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At least 91 records · Page 5

Performance assessment of PHITS simulations for the inverse-kinematic p( 7 Li,n) 7 Be reaction based on fast-neutron measurements with a diamond detector

The inverse-kinematics p( 7 Li,n) 7 Be reaction produces forward-focused neutron emission, offering enhanced usable flux and reduced shielding requirements. Reliable simulation of such neutron fields is essential for the development of compact accelerator-based neutron sources. In this study, a PHITS-based simulation framework for the reaction was experimentally assessed using fast-neutron measurements. Forward-directed neutrons were measured with a diamond neutron detector and quantitatively compared with simulations with newly prepared IK-Frag cross-section file based on the proton-induced reaction data in ENDF/B-VIII.1, TENDL-2023, and JENDL-4.0/HE. Measurements and simulations were performed for incident 7 Li 3+ energies ranging from 15.0 to 25.0 MeV using a 50 μm-thick polypropylene target. For all conditions, the PHITS-based simulation framework reproduced the deposited energy spectra at the correct order of magnitude. The comparison of deposited energy spectra in the diamond detector showed high correlation coefficients across all investigated energies, indicating reasonable agreement in spectral shape between simulations and measurements. This work represents an initial step toward establishing a benchmark for PHITS simulations of the inverse kinematic reaction between an incident lithium-ion and a proton target.

43 PARTICLE ACCELERATORS↗

Preliminary Design of a New Pulsed-Neutron Die--Away Experiments with Absorbers (IER-552 CED-1)

This report presents the preliminary design (CED-1) of IER-552, pulsed-neutron die-away (PNDA) experiments with absorbers, to be conducted by Lawrence Livermore National Laboratory (LLNL). The goal of the PNDA experiments with absorbing materials is to produce high-quality, low-cost integral benchmarks that can be used to validate cross sections that are high priority nuclear data for the Department of Energy’s Nuclear Criticality Safety Program (NCSP). PNDA experiments can be used to generate nuclear data validation benchmarks quickly and cheaply, as they do not require fissile material or a nuclear facility to conduct them. The original PNDA experiments were set up at LLNL under IER-501. Extending the PNDA experiments to include absorbing materials leverages existing facilities and resources at LLNL to validate cross sections, with a basic experiment design that uses a neutron generator to impinge a short, mono-energetic neutron pulse on a poisoned, moderating target sample. The neutron pulse lasts 100 µs, after which the neutron population in the sample reaches thermal equilibrium and later spatial equilibrium. In this fully equilibrized state, the neutron population has a characteristic decay-time eigenvalue. The eigenvalue can be used as an integral parameter to validate nuclear data involved with neutron scattering and absorption. Two observables can be measured: the neutron population and the population of secondary γ-rays produced by inelastic and capture reactions. This report explores the feasibility of both approaches. For γ-ray measurements, this allows for direct measurement of reactions of interest for validation. During the neutron burst time, inelastic (prompt) γ-rays dominate, and these data can be isolated for validation of neutron inelastic scattering data. After the pulse ends, neutron capture (delayed) γ-rays dominate and are produced by many reaction channels as neutrons slow down to thermal energies. Two sets of γ-ray spectra (inelastic, capture) can be produced for validation. Additionally, the time-dependent decay of the capture γ-ray population when the neutron population is thermalized and in its fundamental mode can be used for validation. Two experiments can be imagined where pulsed neutrons are used to validate the nuclear data of absorbing materials. The first integrates well into the existing PNDA testbed at LLNL. The absorber material would be introduced into a moderating target and the same neutron generator, neutron detectors, electronics, and shielding box used for IER-501 would be employed. From the same experimental setup, many absorbing materials can be validated by simply changing the neutron poison in the moderator. The only significant modification would be the introduction of a γ-ray detector. Such an experiment would primarily serve to validate nuclear data in the thermal energy range. The second kind of experiment would validate the fast and epithermal energy range. It would involve pulsing neutron into a bare assembly of the absorber material and measuring the die-away of neutrons. The fast leakage of such an assembly requires nanosecond neutron-generator pulse widths and fast detectors/electronics that could measure ~200 ns die-away curves. This kind of experiment would ideally be performed at a cyclotron, like that available at Lawrence Berkeley National Laboratory.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

The fast camera (Fastcam) imaging diagnostic systems on the DIII-D tokamak

Two camera systems are installed on the DIII-D tokamak at the toroidal positions of 90° (90° system) and 225° (225° system), respectively. The cameras have two types of relay optics, namely, a coherent optical fiber bundle and a periscope system. The periscope system provides absolute intensity calibration stability while sacrificing resolution (10 lp/mm), while the fiber system provides high resolution (16 lp/mm) while sacrificing calibration stability. The periscope is available only for the 90° system. The optics of the 225° system were designed for view stability, repeatability, and easy maintenance. The cameras are located inside optimized neutron, x ray and magnetic shielding in order to reduce electronics damage, reboots, and magnetic and neutron interference, increasing the overall system reliability. An automated filter wheel, providing remote filter change, allows for remote wavelength selection. A software suite automates camera acquisition and data storage, allowing for remote operation and reduced operator involvement. System metadata is used to streamline the data analysis workflow, particularly for intensity calibration. Here, the spatial calibration uses multiple observable wall features, resulting in a reconstruction accuracy ≤2 cm.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Ground calibration and in-flight commissioning of the Gamma-Ray and Neutron Spectrometer (GRNS) for NASA’s Psyche mission

NASA's Psyche spacecraft is currently enroute to the asteroid 16 Psyche, where it will perform an orbital investigation focused on determining the nature of the asteroid. A key part of this investigation is measurements of elemental composition to determine if the asteroid is rich in iron-nickel metal. To that end, the Psyche spacecraft payload includes a Gamma-Ray and Neutron Spectrometer (GRNS). GRNS is composed of two subsystems; a Gamma-Ray Spectrometer (GRS) with a high-purity germanium γ-ray sensor surrounded by a borated plastic scintillator Anti-Coincidence Shield (ACS), and a Neutron Spectrometer (NS) with three 3 He-filled gas proportional counters that are sensitive to different neutron energy regimes. We describe results from the pre-launch calibration campaign, along with early in-flight results from post-launch instrument commissioning. The information detailed here is focused on providing future users of GRNS data with the information needed to properly interpret the observations from the instrument.

Peplowski, Patrick N. [Johns Hopkins Univ., Baltim↗

HighNESS conceptual design report: Volume II. The NNBAR experiment.

A key aim of the HighNESS project for the European Spallation Source is to enable cutting-edge particle physics experiments. This volume presents a conceptual design report for the NNBAR experiment. NNBAR would exploit a new cold lower moderator to make the first search in over thirty years for free neutrons converting to anti-neutrons. The observation of such a baryon-number-violating signature would be of fundamental significance and tackle open questions in modern physics, including the origin of the matter-antimatter asymmetry. This report shows the design of the beamline, supermirror focusing system, magnetic and radiation shielding, and anti-neutron detector necessary for the experiment. A range of simulation programs are employed to quantify the performance of the experiment and show how background can be suppressed. For a search with full background suppression, a sensitivity improvement of three orders of magnitude is expected, as compared with the previous search. Civil engineering studies for the NNBAR beamline are also shown, as is a costing model for the experiment.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Conceptual Design of the Moderator Test Station at the Spallation Neutron Source

We describe the Moderator Test Station (MTS), under construction at the Spallation Neutron Source. We will leverage the Beam Test Facility (BTF) at the Spallation Neutron Source to provide a moderator neutronics test stand with which we will verify the anticipated performance gains expected and required from the innovative moderator concepts central to the SNS Second Target Station (STS) and the future of the First Target Station (FTS). These concepts include large-volume para-hydrogen moderators and high-brightness tube moderators. The MTS will add to the existing BTF a proton beam chopper similar to that already used in the SNS at the RFQ exit (the so-called MEBT chopper), various proton beam transport components, a neutron-producing target, a cryogenic moderator test stand, a reflector-shielding assembly, and a performance assessment neutron beamline. The MTS will provide the ability to test a wide variety of moderators in a prototypic configuration, simultaneously measuring the neutronic performance of the moderator concept central to the anticipated STS gains and developing the instrumentation necessary to provide that performance in a production environment. The presentation will describe the MTS, its progress, and the way we optimize the prototypic nature of the moderators we will test.

Iverson, Erik B↗

Radiation damages the silicates present in polyphasic mineral aggregates causing concrete’s degradation

While many U.S. nuclear power plants have submitted Subsequent License Renewal Application to operate beyond 60 years, others are already considering Operations Beyond Eighty years. In such cases, concrete biological shields are exposed to neutron and gamma radiation exceeding prescribed thresholds. Radiation-induced volumetric expansion (RIVE), extensively studied in single crystals, may also contribute to the degradation of polycrystalline aggregates. Since minerals differ in atomic structure and chemistry, radiation can affect them in distinct ways. This study examines quartzite, marble, and limestone to evaluate how irradiation affects their physical attributes and chemical reactivity. Results show crystalline silicates experience significant RIVE damage and enhanced reactivity in alkaline solutions compared to non-irradiated phases. Enhanced intra- and inter-granular dissolution could compromise aggregate integrity. An empirical correlation links silicate dissolution rate to atomic constraints (density, rigidity) and radiation dose, providing a predictive framework for estimating changes in silicate aggregate properties within radiation-exposed concrete.

Bouissonnié, Arnaud [Univ. of California, Los Ange↗

A Perspective on Scalable AI on High-Performance Computing and Leadership Class Supercomputing Facilities [Industrial and Governmental Activities]

Many scientific applications that support the mission of the US Department of Energy (US-DoE) require modeling complex engineering and/or physical systems. Here, examples of such complex systems arise from: (a) materials science to develop new compounds with exceptional mechanical and thermodynamical properties (e.g., resistance to mechanical stresses and high temperatures), (b) structural and nuclear engineering to model the temporal evolution of the structural damage of concrete shields exposed to continuous neutron and gamma radiations emitted by the nuclear reactor core, (c) urban sciences (e.g., transportation and smart buildings), and (d) power grid systems.

97 MATHEMATICS AND COMPUTING↗

Using quantum noise correlation analysis to measure ion temperature

Quantum noise correlation analysis was tested at the proof-of-concept level as a technique to measure ion temperature in a plasma. If eventually successful, this technique could enable a compact, inexpensive, and robust ion temperature diagnostic suitable for a burning plasma environment. Ion temperature is a key parameter determining the fusion performance of a burning plasma, as the fusion cross-section has a strong dependence on ion temperature. This ion temperature diagnostic would require only a small optical view of the plasma through a port to passively record impurity line emission. The instrumentation would be remote from the reactor behind the neutron and bio-shielding. The technique relies solely on quantum correlations of the photons emitted by a plasma impurity to measure ion temperature; there is no grating dispersion of an emission line-width or pulse-height analysis of photon energy. This measurement innovation was tested with instrumentation consisting of two single-photon detectors with high timing resolution, a time-tagging unit, and simple light collection optics. This instrumentation measures the second-order correlation between the light intensity falling on the two detectors. The next steps beyond the proof-of-concept level will be development of diagnostic designs for application of this technique to high-temperature and burning plasmas. Arrays of single-photon avalanche detectors to multiplex measurements of photon correlation will be required to reduce signal integration time to an acceptable duration.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Neutron Spectrum and 10B(n,α) Measurements in ZPPR-15

Neutron spectra were measured at the core center with proton recoil spectrometers in ZPPR15A loading 66, ZPPR-15B loading 90 and ZPPR loading 186. In addition, neutron spectra were measured in the SSNA shield configuration in ZPPR-15B loading 121 and in the BCNA shield configuration in ZPPR-15B loading 126. The ZPPR-15 neutron spectrum measurement and data processing techniques were described and analyzed. Total uncertainties were derived for all five spectrum measurements. A back-to-back proportional counter was used to measure the 10 B(n,α) reaction rate at six locations in the simulated shield, radial reflector and outer core in the ZPPR-15B BCNA shield experiment. The measurements were described and analyzed. A total uncertainty was derived for the 10 B(n,α) reaction rate measurements. The ZPPR-15 experimental records were used to develop detailed as-built Monte Carlo models for the five neutron spectrum measurement configurations and for the six 10 B(n,α) measurement configurations.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Thermal Scattering Law Data Development for Paraffin Wax

Paraffin wax is often used as a nuclear moderator to slow down the fast neutrons in experimental critical assemblies [1]. It is a colorless and soft solid material that consists primarily of straight-chain alkanes (n-alkanes), which are hydrocarbons with the general formula CnH2n+2 [2-3]. The length of the hydrocarbon chain ranges from C20 to C30 and higher [2]. It is distinguished by its solid state at room temperature and begins to melt above approximately 310 K [4]. Paraffin wax is a commonly employed substance in the manufacture of shielding. One of its noteworthy characteristics is its ability to effectively absorb the neutrons. Also, it possesses a high macroscopic cross section, which enables it to efficiently moderate neutrons. As a result, paraffin wax is extensively utilized in various applications where moderation and shielding of neutrons are needed. For simulations, it is necessary to evaluate its thermal scattering law (TSL) and cross sections. Computationally, classical molecular dynamics (CMD) simulations provide the capability of simulating atomic details. For example, several unary, binary, and few multi component mixtures have been investigated of the paraffin model by using molecular dynamics simulations [5-12]. An assessment of thermal neutron scattering in a heavy paraffinic oil treated both as a solid and a viscous fluid containing 25% linear branched paraffin (C30H62), 35% one ring cycloalkane (C30H60), 15% two rings cycloalkane (C30H58), and 25% aromatic (C30H60) chains has been studied using CMD simulations for producing TSL data [13]. Nevertheless, there is lack of TSL and cross section data for paraffin wax as most of the reported analyses focus on the unary and binary mixture of n-alkanes, which is not consistent with actual paraffin wax [2]. In this work, we applied the equilibrium CMD simulations technique to explore the structure and dynamical properties of wax, which are fundamental input to calculate the TSL. A paraffin wax system was modeled using the CMD code LAMMPS (Large-scale Atomic/Molecular Massively Parallel Simulator) [14-15] with the semi-empirical COMPASS [16] force field. The density of state (DOS) was calculated from the normalized velocity autocorrelation function (VACF), which is the Fourier transform of the normalized VACF. The DOS was used for the calculation of the TSL and thermal scattering cross sections. The paraffin wax atomic system was constructed by using the MedeA material design platform [17], and was benchmarked using available properties (i.e., density, bond lengths, angles, diffusivity, and viscosity).

Nuclear Criticality Safety Program (NCSP)↗

Pulsed-Neutron Experiments at the Inherently Safe Subcritical Assembly

The pulsed neutron technique is a powerful, dynamic method to assay the reactivity of a multiplying system. This work presents the novel application of the pulsed neutron technique to the Inherently Safe Subcritical Assembly, an experimental configuration accepted by the International Criticality Safety Benchmark Evaluation Project Handbook. The experiments were replicated with COG11.3, a continuous-energy Monte Carlo code. The pulsed neutron data were analyzed using the Sjöstrand and Gozani area-ratio methods and by extracting the prompt neutron decay constant. Subsequent static k-eigenvalue and 𝛼-eigenvalue simulations were also performed for the same configurations. Neutron detector dead-time effects from the experiments were corrected using the Backwards Extrapolation Method and shown to have a negligible impact on the estimated reactivities. The results highlight that capturing time-dependent effects like delayed neutron precursor buildup are essential to accurately reproduce experimental results. They also highlight the importance of shielding the detectors from generator source neutrons in deeply subcritical configurations.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Experiment Design and Preparation for a Shielding Benchmark Utilizing Godiva-IV

An experiment is currently being designed to provide a high-quality shielding benchmark for Criticality Accident Alarm System (CAAS) modeling. Previous benchmarks have suffered from uncertainty primarily due to two factors. The first factor is radiation that is not directly coming from the source, also known as room return. Room return is notoriously difficult to account for in experimental data and to model in benchmarks. The second factor is uncertainty associated with the source term itself. In order to reduce these two sources of uncertainty, this experiment will utilize a room return shield [1] that will reduce the effect of room return and previous work performed to ensure the reproducibility of the source term. The experiment will use the Godiva IV [2] assembly located at the National Criticality Experiments Research Center (NCERC) to provide a neutron source representative of a criticality accident. Previous experiments [3]-[4] have shown that Godiva IV is capable of producing both bursts and steady-state emissions of equal magnitude which will allow for reduced uncertainty in the source term. The room return shield will house and isolate the shielding samples, neutron activation foils, and other detectors. Data collected will provide a comparison of the neutron and gamma dose for shielded and unshielded configurations. This data will be used to validate shielding data used for modeling criticality accident alarm systems. Shielding samples included in this benchmark are C, Fe, NaCl, Pb, high density polyethylene, and SiO 2 . This paper details the design of the room return shield, the experimental plan, challenges, and mitigation strategies.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Evaluation of Radiation Transport Through a Nuclear-Grade Sandwich Composite

The development and deployment of microreactors are often synonymous with their transportability; however, designing a shield which is appropriate for both transportation and operations is challenging. A recent approach is the use of composite style shield which combines the reactor pressure vessel and biological shielding into a single unit to enhance the shields effectiveness without degrading the structural properties. To assess the viability of a nuclear grade sandwich composite (NGSC), and understanding of how radiation transports through the shield needs to be understood to select the appropriate materials. This work examines a two-layered NGSC of varying thicknesses with two primary shielding materials (tungsten-tetraboride cermet and boron carbide). To assess the NGSC, quantities of interest including neutron attenuation, photon attenuation, energy deposition, displacements per atom, helium generation, and dose are examined. Altogether, it is found that a combination of both tungsten-tetraboride and boron carbide are necessary to act as an appropriate shield, where the order in which these materials are place in the composite are important to their effectiveness.

22 - GENERAL STUDIES OF NUCLEAR REACTORS↗

Performance evaluation of neutron noise analysis in detecting special nuclear materials

Reliable and rapid inspection techniques play a vital role in preventing illicit trafficking of special nuclear materials. Active interrogation systems using neutrons produced by portable, high-flux deuterium-deuterium or deuterium-tritium neutron generators are being actively developed as a secondary scanning tool for this purpose. In this study, a neutron noise analysis-based approach for detecting unshielded and shielded special nuclear materials by using a pulsed deuterium-tritium neutron generator was evaluated. Here, this approach analyzes the fluctuation of neutron counts. Its performance was quantified with regard to time-to-detection to achieve a minimum probability of detection of 99% and a probability of false alarm of less than 1% considering various amounts of special nuclear materials and different shielding configurations. It was demonstrated that this approach could detect 17 uranium slugs in 5 s given a neutron generator yield of 8.1 × 10 7 n/s. These slugs could be detected within a reasonable time frame (200 s) when they were shielded by 10.16 cm of high-density polyethylene. The results obtained using the neutron noise analysis approach were compared with those obtained using the commonly used differential die-away analysis technique, a sensitive technique for detecting the presence of fissile materials by utilizing the prompt fission neutrons produced when the source neutrons from a neutron generator are completely diminished. For example, the time to detect 2 unshielded uranium slugs was 2.1 s when using the differential die-away analysis technique; it increased to 93 s for the neutron noise analysis approach. Although the noise analysis-based approach exhibits an overall performance which is not as good as that of differential die-away, neutron noise provides an alternative method for effective detection of special nuclear materials.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗