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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 91 records · Page 5
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

BMS symmetry via AdS/CFT

With a view to understanding extended-BMS symmetries in the framework of the AdS 4 /CFT 3 correspondence, asymptotically AdS geometries are constructed with null impulsive shockwaves involving a discontinuity in superrotation parameters. The holographic dual is proposed to be a two-dimensional Euclidean defect conformal field localized on a particular timeslice in a three-dimensional conformal field theory on de Sitter spacetime. The defect conformal field theory generates a natural action of the Virasoro algebra. The large radius of curvature limit ℓ → ∞ yields spacetimes with nontrivial extended-BMS charges corresponding to a single set of Virasoro charges.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2020

Chaos and complementarity in de Sitter space

We consider small perturbations to a static three-dimensional de Sitter geometry. For early enough perturbations that satisfy the null energy condition, the result is a shockwave geometry that leads to a time advance in the trajectory of geodesics crossing it. This brings the opposite poles of de Sitter space into causal contact with each other, much like a traversable wormhole in Anti-de Sitter space. In this background, we compute out-of-time-order correlators (OTOCs) to asses the chaotic nature of the de Sitter horizon and find that it is maximally chaotic: one of the OTOCs we study decays exponentially with a Lyapunov exponent that saturates the chaos bound. We discuss the consequences of our results for de Sitter complementarity and inflation.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2022

Gluon-mediated inclusive Deep Inelastic Scattering from Regge to Bjorken kinematics

We revisit high energy factorization for gluon mediated inclusive Deep Inelastic Scattering (DIS) for which we propose a new semi-classical approach that accounts systematically for the longitudinal extent of the target in contrast with the shockwave limit. In this framework, based on a partial twist expansion, we derive a factorization formula that involves a new gauge invariant unintegrated gluon distribution which depends explicitly on the Feynman x variable. It is shown that both the Regge and Bjorken limits are recovered in this approach. We reproduce in particular the full one loop inclusive DIS cross-section in the leading twist approximation and the all-twist dipole factorization formula in the strict x = 0 limit. Although quantum evolution is not discussed explicitly in this work, we argue that the proper treatment of the x dependence of the gluon distribution encompasses the kinematic constraint that must be imposed on the phase-space of gluon fluctuations in the target to ensure stability of small-x evolution.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

Collisions of localized shocks and quantum circuits

We study collisions between localized shockwaves inside a black hole interior. We give a holographic boundary description of this process in terms of the overlap of two growing perturbations in a shared quantum circuit. The perturbations grow both exponentially as well as ballistically. Due to a competition between different physical effects, the circuit analysis shows dependence on the transverse locations and exhibits four regimes of qualitatively different behaviors. On the gravity side we study properties of the post-collision geometry, using exact calculations in simple setups and estimations in more general circumstances. We show that the circuit analysis offers intuitive and surprisingly accurate predictions about gravity computations involving non-linear features of general relativity.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2022

Collision of localized shocks in AdS 5 as a series expansion in transverse gradients

We introduce a computational framework to more efficiently calculate the collision of localized shocks in five dimensional asymptotically Anti-de Sitter space. We expand the Einstein equations in transverse gradients and find that our numerical results agree well with exact solutions already at first order in the expansion. Moreover, the Einstein equations at first order in transverse gradients can be decoupled into two sets of differential equations. Here, the bulk fields of one of these sets has only a negligible contribution to boundary observables, such that the computation on each time slice can be simplified to the solution of several planar shockwave equations plus four further differential equations for each transverse plane ‘pixel’. At the cost of errors of ≲ 10% at the hydrodynamization time and for low to mid rapidities, useful numerical solutions can be sped up by roughly one order of magnitude.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

Microstructure effects on high velocity microparticle impacts of copper

Constitutive models can fail to predict high-rate deformation behavior due to their inability to account for microstructural effects. In part, this is because of a dearth of experimental benchmarking data in the high strain-rate, low pressure regime, since many high-rate experiments also probe a region of strong shockwaves, at which point microstructure effects no longer play a primary role. This work uses laser-induced particle impact testing to quantitatively study high velocity impacts of small, rigid alumina microspheres on flat copper substrates with varying amounts of initial cold work in the weak shock regime, but at very high strain rates up to ~10 7 s –1 . Through paired experiments and numerical simulations, this work shows that the initial microstructure condition can have significant influence on dynamical mechanical properties in this range. Specifically, prior work hardening of the copper substrate leads to increased rebounding of the microparticles (i.e., less plastic dissipation in the impact) as well as smaller craters. Each of these experimental measurables can be converted into a strength measure, i.e., the dynamic yield strength or dynamic hardness, respectively, neither of which is well predicted consistently by existing constitutive laws. The general trend of hardening can be captured by such models by incorporating an existing “pre-strain,” suggesting that future calibration of the materials parameters may yield a good fit over a broader range of conditions. Our results emphasize the importance of reporting the microstructural condition in dynamic studies, as well as the necessity of accounting for these factors when formulating and optimizing constitutive models.

36 MATERIALS SCIENCE↗
DOE OSTI2026

From atomistic models to machine learning: Predictive design of nanocarbons under extreme conditions

The formation of technologically valuable nanocarbon structures under extreme conditions, such as those produced during high-explosive detonations, remains poorly understood but holds significant potential for the development of controlled synthesis pathways. While detonation shockwaves provide the high-pressure, high-temperature environment required for nanodiamond formation, subsequent cooling and decompression dictate whether the diamond phase is preserved or transformed into other nanocarbon structures. Here, in this study, we employ GPU-accelerated reactive molecular dynamics (ReaxFF) simulations to investigate the graphitization and structural remodeling of detonation nanodiamond under nonlinear quench and pressure-release trajectories. We further investigate how the initial nanodiamond morphology; cuboctahedral, octahedral, or hexagonal prism influences the resulting transformation products. Evolution of nanostructure, allotrope (via simulated x-ray diffraction), carbon hybridization, and ring statistics are tracked during a two-stage quench from 5000 K to 60 GPa. Rapid cooling combined with slow decompression optimizes cubic diamond retention, whereas slow cooling with rapid pressure release promotes surface-to-core graphitization, producing concentric sp 2 -hybridized layers and hollowed inner shells. Octahedral nanodiamonds evolve into carbon nano-onions, initially forming bucky diamonds that progressively transform into fully sp 2 -hybridized structures, while hexagonal prisms preferentially form parallel-stacked graphite layers resembling carbon dots. Transient hexagonal diamond (lonsdaleite) emerges as an interfacial phase, suggesting potential reversibility in the shock-induced graphite-to-diamond transformation pathway transformation route. To extend predictive capabilities, we trained machine learning (ML) regressors on over 10 5 node-hours of molecular dynamics (MD) trajectories. A multilayer perceptron (MLP) model reliably predicts the number of graphitized layers from temperature–pressure trajectories with a coefficient of determination (R 2 ) exceeding 0.90. This high predictive fidelity enables efficient, high-throughput mapping of the synthesis parameter space for optimized graphitization outcomes. Collectively, morphological control combined with optimized quench–decompression conditions promote the selective synthesis of nanocarbon allotropes. This work establishes a data-driven framework for the rational, a priori design of carbon nanomaterials for applications in energy storage, sensing, and biomedicine.

Detonation nanodiamond remodeling↗
DOE OSTI2024

Zircon-to-reidite phase transition enhanced by minor radiation damage: Implications for hypervelocity impacts

Reidite, a high-pressure phase of zircon, is increasingly identified at terrestrial impact sites. Despite its growing recognition, the potential applications for estimating minimum impact pressure face impediments due to existing discrepancies in the condition of zircon-reidite transformation, controversial models governing the transformation mechanism, and unclear effects of pre-existing radiation damage on reidite formation. Here, we show enhanced reidite formation by synchrotron X-ray diffraction, Raman spectroscopy, and transmission electron microscopy analyses of zircon grains that have experienced different alpha-decay doses from U and Th impurities and subsequent pressurization in diamond anvil cells. Below ~1 × 10 18 α-decay events/g, the α-decay-induced isolated point defects in the still crystalline zircon facilitate the minor atomic readjustments required for reidite formation. However, above this dose, the loss of long-range periodicity in severely damaged or even metamict zircon inhibits the transformation. The enhanced reidite formation by minor radiation damage coincides with the more common occurrence of reidite at impact sites for which the precursor zircon has a relatively lower alphadecay- event dose before the impact event. In addition, the detailed atomic-scale structures of twinned reidite provide unambiguous evidence for a characteristic internal stress-induced martensitic transition. Furthermore, these findings have important implications for interpreting the formation conditions of natural reidite due to the convergence of pressure from the static, shockwave, and natural reidite samples.

58 GEOSCIENCES↗
DOE OSTI2020

Reflected shock-initiated ignition probed via simultaneous lateral and endwall high-speed imaging with a transparent, cylindrical test-section

A TRAnsparent cylindrical (TRAC) shock tube test section has been developed to explore the ignition structure behind reflected shockwaves via simultaneous lateral and endwall high-speed imaging using three fuel/oxidizer mixtures: 0.1% n-C 7 H 16 /1.10% O 2 /4.14% N 2 /94.66% Ar, 0.1% iC 8 H 18 /1.25% O 2 /4.69% N 2 /93.96% Ar, and 5% CH 4 /10% O 2 /85% CO 2 . During mild ignition, the first exothermic centers were located outside of the observable test section. It is shown that with increasing temperature the far-wall ignition events move closer to the endwall, until a strong ignition is achieved. The temperature gradients that promote mild ignition were quantified and were found to have a slight dependence on fuel with the RMS temperature gradients being 0.80% for n-heptane and 1.07% for isooctane. The impact of temperature gradients on metrics used to improve kinetic models, such as species time histories, is noteworthy. From this temperature gradient, an experimental correlation is provided to estimate the transition temperature from mild to strong ignition for a mixture. The effect of diagnostic location in non-homogeneous reactions is quantified in reference to ignition delay. In conclusion, the unique and insightful perspective on the ignition process under heavy shock bifurcation is also discussed.

02 PETROLEUM↗
DOE OSTI2024

Shock compression of a low-density carbon foam

Porous polymer foams are found in numerous applications where they may be subjected to dynamic compression. The shockwave properties of polymer foams have several features that make shock Hugoniot measurements and interpretation challenging. Here, we present a comparison of dynamic X-ray phase contrast imaging and traditional optical velocimetry approaches to measuring the shocked states for a low-density carbon foam. Overall, dynamic X-ray phase contrast imaging was found to reduce errors associated with the measured Hugoniot states. In this study, the foam exhibits anomalous compression as expected due to its high initial porosity arising from shock heating.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Influence of Pore Surface Structure and Contents on Shock-Induced Collapse and Energy Localization

The majority of computational efforts in the shockwave driven collapse of porosity focus on idealized pore geometries and structures. These give significant insight into the physical mechanisms in play, but omit some potentially important effects of real energetic materials. Here, to address this, we simulate pore collapse in 1,3,5-triamino-2,4,6-trinitrobenzene (TATB) for four types of pore surfaces and fillings: an idealized cylindrical pore, a pore surface coated with polymer, a melted/amorphous pore surface, and a pore filled with gas molecules. We find that these perturbations to the pore structure result in only minor changes to the highly complex collapse mechanisms. However, significant differences in hotspot temperature are observed, with peak temperatures ranging over several hundred Kelvin. The polymer-coated system has the most effect, lowering the hotspot temperature by 300 K, and also limiting the manifestation of intramolecular strain energy that is known to induce mechanochemistry.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2021

A Hotspot’s Better Half: Non-Equilibrium Intra-Molecular Strain in Shock Physics

Shockwave interactions with a material’s microstructure localizes energy into hotspots, which act as nucleation sites for complex processes such as phase transformations and chemical reactions. To date, hotspots have been described via their temperature fields. Nonreactive, all-atom molecular dynamics simulations of shock-induced pore collapse in a molecular crystal show that more energy is localized as potential energy (PE) than can be inferred from the temperature field and that PE localization persists beyond thermal diffusion. Furthermore, the origin of the PE hotspot is traced to large intramolecular strains, storing energy in modes readily available for chemical decomposition.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Melting and density of MgSiO 3 determined by shock compression of bridgmanite to 1254GPa

The essential data for interior and thermal evolution models of the Earth and super-Earths are the density and melting of mantle silicate under extreme conditions. Here, we report an unprecedently high melting temperature of MgSiO 3 at 500 GPa by direct shockwave loading of pre-synthesized dense MgSiO3 (bridgmanite) using the Z Pulsed Power Facility. We also present the first high-precision density data of crystalline MgSiO 3 to 422 GPa and 7200 K and of silicate melt to 1254 GPa. The experimental density measurements support our density functional theory based molecular dynamics calculations, providing benchmarks for theoretical calculations under extreme conditions. The excellent agreement between experiment and theory provides a reliable reference density profile for super-Earth mantles. Furthermore, the observed upper bound of melting temperature, 9430 K at 500 GPa, provides a critical constraint on the accretion energy required to melt the mantle and the prospect of driving a dynamo in massive rocky planets.

58 GEOSCIENCES↗
DOE OSTI2022

Chemistry-mediated Ostwald ripening in carbon-rich C/O systems at extreme conditions

Abstract There is significant interest in establishing a capability for tailored synthesis of next-generation carbon-based nanomaterials due to their broad range of applications and high degree of tunability. High pressure (e.g., shockwave-driven) synthesis holds promise as an effective discovery method, but experimental challenges preclude elucidating the processes governing nanocarbon production from carbon-rich precursors that could otherwise guide efforts through the prohibitively expansive design space. Here we report findings from large scale atomistically-resolved simulations of carbon condensation from C/O mixtures subjected to extreme pressures and temperatures, made possible by machine-learned reactive interatomic potentials. We find that liquid nanocarbon formation follows classical growth kinetics driven by Ostwald ripening (i.e., growth of large clusters at the expense of shrinking small ones) and obeys dynamical scaling in a process mediated by carbon chemistry in the surrounding reactive fluid. The results provide direct insight into carbon condensation in a representative system and pave the way for its exploration in higher complexity organic materials. They also suggest that simulations using machine-learned interatomic potentials could eventually be employed as in-silico design tools for new nanomaterials.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2022

Traversable wormhole dynamics on a quantum processor

The holographic principle, theorized to be a property of quantum gravity, postulates that the description of a volume of space can be encoded on a lower-dimensional boundary. The anti-de Sitter (AdS)/conformal field theory correspondence or duality is the principal example of holography. The Sachdev–Ye–Kitaev (SYK) model of N >> 1 Majorana fermions has features suggesting the existence of a gravitational dual in AdS 2 , and is a new realization of holography. Here, we invoke the holographic correspondence of the SYK many-body system and gravity to probe the conjectured ER=EPR relation between entanglement and spacetime geometry through the traversable wormhole mechanism as implemented in the SYK model. A qubit can be used to probe the SYK traversable wormhole dynamics through the corresponding teleportation protocol. This can be realized as a quantum circuit, equivalent to the gravitational picture in the semiclassical limit of an infinite number of qubits. Here we use learning techniques to construct a sparsified SYK model that we experimentally realize with 164 two-qubit gates on a nine-qubit circuit and observe the corresponding traversable wormhole dynamics. Despite its approximate nature, the sparsified SYK model preserves key properties of the traversable wormhole physics: perfect size winding, coupling on either side of the wormhole that is consistent with a negative energy shockwave, a Shapiro time delay, causal time-order of signals emerging from the wormhole, and scrambling and thermalization dynamics. Our experiment was run on the Google Sycamore processor. By interrogating a two-dimensional gravity dual system, our work represents a step towards a program for studying quantum gravity in the laboratory. Future developments will require improved hardware scalability and performance as well as theoretical developments including higher-dimensional quantum gravity duals and other SYK-like models.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2021

Hidden order across online extremist movements can be disrupted by nudging collective chemistry

Disrupting the emergence and evolution of potentially violent online extremist movements is a crucial challenge. Extremism research has analyzed such movements in detail, focusing on individual- and movement-level characteristics. But are there system-level commonalities in the ways these movements emerge and grow? Here we compare the growth of the Boogaloos, a new and increasingly prominent U.S. extremist movement, to the growth of online support for ISIS, a militant, terrorist organization based in the Middle East that follows a radical version of Islam. We show that the early dynamics of these two online movements follow the same mathematical order despite their stark ideological, geographical, and cultural differences. The evolution of both movements, across scales, follows a single shockwave equation that accounts for heterogeneity in online interactions. These scientific properties suggest specific policies to address online extremism and radicalization. We show how actions by social media platforms could disrupt the onset and ‘flatten the curve’ of such online extremism by nudging its collective chemistry. Our results provide a system-level understanding of the emergence of extremist movements that yields fresh insight into their evolution and possible interventions to limit their growth.

99 GENERAL AND MISCELLANEOUS↗
DOE OSTI2024

Wee partons in QCD and gravity: Double copy and universality

We discuss a quantitative “double copy” between radiation from shockwave collisions in Einstein gravity and in QCD. The correspondence extends to 2 → N amplitudes in Regge asymptotics. The classicalization and unitarization of these amplitudes at maximal occupancy, corresponding to black hole and Color Glass Condensate (CGC) states respectively, are described by the emergent Goldstone dynamics of wee partons. We outline some consequences of the universal dynamics on both sides of the correspondence.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Laser-driven collisionless shock acceleration of ions from near-critical plasmas

Here, this paper overviews experimental and numerical results on acceleration of narrow energy spread ion beams by an electrostatic collisionless shockwave driven by 1 μm (Omega EP) and 10 μm (UCLA Neptune Laboratory) lasers in near critical density CH and He plasmas, respectively. Shock waves in CH targets produced high-energy ~50 MeV protons (ΔE/E of ≤30%) and 314 MeV C 6+ ions (ΔE/E of ≤10%). Observation of acceleration of both protons and carbon ions to similar velocities is consistent with reflection of particles off the moving potential of a shock front. For shocks driven by CO 2 laser in a gas jet, ~30 MeV peak in He ion spectrum was detected. Particle-in-cell simulations indicate that regardless of the target further control over its density profile is needed for optimization of accelerated ion beams in part of energy spread, yield and maximum kinetic energy.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗