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NASA NTRS2000

Laminar Diffusion Flame Studies (Ground- and Space-Based Studies)

Laminar diffusion flames are of interest because they provide model flame systems that are far more tractable for analysis and experiments than more practical turbulent diffusion flames. Certainly, understanding flame processes within laminar diffusion flames must precede understanding these processes in more complex turbulent diffusion flames. In addition, many properties of laminar diffusion flames are directly relevant to turbulent diffusion flames using laminar flamelet concepts. Laminar jet diffusion flame shapes (luminous flame boundaries) have been of particular interest since the classical study of Burke and Schumann because they are a simple nonintrusive measurement that is convenient for evaluating flame structure predictions. Thus, consideration of laminar flame shapes is undertaken in the following, emphasizing conditions where effects of gravity are small, due to the importance of such conditions to practical applications. Another class of interesting properties of laminar diffusion flames are their laminar soot and smoke point properties (i.e., the flame length, fuel flow rate, characteristic residence time, etc., at the onset of soot appearance in the flame (the soot point) and the onset of soot emissions from the flame (the smoke point)). These are useful observable soot properties of nonpremixed flames because they provide a convenient means to rate several aspects of flame sooting properties: the relative propensity of various fuels to produce soot in flames; the relative effects of fuel structure, fuel dilution, flame temperature and ambient pressure on the soot appearance and emission properties of flames; the relative levels of continuum radiation from soot in flames; and effects of the intrusion of gravity (or buoyant motion) on emissions of soot from flames. An important motivation to define conditions for soot emissions is that observations of laminar jet diffusion flames in critical environments, e.g., space shuttle and space station facilities, cannot involve soot emitting flames in order to ensure that test chamber windows used for experimental observations are not blocked by soot deposits, thereby compromising unusually valuable experimental results. Another important motivation to define conditions where soot is present in diffusion flames is that flame chemistry, transport and radiation properties are vastly simplified when soot is absent, making such flames far more tractable for detailed numerical simulations than corresponding soot-containing flames. Motivated by these observations, the objectives of this phase of the investigation were as follows: (1) Observe flame-sheet shapes (the location of the reaction zone near phi=1) of nonluminous (soot free) laminar jet diffusion flames in both still and coflowing air and use these results to develop simplified models of flame-sheet shapes for these conditions; (2) Observe luminous flame boundaries of luminous (soot-containing) laminar jet diffusion flames in both still and coflowing air and use these results to develop simplified models of luminous flame boundaries for these conditions. In order to fix ideas here, maximum luminous flame boundaries at the laminar smoke point conditions were sought, i.e., luminous flame boundaries at the laminar smoke point; (3) Observe effects of coflow on laminar soot- and smoke-point conditions because coflow has been proposed as a means to control soot emissions and minimize the presence of soot in diffusion flames.

Dai, Z.↗

NASA NTRS1984

The mechanisms of flame holding in the wake of a bluff body

The flame holding mechanism for lean methane and lean propane air flames is examined under conditions where the recirculation zone is absent. The holding process is studied in detail in an attempt to determine the mechanism of flame holding and also the conditions where this mechanism is viable and when it fails and blow off occurs. Inverted flames held in the wake of a flat strip are studied. The velocity flow field is determined using a Laser Doppler Velocimetry technique. Equation of continuity is used to calculate the flame temperature from the change in area of flow streamlines before and after the flame. For methane air flame the controlling factor for blow off is incomplete reaction due to higher blowing rate leading to reduced residence time in the reaction zone.

Strehlow, R. A.↗

NASA NTRS1985

The mechanisms of flame holding in the wake of a bluff body

The flame holding mechanism for lean methane- and lean propane-air flames is examined under conditions where the recirculation zone is absent. The main objective of this work is to study the holding process in detail in an attempt to determine the mechanism of flame holding and also the conditions where this mechanism is viable and when it fails and blow-off occurs. Inverted flames held in the wake of a flat strip were studied. Experiments with different sizes of flame holders were performed. The velocity flow field was determined using a laser Doppler velocimetry technique. Equation of continuity was used to calculate the flame temperature from the change in area of flow streamlines before and after the flame. Observations of the inverted flame itself were obtained using schlieren and direct photography. Results show that there are different mechanisms operative at the time of blow-off for lean propane and methane flames. Blow-off or extinction occurs for lean propane-air flame in spite of the reaction going to completion and the disparity between the heat loss and the gain in mass diffusion in the reaction zone i.e., Le 1.0 causes the flame to blow-off. For methane-air flame the controlling factor or blow-off is incomplete reaction due to higher blowing rate leading to reduced residence time in the reaction zone.

Strehlow, R. A.↗

NASA NTRS1993

An Experimental and Theoretical Study of Radiative Extinction of Diffusion Flames

In a recent paper on 'Observations of candle flames under various atmospheres in microgravity' by Ross et al., it was found that for the same atmosphere, the burning rate per unit wick surface area and the flame temperature were considerably reduced in microgravity as compared with normal gravity. Also, the flame (spherical in microgravity) was much thicker and further removed from the wick. It thus appears that the flame becomes 'weaker' in microgravity due to the absence of buoyancy generated flow which serves to transport the oxidizer to the combustion zone and remove the hot combustion products from it. The buoyant flow, which may be characterized by the strain rate, assists the diffusion process to execute these essential functions for the survival of the flame. Thus, the diffusion flame is 'weak' at very low strain rates and as the strain rate increases the flame is initially 'strengthened' and eventually it may be 'blown out'. The computed flammability boundaries of T'ien show that such a reversal in material flammability occurs at strain rates around 5 sec. At very low or zero strain rates, flame radiation is expected to considerably affect this 'weak' diffusion flame because: (1) the concentration of combustion products which participate in gas radiation is high in the flame zone; and (2) low strain rates provide sufficient residence time for substantial amounts of soot to form which is usually responsible for a major portion of the radiative heat loss. We anticipate that flame radiation will eventually extinguish this flame. Thus, the objective of this project is to perform an experimental and theoretical investigation of radiation-induced extinction of diffusion flames under microgravity conditions. This is important for spacecraft fire safety.

Atreya, Arvind↗

NASA NTRS2016

Experimental Combustion Dynamics Behavior of a Multi-Element Lean Direct Injection (LDI) Gas Turbine Combustor

An experimental investigation of the combustion dynamic characteristics of a research multi-element lean direct injection (LDI) combustor under simulated gas turbine conditions was conducted. The objective was to gain a better understanding of the physical phenomena inside a pressurized flametube combustion chamber under acoustically isolated conditions. A nine-point swirl venturi lean direct injection (SV-LDI) geometry was evaluated at inlet pressures up to 2,413 kPa and non-vitiated air temperatures up to 867 K. The equivalence ratio was varied to obtain adiabatic flame temperatures between 1388 K and 1905 K. Dynamic pressure measurements were taken upstream of the SV-LDI, in the combustion zone and downstream of the exit nozzle. The measurements showed that combustion dynamics were fairly small when the fuel was distributed uniformly and mostly due to fluid dynamics effects. Dynamic pressure fluctuations larger than 40 kPa at low frequencies were measured at 653 K inlet temperature and 1117 kPa inlet pressure when fuel was shifted and the pilot fuel injector equivalence ratio was increased to 0.72.

dynamics↗

NASA NTRS1984

Ceramic composite liner material for gas turbine combustors

The application of ceramics to gas turbine combustor liners to reduce liner metal temperature was studied in an experiment in which yttria-stabilized zirconia plasma was sprayed on compliant metal substrates exposed to near stoichiometric combustion. The strain isolation pad materials chosen were Hoskins Alloy 875 and BRUNSLLOY 534 Fiber Metal of 0.25 and 0.38 cm thicknesses and 35 and 45 percent density levels. Combustor screening tests of all specimens showed no evidence of deterioration or failure. Specimens exposed to flame temperatures in excess of 2100 K were convectively or convective-transpiration cooled and were evaluated in a 10 cm sq flame tube at inlet air temperature of 533 K and pressure of 0.5 MPa. The results suggest the superiority of a system composed of the Hoskins Alloy 875 compliant pad with 0.25 cm thickness and 35 percent density coupled with a NiCrAlY bond coat and a 8 percent Y2O3-ZrO2 ceramic top coat of 0.19 cm thickness.

Ercegovic, D. B.↗

NASA NTRS2007

Flame Radiation, Structure, and Scalar Properties in Microgravity Laminar Fires

Results from microgravity combustion experiments conducted in the Zero Gravity Research Facility (ZGF) 5.18 second drop facility are reported. The results quantify flame radiation, structure, and scalar properties during the early phase of a microgravity fire. Emission mid-infrared spectroscopy measurements have been completed to quantitatively determine the flame temperature, water and carbon dioxide vapor concentrations, radiative emissive power, and soot concentrations in microgravity laminar methane/air, ethylene/nitrogen/air and ethylene/air jet flames. The measured peak mole fractions for water vapor and carbon dioxide are found to be in agreement with state relationship predictions for hydrocarbon/air combustion. The ethylene/air laminar flame conditions are similar to previously reported results including those from the flight project, Laminar Soot Processes (LSP). Soot concentrations and gas temperatures are in reasonable agreement with similar results available in the literature. However, soot concentrations and flame structure dramatically change in long-duration microgravity laminar diffusion flames as demonstrated in this report.

Feikema, Douglas↗

NASA NTRS1981

High temperature durable catalyst development

A program has been carried out to develop a catalytic reactor capable of operation in environments representative of those anticipated for advanced automotive gas turbine engines. A reactor consisting of a graded cell honeycomb support with a combination of noble metal and metal oxide catalyst coatings was built and successfully operated for 1000 hr. At an air preheat temperature of 740 K and a propane/air ratio of 0.028 by mass, the adiabatic flame temperature was held at about 1700 K. The graded cell monolithic reaction measured 5 cm in diameter by 10.2 cm in length and was operated at a reference velocity of 14.0 m/s at 1 atm. Measured NOx levels remained below 5 ppm, while unburned hydrocarbon concentrations registered near zero and carbon monoxide levels were nominally below 20 ppm.

Snow, G. C.↗

NASA NTRS1936

Combustion-engine Temperatures by the Sodium Line-reversal Method

The sodium line-reversal method has been used in some preliminary measurements of flame temperature. Improvements in the method involving a photographic recorder and a means of correcting for the dirtiness of the windows are described. The temperatures so obtained are compared with those calculated from pressure diagrams.

Brevoort, Maurice J↗

NASA NTRS2001

Structure and Early Soot Oxidation Properties of Laminar Diffusion Flames

Soot is an important unsolved problem of combustion science because it is present in most hydrocarbon-fueled flames and current understanding of the reactive and physical properties of soot in flame environments is limited. This lack of understanding affects progress toward developing reliable predictions of flame radiation properties, reliable predictions of flame pollutant emission properties and reliable methods of computational combustion, among others. Motivated by these observations, the present investigation extended past studies of soot formation in this laboratory, to consider soot oxidation in laminar diffusion flames using similar methods. Early work showed that O2 was responsible for soot oxidation in high temperature O2-rich environments. Subsequent work in high temperature flame environments having small O2 concentrations, however, showed that soot oxidation rates substantially exceeded estimates based on the classical O2 oxidation rates of Nagle and Strickland-Constable and suggests that radicals such as O and OH might be strong contributors to soot oxidation for such conditions. Neoh et al. subsequently made observations in premixed flames, supported by later work, that showed that OH was responsible for soot oxidation at these conditions with a very reasonable collision efficiency of 0.13. Subsequent studies in diffusion flames, however, were not in agreement with the premixed flame studies: they agreed that OH played a dominant role in soot oxidation in flames, but found collision efficiencies that varied with flame conditions and were not in good agreement with each other or with Neoh et al. One explanation for these discrepancies is that optical scattering and extinction properties were used to infer soot structure properties for the studies that have not been very successful for representing the optical properties of soot. Whatever the source of the problem, however, these differences among observations of soot oxidation in premixed and diffusion flames clearly must be resolved. Motivated by these findings, the present study undertook measurements of soot and flame properties within the soot oxidation region of some typical laminar diffusion flames and exploited the new measurements to identify soot oxidation mechanisms for these conditions. Present considerations were limited to the early stages of soot oxidation (carbon consumption less than 70%) where reactions at the surface of primary soot particles dominate the process, rather than the later stages when particle porosity and internal particle oxidation become important as discussed by Neoh et al.

El-Leathy, A. M.↗

NASA NTRS2003

Characteristics of Gaseous Diffusion Flames with High Temperature Combustion Air in Microgravity

The characteristics of gaseous diffusion flames have been obtained using high temperature combustion air under microgravity conditions. The time resolved flame images under free fall microgravity conditions were obtained from the video images obtained. The tests results reported here were conducted using propane as the fuel and about 1000 C combustion air. The burner included a 0.686 mm diameter central fuel jet injected into the surrounding high temperature combustion air. The fuel jet exit Reynolds number was 63. Several measurements were taken at different air preheats and fuel jet exit Reynolds number. The resulting hybrid color flame was found to be blue at the base of the flame followed by a yellow color flame. The length and width of flame during the entire free fall conditions has been examined. Also the relative flame length and width for blue and yellow portion of the flame has been examined under microgravity conditions. The results show that the flame length decreases and width increases with high air preheats in microgravity condition. In microgravity conditions the flame length is larger with normal temperature combustion air than high temperature air.

Ghaderi, M.↗

NASA NTRS1985

On the determination of laminar flame speeds from stretched flames

The effects of stretch on the determination of the laminar flame speed are experimentally studied by using the positively-stretched stagnation flame and negatively-stretched bunsen flame, and by using lean and rich mixtures of methane, propane, butane, and hydrogen with air whose effective Lewis numbers are either greater or less than unity. Results demonstrate that flame speed determination can be influenced by stretch through two factors: (1) Preferential diffusion which tends to increase or decrease the flame temperature and burning rate depending on the effective Lewis number, and (2) Flow divergence which causes the flame speed to assume higher values when evaluated at the upstream boundary of the preheat zone instead of the reaction zone. Recent data on flame speed including the present ones are then examined from the unified viewpoint of flame stretch, leading to satisfactory resolution of the discrepancies between them. The present study also proposes a methodology of determining the laminar flame speeds by using the stagnation flame and linearly extrapolating the data to zero stretch rate.

Wu, C. K.↗

NASA NTRS1994

Radiative Heat Transfer in Finite Cylindrical Enclosures with Nonhomogeneous Participating Media

Results of a numerical solution for radiative heat transfer in homogeneous and nonhomogeneous participating media are presented. The geometry of interest is a finite axisymmetric cylindrical enclosure. The integral formulation for radiative transport is solved by the YIX method. A three-dimensional solution scheme is applied to two-dimensional axisymmetric geometry to simplify kernel calculations and to avoid difficulties associated with treating boundary conditions. As part of the effort to improve modeling capabilities for turbulent jet diffusion flames, predicted distributions for flame temperature and soot volume fraction are used to calculate radiative heat transfer from soot particles in such flames. It is shown that the nonhomogeneity of radiative property has very significant effects. The peak value of the divergence of radiative heat flux could be underestimated by 2 factor of 7 if a mean homogeneous radiative property is used. Since recent studies have shown that scattering by soot agglomerates is significant in flames, the effect of magnitude of scattering is also investigated and found to be nonnegligible.

Hsu, Pei-Feng↗

NASA NTRS1972

Measurement of temperature profiles in flames by emission-absorption spectroscopy

An investigation was conducted to explore the use of infrared and ultraviolet emission-absorption spectroscopy for determination of temperature profiles in flames. Spectral radiances and absorptances were measured in the 2.7-micron H2O band and the 3064-A OH band in H2/O2 flames for several temperature profiles which were directly measured by a sodium line-reversal technique. The temperature profiles, determined by inversion of the infrared and ultraviolet spectra, showed an average disagreement with line-reversal measurements of 50 K for the infrared and 200 K for the ultraviolet at a temperature of 2600 K. The reasons for these discrepancies are discussed in some detail.

Simmons, F. S.↗

NASA NTRSDate not supplied

Fire Safety Implications of Preliminary Results from Saffire IV and V Experiments on Large Scale Spacecraft Fires

The spread and growth of flames over large solid fuel samples and their effect on the pressurized spacecraft were studied inside the Cygnus spacecraft while in orbit after departing the International Space Station. These experiments were developed by NASA’s Advanced Exploration Systems Division in the Human Exploration and Operations Mission Directorate. The ignited materials consisted of poly-methyl methacrylate (PMMA), cotton fabric and a cotton/fiberglass fabric blend. The samples were all 40 cm wide and with various lengths ranging from 18 cm for the PMMA samples to 50 cm for the fabrics. The overall results from these tests and their impact on the spacecraft are presented with emphasis on the fire safety implications of the results. The experiments included, a post-fire cleanup system, vehicle internal volume measurements, and transport of acid gases (HCl and HF). Measurements included video images, flame spread rate, flame temperatures and radiant heat output; energy release through oxygen calorimetry; distributed measurements of CO2 concentration and temperature at six locations in the spacecraft; CO2, CO, O2, HF and HCl concentrations; vehicle pressurized volume; and aerosol concentrations. Details of the flame growth and spread are discussed in other papers as are details of the post-fire cleanup system performance. The fire events had a measurable impact on the vehicle pressure, temperature, and carbon dioxide concentration. However, despite having heat release rates up to 10 kW, the average vehicle conditions did not rise to unacceptable levels. The combined results of the experiments provide significant new understanding of the impact of sample and flow duct height on flame spread and growth in addition to an improved perspective of the impact of a fire event on a spacecraft.

micorgravity↗

NASA NTRSDate not supplied

Fire Safety Implications of Preliminary Results from Saffire IV and V Experiments on Large Scale Spacecraft Fires

microgravity fire safety↗

NASA NTRS1986

Diffusion flame extinction in slow convenctive flow under microgravity environment

A theoretical analysis is presented to study the extinction characteristics of a diffusion flame near the leading edge of a thin fuel plate in slow, forced convective flows in a microgravity environment. The mathematical model includes two-dimensional Navier-Stokes momentum, energy and species equations with one-step overall chemical reaction using second-order finite rate Arrhenius kinetics. Radiant heat loss on the fuel plate is applied in the model as it is the dominant mechanism for flame extinguishment in the small convective flow regime. A parametric study based on the variation of convective flow velocity, which varies the Damkohler number (Da), and the surface radiant heat loss parameter (S) simultaneously, is given. An extinction limit is found in the regime of slow convective flow when the rate of radiant heat loss from fuel surface outweighs the rate of heat generation due to combustion. The transition from existent envelope flame to extinguishment consists of gradual flame contraction in the opposed flow direction together with flame temperature reduction as the convective flow velocity decreases continuously until the extinction limit is reached. A case of flame structure subjected to surface radiant heat loss is also presented and discussed.

Chen, C. H.↗

NASA NTRS1986

Diffusion flame extinction in slow convection flow under microgravity environment

A theoretical analysis is presented to study the extinction characteristics of a diffusion flame near the leading edge of a thin fuel plate in slow, forced convective flows in a microgravity environment. The mathematical model includes two-dimensional Navier-Stokes momentum, energy and species equations with one-step overall chemical reaction using second-order finite rate Arrhenius kinetics. Radiant heat loss on the fuel plate is applied in the model as it is the dominant mechanism for flame extinguishment in the small convective flow regime. A parametric study based on the variation of convective flow velocity, which varies the Damkchler number (Da), and the surface radiant heat loss parameter (S) simultaneously, is given. An extinction limit is found in the regime of slow convective flow when the rate of radiant heat loss from fuel surface outweighs the rate of heat generation due to combustion. The transition from existent envelope flame to extinguishment consists of gradual flame contraction in the opposed flow direction together with flame temperature reduction as the convective flow velocity decreases continuously until the extinction limit is reached. A case of flame structure subjected to surface radiant heat loss is also presented and discussed.

Chen, Chiun-Hsun↗