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Radiation effects in concrete for nuclear power plants, Part II: Perspective from micromechanical modeling

The need to understand and characterize the effects of neutron irradiation on concrete has become urgent because of the possible extension of service life of many nuclear power generating stations. Current knowledge is primarily based on a collection of data obtained in test reactors. These results are inherently difficult to interpret because materials and testing conditions are inconsistent. A micromechanical approach based on the Hashin composite sphere model is presented to derive a first-order separation of the effects of radiation on cement paste and aggregate, and, also, on their interaction. Although the scarcity of available data limits the validation of the model, it appears that, without negating a possible gamma-ray induced effect, the neutron-induced damage and swelling of aggregate plays a predominant role on the overall concrete expansion and the damage of the cement paste. Finally, the radiation-induced volumetric expansion (RIVE) effects can also be aided by temperature elevation and shrinkage in the cement paste.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Second Annual Progress Report on Correlation Between Microstructure and Mechanical Properties of Neutron-Irradiated Ferritic-Martensitic and Austenitic Steels

Ferritic-martensitic steels G92-2b (an optimized Grade 92 heat), NF616 and T91, and austenitic stainless steel 800H and its Grain Boundary Engineering (GBE)-treated version 800H-TMP (ThermoMechanical Processing) were irradiated in the High Flux Isotope Reactor (HFIR) of Oak Ridge National Laboratory (ORNL) and the Advanced Test Reactor (ATR) of Idaho National Laboratory (INL). Selected G92-2b samples were irradiated up to 14.66 dpa in the HFIR at two temperature ranges: 400–496.7°C and 683.3– 720°C. NF616 and T91 were irradiated in the ATR up to 8.16 dpa with the irradiation temperatures ranged from 241°C to 447.5°C. Alloy 800H and 800H-TMP samples were irradiated in both the HFIR and the ATR. Selected 800H and 800H-TMP samples had HFIR irradiation to 1.28 dpa at 580°C and ATR irradiation up to 9.12 dpa at 359°C to 431°C. Vickers hardness measurements, fractography, and microstructural characterization were performed on the selected samples in the Low Activation Materials Design and Analysis (LAMDA) laboratory. Radiation-hardening of G92-2b was observed at the lower doses and lower irradiation temperatures (400- 496.7°C), with GB03 (0.52 dpa at 400°C) and GB04 (7.44 dpa at ~490°C) showing ~12% and ~8% hardening, respectively. Softening by ~14% was observed for GB05 (14.66 dpa at 496.7°C). Radiationsoftening of G92-2b was more prevalent at the higher irradiation temperatures (683.3-~720°C), with GB10 (0.46 dpa at 683.3°C), GB11 (7.44 dpa at ~720°C), and GB12 (14.63 dpa at ~720°C) showing ~8%, ~8%, and ~40% softening, respectively. Radiation-hardening of NF616 and T91 was observed with the hardness increased by ~37% to ~65% depending on the irradiation doses and irradiation temperatures. Within the studied irradiation conditions of NF616 and T91, samples with a higher dose had a larger hardness after irradiation. All the tested alloy 800H and 800H-TMP samples in this work showed radiation-hardening by ~96±7% to ~152±10%. Alloy 800H-TMP tended to have slightly smaller radiation-hardening than alloy 800H. The fractography results of G92-2b sample GB03, GB10, and GB11, together with the previously characterized fractography of GB04, GB05, and GB12, indicated that the ductility of G92-2b was maintained up to 14.66 dpa at the lower irradiation temperatures of 400-496.7°C, while some loss of ductility (less necking) was observed for higher doses at the higher irradiation temperatures of 683.3-720°C. This agrees with the previously reported tensile test results of G92-2b, where the elongation of G92-2b was reduced at higher doses at the higher irradiation temperatures. Dimple sizes increased at higher doses, which are more evident at the higher irradiation temperatures of 683.3-~720°C. The fractography of NF616 sample D2 (2.96 dpa at 291.5°C), D4 (5.91 dpa at 359°C), and D6 (8.16 dpa at 431°C) indicated loss of ductility with negligible necking for sample D2, while ductile failure for samples D4 and D6. Fractography of alloy 800H and 800H-TMP samples in various irradiation conditions showed ductile failure with obvious necking. Dimples were observed, with some of them containing large Ti-rich particles, in all the 800H/800H-TMP samples. Electron backscatter diffraction characterization of GB12 indicated the recovery of the lath structure, which was generally replaced by an equiaxed grain structure. Transmission electron microscopy (TEM) characterization showed the presence of frequent M 23 C 6 (M = primarily Cr), MX (M = primarily V), spherical Nb(C,N) precipitates, and occasional Laves phase precipitates in the G92-2b samples. MX precipitates with sizes of 20-30 nm were observed at boundaries of smaller grains, indicating the pinning effect of the V-rich precipitates. The lath structure recovery was more evident at the higher irradiation temperatures (683.3-~720°C), with decreased densities of line dislocations and M23C6 precipitates. The irradiated T91 (TA04) showed the growth of M23C6 precipitates to 101 ± 40 nm from the initial 68 ± 22 nm in the unirradiated condition. Dislocation loops of both {100} and {111} types were present in TA04. TEM characterization was also performed on the irradiated 800H (N4, N5, N6, and AR2) and 800H-TMP (P4, P5, P6, and HG1). Accumulation of M 23 C 6 precipitates at grain boundaries was observed in all the xii 800H/800H-TMP samples, and the presence of Ti(C,N) precipitates at grain boundaries and in the matrix was observed in the irradiated 800H-TMP. Some Ti(C,N) precipitates are embedded in the M 23 C 6 precipitates, maintaining specific orientation relationships between the precipitates and between the precipitate and matrix. In addition, nanoscale Si-rich clusters were observed in the matrix of all the 800H/800H-TMP samples, with EDS Si maps tending to have a lower contrast in 800H-TMP samples. Atom probe tomography was conducted on the same samples, supported by a Rapid Turnaround Examination project under Nuclear Science User Facilities. The results are being analyzed to be integrated with the TEM results for a confident description of the γ’ precipitates. Dislocation loops also formed in all the 800H/800H-TMP samples. The density and the average size of dislocation loops were quantified to be in the order of 10 22 – 10 23 m -3 and 11.7 – 15.9 nm, respectively, in the ATR-irradiated 800H/800H-TMP samples. The loop densities in irradiated 800H were higher than that in irradiated 800H-TMP under the same irradiation conditions. Further systematic data analyses, together with some complementary experiments, will be pursued for these samples to foster peer-reviewed journal article publications.

36 MATERIALS SCIENCE↗

Generating unstructured nuclear reactor core meshes in parallel

Recent advances in supercomputers and parallel solver techniques have enabled users to run large simulations problems using millions of processors. Techniques for multiphysics nuclear reactor core simulations are under active development in several countries. Most of these techniques require large unstructured meshes that can be hard to generate in a standalone desktop computers because of high memory requirements, limited processing power, and other complexities. We have previously reported on a hierarchical lattice-based approach for generating reactor core meshes. Here, we describe efforts to exploit coarse-grained parallelism during reactor assembly and reactor core mesh generation processes. We highlight several reactor core examples including a very high temperature reactor, a full-core model of the Korean MONJU reactor, a ¼ pressurized water reactor core, the fast reactor Experimental Breeder Reactor-II core with a XX09 assembly, and an advanced breeder test reactor core. The times required to generate large mesh models, along with speedups obtained from running these problems in parallel, are reported. A graphical user interface to the tools described here has also been developed.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Coordination of Plutonium Separations

NASA and the Department of Energy (DOE) are currently working together to reestablish a 238Pu supply capability using DOE's existing facilities and reactors. The effort is being led by Oak Ridge National Laboratory (ORNL). Target rods, containing neptunium oxide (NpO2), are fabricated at ORNL and irradiated in the ORNL High Flux Isotope Reactor (HFIR) currently and soon will be irradiated in the Advanced Test Reactor (ATR) at Idaho National Laboratory (INL). Irradiated targets are processed in hot cells at the ORNL Radiochemical Engineering Center to recover the plutonium (Pu) product and unconverted neptunium (Np) for recycle. The 238PuO2 product is shipped to Los Alamos National Laboratory (LANL) for fabrication of heat source pellets. Key activities, such as the transport of the neptunium to ORNL, irradiation of neptunium, and chemical processing to recover the newly generated 238Pu, have been demonstrated with the initial amounts of ~100 g heat-source plutonium oxide (HS PuO2) produced. Product samples have been shipped to LANL for evaluation, including chemical impurity analysis. This paper will examine the status of producing new 238Pu from irradiated targets.

Wham, Robert↗

Ceramography and Thermal Modelling of Irradiated TRISO Particles using BISON

This study presents a comprehensive analysis of irradiated TRISO fuel particles from the Advanced Gas Reactor (AGR) Fuel Development and Qualification Program conducted at the Advanced Test Reactor (ATR) as part of my internship. Failure Analysis using high-resolution microscopy was performed to characterize mechanisms in TRISO particle layers, including the kernel, buffer, inner pyrolytic carbon (IPyC), silicon carbide (SiC), and outer pyrolytic carbon (OPyC) coatings. Failure modes were systematically classified. Thermal conductivity properties of each TRISO layer were evaluated through experimental measurements and computational models for use in BISON finite element code. Experimental thermal conductivity values ranged from 0.5 W/m·K for the buffer layer to 168 W/m·K for SiC, while BISON simulations provided averaged values of 0.57 W/m·K (buffer), 4.0 W/m·K (PyC layers), and 15.95 W/m·K (SiC). Temperature-dependent correlations from PARFUME were implemented for kernel thermal properties.

BISON↗

Expansion of the Fuel Motion Monitoring System

The Idaho National Laboratory (INL) Transient Reactor Test Facility (TREAT) Fuel Motion Monitoring System (FMMS) is a diagnostic tool used to visualize the movement and location of fuel within the nuclear reactor during transient experiments. TREAT is designed to test the behavior of nuclear fuel under accident conditions, such as a rapid power increase. The TREAT FMMS, also referred to as the “hodoscope” because of the system’s massive steel collimator component, is located on the North beam port of the reactor. While the FMMS system is capable of incorporating a total of 360 sensors, initial refurbishment efforts resulted in a array of 96 fast neutron detectors. This initial array was configured to provide a narrow (2 channels) full-length view of experiment vessels with an extended 4-channel–wide region in the center of the array capable of providing a full view of all initially planned experiments. Planning and efforts to expand the FMMS array began immediately following the restart of TREAT. An additional 96 detectors were evaluated, characterized, and prepared for installation at TREAT during the summer of 2018. Unfortunately, funding reductions forced the project towards a 5-year hiatus. In October of 2023 funding from the Department of Energy’s Nuclear Science User Facilities enabled the expansion to recommence. This report serves to document the activities performed to expand the FMMS detector array to 192 channels in order to provide a broader view of the larger and more sophisticated test capsules currently planned for future irradiation in the TREAT reactor. This expansion also included doubling the data acquisition capability, addressing the new heat load on the system, and synchronizing the time for all digital components.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Transient testing of uranium silicide fuel in zircaloy and silicon carbide cladding

Using the newly restarted Transient Reactor Test (TREAT) facility at Idaho National Laboratories, fresh (unirradiated) U 3 Si 2 fuel pellets were tested under reactivity-initiated accident conditions in dry helium capsules. These tests were performed with total energy depositions sufficient to induce melting of the U 3 Si 2 fuel pellets based on available thermophysical property data. The instrumented experiments utilized in-pile thermocouples and infrared pyrometers to measure the cladding temperature during the transient, which are in reasonable agreement with predicted peak cladding temperatures using a simple BISON fuel performance model. This same model is then used to predict expected cladding stresses during the transients in areas where pellet cladding interaction is expected. It was shown that for transient energy depositions up to 528J/g rod like geometry of the test articles was maintained. While it is acknowledged that more confirmatory testing is required in more prototypic environments, these first of their kind experiments have demonstrated that unirradiated U 3 Si 2 fuel and unirradiated SiC-SiC claddings can likely retain a “rod like” geometry for transient energy depositions up to 528J/g.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Transmission Electron Microscopy based Characterization of a U-20Pu-10Zr Fuel Irradiated in Experimental Breeder Reactor-II

U-Pu-Zr metallic fuels are important fuel candidate for future advanced and/or test reactors. To better understand fuel performance and guide future fuel development, a U-20Pu-10Zr (in weight) metallic fuel irradiated in the Experimental Breeder Reactor was revisited using advanced electron microscopies. This fuel was irradiated to a burnup of 7.6 % at a peak cladding temperature of 521 °C. In this research, several transmission electron microscopy samples were extracted from different but representative radial locations of the fuel cross section using focused ion beam technique. Phase identification and chemical analysis with sub-micron spatial resolution was carried out using scanning transmission electron microscopy. Multiple phenomena that are critical to fuel performance, such as Zr phase and its distribution in a different matrix, were revealed in an unpreceded and highly detailed manner. An improved understanding of fuel reconstruction in U-Pu-Zr metallic fuel under reactor irradiation is provided.

36 MATERIALS SCIENCE↗

Simulation of natural circulation cartridge loop experiments and application to molten salt reactors

This work uses the TRAC/RELAP Advanced Computational Engine (TRACE) thermal hydraulics (TH) code to model natural circulation cartridge loop experiments previously conducted at Oak Ridge National Laboratory (ORNL) using water and compares the simulated and experimental results. TRACE is also used to characterize natural circulation in the cartridge loop vehicle using FLiNaK as the working fluid. The experimental vehicle is a buoyancy-aided, annular cartridge loop, referred to as a thermosyphon, and is designed to aid in qualifying liquid–fueled and/or liquid–cooled irradiation experiments for the Versatile Test Reactor (VTR), which is currently being designed in the United States. Out-of-pile water experiments have been conducted using the cartridge and the Thermosyphon Test Loop facility at ORNL, and future experiments are anticipated that would use other molten salt surrogates as the working fluid, followed by eventual insertion of a similar cartridge into VTR. Additionally, this work aims to determine how well TRACE can replicate the natural convection conditions that were observed experimentally; this serves as an initial step for validating the modeling tool for design and safety calculations to support future irradiation experiments in VTR. Initial predictions of potential experiments were made using FLiNaK as the natural circulation fluid to demonstrate the relevance of the cartridge design to molten salt reactors (MSRs). Results from this study indicate that TRACE can accurately capture natural convection phenomena in the thermosyphon and that several design changes to the current cartridge vehicle are necessary to achieve hydraulic conditions similar to those expected in MSRs.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

AGR-3/4 Irradiation Test Train Disassembly and Component Metrology First Look Report

The AGR-3/4 experiment was designed to study fission product transport within graphitic matrix material and nuclear-grade graphite. To this end, this experiment consisted of 12 capsules, each fueled with 4 compacts containing UCO TRISO particles as driver fuel and 20 UCO designed-to-fail (DTF) fuel particles in each compact. The DTF fuel was fabricated with a thin pyrocarbon layer which was intended to fail during irradiation and provide a source of fission products. These fission products could then migrate through the compact and into the surrounding concentric rings of graphitic matrix material and/or nuclear graphite. Through post-irradiation examination (PIE) of the rings (including physical sampling and gamma scanning) fission product concentration profiles within the rings can be determined. These data can be used to elucidate fission product transport parameters (e.g. diffusion coefficients within the test materials) which will be used to inform and refine models of fission product transport. After irradiation in the Advanced Test Reactor (ATR) had been completed in April 2014, the AGR-3/4 experiment was shipped to the Hot Fuel Examination Facility (HFEF) at the Materials and Fuels Complex (MFC) for inspection, disassembly, and metrology. The AGR-3/4 test train was received at MFC in two separate shipments between February and April 2015. Visual examinations of the test train exterior did not indicate dimensional distortion, and only two small discolored areas were observed at the bottom of Capsules 8 and 9. No corresponding discoloration was found on the inside of these capsules, however. Prior to disassembly, the two test train sections were subject to analysis via the Precision Gamma Scanner (PGS), which did not indicate that any gross fuel relocation had occurred. A series of specialized tools (including clamps, cutters, and drills) had been designed and fabricated in order to carry out test train disassembly and recovery of capsule components (graphite rings and fuel compacts). This equipment performed well for separating each capsule in the test train and extracting the capsule components. Only a few problems were encountered. In one case, the outermost ring (the sink ring) was cracked during removal of the capsule through tubes. Although the sink ring will be analyzed in order to obtain a mass balance of fission products in the experiment, these cracks do not pose a major concern because the sink ring will not be analyzed in detail to obtain the spatial distribution of fission products. In Capsules 4 and 5, the compacts could not be removed from the inner rings. Strategies for removing the compacts are being evaluated. Sampling the inner rings with the compacts in-place is also an option. Dimensional measurements were made on the compacts, inner rings, outer rings, and sink rings. The diameters of all compacts decreased by 0.5 to 2.0 %. Generally, the extent of diametric shrinkage increased linearly with increasing neutron fluence. Most compact lengths also decreased. Compact lengths decreased with increasing fluence, reaching maximum shrinkage of about 0.9 % at a fast fluence of 4.0x1025 n/m2 E > 0.18 MeV. Above this fluence, the extent of length shrinkage appeared to decrease with fluence, and two compacts from Capsule 7 were found to have slightly increased in length (< 0.1 %) after a fluence of 5.2x1025 n/m2.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

01-07 Reactor Supplemental Shielding For the NRIC DOME Test Bed 01-07 Reactor Supplemental Shielding For the NRIC DOME Test Bed 2

A radiation shielding system is needed to protect personnel and equipment from harsh neutron and photon fluxes during: Reactor operations Post shut down operations Disassembly Decommissioning Examples of RSS driving requirements Radiological Controls Operating dose rate: the dose rate during normal reactor operations shall be <0.5 mrem/hr at the exterior wall of DOME containment Outdoor radiation limit: shielding shall provide the dose to a facility worker outside of DOME to <0.05 mrem/hr at 50 ft from the exterior wall of the DOME Temperature Reactors may have operating temperatures up to 800C The RSS shall be capable of removing up to 100 KW of heat during normal operating conditions the concrete structure has an upper temperature limit of 100°C

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Overview and Current Status of Analyses of Potential LEU Design Concepts for TREAT

Neutronic and thermal-hydraulic analyses have been performed to evaluate the performance of different low-enriched uranium (LEU) fuel design concepts for the conversion of the Transient Reactor Test Facility (TREAT) from its current high-enriched uranium (HEU) fuel. TREAT is an experimental reactor developed to generate high neutron flux transients for the testing of nuclear fuels. The goal of this work was to identify an LEU design which can maintain the performance of the existing HEU core while continuing to operate safely. A wide variety of design options were considered, with a focus on minimizing peak fuel temperatures and optimizing the power coupling between the TREAT core and test samples. Designs were also evaluated to ensure that they provide sufficient reactivity and shutdown margin for each control rod bank. Analyses were performed using the core loading and experiment configuration of historic M8 Power Calibration experiments (M8CAL). The Monte Carlo code MCNP was utilized for steady-state analyses, and transient calculations were performed with the point kinetics code TREKIN. Thermal analyses were performed with the COMSOL multi-physics code. Using the results of this study, a new LEU Baseline design concept is being established, which will be evaluated in detail in a future report.

Connaway, H. M.↗

Confirmatory LBL Analysis of AGR-5/6/7 Compacts and Over-Coated Particles BWXT Batches 11034, 14154C, 14156C, AND 14156D

Fuel for the Advanced Gas Reactor Fuel Development and Qualification (AGR) Program’s AGR-5/6/7 irradiation test in the Idaho National Laboratory (INL) Advanced Test Reactor (ATR) was produced by BWX Technologies (BWXT) Nuclear Operations Group in Lynchburg, Virginia. Tristructural isotropic (TRISO) coatings were deposited using a 150-mm-diameter production-scale fluidized-bed chemical vapor deposition (CVD) furnace on 425-μm-nominal-diameter spherical kernels from Lot J52R-16-69317 containing a mixture of 15.5% 235U low-enriched uranium carbide and uranium oxide (UCO). The TRISO coatings consisted of four consecutive CVD layers: a ~50% dense carbon buffer layer with 100-μmnominal thickness, a dense inner pyrolytic carbon (IPyC) layer with 40-μm-nominal thickness, a silicon carbide (SiC) layer with 35-μm-nominal thickness, and a dense outer pyrolytic carbon (OPyC) layer with 40-μm-nominal thickness. TRISO-coated particle Lot J52R-16-98005 was over-coated with a graphite/resin blend and these over-coated particles were pressed in half-inch-diameter, one-inch-long cylindrical compacts. Two packing fractions (PF) were produced, 40%PF and 25%PF, where the TRISO particle volume made up approximately 40% and 25% of the total compact volume, respectively. The AGR-5/6/7 Fuel Specification, SPC-1352 [Marshall 2016], provides the requirements necessary for acceptance of the fuel manufactured for the AGR-5/6/7 irradiation test. Quality control (QC) acceptance testing for all AGR-5/6/7 composited lots and single batches was performed by BWXT, with the exception of pyrolytic carbon (PyC) anisotropy and defective IPyC fraction in the TRISO candidate batches and final composite, which were measured at the Oak Ridge National Laboratory (ORNL) and reported in ORNL/TM-2017/036 [Hunn et al. 2017] and ORNL/TM-2017/037 [Helmreich et al. 2017a].

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Neutronics and Transient Calculations for the Conversion of the Transient Reactor Rest Facility (TREAT)

The Transient Reactor Test Facility (TREAT) is a graphite-reflected, graphitemoderated, and air-cooled reactor fueled with 93.1% enriched UO2 particles dispersed in graphite, with a carbon-to-235U ratio of ~10000:1. TREAT was used to simulate accident conditions by subjecting fuel test samples placed at the center of the core to high energy transient pulses. The transient pulse production is based on the core’s selflimiting nature due to the negative reactivity feedback provided by the fuel graphite as the core temperature rises. The analysis of the conversion of TREAT to low enriched uranium (LEU) is currently underway. This paper presents the analytical methods used to calculate the transient performance of TREAT in terms of power pulse production and resulting peak core temperatures. The validation of the HEU neutronics TREAT model, the calculation of the temperature distribution and the temperature reactivity feedback as well as the number of fissions generated inside fuel test samples are discussed.

Kontogeorgakos, Dimitrios C.↗

Postirradiation Examination of the ATF-1 Experiments - 2018 Status

The Advanced Fuels Campaign in collaboration with industry are working to develop enhanced accident tolerant fuels for light water reactors. The initial irradiations of these concepts were performed in the Idaho National Laboratory Advanced Test Reactor using simple drop-in style irradiations. These irradiations are collectively referred to as ATF 1. The postirradiation examination of ATF 1 has begun and some concepts have now completed initial examination. This report describes the results of examinations on ATF 1 irradiations designed to test the feasibility of enhancing UO 2 thermal conductivity with additives, ATF 1 irradiations of uranium silicide, and the current status of ATF 1 irradiations that are in process at the hot cell. Enhanced thermal conductivity uranium dioxide composites containing silicon carbide (UO 2 SiC) and diamond (UO 2 diamond) have been irradiated to low burnup. The conditions of this irradiation test and subsequent postirradiation examinations are discussed. These irradiations evaluate fuel microstructure and potential fuel cladding interaction under representative light water reactor power conditions. Both non destructive and destructive techniques have been used to evaluate fuel integrity, fission gas release, fission product distribution, burnup, fuel swelling and cladding strain. Examination of the UO 2 SiC pellets revealed enhanced cracking when compared to a UO 2 rodlet also irradiated under similar conditions. Additionally, instability of the SiC whiskers in the uranium dioxide matrix was observed in the pellet central region, where the local temperatures exceeded 1300 °C. The microstructure of the diamond added UO 2 was severely disrupted during irradiation, resulting in local migration of cesium along the fuel stack and increased fission gas release when compared with the expected release from the Vitanza curve at corresponding values of burnup and irradiation temperature. The postirradiation examination results cast doubt on the suitability of these additives to improve UO 2 fuel performance in a way that would lead to enhanced accident tolerance. Additionally, postirradiation examination data of U 3 Si 2 fuels at low burnup (i.e., < 20 GWd/tHM) for application in advanced Light Water Reactor (LWR) is presented. The U 3 Si 2 pellets show limited cracking in comparison to the expected behavior of UO 2 at same power level. In addition, gamma scanning data did not reveal migration of fission products. Minor homogeneous hardening along the pellet radius due to accumulation of fission products and radiation damage was measured by microindentation. The fission gas release and swelling remains very low. Formation of fission gas bubbles resolvable with optical microscopy occurs from the pellets center outward to approximately 60% of the fuel pellet radius. The overall data suggest a good performance of this accident tolerant fuel candidate at low burnup. Finally, the current status of postirradiation examination on other ATF 1 irradiations will be discussed. These irradiations include UO 2 clad in an FeCrAl alloy, an alternative uranium silicide compound U 3 Si 5 also clad in a FeCrAl alloy, and an interaction test between UO 2 and different FeCrAl alloys.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

NEA HTTR LOFC Project Test#3 Benchmark Results

In the second half of FY23, the High Temperature Engineering Test Reactor (HTTR) Loss Of Forced Cooling (LOFC)#3 data for the 9 MW test case with Vessel Cooling System (VCS) off were made available through the Nuclear Energy Agency (NEA) LOFC project framework; the neutronic model developed for the initial test (LOFC#1) achieved a satisfactory level of maturity, demonstrating its accuracy in predicting power evolution and core re-criticality, but LOFC#3 should be used primarily to investigate thermal hydraulic phenomena, as the reactor was shut down prematurely due to overheating in the upper reactor components, which prevented re-criticality; this report focuses on advancing the HTTR thermal hydraulic model to accurately simulate the LOFC#3 scenario, including simulating the LOFC#3 benchmark and generating the corresponding benchmark specifications, aiming to ensure consistency across participant models and provide essential data for future participants, including private industry stakeholders seeking to validate their computational tools.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

VALIDATION OF A RELAP5 POINT KINETICS MODEL OF TREAT

Development of advanced nuclear fuels requires testing of fuel specimens under various power-cooling mismatch conditions. The Transient Reactor Test (TREAT) facility at the Idaho National Laboratory will be used to provide transient nuclear heating of fuel specimens. Experiments will be conducted to support assessment of accident tolerant fuel designs being proposed for light water reactor applications. The experiments to be conducted at TREAT will provide data for the assessment of advanced, multi-physics computer codes. However, before the experiments can be performed, calculations are required to demonstrate that they will meet program objectives and that they can be performed safely in TREAT in the event of an unplanned reactivity insertion accident that occurs during the experiment. The safety calculations for the first experiments need to be performed in the next year and therefore will be performed with an existing computer code, RELAP5-3D. A point kinetics model of TREAT was developed for RELAP5-3D. The purpose of the model is to calculate the reactor power during experiments and to support the accident analyses of those experiments. The RELAP5-3D model was validated using data from nine TREAT experiments conducted previously. The RELAP5-3D model generates results that are in reasonable agreement with measured values of maximum core power, energy deposition, and maximum fuel temperature for a wide range of reactivity insertions.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗