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85 records · Page 5

Aerosol hygroscopicity over the South-East Atlantic Ocean during the biomass burning season – Part 2: Influence of sea salt and burning conditions on CCN hygroscopicity

Biomass burning (BB) significantly influences cloud condensation nuclei (CCN) concentrations over the southeastern Atlantic; however, aerosol hygroscopicity (κ) – a key factor for CCN activation – remains poorly constrained during the BB season. This study investigates κ variability using in situ measurements from Ascension Island during the 2016 and 2017 BB seasons. Results show substantial monthly variability, with κ values lowest in August and increasing through October. On average, κ was significantly higher in 2017 (∼ 0.55) than in 2016 (∼ 0.33), suggesting that the aerosols in 2017 were more hygroscopic and more easily activated as CCN. Sulfate and sea salt were the two dominant contributors to κ and the primary drivers of its interannual variability. During the 2017 BB season, sulfate – the major inorganic component – accounted for ∼ 34 % of the submicron aerosol mass, while sea salt, estimated via κ-closure analysis, contributed ∼ 17 %. The higher κ in 2017 was largely attributed to increased sea salt, likely driven by stronger marine winds. Approximately 67 % of sulfate was linked to BB emissions. Variations in BB combustion efficiency, modulated by regional meteorology, influenced sulfate fraction and thus κ values. Specifically, higher relative humidity and lower wind speeds over BB source regions in 2017 favored smoldering combustion, explaining the higher sulfate fraction. Overall, the observed interannual differences in aerosol hygroscopicity reflect the combined impacts of BB combustion characteristics and sea salt emissions, underscoring the critical roles of both BB and marine aerosol sources in regulating aerosol-cloud interactions over the southeastern Atlantic.

54 ENVIRONMENTAL SCIENCES↗

Low-Level Liquid-Bearing Clouds Contribute to Seasonal Lower Atmosphere Stability and Surface Energy Forcing over a High-Mountain Watershed Environment

Measurements of atmospheric structure and surface energy budgets distributed along a high-altitude moun tain watershed environment near Crested Butte, Colorado, from two separate, but coordinated, field campaigns, Surface Atmosphere Integrated field Laboratory (SAIL) and Study of Precipitation, the Lower Atmosphere, and Surface for Hydrometeorology (SPLASH), are analyzed. This study identifies similarities and differences in how clouds influence the radiative budget over one snow-free summer season (2022) and two snow-covered seasons (2021/22; 2022/23) for this alpine location. A relationship between lower-tropospheric stability stratification and longwave radiative flux from the presence or absence of clouds is identified. When low clouds persisted, often with signatures of supercooled liquid in win ter, the lower troposphere experienced weaker stability, while radiatively clear skies that are less likely to be influenced by liquid droplets were associated with appreciably stronger lower-tropospheric stratification. Corresponding surface turbu lent heat fluxes partitioned differently based upon the cloud–stability stratification regime derived from early morning radiosounding profiles. Combined with the differences in the radiative budget largely resulting from dramatic seasonal dif ferences in surface albedo, the lower atmosphere stratification, surface energy budget, and near-surface thermodynamics are shown to be modified by the effective longwave radiative forcing of clouds. The diurnal evolution of thermodynamics and surface energy components varied depending on the early morning stratification state. Thus, the importance of quies cent versus synoptically active large-scale meteorology is hypothesized as a critical forcing for cloud properties and associ ated surface energy budget variations. The physical relationships between clouds, radiation, and stratification can provide a useful suite of metrics for process understanding and to evaluate numerical models in such an undersampled, highly com plex terrain environment.

54 ENVIRONMENTAL SCIENCES↗

Elastic deformation as a tool to investigate watershed storage connectivity

Storage-discharge relationships and dynamic changes in storage connectivity remain key unknowns in understanding and predicting watershed behavior. In this study, we use Global Positioning System measurements of load-induced Earth surface displacement as a proxy for total water storage change in four climatologically diverse mountain watersheds in the western United States. Comparing total water storage estimates with stream-connected storage derived from hydrograph analysis, we find that each of the investigated watersheds exhibits a characteristic seasonal pattern of connection and disconnection between total and stream-connected storage. We investigate how the degree and timing of watershed-scale connectivity is related to the timing of precipitation and seasonal changes in dominant hydrologic processes. Our results show that elastic deformation of the Earth due to water loading is a powerful new tool for elucidating dynamic storage connectivity and watershed discharge response across scales in space and time.

Environmental Sciences & Ecology↗

Energetics of surface melt in West Antarctica

We use reanalysis data and satellite remote sensing of cloud properties to examine how meteorological conditions alter the surface energy balance to cause surface melt that is detectable in satellite passive microwave imagery over West Antarctica. This analysis can detect each of the three primary mechanisms for inducing surface melt at a specific location: thermal blanketing involving sensible heat flux and/or longwave heating by optically thick cloud cover, all-wave radiative enhancement by optically thin cloud cover, and föhn winds. We examine case studies over Pine Island and Thwaites glaciers, which are of interest for ice shelf and ice sheet stability, and over Siple Dome, which is more readily accessible for field work. During January 2015 over Siple Dome we identified a melt event whose origin is an all-wave radiative enhancement by optically thin clouds. During December 2011 over Pine Island and Thwaites glaciers, we identified a melt event caused mainly by thermal blanketing from optically thick clouds. Over Siple Dome, those same 2011 synoptic conditions yielded a thermal-blanketing-driven melt event that was initiated by an impulse of sensible heat flux and then prolonged by cloud longwave heating. The December 2011 synoptic conditions also generated föhn winds at a location on the Ross Ice Shelf adjacent to the Transantarctic Mountains, and we analyze this case with additional support from automatic weather station data. In contrast, a late-summer thermal blanketing period over Pine Island and Thwaites glaciers during February 2013 showed surface melt initiated by cloud longwave heating and then prolonged by enhanced sensible heat flux. One limitation thus far with this type of analysis involves uncertainties in the cloud optical properties. Nevertheless, with improvements this type of analysis can enable quantitative prediction of atmospheric stress on the vulnerable Antarctic ice shelves in a steadily warming climate.

54 ENVIRONMENTAL SCIENCES↗

Heavy metal imprints in Antarctic snow from research and tourism

Antarctica, long regarded as one of the last pristine environments on Earth, is increasingly affected by human activity. As tourism surges and scientific operations expand, air pollution from local emissions is raising new environmental concerns. Here, in this study, we analyze surface snow samples collected along a ~2,000 km transect, from the South Shetland Islands (62°S) to the Ellsworth Mountains (79°S), to map the geochemical fingerprints of aerosol deposition. We identify distinct spatial patterns shaped by crustal, marine, biogenic, and anthropogenic sources. Notably, we detect heavy metal imprints in the snow chemistry of the northern Antarctic Peninsula, where major research stations are concentrated and marine tourism traffic is most intense. Our findings shed light on the extent of the impacts from energy-intensive local activities in Antarctica, underscoring the need for enhanced environmental monitoring and sustainable management strategies in this fragile region.

Cordero, Raúl R. [Univ. of Groningen, Leeuwarden (↗

AmeriFlux FLUXNET-1F US-Bar Bartlett Experimental Forest

This is the AmeriFlux Management Project (AMP) created FLUXNET-1F version of the carbon flux data for the site US-Bar Bartlett Experimental Forest. This is the FLUXNET version of the carbon flux data for the site US-Bar Bartlett Experimental Forest produced by applying the standard ONEFlux (1F) software. Site Description - The Bartlett Experimental Forest (448170 N, 71830 W) is located within the White Mountains National Forest in north-central New Hampshire, USA. The 1050 ha forest extends across an elevational range from 200 to 900 m a.s.l. It was established in 1931 and is managed by the USDA Forest Service Northeastern Research Station in Durham, NH. The climate is humid continental with short, cool summers (mean July temperature, 19.8C) and long, cold winters (mean January temperature, 9.8C). Annual precipitation averages 130 cm and is distributed evenly throughout the year. Soils are developed from glacial till and are predominantly shallow, well-drained spodosols. At lowto mid-elevation, vegetation is dominated by northern hardwoods (American beech, Fagus grandifolia; sugar maple, Acer saccharum; yellow birch, Betula alleghaniensis; with some red maple, Acer rubrum and paper birch, Betula papyrifera). Conifers (eastern hemlock, Tsuga canadensis; eastern white pine, Pinus strobus; red spruce, Picea rubens) are occasionally found intermixed with the more abundant deciduous species but are generally confined to the highest (red spruce) and lowest (hemlock and pine) elevations. In 2003, the site was adopted as a NASA North American Carbon Program (NACP) Tier-2 field research and validation site. A 26.5 m high tower was installed in a low-elevation northern hardwood stand in November, 2003, for the purpose of making eddy covariance measurements of the forest–atmosphere exchange of CO2, H2O and radiant energy. Continuous flux and meteorological measurements began in January, 2004, and are ongoing. Average canopy height in the vicinity of the tower is approximately 20–22 m. In the tower footprint, the forest is predominantly classified into red maple, sugar maple, and American beech forest types. Leaf area index in the vicinity of the tower is 3.6 as measured by seasonal litterfall collection, and 4.5 as measured by the optically based Li-Cor LAI-2000 instrument. Further site information: http://www.fs.fed.us/ne/durham/4155/bartlett.htm

Richardson, Andrew↗

Nature-based solutions in mountain catchments reduce impact of anthropogenic climate change on drought streamflow

Quantifying how well Nature-based Solutions can offset anthropogenic climate change impacts is important for adaptation planning, but has rarely been done. Here we show that a widely-applied Nature-based Solution in South Africa – invasive alien tree clearing – reduces the impact of anthropogenic climate change on drought streamflow. Using a multi-model joint-attribution of climate and landscape-vegetation states during the 2015–2017 Cape Town “Day Zero” drought, we find that anthropogenic climate change reduced streamflow by 12–29% relative to a counterfactual world with anthropogenic emissions removed. This impact on streamflow was larger than corresponding reductions in rainfall (7–15%) and reference evapotranspiration (1.7–2%). Clearing invasive alien trees could have ameliorated streamflow reductions by 3–16% points for moderate invasions levels. Preventing further invasive alien tree spread avoided potential additional reductions of 10–27% points. Total clearing could not have offset the anthropogenic climate change impact completely. Invasive alien tree clearing is an important form of catchment restoration for managing changing hydroclimatic risk, but will need to be combined with other adaptation options as climate change accelerates.

54 ENVIRONMENTAL SCIENCES↗

Impacts of Latent Energy and Snow Fall Speed on a Wintertime Midlatitude Cyclone

This study aimed to understand the impacts of latent energy as well as snow fall speeds on precipitation properties and synoptic-scale storm characteristics of a wintertime midlatitude cyclone. Simulations of a potent winter storm that impacted the Rocky Mountains and northern Great Plains of the United States in February 2017 were performed using the Weather Research and Forecasting model with latent heating or cooling from individual microphysical processes systematically turned off and fall speeds adjusted by ±50%. Results indicated substantial impacts on the microphysical characteristics of the simulated storm to fall speed, cooling from sublimation, and warming from deposition. The impacts of cooling and warming were manifested as differences in accumulated snowfall. Increased (decreased) fall speeds led to smaller (larger) ice crystals and total mass, resulting in offsetting effects on the precipitation flux, and thus minimal impacts on snowfall and large-scale characteristics of the storm. Warming and cooling associated with deposition and sublimation, respectively, impacted the synoptic-scale dynamics, whereby removing warming from deposition resulted in an increased meridional temperature gradient near the jet stream, thus increasing the jet strength and causing it to be more westerly with less curvature aloft. This in turn limited upper-level divergence, creating a weaker surface low and shifting the precipitation shield southward. The opposite occurred with the removal of latent cooling due to sublimation. This study highlights the potential importance of latent energy associated with ice sublimation and deposition and fall speeds in the larger-scale characteristics of winter storms.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Evaluating 3 decades of precipitation in the Upper Colorado River basin from a high-resolution regional climate model

Abstract. Convection-permitting regional climate models (RCMs) have recently become tractable for applications at multi-decadal timescales. These types of models have tremendous utility for water resource studies, but better characterization of precipitation biases is needed, particularly for water-resource-critical mountain regions, where precipitation is highly variable in space, observations are sparse, and the societal water need is great. This study examines 34 years (1987–2020) of RCM precipitation from the Weather Research and Forecasting model (WRF; v3.8.1), using the Climate Forecast System Reanalysis (CFS; CFSv2) initial and lateral boundary conditions and a 1 km × 1 km innermost grid spacing. The RCM is centered over the Upper Colorado River basin, with a focus on the high-elevation, 750 km2 East River watershed (ERW), where a variety of high-impact scientific activities are currently ongoing. Precipitation is compared against point observations (Natural Resources Conservation Service Snow Telemetry or SNOTEL), gridded climate datasets (Newman, Livneh, and PRISM), and Bayesian reconstructions of watershed mean precipitation conditioned on streamflow and high-resolution snow remote-sensing products. We find that the cool-season precipitation percent error between WRF and 23 SNOTEL gauges has a low overall bias (x^ = 0.25 %, s = 13.63 %) and that WRF has a higher percent error during the warm season (x^ = 10.37 %, s = 12.79 %). Warm-season bias manifests as a high number of low-precipitation days, though the low-resolution or SNOTEL gauges limit some of the conclusions that can be drawn. Regional comparisons between WRF precipitation accumulation and three different gridded datasets show differences on the order of ± 20 %, particularly at the highest elevations and in keeping with findings from other studies. We find that WRF agrees slightly better with the Bayesian reconstruction of precipitation in the ERW compared to the gridded precipitation datasets, particularly when changing SNOTEL densities are taken into account. The conclusions are that the RCM reasonably captures orographic precipitation in this region and demonstrates that leveraging additional hydrologic information (streamflow and snow remote-sensing data) improves the ability to characterize biases in RCM precipitation fields. Error characteristics reported in this study are essential for leveraging the RCM model outputs for studies of past and future climates and water resource applications. The methods developed in this study can be applied to other watersheds and model configurations. Hourly 1 km × 1 km precipitation and other meteorological outputs from this dataset are publicly available and suitable for a wide variety of applications.

Geology↗

Data from: "Moisture rivals temperature in limiting photosynthesis by trees establishing beyond their cold-edge range limit under ambient and warmed conditions"

This archive contains data files that were used to draw conclusions in “Moisture rivals temperature in limiting photosynthesis by trees establishing beyond their cold-edge range limit under ambient and warmed conditions”, by Moyes et al., 2015. All field research was completed in common garden plots set up as part of the Alpine Treeline Warming Experiment (ATWE) on Niwot Ridge, Colorado, USA.There are two main data file formats in this archive: comma-separated values (.csv), and Microsoft Excel (.xls and .xlsx). .xlsx files can be read using Microsoft Excel and Google Sheets, and .csv files can be read using any simple text editor program, such as TextEdit (Mac) and Notepad (Windows). This .pdf data user’s guide can be read using Adobe Acrobat Reader, or any other compatible software. Seedling photographs and their corresponding leaf area-processed images are available in .jpg/.JPG image format, and can be opened using Preview (Mac) and Photos (Windows). To provide additional spatial context, two types of geospatial files are also published in this data package: ESRI shapefiles (.shp) and .kml files. Shapefiles are compatible with any GIS software able to read the file type (such as QGIS or ESRI’s ArcGIS suite), and .kml files can be opened with Google Earth or Google Maps. Figures 3 and 4 in the publication contain data from Moyes et al. 2013. This publication is cited in the References section in this archive, and data files can be accessed via the Alpine Treeline Warming Experiment project portal on ESS-DIVE. ---------------------------------------------------------------------------------------------------------------------------------------------------------------------------------------------------------- Climate change is altering plant species distributions globally, and warming is expected to promote uphill shifts in mountain trees. However, at many cold-edge range limits, such as alpine treelines in the western United States, tree establishment may be colimited by low temperature and low moisture, making recruitment patterns with warming difficult to predict.- We measured response functions linking carbon (C) assimilation and temperature- and moisture-related microclimatic factors for limber pine (Pinus flexilis) seedlings growing in a heating × watering experiment within and above the alpine treeline. We then extrapolated these response functions using observed microclimate conditions to estimate the net effects of warming and associated soil drying on C assimilation across an entire growing season.- Moisture and temperature limitations were each estimated to reduce potential growing season C gain from a theoretical upper limit by 15–30% (c. 50% combined). Warming above current treeline conditions provided relatively little benefit to modeled net assimilation, whereas assimilation was sensitive to either wetter or drier conditions.- Summer precipitation may be at least as important as temperature in constraining C gain by establishing subalpine trees at and above current alpine treelines as seasonally dry subalpine and alpine ecosystems continue to warm.

54 ENVIRONMENTAL SCIENCES↗

Data from: "Soil moisture mediates alpine life form and community productivity responses to warming"

This dataset contains values that were used to support conclusions drawn in the publication “Soil moisture mediates alpine life form and community productivity responses to warming”, originally published in 2016 by Winkler et al. All data were collected in the alpine site of the Alpine Treeline Warming Experiment (ATWE), located on Niwot Ridge, in the Front Range of the Colorado Rocky Mountains, USA. The file types in this archive include comma-separated-values (.csv) files, and two types of geospatial files: .kml and shapefiles (.shp). The csv files can be opened by R, Microsoft Excel, or any simple text editor software. The geospatial files can be opened by Google Earth/Google Maps, and the ESRI shapefiles can be opened by geographic information systems softwares that can read shapefiles, including ESRI’s ArcGIS Desktop suite, and QGIS.Climate warming is expected to alter primary production and community composition in alpine systems around the globe. Whether production will increase in response to warming in the absence of additional precipitation remains underexplored. We experimentally warmed an alpine plant community on Niwot Ridge, Colorado to test whether warming increases or decreases productivity of multiple plant life form groups and the entire plant community. We also provided supplemental water to a subset of plots to alleviate potential drying effects of warming. We predicted alpine community above-ground productivity would increase in response to warming only when combined with supplemental water to limit soil drying. We also predicted plant life form groups would vary in their responses and would like buffer changes in community productivity.

54 ENVIRONMENTAL SCIENCES↗

Next generation Arctic vegetation maps: Aboveground plant biomass and woody dominance mapped at 30 m resolution across the tundra biome

The Arctic is warming faster than anywhere else on Earth, placing tundra ecosystems at the forefront of global climate change. Plant biomass is a fundamental ecosystem attribute that is sensitive to changes in climate, closely tied to ecological function, and crucial for constraining ecosystem carbon dynamics. However, the amount, functional composition, and distribution of plant biomass are only coarsely quantified across the Arctic. Therefore, we developed the first moderate resolution (30 m) maps of live aboveground plant biomass (g m −2 ) and woody plant dominance (%) for the Arctic tundra biome, including the mountainous Oro Arctic. We modeled biomass for the year 2020 using a new synthesis dataset of field biomass harvest measurements, Landsat satellite seasonal synthetic composites, ancillary geospatial data, and machine learning models. Additionally, we quantified pixel-wise uncertainty in biomass predictions using Monte Carlo simulations and validated the models using a robust, spatially blocked and nested cross-validation procedure. Observed plant and woody plant biomass values ranged from 0 to ∼6000 g m −2 (mean ≈ 350 g m −2 ), while predicted values ranged from 0 to ∼4000 g m −2 (mean ≈ 275 g m −2 ), resulting in model validation root-mean-squared-error (RMSE) ≈ 400 g m −2 and R 2 ≈ 0.6. Our maps not only capture large-scale patterns of plant biomass and woody plant dominance across the Arctic that are linked to climatic variation (e.g., thawing degree days), but also illustrate how fine-scale patterns are shaped by local surface hydrology, topography, and past disturbance. By providing data on plant biomass across Arctic tundra ecosystems at the highest resolution to date, our maps can significantly advance research and inform decision-making on topics ranging from Arctic vegetation monitoring and wildlife conservation to carbon accounting and land surface modeling.

Climate change↗

Tropospheric aerosols over the western North Atlantic Ocean during the winter and summer deployments of ACTIVATE 2020: life cycle, transport, and distribution

The Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment (ACTIVATE) is a NASA mission to characterize aerosol–cloud interactions over the western North Atlantic Ocean (WNAO). Such characterization requires understanding of life cycle, composition, transport pathways, and distribution of aerosols over the WNAO. This study uses the GEOS-Chem model to simulate aerosol distributions and properties that are evaluated against aircraft, ground-based, and satellite observations during the winter and summer field deployments in 2020 of ACTIVATE. Transport in the boundary layer (BL) behind cold fronts was a major mechanism for the North American continental outflow of pollution to the WNAO in winter. Turbulent mixing was the main driver for the upward transport of sea salt within and ventilation out of BL in winter. The BL aerosol composition was dominated by sea salt, which increased in the summer, followed by organics and sulfate. Aircraft in situ aerosol measurements provided useful constraints on wet scavenging in GEOS-Chem. The model generally captured observed features such as continental outflow, land–ocean gradient, and mixing of anthropogenic aerosols with sea salt. Model sensitivity experiments with elevated smoke injection heights to the mid-troposphere (versus within BL) better reproduced observations of smoke aerosols from the western US wildfires over the WNAO in the summer. Model analysis suggests strong hygroscopic growth of sea salt particles and their seeding of marine BL clouds over the WNAO (< 35° N). Future modeling efforts should focus on improving parameterizations for aerosol wet scavenging, implementing realistic smoke injection heights, and applying high-resolution models that better resolve vertical transport.

54 ENVIRONMENTAL SCIENCES↗