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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 91 records · Page 5
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

Multinucleon transfer mechanism in Cf 250 + Th 232 collisions using the quantal transport description based on the stochastic mean-field approach

Production cross sections of heavy neutron-rich isotopes are calculated by employing quantal transport description in 250 Cf + 232 Th collisions. This quantal transport description is based on the stochastic mean-field approach, and it provides a microscopic approach beyond time-dependent Hartree-Fock theory to include mean-field fluctuations. Deexcitation of primary fragments is determined by employing the statistical GEMINI++ code. Here, calculations provide predictions for production cross sections of neutron rich transfermium isotopes without any adjustable parameters.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Multinucleon transfer mechanism in Gd 160 + W 186 collisions in stochastic mean-field theory

The multinucleon transfer mechanism in 160 Gd + 186 W collisions is investigated in the framework of quantal transport description, based on the stochastic mean-field (SMF) theory. The SMF theory provides a microscopic approach for nuclear dynamics beyond the time-dependent Hartree-Fock approach by including mean-field fluctuations. Finally, cross sections for the primary fragment production are determined in the quantal transport description and compared with the available data.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
NASA NTRS1989

Spectral evolution and cascade constant of solar wind Alfvenic turbulence

The theoretical model of Tu (1988) for the turbulent evolution of solar wind fluctuations assumed the constancy of the ratio alpha(1) between the energy in inward and outward propagating Alfven waves. Here, this model is extended to reflect the observed evolution in the propagation directions of the interplanetary fluctuations. The radial dependence of alpha(1) is determined by direct time domain correlations of the normalized cross helicity. The theoretical results match the observations at least as well as those of the previous, constant alpha(1), model. Measured values of alpha(1) are then used to find the value of the cascade constant that determines the overall level of the energy spectrum. The value of 1.25 for this constant is very close to the value observed in fluid turbulence if it is assumed that the correspondence between fluid and magnetofluid theories should be made for uncorrelated (zero cross helicity) MHD turbulence.

Tu, Chuan-Yi↗
NASA NTRS1992

Modeling orbital changes on tectonic time scales

Geologic time series indicate significant 100 ka and 400 ka pre-Pleistocene climate fluctuations, prior to the time of such fluctuations in Pleistocene ice sheets. The origin of these fluctuations must therefore depend on phenomena other than the ice sheets. In a previous set of experiments, we tested the sensitivity of an energy balance model to orbital insolation forcing, specifically focusing on the filtering effect of the Earth's geography. We found that in equatorial areas, the twice-yearly passage of the sun across the equator interacts with the precession index to generate 100 ka and 400 ka power in our modeled time series. The effect is proportional to the magnitude of land in equatorial regions. We suggest that such changes may reflect monsoonal variations in the real climate system, and the subsequent wind and weathering changes may transfer some of this signal to the marine record. A comparison with observed fluctuations of Triassic lake levels is quite favorable. A number of problems remain to be studied or clarified: (1) the EBM experiments need to be followed up by a limited number of GCM experiments; (2) the sensitivity to secular changes in orbital forcing needs to be examined; (3) the possible modifying role of sedimentary processes on geologic time series warrants considerably more study; (4) the effect of tectonic changes on Earth's rotation rate needs to be studied; and (5) astronomers need to make explicit which of their predictions are robust and geologists and astronomers have to agree on which of the predictions are most testable in the geologic record.

Crowley, Thomas J.↗
DOE OSTI2025

Detecting gravitational signatures of dark matter with atom gradiometers

We study the purely gravitational signatures of dark matter from the ultralight to the ultraheavy mass range in proposed long-baseline atom gradiometers, focusing on terrestrial designs, such as AION-km and MAGIS-km, as well as space-based concepts, such as MAGIS-space, AEDGE and AEDGE+. Due to its exceptional acceleration sensitivity and depending on astrophysical backgrounds, a detector similar to AEDGE+ could detect a dark matter subcomponent which constitutes 𝒪⁡(10%) of the local dark matter energy density and is populated by compact clumps of mass between 10 6 kg and 10 10 kg (10 −25 ⁢𝑀⊙ ≲ 𝑀 ≲10 −21⁢ 𝑀⊙) in an otherwise unexplored region of dark matter model space. Furthermore, because the gravitational observable depends on the relative gravitational time delay measured by spatially separated atomic clouds, we find that atom gradiometers are parametrically more sensitive than laser interferometers, such as LIGO and LISA, to fast-oscillating spacetime perturbations sourced by energy density and pressure fluctuations of ultralight dark matter. Depending on astrophysical backgrounds, a detector akin to AEDGE+ could probe a DM overdensity of 𝒪⁡(10) times the local dark matter energy density for masses 𝑚 ≲10 −17 eV.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2021

Enhanced Diffusive Transport in Fluctuating Porous Media

Mass transport within porous structures is a ubiquitous process in biological, geological, and technological systems. Despite the importance of these phenomena, there is no comprehensive theory that describes the complex and diverse transport behavior within porous environments. While the porous matrix itself is generally considered a static and passive participant, many porous environments are in fact dynamic, with fluctuating walls, pores that open and close, and dynamically changing cross-links. While diffusion has been measured in fluctuating structures, notably in model biological systems, it is rarely possible to isolate the effect of fluctuations because of the absence of control experiments involving an identical static counterpart, and it is generally impossible to observe the dynamics of the structure. In this paper, we present a direct comparison of the diffusion of nanoparticles of various sizes within a trackable, fluctuating porous matrix and a geometrically equivalent static matrix, in conditions spanning a range of regimes from obstructed to highly confined. The experimental system comprised a close-packed layer of colloidal spheres that were either immobilized to a planar surface or allowed to fluctuate locally, within the space defined by their nearest neighbors. Interestingly, the effective long-time diffusion coefficient was approximately 35–65% greater in the fluctuating porous matrix than in the static one (depending on the size of the nanoparticle probes), regardless of the geometric regime. This was explained by considering the enhancing effects of matrix fluctuations on the short-time diffusion coefficient and cooperative “gate-opening” motions of matrix particles and nanoparticle probes.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2022

An Online Dynamic Amplitude-Correcting Gradient Estimation Technique to Align X-ray Focusing Optics

High-brightness X-ray pulses, as generated at synchrotrons and X-ray free electron lasers (XFELs), are used in a variety of scientific experiments. At these facilities, measurements often require optical equipment, e.g Compound Refractive Lenses (CRLs) to be precisely aligned and focused. The lateral alignment of CRLs to a beamline requires precise positioning along four axes: two translational, and the two rotational. At a synchrotron, alignment is often accomplished manually. However, XFEL beamlines present a beam brightness that fluctuates stochastically, making manual alignment a time-consuming endeavor. Automation using simplex or classic stochastic descent often fails, given the errant gradient estimates. Herein we present a dynamic-amplitude correction to the usual gradient based on the combination of a generalized finite difference stencil and a time-dependent sampling pattern. Intensity is recorded periodically, then used to normalize numerical derivatives against fluctuations. Error expectation is analyzed, and efficacy is demonstrated on classic benchmarks. We provide a proof of concept by laterally aligning optics on a simulated XFEL beamline using data recorded at both synchrotron and XFEL facilities.

97 MATHEMATICS AND COMPUTING↗
NASA NTRS1998

The Role of Marangoni Convection for the FZ-Growth of Silicon

In growing crystals by the floating zone (FZ) technique under microgravity, the size restriction we have under earth conditions because of the hydrostatic pressure are avoided. Further, buoyancy related convection is eliminated to a high degree. But in the case of silicon, the gravity independent thermocapillary (Marangoni) convection is time-dependent even for small zone geometries. This has been demonstrated in several Technische Experimente unter Schwerelosigkeit (TEXUS) - technical experiments under reduced gravity) flights. Thus, to really take advantage of microgravity with respect to improve crystal quality, tools are required to control Marangoni convection in space facilities. Applying magnetic fields, convection can be influenced; fluid flow can either be damped (static magnetic fields) or overlaid by a regular flow regime (rotating magnetic fields). In floating zones of 8-10mm diameter and height (Ma approximately equals 6 x 10(exp 3)), a static magnetic field of about 2OOmT is sufficient to suppress time-dependent Marangoni convection to a high degree, but in dependence on the kind and the concentration of the added dopant, a new type of strongly pronounced dopant inhomogeneities have been detected. They are originated by thermoelectromagnetic convection. This can be avoided as well as detrimental effects on the radial dopant distribution by using rotating magnetic fields instead of static ones. Applying 75mT/50Hz to the FZ, the intensity of the dopant fluctuations is reduced to a high degree. Considering the rather low power consumption of rotating magnetic fields, this will be a useful tool for control or elimination of time-dependent Marangoni convection under microgravity. The strong time dependent character of thermocapillary flow and its influence on the temperature field has been measured in silicon half-zones for Marangoni numbers of Ma is approximately equal to 1-1.5 x 10(exp 4): temperature fluctuations up to 4C have been determined. Their frequency range was 0.1 and 0.4 Hz. Between certain thermocouple or sensor pairs, strong correlation has been detected.

Dold, P.↗
NASA NTRS1999

The Role of Marangoni Convection for the FZ-Growth of Silicon

Growing crystals by the floating zone (FZ) technique under microgravity avoids the size restriction we have under earth conditions due to hydrostatic pressure. Further, buoyancy related convection is eliminated to a great degree. But in the case of silicon, the gravity independent thermocapillary (Marangoni) convection is time-dependent even for small zone geometries. This has been demonstrated in several Technische Experimente unter Schwerelosigkeit (TEXUS) technical experiments under reduced gravity flights. Thus, to really take advantage of microgravity with respect to improved crystal quality, tools are required to control Marangoni convection in space facilities. With the application of magnetic fields, convection can be influenced; fluid flow can either be damped (static magnetic fields) or overlaid by a regular flow regime (rotating magnetic fields). In floating zones of 8-10 mm diameter and height (i.e., Ma is much greater than 6X 10(exp 3), a static magnetic field of about 2OOmT is sufficient to suppress time-dependent Marangoni convection to a high degree, but in dependence on the kind and the concentration of the added dopant, a new type of strongly pronounced dopant inhomogeneities have been detected. They are originated by thermoelectromagnetic convection. This can be avoided as well as detrimental effects on the radial dopant distribution by using rotating magnetic fields instead of static ones. Applying 7.5mT/5OHz to the FZ, the intensity of the dopant fluctuations is reduced to a high degree. Considering the rather low power consumption of rotating magnetic fields, this will be a useful tool for control or elimination of time-dependent Marangoni convection under microgravity. The strong time-dependent character of thermocapillary flow and its influence on the temperature field has been measured in silicon half-zones for Marangoni numbers of Ma is much greater than l - 1.5 X 10(exp 4): temperature fluctuations up to 4C have been determined, their frequency range was 0.4 and 0.4Hz. Between certain thermocouple or sensor pairs, strong correlation has been detected.

Dold, P.↗
DOE OSTI2020

Robust Distribution System Load Restoration With Time-Dependent Cold Load Pickup

Service restoration is one of the critical functions to enable the future self-healing distribution system. To restore the distribution system in a timely and reliable manner, the realistic system operating conditions need to be accurately characterized. Here, two main factors that have great impacts on distribution system restoration (DSR) in practice are investigated. First, cold load pickup (CLPU), generally caused by thermostatically controlled loads (TCLs), is a common phenomenon after an outage and shaped by the outage duration. However, the time-dependent behaviors of CLPU are rarely considered in literature. In this paper, the operating state evolution of TCLs after an outage is analyzed to characterize time-dependent CLPU. And the time-dependent CLPU is analytically embedded in DSR to accurately represent the actual behaviors of the restored loads. Second, it is difficult to predict loads that fluctuate during DSR due to the lack of real-time measurement data. Accordingly, a robust DSR based on the information gap decision theory (IGDT) is proposed to address this challenge, fully considering the uncertainty of CLPU. The proposed models are tested in IEEE 13-node and 123-node test feeders. Simulation results demonstrate that the time-dependent CLPU model and the uncertainty modeling of CLPU can accurately capture the actual behaviors of loads with TCLs after an outage, which greatly improves DSR decisions in practice.

24 POWER TRANSMISSION AND DISTRIBUTION↗
DOE OSTI2021

Implementation of an Experimental Setup Based on the Three-Omega Method for Thermal Conductivity Measurements of Molten Salts

Molten salt reactors (MSRs) are one of the most promising next-generation nuclear reactor designs which use molten salts as the fuel and coolant. To design, model, predict, license, and operate MSRs, the behavior of the fuel and coolant must be understood as a function of temperature and irradiation, i.e., burnup. Of particular importance and complexity is the reliable and reproducible measurement of thermal conductivity of molten salts at high temperatures (> 500 °C). Thermal conductivity provides information on the rate at which heat passes through a specified material and is dependent on chemical composition. Currently, in the national laboratory complex, several methods for measuring thermal conductivity on molten salt systems are under development, however, to date, consistent data have not been produced. Typically, thermal conductivity measurements of high-temperature melts have been conducted by using the Transient Hot Wire (THW) method where thermal conductivity is determined by the change in temperature over time at a certain distance from a heating wire. Another time-dependent technique is the laser flash method, commonly used for solid samples. Laser flash requires prior measurements of density and heat capacity to calculate the thermal conductivity of the sample, introducing additional measurement errors. Steady state and time-dependent measurements such as THW and laser flash have errors from convection and ambient temperature fluctuations (heat radiation). In order to produce high fidelity thermal conductivity data, a measurement technique needs to be developed that will reduce the effect of convection at high temperatures by measuring in a very fast time window. In addition, to measure on actinide and irradiated salts the sample size should be small. Therefore, this project aims to develop a frequency-domain technique based on the three-omega (3?) method, previously proven to work on solids, nanofluids and low temperature solar salts (25 to 250 °C). If the 3?-device can be designed with materials that can withstand high temperatures (>500 °C) and can be configured to reduce errors due to convection, then it would prove to be a valuable technique for ensuring thermal conductivity on molten salt systems needed for MSR development. For this proposal, the 3? instrument will be designed, assembled, and tested on non-radioactive salts before being used on actinide bearing salts. In addition, a thermal model will be developed to determine the thermal conductivity of the sample from the measured thermal oscillation of the sensor. Because 3? is a direct method that requires a small volume of sample and works in a very fast time window, it will aid in suppressing the interference due to convection which is ideal when working with high temperature liquid samples.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
NASA NTRS1995

Trajectory modeling of emissions from lower stratospheric aircraft

A series of isentropic trajectory calculations has been performed for emissions by stratospheric aircraft moving across the northern midlatitude oceanic flight corridors. Emission of exhaust is simulated by the daily initialization of air parcels along a flight path on the 500 K isentropic surface. Parcels are tracked during the first three weeks of each January from 1980 to 1994 in order to determine the interannual variability in the spatial distribution of the exhaust and the likelihood of exposure to cold temperatures. Few parcels emitted along these flight paths at this time of year had experienced nitric acid trihydrate (NAT) formation temperatures, except for the particularly cold Januarys 1986, 1987, and 1992. Large zonal fluctuations in the distribution of the emissions are typical for this time year and are strongly dependent on flight path. An extended 6-month (January-June) run in which parcels were released daily along the New York-London route shows that emissions in the flight corridor increase at a time-averaged rate which is nearly twice the rate at which the zonal average increases. In addition, local fluctuations of pollutant density can be several times higher than the zonal average and can persist for several weeks. A rapid buildup of emissions occurred during the summer months. These elevated emission levels must be considered in the interpretation of environmental impact assessments based on two-dimensional transport models.

Sparling, Lynn C.↗
DOE OSTI2025

Measurement of turbulent velocity and bounds for thermal diffusivity in laser shock compressed foams by x-ray photon correlation spectroscopy

Experimental benchmarking of transport coefficients under extreme conditions is required for validation of differing theoretical models. To date, measurement of transport properties of dynamically compressed samples remains a challenge with only a limited number of studies able to quantify transport in high pressure and temperature matter. x-ray photon correlation spectroscopy utilizes coherent x-ray sources to measure time correlations of density fluctuations, thus providing measurements of length and timescale-dependent transport properties. Here, we present a first-of-a-kind experiment to conduct x-ray photon correlation spectroscopy in laser shock compression experiments. We report measurement of the turbulent velocity in the wake of a laser driven supersonic shock and place an upper bound on thermal diffusivity in a solid density plasma on nanosecond timescales.

High-energy-density plasmas↗
NASA NTRS1974

Statistical time-dependent model for the interstellar gas

We present models for temperature and ionization structure of low, uniform-density (approximately 0.3 per cu cm) interstellar gas in a galactic disk which is exposed to soft X rays from supernova outbursts occurring randomly in space and time. The structure was calculated by computing the time record of temperature and ionization at a given point by Monte Carlo simulation. The calculation yields probability distribution functions for ionized fraction, temperature, and their various observable moments. These time-dependent models predict a bimodal temperature distribution of the gas that agrees with various observations. Cold regions in the low-density gas may have the appearance of clouds in 21-cm absorption. The time-dependent model, in contrast to the steady-state model, predicts large fluctuations in ionization rate and the existence of cold (approximately 30 K), ionized (ionized fraction equal to about 0.1) regions.

Gerola, H.↗
NASA NTRS2000

Star Formation in the Galaxy and the Fluctuating UV Radiation Field

We examine the formation of massive stars in the Galaxy, the resultant fluctuating UV radiation field, and the effect of this Field on the star-forming interstellar medium. Following previous researchers such as Habing (1968), we calculate the average interstellar radiation field at the Solar Circle of the Galaxy. However, our new calculations follow more closely the time dependence of the field at any point. We show that there is a significant difference between the mean field and the median field, and that there are substantial fluctuations of the field (on timescales of order 100 million years) at a given point. Far Ultraviolet Radiation (FUV, photon energies of 6 eV - 13.6 eV) has been recognized as the main source of heating of the neutral interstellar gas. Given the pressure of the interstellar medium (ISM) the FUV field determines whether the thermal balance of the neutral gas results in cold (T approximately 50 - 100 K) clouds (CNM), warm (T about 10,000 K) (WNM), for a combination of the two (the two phase ISM) We present results for the time history of the FUV field for points in the local ISM of the Milky Way Galaxy. The presence of this fluctuating heating rate converts CNM to WNM and vice versa. We show how to calculate the average fractions of the gas in the CNM and WNM when the interstellar gas is subject to this fluctuating FUV field. The knowledge of how these fractions depend on the gas properties (i.e. mean density and composition) and on the FUV-sources (i.e. the star formation rate, or the IMF, or the size distribution of associations) is a basic step in building any detailed model of the large scale behavior of the ISM and the mutual relation between the ISM and the SFR.

Hollenbach, David↗
DOE OSTI2021

Probing Quantum Speed Limits with Ultracold Gases

Here, quantum speed limits (QSLs) rule the minimum time for a quantum state to evolve into a distinguishable state in an arbitrary physical process. These fundamental results constrain a notion of distance traveled by the quantum state, known as the Bures angle, in terms of the speed of evolution set by nonadiabatic energy fluctuations. I theoretically propose how to measure QSLs in an ultracold quantum gas confined in a time-dependent harmonic trap. In this highly-dimensional system of continuous variables, quantum tomography is prohibited. Yet, QSLs can be probed whenever the dynamics is self-similar by measuring as a function of time the cloud size of the ultracold gas. This makes it possible to determine the Bures angle and energy fluctuations, as I discuss for various ultracold atomic systems.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
NASA NTRS2020

Desorption Kinetics of O and CO from Graphitic Carbon Surfaces

The desorption of O/CO from graphitic carbon surfaces is investigated using a one-dimensional model describing the adsorbate interactions with the surface phonon bath. The kinetics of desorption are described through the solution of a master equation for the time-dependent population of the adsorbate in an oscillator state, which is modified through thermal fluctuations at the surface. The interaction of the adsorbate with the surface phonons is explicitly captured by using the computed phonon density Of states (PDOS) of the surface. The coupling of the adsorbate with the phonon bath results in the transition of the adsorbate up and down a vibrational ladder. The adsorbate-surface interaction is represented in the model using a Morse potential, which allows for the desorption process to be directly modeled as a transition from bound to free (continuum) state. The PDOS is a property of the material and the lattice; and is highly sensitive to the presence of defects. The effect of etch pits along with random surface defects on the PDOS is considered in the present work. The presence of defects causes a redshift and broadening of the PDOS, which in turn changes the phonon frequency modes available for adsorbate coupling at the surface. Using the realistic PDOS distributions, the phonon-induced desorption (PID) model was used to compute the transition and desorption rates for both pristine and defective systems. Mathissen’s rule is used to compute the phonon relaxation time for pristine and defective systems based on the phonon scattering times for each of the different scattering processes. First, the desorption rates of the pristine system is fitted against the experimental values to obtain the Morse potential parameters for each of the observed adatoms. These Morse potential parameters are used along with the defective PDOS and phonon relaxation time to compute the desorption rates for the defective system. The defective system rates (both transition and desorption) were consistently lower in comparison with the pristine system. The difference between the transition rates is more significant at lower initial states due to higher energy spacing between the levels. In the case of the desorption rates, the difference between the defective and pristine system is more significant at higher temperatures. The desorption rates for each of the system shows an order of magnitude decrease with the strongly bound systems exhibiting the greatest reduction in the desorption rates.

Swaminathan-Gopalan, Krishnan↗
NASA NTRS1982

Time-dependent solutions of multimode convection equations

Truncated modal equations are used to study the time evolution of thermal convection. In the Boussinesq approximation these nonlinear equations are obtained by expanding the fluctuating velocity and temperature fields in a finite set of planforms of the horizontal coordinates. Numerical studies dealing with two or three modes with triad interactions are discussed. Rich time dependence was found in these cases: periodic and aperiodic solutions can be obtained, along with various steady solutions. Three-mode solutions reproduce the qualitative appearance of spoke-pattern convection as observed in experiments at high Prandtl numbers. Though the values of the periods of the time-dependent solutions do not agree with those of the experiments, their variation with Rayleigh number compares favorably. Except at the highest Rayleigh number considered (10,000,000), the theoretical Nusselt numbers agree well with experiment.

Toomre, J.↗