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At least 91 records · Page 5

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DOE OSTI2026

Equivalent equilibrium ion distributions in ion sources and beams

Ion sources and ion beams often contain ions of more than one charge-to-mass ratio, due to the presence of multiple ionization states and/or multiple atomic and molecular ion species in the source. We show that, under certain conditions, analysis of these systems can be simplified using the notion of “equivalent equilibrium ion distributions” (EEIDs). These distributions have identical ion trajectories, space-charge distributions, and electric-field distributions, but can be composed of ion species with arbitrary charge-to-mass ratios. We use this result to obtain multi-species generalizations for the perveance of an ion diode, which relates the diode voltage to the extracted beam current, and for the perveance of a drifting ion beam, which determines the axial length-scale for beam expansion due to the self-electric field. Applied to a quasi-neutral plasma ion source containing cold ions and hot electrons, we find that the location of the beam-plasma interface (meniscus), where ions are extracted from the plasma, depends on the electron density and ion energy per unit charge at the interface, independent of the ion composition. For certain types of numerical simulations, EEIDs allow one to calculate the beam optics of an intense multi-species ion source by doing a simulation for a single ion species with an artificial charge-to-mass ratio chosen to minimize computation time. We illustrate these results using the 3D particle-in-cell, finite-element code Aleph. The simulations show how ions in a plasma source self-consistently accelerate to the supersonic speed needed for steady, radially expanding flow. Multi-species equilibria are subject to streaming instabilities because, while the different species have the same kinetic energy per unit charge, their velocities scale with the square root of the charge-to-mass ratio. The simulations show that a strong ion streaming instability can occur in a multi-species plasma ion source.

74 ATOMIC AND MOLECULAR PHYSICS↗

DOE OSTI2024

Use of a deuterium-deuterium neutron generator for the Add-A-Source waste matrix correction technique

Neutron generators offer an alternative to radioactive sources in the application of active techniques for nondestructive assay of nuclear materials. The Add-A-Source technique has enabled improvements in the ability to accurately measure waste bearing nuclear materials by measuring and correcting for the non-nuclear matrix effect. The technique has historically been performed with a Cf-252 spontaneous fission source. Here, in this work, we have demonstrated the use of a Deuterium-deuterium neutron generator in place of the Cf-252 source. A DD generator enables operational advantages and allows the simplification of the instrument design, while offering equivalent corrective performance as a Cf-252 source.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DOE OSTI2026

Fluid-kinetic modeling of a high power density radio frequency inductively coupled positive hydrogen ion source

High power density radio-frequency (RF) inductively coupled positive ion sources are attractive candidates for next-generation neutral beam injection (NBI) systems, where higher injected power and longer pulse lengths are desired without sacrificing source reliability. Operating at absorbed power densities of order $\gt 1~\mathrm{W\,cm}^{-3}$ places these sources in a regime with stronger gas heating, higher dissociation, and non-Maxwellian electron energy distributions. The Large Uniform Plasma for Ionizing Neutrals (LUPIN) is an RF inductively coupled plasma source designed to explore this high power density regime and to provide guidance for a positive ion source upgrade for the DIII-D NBI system. LUPIN is designed to operate at up to 20 kW of RF power at 2 MHz, coupling energy through a cylindrical quartz vessel to achieve target ion current densities of $2100\,\mathrm{A\,m}^{-2}$ . This paper presents fluid-kinetic modeling of LUPIN using the hybrid plasma equipment model where electrons are treated kinetically, and the simulations reveal that electron energy distribution function transitions from nearly Maxwellian in the core to bi-Maxwellian towards the edge. Parametric simulations investigate the effects of RF power, gas pressure, and frequency on plasma density, ion flux, and uniformity. Parametric sweeps reveal that increasing power shifts the primary ionization channel from molecular to atomic with diminishing flux gains due to skin-depth contraction and gas rarefaction. Higher frequency localizes heating and increases $\mathrm{H}_2^+$ and $\mathrm{H}_3^+$ delivery to the grid, while elevated pressure boosts ionization yet hinders ion transport due to increase in collisionality.

inductively coupled plasma↗

DOE OSTI2025

Performance evaluation of the SPES FEBIAD ion source

SPES (Selective Production of Exotic Species) is the Radioactive Ion Beam (RIB) facility that is currently in the installation phase at the Istituto Nazionale di Fisica Nucleare in the Laboratori Nazionali di Legnaro (LNL-INFN). The main purpose of the facility is to deliver neutron-rich radioactive beams with a range of mass between 60 and 160 amu produced as fission products originated within a Uranium Carbide (UC x ) target impinged by high energy protons (40–70 MeV). In the last few years, the SPES group and their collaborators have focused on multiple aspects: development of various ISOL targets, ion sources, a high-power beam dump, versatile Front-End designs, primary proton beam and RIB diagnostics, design of beam optic components, and remote target handling. The development and optimization of ionization sources represents one of the most important R&D activities. The collaboration between SPES and ISOLDE (CERN) groups has enabled the evaluation of the performances of a novel FEBIAD ion source taking advantage of the ISOLDE off-line Front-End. In this paper, the results of efficiency and transversal emittance measurements of the new SPES FEBIAD ion source are presented and discussed. Particular attention is dedicated to the description of the experimental setup and to the comparison of experimental data with simulation to promote the reproducibility of the experimental tests with other types of sources.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DOE OSTI2026

Source-Resolved Inversion of Elemental Carbon Emissions in California Using Log-Space Bayesian Inference

Elemental carbon (EC), operationally quantified by thermal-optical analysis, is widely used as a proxy for black carbon (BC) relevant to short-term climate forcing and public health. Current EC emission inventories remain highly uncertain, with persistent discrepancies between bottom-up and top-down estimates. In this study, we develop a source-resolved, log-space Bayesian inversion framework applied to estimate California’s statewide EC emissions in 2019. By integrating surface EC measurements from the EPA’s Air Quality System network with high-resolution source contributions simulated by a chemical transport model, we identify a one-third underestimation in the existing statewide EC inventory, requiring an increase of the total from a prior of 8.58 [5.49–13.75] Gg year–1 to a posterior estimate of 12.78 [10.71–15.37] Gg year–1. This discrepancy is primarily driven by substantial underestimations in the power and industrial and off-road mobile sectors. Furthermore, population-weighted exposure analysis reveals a marked sectoral divergence between emission mass and health burden: off-road mobile sources dominate both emissions and exposure, accounting for 31% of statewide exposure, while residential wood combustion contributes 26% of total exposure despite comprising only 19% of total emissions, due to its source proximity to population. These findings underscore the need to update sector-specific EC speciation profiles and demonstrate that mitigation strategies targeting off-road mobile sources and residential wood combustion are critical for reducing EC-related health impacts in California.

Zhang, Jie↗

DOE OSTI2024

Investigating Mountain Watershed Headwater‐To‐Groundwater Connections, Water Sources, and Storage Selection Behavior With Dynamic‐Flux Particle Tracking

Abstract Climate change will impact mountain watershed streamflow both directly—with changing precipitation amounts and variability—and indirectly—through temperature shifts altering snowpack, melt, and evapotranspiration. To understand how these complex processes will affect ecosystem functioning and water resources, we need tools to distinguish connections between water sources (rain/snowmelt), groundwater storage, and exit fluxes (streamflow/evapotranspiration), and to determine how these connections change seasonally and as climate shifts. Here, we develop novel watershed‐scale approaches to understand water source, storage, and exit flux connections using a dynamic‐flux particle tracking model (EcoSLIM) applied in California's Cosumnes Watershed, which connects the Sierra Nevada and Central Valley. This work develops new visualizations and applications to provide mechanistic understanding that underpins the interpretation of isotopic field data at watershed scales to distinguish sources, flow paths, residence times, and storage selection. In our simulations, streamflow comes primarily from snow‐derived water while evapotranspiration generally comes from rain. Most streamflow starts above 1,000 m while evapotranspiration is sourced relatively evenly across the watershed and is generally younger than streamflow. Modeled streamflow consists primarily of water sourced from precipitation in the previous 5 years but before the current water year, while ET consists primarily of water from precipitation in the current water year. ET, and to a lesser extent streamflow, are both younger than water in groundwater storage. However, snowmelt‐derived streamflow preferentially discharges older water from snow‐derived storage. Dynamic‐flux particle tracking and new approaches presented here enable novel model‐tracer comparisons in large‐scale watersheds to better understand watershed behavior in a changing climate.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2025

Glacial‐Interglacial and Millennial‐Scale Changes in Nitrous Oxide Emissions Pathways and Source Regions

During the transition from the Last Glacial Maximum (LGM) to the Holocene, the atmospheric N 2 O mole fraction increased by 80 nmol mol −1 . Using ice core measurements of N 2 O isotopomer ratios, we show that this increase was driven by increases in both nitrification and denitrification, with the relative partitioning between both production pathways depending on the assumed isotopic end-member source signatures. Similarly, we also attribute a 35 nmol mol −1 N 2 O mole fraction increase during the Heinrich Stadial 4/Dansgaard Oeschger 8 (HS4/DO8) millennial-scale event to increases in both N 2 O production pathways. In contrast, the 25 nmol mol −1 N 2 O mole fraction decrease during the Younger Dryas was driven almost exclusively by a decrease in nitrification. The deglacial and HS4/DO8 increases in N 2 O production occurred in both marine and terrestrial environments, with the terrestrial source responding faster to warming by about two centuries. Constraints on changes in nitrification and denitrification emissions are robust and consistent with previous studies showing the sensitivity of N 2 O emissions to abrupt Northern Hemisphere warming. This study demonstrates for the first time the importance of both denitrification and nitrification pathways in driving source changes. Absolute emissions are more uncertain due to uncertainty about source isotopomer signatures. For instance, the contribution of denitrification to emissions at the LGM shifts from (65 ± 10) % to (91 ± 6) % when factoring in isotope enrichment due to partial reduction of N 2 O to N 2 during denitrification. Reducing uncertainty in source signatures will increase the power of ice core N 2 O isotope records in deducing environmental change.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2025

High average-flux laser-driven neutron source

Laser-driven neutron generation is an attractive alternative to more established methods for compact, short-pulse-duration neutron sources with applications in medical science, material science and imaging. Despite extensive investigation of various techniques, achieving performance comparable to nuclear reactors or conventional accelerators remains challenging. In this work, we generate a stable, high-repetition-rate laser-driven neutron source reaching a record average flux of 7.8 × 10 7 n/sr/s, improving on other existing laser-based sources by more than one order of magnitude. Our approach is based on a two-step process where electrons are accelerated to relativistic energies via laser wakefield acceleration (LWFA), and subsequently generate neutrons through Bremsstrahlung emission followed by photonuclear reactions in a tungsten converter. Experimental results, supported by Monte Carlo simulations, show a neutron flux of 3.0 × 10 7 n/cm 2 /s near the target, on par with some compact accelerator-based neutron sources. Additionally, a direct comparison with the target-normal sheath acceleration (TNSA) pitcher-catcher scheme, performed on the same laser system, reveals a significantly higher total neutron yield of 3.9 × 10 8 neutrons per shot, outperforming the TNSA scheme by several orders of magnitude. These findings represent a significant advancement towards the development of practical laser-driven neutron sources and highlight the advantages of LWFA-based neutron generation for future applications.

Vallières, Simon [Institut National de la Recherch↗

DOE OSTI2025

Demonstration of active neutron interrogation of special nuclear materials using a high-intensity short-pulse-laser-driven neutron source

Detecting shielded special nuclear material, such as nuclear explosives, is a difficult challenge pursued by non-proliferation, anti-terrorism, and nuclear security programs worldwide. Interrogation with intense fast-neutron pulses is a promising method to characterize concealed nuclear material rapidly but is limited by suitable source availability and proven instrumentation. In this study we have pioneered a demonstration of such an interrogation method using a high-intensity, short-pulse, laser-driven neutron source that offers potential benefits compared to conventional neutron sources. The measurement results reported here represent the first experimental demonstration of this interrogation approach on enriched uranium items and demonstrate the feasibility of a precise measurement using realistic nuclear materials, representative of field scenarios, even with just a single laser-driven neutron pulse. Bright pulsed sources can overcome the nuisance background of items with strong internal neutron sources, improving analytical power, while single-shot assay is attractive in high-throughput situations where time is at a premium. The science and technology of this type of neutron production is developing rapidly, and we anticipate that practical mobile interrogation systems will become available based on the detection concepts demonstrated here to meet the growing measurement needs.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

DOE OSTI2024

Source size of x rays from self-modulated laser wakefield accelerators

A comparative study of x-ray sources generated with different mechanisms from self-modulated laser wakefield acceleration (SM-LWFA) electrons was performed to compare the source size or spatial resolution for use in high energy density science applications. We examine the source size of betatron, inverse Compton scattering, and bremsstrahlung radiation with a Fresnel diffraction based formalism and a modified x-ray ray tracing model. We observe the dependence of source size on the radiation generation process, laser parameters, and compare to what is possible in other regimes of LWFA, as well as current methods. This information is significant as we begin to explore the use of light sources driven by SM-LWFA for use as a diagnostic at large-scale laser facilities where blowout regime LWFA is not possible.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2024

Source localization for neutron imaging systems using convolutional neural networks

The nuclear imaging system at the National Ignition Facility (NIF) is a crucial diagnostic for determining the geometry of inertial confinement fusion implosions. The geometry is reconstructed from a neutron aperture image via a set of reconstruction algorithms using an iterative Bayesian inference approach. An important step in these reconstruction algorithms is finding the fusion source location within the camera field-of-view. Currently, source localization is achieved via an iterative optimization algorithm. In this paper, we introduce a machine learning approach for source localization. Specifically, we train a convolutional neural network to predict source locations given a neutron aperture image. We show that this approach decreases computation time by several orders of magnitude compared to the current optimization-based source localization while achieving similar accuracy on both synthetic data and a collection of recent NIF deuterium–tritium shots.

47 OTHER INSTRUMENTATION↗

DOE OSTI2024

X-ray sources for in situ wavelength calibration of x-ray imaging crystal spectrometers

X-ray sources for a range of wavelengths are being considered for in situ calibration of X-ray Imaging Crystal Spectrometers (XICSs) and for monitoring line shifts due to changes in the crystal temperature, which can vary during experimental operation over a day [A. Ince-Cushman et al., Rev. Sci. Instrum. 79, 10E302 (2008), L. Delgado-Aparicio et al., Plasma Phys. Control. Fusion 55, 125011 (2013)]. Such crystal temperature dependent shifts, if not accounted for, could be erroneously interpreted as Doppler shifts leading to errors in plasma flow-velocity measurements. The x-ray sources encompass characteristic x-ray lines falling within the wavelength range of 0.9–4.0 Å, relevant for the XICSs on present and future fusion devices. Several technological challenges associated with the development of x-ray sources for in situ calibration are identified and are being addressed in the design of multiple x-ray tubes, which will be installed inside the spectrometer housing of the XICS for the JT-60SA tokamak. These x-ray sources will be especially useful for in situ calibration between plasma discharges. Here, in this paper, laboratory experiments are described that were conducted with a Cu x-ray source, a heated quartz (102) crystal, and a pixelated Pilatus detector to measure the temperature dependent shifts of the Cu Kα 1 and Kα 2 lines at 1.5405 and 1.5443 Å, respectively, and to evaluate the 2d-lattice constant for the Bragg reflecting crystal planes as a function of temperature, which, in the case of in situ wavelength calibration, would have to be used for numerical analysis of the x-ray spectra from the plasma.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2025

Noncollinear ground states of solids with a source-free exchange correlation functional

In this paper, we expand upon the source-free (SF) exchange correlation (XC) functional developed by Sangeeta Sharma and coworkers to plane-wave density functional theory (DFT) based on the projector augmented wave (PAW) method. This constraint is implemented by the current authors within the VASP source code, using a fast Poisson solver that capitalizes on the parallel three-dimensional fast Fourier transforms (FFTs) implemented in VASP. Using this modified XC functional, we explore the improved convergence behavior that results from applying this constraint to the GGA-PBE+U+J functional. In the process, we compare the noncollinear magnetic ground state computed by each functional and their SF counterpart for a select number of magnetic materials in order to provide a metric for comparing with experimentally determined magnetic orderings. We observe significantly improved agreement with experimentally measured magnetic ground-state structures after applying the source-free constraint. Furthermore, we explore the importance of considering probability current densities in spin-polarized systems, even under no applied field. We analyze the XC torque as well, in order to provide theoretical and computational analyses of the net XC magnetic torque induced by the source-free constraint. Along these lines, we highlight the importance of properly considering the real-space integral of the source-free local magnetic XC field. Our analyses on probability currents, net torque, and constant terms draw additional links to the rich body of previous research on spin-current density functional theory (SCDFT), and pave the way for future extensions and corrections to the SF corrected XC functional.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2026

Searches for nonstandard neutrino oscillations at neutrino telescopes with a TeV muon accelerator source

Muon accelerators, a potential technology for enabling O ( 10 TeV ) parton center of mass energy collisions, would also source an intense, collimated beam of neutrinos at TeV energies. The energy and size of this beam would be excellently matched as a source for existing and planned neutrino telescopes: gigaton-sized detectors of astrophysical neutrinos at and above TeV energies. In this paper, we introduce the technical considerations and scientific reach of pairing a muon accelerator source of neutrinos with a neutrino telescope detector, a combination we dub the “Neutrino Kaleidoscope.” In particular, such a pairing would enable searches for non-standard oscillations of the beam neutrinos as they traverse the earth between source and detector. These nonstandard neutrino oscillations could be sourced by Lorentz invariance violation, which a neutrino kaleidoscope could probe up to the Planck scale. Such a search would also have a reach on sterile neutrinos orders of magnitude beyond existing terrestrial limits. Finally, we touch on the nonoscillation physics case for a neutrino kaleidoscope.

Kamp, Nicholas W. [Harvard U.] (ORCID:000000019232↗

DOE OSTI2026

Identifying neutron sources using recoil and time-of-flight spectroscopy

Identification of neutron sources is central to nuclear physics and its applications, from planetary science to nuclear security, yet direct source discrimination from measured neutron spectra remains fundamentally elusive. Here, we introduce a Bayesian protocol that directly infers source ensembles from measured neutron spectra by combining full-spectrum template matching with probabilistic evidence evaluation. Applying this protocol to recoil and time-of-flight spectroscopy, we recover single- and two-source configurations with strong statistical significance (beyond 4⁢𝜎) at event counts as low as ∼10 3 . These results demonstrate that neutron spectral signatures can be leveraged for robust source identification, opening a new observational window for both fundamental research and operationally driven applications.

neutron physics↗

DOE OSTI2026

Universal CMB 𝐵-mode spectrum from early causal tensor sources

Many early Universe scenarios predict postinflationary tensor perturbations from causality-limited, subhorizon sources. While the microphysical details may be different, as long as these sources are bounded in duration and correlation length, their tensor power spectra exhibit a universal scaling behavior at small wave number: 𝒫 ℎ ⁡(𝑘)∝𝑘 3 , corresponding to white noise on superhorizon scales at the time of production. If these early causal tensor sources (ECTs) exclusively produce gravitational waves before redshift 𝑧 ∼10 5 , this scaling is realized on all of the scales observed in the CMB, and thus yields a universal multipole distribution for the 𝐵-mode angular power spectrum. Unlike the scale-invariant distributions of inflationary 𝐵 modes, ECTs generically predict enhanced power on small scales and suppressed power on large scales, which allows these source classes to be distinguished given measurements over a sufficient range of angular scales. In this paper, we introduce a unified framework for characterizing ECTs and demonstrate how their universal infrared scaling manifests in low-frequency observables, including CMB 𝐵 modes and stochastic gravitational wave spectral densities. We illustrate this mapping with representative case studies of this universality class involving first-order phase transitions, topological defects, and enhanced scalar perturbations, which source tensor modes at second order in perturbation theory.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2025

An infrasound source analysis of the OSIRIS-REx sample return capsule hypersonic re-entry

The OSIRIS-REx sample return capsule's hypersonic re-entry into the atmosphere is a rare opportunity to test a variety of sonic boom source models since the projectile dimensions are well characterized. While the as-flown flight path is unknown, the predicted flight path enables a rough approximation of the source Mach number and location. Six infrasound microphones deployed in the boom carpet along the predicted flight path recorded impulsive signals from the OSIRIS-REx re-entry. Using a suite of atmosphere profiles and the geometric acoustics approximation, we estimate locations with uncertainty estimates along the flight path from which the signals were emitted. Acoustic overpressure and signal duration predictions from Whitham's far field theory, Carlson's simplified sonic boom prediction method, and a drag-dominated hypersonic model are analyzed with uncertainty estimates from the location estimate. While the Carlson simplified sonic boom prediction method could be accurate, our preference is for the drag-dominated source model. Using this source model with an inviscid Burgers's equation solver for propagation, we obtained an excellent match to the recorded data. In conclusion, these results will help better inform future sample return capsule re-entry observation campaigns as well as contribute to a better understanding of high altitude infrasonic sources.

58 GEOSCIENCES↗

DOE OSTI2025

Compact fiber-coupled narrowband two-mode squeezed light source

Quantum correlated states of light, such as squeezed states, are a fundamental resource for the development of quantum technologies, as they are needed for applications in quantum metrology, quantum computation, and quantum communications. It is thus critical to develop compact, efficient, and robust sources to generate such states. Here, we report on a compact, narrowband, fiber-coupled source of two-mode squeezed states of light at 795 nm based on four-wave mixing (FWM) in an 85 Rb atomic vapor. The source is designed in a small modular form factor, with two input fiber-coupled beams, the seed and pump beams required for the FWM, and two output fibers, one for each of the modes of the squeezed state. The system is optimized for low pump power (135 mW) to achieve a maximum intensity-difference squeezing of 4.4 dB after the output of fibers at an analysis frequency of 1 MHz. Furthermore, the narrowband nature of the source makes it ideal for atomic-based quantum sensing and quantum networking configurations that rely on atomic quantum memories. Such a source paves the way for a versatile and portable platform for applications in quantum information science.

Jain, Umang [University of Oklahoma, Norman, OK (U↗