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Lessons Learned From Developing Reactor Pressure Vessel Steel Embrittlement Database

Materials behaviors caused by neutron irradiation under fission and/or fusion environments can be little understood without practical examination. Easily accessible material information system with large material database using effective computers is necessary for design of nuclear materials and analyses or simulations of the phenomena. The developed Embrittlement Data Base (EDB) at ORNL is this comprehensive collection of data. EDB database contains power reactor pressure vessel surveillance data, the material test reactor data, foreign reactor data (through bilateral agreements authorized by NRC), and the fracture toughness data. The lessons learned from building EDB program and the associated database management activity regarding Material Database Design Methodology, Architecture and the Embedded QA Protocol are described in this report. The development of IAEA International Database on Reactor Pressure Vessel Materials (IDRPVM) and the comparison of EDB database and IAEA IDRPVM database are provided in the report. The recommended database QA protocol and database infrastructure are also stated in the report.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Validation of numerical models for seismic fluid-structure-interaction analysis of nuclear, safety-related equipment

Seismic design, qualification, and risk assessment of nuclear safety-related vessels filled with liquid will have to consider the interaction between the vessel (tank), the contained liquid, and submerged components, if any. Seismic fluid-structure-interaction (FSI) analysis of nuclear vessels will rely on numerical models, which are required to be verified and validated. This study validates previously-verified numerical models using test data generated from earthquake-simulator experiments involving a cylindrical tank. Two solvers in LS-DYNA for FSI simulations are used for the numerical analysis: Arbitrary-Lagrangian-Eulerian (ALE) and Incompressible Computational Fluid Dynamics (ICFD). Numerical and test results are compared for responses critical to seismic design of advanced reactor vessels: hydrodynamic pressures on the tank wall, reactions at the support, and wave heights of the contained liquid. Analysis is performed for one-, two-, and three-directional seismic inputs with a range of intensity, and rocking motions. The accuracy of the numerical results and different methods for outputting wave heights are discussed. Recommendations for validation of seismic FSI numerical models of advanced reactors are provided. As a result, the validation exercise presented in this study is broadly applicable to cylindrical tanks, regardless of industry sector.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

ORNL Trusted Corridors Project: Watts Bar Dam Inland Waterway Project

Radiation has existed everywhere in the environment since the Earth's formation - in rocks, soil, water, and plants. The mining and processing of naturally occurring radioactive materials for use in medicine, power generation, consumer products, and industry inevitably generate emissions and waste. Radiological measuring devices have been used by industry for years to measure for radiation in undesired locations or simply identify radioactive materials. Since the terrorist attacks on the United States on 9-11-01 these radiation measuring devices have proliferated in many places in our nation's commerce system. DOE, TVA, the Army Corps and ORNL collaborated to test the usefulness of these devices in our nation's waterway system on this project. The purpose of the Watts Bar Dam ORNL Trusted Corridors project was to investigate the security, safety and enforcement needs of local, state and federal government entities for state-of-the-art sensor monitoring in regards to illegal cargo including utilization of the existing infrastructure. TVA's inland waterways lock system is a recognized and accepted infrastructure by the commercial carrier industry. Safety Monitoring activities included tow boat operators, commercial barges and vessels, recreational watercraft and their cargo, identification of unsafe vessels and carriers, and, monitoring of domestic and foreign commercial vessels and cargo identification. Safety Enforcement activities included cargo safety, tracking, identification of hazardous materials, waterway safety regulations, and hazardous materials regulations. Homeland Security and Law Enforcement Applications included Radiological Dispersive Devices (RDD) identification, identification of unsafe or illicit transport of hazardous materials including chemicals and radiological materials, and screening for shipments of illicit drugs. In the Fall of 2005 the SensorNet funding for the project expired. After several unsuccessful attempts to find a Federal sponsor to continue with the project, the Watts Bar Dam Project was canceled and the Exploranium radiation monitors were removed from the doors of Watts Bar Dam in early 2006. The DHS Domestic Nuclear Detection Office decided to proceed with a Pilot building on the ORNL work performed at the TN and SC weigh stations in the highway sector of the Trusted Corridors project and eventually expanded it to other southern states under the name of Southeastern Corridor Pilot Project (SETCP). Many of the Phase I goals were achieved however real-world test data of private watercraft and barges was never obtained.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Operation Upshot-Knothole

A thundering boom and sheet of fire announced a dramatic, once in a lifetime event – the firing of a nuclear projectile from a 280 mm cannon. Travelling seven miles downrange, the projectile detonated 500 feet over the Nevada Test Site’s Frenchman Flat with a force of fifteen kilotons. Although the test was successful, the massive cannon, designed for tactical battlefield use, had a critical flaw. It was too large and cumbersome for mobile combat. The cannon test, codenamed Grable, was part of Operation Upshot-Knothole, the fourth test series conducted in Nevada. Beginning with the Annie test on March 17, 1953, and concluding with the Climax test on June 4th, the Operation consisted of three airdrops, seven tower detonations, and the one artillery shot. As with previous Nevada tests, the demarcation between the weapon development series, Upshot, and the DOD effects tests, Knothole, was blurred. All eleven tests generated data in support of weapon development as well as tactical battlefield applications. During Upshot-Knothole, the University of California Radiation Laboratory (UCRL), conducted its first ever tests, Ruth and Ray. Although neither test was successful, these failures, along with another a year later at Operation Castle, provided the new laboratory with design data leading to future successful tests. The Federal Civil Defense Administration (FCDA) participated in a test series with the general goal of preparing for societal recovery from a nuclear attack. Known as Operation Doorstep, the FCDA’s experiments evaluated the effects of a nuclear attack on food supplies, housing and urban structures, and even a copse of trees transplanted from nearby Mt. Charleston. A contingent of the press witnessed test Annie from an outcropping of rocks, subsequently named News Nob. The presence of the news media, along with the FCDA’s participation, marked a fundamental change in the Nevada test program - a change that that now included the general populace, whose survival was, of course, the rationale for testing. The Department of Defense continued and expanded its Desert Rock exercises of troop exercises, helicopter operations, and evaluation of blast damage to military aircraft, tanks, and guns. Annie, Nancy, Badger, Simon, Encore, and Grable involved larger numbers of personnel than the other five shots. Below is an edited and condensed account of Desert Rock activities compiled by the Defense Threat Reduction Agency.

45 MILITARY TECHNOLOGY, WEAPONRY, AND NATIONAL DEF↗

IMPLEMENTING THE STANDARD SPECTRUM METHOD FOR ANALYSIS OF β-γ COINCIDENCE SPECTRA

The standard deconvolution analysis tool (SDAT) algorithms were developed and tested at the University of Texas at Austin. These algorithms utilize the standard spectrum technique for spectral analysis of {beta}-{gamma} coincidence spectra for nuclear explosion monitoring. Work has been conducted under this contract to implement these algorithms into a useable scientific software package with a graphical user interface. Improvements include the ability to read in PHD formatted data, gain matching, and data visualization. New auto-calibration algorithms were developed and implemented based on 137Cs spectra for assessment of the energy vs. channel calibrations. Details on the user tool and testing are included.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

NEET In-Pile Ultrasonic Sensor Enablement-FY-2013

Several programs funded by the Department of Energy Office of Nuclear Energy (DOE-NE), such as the Fuel Cycle Research and Development, Advanced Reactor Concepts, Light Water Reactor Sustainability, and Next Generation Nuclear Plant programs, are investigating new fuels and materials for advanced and existing reactors. A key objective of such programs is to understand the performance of these fuels and materials when irradiated. The Nuclear Energy Enabling Technology (NEET) Advanced Sensors and Instrumentation (ASI) in-pile instrumentation development activities are focused upon addressing cross-cutting needs for DOE-NE irradiation testing by providing higher fidelity, real-time data, with increased accuracy and resolution from smaller, compact sensors that are less intrusive.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Corrective Action Investigation Plan for Corrective Action Unit 414: Clean Slate III Plutonium Dispersion (TTR) Tonopah Test Range, Nevada, Revision 1

Corrective Action Unit (CAU) 414 is located on the Tonopah Test Range, which is approximately 130 miles northwest of Las Vegas, Nevada, and approximately 40 miles southeast of Tonopah, Nevada. The CAU 414 site consists of the release of radionuclides to the surface and shallow subsurface from the conduct of the Clean Slate III (CSIII) storage–transportation test conducted on June 9, 1963. CAU 414 includes one corrective action site (CAS), TA-23-03CS (Pu Contaminated Soil). The known releases at CAU 414 are the result of the atmospheric dispersal of contamination from the 1963 CSIII test. The CSIII test was a nonnuclear detonation of a nuclear device located inside a reinforced concrete bunker covered with 8 feet of soil. This test dispersed radionuclides, primarily uranium and plutonium, on the ground surface. The presence and nature of contamination at CAU 414 will be evaluated based on information collected from a corrective action investigation (CAI). The investigation is based on the data quality objectives (DQOs) developed on June 7, 2016, by representatives of the Nevada Division of Environmental Protection; the U.S. Air Force; and the U.S. Department of Energy (DOE), National Nuclear Security Administration Nevada Field Office. The DQO process was used to identify and define the type, amount, and quality of data needed to develop and evaluate appropriate corrective action alternatives for CAU 414.

54 ENVIRONMENTAL SCIENCES↗

Measurements and computational analysis of the natural decay of 176 Lu

Background: Mainly because of its long half-life and despite its scientific relevance, spectroscopic measurements of 176 Lu forbidden β decays are very limited and lack formulation of shape factors. A direct precise measurement of its Q value is also presently unreported. In addition, the description of forbidden decays provides interesting challenges for nuclear theory. The comparison of precise experimental results with theoretical calculations for these decays can help to test underlying models and can aid the interpretation of data from other experiments. Purpose: Perform the first precision measurements of 176 Lu β-decay spectra and attempt the observation of its electron capture decays, as well as perform the first precision direct measurement of the 176 Lu β-decay Q value. Compare the shape of the precisely determined experimental β spectra to theoretical calculations, and compare the end point energy to that obtained from an independent Q value measurement. Method: Here, the 176 Lu β-decay spectra measurements and the search for electron capture decays were performed with an experimental setup that employed lutetium-containing scintillator crystals and a NaI(Tl) spectrometer for coincidence counting. The β decay Q value was determined via high-precision Penning trap mass spectrometry (PTMS) with the LEBIT facility at the National Superconducting Cyclotron Laboratory. The β-spectrum calculations were performed within the Fermi theory formalism with nuclear structure effects calculated using a shell model approach. Results: Both β transitions of 176 Lu were experimentally observed and corresponding shape factors formulated in their entire energy ranges. The search for electron capture decay branches led to an experimental upper limit of 6.3×10 –6 relative to its β decays. The 176 Lu β-decay and electron capture Q values were measured using PTMS to be 1193.0(6) and 108.9(8) keV, respectively. This enabled precise β end point energies of 596.2(6) and 195.3(6) keV to be determined for the primary and secondary β decays, respectively. The conserved vector current hypothesis was applied to calculate the relativistic vector matrix elements. The β-spectrum shape was shown to significantly depend on the Coulomb displacement energy and on the value of the axial vector coupling constant gA, which was extracted according to different assumptions. Conclusion: The implemented self-scintillation method has provided unmatched observations of 176 Lu, independently validated by the first direct measurements of its β-decay Q value by Penning trap mass spectrometry. Theoretical study of the main β transition led to the extraction of very different effective gA and log10f values, showing that a high-precision description of this transition would require a realistic nuclear structure with nucleus deformation.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Experimental study of heat transfer in a 7-element bundle cooled with supercritical Freon-12

Experimental data on Supercritical-Water (SCW) cooled bundles are very limited. Major problems with performing such experiments are technical difficulties in testing and experimental costs at high pressures, temperatures and heat fluxes. Also, there are only a few SCW experimental setups currently in the world capable of providing data. Supercritical Water-cooled nuclear Reactors (SCWRs), as one of the six concepts of Generation IV reactors, cannot be designed without such data. Therefore, a preliminary approach uses modeling fluids such as carbon dioxide and refrigerants instead of water is practical. In particularly, experiments in supercritical refrigerant-cooled bundles can be used. One of the SC modeling fluids typically used is Freon-12 (R-12) with the critical pressure of 4.136 MPa and the critical temperature of 111.97 deg. C. These conditions correspond to the critical pressure of 22.064 MPa and critical temperature of 373.95 deg. C in water. A set of experimental data obtained at the Inst. of Physics and Power Engineering (IPPE, Obninsk, Russia) in a vertically-oriented bundle cooled with supercritical R-12 was analyzed. This dataset consisted of 20 runs. The test section was 7-element bundle installed in a hexagonal flow channel with 3 grid spacers. Data was collected at pressures of approximately 4.65 MPa for several different combinations of wall and bulk-fluid temperatures that were below, at, or above the pseudo-critical temperature. The values of mass flux were ranged from 400 to 1320 kg/m{sup 2}s and inlet temperatures ranged from 72 to 120 deg. C. The test section consisted of fuel-element simulators that were 9.5 mm in OD with the total heated length of about 1 m. Bulk-fluid and wall temperature profiles were recorded using a combination of 8 different thermocouples. Analysis of the data has confirmed that there are three distinct heat-transfer regimes for forced convention in supercritical fluids: 1) Normal heat transfer; 2) Deteriorated heat transfer characterized with higher than expected wall temperatures; and 3) Enhanced heat transfer characterized with lower than expected wall temperatures. It was also confirmed that the effects of spacers are evident which was previously observed in sub-critical experimental data. (authors)

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Assessment of Condition Monitoring Methods and Technologies for Inservice Inspection and Testing of Nuclear Power Plant Components

This report was prepared for the U.S. Nuclear Regulatory Commission (NRC) to explore the application of advanced technologies toward meeting the current and future regulatory requirements for maintenance and condition monitoring of structures, systems, and components. The advanced technologies considered in this work are advanced sensors and instrumentation, data analytics, machine learning and artificial intelligence (ML/AI), physics-based models, and digital twins (DT). The interest in the application of advanced technologies for condition monitoring in nuclear power plants continues to grow, and current and future licensees are expected to implement advanced technologies as part of their inservice inspection (ISI) and inservice testing (IST) programs. This report delineates the outcomes of an exploratory investigation into the implementation of advanced condition monitoring technologies to address ISI and IST requirements. A thorough review was conducted of the existing regulatory requirements for ISI and IST, along with an analysis of associated industry practices. Additionally, a state-of-the-art assessment was performed on advanced condition monitoring technologies frequently employed in non-nuclear sectors. This research incorporated two nuclear-specific case studies to illustrate the application of these technologies within the current nuclear fleet. The report provides an exhaustive discussion on the technical challenges, considerations, and opportunities associated with the deployment of advanced condition monitoring technologies. The following are key considerations in the application of advanced technologies for the ISI and IST of nuclear power plant components: • Developing adequate verification and validation procedures to confirm the functional and non-functional requirements, • Developing technical capabilities to conduct real-time asset condition monitoring, • Establishing guidance and protocol for modeling and simulation tools to continuously meet regulatory requirements, • Addressing trustworthiness, explainability, and interpretability of ML/AI methods, • Evaluating maintenance activities to maintain an adequate safety margin and avoid undesirable conditions, • Establishing cybersecure condition monitoring programs associated with a computer-based software system, and • Establishing standardized evaluation metrics for advanced condition monitoring programs. Interest in the use of advanced technologies for condition monitoring in ISI and IST programs continues to grow, and the technology is expected to experience rapid and wide industry adoption in the near future. Adoption of advanced technologies for condition monitoring could have novel and unique impacts on regulatory activities associated with ISI and IST programs. The NRC is continuing to explore the regulatory aspects of advanced technologies as part of ISI and IST programs by pursuing additional research in this technical area.

22 - GENERAL STUDIES OF NUCLEAR REACTORS↗

Transportation Modeling and Global Health

A patient in the United States has been diagnosed with Ebola. Fear and panic kicks in across the country, and hospitals are inundated with hundreds of people, some infected with the highly contagious disease and others not. Blood tests are needed for positive diagnoses, but the diagnostic labs are overwhelmed with blood samples to test, and staff are overworked and stressed. Infected people need to be quarantined and treated, but it's hard to find rooms to quarantine so many patients. Sick people who need triage and regular care for other emergencies are afraid to go to hospitals for fear of Ebola, which has a 50% fatality rate. And since hospitals are so overwhelmed, sick people often stay home, infecting heathy people around them; the U.S. is now in the grips a full-blown Ebola outbreak. Sandia's high-performance computers simulated such a nightmare scenario recently, and with good reason. An Ebola outbreak in the United States could be devastating if hospitals are not prepared. When an Ebola outbreak in West Africa became a global concern in 2014, health advisers were alarmed at the length of time it took to properly diagnose infected people. In rural areas in Liberia, for example, blood samples from ailing people would be sent to a laboratory for testing, but the closest lab was hundreds of miles away through difficult and sometimes impassable roads. In more urban areas, blood samples would be sent to nearby labs, but those labs were often already overburdened by the sheer volume of samples to test. Staff at some treatment centers were unaware that a lab a little farther away might have the capacity to take in more samples. Meanwhile, undiagnosed infected people were unknowingly spreading the disease to many others around them, worsening the outbreak. The U.S. Defense Threat Reduction Agency (DTRA) and Centers for Disease Control and Prevention (CDC) posed a serious question: how do we improve blood-sample transportation routes in Liberia to ensure that samples taken from ill people are tested as quickly as possible, ensuring a proper diagnosis and faster treatment? Sandia scientists, already experts in transportation modeling for nuclear materials, quickly swarmed on this problem. The Sandia Ebola response team immediately set out to collect data from the region using available maps and local information, and transformed the raw data to GIS maps. Then, applying Sandia transportation routing algorithms, the team identified the optimal routes to get blood samples to the best laboratory for testing, even if that lab was not geographically the closest. The models also showed the best possible locations for mobile diagnostic laboratories that would better support the very rural regions that were most affected by the Ebola outbreak.

59 BASIC BIOLOGICAL SCIENCES↗

Design, Fabrication and Start-up of Test Facilities for the LAWPS Full-Scale IX Column Test and Engineering Scale Test - 17418

The U.S. Department of Energy (DOE), Office of River Protection's (ORP) primary mission is to retrieve and treat Hanford's tank waste and close the Tank Farms to protect the Columbia River. Mixed radioactive waste is stored in 177 underground tanks at the Hanford Site as reported in DOE/ORP 2003-02, Environmental Impact Statement for Retrieval, Treatment, and Disposal of Tank Waste and Closure of the Single Shell Tanks at the Hanford Site, Richland WA, Inventory and Source Term Data Package. The 177 underground tanks are estimated to contain about 56 million gallons of waste. The Low Activity Waste Pretreatment System (LAWPS) Project provides for the early production of immobilized low activity waste (ILAW) by feeding LAW directly from Tank Farms to the Hanford Waste Treatment Plant's (WTP's) LAW Facility, bypassing the Pretreatment Facility. Prior to the transfer of feed to the WTP LAW Vitrification Facility, tank supernatant waste will be pretreated in the LAWPS to meet the WTP LAW waste acceptance criteria. The LAWPS will also facilitate the return of secondary liquid wastes from the WTP LAW Vitrification Facility to the Tank Farms. In November of 2015 DOE's Tank Operations Contractor, Washington River Protection Solutions (WRPS), awarded a contract to the AECOM Team to design, fabricate and operate two test platforms to generate performance data at two different scales and demonstrate technology maturation. The first platform models the ion exchange (IX) columns at full scale, and the second platform models the integrated flowsheet (cross flow filter (CFF) and IX) at 1/9. scale. Both test platforms underwent shakedown and start-up testing in August 2016 and moved into actual testing and NQA-1 data generation shortly thereafter. This paper covers the engineering design, procurement, construction, installation, and acceptance testing of the test platforms (which are now operational) under an aggressive fast track schedule, and initial test data as available. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

New Los Alamos space instrument goes for a spin

Scientists and engineers at Los Alamos National Laboratory are using a unique centrifuge facility to evaluate a flight-ready telemetry system for evaluating a nuclear weapons test missile launch. "The telemetry unit was designed and manufactured by Los Alamos' Intelligence and Space Research Division," said Telemetry Program Manager Myles Fitzgerald. "Telemetry is a data stream of information on temperature, acceleration, vibration, strain, all the conditions a system encounters during a test flight." Because a test missile flight ultimately ends with the test system completely destroyed, telemetry data from the flight must be collected by receiving stations along the flight path. "The purpose of the centrifuge test is to subject the electronics to a high gravitational load (G-load) that's representative of what the system will experience when re-entering the Earth's atmosphere," said weapons test engineer Alex Cusick.

45 MILITARY TECHNOLOGY, WEAPONRY, AND NATIONAL DEF↗

A direct test of Auger cascade induced nucleation from heavy element contamination in C 3 F 8 bubble chambers

Understanding and quantifying the gamma-induced bubble nucleation background in clean nuclear recoil detection bubble chambers is of utmost importance to bubble chamber based dark matter searches. Here, we present data confirming the hypothesis that large Auger cascades from high-Z elements such as iodine and xenon dramatically increase the response of C 3 F 8 bubble chambers to gamma rays. These tests, performed with a small calibration bubble chamber filled with C 3 F 8 +$\mathcal{O}$ (10) ppm xenon, show that the probability of bubble nucleation scales with the rate of xenon inner-shell vacancies, reaching values >10% per K-Shell vacancy for Seitz thresholds of interest to future dark matter searches in bubble chambers. We also place an upper limit on bubble nucleation probability for argon Auger events, relevant to large future bubble chambers which may contain some residual atmospheric argon after the active fluid fill.

47 OTHER INSTRUMENTATION↗

Online monitoring of rod control systems in combustion engineering pressurized water reactors - 195

Current designs of Pressurized Water Reactors (PWRs) are equipped with control and shutdown rods that are inserted and withdrawn from the reactor core to control reactivity. In Combustion Engineering (CE) plants, these rods are moved using the Control Element Drive Mechanism (CEDM) and controlled by the CEDM Control System (CEDMCS). In the event of system failure, troubleshooting activities can have a substantial impact on plant resources. Furthermore, CEDM component failures have occurred without warning, which has led to increased costs for the plants. These issues, combined with the inherently complex design of the CEDMCS, create a need for an online diagnostics system that can improve system health monitoring, increase diagnostic capabilities, and decrease troubleshooting time. This paper describes an advanced analysis and diagnostics system that monitors the CEDMCS during plant operation and provides critical information to onsite personnel to help detect and prevent problems before they impact normal plant operation. This system uses existing CEDMCS test points to acquire data and needs no modifications to the CEDMCS for implementation. The online monitoring capabilities automatically collect data during normal operation and diagnose failure events, reduce troubleshooting time and provide plant personnel with valuable information which is not currently available. Additionally, the system has built-in features used to streamline routine surveillance testing, collect stationary and movement data on multiple rods simultaneously, automate analysis, and generate reports. This system was developed with input from industry CEDMCS engineers at existing commercial facilities and has been deployed in multiple operating nuclear plants. The system has demonstrated itself to be a valuable tool for CEDMCS health monitoring, not only in reducing required man-power for routine system testing, but also in detected impending coil faults and allowing plant engineers to mitigate system component failures to prevent impending plant shut downs. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

New Los Alamos space instrument goes for a spin

Scientists and engineers at Los Alamos National Laboratory are using a unique centrifuge facility to evaluate a flight-ready telemetry system for evaluating a nuclear weapons test missile launch. "The telemetry unit was designed and manufactured by Los Alamos' Intelligence and Space Research Division," said Telemetry Program Manager Myles Fitzgerald. "Telemetry is a data stream of information on temperature, acceleration, vibration, strain, all the conditions a system encounters during a test flight." Because a test missile flight ultimately ends with the test system completely destroyed, telemetry data from the flight must be collected by receiving stations along the flight path. "The purpose of the centrifuge test is to subject the electronics to a high gravitational load (G-load) that's representative of what the system will experience when re-entering the Earth's atmosphere," said weapons test engineer Alex Cusick.

45 MILITARY TECHNOLOGY, WEAPONRY, AND NATIONAL DEF↗

Roadmap for the Application of Ion Beam Technologies to Challenges for the Advancement and Implementation of Nuclear Energy Technologies

The use of ion beams in interrogating materials performance for nuclear energy applications is advancing at a rapid rate. Ion irradiations have been proven to produce radiation effects data that are of direct relevance for understanding neutron-induced displacement damage. This development reflects significant and continued investment in infrastructure by the U.S. Department of Energy (DOE) as well as support of science and engineering research at universities and national laboratories. Application of ion beam irradiation methods to enhance the deployment of materials in reactors is in the spirit of the Gateway for Accelerated Innovation in Nuclear (GAIN) initiative sponsored by DOE to accelerate the deployment of innovation in the U.S. nuclear industry. Ion beam irradiation shows considerable promise for assisting in down selecting candidate materials for use in both current and advanced nuclear energy systems. Ion beams allow rapid achievement of materials damage levels not accessible by neutron irradiation in test reactors due to cost and time constraints. Ion beam studies provide data on the effects of irradiation under very specific conditions of temperature, radiation dose, and radiation dose rate that are difficult or impossible to achieve via reactor irradiation experiments. This data can be used to develop and validate detailed predictive radiation effects models for use in reactor materials research and development. Despite the current high state of the art and the maturity of quality assurance, there are still challenges to the deployment of ion beam data in support of reactor materials qualification. For the most part, these challenges arise from the lack of a detailed mechanistic understanding of potential difference between ion induced and neutron induced materials damage, which is exacerbated by difficulties in obtaining bulk physical and mechanical properties data from the micron-scale heavy ion irradiation depths. In particular, improved understanding of dose rate effects, as a function of temperature, are needed. This document offers a roadmap for the development and enhancement of current U.S. ion beam irradiation technologies within university and national laboratory settings, and especially for the deployment of new highly controlled in situ interrogation of materials during irradiation to provide dynamic and mechanistic data for model development. The status and capabilities of relevant U.S. ion beam facilities are summarized and recommended “best practices” for performing ion irradiations are described. The potential role of ion beam irradiations to assist the development and deployment of reactor materials is outlined. Key principles include developing methods for rapid and cost-effective materials selection and development, characterizing fundamental material response under irradiation, and developing a robust mechanistic understanding of microstructure evolution under irradiation (including development and validation of reliable predictive models for microstructure evolution).

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗