Search NASA⌕ Search

SEARCH · Search NASA

Results for “aerosol optical depth”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.

At least 91 records · Page 5

Airborne Sunphotometry of Aerosol Optical Depth and Columnar Water Vapor During ACE-Asia

During the Intensive Field Campaign (IFC) of the Aerosol Characterization Experiment - Asia (ACE-Asia), March-May 2001, the 6-channel NASA Ames Airborne Tracking Sunphotometer (AATS-6) operated during 15 of the 19 research flights aboard the NCAR C- 130, while its 14-channel counterpart (AATS- 14) was flown successfully on all 18 research flights of a Twin Otter aircraft operated by the Center for Interdisciplinary Remotely Piloted Aircraft Studies (CIRPAS), Monterey, CA. ACE-Asia was the fourth in a series of aerosol characterization experiments and focused on aerosol outflow from the Asian continent to the Pacific basin. Each ACE was designed to integrate suborbital and satellite measurements and models so as to reduce the uncertainty in calculations of the climate forcing due to aerosols. The Ames Airborne Tracking Sunphotometers measured solar beam transmission at 6 (380-1021 nm, AATS-6) and 14 wavelengths (353-1558 nm, AATS-14) respectively, yielding aerosol optical depth (AOD) spectra and column water vapor (CWV). Vertical differentiation in profiles yielded aerosol extinction and water vapor concentration. The wavelength dependence of AOD and extinction indicates that supermicron dust was often a major component of the aerosol. Frequently this dust-containing aerosol extended to high altitudes. For example, in data flights analyzed to date 34 +/- 13% of full-column AOD(525 nm) was above 3 km. In contrast, only 10 +/- 4% of CWV was above 3 km. In this paper, we will show first sunphotometer-derived results regarding the spatial variation of AOD and CWV, as well as the vertical distribution of aerosol extinction and water vapor concentration. Preliminary comparison studies between our AOD/aerosol extinction data and results from: (1) extinction products derived using in situ measurements and (2) AOD retrievals using the Multi-angle Imaging Spectro-Radiometer (MISR) aboard the TERRA satellite will also be presented.

Redemann, Jens↗

Aerosol Optical Properties Derived from the DRAGON-NE Asia Campaign, and Implications for a Single-Channel Algorithm to Retrieve Aerosol Optical Depth in Spring from Meteorological Imager (MI) On-Board the Communication, Ocean, and Meteorological Satellite (COMS)

An aerosol model optimized for northeast Asia is updated with the inversion data from the Distributed Regional Aerosol Gridded Observation Networks (DRAGON)-northeast (NE) Asia campaign which was conducted during spring from March to May 2012. This updated aerosol model was then applied to a single visible channel algorithm to retrieve aerosol optical depth (AOD) from a Meteorological Imager (MI) on-board the geostationary meteorological satellite, Communication, Ocean, and Meteorological Satellite (COMS). This model plays an important role in retrieving accurate AOD from a single visible channel measurement. For the single-channel retrieval, sensitivity tests showed that perturbations by 4 % (0.926 +/- 0.04) in the assumed single scattering albedo (SSA) can result in the retrieval error in AOD by over 20 %. Since the measured reflectance at the top of the atmosphere depends on both AOD and SSA, the overestimation of assumed SSA in the aerosol model leads to an underestimation of AOD. Based on the AErosol RObotic NETwork (AERONET) inversion data sets obtained over East Asia before 2011, seasonally analyzed aerosol optical properties (AOPs) were categorized by SSAs at 675 nm of 0.92 +/- 0.035 for spring (March, April, and May). After the DRAGON-NE Asia campaign in 2012, the SSA during spring showed a slight increase to 0.93 +/- 0.035. In terms of the volume size distribution, the mode radius of coarse particles was increased from 2.08 +/- 0.40 to 2.14 +/- 0.40. While the original aerosol model consists of volume size distribution and refractive indices obtained before 2011, the new model is constructed by using a total data set after the DRAGON-NE Asia campaign. The large volume of data in high spatial resolution from this intensive campaign can be used to improve the representative aerosol model for East Asia. Accordingly, the new AOD data sets retrieved from a single-channel algorithm, which uses a precalculated look-up table (LUT) with the new aerosol model, show an improved correlation with the measured AOD during the DRAGON-NE Asia campaign. The correlation between the new AOD and AERONET value shows a regression slope of 1.00, while the comparison of the original AOD data retrieved using the original aerosol model shows a slope of 1.08. The change of y-offset is not significant, and the correlation coefficients for the comparisons of the original and new AOD are 0.87 and 0.85, respectively. The tendency of the original aerosol model to overestimate the retrieved AOD is significantly improved by using the SSA values in addition to size distribution and refractive index obtained using the new model.

Kim, M.↗

Validating MODIS Above-Cloud Aerosol Optical Depth Retrieved from Color Ratio Algorithm Using Direct Measurements Made by NASA's Airborne AATS and 4STAR Sensors

We present the validation analysis of above-cloud aerosol optical depth (ACAOD) retrieved from the color ratio method applied to MODIS cloudy-sky reflectance measurements using the limited direct measurements made by NASAs airborne Ames Airborne Tracking Sunphotometer (AATS) and Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research (4STAR) sensors. A thorough search of the airborne database collection revealed a total of five significant events in which an airborne sun photometer, coincident with the MODIS overpass, observed partially absorbing aerosols emitted from agricultural biomass burning, dust, and wildfires over a low-level cloud deck during SAFARI-2000, ACE-ASIA 2001, and SEAC4RS 2013 campaigns, respectively. The co-located satellite-airborne match ups revealed a good agreement (root-mean-square difference less than 0.1), with most match ups falling within the estimated uncertainties associated with the MODIS retrievals (about -10 to +50 ). The co-retrieved cloud optical depth was comparable to that of the MODIS operational cloud product for ACE-ASIA and SEAC4RS, however, higher by 30-50% for the SAFARI-2000 case study. The reason for this discrepancy could be attributed to the distinct aerosol optical properties encountered during respective campaigns. A brief discussion on the sources of uncertainty in the satellite-based ACAOD retrieval and co-location procedure is presented. Field experiments dedicated to making direct measurements of aerosols above cloud are needed for the extensive validation of satellite based retrievals.

airborne sun photometer↗

Aerosol optical depth and planetary Albedo in the visible from the Solar Mesosphere Explorer

The Solar Mesosphere Explorer (SME) satellite has observed the visible sunlight scattered at the earth's limb since early 1982. By using a radiative-transfer model including multiple scattering and albedo effects, observations at 20 deg N latitude have been interpreted in terms of aerosol optical depth. The ratio of aerosol extinction to Rayleigh extinction at 431.8 nm shows a large increase after the eruption of El Chichon. A maximum ratio of 5 at 36 km and larger than 11 at 30 km occurred in the summer of 1982 followed by a decrease through 1983 and 1984. Aspects of the aerosol time evolution appear to be consistent with other observations and model predictions. Quantitative differences exist between inferred SME and lidar extinction coefficients, possibly due to the different wavelengths of the measurements and to the different scattering phase functions used in the two analyses. It is also shown that visible limb radiances provide information on the planetary albedo, which shows an increase from the equator to the poles with a maximum in the winter hemisphere and a minimum in the summer hemisphere.

Naudet, J. P.↗

A 4-D Climatology (1979-2009) of the Monthly Tropospheric Aerosol Optical Depth Distribution over the Mediterranean Region from a Comparative Evaluation and Blending of Remote Sensing and Model Products

Since the 1980s several spaceborne sensors have been used to retrieve the aerosol optical depth (AOD) over the Mediterranean region. In parallel, AOD climatologies coming from different numerical model simulations are now also available, permitting to distinguish the contribution of several aerosol types to the total AOD. In this work, we perform a comparative analysis of this unique multiyear database in terms of total AOD and of its apportionment by the five main aerosol types (soil dust, seasalt, sulfate, black and organic carbon). We use 9 different satellite-derived monthly AOD products: NOAA/AVHRR, SeaWiFS (2 products), TERRA/MISR, TERRA/MODIS, AQUA/MODIS, ENVISAT/MERIS, PARASOL/POLDER and MSG/SEVIRI, as well as 3 more historical datasets: NIMBUS7/CZCS, TOMS (onboard NIMBUS7 and Earth- Probe) and METEOSAT/MVIRI. Monthly model datasets include the aerosol climatology from Tegen et al. (1997), the climate-chemistry models LMDz-OR-INCA and RegCM-4, the multi-model mean coming from the ACCMIP exercise, and the reanalyses GEMS and MACC. Ground-based Level- 2 AERONET AOD observations from 47 stations around the basin are used here to evaluate the model and satellite data. The sensor MODIS (on AQUA and TERRA) has the best average AOD scores over this region, showing a relevant spatio-temporal variability and highlighting high dust loads over Northern Africa and the sea (spring and summer), and sulfate aerosols over continental Europe (summer). The comparison also shows limitations of certain datasets (especially MERIS and SeaWiFS standard products). Models reproduce the main patterns of the AOD variability over the basin. The MACC reanalysis is the closest to AERONET data, but appears to underestimate dust over Northern Africa, where RegCM-4 is found closer to MODIS thanks to its interactive scheme for dust emissions. The vertical dimension is also investigated using the CALIOP instrument. This study confirms differences of vertical distribution between dust aerosols showing a large vertical spread, and other continental and marine aerosols which are confined in the boundary layer. From this compilation, we propose a 4-D blended product from model and satellite data, consisting in monthly time series of 3-D aerosol distribution at a 50 km horizontal resolution over the Euro-Mediterranean marine and continental region for the 2003-2009 period. The product is based on the total AOD from AQUA/MODIS, apportioned into sulfates, black and organic carbon from the MACC reanalysis, and into dust and sea-salt aerosols from RegCM-4 simulations, which are distributed vertically based on CALIOP climatology.We extend the 2003-2009 reconstruction to the past up to 1979 using the 2003-2009 average and applying the decreasing trend in sulfate aerosols from LMDz-OR-INCA, whose AOD trends over Europe and the Mediterranean are median among the ACCMIP models. Finally optical properties of the different aerosol types in this region are proposed from Mie calculations so that this reconstruction can be included in regional climate models for aerosol radiative forcing and aerosol-climate studies.

troposphere↗

Application of Spectral Analysis Techniques in the Intercomparison of Aerosol Data: 1. an EOF Approach to the Spatial-Temporal Variability of Aerosol Optical Depth Using Multiple Remote Sensing Data Sets

Many remote sensing techniques and passive sensors have been developed to measure global aerosol properties. While instantaneous comparisons between pixel-level data often reveal quantitative differences, here we use Empirical Orthogonal Function (EOF) analysis, also known as Principal Component Analysis, to demonstrate that satellite-derived aerosol optical depth (AOD) data sets exhibit essentially the same spatial and temporal variability and are thus suitable for large-scale studies. Analysis results show that the first four EOF modes of AOD account for the bulk of the variance and agree well across the four data sets used in this study (i.e., Aqua MODIS, Terra MODIS, MISR, and SeaWiFS). Only SeaWiFS data over land have slightly different EOF patterns. Globally, the first two EOF modes show annual cycles and are mainly related to Sahara dust in the northern hemisphere and biomass burning in the southern hemisphere, respectively. After removing the mean seasonal cycle from the data, major aerosol sources, including biomass burning in South America and dust in West Africa, are revealed in the dominant modes due to the different interannual variability of aerosol emissions. The enhancement of biomass burning associated with El Niño over Indonesia and central South America is also captured with the EOF technique.

variability↗

Estimation of Aerosol Optical Depth, Pressure Elevation, Water Vapor and Calculation of Apparent Surface Reflectance from Radiance Measured by the Airborne Visible/Infrared Imaging Spectrometer (AVIRIS) Using a Radiative Transfer Code

The Airborne Visible/Infrared Imaging Spectrometer (AVIRIS) is an imaging spectrometer that measures spatial images of the total up welling spectral radiance from 400 to 2500 nm at 10 nm spectral intervals. Quantitiative research and application objectives for surface investigations require conversion of the measured radiance to surface reflectance or surface leaving radiance. In this paper we describe a set of algorithms to estimate aerosol optical depth, atmospheric water vapor, and surface pressure height from the AVIRIS measured radiance.

infrared↗

Airborne Sunphotometer Measurements of Aerosol Optical Depth and Water Vapor in ACE-Asia and Their Comparisons to Correlative Measurements

In the Spring 2001 phase of the Asian Pacific Regional Aerosol Characterization Experiment (ACE-Asia), the 6-channel NASA Ames Airborne Tracking Sunphotometer (AATS-6) operated on 15 of the 19 research flights of the NCAR C-130, while its 14-channel counterpart (AATS-14) flew successfully on all 19 research flights of the CIRPAS Twin Otter. ACE-Asia studied aerosol outflow from the Asian continent to the Pacific basin. It was designed to integrate suborbital and satellite measurements and models to reduce the uncertainty in calculations of the climate forcing due to aerosols. AATS-6 and AATS-14 measured solar beam transmission at six and 14 wavelengths (380-1021 and 354-1558 nm, respectively), yielding aerosol optical depth (AOD) spectra and columnar water vapor (CWV). Vertical differentiation in profiles yielded aerosol extinction spectra and water vapor concentration. In this paper, we plan to present examples of the following, preliminary findings that are based in part on our airborne sunphotometer measurements: (1) The wavelength dependence of sunphotometer-derived AOD and extinction indicates that supermicron dust was often a major component of the aerosol, frequently extending to high altitudes. The percentage of full-column AOD (525 nm) that Jay above 3 km was typically 34+/-13%. In contrast, the analogous percentage of columnar water vapor was only 10+/-4%; (2) Initial comparison studies between AOD data obtained by AATS-6 and AATS-14 during coordinated low-level flight legs show agreement well within the instruments' error bars; (3) Aerosol extinction has been derived from airborne in situ measurements of scattering (nephelometers) and absorption (particle soot/ absorption photometer, PSAP) or calculated from particle size distribution measurements (mobility analyzers and aerodynamic particle sizers). Comparison with corresponding extinction values derived from the Ames airborne sunphotometer measurements shows good agreement for the vertical distribution of aerosol layers. However, the level of agreement in absolute magnitude of the derived aerosol extinction/optical depth varied among the aerosol layers sampled; (4) Initial comparisons of sunphotometer and satellite-derived AOD using SeaWiFS, MISR and AVHRR show promising results. We also plan to include comparisons with MODIS and TOMS: (5) Initial comparisons of sunphotometer-derived AOD and aerosol extinction profiles with lidars in Tokyo and on a ship show reasonable agreement.

Schmid, B.↗

The Diurnal Variation of Dust and Water Ice Aerosol Optical Depth at Jezero Crater Observed By MEDA/TIRS Over A Full Martian Year

The Thermal InfraRed Sensor (TIRS) on the Perseverance rover has provided nearly two full Mars years of systematic monitoring of the total aerosol optical depth above Jezero Crater. These observations span a wide range of timescales, capturing seasonal patterns, diurnal variations, and minute-to-minute fluctuations in aerosol loading. By combining TIRS retrievals with orbital observations, the relative contributions of dust and water ice aerosols can be estimated, revealing their different seasonal and diurnal behaviors. The TIRS record shows distinct periods of dust storm activity, including strong regional storms during the perihelion season as well as short lived but intense dust events outside the typical dust storm season. Water ice clouds exhibit pronounced seasonal and diurnal variability, with peak activity occurring during the aphelion season but with a presence throughout the year. The diurnal variation of clouds differs significantly between the aphelion and perihelion seasons, with clouds persisting throughout the night during the aphelion season, while largely absent outside of specific periods after sunrise and sunset during the perihelion season. These results provide new insights into the complex behavior of aerosols at Jezero Crater and their connections to atmospheric dynamics and the Martian dust and water cycles.

Michael D Smith↗

Total Volcanic Stratospheric Aerosol Optical Depths and Implications for Global Climate Change

Understanding the cooling effect of recent volcanoes is of particular interest in the context of the post-2000 slowing of the rate of global warming. Satellite observations of aerosol optical depth above 15 km have demonstrated that small-magnitude volcanic eruptions substantially perturb incoming solar radiation. Here we use lidar, Aerosol Robotic Network, and balloon-borne observations to provide evidence that currently available satellite databases neglect substantial amounts of volcanic aerosol between the tropopause and 15 km at middle to high latitudes and therefore underestimate total radiative forcing resulting from the recent eruptions. Incorporating these estimates into a simple climate model, we determine the global volcanic aerosol forcing since 2000 to be 0.19 +/- 0.09W/sq m. This translates into an estimated global cooling of 0.05 to 0.12 C. We conclude that recent volcanic events are responsible for more post-2000 cooling than is implied by satellite databases that neglect volcanic aerosol effects below 15 km.

aerosols↗

ACE-Asia Aerosol Optical Depth and Water Vapor Measured by Airborne Sunphotometers and Related to Other Measurements and Calculations

In the Spring 2001 phase of the Asian Pacific Regional Aerosol Characterization Experiment (ACE-Asia), the 6-channel NASA Ames Airborne Tracking Sunphotometer (AATS-6) operated on 15 of the 19 research flights of the NCAR C-130, while its 14-channel counterpart (AATS- 14) flew successfully on all 18 research flights of the CIRPAS Twin Otter. ACE-Asia studied aerosol outflow from the Asian continent to the Pacific basin. It was designed to integrate suborbital and satellite measurements and models so as to reduce the uncertainty in calculations of the climate forcing due to aerosols. AATS-6 and AATS-14 measured solar beam transmission at 6 and 14 wavelengths (380-1021 and 354-1558 nm, respectively), yielding aerosol optical depth (AOD) spectra and column water vapor (CWV). Vertical differentiation in profiles yielded aerosol extinction spectra and water vapor concentration. The wavelength dependence of these AOD and extinction spectra indicates that supermicron dust was often a major component of the ACE-Asia aerosol. Frequently this dust-containing aerosol extended to high altitudes. For example, in AATS- 14 profiles analyzed to date, 36% of full-column AOD at 525 nm was above 3 km. In contrast, only 10% of CWV was above 3 km. Analyses and applications of AATS-6 and AATS-14 data to date include comparisons to (i) extinction products derived using in situ measurements, (ii) extinction profiles derived from lidar measurements, and (iii) AOD retrievals from the Multi-angle Imaging Spectro-Radiometer (MISR) aboard the TERRA satellite. Other planned collaborative studies include comparisons to results from size spectrometers, chemical measurements, other satellite sensors, flux radiometers, and chemical transport models. Early results of these studies will be presented.

Livingston, John M.↗

Total ozone and aerosol optical depths inferred from radiometric measurements in the Chappuis absorption band

A second-derivative smoothing technique, commonly used in inversion work, is applied to the problem of inferring total columnar ozone amounts and aerosol optical depths. The application is unique in that the unknowns may be solved for directly without employing standard inversion methods. It is shown, however, that by employing inversion constraints, better solutions are normally obtained. The method is quite versatile and able to deal with varying total ozone and various aerosol size distributions. The technique is applied first in simulation, then to 119 days of measurements taken in Tucson, Arizona, that are compared to TOMS values for the same dates. The technique is also applied to two measurements taken at Mauna Loa, Hawaii, for which Dobson ozone values are available in addition to the TOMS values, and the results agree to within 15 percent. It is also shown through simulations that additional information can be obtained from measurements outside the Chappuis band. This approach reduces the bias and spread of the estimated total ozone and is unique in that it uses measurements from both the Chappuis and Huggins absorption bands.

Flittner, D. E.↗

Retrieving Aerosol Optical Depth and High Spatial Resolution Ocean Surface Wind Speed from CALIPSO: A Neural Network Approach

An innovative neural network retrieval algorithm is developed for retrieving ocean surface wind speed from the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) lidar measurements. The neural network is trained with CALIPSO ocean surface and atmospheric backscatter measurements together with collocated Advanced Microwave Scanning Radiometer for EOS(AMSR-E) ocean surface wind speed. Ocean surface wind speeds are derived by applying the neural network algorithm to CALIPSO measurements between 2008 and 2020. CALIPSO wind speed measurement of 2015 also compare with Advanced Microwave Scanning Radiometer 2 (AMSR-2) measurements on the Global Change Observation Mission –Water "Shizuku"(GCOM-W) satellite. Aerosol optical depths are then derived from CALIPSO’s ocean surface backscatter signal and theoretical ocean surface reflectance calculated from CALIPSO wind speed and Cox-Munk wind –surface slope variance relation. This CALIPSO wind speed retrieval technique is an improvement from Hu et al. (2008), as it can be applied to most clear skies with optical depths up to 1.5 without making assumptions about aerosol lidar ratio.

wind aerosols CALIPSO↗

Regional Aerosol Optical Depth Characteristics from Satellite Observations: ACE-1, TARFOX and ACE-2 Results

Analysis of the aerosol properties during 3 recent international field campaigns ACE-1, TARFOX and ACE-2 are described using satellite retrievals from NOAA AVHRR data. Validation of the satellite retrieval procedure is performed with airborne, shipboard, and land-based sunphotometry during ACE-2. The intercomparison between satellite and surface optical depths has a correlation coefficient of 0.93 for 630 nm wavelength and 0.92 for 860 nm wavelength, The standard error of estimate is 0.025 for 630 nm wavelength and 0.023 for 860 nm wavelength. Regional aerosol properties are examined in composite analysis of aerosol optical properties from the ACE-1, TARFOX and ACE-2 regions. ACE-1 and ACE-2 regions have strong modes in the distribution of optical depth around 0.1, but the ACE-2 tails toward higher values yielding an average of 0.16 consistent with pollution and dust aerosol intrusions. The TARFOX region has a noticeable mode of 0.2, but has significant spread of aerosol optical depth values consistent with the varied continental aerosol constituents off the eastern North American Coast.

Durkee, P. A.↗

Accuracy Assessment of Aqua-MODIS Aerosol Optical Depth Over Coastal Regions: Importance of Quality Flag and Sea Surface Wind Speed

Coastal regions around the globe are a major source for anthropogenic aerosols in the atmosphere, but the underlying surface characteristics are not favorable for the Moderate Resolution Imaging Spectroradiometer (MODIS) algorithms designed for retrieval of aerosols over dark land or open-ocean surfaces. Using data collected from 62 coastal stations worldwide from the Aerosol Robotic Network (AERONET) from approximately 2002-2010, accuracy assessments are made for coastal aerosol optical depth (AOD) retrieved from MODIS aboard Aqua satellite. It is found that coastal AODs (at 550 nm) characterized respectively by the MODIS Dark Land (hereafter Land) surface algorithm, the Open-Ocean (hereafter Ocean) algorithm, and AERONET all exhibit a log-normal distribution. After filtering by quality flags, the MODIS AODs respectively retrieved from the Land and Ocean algorithms are highly correlated with AERONET (with R(sup 2) is approximately equal to 0.8), but only the Land algorithm AODs fall within the expected error envelope greater than 66% of the time. Furthermore, the MODIS AODs from the Land algorithm, Ocean algorithm, and combined Land and Ocean product show statistically significant discrepancies from their respective counterparts from AERONET in terms of mean, probability density function, and cumulative density function, which suggest a need for future improvement in retrieval algorithms. Without filtering with quality flag, the MODIS Land and Ocean AOD dataset can be degraded by 30-50% in terms of mean bias. Overall, the MODIS Ocean algorithm overestimates the AERONET coastal AOD by 0.021 for AOD less than 0.25 and underestimates it by 0.029 for AOD greater than 0.25. This dichotomy is shown to be related to the ocean surface wind speed and cloud contamination effects on the satellite aerosol retrieval. The Modern Era Retrospective-Analysis for Research and Applications (MERRA) reveals that wind speeds over the global coastal region 25 (with a mean and median value of 2.94 meters per second and 2.66 meters per second, respectively) are often slower than 6 meters per second assumed in the MODIS Ocean algorithm. As a result of high correlation (R(sup 2) greater than 0.98) between the bias in binned MODIS AOD and the corresponding binned wind speed over the coastal sea surface, an empirical scheme for correcting the bias of AOD retrieved from the MODIS Ocean algorithm is formulated and is shown to be effective over the majority of the coastal AERONET stations, and hence can be used in future analysis of AOD trend and MODIS AOD data assimilation.

Anderson, J. C.↗

Application of Low-Cost Fine Particulate Mass Monitors to Convert Satellite Aerosol Optical Depth Measurements to Surface Concentrations in North America and Africa

Low-cost particulate mass sensors provide opportunities to assess air quality at unprecedented spatial and temporal resolutions. Established traditional monitoring networks have limited spatial resolution and are simply absent in many major cities across sub-Saharan Africa (SSA). Satellites provide snapshots of regional air pollution but require ground-truthing. Low-cost monitors can supplement and extend data coverage from these sources worldwide, providing a better overall air quality picture. We investigate the utility of such a multi-source data integration approach using two case studies. First, in Pittsburgh, Pennsylvania, both traditional monitoring and dense low-cost sensor networks are compared with satellite aerosol optical depth (AOD) data from NASA's MODIS system, and a linear conversion factor is developed to convert AOD to surface fine particulate matter mass concentration (as PM2.5). With 10 or more ground monitors in Pittsburgh, there is a 2-fold reduction in surface PM2.5 estimation mean absolute error compared to using only a single ground monitor. Second, we assess the ability of combined regional-scale satellite retrievals and local-scale low-cost sensor measurements to improve surface PM2.5 estimation at several urban sites in SSA. In Rwanda, we find that combining local ground monitoring information with satellite data provides a 40 % improvement in surface PM2.5 estimation accuracy with respect to using low-cost ground monitoring data alone. A linear AOD-to-surface-PM2.5 conversion factor developed in Kigali, Rwanda, did not generalize well to other parts of SSA and varied seasonally for the same location, emphasizing the need for ongoing and localized ground-based monitoring, which can be facilitated by low-cost sensors. Overall, we find that combining ground-based low-cost sensor and satellite data, even without including additional meteorological or land use information, can improve and expand spatiotemporal air quality data coverage, especially in data-sparse regions.

AOD↗

Toward Improving Short-Term Predictions of Fine Particulate Matter Over the United States Via Assimilation of Satellite Aerosol Optical Depth Retrievals

This study develops a new approach to improve simulations of the particulate matter of aerodynamic diameter smaller than 2.5μm (PM2.5) in the Community Multiscale Air Quality (CMAQ) model via assimilation of Moderate Resolution Imaging Spectroradiometer (MODIS) aerosol optical depth(AOD) retrievals using the Grid point Statistical Interpolation (GSI) system. In contrast to previous studies that only consider errors due to transport, our computation of the background error covariance matrix incorporates uncertainties in anthropogenic emissions. To understand the impact of this approach, three experiments (one background and two assimilations) are performed over the contiguous United States(CONUS) from 15 July to 14 August 2014. The background CMAQ experiment significantly underestimates both the MODIS AOD and surface PM2.5levels. MODIS AOD assimilation pushes both the CMAQ AOD and surface PM2.5distributions toward the observed distributions, but CMAQ still underestimates the observations. Averaged over CONUS, the two assimilation experiments with and without including the anthropogenic emission uncertainties improve the correlation coefficient between the model and independent observations of PM2.5 by ~67% and ~48%, respectively, and reduces the mean bias by ~38% and~10%, respectively. The assimilation improves the model performance everywhere over CONUS, except the New York and Wisconsin, where CMAQ overestimates the observed PM2.5during nighttime after assimilation likely because of overcorrection of aerosol mass concentrations by the AOD assimilation. Future work should incorporate uncertainties in other processes (biomass burning and biogenic emissions, deposition, chemistry, transport, and boundary conditions) to further enhance the value of assimilating spaceborne AOD retrievals.

Assimilation↗

Validation of MODIS 3 km Land Aerosol Optical Depth from NASA's EOS Terra and Aqua Missions

In addition to the standard resolution product (10km), the MODerate resolution Imaging Spectroradiometer (MODIS) Collection 6 (C006) data release included a higher resolution (3km). Other than accommodations for the two different resolutions, the 10 and 3km Dark Target (DT) algorithms are basically the same. In this study, we perform global validation of the higher-resolution aerosol optical depth (AOD) over global land by comparing against AErosol RObotic NETwork (AERONET) measurements. The MODIS-AERONET collocated data sets consist of 161410 high-confidence AOD pairs from 2000 to 2015 for Terra MODIS and 2003 to 2015 for Aqua MODIS. We find that 62.5 and 68.4% of AODs retrieved from Terra MODIS and Aqua MODIS, respectively, fall within previously published expected error bounds of +/-(0.05+0.2 × AOD), with a high correlation (R = 0.87). The scatter is not random, but exhibits a mean positive bias of ∼ 0.06 for Terra and ∼ 0.03 for Aqua. These biases for the 3km product are approximately 0.03 larger than the biases found in similar validations of the 10km product. The validation results for the 3km product did not have a relationship to aerosol loading (i.e., true AOD), but did exhibit dependence on quality flags, region, viewing geometry, and aerosol spatial variability. Time series of global MODIS-AERONET differences show that validation is not static, but has changed over the course of both sensors' lifetimes, with Terra MODIS showing more change over time. The likely cause of the change of validation over time is sensor degradation, but changes in the distribution of AERONET stations and differences in the global aerosol system itself could be contributing to the temporal variability of validation.

Gupta, Pawan↗