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SAGE III/ISS v5.3 Level 2 Data Product Changes and Improvements

The Stratospheric Aerosol and Gas Experiment on the International Space Station (SAGE III/ISS) is an occultation instrument that acquires measurements of aerosols and gases within the Earth’s stratosphere and upper troposphere. SAGE III/ISS provides level 2 solar species products for aerosol extinction (9 channels), nitrogen dioxide (NO2), ozone (O3), and water vapor (H2O). The level 2 products currently provide three O3 profiles based on differing retrievals. The first O3 profile is based on measurements at short wavelengths within the Hartley-Huggins band (MesO3), the second O3 profile is based on measurements made at visible wavelengths within the Chappius band (MLR O3), and the final profile is found using a more SAGE II like approach (AO3). The SAGE III/ISS also provides level 2 lunar species products for ozone (O3), nitrogen dioxide (NO2), and nitrogen trioxide (NO3). Version 5.3 of the SAGE III/ISS retrieval algorithm introduces improvements that affect the level 2 data products. The largest change to the solar algorithm is the implementation of disturbance monitoring package (DMP) corrections to improve pointing accuracy. The DMP is comprised of a miniature inertial measurement unit that measures rotation in inertial space using ring laser gyroscopes oriented about three orthogonal axes which can be used to correct pointing errors caused by mechanical disturbances. A major change common to solar and lunar algorithms is meteorological input from the coarser 42 level Modern-Era Retrospective analysis for Research and Applications, Version 2 (MERRA-2) model data to the 72 level MERRA-2 model data. The final major change involves improving the automated quality assurance (QA) algorithm to recover events that were withheld from the public release because differences between the AO3 and MLR O3 for some events after the eruption of Tonga–Hunga Haʻapai. Other changes for v5.3 include minor bug fixes as well as restoration of some data quality flags that were removed in v5.21. This presentation presents the impacts of these changes as well as overall observations of interest from v5.3 level 2 data products.

Carter Hulsey↗

SAGE III/ISS v5.3 Level 2 Data Product Changes and Improvements

The Stratospheric Aerosol and Gas Experiment on the International Space Station (SAGE III/ISS) is an occultation instrument that acquires measurements of aerosols and gases within the Earth’s stratosphere and upper troposphere. SAGE III/ISS provides level 2 solar species products for aerosol extinction (9 channels), nitrogen dioxide (NO2), ozone (O3), and water vapor (H2O). The level 2 products currently provide three O3 profiles based on differing retrievals. The first O3 profile is based on measurements at short wavelengths within the Hartley-Huggins band (MesO3), the second O3 profile is based on measurements made at visible wavelengths within the Chappius band (MLR O3), and the final profile is found using a more SAGE II like approach (AO3). The SAGE III/ISS also provides level 2 lunar species products for ozone (O3), nitrogen dioxide (NO2), and nitrogen trioxide (NO3). Version 5.3 of the SAGE III/ISS retrieval algorithm introduces improvements that affect the level 2 data products. The largest change to the solar algorithm is the implementation of disturbance monitoring package (DMP) corrections to improve pointing accuracy. The DMP is comprised of a miniature inertial measurement unit that measures rotation in inertial space using ring laser gyroscopes oriented about three orthogonal axes which can be used to correct pointing errors caused by mechanical disturbances. A major change common to solar and lunar algorithms is meteorological input from the coarser 42 level Modern-Era Retrospective analysis for Research and Applications, Version 2 (MERRA-2) model data to the 72 level MERRA-2 model data. The final major change involves improving the automated quality assurance (QA) algorithm to recover events that were withheld from the public release because differences between the AO3 and MLR O3 for some events after the eruption of Tonga–Hunga Haʻapai. Other changes for v5.3 include minor bug fixes as well as restoration of some data quality flags that were removed in v5.21. This presentation presents the impacts of these changes as well as overall observations of interest from v5.3 level 2 data products.

Carter Hulsey↗

Aerosol Thermodynamics (Aerosol Liquid Water Concentration and Aerosol pH) at S2 during CoURAGE

These data report aerosol liquid water content (ALWC) and aerosol pH for the S2 (Mt. Airy) site during CoURAGE for April - June 2025. The ISORROPIA-II aerosol thermodynamic equilibrium model was used to compute ALWC and pH. The model was run in forward mode, with solids formation disabled (metastable mode), according to Pye et al. (Atmospheric Chemistry and Physics, 2020). Information about the model can be found at https://www.epfl.ch/labs/lapi/models-and-software/isorropia/, and in Fountoukis and Nenes (Atmospheric Chemistry and Physics, 2007). Inputs to the model were: (1) measured Temperature and relative humidity, both from the DoE ARM “metwxt” data products at S2, (2) aerosol chemical composition from the ARM ACSM, and (3) gas-phase ammonia concentrations. For ISORROPIA-II, ambient RH values above 0.995 were input to the model as 0.995; therefore, caution should be exercised interpreting ALWC when RH was above 0.995. Aerosol composition or NH3(g) concentrations below the LOD were input into the model as 0.5*LOD. Model runs were only conducted for data points at 30-min resolution with all three inputs (meteorology, ACSM, and NH3). If any of the three model inputs were missing, aerosol thermodynamic outputs are flagged as -999. Similarly, aerosol thermodynamic outputs are flagged as -999 if measured NH3(g) and aerosol ammonium (NH4+) were simultaneously below the respective LODs. The ALWC includes liquid water from inorganic aerosol components, calculated directly by ISORROPIA-II, as well as liquid water from organics, estimated from the ACSM organics assuming a kappa value of 0.12 according to Guo et al. (Atmospheric Chemistry and Physics, 2015).

Aerosol Liquid Water Content↗

Cloud - Aerosol LIDAR Infrared Pathfinder Satellite Observations (CALIPSO) - Data Management System: Data Products Catalog V4.95

The CALIPSO V4.51 Lidar Level 1 and Level 2 data product is an updated version of an already order-able dataset. The changes were signed off by the CALIPSO Configuration Control Board, versioned, and the code uploaded to a code repository. There is no ITAR/SBU data or code associated with this product. Data will be publicly order-able at the NASA LaRC Atmospheric Sciences Data Center (ASDC). All documentation and web sites will be made public once the data product is released. The data is in HDF4 format and will be generated for majority of the mission (June 2006 - August 2023). The attached Data Products Catalog (v4.95) describes the content of these new data products.

Mark Vaughan↗

Creating Seasonal Climatologies of Aerosol Lidar Ratios Over Ocean Using MODIS AOD Constrained Retrievals and GOCART Model Simulations

The current CALIPSO algorithms assign one lidar ratio (i.e., extinction-to-backscatter ratio; LR) value globally for each of the seven tropospheric aerosol types. In a future data products release, the CALIPSO project aims to improve these algorithms through the development of regional and seasonal LR climatologies. In this work, aerosol LRs are inferred through CALIOP backscatter profiles constrained by collocated aerosol optical depth (AOD) from Aqua Moderate Resolution Imaging Spectroradiometer (MODIS) data. This analysis is subsampled for those profiles that are cloud-free and contain only one CALIOP-classified aerosol type (e.g., marine). The CALIOP profiles are then collocated with aerosol volume fractions obtained through Goddard Chemistry Aerosol Radiation and Transport (GOCART) model simulations. In this poster, we show twelve-year (June 2006-August 2018) mean spatial distributions of inferred aerosol LRs for CALIOP-classified marine aerosols and how they correspond inversely with patterns of GOCART sea salt volume fraction (SSVF). Near land masses, smaller SSVFs and larger LRs are found (due to the influence of over-land aerosols). In the remote ocean regions (likely less impacted by over-land aerosols), larger SSVFs and smaller LRs are found. The developed relationship between the GOCART model SSVFs and MODIS AOD constrained LRs is used to create model-assisted seasonal LR maps. Additionally, we show maps of inferred LRs from constrained retrievals using the CALIPSO Ocean Derived Column Optical Depth (ODCOD) product and comparisons with those from the MODIS analyses. The technique demonstrated here benefits CALIPSO in the near-term, but similar methods can also be applied to the next generation space-based elastic backscatter lidars with collocated passive sensors, such as those of the upcoming NASA Atmosphere Observing System (AOS).

Travis Toth↗

The Surface Longwave Downward Fluxes of the NASA GEWEX SRB Release 4.0 IP Products: Validation Against the Surface-Based BSRN and PMEL Observed Data

Since the NASA Global Energy Water Exchanges (GEWEX) Surface Radiation Budget (SRB) project released its 3rd version of products in 2010, the GEWEX Data Assessments Panel (GDAP) has been working on integrating various data products to address issues in the closing of the global energy and water cycles. The 4th version of the SRB products, Rel. 4.0-IP, has integrated data products from the cloud, aerosol, atmosphere, ocean surface, and land surface projects, coordinating within GDAP, to produce a long-term time series of TOA and surface radiative estimates. The Rel. 4-IP shortwave products span 34 years continuously from July 1983 to June 2017 on a quasi-equal-area 1degree longitude by 1degree latitude grid system. The longwave products are for land only from 1983-07 to 1987-12; for both land and ocean from 1988-01 to 2009-12; and ocean only from 2010-01 to 2017-06. The data are provided at 3 hourly, 3-hourly-monthly, daily and monthly means. The ISCCP HXS clouds and radiances are the key cloud input of the current GEWEX SRB algorithms. In addition, the longwave algorithm has also made changes in cloud microphysical property, surface skin temperature input, surface emissivity, atmospheric profile, adding longwave aerosol optical properties, revising cloud overlap procedure, and so on. Details of changes in both inputs and algorithms are documented in a NASA Algorithm Theoretical Basis Document (ATBD). We have validated the surface longwave downward fluxes against the surface-based Baseline Surface Radiation Network (BSRN) and the Pacific Marine Environmental Laboratory (PMEL) buoy data. As of 2020, the BSRN archive has 12,116 site-months of observed records from 73 stations on all seven continents, and as of 2017, PMEL archive has 4389 buoy months of observed records from 64 buoys deployed in the tropics of Pacific, Atlantic and Indian Oceans. This paper presents how the SRB Rel. 4.0-IP surface longwave downward fluxes compare with these surface-based measurements and how the comparison statistics differ from that of Rel. 3.0.

GEWEX SRB↗

Mapping Aerosol Lidar Ratios Over Ocean Using Constrained Retrievals and A Global Aerosol Model

The current NASA Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) algorithms assign one lidar ratio (i.e., extinction-to-backscatter ratio; LR) value globally for each of the seven tropospheric aerosol types. In a future data products release, the CALIPSO project aims to improve these algorithms through the development of regional and seasonal LR climatologies. In this work, aerosol LRs are inferred through Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) backscatter profiles constrained by collocated aerosol optical depth (AOD) from Aqua Moderate Resolution Imaging Spectroradiometer (MODIS) data. This analysis is subsampled for those profiles that are cloud-free and contain only one CALIOP-classified aerosol type (e.g., marine). The CALIOP profiles are then collocated with aerosol volume fractions obtained through Goddard Chemistry Aerosol Radiation and Transport (GOCART) model simulations. In this presentation, we show that the twelve-year (June 2006-August 2018) mean spatial distributions of inferred aerosol LRs for CALIOP-classified marine aerosols correspond inversely with patterns of GOCART sea salt volume fraction (SSVF). For example, smaller SSVFs (< 65%) and larger LRs (> 55 sr), are found near land masses. This is indicative of the influence of over-land aerosols (e.g., pollution and biomass burning smoke). In the remote oceans (i.e., regions likely less impacted by non-sea salt aerosols), larger SSVFs (> 95%) and smaller LRs (< 25 sr) are found. The developed relationship between the GOCART SSVFs and MODIS AOD constrained LRs (polynomial fit intersect values of ~56 sr for SSVF of 0% and ~21 sr for SSVF of 100%) is used to produce model-assisted climatological LR maps on seasonal scales. Additionally, we show maps of inferred LRs from constrained retrievals using the CALIPSO Ocean Derived Column Optical Depth (ODCOD) product and comparisons with those from the MODIS analyses. The technique demonstrated in this study not only benefits CALIPSO in the near-term, but similar methods can be applied to future spaceborne elastic backscatter lidars with collocated passive sensors, such as those associated with the upcoming NASA Atmosphere Observing System (AOS).

Travis Toth↗

Global Monitoring of Clouds and Aerosols Using a Network of Micro-Pulse Lidar Systems

Long-term global radiation programs, such as AERONET and BSRN, have shown success in monitoring column averaged cloud and aerosol optical properties. Little attention has been focused on global measurements of vertically resolved optical properties. Lidar systems are the preferred instrument for such measurements. However, global usage of lidar systems has not been achieved because of limits imposed by older systems that were large, expensive, and logistically difficult to use in the field. Small, eye-safe, and autonomous lidar systems are now currently available and overcome problems associated with older systems. The first such lidar to be developed is the Micro-pulse lidar System (MPL). The MPL has proven to be useful in the field because it can be automated, runs continuously (day and night), is eye-safe, can easily be transported and set up, and has a small field-of-view which removes multiple scattering concerns. We have developed successful protocols to operate and calibrate MPL systems. We have also developed a data analysis algorithm that produces data products such as cloud and aerosol layer heights, optical depths, extinction profiles, and the extinction-backscatter ratio. The algorithm minimizes the use of a priori assumptions and also produces error bars for all data products. Here we present an overview of our MPL protocols and data analysis techniques. We also discuss the ongoing construction of a global MPL network in conjunction with the AERONET program. Finally, we present some early results from the MPL network.

Welton, Ellsworth J.↗

Biomass Burning Aerosol Absorption Measurements with MODIS Using the Critical Reflectance Method

This research uses the critical reflectance technique, a space-based remote sensing method, to measure the spatial distribution of aerosol absorption properties over land. Choosing two regions dominated by biomass burning aerosols, a series of sensitivity studies were undertaken to analyze the potential limitations of this method for the type of aerosol to be encountered in the selected study areas, and to show that the retrieved results are relatively insensitive to uncertainties in the assumptions used in the retrieval of smoke aerosol. The critical reflectance technique is then applied to Moderate Resolution Imaging Spectrometer (MODIS) data to retrieve the spectral aerosol single scattering albedo (SSA) in South African and South American 35 biomass burning events. The retrieved results were validated with collocated Aerosol Robotic Network (AERONET) retrievals. One standard deviation of mean MODIS retrievals match AERONET products to within 0.03, the magnitude of the AERONET uncertainty. The overlap of the two retrievals increases to 88%, allowing for measurement variance in the MODIS retrievals as well. The ensemble average of MODIS-derived SSA for the Amazon forest station is 0.92 at 670 nm, and 0.84-0.89 for the southern African savanna stations. The critical reflectance technique allows evaluation of the spatial variability of SSA, and shows that SSA in South America exhibits higher spatial variation than in South Africa. The accuracy of the retrieved aerosol SSA from MODIS data indicates that this product can help to better understand 44 how aerosols affect the regional and global climate.

Zhu, Li↗

Aerosol Measurements by the Globally Distributed Micro Pulse Lidar Network

Full time measurements of the vertical distribution of aerosol are now being acquired at a number of globally distributed MP (micro pulse) lidar sites. The MP lidar systems provide full time profiling of all significant cloud and aerosol to the limit of signal attenuation from compact, eye safe instruments. There are currently eight sites in operation and over a dozen planned. At all sited there are also passive aerosol and radiation measurements supporting the lidar data. Four of the installations are at Atmospheric Radiation Measurement program sites. The network operation includes instrument operation and calibration and the processing of aerosol measurements with standard retrievals and data products from the network sites. Data products include optical thickness and extinction cross section profiles. Application of data is to supplement satellite aerosol measurements and to provide a climatology of the height distribution of aerosol. The height distribution of aerosol is important for aerosol transport and the direct scattering and absorption of shortwave radiation in the atmosphere. Current satellite and other data already provide a great amount of information on aerosol distribution, but no passive technique can adequately resolve the height profile of aerosol. The Geoscience Laser Altimeter System (GLAS) is an orbital lidar to be launched in early 2002. GLAS will provide global measurements of the height distribution of aerosol. The MP lidar network will provide ground truth and analysis support for GLAS and other NASA Earth Observing System data. The instruments, sites, calibration procedures and standard data product algorithms for the MPL network will be described.

Spinhirne, James↗

Absorption Properties of Mediterranean Aerosols Obtained from Multi-year Ground-based and Satellite Remote Sensing Observations

Aerosol absorption properties are of high importance to assess aerosol impact on regional climate. This study presents an analysis of aerosol absorption products obtained over the Mediterranean Basin or land stations in the region from multi-year ground-based AERONET and satellite observations with a focus on the Absorbing Aerosol Optical Depth (AAOD), Single Scattering Albedo (SSA) and their spectral dependence. The AAOD and Absorption Angstrom Exponent (AAE) data set is composed of daily averaged AERONET level 2 data from a total of 22 Mediterranean stations having long time series, mainly under the influence of urban-industrial aerosols and/or soil dust. This data set covers the 17 yr period 1996-2012 with most data being from 2003-2011 (approximately 89 percent of level-2 AAOD data). Since AERONET level-2 absorption products require a high aerosol load (AOD at 440 nm greater than 0.4), which is most often related to the presence of desert dust, we also consider level-1.5 SSA data, despite their higher uncertainty, and filter out data with an Angstrom exponent less than 1.0 in order to study absorption by carbonaceous aerosols. The SSA data set includes both AERONET level-2 and satellite level-3 products. Satellite-derived SSA data considered are monthly level 3 products mapped at the regional scale for the spring and summer seasons that exhibit the largest aerosol loads. The satellite SSA dataset includes the following products: (i) Multi-angle Imaging SpectroRadiometer (MISR) over 2000-2011, (ii) Ozone Monitoring Instrument (OMI) near-UV algorithm over 2004-2010, and (iii) MODerate resolution Imaging Spectroradiometer (MODIS) Deep-Blue algorithm over 2005-2011, derived only over land in dusty conditions. Sun-photometer observations show that values of AAOD at 440 nm vary between 0.024 +/- 0.01 (resp. 0.040 +/- 0.01) and 0.050 +/- 0.01 (0.055 +/- 0.01) for urban (dusty) sites. Analysis shows that the Mediterranean urban-industrial aerosols appear "moderately" absorbing with values of SSA close to approximately 0.94-0.95 +/- 0.04 (at 440 nm) in most cases except over the large cities of Rome and Athens, where aerosol appears more absorbing (SSA approximately 0.89-0.90 +/- 0.04). The aerosol Absorption Angstrom Exponent (AAE, estimated using 440 and 870 nm) is found to be larger than 1 for most sites over the Mediterranean, a manifestation of mineral dust (iron) and/or brown carbon producing the observed absorption. AERONET level-2 sun-photometer data indicate the existence of a moderate East-West gradient, with higher values over the eastern basin (AAEEast. = 1.39/AAEWest. = 1.33) due to the influence of desert dust. The North-South AAE gradient is more pronounced, especially over the western basin. Our additional analysis of AERONET level-1.5 data also shows that organic absorbing aerosols significantly affect some Mediterranean sites. These results indicate that current climate models treating organics as nonabsorbing over the Mediterranean certainly underestimate the warming effect due to carbonaceous aerosols. A~comparative analysis of the regional SSA variability has been attempted using satellite data. OMI and MODIS data show an absorbing zone (SSA approximately 0.90 at 470-500 nm) over Northeastern Africa that does not appear in the MISR retrievals. In contrast, MISR seems able to observe the East-West SSA gradient during summer, as also detected by AERONET. Also, the analysis of SSA provided by satellites indicates that the aerosol over the Mediterranean Sea appears less absorbing during spring (MAM) than summer (JJA).

satellite remote sensing observations↗

GEWEX (Global Energy and Water Exchanges Project): Surface Radiation Budget (SRB) Release 4 Integrated Product (IP4) - Algorithm Theoretical Basis Document and Evaluation

The World Climate Research Programme’s (WCRP) Global Energy and Water Exchanges (GEWEX) program is an integrated program of research, observations, and science activities with the mission to “Observe, understand and model the hydrological cycle and energy fluxes in the Earth’s atmosphere and at the surface.” Since the public release in 2010 of SRB Release 3, GEWEX reorganized to formulate the Data and Assessments Panel (GDAP) aimed at performing community assessments of the long-term global data products with focus on integrating various data products to address issues in the closing of the global energy and water cycles. SRB Release 4 Intergrated Product (Rel4-IP) integrates data products from the cloud, aerosol, atmosphere, ocean surface, and land surface projects within GDAP to produce a long-term time series of Top-of-Atmosphere (TOA) and surface radiative estimates. This Algorithm Theoretical Basis Document (ATBD) describes the various inputs, algorithms and resulting top-of-atmosphere and surface flux products that span from July 1983 through June 2017. Comparisons of the TOA flux products are made to overlapping CERES data products when possible. The surface radiative flux products are assessed relative to the globally distribution Baseline Surface Radiation Network measurements sites. Variability of the various products are compared to ERBE and CERES during overlapping time periods. The variability of the product show excellent correspondent to CERES during overlap years and improved statistical agreement with surface measurements. This document also discusses known issues with the data products to help the user understand the uncertainty and known issues.

Surface radiation budget↗

Large Scale Covariability in the Aerosol-SST-Precipitation Relation: A Satellite Perspective

Although large scale aerosol effects on precipitation have attracted increasing attention in recent years, significant uncertainties still remain in the current understanding of'such effects. One of the factors contributing to these uncertainties is the availability of aerosol data sets that are sufficiently long, stable, and comprehensive to be used for climate analysis. Such data sets are crucial for any long-term studies that are needed to demonstrate the statistical significance of large scale aerosol effects on precipitation when compared to the effects from other climate factors, such as remote or local sea surface temperature (SST) variability (ENSO. etc.). A longterm consistent aerosol product that complements the existing MODIS and AVHRR aerosol products is therefore needed to minimize aerosol data uncertainty issues for such Studies. The SeaWiFS instrument was primarily designed to measure ocean color, and it has been the mayor source for providing a comprehensive global data set of such measurements since its launch in 1997. Besides being used in this capacity, however, the well-calibrated set of radiances measured in the wavelength range from the visible (0.41 m) to the near infrared (0.87 m) is also well suited to creating long-term climate data records of aerosols. Recently, a new 13-year SeaWiFS aerosol optical depth dataset has been developed that expands its capacity to be used for such atmospheric studies. This SeaWiFS aerosol product provides us with an unprecedented opportunity to examine the covariability of aerosol, SST and precipitation on both a regional and global scale. We also use concurrent independent SST (NOAA Optimum Interpolation, OI, SST V2) and precipitation (GPCP V2) datasets for this study. We will present and discuss results from this study over several aerosol hot spot regions ( -,North Atlantic. South Atlantic, Western Pacific, Indian Ocean etc.) during the SeaWIFS data period (1997 -- current) from this study will be presented and discussed. These results will highlight the value and impact of this unique product to climate studies

Hsu, N. Christina↗

Global distribution of SAGE II data products

Techniques employed to map the global distribution of stratospheric aerosols using SAGE II data at four wavelengths (385, 453, 525 and 1020 microns) are described. The methods were devised to integrate the 900 data points scanned by the instrument with account taken of the different times the vertical profiles were obtained. The data have been used to calculate the O3, H2O, NO2 and aerosol optical thicknesses. Sample details of data gathered during April 1985 are discussed, with emphasis on difficulties being encountered in analyzing the differences being observed in the dawn and dusk data.

Rind, D.↗

Atmospheric Measurements by the 2002 Geoscience Laser Altimeter System Mission

The NASA Earth Observing System (EOS) program is a multiple platform NASA initiative for the study of global change. As part of the EOS project, the Geoscience Laser Altimeter System (GLAS) was selected as a laser sensor filling complementary requirements for several earth science disciplines including atmospheric and surface applications. Late in 2002, the GaAs instrument is to be launched for a three to five year observational mission. For the atmosphere, the instrument is designed to full fill comprehensive requirements for profiling of radiatively significant cloud and aerosol. Algorithms have been developed to process the cloud and aerosol data and provide standard data products. After launch there will be a three-month project to analyze and understand the system performance and accuracy of the data products. As an EOS mission, the GaAs measurements and data products will be openly available to all investigators. An overview of the instrument, data products and evaluation plan is given.

Spinhirne, James D.↗

Assessment of urban aerosol pollution over the Moscow megacity by the MAIAC aerosol product

We estimated the distribution of aerosol optical thickness (AOT) with a spatial resolution of 1 km over the Moscow megacity using the MAIAC aerosol product based on MODIS satellite data (Lyapustin et al., 2018) for the warm period of the year (May–September, 2001–2017). AERONET (Aerosol Robotic Network)-based validation of satellite estimates near the city centre at Moscow_MSU_MO and over the Moscow suburbs at Zvenigorod revealed that MAIAC AOT at 0.47 μm is in agreement with AERONET AOT though underestimated by 0.05–0.1 for AOT < 1 and overestimated for smoke conditions with AOT > 1. The MAIAC AOT biases were almost the same for the Moscow_MSU_MO and Zvenigorod AERONET sites, which indicated that the MAIAC algorithm effectively removed the effect of the bright urban surface in the city centre. For the ground-based measurements, the difference between annual median AOT at Moscow_MO_MSU and Zvenigorod (∆AOT) varied within -0:002 to +0:03, with statistically significant positive bias for most years, and an average ∆AOT was about 0.02. According to the MAIAC dataset, the ∆AOT varied within ±0:01 and was not statistically significant. The ∆AOT started decreasing recently due to intensive urban development of the territory around Zvenigorod and the decrease in pollutant emissions in Moscow, which is mainly caused by the environmental regulations. According to the MAIAC dataset, the most pronounced spatial AOT differences over the territory of Moscow were observed at the 5% quantile level, where they reached 0.05–0.06 over several locations and could be attributed to the stationary sources of aerosol pollution, for example, large areas of construction sites, aerosol pollution from roads and highways, or agriculture activities. The differences between the maximum and the mean AOT for different quantiles, except the 95% quantile, within the Moscow region, were about 0.02–0.04, which could be attributed to the local aerosol sources. The application of the MAIAC algorithm over the whole Moscow region has revealed a decreasing AOT trend over the centre of Moscow and an increasing trend over the “New” Moscow territory which experienced an intensive build-up and agricultural development.

urban aerosol pollution↗

Mapping Aerosol Lidar Ratios Over Ocean for CALIPSO Using Modis AOD-Constrained Retrievals and A Global Aerosol Model

The CALIPSO aerosol algorithms currently assign one lidar ratio value for each of the seven tropospheric aerosol types. In a future data products release, the CALIPSO project aims to improve these algorithms by developing regional and seasonal lidar ratio climatologies. In this study, aerosol lidar ratios are inferred through Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) backscatter profiles constrained by collocated aerosol optical depth from Aqua Moderate Resolution Imaging Spectroradiometer (MODIS) datasets. The analysis is subsampled for only those profiles that are cloud-free and contain one aerosol type (based on CALIOP feature classification). In addition, the CALIOP profiles are collocated with aerosol volume fractions simulated by the Goddard Chemistry Aerosol Radiation and Transport (GOCART) model. In this talk, the twelve-year (2006-2017) mean spatial distributions of inferred aerosol lidar ratios for CALIOP-classified marine aerosols and the corresponding modeled sea salt volume fractions (SSVF) will be shown. Model-assisted climatological lidar ratio maps on a seasonal scale will also be presented, developed from the empirical relationship found between the modeled SSVF and lidar ratios. A comparison with past studies will be provided as well as results of a sensitivity study regarding the variability of retrieved lidar ratios as a function of horizontal averaging resolution. While the majority of this talk will focus on lidar ratios for CALIOP-classified marine aerosols, preliminary results will be shown for other aerosol types over ocean, such as dust and elevated smoke.

Travis Toth↗