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DOE OSTI2013

Temporal Variability of Aerosol Properties during TCAP: Impact on Radiative Forcing

Ground-based remote sensing and in situ observations of aerosol microphysical and optical properties have been collected during summertime (June-August, 2012) as part of the Two-Column Aerosol Project (TCAP; http://campaign.arm.gov/tcap/), which was supported by the U.S. Department of Energy’s (DOE’s) Atmospheric Radiation Measurement (ARM) Program (http://www.arm.gov/). The overall goal of the TCAP field campaign is to study the evolution of optical and microphysical properties of atmospheric aerosol transported from North America to the Atlantic and their impact on the radiation energy budget. During TCAP, the ground-based ARM Mobile Facility (AMF) was deployed on Cape Cod, an arm-shaped peninsula situated on the easternmost portion of Massachusetts (along the east coast of the United States) and that is generally downwind of large metropolitan areas. The AMF site was equipped with numerous instruments for sampling aerosol, cloud and radiative properties, including a Multi-Filter Rotating Shadowband Radiometer (MFRSR), a Scanning Mobility Particle Sizer (SMPS), an Aerodynamic Particle Sizer (APS), and a three-wavelength nephelometer. In this study we present an analysis of diurnal and day-to-day variability of the column and near-surface aerosol properties obtained from remote sensing (MFRSR data) and ground-based in situ measurements (SMPS, APS, and nephelometer data). In particular, we show that the observed diurnal variability of the MFRSR aerosol optical depth is strong and comparable with that obtained previously from the AERONET climatology in Mexico City, which has a larger aerosol loading. Moreover, we illustrate how the variability of aerosol properties impacts the direct aerosol radiative forcing at different time scales.

aerosol microphysical and optical properties↗

DOE OSTI2016

Use of a Ca-Citrate-Phosphate Solution to Form Hydroxyapatite for Uranium Stabilization of Old Rifle Sediments: Laboratory Proof of Principle Studies

The Old Rifle Site is a former vanadium and uranium ore-processing facility located adjacent to the Colorado River and approximately 0.3 miles east of the city of Rifle, CO. The former processing facilities have been removed and the site uranium mill tailings are interned at a disposal cell north of the city of Rifle. However, some low level remnant uranium contamination still exists at the Old Rifle site. In 2002, the United States Nuclear Regulatory Commission (US NRC) concurred with United States Department of Energy (US DOE) on a groundwater compliance strategy of natural flushing with institutional controls to decrease contaminant concentrations in the aquifer. In addition to active monitoring of contaminant concentrations, the site is also used for DOE Legacy Management (LM) and other DOE-funded small-scale field tests of remediation technologies. The purpose of this laboratory scale study was to evaluate the effectiveness of a hydroxyapatite (Ca 10 (PO 4 ) 6 (OH) 2 ) permeable reactive barrier and source area treatment in Old Rifle sediments. Phosphate treatment impact was evaluated by comparing uranium leaching and surface phase changes in untreated to PO 4 -treated sediments. The impact of the amount of phosphate precipitation in the sediment on uranium mobility was evaluated with three different phosphate loadings. A range of flow velocity and uranium concentration conditions (i.e., uranium flux through the phosphate-treated sediment) was also evaluated to quantify the uranium uptake mass and rate by the phosphate precipitate.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

NASA NTRS2018

Development of the Multi-Purpose Transportation System for the Space Launch System (SLS) Core Stage (CS) Flight Article

NASA's Multi-Purpose Transportation System (MPTS) is designed to transport the Space Launch System (SLS) vehicle segments by waterway and roadway. It is tasked with transporting the vehicle from where it is manufactured to its intermediate test location and final launch destination. Its design incorporates mechanisms that release degrees of freedom to prevent excessive loading during transit and ensure a successful delivery of the vehicle to its intended destination. In addition to the Core Stage (CS) flight article, the system will also move three Structural Test Articles (STAs), the Dynamic Demonstration Unit (DDU), and a simulated CS Pathfinder (weight, center of gravity, outer mold line dimensions, and overall length) over road terrain at four NASA centers and on the Pegasus barge. The MPTS independently supports the article at both ends while operating as a combined unit through automated monitoring of its released degree of freedom and corrective responses. This allows the system to constrain its payload in a statically determinate manner while traversing highly variable terrain. Multi-body simulation of the transportation route is useful to predict free-body motion within its range of mobility. The MPTS has completed its design and analysis developmental cycles. This paper describes the design challenges encountered in developing this system of large-scale structure, which incorporates complex mechanisms. The unique techniques and methodologies developed for analytical assessment of the hardware are also discussed.

Sandridge, Sarah↗

NASA NTRS2013

Project Profile: Hydrogen Fuel Cell Mobile Lighting Tower (HFCML)

NASA is committed to finding innovative solutions that improve the operational performance of ground support equipment while providing environment and cost benefits, as well. Through the Hydrogen Fuel Cell Mobile Lighting Tower (HFCML) project, NASA gained operational exposure to a novel application of high efficiency technologies. Traditionally, outdoor lighting and auxiliary power at security gates, launch viewing sites, fallback areas, outage support, and special events is provided by diesel generators with metal halide lights. Diesel generators inherently contribute to C02, NOx, particulate emissions, and are very noisy. In 2010, engineers from NASA's Technology Evaluation for Environmental Risk Mitigation Principal Center (TEERM) introduced KSC operations to a novel technology for outdoor lighting needs. Developed by a team led by Sandia National Laboratory (SNL), the technology pairs a 5kW hydrogen fuel cell with robust high efficiency plasma lights in a towable trailer. Increased efficiency, in both the fuel cell power source and lighting load, yields longer run times between fueling operations while providing greater auxiliary power. Because of the unit's quiet operation and no exhaust fumes, it is capable of being used indoors and in emergency situations, and meets the needs of all other operational roles for metal halide/diesel generators. The only discharge is some water and warm air. Environmental benefits include elimination of diesel particulate emissions and estimated 73% greenhouse gas emissions savings when the hydrogen source is natural gas (per GREET model). As the technology matures the costs could become competitive for the fuel cell units which are approximately 5 times diesel units. Initial operational . concerns included the hydrogen storage tanks and valves, lightning safety/grounding, and required operating and refueling procedures. TEERM facilitated technical information exchange (design drawings, technical standards, and operations manuals) necessary for KSC hydrogen system experts to approve use of the HFCML unit, including initiating the environmental checklist (i.e. exterior lighting waiver due to sea turtles), and development of operations and maintenance instructions. TEERM worked with SNL to establish a bailment agreement for KSC to utilize a Beta unit as part of normal Center Operations for a period of twelve months.

McLaughlin, Russell↗

NASA NTRSDate not supplied

Space Suit Portable Life Support System Thermal Control Valve Ball Design

A Thermal Control Valve (TCV) has been in development for the Exploration Extravehicular Mobility Unit Portable Life Support System (xEMU PLSS). The xEMU PLSS TCV controls flow going to the liquid cooling and ventilation garment that the crew member wears during extra-vehicular activity to expel waste heat. A previous TCV version with a linear actuator and diverter valve has been tested to attempt to control the flow accurately. The previous valve has a non-linear flow response relative to valve position and has struggled to meet the setpoints desired for precise thermal control. While many diverter valve design variations have been attempted, all previous designs have had difficulty meeting set points. Additionally, high precision machining is required to create a metal-on-metal seal which has its own drawbacks and does not always meet requirements for internal leakage. This metal seal also requires stalling a linear actuator to load the seal in compression or tension which has caused sticking failures when stalled. A new approach and design for a TCV has been developed which uses a rotational ball to control flow and has demonstrated a much more precise and linear flow control. The design functions like a two-way ball valve with two Teflon seats that cradle and compress the ball for sealing. The ball outlet has a unique geometric design to create a set-able orifice like hole which is more predictable at controlling flow. Additionally, the Teflon seat performs much better for preventing internal leakage than the metal seal and prevents sticking by having a large range in which it is sealed without having to stall the actuator. This paper will review a new proposed xEMU PLSS TCV ball design and compare it with previous iterations of the design.

Ryan Ogilvie↗

NASA NTRSDate not supplied

Space Suit Portable Life Support System Thermal Control Valve Ball Design

Ryan Ogilvie↗

DOE OSTI2019

Experimental Investigation of a Novel High Energy Density Mobile Sorption–based Thermal Battery

Around 20% of the total primary energy use in the United States is for thermal demands of buildings, such as space cooling, dehumidification, and space heating. Low-grade geothermal energy is abundant and could effectively satisfy these thermal demands. However, low-grade geothermal energy is underused because geothermal fluids have an energy density too low to justify transportation between the existing resources and buildings. The mobile sorption-based thermal battery (MSTB) system was thus developed to store the low-temperature heat using three-phase (vapor-liquid solution-solid crystal) sorption technology with a much higher energy density than a geothermal fluid provides. The energy density of an MSTB is over 6 times that of conventional hot water, enabling economical long-distance transport of low-temperature heat for thermal end uses. This can alleviate peak demand on the electricity grid by offsetting space-conditioning loads, improving the reliability and resilience of US energy systems. High energy density, fast crystallization, and crystal dissolution of the sorption material are critical to the viability and performance of the MSTB system. Therefore, the design and operation of MSTB systems must ensure effective generation and dissolution of the salt crystals inside the MSTB. To achieve this target, this study developed a prototype MSTB and its testing apparatus, and experimentally investigated the prototype MSTB. The crystallization and dissolution performance were also theoretically defined and quantified. The experimental results showed that the prototype MSTB was able to achieve an energy storage density of 903.0 kJ/kg and a maximum discharge rate of 1.3 kW. This study proves the feasibility and high performance of the MSTB concept, which is helpful to further study and development of the MSTB system.

Wang, Lingshi↗

NASA NTRSDate not supplied

Space Suit Portable Life Support System Thermal Control Valve Ball Design

A Thermal Control Valve (TCV) has been in development for the Exploration Extravehicular Mobility Unit Portable Life Support System (xEMU PLSS). The xEMU PLSS TCV controls flow going to the liquid cooling and ventilation garment that the crew member wears during extra-vehicular activity to expel waste heat. A pervious TCV version with a linear actuator and diverter valve has been tested extensively to attempt to control the flow accurately. The previous TCV diverter valve has a non-linear flow response relative to valve position and has struggled to accurately meet the setpoints desired for precision thermal control. While many diverter valve design variations have been attempted, previous designs have all had difficulty in meeting set points. Additionally, high precision machining is required for these diverter valves to create a metal-on-metal seal which has its own drawbacks and doesn’t always meet requirements for internal leakage. This metal compression seal also requires stalling the linear actuator to load the seal in compression or tension which has demonstrated valve sticking failures when stalled. The xEMU PLSS TCV implements a new approach and design for a TCV which uses a rotational ball to control flow and has demonstrated a much more precise and linear flow control. The design functions like a two-way ball valve with two Teflon seats that cradle and compress the ball for sealing. A new geometric design modification to the ball outlet can create a set-able orifice like hole which is more predictable at controlling flow than using an annulus with the previous diverter valve. Additionally, the Teflon seat performs much better for preventing internal leakage than the metal seal and prevents sticking by having a large range in which it is sealed without having to stall the actuator. This paper will review a new proposed xEMU PLSS TCV ball design and compare it with previous iterations of the design.

Ryan Ogilvie↗

DOE OSTI2025

Summary of Factory Fueling and Testing Risks to Support the Transformation of Regulatory Requirements for Microreactors

Microreactors have the potential to open new markets and applications for nuclear energy. New manufacturing and operational regimes, such as factory fueling and testing prior to site installation, are being proposed to meet these new markets. The radiological hazards associated with traditional commercial power reactors are not the same as the hazards of a reactor being constructed in a factory. Currently, a reactor operating license specified under 10 CFR Part 50, Part 52, or (in the near future) Part 53 is required prior to loading fuel in the reactor. This is logical for plants that are immediately to begin full-power operations soon after fuel loading. However, for microreactors, this may not be the case. Some deployment concepts may stage reactors as “ready to go” in a factory prior to site installation and startup. This approach is being considered in the case of diesel generator replacements, mobile or roaming mining operations, and emergency response situations, such as after a major disaster event. Therefore, it is necessary to evaluate hazards assuming low power operation for a short irradiation time. This report investigates the primary hazards unique to microreactors associated with low power reactor and physics tests necessary to confirm core safety assumptions, neutronic and core design performance parameters, and other assumptions.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

DOE OSTI2026

Structure and Flow-Viscosity of Filled-Polymer-Based 3D Printing Ink: Exploration through Coarse-Grained Molecular Dynamics

The addition of nanofiller particles to a polymer matrix has long been known to enhance or modify the composite’s mechanical and rheological properties. However, quantitatively capturing such changes with molecular level simulations remains computationally challenging. Toward that goal, we performed coarse-grained molecular dynamics of a nanocomposite system at a fixed (25 vol %) filler loading under nonspecific, weak polymer–filler interactions representative of a broad class of technologically important materials. We report several interesting results, including: (1) the equilibrium chain-configuration remains Gaussian-like as in an unfilled melt; (2) smaller filler particles display a stronger tendency to cluster; (3) larger fillers act as plasticizers by reducing the entanglement density and accelerating the chain mobility; and (4) fillers enhance the tensile response modulus, with the effect being stronger for larger particles. We also simulate cluster breakup, yielding, and elongational flow under an applied time-linear tensile strain and study the flow viscosity as a function of filler-size and chain-length.

Materials science↗

DOE OSTI2025

Operando Neutron Imaging of Lithium Flux and Gradient Cathode Design for Enhanced Kinetics in High‐Loading All‐Solid‐State Li─S Batteries

All-solid-state Li–sulfur batteries (ASSLSBs) are considered promising candidates for next-generation energy storage owing to their inherent safety, high energy density, and abundant sulfur resources. However, slow redox kinetics greatly limit sulfur utilization during solid-solid sulfur reactions, leading to significant challenges to achieve efficient performance in high-mass-loading ASSLSBs. Here, operando neutron image is employed to directly visualize, for the first time, that sluggish Li + transport kinetics and the uneven distribution of Li + during cathodic reactions are critical factors limiting sulfur conversion. To address this issue, gradient cathode architectures comprising three and five layers are designed, in which catholyte concentrations are strategically varied to optimize Li-ion flux and enhance ionic conductivity of the whole composite cathode electrode. Operando neutron imaging distinctly visualizes and confirms that three-layer gradient approach significantly enhances Li-ion mobility, resulting in more uniform redox reactions and greatly improved sulfur utilization compared to traditional non-gradient structures. Consequently, the three-layer gradient cathode achieves superior rate performance and reduced electrode polarization at high sulfur mass loadings of 4.5 and 6.0 mg cm −2 . Furthermore, the applicability and scalability of this design are demonstrated in a five-layer gradient cathode architecture, achieving an impressive discharge specific capacity increase from 656 mAh g −1 (three-layer gradient) to 1232 mAh g −1 at 1/20 C for ultra-high sulfur loading of 7.5 mg cm −2 . In conclusion, this innovative gradient cathode design offers substantial advancements in understanding and overcoming Li-ion transport limitations, paving the way toward practical, high-energy-density ASSLSBs.

25 ENERGY STORAGE↗

DOE OSTI2025

Water effects on NH 3 -SCR over Cu-based small-pore zeolite catalysts: A review

The selective catalytic reduction (SCR) of NO x with NH 3 as the reductant over small-pore Cu-zeolite catalysts is a leading strategy for controlling emissions from diesel engines and mobile sources. While the hydrothermal stability of Cu-zeolites such as Cu-SSZ-13, Cu-SAPO-34, and Cu-SSZ-39 has been extensively studied, the multifaceted role of water vapor under operating conditions has only recently received systematic attention. Water impacts multiple aspects of SCR catalysis, including NO x conversion, N 2 O formation, Cu ion speciation, redox kinetics, and surface reactions. This review comprehensively summarizes recent advances in understanding the effect of water on NH 3 -SCR over Cu-based catalysts. For Cu-SSZ-13, water vapor induces both inhibitory and promotive effects depending on temperature, Cu loading, and Si/Al ratio by altering NH 3 adsorption, Cu mobility, and redox half-cycle kinetics. Studies have revealed that water can suppress ammonium nitrate formation at low temperatures and enhance nitrate pathways at higher temperatures. Over Cu-SAPO-34, water promotes NO conversion by improving Cu(II) reducibility and strengthening Brønsted acidity. First-principles calculations confirm that water-coordinated Cu species lower O 2 activation barriers. In Cu-SSZ-39, water was found to facilitate Cu reduction, migration, and O 2 activation, resulting in superior water tolerance and unexpected catalytic promotion. Both experimental and computational studies highlight that water vapor exerts complex, catalyst-dependent effects on NH 3 -SCR performance, underscoring the need for tailored catalyst designs that leverage beneficial water interactions while minimizing inhibitory impacts.

Ammonia selective catalytic reduction↗

NASA NTRSDate not supplied

Analytical Review of Exploration Extravehicular Mobility Unit Heat Rejection Performance

The Primary Thermal Control Loop (PTCL) in the Exploration Extravehicular Mobility Unit (xEMU) uses a Spacesuit Water Membrane Evaporator (SWME) to provide cooling for the crew member and spacesuit avionics. A secondary emergency cooling system, the Auxiliary Thermal Control Loop (ATCL), also uses a smaller version of the SWME, called the Mini-ME, in the event of a failure in the primary system. These are integral to the comfort of the crew member (through heat rejection) during an Extravehicular Activity (EVA). This paper examines the effectiveness of the heat rejection of the PTCL and the ATCL during thermal vacuum testing and the absolute limit of heat rejection to maintain an approximately 10C outlet temperature. During this thermal vacuum test, the PTCL was taken from a heat input of 0W up to 900W, far past the design point, and the ATCL was tested from 0W to 300W. Testing showed that the PTCL and the ATCL can maintain crew member outlet temperature throughout an entire 8-hour thermally controlled EVA environment (hot and cold). The results and effectiveness of the test will be detailed throughout this paper for all EVAs (whether a full mapping profile or a standard continuous heat load).

PLSS↗

DOE OSTI2016

SU-F-T-670: From the OR to the Radiobiology Lab: The Journey of a Small X-Ray Source

Purpose: Irradiation of small animal tumor models within laboratories is vital to radiobiological experiments. Often the animals are not able to be brought back into the lab after being taken out for irradiation. Cell biology laboratories benefit from irradiation capability available around the clock without regard to patient load in an associated radiotherapy clinic. Commercial systems are available, but bulky and expensive. Methods: An intraoperative kV irradiation system (IntraBeam™) designed to deliver spherical dose distributions to surgical cavities has been repurposed for the irradiation of cell plates and small laboratory animals. An applicator has been altered to allow for simple, open fields. Special collimators are being developed. BEAMnrc Monte Carlo simulations with the “NRC swept BEAM” source model have been performed to characterize the dose distributions, to develop optimal collimators and as basis for dose prescription. Measurements with radiochromic film and with an ionization chamber were performed to characterize the beam and to validate the simulations. Results: Using its highest setting (50 kV and 40 µA) the x-ray unit is capable of delivering dose rates over 1 Gy/min homogeneously to standard cell plates even without an optimized collimator. Smaller areas (tumors in animals) can be irradiated with significantly higher dose rates (> 20 Gy/min) depending on distance of the source to the tumor. The HVL was found to be 0.21 mm Al which means the shielding requirements for the device are easily achievable in the lab. Conclusion: A mobile irradiation facility is feasible. It will allow easier access to radiation for radiobiology experiments. The modified system is versatile in that for cell plates homogenous irradiations can be achieved through distance from the source, while for high dose rate small field irradiations the source can be brought in close proximity to the target.

60 APPLIED LIFE SCIENCES↗

DOE OSTI2018

U.S. Light-Duty Vehicle Air Conditioning Fuel Use and Impact of Solar/Thermal Control Technologies

To reduce fuel consumption and carbon dioxide (CO2) emissions from mobile air conditioning (A/C) systems, 'U.S. Light-Duty Vehicle Greenhouse Gas Emissions and Corporate Average Fuel Economy Standards' identified solar/thermal technologies such as solar control glazings, solar reflective paint, and active and passive cabin ventilation in an off-cycle credit menu. National Renewable Energy Laboratory (NREL) researchers developed a sophisticated analysis process to calculate U.S. light-duty A/C fuel use that was used to assess the impact of these technologies, leveraging thermal and vehicle simulation analysis tools developed under previous U.S. Department of Energy projects. Representative U.S. light-duty driving behaviors and weighting factors including time-of-day of travel, trip duration, and time between trips were characterized and integrated into the analysis. In addition, U.S. weather conditions weighted based on light-duty vehicle registrations were generated and used for the analysis. Three representative vehicle types for the light-duty fleet were selected based on registration data containing vehicle size information. These key inputs were used to support a weighted parametric analysis that quantified vehicle thermal load, vehicle accessory load, and vehicle fuel use. This analysis estimates that 7.6 billion gallons of fuel a year are used in the United States for vehicle A/C, equivalent to 6.1% of the total national light-duty vehicle fuel use. This equates to 30.0 gallons/year per vehicle or 23.5 grams CO 2 per mile (g/mi) for an average U.S. light-duty vehicle. A/C is a significant contributor to national fuel use; therefore, technologies that reduce A/C loads have an opportunity to reduce fuel consumption, reduce imported oil, and improve energy security. Implementing solar control glass reduced the CO 2 emissions by 2.0 g/mi and the reduction due to solar reflective paint was 0.8 g/mi. The active and passive ventilation strategies as defined in this analysis only reduced emissions by 0.1 and 0.2 g/mi, respectively. This analysis shows the potential to reduce operational costs, A/C fuel use, and CO 2 emissions by implementing advanced vehicle climate control technologies including the solar/thermal technologies.

29 ENERGY PLANNING, POLICY, AND ECONOMY↗

DOE OSTI2022

Sensing Electrical Networks Securely & Economically (SENSE)

The growing adoption of distributed energy resources (DERs) like battery energy storage systems and roof top solar/PV and the rapid penetration of electric vehicles (EVs), the electric grid is undergoing a major transformation with elevated stress on legacy grid assets. Despite a lot of expenditure to address these challenges, both in dollars and manpower, utilities have not been able to receive the value that was promised. The gains have been most visible at the transmission and substation level, especially where the main objective was improving operational and economic efficiency for the utility. Improving visibility and control at a few select points enhances the existing and established paradigm of centralized command and control. With changing load patterns, load types and the overall transition to an “active grid”, the centralized control and coordination paradigm gets challenged. To address the challenges, a new architecture and mechanism is needed, one that supports decentralized control and decision making, extracting value streams at the grid edge, particularly as the changes are fueled by transitions occurring in the distribution system. To address this, a communications and data processing platform, “GAMMA” was developed and demonstrated through the project. At the heart of the platform, are distributed, intelligent edge nodes with sensing and compute capabilities, that can record and analyze information locally. They are embedded in sensors and actuators specific to different distribution system applications. Phase 1 of the project focused on developing novel sensor technology that can be used for monitoring utility pole top distribution transformers. The sensors were designed with the objective of being low-cost, communicating with the GAMMA cloud using novel “delay-tolerant” networking using Bluetooth and a secure mobile application. They were non-intrusive in nature so that they can be installed quickly in the field, resulting in overall low cost of deployment and operations. Following the successful completion of Phase 1, the team manufactured 100 units for a field demonstration in Phase 2. The field demonstration was carried out on two real feeder systems with the local utility partner. In total, 100 sensors were installed and operated over a period of 6 months in the state of Georgia. The platform is operational end to end, with the cloud infrastructure deployed on a distributed, serverless environment that can serve multiple data streams, an analytics engine and a portal to securely view the data from multiple assets. The data collected through the GAMMA Mobile Phone app showcased the viability of the novel delay tolerant networking architecture, and the data processing algorithms developed through the course of the project, were successful in extracting important information about the overall network, improving the utility’s visibility and situational awareness in the distribution feeder.

24 POWER TRANSMISSION AND DISTRIBUTION↗

DOE OSTI2026

Urban wash-off of tire wear particles

Tire wear particles (TWPs) are an important class of microplastics due to their toxicity and abundance. Because most TWPs are generated on impervious road surfaces, urban wash-off is the critical first phase of waterborne transport from their zone of production to stormwater drainage. However, little is known about the driving factors behind their mobilization. In this study, we use a rainfall simulator to investigate how surface roughness, rainfall intensity, and surface slope affect wash-off behaviors of TWPs. We also analyze how the size and shape of mobilized TWPs change over the course of simulated storm events. We found that low surface roughness, high rainfall intensity (most significant factor), and low slope result in the most rapid conveyance of TWP load. On average, large particles (>1000 µm) travelled faster than small particles (<125 µm). Particle shape explained a very small amount of variance in TWP wash-off velocity but was found to be more important under higher surface roughness conditions. In addition to wash-off velocity, we found similar conditions controlled the percent mobilization of TWPs. Low surface roughness and high rainfall intensity resulting in higher TWP wash-off rates is consistent with mineral sediment wash-off behavior. Conversely, low surface slope and large particle size leading to faster conveyance is directly opposed to mineral sediment wash-off. Our findings suggest drag-dominated flow and that sufficient runoff depth is the most important parameter governing TWP wash-off. These findings are important first steps to understanding wash-off behaviors of TWPs and informing future modeling efforts and mitigation strategies.

13 HYDRO ENERGY↗

DOE OSTI2017

Black Carbon at the Mt. Bachelor Observatory Field Campaign Report

This campaign was initiated to measure refractory black carbon (rBC, as defined in Schwarz et al. (2010)) at the Mt. Bachelor Observatory (MBO) using the U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) Climate Research Facility single-particle soot photometer (SP2; unit 54). MBO is a high-elevation site located on the summit of Mt. Bachelor in central Oregon, USA (43.979°N, 121.687°W, 2,763 meters ASL). This site is operated by Professor Dan Jaffe’s group at the University of Washington Bothell and has been used continuously as an atmospheric observatory for the past 12 years (Jaffe et al., 2005; Gratz et al., 2014). The location of MBO allows frequent sampling of the free troposphere along with a wide array of plumes from regional and distant sources. MBO is currently supported with funding from the National Science Foundation (NSF) to the Principal Investigator (PI; D. Jaffe) via the project “Influence of Free Tropospheric Ozone and PM on Surface Air Quality in the Western U.S.” (#1447832) covering the period 03/15/2015 to 02/28/2018. The SP2 instrument from Droplet Measurement Technologies provides particle-resolved measurements of rBC mass loading, size and mass distributions, and mixing state. The SP2 was installed at MBO on 6/27/2016 and ran through 9/23/2016. Additional measurements at MBO during this campaign included carbon monoxide (CO), fine particulate matter (PM1), aerosol light scattering coefficients (σscat) at three wavelengths using a TSI nephelometer, aerosol absorption coefficients (σabs) with the Brechtel tricolor absorption photometer (TAP), aerosol number size distributions with a scanning mobility particle sizer spectrometer (SMPS), and black carbon (eBC) with an aethalometer. BC data from this campaign have been submitted to the ARM Data Archive. Black carbon (BC) is the predominant light-absorbing aerosol constituent in the atmosphere, and is estimated to exert a positive radiative forcing second only to CO 2 (Ramanathan and Carmichael, 2008). One of the largest sources of BC globally is biomass burning (BB). (Akagi et al., 2011; Andreae and Merlet, 2001; Bond et al., 2013; Bond et al., 2004; Reid et al., 2005b): a source that is likely to increase in the Western U.S. due to climate change (Dennison et al., 2014; Abatzoglon and Williams, 2016; Westerling et al., 2006). Given the likely increased role of BB aerosol in atmospheric forcing, we need to improve our understanding of the physical and optical properties of aged BB aerosol. During the SP2 deployment period at MBO we observed seven BB events, all of which originated from the Gap Fire in Northern California, which burned 33,867 acres in the Klamath National Forest (https://inciweb.nwcg.gov/incident/4997/). Heavy smoke plumes from this fire were transported to MBO from 8/29/2016 to 8/31/2016. We calculated back-trajectories using the National Oceanic and Atmospheric Administration (NOAA) Hybrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) model, version 4 (Draxler, 1999; Draxler and Hess, 1997, 1998; Stein et al., 2015) to confirm transport from the fire locations to MBO. We identified the fire locations using moderate resolution imaging spectroradiometer (MODIS) satellite-derived active fire counts (Justice et al., 2002). Transport time for all of the BB events ranged from 8 to 32 hours.

54 ENVIRONMENTAL SCIENCES↗