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At least 919 records · Page 51

A New Era of Nuclear Criticality Experiments: The First 10 Years of Radiation Test Object Operations at NCERC

The work presented in this paper focuses on the first 10 years (2011–2020) of radiation test object (RTO) operations at the National Criticality Experiments Research Center. RTOs are subcritical configurations of special nuclear material that are built by hand. These configurations are utilized for benchmark experiments, detector testing/characterization, and training. An overview of the types of measurements used in RTO operations is given as well as a history of RTO operations at Los Alamos National Laboratory from 1944–2011.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Morphology and particle size (MaPS) exercise: testing the applications of image analysis and morphology descriptions for nuclear forensics

Image analysis techniques have been applied and shown to be a valuable tool in nuclear forensics analysis. The interlaboratory exercise reported here has tested quantitative and qualitative approaches for characterizing nuclear materials. Particle size, surface features and morphology descriptions were compared by four laboratories on a common image set generated by Scanning Electron Microscopy and Digital Light Microscopy. Quantitative analysis of the image sets through the Morphological Analysis for MAterials software highlighted the strength of image analysis, but also that the application of the software alone can introduce significant bias in the analysis. Qualitative morphology descriptions following the process outlined by Tamasi et al. (J Radioanal Nuclear Chem 307:1611–1619, 2015) were compared with a discussion on the robustness and reproducibility of the results. Finally, future work should continue to focus on proficiency and standardization of image analysis through continued exercises within the extended nuclear forensics community.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

BISON As-run AGR-3/4 Irradiation Test Predictions

BISON, a nuclear fuel performance application built using the Multiphysics Object-Oriented Simulation Environment (MOOSE) finite element library, was used to model the Advanced Gas Reactor (AGR)-3/4 irradiation test using as-run physics and thermal hydraulics data. The AGR-3/4 test consists of the combined third and fourth planned irradiations of the AGR Fuel Development and Qualification Program. The AGR-3/4 test train consists of twelve separate and independently controlled and monitored capsules. Each capsule contains four compacts filled with both uranium oxycarbide (UCO) unaltered “driver” fuel particles and UCO designed-to-fail (DTF) fuel particles. The DTF fraction was specified to be 1×10-2. This report documents the calculations performed to predict the failure probability of tristructural isotropic (TRISO) coated driver fuel particles during the AGR-3/4 experiment on a single compact. This report will demonstrate the capabilities of BISON to model the complex AGR-3/4 irradiation test and identify further development needed to capture the fuel particle failure probability and source term on every compact for further comparison from post-irradiation examination (PIE) data. The calculations include the modeling of the AGR-3/4 irradiation that occurred from December 2011 to April 2014 in the Advanced Test Reactor (ATR) over a total of 10 ATR cycles including seven normal cycles, one low power cycle, one unplanned outage cycle, and one Power Axial Locator Mechanism (PALM) cycle.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Brayton-Cycle Power-Conversion Unit Tested With Ion Thruster

Nuclear electric propulsion has been identified as an enabling technology for future NASA space science missions, such as the Jupiter Icy Moons Orbiter (JIMO) now under study. An important element of the nuclear electric propulsion spacecraft is the power conversion system, which converts the reactor heat to electrical power for use by the ion propulsion system and other spacecraft loads. The electrical integration of the power converter and ion thruster represents a key technical challenge in making nuclear electric propulsion technology possible. This technical hurdle was addressed extensively on December 1, 2003, when a closed- Brayton-cycle power-conversion unit was tested with a gridded ion thruster at the NASA Glenn Research Center. The test demonstrated end-to-end power throughput and marked the first-ever coupling of a Brayton turbo alternator and a gridded ion thruster, both of which are candidates for use on JIMO-type missions. The testing was conducted at Glenn's Vacuum Facility 6, where the Brayton unit was installed in the 3-m-diameter vacuum test port and the ion thruster was installed in the 7.6-m-diameter main chamber.

Hervol, David S.↗

Observation of excited states in 20 Mg sheds light on nuclear forces and shell evolution

The exotic Borromean nucleus 20 Mg with N = 8, located at the proton drip line provides a unique testing ground for nuclear forces and the evolution of shell structure in the neutron-deficient region. We report on the first observation of proton unbound resonances together with bound states in 20 Mg from the 20 Mg (d, d ') reaction performed at TRIUMF. Phenomenological shell-model calculations offer a reasonable description. However, our experimental results present a challenge for current first-principles nuclear structure approaches and point to the need for improved chiral forces and ab initio calculations. Furthermore, the differential cross section of the first excited state is compared with distorted-wave Born approximation calculations to deduce a neutron quadrupole deformation parameter of β$_n$ = 0.46 ± 0.21 . Lastly, this provides the first indication of a possible weakening of the N = 8 shell closure at the proton drip line.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Enhancing TREAT’s Pulsing Capabilities Using TREAT Upgrade Fuel

The Transient Reactor Test Facility (TREAT) at Idaho National Laboratory is an air-cooled, thermal, heterogeneous facility used to test reactor materials in simulated accident conditions by inducing fission heating with intense neutron pulses. TREAT operated from 1959 until 1994 with the primary goal of testing fast reactor fuels and was brought back online in 2017 to re-establish DOE's nuclear fuels transient testing capabilities. Beginning in the late 1970s, Idaho National Laboratory worked in conjunction with other organizations to increase TREAT's capability for in-pile testing. While these upgrades had not been implemented by the time the reactor was put into standby mode, new assemblies and graphite-urania fuel blocks with increased uranium concentrations had already been designed and fabricated. This project, as part of Idaho National Laboratory's Department of Reactor Physics, modeled the TREAT Upgrade (TU) fuel assemblies in MCNP and implemented them in an existing TREAT model. Calculations were performed using INL's high performance computer to find a critical combination of TU and standard fuel and this geometry's excess reactivity. Future work will include calculating a power coupling factor in the experiment, determining power peaking factors throughout the core, and assessing how much reactivity would be added by replacing the Inconel-625 cladding with silicon carbide.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Enhancing TREAT's pulsing abilities using TREAT upgrade fuel. SULI Intern Report

The Transient Reactor Test Facility (TREAT) at Idaho National Laboratory is an air-cooled, thermal, heterogeneous facility used to test reactor materials in simulated accident conditions by inducing fission heating with intense neutron pulses. TREAT operated from 1959 until 1994 with the primary goal of testing fast reactor fuels and was brought back online in 2017 to re-establish DOE’s nuclear fuels transient testing capabilities. Beginning in the late 1970s, Idaho National Laboratory worked in conjunction with other organizations to increase TREAT’s capability for in-pile testing. While these upgrades had not been implemented by the time the reactor was put into standby mode, new assemblies and graphite-urania fuel blocks with increased uranium concentrations had already been designed and fabricated. This project, as part of Idaho National Laboratory’s Department of Reactor Physics, modeled the TREAT Upgrade (TU) fuel assemblies in MCNP and implemented them in an existing TREAT model. Calculations were performed using INL’s high performance computer to find a critical combination of TU and standard fuel and this geometry’s excess reactivity. Future work will include calculating a power coupling factor in the experiment, determining power peaking factors throughout the core, and assessing how much reactivity would be added by replacing the Inconel-625 cladding with silicon carbide.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Electron scattering and neutrino physics

Abstract A thorough understanding of neutrino–nucleus scattering physics is crucial for the successful execution of the entire US neutrino physics program. Neutrino–nucleus interaction constitutes one of the biggest systematic uncertainties in neutrino experiments—both at intermediate energies affecting long-baseline deep underground neutrino experiment, as well as at low energies affecting coherent scattering neutrino program—and could well be the difference between achieving or missing discovery level precision. To this end, electron–nucleus scattering experiments provide vital information to test, assess and validate different nuclear models and event generators intended to test, assess and validate different nuclear models and event generators intended to be used in neutrino experiments. Similarly, for the low-energy neutrino program revolving around the coherent elastic neutrino–nucleus scattering (CEvNS) physics at stopped pion sources, such as at ORNL, the main source of uncertainty in the evaluation of the CEvNS cross section is driven by the underlying nuclear structure, embedded in the weak form factor, of the target nucleus. To this end, parity-violating electron scattering (PVES) experiments, utilizing polarized electron beams, provide vital model-independent information in determining weak form factors. This information is vital in achieving a percent level precision needed to disentangle new physics signals from the standard model expected CEvNS rate. In this white paper, we highlight connections between electron- and neutrino–nucleus scattering physics at energies ranging from 10 s of MeV to a few GeV, review the status of ongoing and planned electron scattering experiments, identify gaps, and lay out a path forward that benefits the neutrino community. We also highlight the systemic challenges with respect to the divide between the nuclear and high-energy physics communities and funding that presents additional hurdles in mobilizing these connections to the benefit of neutrino programs.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

How to make Progress with North Korea Now

In early 2017 the United States should have taken up the Chinese and Russian-backed proposal to suspend United States – South Korean joint military exercises in exchange for suspension of North Korean nuclear and missile tests. South Korea was signaling that it would support this proposal. That was before North Korea tested inter-continental ballistic missiles (ICBMs), capable of reaching anywhere in the U.S., and an advanced nuclear explosive, some ten times more powerful than those the U.S. used against Japan in WWII. The Trump administration brushed aside that original international proposal. The Singapore Summit, however, has put just such a suspension-for-suspension agreement in place. A little late, but much better than never.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

Seismic moment tensor classification using elliptical distribution functions on the hypersphere

Discrimination of underground explosions from naturally occurring earthquakes and other anthropogenic sources is one of the fundamental challenges of nuclear explosion monitoring. In an operational setting, the number of events that can be thoroughly investigated by analysts is limited by available resources. The capability to rapidly screen out events that can be robustly identified as not being explosions is, therefore, of great potential benefit. Nevertheless, possible mis-classification of explosions as earthquakes currently limits the use of screening methods for verification of test-ban treaties. Moment tensors provide a physics-based classification tool for the characterization of different seismic sources and have enabled the advent of new techniques for discriminating between earthquakes and explosions. Following normalization and projection of their six-degree vectors onto the hypersphere, existing screening approaches use spherically symmetric metrics to determine whether any new moment tensor may have been an explosion. Here, we show that populations of moment tensors for both earthquakes and explosions are anisotropically distributed on the hypersphere. Distributions possessing elliptical symmetry, such as the scaled von Mises–Fisher distribution, therefore provide a better description of these populations than the existing spherically symmetric models. We describe a method that uses these elliptical distributions in combination with a Bayesian classifier to achieve successful classification rates of 99 per cent for explosions and 98 per cent for earthquakes using existing catalogues of events from the western United States. The 1983 May 5 Crowdie underground nuclear test and 2018 July 20 DAG-1 deep-borehole chemical explosion are the only two explosions out of 140 that are incorrectly classified. Application of the method to the 2006–2017 nuclear tests in the Democratic People’s Republic of Korea yields 100 per cent identification rates and we provide a simple routine MTid for general usage. The approach provides a means to rapidly assess the likelihood of an event being an explosion and can be built into monitoring workflows that rely on simultaneously assessing multiple different discrimination metrics.

58 GEOSCIENCES↗

The Fission Accelerated Steady State Test (FAST) -- A Revised Capsule Design for the Accelerated Testing of Advanced Reactor Fuels

In an effort to improve the development and testing of novel nuclear fuels, a detailed evaluation on reducing the size of fuel specimens for irradiation has been performed. Theoretically speaking, reducing the fuels diameter and incorporating an inner capsule while maintaining the original outside diameter of the experiment significantly reduces the experiment’s sensitivity to fabrication tolerances and drastically reduces the time necessary to reach a desired fuel burnup; both of which improve the cost and schedule associated with the fuel testing. Simulations of this reduced diameter, double encapsulated concept have been performed using Abaqus, MCNP, and ORIGEN. The results of the Abaqus simulations are beyond the scope of this summary and will not be presented herein. For results of these Abaqus simulations, see Beausoleil [2]. The models were tested using various parameters and design deviations which were then compared to the original Advanced Fuels Campaign (AFC) designs. The results of these simulations confirmed that the introduction of a second capsule coupled to a reduction in the fuel pin diameter significantly reduces the experiment’s sensitivity to fabrication tolerances and reduces the time to reach a desired burnup by nearly an order of magnitude. The original AFC design requires approximately 11.7 years to reach 30 Atom % Heavy Metal (at% HM) burnup. A burnup of 30 at% HM can be reached in approximately 2.5 to 3.5 years (irradiation position dependent) with a fuel diameter ½ (~0.097 in. diameter) that of the original AFC design. An added benefit to the fuel pin diameter reduction is that more specimens can be irradiated in any given cycle. Essentially, significantly more specimens can be tested and incur more burnup over a given operating cycle relative to the AFC design. This allows the development of a large test matrix of samples with rapid throughput in ATR.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Experimental test of the ratio method for nuclear-reaction analysis

Nuclear halos are exotic quantal structures observed far from stability. They are mostly studied through reactions. The ratio of angular cross sections for breakup and scattering is predicted to be independent of the reaction process and to be very sensitive to the halo structure. We test this new observable experimentally for the first time on the collision of 11 Be on C at 22.8 MeV/nucleon and using existing data on Pb at 19.1 MeV/nucleon. The theoretical predictions are verified, which offers the possibility to develop a new spectroscopic tool to study nuclear structure far from stability.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Experimental Test of the Ratio Method for Nuclear-Reaction Analysis

Nuclear halos are exotic quantal structures observed far from stability. They are mostly studied through reactions. The ratio of angular cross sections for breakup and scattering is predicted to be independent of the reaction process and to be very sensitive to the halo structure. Here, we test this new observable experimentally for the first time on the collision of 11 Be on C at 22.8 MeV/nucleon and using existing data on Pb at 19.1 MeV/nucleon. The theoretical predictions are verified, which offers the possibility of developing a new spectroscopic tool to study nuclear structure far from stability.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Materials and Fuels Complex FY-22 – FY-26 Five-Year Mission Strategy

The Idaho National Laboratory (INL), through its designated mission of advancing innovative nuclear energy solutions, is actively engaged in the research, development, demonstration and deployment of advanced nuclear technology. Key to the success of INL’s mission is the Materials and Fuels Complex (MFC), the only complex in the U.S. that hosts a world-class assemblage of facilities, capabilities and instruments for handling, testing, and characterizing nuclear fuel and radioactive materials. Driven by its mission/vision of “Engineering and Experiments that Drive the World’s Nuclear Energy Future,” MFC is at the center of INL’s – and indeed the Department of Energy’s – advanced nuclear technology development initiatives, providing essential capabilities such as research-scale high-assay low-enriched uranium (HALEU) fuel production, reactor demonstration facilities, post-irradiation examination, and transient irradiation testing. Furthermore, MFC provides an ideal environment for test beds that are utilized for research, development and demonstration (RD&D) activities on used fuel treatment, nuclear non-proliferation, forensics, and nuclear power sources used for space exploration missions conducted by the National Aeronautics and Space Administration (NASA).

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Characterizing The Mechanical Properties of Polyurethane Foams

The Department of Energy has many radioactive facilities that are on the path of deactivation and decommissioning (D and D). These facilities can sit cold and dark for many years before final disposition, and must be maintained to ensure no radiological release occurs in the interim. Improvements and additions to D and D tool sets can greatly: Save time and money, Reduce worker risk. Conventional fixatives widely used often take the form of paints or films that are not readily applicable to 3-dimensional void spaces. Foams are one promising platform that may offer solutions to a number of contaminated problem sets such as: Gloveboxes, Pipes, Tanks. SRNL is working to characterize various commercial foams that would encapsulate the interior volume of a given space and are capable of immobilizing any remaining contamination. One key performance metric of these foams is how well they will perform in an accident scenario. To this end, SRNL is researching the mechanical properties of these foams to ensure that the material can withstand the environment of application while maintaining structural integrity. ASTM standard E3191-18 served as a guiding document for this project, outlining the requirements that foaming fixatives used for the mitigation of radioactive contamination need to meet before being implemented. Objective: Quantification of the mechanical properties of 6 commercial polyurethane foams was performed using multiple ASTM standards to record measurements for: Compression testing: Flexible Foams, Force required to produce 50% compression, Rigid Foams, Compressive and apparent modulus, Point of 10% core deformation, The 'Zero Deformation' point, Compressive strength, Yield point. Tensile testing: Tensile strength, Tensile stress, Percent elongation. Experiment 1: An electromechanical compressive tester (MTS Criterion Series 43) was used to evaluate 6 foams (4 flexible, 2 rigid). Per ASTM D1621, each rigid foam was compressed at 10% of the measured thickness per minute until the sample was 13% of it's original thickness. Per ASTM D35/4, each flexible foam was pre-flexed twice to 80% original thickness at a rate of 250 mm/min, then compressed to 80% original thickness at a rate of 50 mm/min. Experiment 2: An electromechanical tensile tester (MTS Criterion Series 43) was used to evaluate 6 foams (4 flexible, 2 rigid). Per ASTM D1623, rigid foams were pulled apart at a rate of 1.27 mm/min until the sample broke. Per ASTM D35/4, flexible foams were pulled apart at a rate of 500 mm/min until the sample broke. The strongest material in both compression and tensile testing scenarios was found to be the rigid intumescent polyurethane Hilti foam. The experiments revealed that the Hilti foam in a tensile scenario had a peak stress value that was larger than the closest competitor by a factor of 2.3 and a compressive yield point that was larger than the closest competitor by a factor of 1.4, indicating that the Hilti foam is the best choice for implementation in mechanically harsh environments. The performance metrics measured can serve as a basis for future mechanical tests that would help set relevant ASTM standards (E3191) for intumescent polyurethane foams in fixating applications. Tests like surface adhesion, impact, and flame tests would serve as a better indicator as to how this material would perform in environmentally harsh scenarios often found in decommissioned nuclear facilities. Further tests of the foams' intumescent properties would also be important should these foams be implemented in environmentally harsh scenarios.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

How to achieve patient-centered testing: role of the protocol nurse

Introduction: Patient-centered cardiac testing is predicated on choosing the right test for the right patient. We studied the effects of changing from script-driven scheduling to nurse-driven protocoling of stress tests. Methods and Results: A protocol nurse reviewed records before scheduling and communicated with patients and ordering providers if needed. We found that instituting nurse protocolling of all non-imaging (ETT) and nuclear (MPI) stress tests (N = 3071) resulted in protocol changes in 37% of our patients, and reduced the proportion of tests that could not be performed as scheduled by 56% and cancelations by 71% (P < 0.001 for each). These changes were sustained over two successive 6-month periods following a baseline observation period of 6 months. For MPI, the most frequent nurse interventions were re-protocoling as stress-first MPI (12% of tests), changing test location for clinical reasons (13%), changing stress modality (7%), and care coordination (5%). Conclusions: Changing from script-driven scheduling to protocol nursing contributed measurably to patient-centered testing.

62 RADIOLOGY AND NUCLEAR MEDICINE↗