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NASA NTRS2001

Combustion of Unconfined Droplet Clusters in Microgravity

Combustion experiments using arrays of droplets seek to provide a link between single droplet combustion phenomena and the behavior of complex spray combustion systems. Both single droplet and droplet array studies have been conducted in microgravity to better isolate the droplet interaction phenomena and eliminate or reduce the confounding effects of buoyancy-induced convection. In most experiments involving droplet arrays, the droplets are supported on fibers to keep them stationary and close together before the combustion event. The presence of the fiber, however, disturbs the combustion process by introducing a source of heat transfer and asymmetry into the configuration. As the number of drops in a droplet array increases, supporting the drops on fibers becomes less practical because of the cumulative effect of the fibers on the combustion process. To eliminate the effect of the fiber, several researchers have conducted microgravity experiments using unsupported droplets. Jackson and Avedisian investigated single, unsupported drops while Nomura et al. studied droplet clouds formed by a condensation technique. The overall objective of this research is to extend the study of unsupported drops by investigating the combustion of well-characterized drop clusters in a microgravity environment. Direct experimental observations and measurements of the combustion of droplet clusters would fill a large gap in our current understanding of droplet and spray combustion and provide unique experimental data for the verification and improvement of spray combustion models. In this work, the formation of drop clusters is precisely controlled using an acoustic levitation system so that dilute, as well as dense clusters can be created and stabilized before combustion in microgravity is begun. This paper describes the design and performance of the 1-g experimental apparatus, some preliminary 1-g results, and plans for testing in microgravity.

Ruff, G. A.↗
NASA NTRSDate not supplied

Utilization of Streamtubes to Analyze the Physical Interaction of a Dispersed Cloud with the CRM65 Hybrid Midspan Model

Recently there have been numerous efforts to identify the relevant icing physics related to the formation of complex three dimensional features, sometimes referred to as ’scallops’, on swept wings. However, much of the physics is still not well understood. This paper computationally investigates the interaction of the icing cloud with the 65 percent Common Research Model (CRM65). Both the interaction with an uniced model, and the interaction with a representative simulated three dimensional ice accretion are analyzed. Preliminary results suggest that the liquid water content increases near the aerodynamic body. For small droplets on the uniced geometry, the particle velocity vector becomes nearly parallel with the aerodynamic model resulting in a low value of collection efficiency. When a three dimensional feature with a length scale much smaller than the leading edge of the airfoil is introduced into the flow, the impingement of small particles can become significantly more perpendicular to the particle velocity vector in the region of these features. Since the liquid water content near the body has increased due to the interaction with the larger scale features of the aerodynamic model, i.e. the leading edge of the swept wing, extremely high collection efficiency is observed. These results suggest that three dimensional features are likely a significant physical driver that should be modeled in some capacity when simulating the impingement of a cloud on an aerodynamic model.

Icing↗
NASA NTRSDate not supplied

Utilization of Streamtubes to Analyze the Physical Interaction of a Dispersed Cloud with the CRM65 Hybrid Midspan Model

Recently there have been numerous efforts to identify the relevant icing physics related to the formation of complex three dimensional features, sometimes referred to as ’scallops’, on swept wings. However, much of the physics is still not well understood. This paper computationally investigates the interaction of the icing cloud with the 65 percent Common Research Model (CRM65). Both the interaction with an uniced model, and the interaction with a representative simulated three dimensional ice accretion are analyzed. Preliminary results suggest that the liquid water content increases near the aerodynamic body. For small droplets on the uniced geometry, the particle velocity vector becomes nearly parallel with the aerodynamic model resulting in a low value of collection efficiency. When a three dimensional feature with a length scale much smaller than the leading edge of the airfoil is introduced into the flow, the impingement of small particles can become significantly more perpendicular to the particle velocity vector in the region of these features. Since the liquid water content near the body has increased due to the interaction with the larger scale features of the aerodynamic model, i.e. the leading edge of the swept wing, extremely high collection efficiency is observed. These results suggest that three dimensional features are likely a significant physical driver that should be modeled in some capacity when simulating the impingement of a cloud on an aerodynamic model.

Icing↗
NASA NTRS2013

Saharan Dust Event Impacts on Cloud Formation and Radiation over Western Europe

We investigated the impact of mineral dust particles on clouds, radiation and atmospheric state during a strong Saharan dust event over Europe in May 2008, applying a comprehensive online-coupled regional model framework that explicitly treats particle-microphysics and chemical composition. Sophisticated parameterizations for aerosol activation and ice nucleation, together with two-moment cloud microphysics are used to calculate the interaction of the different particles with clouds depending on their physical and chemical properties. The impact of dust on cloud droplet number concentration was found to be low, with just a slight increase in cloud droplet number concentration for both uncoated and coated dust. For temperatures lower than the level of homogeneous freezing, no significant impact of dust on the number and mass concentration of ice crystals was found, though the concentration of frozen dust particles reached up to 100 l-1 during the ice nucleation events. Mineral dust particles were found to have the largest impact on clouds in a temperature range between freezing level and the level of homogeneous freezing, where they determined the number concentration of ice crystals due to efficient heterogeneous freezing of the dust particles and modified the glaciation of mixed phase clouds. Our simulations show that during the dust events, ice crystals concentrations were increased twofold in this temperature range (compared to if dust interactions are neglected). This had a significant impact on the cloud optical properties, causing a reduction in the incoming short-wave radiation at the surface up to -75Wm-2. Including the direct interaction of dust with radiation caused an additional reduction in the incoming short-wave radiation by 40 to 80Wm-2, and the incoming long-wave radiation at the surface was increased significantly in the order of +10Wm-2. The strong radiative forcings associated with dust caused a reduction in surface temperature in the order of -0.2 to -0.5K for most parts of France, Germany, and Italy during the dust event. The maximum difference in surface temperature was found in the East of France, the Benelux, and Western Germany with up to -1 K. This magnitude of temperature change was sufficient to explain a systematic bias in numerical weather forecasts during the period of the dust event.

Bangert, M.↗
NASA NTRS1984

The atmospheric effects of El Chichon

The eruption of the Mexican volcano El Chichon in late March and early April of 1982 injected an unusually large amount of volcanic material into the stratosphere. This event demonstrates for the first time that a relatively small but sulfur-rich volcanic eruption can produce a dense, widespread stratospheric cloud. Sulfuric acid aerosol is formed by the photochemical reaction of sulfur gases released by a volcano with water vapor in the atmosphere. The aerosol causes a decrease in the mean global temperature because the droplets both absorb solar radiation and scatter it back into space. Attention is given to details concerning the volcanic eruption, the relation of El Chichon to the Mexican and Guatemalan volcanic belts, sources for the sulfur erupted by the volcano, and the mechanisms involved in the formation of sulfuric acid.

Rampino, M. R.↗
NASA NTRS1990

ETO lidar studies of cirrostratus altocumulogenitus: Another role for supercooled liquid water in cirrus cloud formation

Cirrus clouds have traditionally been viewed as cold, wispy, or stratiform ice clouds, typically displaying optical phenomena such as haloes. A composition entirely of hexagonal ice crystals, of one habit or another could only have a transitory existence in cirrus, since the concentrations of ice nuclei (IN) measured by various techniques (at the surface or in the lower troposphere) indicate an enormous number of IN that should be active at cirrus cloud temperatures. In light of recent instrumental aircraft and polarization lidar studies of cirrus clouds, it is clear that highly supercooled cloud droplets can sometimes be a component of cirrus clouds. It remains to be determined if supercooled liquid water (SLW) is present abundantly enough in cirrus to play a significant role in earth's radiance balance, or is merely a curious, infrequent occurrence. To help evaluate this issue, the UH polarization lidar FIRE Extended Time Observation (ETO) of cirrus clouds are being utilized to compile, among other parameters, a climatological record of SLW clouds associated with and within cirrus.

Sassen, Kenneth↗
NASA NTRSDate not supplied

Towards a Marine Stratus Climatology on Drizzle Occurrence from CALIPSO

Marine stratus are a predominant feature of our planet with the annual mean coverage exceeding 20%. They strongly reflect sunlight, yet exert only a modest effect on outgoing infrared radiation, providing a significant net cooling to the Earth’s radiative balance. Their formation is coupled to boundary layer circulations that are driven, in part, by cloud top radiative cooling and evaporative cooling from precipitation in downdrafts. Understanding how these cloud systems evolve as the climate changes is a key question that requires additional information on their lifecycle and microphysical properties to accurately represent their behavior in global circulation models. From a large-scale perspective, insight into the microphysical properties of marine stratus at cloud top can be realized through estimates of the effective radius (Re) of the droplet size distributions derived from MODIS observations. Estimates on the occurrence of rain/drizzle are available from CloudSat. Together these observations indicate that precipitation frequently occurs in clouds with higher cloud top Re. This relationship is consistent with the well documented shift in cloud top droplet size distributions towards fewer, yet larger droplets prior the onset of precipitation. Here we report on a new and complementary set observations from the CALIPSO mission. The approach derives an extinction-to-backscatter ratio (Sc, also known as the cloud lidar ratio) using an established relationship that depends on observations of the lidar attenuated backscatter and volume depolarization ratio within the cloud. Because Sc is strongly and inversely related to Re, a change in the derived Sc from higher to lower values corresponds to a change in the droplet size distribution as seen by MODIS. This change in the lidar signals at cloud top clearly identifies clouds that are capable of precipitation. The presentation provides a brief overview of the approach for deriving Sc and compares CALIOP-derived Sc with observations from other techniques. CALIOP classifications of drizzling clouds, based on the retrieved values Sc, are compared to independent, collocated assessments of drizzle occurrence reported in the standard CloudSat data products. Regional and seasonal comparisons highlight the strengths and weaknesses of the two sensors. A machine learning approach that combines information from both CALIOP and CloudSat showcases possible improvements in the global identification of scenes likely to contain rain-bearing clouds.

CALIPSO↗
NASA NTRS2012

On the Ice Nucleation Spectrum

This work presents a novel formulation of the ice nucleation spectrum, i.e. the function relating the ice crystal concentration to cloud formation conditions and aerosol properties. The new formulation is physically-based and explicitly accounts for the dependency of the ice crystal concentration on temperature, supersaturation, cooling rate, and particle size, surface area and composition. This is achieved by introducing the concepts of ice nucleation coefficient (the number of ice germs present in a particle) and nucleation probability dispersion function (the distribution of ice nucleation coefficients within the aerosol population). The new formulation is used to generate ice nucleation parameterizations for the homogeneous freezing of cloud droplets and the heterogeneous deposition ice nucleation on dust and soot ice nuclei. For homogeneous freezing, it was found that by increasing the dispersion in the droplet volume distribution the fraction of supercooled droplets in the population increases. For heterogeneous ice nucleation the new formulation consistently describes singular and stochastic behavior within a single framework. Using a fundamentally stochastic approach, both cooling rate independence and constancy of the ice nucleation fraction over time, features typically associated with singular behavior, were reproduced. Analysis of the temporal dependency of the ice nucleation spectrum suggested that experimental methods that measure the ice nucleation fraction over few seconds would tend to underestimate the ice nuclei concentration. It is shown that inferring the aerosol heterogeneous ice nucleation properties from measurements of the onset supersaturation and temperature may carry significant error as the variability in ice nucleation properties within the aerosol population is not accounted for. This work provides a simple and rigorous ice nucleation framework where theoretical predictions, laboratory measurements and field campaign data can be reconciled, and that is suitable for application in atmospheric modeling studies.

Barahona, D.↗
NASA NTRS1973

Venus - Composition and structure of the visible clouds

It is proposed that the visible cloud deck on Venus is composed of droplets of sulfuric acid. These are formed by the very rapid photooxidation of carbonyl sulfide in the upper atmosphere. The clouds are best described as an extensive haze since the predicted particulate scale height probably exceeds the gas scale height within the layer. The predicted mixing ratio for water is .000001 (lower limit), and for both carbonyl sulfide and sulfur dioxide it is .0000001 (upper limit); these are in good agreement with observations. Gaps in the layer are not possible unless the planetary scale dynamics produce cloud turnover times of less than a few days. Under these conditions, the water mixing ratio could approach .0001, and the formation of a thin hydrochloric acid haze at high altitude above the main cloud is possible.

Prinn, R. G.↗
NASA NTRS2009

Convective and Stratiform Precipitation Processes and their Relationship to Latent Heating

The global hydrological cycle is central to the Earth's climate system, with rainfall and the physics of its formation acting as the key links in the cycle. Two-thirds of global rainfall occurs in the Tropics. Associated with this rainfall is a vast amount of heat, which is known as latent heat. It arises mainly due to the phase change of water vapor condensing into liquid droplets; three-fourths of the total heat energy available to the Earth's atmosphere comes from tropical rainfall. In addition, fresh water provided by tropical rainfall and its variability exerts a large impact upon the structure and motions of the upper ocean layer. An improved convective -stratiform heating (CSH) algorithm has been developed to obtain the 3D structure of cloud heating over the Tropics based on two sources of information: 1) rainfall information, namely its amount and the fraction due to light rain intensity, observed directly from the Precipitation Radar (PR) on board the TRMM satellite and 2) synthetic cloud physics information obtained from cloud-resolving model (CRM) simulations of cloud systems. The cloud simulations provide details on cloud processes, specifically latent heating, eddy heat flux convergence and radiative heating/cooling, that. are not directly observable by satellite. The new CSH algorithm-derived heating has a noticeably different heating structure over both ocean and land regions compared to the previous CSH algorithm. One of the major differences between new and old algorithms is that the level of maximum cloud heating occurs 1 to 1.5 km lower in the atmosphere in the new algorithm. This can effect the structure of the implied air currents associated with the general circulation of the atmosphere in the Tropics. The new CSH algorithm will be used provide retrieved heating data to other heating algorithms to supplement their performance.

Tao, Wei-Kuo↗
NASA NTRS1995

Microgravity combustion of dust clouds: Quenching distance measurements

The current level of physical understanding of dust combustion phenomena is still in a rudimentary state compared with the understanding of gas combustion processes. The reason for such a lack of fundamental understanding is partially based on the complexity of multiphase combustion and the enormous diversity of chemical-physical properties of heterogeneous combustible mixtures but is largely due to difficulties in the experimental investigation of dust combustion. The influence of gravity on a dust suspension is the main reason. First of all, when particulates (either solid particles or liquid droplets) with a characteristic size of the order of tens of microns are suspended, they rapidly settle in the gravitational field. To maintain a particulate suspension for a time duration adequate to carry out combustion experiments invariably requires continuous convection of particulates at or in excess of the gravitational settling velocity. Of necessity, this makes the experiments turbulent in character and makes it impossible to study laminar dust flames. For particle sizes of the order of microns a stable laminar dust flow can be maintained only for relatively small dust concentrations (e.g., for low fuel equivalence ratios) at normal gravity conditions. High dust loading leads to gravitational instability of the dust cloud and to the formation of recirculation cells in a dust suspension in a confined volume, or to the rapid sedimentation of the dense dust cloud as a whole in an unconfined volume. In addition, many important solid fuels such as low volatile coal, carbon, and boron have low laminar flame speeds (of the order of several centimeters per second). Gravitational convection that occurs in combustion products due to the buoyancy forces disrupts low speed dust flames and, therefore, makes observation of such flames at normal gravity impossible. The only way to carry out 'clean' fundamental experiments in dust combustion over a wide range of dust cloud parameters is in a gravity-free environment. Access to the microgravity environment provided by the use of large-scale drop towers, parabolic flights of aircraft and rockets, and shuttle and space station orbits has permitted now to proceed with a systematic program of dust combustion microgravity research. For example, the NASA-Lewis drop tower and a Lear jet parabolic flight aircraft were used by Ross et al. and by Berlad and Tangirala for experiments with Iycopodium/air mixtures. The Japan Microgravity Center drop shaft (JAMIC) where a microgravity condition of 10(exp -4) g for 10 s is available, was recently used by Kobayashi, Niioka et al. for measuring flame propagation velocities in polymethyl methacrylate dust/air suspensions. Microgravity dust combustion experiments were started at McGill University in the early 90's under the sponsorship of the Canadian Space Agency. Several generations of dust combustion platforms permitting dust combustion microgravity experiments to be carried out on board a parabolic flight aircraft (KC-135, NASA) have been designed and tested. The experimental data and experience gained from this research allowed us to design and build in a current phase of this program the microgravity apparatus for the visual observation of freely propagating constant pressure laminar dust flames. Quenching distances in aluminum dust suspensions have been measured in a wide range of dust cloud parameters in ground-based experiments and in recent microgravity experiments (KC-135 parabolic flights, Houston, February 1995).

Goroshin, S.↗
NASA NTRS2011

On the Effect of Dust Particles on Global Cloud Condensation Nuclei and Cloud Droplet Number

Aerosol-cloud interaction studies to date consider aerosol with a substantial fraction of soluble material as the sole source of cloud condensation nuclei (CCN). Emerging evidence suggests that mineral dust can act as good CCN through water adsorption onto the surface of particles. This study provides a first assessment of the contribution of insoluble dust to global CCN and cloud droplet number concentration (CDNC). Simulations are carried out with the NASA Global Modeling Initiative chemical transport model with an online aerosol simulation, considering emissions from fossil fuel, biomass burning, marine, and dust sources. CDNC is calculated online and explicitly considers the competition of soluble and insoluble CCN for water vapor. The predicted annual average contribution of insoluble mineral dust to CCN and CDNC in cloud-forming areas is up to 40 and 23.8%, respectively. Sensitivity tests suggest that uncertainties in dust size distribution and water adsorption parameters modulate the contribution of mineral dust to CDNC by 23 and 56%, respectively. Coating of dust by hygroscopic salts during the atmospheric aging causes a twofold enhancement of the dust contribution to CCN; the aged dust, however, can substantially deplete in-cloud supersaturation during the initial stages of cloud formation and can eventually reduce CDNC. Considering the hydrophilicity from adsorption and hygroscopicity from solute is required to comprehensively capture the dust-warm cloud interactions. The framework presented here addresses this need and can be easily integrated in atmospheric models.

Karydis, V. A.↗
NASA NTRS2004

Effects of Kinetic Roughening and Liquid-Liquid Phase Transition on Lysozyme Crystal Growth Velocities

We measured the growth velocities of the (110) face of tetragonal lysozyme, V (centimeters per second), at four different concentrations, c (milligrams per milliliter), as the solution temperature, T (Centigrade), was reduced. For a broad range of T dependent on c, we find that the growth velocities increased as the solution temperature was reduced. The initial increase in V is well characterized by the 2D nucleation model for crystal growth, yielding the magnitude of an effective barrier for growth, gamma(sub s) = 1.2 plus or minus 0.1 x 10(exp -13) erg/molecule. Below certain temperatures, T(sub cr), dependent on c, however, a kinetic roughening hypothesis that considers the continuous addition of molecules anywhere on the crystal surface better describes the observed growth velocities. The application of the continuous growth model, up to the solution cloud-point temperatures, T(sub cl), enabled the determinations of the crossover concentration, c(sub r), from estimated values of T(sub cr). For all conditions presented, we find that the crossover from growth by 2D nucleation to continuous addition occurs at a supersaturation, sigma (sub c), = 2.0 plus or minus 0.1. Moreover, we find the energy barrier for the continuous addition, E(sub c), within the temperature range T(sub cl) less than T less than T less than T (sub cr), to be 6 plus or minus 1 x 10(exp -13) erg/molecule. Further reduction of T below approximately 2-3 C of T(sub cl), also revealed a rapid slowing of crystal growth velocities. From quasi-elastic light scattering investigations, we find that the rapid diminishment of crystal growth velocities can be accounted for by the phase behavior of lysozyme solutions. Namely, we find the reversible formation of dense fluid proto-droplets comprised of lysozyme molecules to occur below approximately 0.3 C of T(sub cl). Hence, the rapid slowing of growth velocities may occur as a result of the sudden depletion of "mobile" molecules within crystal growth solutions as dense fluid proto-droplets form.

Gorti, Sridhar↗
NASA NTRS1992

Radiation pressure: A possible cause for the superrotation of the Venusian atmosphere

The superrotation of the venusian atmosphere relative to the planet's surface has long been known. Yet the process by which this vigorous circulation is maintained is poorly understood. The purpose of this report is to show that a mechanism by which the solar radiation interacts with the cloudy atmosphere of Venus could be the principle cause of the superrotation. It has been long known that Venus has a high albedo due to the scattering (similar to the reflection process) of solar radiation by the cloud droplets in its atmosphere. The radiation not scattered, but intercepted by the planet and its atmosphere, is mainly absorbed within the cloud layers. Therefore, momentum (equal, more or less, to that of the solar radiation intercepted) is continually transferred to the venusian atmosphere. The atmospheric system presents a symmetrical surface (same radiation-matter interaction) toward the solar radiation at its morning and evening limbs. If the cross-sectional areas at both limbs were equal, the momentum transfer at the morning limb would decelerate the atmosphere's rotation while at the evening limb the same transfer would accelerate the rotation an equal amount. The net result of this is that the overall rate of rotation would be unchanged. Such a symmetrical configuration is not likely since the atmosphere must be warmed as it rotates across the planet's day hemisphere and cooled as it rotates across the planet's night hemisphere. This warming and cooling must result in a formation of an asymmetrical configuration. It is apparent that the momentum transfer at the evening limb must be greater than that at the morning limb because the atmosphere's greater cross section at the evening limb intercepts a greater amount of solar radiation. It should be noted that very little of the solar radiation is transmitted through the cloud layers, especially at or near the limbs where the atmospheric path length of the radiation is long. This net momentum transfer must be continually added to the angular momentum of the atmospheric system at the same time angular momentum is continually removed from the atmosphere by the frictional drag imposed on the atmosphere by the slowly rotating planet's surface. This completes the description of this mechanism.

Krause, J. L.↗
NASA NTRS1986

Study of ice accretion on icing wind tunnel components

In a closed loop icing wind tunnel the icing cloud is simulated by introducing tiny water droplets through an array of nozzles upstream of the test section. This cloud will form ice on all tunnel components (e.g., turning vanes, inlet guide vanes, fan blades, and the heat exchanger) as the cloud flows around the tunnel. These components must have the capacity to handle their icing loads without causing significant tunnel performance degradation during the course of an evening's run. To aid in the design of these components for the proposed Altitude Wind Tunnel (AWT) at NASA Lewis Research Center the existing Icing Research Tunnel (IRT) is used to measure icing characteristics of the IRT's components. The results from the IRT are scaled to the AWT to account for the AWT's larger components and higher velocities. The results show that from 90 to 45 percent of the total spray cloud froze out on the heat exchanger. Furthermore, the first set of turning vanes downstream of the test section, the FOD screen and the fan blades show significant ice formation. The scaling shows that the same results would occur in the AWT.

Newton, J. E.↗
NASA NTRS1986

Study of ice accretion on icing wind tunnel components

In a closed loop icing wind tunnel the icing cloud is simulated by introducing tiny water droplets through an array of nozzles upstream of the test section. This cloud will form ice on all tunnel components (e.g., turning vanes, inlet guide vanes, fan blades, and the heat exchanger) as the cloud flows around the tunnel. These components must have the capacity to handle their icing loads without causing significant tunnel performance degradation during the course of an evening's run. To aid in the design of these components for the proposed Altitude Wind Tunnel (AWT) at NASA Lewis Research Center the existing Icing Research Tunnel (IRT) is used to measure icing characteristics of the IRT's components. The results from the IRT are scaled to the AWT to account for the AWT's larger components and higher velocities. The results show that from 90 to 45 percent of the total spray cloud froze out on the heat exchanger. Furthermore, the first set of turning vanes downstream of the test section, the FOD screen and the fan blades show significant ice formation. The scaling shows that the same results would occur in the AWT.

Newton, J. E.↗
NASA NTRS2018

Thermodynamic and Dynamic Aspects of Ice Nucleation

It is known that ice nucleating particles (INP) immersed within supercooled droplets promote the formation of ice. Common theoretical models used to represent this process assume that the immersed particle lowers the work of ice nucleation without significantly affecting the dynamics of water in the vicinity of the particle. This is contrary to evidence showing that immersed surfaces significantly affect the viscosity and diffusivity of vicinal water. To study how this may affect ice formation this work introduces a model linking the ice nucleation rate to the modification of the dynamics and thermodynamics of vicinal water by immersed particles. It is shown that INP that significantly reduce the work of ice nucleation also pose strong limitations to the growth of the nascent ice germs. This leads to the onset of a new ice nucleation regime, called spinodal ice nucleation, where the dynamics of ice germ growth instead of the ice germ size determines the nucleation rate. Nucleation in this regime is characterized by an enhanced sensitivity to particle area and cooling rate. Comparison of the predicted ice nucleation rate against experimental measurements for a diverse set of species relevant to cloud formation suggests that spinodal ice nucleation may be common in nature.

Barahona, Donifan↗
NASA NTRS2003

Aerosol-Cloud Interactions during Tropical Deep Convection: Evidence for the Importance of Free Tropospheric Aerosols

NASA's 2002 CRYSTAL-FACE field experiment focused on the formation and evolution of tropical cirrus cloud systems in southern Florida. Multiple aircraft extensively sampled cumulonimbus dynamical and microphysical properties, as well as characterizing ambient aerosol populations both inside and outside the full depth of the convective column. On July 18, unique measurements were taken when a powerful updraft was traversed directly by aircraft, providing a window into the primary source region of cumulonimbus anvil crystals. Observations of the updraft, entered at approximately l0 km altitude and -34 C, indicated more than 200 cloud particles per mL at vertical velocities exceeding 20 m/s and the presence of significant condensation nuclei and liquid water within the core. In this work, aerosol and cloud phase observations are integrated by simulating the updraft conditions using a large-eddy resolving model with 3 explicit multiphase microphysics, including treatment of size-resolved aerosol fields, aerosol activation and freezing, and evaporation of cloud particles back to the aerosol phase. Simulations were initialized with observed thermodynamic and aerosol size distributions profiles and convection was driven by surface fluxes assimilated from the ARPS forecast model. Model results are consistent with the conclusions that most crystals are homogeneously frozen droplets and that entrained free tropospheric aerosols may contribute a significant fraction of the crystals. Thus most anvil crystals appear to be formed aloft in updraft cores, well above cloud base. These conclusions are supported by observations of hydrometeor size distribution made while traversing the dore, as well as aerosol and cloud particle size distributions generally observed by aircraft below 4km and crystal properties generally observed by aircraft above 12km.

Ackerman, A.↗