vibrational signals due to classical cavity-enhanced optical effects. This effort lays the groundwork to pursue direct excited-state VSC aimed at modulating photochemical reactivity.

cavity-enhanced spectroscopy↗
DOE OSTI2024

Generalized gluon distribution for quarkonium dynamics in strongly coupled N = 4 Yang-Mills theory

We study the generalized gluon distribution that governs the dynamics of quarkonium inside a non-Abelian thermal plasma characterizing its dissociation and recombination rates. This gluon distribution can be written in terms of a correlation function of two chromoelectric fields connected by an adjoint Wilson line. We formulate and calculate this object in N = 4 supersymmetric Yang-Mills theory at strong coupling using the AdS/CFT correspondence, allowing for a nonzero center-of-mass velocity v of the heavy quark pair relative to the medium. The effect of a moving medium on the dynamics of the heavy quark pair is described by the simple substitution T → γ T in agreement with previous calculations of other observables at strong coupling, where T is the temperature of the plasma in its rest frame, and γ = ( 1 − v 2 ) − 1 / 2 is the Lorentz boost factor. Such a velocity dependence can be important when the quarkonium momentum is larger than its mass. Contrary to general expectations for open quantum systems weakly coupled with large thermal environments, the contributions to the transition rates that are usually thought of as the leading ones in Markovian descriptions vanish in this strongly coupled plasma. This calls for new theoretical developments to assess the effects of strongly coupled non-Abelian plasmas on in-medium quarkonium dynamics. Finally, we compare our results with those from weakly coupled QCD, and find that the QCD result moves toward the N = 4 strongly coupled result as the coupling constant is increased within the regime of applicability of perturbation theory. This behavior makes it even more pressing to develop a non-Markovian description of quarkonium in-medium dynamics. Published by the American Physical Society 2024

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2010

Exact non-Markovian cavity dynamics strongly coupled to a reservoir

The exact non-Markovian dynamics of a microcavity strongly coupled to a general reservoir at arbitrary temperature are studied. With the exact master equation for the reduced density operator of the cavity system, we analytically solve the time evolution of the cavity state and the associated physical observables. We show that the non-Markovian dynamics are completely determined by the propagating (retarded) and correlation Green functions. Comparing the non-Markovian behavior at finite temperature with those at the zero-temperature limit or Born-Markov limit, we find that the non-Markovian memory effect can dramatically change the coherent and thermal dynamics of the cavity. We also numerically study the dissipation dynamics of the cavity through the mean mode amplitude decay and the average photon number decay in the microwave regime. It is shown that the strong coupling between the cavity and the reservoir results in a long-time dissipationless evolution to the cavity field amplitude, and its noise dynamics undergo a critical transition from the weak to the strong coupling due to the non-Markovian memory effect.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2016

Sub- and super-luminar propagation of structures satisfying Poynting-like theorem for incompressible generalized hydrodynamic fluid model depicting strongly coupled dusty plasma medium

The strongly coupled dusty plasma has often been modelled by the Generalized Hydrodynamic (GHD) model used for representing visco-elastic fluid systems. The incompressible limit of the model which supports transverse shear wave mode is studied in detail. In particular, dipole structures are observed to emit transverse shear waves in both the limits of sub- and super-luminar propagation, where the structures move slower and faster than the phase velocity of the shear waves, respectively. In the sub-luminar limit the dipole gets engulfed within the shear waves emitted by itself, which then backreacts on it and ultimately the identity of the structure is lost. However, in the super-luminar limit the emission appears like a wake from the tail region of the dipole. The dipole, however, keeps propagating forward with little damping but minimal distortion in its form. A Poynting-like conservation law with radiative, convective, and dissipative terms being responsible for the evolution of W, which is similar to “enstrophy” like quantity in normal hydrodynamic fluid systems, has also been constructed for the incompressible GHD equations. The conservation law is shown to be satisfied in all the cases of evolution and collision amidst the nonlinear structures to a great accuracy. It is shown that monopole structures which do not move at all but merely radiate shear waves, the radiative term, and dissipative losses solely contribute to the evolution of W. The dipolar structures, on the other hand, propagate in the medium and hence convection also plays an important role in the evolution of W.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2016

Towards achieving strong coupling in three-dimensional-cavity with solid state spin resonance

We investigate the microwave magnetic field confinement in several microwave three-dimensional (3D)-cavities, using a 3D finite-element analysis to determine the best design and achieve a strong coupling between microwave resonant cavity photons and solid state spins. Specifically, we design cavities for achieving strong coupling of electromagnetic modes with an ensemble of nitrogen vacancy (NV) defects in diamond. We report here a novel and practical cavity design with a magnetic filling factor of up to 4 times (2 times higher collective coupling) than previously achieved using one-dimensional superconducting cavities with a small mode volume. In addition, we show that by using a double-split resonator cavity, it is possible to achieve up to 200 times better cooperative factor than the currently demonstrated with NV in diamond. These designs open up further opportunities for studying strong and ultra-strong coupling effects on spins in solids using alternative systems with a wider range of design parameters. The strong coupling of paramagnetic spin defects with a photonic cavity is used in quantum computer architecture, to interface electrons spins with photons, facilitating their read-out and processing of quantum information. To achieve this, the combination of collective coupling of spins and cavity mode is more feasible and offers a promising method. This is a relevant milestone to develop advanced quantum technology and to test fundamental physics principles.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2016

Shock structures in a strongly coupled self-gravitating opposite-polarity dust plasma

A strongly coupled, self-gravitating, opposite-polarity dust plasma (containing strongly coupled inertial positive and negative dust fluids, and inertialess weakly coupled ions) is considered. The generalized hydrodynamic model and the reductive perturbation method are employed to examine the possibility for the formation of the dust-acoustic (DA) shock structures in such an opposite-polarity dust plasma. It has been shown that the strong correlation among charged dust is a source of dissipation and is responsible for the formation of the DA shock structures in such the opposite-polarity dust plasma medium. The parametric regimes for the existence of the DA shock structures (associated with electrostatic and gravitational potentials) and their basic properties (viz., polarity, amplitude, width, and speed) are found to be significantly modified by the combined effects of positively charged dust component, self-gravitational field, and strong correlation among charged dust. The implications of our results in different space plasma environments and laboratory plasma devices are briefly discussed.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2014

Strong coupling in hybrid plasmon-modulated nanostructured cavities

The understanding of strong coupling between local restricted electromagnetic field of cavity and surface-plasmon (SP) on the metal surface lays the groundwork for many photonic applications. However, much of the fundamental photophysical properties underlying this performance such as how this strong coupling is induced by these two components, namely, the SP modes and cavity modes have remained unknown. Here, we present a study of a hybrid plasmon-modulated coupled system with Rabi splitting energy at 336 meV, and the coupled hybrid states are highly sensitive to the prosperity of SP mode which is induced by morphology of inlaid grating surfaces.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2015

Coupling of dust acoustic and shear mode through velocity shear in a strongly coupled dusty plasma

In the strongly coupled limit, the generalized hydrodynamic model shows that a dusty plasma, acquiring significant rigidity, is able to support a “shear” like mode. It is being demonstrated here that in presence of velocity shear gradient, this shear like mode gets coupled with the dust acoustic mode which is generated by the compressibility effect of the dust fluid due to the finite temperatures of the dust, electron, and ion fluids. In the local analysis, the dispersion relation shows that velocity shear gradient not only couples the two modes but is also responsible for the instabilities of that coupled mode which is confirmed by nonlocal analysis with numerical techniques.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2017

Strong Coupling and Entanglement of Quantum Emitters Embedded in a Nanoantenna-Enhanced Plasmonic Cavity

Establishing strong coupling between spatially separated and thus selectively addressable quantum emitters is a key ingredient to complex quantum optical schemes in future technologies. Insofar as many plasmonic nanostructures are concerned, however, the energy transfer and mutual interaction strength between distant quantum emitters can fail to provide strong coupling. Here, based on mode hybridization, the longevity and waveguide character of an elliptical plasmon cavity are combined with intense and highly localized field modes of suitably designed nanoantennas. Based on FDTD simulations a quantum emitter-plasmon coupling strength hg = 16.7 meV is reached while simultaneously keeping a small plasmon resonance line width h gamma(s) = 33 meV. This facilitates strong coupling, and quantum dynamical simulations reveal an oscillatory exchange of excited state population arid a notable degree of entanglement between the quantum emitters spatially separated by 1.8 mu m, i.e., about twice the operating wavelength.

Hensen, Matthias↗
DOE OSTI2021

Strong-coupling expansion of multi-band interacting models: Mapping onto the transverse-field J 1 - J 2 Ising model

We investigate a class of two-dimensional two-band microscopic models in which the inter-band repulsive interactions play the dominant role. We first demonstrate three different schemes of constraining the ratios between the three types of inter-band interactions – density-density, spin exchange, and pair-hopping – that render the model free of the fermionic sign-problem for any filling and, consequently, amenable to efficient Quantum Monte Carlo simulations. We then study the behavior of these sign-problem-free models in the strong-coupling regime. In the cases where spin-rotational invariance is preserved or lowered to a planar symmetry, the strong-coupling ground state is a quantum paramagnet. However, in the case where there is only a residual Ising symmetry, the strong-coupling expansion maps onto the transverse-field J 1 - J 2 Ising model, whose pseudospins are associated with local inter-band magnetic order. We show that by varying the band structure parameters within a reasonable range of values, a variety of ground states and quantum critical points can be accessed in the strong-coupling regime, some of which are not realized in the weak-coupling regime. Here, we compare these results with the case of the single-band Hubbard model, where only intra-band repulsion is present, and whose strong-coupling behavior is captured by a simple Heisenberg model.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2015

Amplification of a seed pumped by a chirped laser in the strong coupling Brillouin regime

Seed amplification via Brillouin backscattering of a long pump laser-pulse is considered. The interaction takes place in the so called strong coupling regime. Pump chirping is applied to mitigate spontaneous Raman backscattering of the pump before interacting with the seed. The strong coupling regime facilitates stronger exponential growth and narrower seeds compared to the so called weak coupling regime, although in the latter the scaling with pump amplitude is stronger. Strong coupling is achieved when the pump laser amplitude exceeds a certain threshold. It is shown how the chirp influences both the linear as well as the nonlinear amplification process. First, linear amplification as well as the seed profiles are determined in dependence of the chirping rate. In contrast to the weak coupling situation, the evolution is not symmetric with respect to the sign of the chirping rate. In the nonlinear stage of the amplification, we find an intrinsic chirp of the seed pulse even for an un-chirped pump. We show that chirping the pump may have a strong influence on the shape of the seed in the nonlinear amplification phase. Also, the influence of pump chirp on the efficiency of Brillouin seed amplification is discussed.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2024

Nonperturbative resolution of strong coupling singularities in 4D 𝒩 = 1 heterotic M-theory

We investigate the interior of the moduli space of four-dimensional 𝒩 = 1 theories of gravity arising from compactifications of the 𝐸 8 × 𝐸 8 heterotic string on Calabi-Yau threefolds. By studying the threshold corrections to the coupling of the heterotic gauge groups, we infer the existence of a strong coupling singularity for one of the perturbative heterotic gauge groups, which effectively yields an additional finite distance boundary of the classical scalar field space. In heterotic M-theory, this boundary maps to a domain wall solution for which the gauge coupling and the warp factor on one of the Horava-Witten 9-branes diverge, thus highlighting the gravitational origin of the classical strong coupling singularity. The divergence of the warp factor is, however, regulated once nonperturbative effects are taken into account, as we demonstrate by studying the instanton corrections to the 5D BPS domain wall equations. This regularization implies that the classical strong coupling boundary of the scalar field 4D 𝒩 = 1 heterotic M-theory is resolved, indicating that, at the quantum level, the field space can be extended beyond this classical boundary.

Cvetič, Mirjam↗
DOE OSTI2015

Circuit electromechanics with single photon strong coupling

In circuit electromechanics, the coupling strength is usually very small. Here, replacing the capacitor in circuit electromechanics by a superconducting flux qubit, we show that the coupling among the qubit and the two resonators can induce effective electromechanical coupling which can attain the strong coupling regime at the single photon level with feasible experimental parameters. We use dispersive couplings among two resonators and the qubit while the qubit is also driven by an external classical field. These couplings form a three-wave mixing configuration among the three elements where the qubit degree of freedom can be adiabatically eliminated, and thus results in the enhanced coupling between the two resonators. Therefore, our work constitutes the first step towards studying quantum nonlinear effect in circuit electromechanics.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2023

Dissociation slowdown by collective optical response under strong coupling conditions

We consider an ensemble of diatomic molecules resonantly coupled to an optical cavity under strong coupling conditions at normal incidence. Photodissociation dynamics is examined via direct numerical integration of the coupled Maxwell–Schrödinger equations with molecular rovibrational degrees of freedom explicitly taken into account. It is shown that the dissociation is significantly affected (slowed down) when the system is driven at its polaritonic frequencies. The observed effect is demonstrated to be of transient nature and has no classical analog. An intuitive explanation of the dissociation slowdown at polaritonic frequencies is proposed.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2024

Quarkonium transport in weakly and strongly coupled plasmas

We report on progress in the nonperturbative understanding of quarkonium dynamics inside a thermal plasma. The time evolution of small-size quarkonium is governed by two-point correlation functions of chromoelectric fields dressed with an adjoint Wilson line, known in this context as generalized gluon distributions (GGDs). The GGDs have been calculated in both weakly and strongly coupled plasmas by using perturbative and holographic methods. Strikingly, the results of our calculations for a strongly coupled plasma indicate that the quarkonium dissociation and recombination rates vanish in the transport descriptions that assume quarkonium undergoes Markovian dynamics. However, this does not imply that the dynamics is trivial. As a starting point to explore the phenomenological consequences of the result at strong coupling, we show a calculation of the Y(1 S ) formation probability in time-dependent perturbation theory. This is a first step towards the development of a transport formalism that includes non-Markovian effects, which, depending on how close the as of yet undetermined nonperturbative QCD result of the GGDs is to the strongly coupled N = 4 SYM result, could very well dominate over the Markovian ones in quark-gluon plasma produced at RHIC and the LHC.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2012

Dark energy from dark radiation in strongly coupled cosmologies with no fine tuning

A dual component made of non-relativistic particles and a scalar field, exchanging energy, naturally falls onto an attractor solution, making them a (sub)dominant part of the cosmic energy during the radiation dominated era, provided that the constant β, measuring the coupling, is strong enough. The density parameters of both components are then constant, as they expand as a{sup −4}. If the field energy is then prevalently kinetic, as is expected, its energy is exactly half of the pressureless component; the dual component as a whole, then, has a density parameter Ω{sub cd} = 3/4β{sup 2} (e.g., for β ≅ 2.5, Ω{sub cd} ≅ 0.1, in accordance with Dark Radiation expectations). The stationary evolution can only be broken by the rising of other component(s), expanding as a{sup −3}. In a realistic scenario, this happens when z ∼ 3–5 × 10{sup 3}. When such extra component(s) become(s) dominant, the densities of the dual components also rise above radiation. The scalar field behavior can be easily tuned to fit Dark Energy data, while the coupled DM density parameter becomes O(10{sup −3}). This model however requires that, at present, two different DM components exist. The one responsible for the break of the stationary regime could be made, e.g., by thermally distributed particles with mass even >> 1–2 keV (or non-thermal particles with analogous average speed) so accounting for the size of observed galactic cores; in fact, a fair amount of small scale objects is however produced by fluctuation re-generated by the coupled DM component, in spite of its small density parameter, after the warm component has become non-relativistic.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2012

Kelvin-Helmholtz instability in a strongly coupled dusty plasma medium

The Kelvin-Helmholtz (KH) instability in the context of strongly coupled dusty plasma medium has been investigated. In particular, the role of transverse shear and the compressional acoustic modes in both the linear and nonlinear regimes of the KH instability has been studied. It is observed that in addition to the conventional nonlocal KH instability, there exists a local instability in the strong coupling case. The interplay of the KH mode with this local instability shows up in the simulations as an interesting phenomenon of recurrence in the nonlinear regime. Thus, a cyclic KH instability process is observed to occur. These cyclic events are associated with bursts of activity in terms of transverse and compressional wave generation in the medium.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2016

Jeans instability in collisional strongly coupled dusty plasma with radiative condensation and polarization force

The influence of dust-neutral collisions, polarization force, and electron radiative condensation is analysed on the Jeans (gravitational) instability of partially ionized strongly coupled dusty plasma (SCDP) using linear perturbation (normal mode) analysis. The Boltzmann distributed ions, dynamics of inertialess electrons, charged dust and neutral particles are considered. Using the plane wave solutions, a general dispersion relation is derived which is modified due to the presence of dust-neutral collisions, strong coupling effect, polarization force, electron radiative condensation, and Jeans dust/neutral frequencies. In the long wavelength perturbations, the Jeans instability criterion depends upon strong coupling effect, polarization interaction parameter, and thermal loss, but it is independent of dust-neutral collision frequency. The stability of the considered configuration is analysed using the Routh–Hurwitz criterion. The growth rates of Jeans instability are illustrated, and stabilizing influence of viscoelasticity and dust-neutral collision frequency while destabilizing effect of electron radiative condensation, polarization force, and Jeans dust-neutral frequency ratio is observed. This work is applied to understand the gravitational collapse of SCDP with dust-neutral collisions.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗