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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 901 records · Page 50

Patterning via optical-saturable transformations: A review and simple simulation model

Most of the nanoscale fabrication in the semiconductor industry is based on patterning with scanning-electron beam lithography (SEBL). Although this approach is very versatile and has very high resolution, it is intrinsically a serial writing process, and therefore, relatively slow. Our group has been investigating alternative nano-fabrication techniques, adapted from ideas of saturating optical transitions such as those used in stimulated emission-depletion microscopy and related methods, and optical interference lithography. Linewidths and resolutions on the scale of a few tens of nanometers and below are highly desirable for various applications in nanotechnology. However, the spatial resolution of optical lithography is restricted by diffraction. In the past, we developed absorbance modulation to overcome this limit. This approach utilizes photochromic molecules that can be optically switched between two thermally stable states, one opaque and the other transparent. However, absorbance modulation is limited to surface (2-D) patterning. Here, we report on an alternative approach that exploits unique combinations of spectrally selective reversible and irreversible photochemical transitions to achieve deep subwavelength resolution with potential extension to 3-dimensions. This approach, which we refer to as patterning via optical-saturable transformations have the potential for massive parallelism, enabling the creation of nanostructures and devices at a speed far surpassing what is possible with SEBL. The aim of our research is to translate the success in circumventing Abbe's diffraction limit in optical microscopy to optical lithography.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Noncontact measurement of high temperature using optical fiber sensors

The primary goal of this research program was the investigation and application of noncontact temperature measurement techniques using optical techniques and optical fiber methods. In particular, a pyrometer utilizing an infrared optical light pipe and a multiwavelength filtering approach was designed, revised, and tested. This work was motivated by the need to measure the temperatures of small metallic pellets (approximately 3 mm diameter) in free fall at the Microgravity Materials Processing Drop Tube at NASA Marshall Space Flight Center. In addition, research under this program investigated the adaptation of holography technology to optical fiber sensors, and also examined the use of rare-earth dopants in optical fibers for use in measuring temperature. The pyrometer development effort involved both theoretical analysis and experimental tests. For the analysis, a mathematical model based on radiative transfer principles was derived. Key parameter values representative of the drop tube system, such as particle size, tube diameter and length, and particle temperature, were used to determine an estimate of the radiant flux that will be incident on the face of an optical fiber or light pipe used to collect radiation from the incandescent falling particle. An extension of this work examined the advantage of inclining or tilting the collecting fiber to increase the time that the falling particle remains in the fiber field-of-view. Those results indicate that increases in total power collected of about 15 percent may be realized by tilting the fiber. In order to determine the suitability of alternative light pipes and optical fibers, and experimental set-up for measuring the transmittance and insertion loss of infrared fibers considered for use in the pyrometer was assembled. A zirconium fluoride optical fiber and several bundles of hollow core fiber of varying diameters were tested. A prototype two-color pyrometer was assembled and tested at Virginia Tech, and then tested on the Drop Tube at Marshall Space Flight Center. Radiation from 5 mm diameter niobium drops falling in the Drop Tube was successfully detected, and recorded for later analysis. Subsequent analysis indicated that the imaging of light output from the light pipe onto the detector active areas was not identical for both detectors.

Claus, R. O.↗

Sources of noise in magneto-optical readout

The various sources of noise which are often encountered in magneto-optical readout systems are analyzed. Although the focus is on magneto-optics, most sources of noise are common among the various optical recording systems and one can easily adapt the results to other media and systems. A description of the magneto-optical readout system under consideration is given, and the standard methods and the relevant terminology of signal and noise measurement are described. The characteristics of thermal noise, which originates in the electronic circuitry of the readout system, are described. The most fundamental of all sources of noise, the shot noise, is considered, and a detailed account of its statistical properties is given. Shot noise, which is due to random fluctuations in photon arrival times, is an ever-present noise in optical detection. Since the performance of magneto-optical recording devices in use today is approaching the limit imposed by the shot noise, it is important that the reader have a good grasp of this particular source of noise. A model for the laser noise is described, and measurement results which yield numerical values for the strength of the laser power fluctuations are presented. Spatial variations of the disk reflectivity and random depolarization phenomena also contribute to the overall level of noise in readout; these and related issues are treated. Numerical simulation results describing some of the more frequently encountered sources of noise which accompany the recorded waveform itself, namely, jitter noise and signal-amplitude fluctuation noise are presented.

Mansuripur, M.↗

Three-Dimensional Geometry of Collagenous Tissues by Second Harmonic Polarimetry

Collagen is a biological macromolecule capable of second harmonic generation, allowing label-free detection in tissues; in addition, molecular orientation can be determined from the polarization dependence of the second harmonic signal. Previously we reported that in-plane orientation of collagen fibrils could be determined by modulating the polarization angle of the laser during scanning. We have now extended this method so that out-of-plane orientation angles can be determined at the same time, allowing visualization of the 3-dimensional structure of collagenous tissues. This approach offers advantages compared with other methods for determining out-of-plane orientation. First, the orientation angles are directly calculated from the polarimetry data obtained in a single scan, while other reported methods require data from multiple scans, use of iterative optimization methods, application of fitting algorithms, or extensive post-optical processing. Second, our method does not require highly specialized instrumentation, and thus can be adapted for use in almost any nonlinear optical microscopy setup. It is suitable for both basic and clinical applications. We present three-dimensional images of structurally complex collagenous tissues that illustrate the power of such 3-dimensional analyses to reveal the architecture of biological structures.

59 BASIC BIOLOGICAL SCIENCES↗

Ab initio translationally invariant nucleon-nucleus optical potentials

We combine the ab initio symmetry-adapted no-core shell model (SA-NCSM) with the single-particle Green's function approach to construct optical potentials rooted in first principles. Specifically, we show that total cross sections and phase shifts for neutron elastic scattering from a 4 He target with projectile energies between 0.5 and 10 MeV closely reproduce the experiment. In addition, we discuss an important new development that resolves a long-standing issue with spurious center-of-mass motion in the Green's function formalism for many-body approaches. Furthermore, the new development opens a path for first-principle predictions of cross sections for elastic scattering of single-nucleon projectiles, nucleon capture, and deuteron breakup reactions, feasible for a broad range of open-shell spherical and deformed nuclei in the SA-NCSM approach.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Anisotropic Photoluminescence from Isotropic Optical Transition Dipoles in Semiconductor Nanoplatelets

Many important light-matter coupling and energy-transfer processes depend critically on the dimensionality and orientation of optical transition dipoles in emitters. We investigate individual quasi-two-dimensional nanoplatelets (NPLs) using higher-order laser scanning microscopy and find that absorption dipoles in NPLs are isotropic in three dimensions at the excitation wavelength. Correlated polarization studies of the NPLs reveal that their emission polarization is strongly dependent on the aspect ratio of the lateral dimensions. Our simulations reveal that this emission anisotropy can be readily explained by the electric held renormalization ettect caused by the dielectric contrast between the NPLs and the surrounding medium, and we conclude that emission dipoles in NPLs are isotropic in the plane of the NPLs. Our study presents an approach for disentangling the effects of dipole degeneracy and electric field renormalization on emission anisotropy and can be adapted for studying the intrinsic optical transition dipoles of various nanostructures.

Ma, Xuedan↗

Wide bandgap optical switch circuit breaker for controlling propagation of current therethrough a wide bandgap optical device

A high-voltage switch is adapted for use as a medium-voltage direct current circuit breaker, which provides a low-cost, small-footprint device to mitigate system faults. In one example, a method for operating a wideband optical device includes illuminating the wide bandgap optical device with a light within a first range of wavelengths and a first average intensity, allowing a current to propagate therethrough without substantial absorption of the current, illuminating the wide bandgap optical device with light within the first range of wavelengths and a second average intensity that is lower than the first average intensity to allow a sustained current flow though the wide bandgap optical device, and illuminating the wide bandgap optical device with light within a second range of wavelengths to stop or substantially restrict propagation of the current through the wide gap material.

Voss, Lars F.↗

Improving optical performance of concentrator cells by means of a deposited nanopattern layer

Multijunction solar cells (MJSC) use anti-reflective coatings (ARC) to minimize Fresnel reflection losses for a family of light incidence angles. These coatings adapt the refractive index of the cell to that of the surrounding medium. Patterns with sizes in the range of the light wavelength can be used to further reduce reflections through diffraction. Transparent nanopatterns with a gradual profile, called moth-eye nanostructures, can adapt the refractive index of the optical interfaces (often with n∼1.5) used to encapsulate concentrator solar cells to that of the air (n{sub air}∼1). Here we show the effect of a nanometric moth-eye ARC with a round motif deposited on commercial MJSC that achieves short-circuit current (I{sub SC}) gains greater than 2% at normal incidence and even higher in the case of tilted illumination. In this work, MJSC with different moth-eye ARC are characterized under quantum efficiency (QE) as well as under concentrated illumination I-V in order to assess their potential. Simulations based on coupled wave analysis (RCWA) are used to fit the experimental results with successful results.

14 SOLAR ENERGY↗

Ab initio leading order effective potential for elastic proton scattering based on the symmetry-adapted no-core shell model

Calculating microscopic optical potentials for elastic scattering at intermediate energies from light nuclei in an ab initio fashion within the Watson expansion has been established within the last few years. Based on the Watson expansion of the multiple scattering series, we employ a nonlocal translationally invariant nuclear density derived within the symmetry-adapted no-core shell model (SA-NCSM) framework from a chiral next-to-next-to-leading order (NNLO) nucleon-nucleon interaction and the very same interaction for a consistent full-folding calculation of the effective (optical) potential for nucleon-nucleus scattering for medium-heavy nuclei. The leading order effective (optical) folding potential is computed by integrating over a translationally invariant SA-NCSM one-body scalar density, spin-projected momentum distribution, and the Wolfenstein amplitudes 𝐴, 𝐶, and 𝑀. The resulting nonlocal potentials serve as input for a momentum space Lippmann-Schwinger equation. In the SA-NCSM, the model space is systematically up-selected using Sp⁡(3,ℝ) symmetry considerations. For the light nucleus of 6 He, we establish a systematic selection scheme in the SA-NCSM for scattering observables. Then, we apply this scheme to calculations of scattering observables, such as differential cross sections, analyzing powers, and spin rotation functions for elastic proton scattering from 20 Ne and 40 Ca in the energy regime between 65 and 200 MeV, and compare to available data. Furthermore, our calculations show that the leading order effective nucleon-nucleus potential in the Watson expansion of multiple scattering theory obtained from an up-selected SA-NCSM model space describes 40 Ca elastic scattering observables reasonably well to about 60 degrees in the center-of-mass frame, which coincides roughly with the validity of the NNLO chiral interaction used to calculate both the nucleon-nucleon amplitudes and the one-body scalar and spin nuclear densities.

Ab initio calculations↗

Development of a Novel Accelerator for Neutron Transport Solution Using the Galerkin Spectral Element Methods (Final Report)

This report summarizes the results of a three-year research project sponsored by the U.S. Department of Energy (DOE) Nuclear Energy University Program (NEUP) to develop and implement advanced acceleration schemes for the DOE NEAMS neutronics code PROTEUSSN. The project team included the University of Massachusetts Lowell, The Ohio State University, University of Michigan, and Argonne National Laboratory. The PROTEUS code is a high-fidelity capable deterministic neutron transport code based on unstructured finite element meshes, which solves the steady-state and transient neutron transport problem using the 2nd-order discrete ordinate method (SN2ND), the method of characteristics (MOC), and the advanced nodal transport method (NODAL). The DSA scheme has been implemented in PROTEUS to speed up SN transport calculations. The existing DSA scheme employs a consistent finite element formulation on the same fine mesh structure as the SN solution While the use of consistent discretizations makes the DSA method effective, it does not necessarily make it efficient because the numerical solution of a discretized elliptic diffusion problem itself can be costly, particularly when the problem size becomes large. We developed a new discontinuous Galerkin (DG) discretization of the diffusion equation, called DG-DSA, which can effectively and efficiently accelerate the SN transport iterations. As compared with the previous work, the novelty of our method is that the diffusion equation is solved on a coarse-mesh grid using the DG methods, and the DG diffusion discretization incorporates local hp adaptation, i.e., local adaptation of mesh size and/or polynomial degree, based on local total cross section (or optical thickness). Therefore, the resulting number of degrees of freedom (DOF) of the DG discretization is much less than the conventional consistent DSA discretizations, and thus DG-DSA can achieve significant improvement in computational efficiency. We implemented this scheme in PROTEUS-SN. In addition, we developed a new stabilization scheme named linear prolongation CMFD (lpCMFD). A novel feature of this scheme is that the conventional flat flux ratio–based scaling approach is replaced with a linear interpolation of the scalar flux differences at the coarse-mesh cell edges between the neutron transport and CMFD calculations. Fourier convergence analysis and numerical results show that lpCMFD is unconditionally stable and more effective than other CMFD based on acceleration schemes such as pCMFD, odCMFD. We also developed a new nonlinear diffusion acceleration scheme for solving neutron transport equations. This scheme, called LR-NDA, employs a local refinement approach on the framework of CMFD by solving a local boundary value problem of the scalar flux on the coarse-mesh structure to replace the piecewise constant scalar flux obtained by CMFD. The refined flux is then used to update the scalar flux in the neutron transport source iteration. It has been demonstrated that that LR-NDA is much more effective and stable than CMFD for a wide range of optical thicknesses. LR-NDA is a local adaptive method, which means LR-NDA does not necessarily require local refinement for all the coarse-mesh cells on the problem domain, i.e., it can be used only for relatively optically thick regions where the standard CMFD scheme would encounter the convergence problem.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Visual perception system and method for a humanoid robot

A robotic system includes a humanoid robot with robotic joints each moveable using an actuator(s), and a distributed controller for controlling the movement of each of the robotic joints. The controller includes a visual perception module (VPM) for visually identifying and tracking an object in the field of view of the robot under threshold lighting conditions. The VPM includes optical devices for collecting an image of the object, a positional extraction device, and a host machine having an algorithm for processing the image and positional information. The algorithm visually identifies and tracks the object, and automatically adapts an exposure time of the optical devices to prevent feature data loss of the image under the threshold lighting conditions. A method of identifying and tracking the object includes collecting the image, extracting positional information of the object, and automatically adapting the exposure time to thereby prevent feature data loss of the image.

Wells, James W.↗

Accurate Taylor transfer maps for large aperture iron dominated magnets used in charged particle separators and spectrometers

For high-resolution separators like the projected Super-FRS at FAIR, an adapted and accurate ion-optical model considering realistic $B$-dependent magnet parameters is crucial in achieving the desired parameters (e.g. resolution) and to enable a fast optimization. Starting from the magnetic field measurements and simulations, rigidity-dependent Taylor transfer maps are generated for the Super-FRS preseparator dipole magnets. The effects of the magnetic saturation in the steel yoke on the image aberrations are analyzed.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Dielectric response of polyethersulphone (PES) polymer irradiated with 145 MeV Ne{sup 6+} ions

Heavy ion irradiation produces modifications in polymers and adapts their electrical, chemical and optical properties in the form of rearrangement of bonding, cross-linking, chain scission and formation of carbon rich clusters. Modification depends on the ion, its energy and fluence and the polymeric material. In the present work, a study of the dielectric response of pristine and heavy ion irradiated Polyethersulphone (PES) polymer film is carried out. 250 {mu}m thick PES films were irradiated to the fluences of 10{sup 12} and 10{sup 13} ions/cm{sup 2} with Ne{sup 6+} ions of 145 MeV energy from Variable Energy Cyclotron Centre, Kolkata On irradiation with heavy ions dielectric constant ({epsilon} Prime ) decreases at higher frequencies and increases with fluences. Variation of loss factor (tan {delta}) with frequency for pristine and irradiated with Si ions reveals that tan {delta} increases as the frequency increases. The tan{delta} also increases with fluence. Tan {delta} has positive values indicating the dominance of inductive behavior.

36 MATERIALS SCIENCE↗

Measurement of Photovoltaic Module Deformation Dynamics During Hail Impact Using Digital Image Correlation

Stereo high-speed video of photovoltaic modules undergoing laboratory hail tests was processed using digital image correlation to determine module surface deformation during and immediately following impact. The purpose of this work was to demonstrate a methodology for characterizing module impact response differences as a function of construction and incident hail parameters. Video capture and digital image analysis were able to capture out-of-plane module deformation to a resolution of ±0.1 mm at 11 kHz on an in-plane grid of 10 × 10 mm over the area of a 1 × 2 m commercial photovoltaic module. With lighting and optical adjustments, the technique was adaptable to arbitrary module designs, including size, backsheet color, and cell interconnection. Furthermore, impacts were observed to produce an initially localized dimple in the glass surface, with peak deflection proportional to the square root of incident energy. Subsequent deformation propagation and dissipation were also captured, along with behavior for instances when the module glass fractured. Natural frequencies of the module were identifiable by analyzing module oscillations postimpact. Limitations of the measurement technique were that the impacting ice ball obscured the data field immediately surrounding the point of contact, and both ice and glass fracture events occurred within 100 μs, which was not resolvable at the chosen frame rate. Increasing the frame rate and visualizing the back surface of the impact could be applied to avoid these issues. Applications for these data include validating computational models for hail impacts, identifying the natural frequencies of a module, and identifying damage initiation mechanisms.

14 SOLAR ENERGY↗

Spectral ellipsometry as a method for characterization of nanosized films with ferromagnetic layers

Nanosized films with ferromagnetic layers are widely used in nanoelectronics, sensor systems and telecommunications. Their properties may strongly differ from those of bulk materials that is on account of interfaces, intermediate layers and diffusion. In the present work, spectral ellipsometry and magnetooptical methods are adapted for characterization of the optical parameters and magnetization processes in two- and three-layer Cr/NiFe, Al/NiFe and Cr(Al)/Ge/NiFe films onto a sitall substrate for various thicknesses of Cr and Al layers. At a layer thickness below 20 nm, the complex refractive coefficients depend pronouncedly on the thickness. In two-layer films, remagnetization changes weakly over a thickness of the top layer, but the coercive force in three-layer films increases by more than twice upon remagnetization, while increasing the top layer thickness from 4 to 20 nm.

77 NANOSCIENCE AND NANOTECHNOLOGY↗

Simultaneous observations by television camera and radar

The original image-orthicon equipment used for simultaneous radar and optical observations is described. The adaptations made to enhance its usefulness for meteor observations, and the specialized calibration and photometric procedures developed for this purpose are also described. Some brief comments concerning the use of the secondary electron conduction vidicon are included.

Mccrosky, R. E.↗

Effects of multiple scattering on scintillation of transionospheric radio signals

Recent development in the optical scintillation theory has been adapted to the ionospheric geometry in order to study the ionospheric scintillation phenomenon in the presence of multiple scattering. Under approximations well satisfied in typical ionospheres for a frequency above about 20 MHz, the first through fourth moment equations have been derived and some analytic solutions given. The fourth moment equation has also been solved numerically. The numerical results show clearly the occurrence of focusing and saturation phenomena. The new multiple-scatter effects are emphasized.

Liu, C. H.↗