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Results for “below- threshold ionization”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 91 records · Page 5
All sourcesNASA NTRSDOE OSTI
DOE OSTI2019

Double-resonance studies of electronically autoionizing states of molecular nitrogen

Double-resonance excitation of molecular nitrogen, N 2 , via selected rotational levels of the a" 1 Σ g + , v' = 0 state has been used to probe the first two bands in the new Ogawa series [M. Ogawa, Can. J. Phys. 42, 1087 (1964)], which lie above the first ionization threshold of the molecule. These bands are rotationally unresolved in room-temperature and jet-cooled absorption spectra, but the double-resonance technique allows a rotational analysis and first confirmation of the assignment as transitions to n = 4 members of the (A 2 II u )ndπ, v Rydberg series. In principle, the probe transition from the a" 1 Σ g + , v= 0 level to these Rydberg states corresponds to a two-electron transition, and this aspect of the results is explored. Lastly, velocity map imaging allows a determination of the photoelectron branching fractions and angular distributions, providing insight into the electronic autoionization dynamics.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2017

Absolute single photoionization cross-section measurements of Rb 2+ ions: experiment and theory

Absolute single photoionization cross-section measurements of Rb 2+ ions were performed at the Advanced Light Source at Lawrence Berkeley National Laboratory using synchrotron radiation and the photo-ion, merged-beams technique. Measurements were made at a photon energy resolution of 13.5 2.5 meV from 37.31 to 44.08 eV spanning the 2 P ground state and 2 P metastable state ionization thresholds. Multiple autoionizing resonance series arising from each initial state are identified using quantum defect theory. The measurements are compared to Breit-Pauli R-matrix calculations with excellent agreement between theory and experiment.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2025

Oxygen Opacity Measurements at High-Energy-Density Conditions

We present the first benchmark measurements of oxygen opacity at high-energy-density, crucial for understanding stellar interiors. A 3–5−μm thick SiO 2 sample was heated using a Z facility x-ray source, and opacity was measured in the 5–19.5 Å range with multiple spectrometers. The electron temperature and density inferred from Si 𝐾-shell spectra were 148 ± 4 eV and 8.6 ±1.4 × 10 21 cm −3 , respectively. Six experiments showed opacity reproducibility within ±15% and 5%–25% opacity uncertainty. Measured oxygen opacity and seven different opacity models exhibit extraordinary overall agreement. Discrepancies near the H-like photon ionization threshold and in certain spectral lines suggest the need for model refinements.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2020

Analysis of THz generation by multicolor laser pulses with various frequency ratios

Here, terahertz (THz) generation in a gas medium is simulated by quantum calculations with multicolor intense laser pulses of various frequency ratios. By correlating THz radiation with the above-threshold-ionization photoelectron spectrum, we confirm that our previously proposed free-free transition model for the generation of THz radiation is also applicable to multicolor pulses. THz photon emissions can proceed through transitions between continuous states with similar energies that have opposite parities. This mechanism predicts that THz waves can be efficiently generated at special two-color laser frequency ratios when the multiphoton mixing condition is satisfied. Applying this model to multicolor fields (sawtooth wave shape), we provide a quantum-mechanical interpretation for the reason for THz radiation enhancement. A scheme combining multiple lasers to raise THz radiation satisfying multiphoton mixing conditions is also proposed.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2020

Observation of attosecond electron dynamics in the photoelectron momentum distribution of atoms using few-cycle laser pulses

The method of time-resolved measurement with ultrashort laser pulses is vital to the development of attosecond science. Pump-probe measurements using a train of attosecond pulses in combination with a near-infrared (NIR) multicycle driving laser have been successful in capturing the intercycle electron dynamics which repeats every optical cycle and leads to above-threshold ionization (ATI) spectra in the frequency domain. Here in this work, we study the effect of a carrier-envelope phase (CEP) in a few-cycle (< 6 fs) NIR laser pulse on the photoelectron momentum distribution (PMD) of a hydrogen atom and show that interference patterns in a PMD change dramatically with CEPs in the few-cycle regime. When the few-cycle driving laser pulse has a sine shape, the double-slit interference with characteristic modulation of ATI peaks dominates the PMD. On the other hand, when the driving pulse has a cosine shape, the holographical interference featured by a spider-like pattern is isolated. Our results suggest that the CEP-stable few-cycle laser pulses can be used to identify different types of intracycle interference structures in a PMD which reveal the underlying subcycle electron dynamics on an attosecond timescale.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2022

Manifestation of postcollision interaction in Krypton LMN Auger spectra following K-shell photoionization

In this work, we report on an experimental and theoretical study of post-collision interaction (PCI) effects on L 2 -M 4,5 N 2,3 Auger electrons measured above the Kr K-edge in which L 2 vacancies are primarily generated by KL 2 x-ray emission. Such cascade processes, in which a deep inner-shell vacancy decays first by x-ray emission followed by Auger electron emission, is a strong decay mode in heavy atoms. The L 2 -M 4,5 N 2,3 Auger electron peak is observed to become increasingly asymmetric with a shifting peak maximum as the absorbed x-ray energy approaches the K-shell ionization threshold. This is attributed to PCI energy exchanges of the Auger electron with the 1s photoelectron. To model the PCI effects, we have applied a semiclassical approach modified to account for the combined lifetimes of the K and L 2 hole states. In addition, our analysis treats several closely spaced Auger transitions with final ionic states having different terms and angular momenta.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2017

Analysis of THz generation through the asymmetry of photoelectron angular distributions

In this work, we analyze the mechanism of THz generation in a gas medium with intense two-color infrared lasers pulses. The dependence of the amplitude of THz emission on the relative phase between the fundamental color (800 nm) and its second harmonic (400 nm) is shown to be identical to the residual current as well as to the asymmetry of the above-threshold-ionization (ATI) photoelectrons along the left versus the right side of the linear polarization axis of the laser, thus confirming the validity of the semiclassical photocurrent model for the THz emission. We further analyze the even vs odd angular momentum distributions of the ATI electrons. The degree of overlap between the even-parity dominant electrons and the odd-parity dominant electrons within each ATI peak determines the strength of the THz emission, thus favoring the model that THz is generated through free-free transitions in the laser field. A model is also provided to obtain the same phase dependence as the four-wave mixing model.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2017

Resonant two- or three-photon ionization of noble-gas atoms captured by time-resolved photoelectron momentum spectroscopy

In this work, we present an all-electron, ab initio calculation of time-resolved photoelectron momentum distributions (PMDs) induced by resonant two-color, two- or three-photon ionization of helium and neon atoms, as recently measured by Villeneuve et al. [Science 356, 1150 (2017)] using a femtosecond infrared (IR) laser pulse and an attosecond pulse train (APT) produced with high harmonic generation as an extreme ultraviolet (XUV) photon source. In contrast to a monochromatic XUV pulse commonly used at the free-electron laser facilities, an APT is broadband and ultrashort (<1 fs), so that it could induce nonresonant one-photon transitions above ionization threshold as well as a resonantly excited state. They may interfere with each other upon subsequent absorption or emission of an IR photon, so that the resultant PMD loses clear orbital symmetry. Our time-dependent density functional calculation demonstrates that the selection of a particular excited state in the time-resolved PMD is nevertheless possible if energy and timing of an APT are adjusted properly.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2018

Low-mass dark matter search with CDMSlite

The SuperCDMS experiment is designed to directly detect WIMPs (Weakly Interacting Massive Particles) that may constitute the dark matter in our galaxy. During its operation at the Soudan Underground Laboratory, germanium detectors were run in the CDMSlite (Cryogenic Dark Matter Search low ionization threshold experiment) mode to gather data sets with sensitivity specifically for WIMPs with masses ${<}10$ GeV/$c^2$. In this mode, a large detector-bias voltage is applied to amplify the phonon signals produced by drifting charges. This paper presents studies of the experimental noise and its effect on the achievable energy threshold, which is demonstrated to be as low as 56 eV$_{\text{ee}}$ (electron equivalent energy). The detector biasing configuration is described in detail, with analysis corrections for voltage variations to the level of a few percent. Detailed studies of the electric-field geometry, and the resulting successful development of a fiducial parameter, eliminate poorly measured events, yielding an energy resolution ranging from ${\sim}$9 eV$_{\text{ee}}$ at 0 keV to 101 eV$_{\text{ee}}$ at ${\sim}$10 keV$_{\text{ee}}$. New results are derived for astrophysical uncertainties relevant to the WIMP-search limits, specifically examining how they are affected by variations in the most probable WIMP velocity and the galactic escape velocity. These variations become more important for WIMP masses below 10 GeV/$c^2$. Finally, new limits on spin-dependent low-mass WIMP-nucleon interactions are derived, with new parameter space excluded for WIMP masses ${\lesssim}$3 GeV/$c^2$.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2017

Plasma q -plate for generation and manipulation of intense optical vortices

An optical vortex is a light wave with a twisting wavefront around its propagation axis and null intensity in the beam center. Its unique spatial structure of field lends itself to a broad range of applications, including optical communication, quantum information, superresolution microscopy, and multidimensional manipulation of particles. However, accessible intensity of optical vortices have been limited to material ionization threshold. This limitation might be removed by using the plasma medium. Here in this paper, we propose the design of suitably magnetized plasmas which, functioning as a q-plate, leads to a direct conversion from a high-intensity Gaussian beam into a twisted beam. A circularly polarized laser beam in the plasma accumulates an azimuthal-angle-dependent phase shift and hence forms a twisting wavefront. Our three-dimensional particle-in-cell simulations demonstrate extremely high-power conversion efficiency. The plasma q-plate can work in a large range of frequencies spanning from terahertz to the optical domain.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2023

Even lighter particle dark matter

We report on recent progress in the search for dark matter particles with masses from 1 Mev c ^{-2} − 2 to 1 Gev c ^{-2} − 2 . Several dark matter candidates in this mass range are expected to generate measurable electronic-recoil signals in direct-detection experiments. We focus on dark matter particles scattering with electrons in semiconductor detectors since they have fundamentally the highest sensitivity due to their low ionization threshold. Charge-coupled device (CCD) silicon detectors are the leading technology, with significant progress expected in the coming years. We present the status of the CCD program and briefly report on other efforts.

Chavarria, Alvaro E.↗
DOE OSTI2019

A boron-coated CCD camera for direct detection of Ultracold Neutrons (UCN)

A new boron-coated CCD camera is described for direct detection of ultracold neutrons (UCN) through the capture reactions 10 B (n,α0γ) 7 Li (6%) and 10 B(n,α1γ) 7 Li (94%). The experiments, which extend earlier works using a boron-coated ZnS:Ag scintillator, are based on direct detections of the neutron-capture byproducts in silicon. The high position resolution, energy resolution and particle ID performance of a scientific CCD allows for observation and identification of all the byproducts α, 7 Li and γ (electron recoils). A signal-to-noise improvement on the order of 10 4 over the indirect method has been achieved. Sub-pixel position resolution of a few microns is demonstrated. The technology can also be used to build UCN detectors with an area on the order of 1 m 2 . The combination of micrometer scale spatial resolution, few electrons ionization thresholds and large area paves the way to new research avenues including quantum physics of UCN and high-resolution neutron imaging and spectroscopy.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

Ionization-Based Optical Structures for the Control of Short-Pulse Lasers (Abbreviated LDRD Report)

The intensity of light from the highest-power lasers is limited by the size of the optics required to amplify, compress, transport, and focus a laser beam. Indeed, optics damage puts strict constraints on the laser energy density that solid optics can sustain; this leads to enormous optics sizes and limits the maximum intensity that these lasers can achieve. In this project we investigated new types of diffractive optics based on mixtures of neutral gas and plasmas. The basic idea is to interfere laser beams in a gas near the ionization threshold, so that plasma is created in the constructive interference regions (i.e., the “bright” fringes of the interference pattern) while the destructive interference regions remain a neutral gas. The resulting refractive index modulation, due to the different indices in gas vs. plasma, effectively turns such structures into diffractive optics elements. We proposed several new types of optics based on this general concept: i) reflection gratings, which can act as mirrors of “pulse cleaners” to eliminate laser pre-pulse; ii) transmission gratings, as part of a new type of pulse compression scheme with the potential to achieve laser intensities orders of magnitude above what is currently feasible using solid-state optics; and iii) holographic lenses, to focus high-power lasers. We conducted laboratory experiments which demonstrated high efficiency reflection gratings, paving the way for practical applications of our new concepts.

47 OTHER INSTRUMENTATION↗
DOE OSTI2022

Photoemission Induced Plasma Breakdown (Update)

Laser-induced photoemission of electrons offers opportunities to trigger and control plasmas and discharges. However, the underlying mechanisms are not sufficiently characterized to be fully utilized. Photoemission is highly nonlinear, achieved through multiphoton absorption, above threshold ionization, photo-assisted tunneling, etc., where the dominant process depends on the work function of the material, photon energy and associated fields, surface heating, background fields, etc. To characterize the effects of photoemission on breakdown, breakdown experiments were performed and interpreted using a 0D plasma discharge circuit model and quantum model of photoemission.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2016

A high-resolution vacuum ultraviolet laser photoionization and photoelectron study of the Co atom

We have measured the vacuum ultraviolet–photoionization efficiency (VUV–PIE) spectrum of Co in the energy range of 63,500–67,000 cm{sup −1}, which covers the photoionization transitions of Co(3d{sup 7}4s{sup 2 4}F{sub 9/2}) → Co{sup +}(3d{sup 8 3}F{sub 4}), Co(3d{sup 7}4s{sup 2 4}F{sub 7/2}) → Co{sup +}(3d{sup 8 3}F{sub 3}), Co(3d{sup 7}4s{sup 2 4}F{sub 9/2}) → Co{sup +}(3d{sup 8 3}F{sub 3}), Co(3d{sup 7}4s{sup 2 4}F{sub 9/2}) → Co{sup +}(3d{sup 8 3}F{sub 2}), and Co(3d{sup 7}4s{sup 2 4}F{sub 9/2}) → Co{sup +}(3d{sup 7}4s{sup 1 5}F{sub 5}). We have also recorded the pulsed field ionization photoelectron spectrum of Co in the same energy range, allowing accurate determinations of ionization energies (IEs) for the photoionization transitions from the Co(3d{sup 7}4s{sup 2 4}F{sub 9/2}) ground neutral state to the Co{sup +}({sup 3}F{sub J}) (J = 4 and 3) and Co{sup +}({sup 5}F{sub 5}) ionic states, as well as from the Co(3d{sup 7}4s{sup 2 4}F{sub 7/2}) excited neural state to the Co{sup +}(3d{sup 8 3}F{sub 3}) ionic state. The high-resolution nature of the VUV laser used has allowed the observation of many well-resolved autoionizing resonances in the VUV–PIE spectrum, among which an autoionizing Rydberg series, 3d{sup 7}4s{sup 1}({sup 5}F{sub 5})np (n = 19–38), converging to the Co{sup +}(3d{sup 7}4s{sup 1 5}F{sub 5}) ionic state from the Co(3d{sup 7}4s{sup 2 4}F{sub 9/2}) ground neutral state is identified. The fact that no discernible step-like structures are present at these ionization thresholds in the VUV–PIE spectrum indicates that direct photoionization of Co is minor compared to autoionization in this energy range. The IE values, the autoionizing Rydberg series, and the photoionization cross sections obtained in this experiment are valuable for understanding the VUV opacity and abundance measurement of the Co atom in stars and solar atmospheres, as well as for benchmarking the theoretical results calculated in the Opacity Project and the IRON Project, and thus are of relevance to astrophysics.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2018

Production Rate Measurement of Tritium and Other Cosmogenic Isotopes in Germanium with CDMSlite

Future direct searches for low-mass dark matter particles with germanium detectors, such as SuperCDMS SNOLAB, are expected to be limited by backgrounds from radioactive isotopes activated by cosmogenic radiation inside the germanium. There are limited experimental data available to constrain production rates and a large spread of theoretical predictions. We examine the calculation of expected production rates, and analyze data from the second run of the CDMS low ionization threshold experiment (CDMSlite) to estimate the rates for several isotopes. We model the measured CDMSlite spectrum and fit for contributions from tritium and other isotopes. Using the knowledge of the detector history, these results are converted to cosmogenic production rates at sea level. The production rates in atoms/(kg$\cdot$day) are 74$\pm$9 for $^3$H, 1.5$\pm$0.7 for $^{55}$Fe, 17$\pm$5 for $^{65}$Zn, and 30$\pm$18 for $^{68}$Ge.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2019

A boron-coated CCD camera for direct detection of Ultracold Neutrons (UCN)

A new boron-coated CCD camera is described for direct detection of ultracold neutrons (UCN) through the capture reactions $^{10}$B (n,$\alpha$0$\gamma$)$^7$Li (6%) and $^{10}$B(n,$\alpha$1$\gamma$)$^7$Li (94%). The experiments, which extend earlier works using a boron-coated ZnS:Ag scintillator, are based on direct detections of the neutron-capture byproducts in silicon. The high position resolution, energy resolution and particle ID performance of a scientific CCD allows for observation and identification of all the byproducts $\alpha$, $^7$Li and $\gamma$ (electron recoils). A signal-to-noise improvement on the order of 10$^4$ over the indirect method has been achieved. Sub-pixel position resolution of a few microns is demonstrated. The technology can also be used to build UCN detectors with an area on the order of 1 m$^2$. The combination of micrometer scale spatial resolution, few electrons ionization thresholds and large area paves the way to new research avenues including quantum physics of UCN and high-resolution neutron imaging and spectroscopy.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2018

SuperCDMS Background Models for Low-Mass Dark Matter Searches

An abundance of astrophysical and cosmological evidence indicates the existence of a non-luminous, non-baryonic form of matter, called dark matter, that is approximately a quarter of all energy in the universe. One promising candidate for dark matter is the Weakly Interacting Massive Particle (WIMP) which interacts with baryonic matter at most on the scale of the weak force. The Cryogenic Dark Matter Search (CDMS) experiment aims to detect the nuclear recoils induced by the elastic scattering of WIMPs off of germanium nuclei. This is a rare signal and difficult to detect, especially the low-energy recoils that are produced by low-mass dark matter. The CDMS project operated at the Soudan Underground Laboratory from 2003--2015, with an upgrade to the SuperCDMS experiment in 2012. The germanium detectors were operated at 50~mK and able to measure both the ionization and athermal phonons produced in a particle interaction. Measuring two signals enables discrimination between electron recoil and nuclear recoil events. An alternative operating mode for the detectors is called the CDMS low ionization threshold experiment (CDMSlite), where a higher bias was applied to the detectors and only the phonon signal analyzed. This method increased sensitivity to low-mass dark matter interactions, but sacrificed discrimination capability. The CDMSlite spectrum had a large contribution from electron recoil background events. From the information gained during the first two CDMSlite Runs, a background model was developed for the third and final CDMSlite Run. Analytical descriptions were identified for those backgrounds that were theoretically known, e.g. tritium $\beta$-spectrum, and Geant simulations were used to understand and predict the low-energy spectra from other sources, e.g. Compton scattering. Multiple new models were developed for detectors operated in CDMSlite at Soudan. These include the analytical formula for Compton scattering, and empirical models for surface backgrounds from $^{210}$Pb contamination of the germanium crystals and detector housing. In order to accurately describe the surface events, a new detector response function was developed that included information about the electric field and energy resolution of the detector. These models were essential to the implementation of a profile likelihood analysis of the CDMSlite Run 3 data, which improved on the sensitivity to dark matter over the Run 2 optimum interval analysis for WIMP masses above 2.5~GeV/$c^2$. This demonstrated a successful application of a likelihood analysis to the high-voltage operating mode, and the potential for these analyses in the future SuperCDMS SNOLAB experiment. For the SuperCDMS SNOLAB experiment, the change in background rates from radiogenic neutrons was considered as additional towers of detectors were added, and the feasibility of an active neutron veto as a potential upgrade for large payloads was studied. This veto could be constructed of plastic scintillator with layers of gadolinium resin, and would aid in reducing the nuclear recoil single scatter background that is indistinguishable from the WIMP signal.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗