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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 919 records · Page 51
All sourcesNASA NTRSDOE OSTI
DOE OSTI2016

Aging of Black Carbon during Atmospheric Transport: Understanding Results from the DOE's 2010 CARES and 2012 ClearfLo Campaigns

Over the course of this project, we have analyzed data and samples from the CARES and ClearfLo campaigns, as well as conducted or participated in laboratory experiments designed to better understand black carbon mixing state and climate-relevant properties. The laboratory campaigns took place at PNNL and CMU to study various climate-relevant aerosol properties of different sources of soot mixing with secondary organic aerosol precursors. The DMT photoacoustic extinctiometers (PAXs) procured by CMU through this grant were deployed for these experiments, as well as experiments characterizing the optical properties of cookstove soot emissions at Colorado State University (CSU). Results from some of these activities were summarized in the previous progress report. This final report presents the manuscripts that have been published (many in the period since the last progress report), lists presentations at different conferences based on grant-related activities, and presents some results that are likely to be submitted for publication in 2016.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2019

Competing Orders in Correlated Materials: Impact of Disorder and Non-Equilibrium Perturbationsn (Final Report)

The goal of this project was to explore, understand, and ultimately control the competing electronic ordered states ubiquitously present in correlated materials, with particular emphasis in unconventional superconductors, such as iron based and copper based materials. While on the one hand the competition with different types of magnetic, orbital, and charge order limits the transition temperatures of these unconventional superconductors, on the other hand the enlarged ground state degeneracy associated with these multiple many body instabilities can give rise to unusual inhomogeneous correlated normal states, such as electronic smectic and nematic phases. To achieve the aforementioned goals, we employed a multi faceted theoretical approach consisting of: (i) The investigation of relatively unexplored regimes with the potential to unveil novel behaviors – in particular, the study of competing phases taken out of equilibrium to explore the potential to enhance the transition temperatures of unconventional superconductors by optical pulses. (ii) The embracement of realistic features of correlated materials in their microscopic descriptions – in particular, the investigation of the impact that disorder, in its various forms, has on competing and emergent inhomogeneous states present in the phase diagrams of unconventional superconductors. (iii) The promotion of synergy with established and novel experimental probes (with particular emphasis on scanning tunneling microscopy and ultrafast spectroscopy) not only by using data as input of theoretical models, but also by providing concrete guidance for experiments. Selected highlights include: the development of a unifying model to explain the rich landscape of electronic ordered phases observed in iron-based superconductors; the demonstration, in concrete settings, of how disorder and optical pulses can be used to tilt the balance between competing orders; the development and application of the concept of vestigial orders beyond electronic nematicity; the elucidation of nematic properties of several correlated systems, such as iron pnictides, iron chalcogenides, cuprates, f-electron systems, and nickel arsenides. Overall, significant progress in the understanding of competing and emergent states in correlated materials was achieved during this award, providing promising avenues to control and tune the different types of electronic orders observed in their phase diagrams.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2021

Developing and Testing a Novel Stochastic Ice Microphysics Parameterization for Cloud and Climate Models Using ARM Field Campaign Data (Final Progress Report)

The major goals of this project were: 1) to use field campaign measurements from DOE’s Atmospheric Radiation Measurement (ARM) program to characterize variability of important parameters describing properties of ice particles in the atmosphere; 2) based on this observational analysis, to develop a parameterization scheme for weather and climate models that stochastically varies these parameters, and implement the new scheme into a weather model called the Weather Research and Forecasting model (WRF); 3) to use WRF coupled with the new stochastic scheme to simulate ARM field campaign thunderstorm cases and analyze how accounting for this parameter variability affects the model simulations. This work was performed jointly between the National Center for Atmospheric Research, University of Oklahoma, and University of Utah. To accomplish these goals, we extended an approach previously developed to characterize the variability in the size distribution of ice particles to parameters that are explicitly represented in models (i.e., relationships between ice particle mass and size, and between particle fall velocity and size). Our project was, to our knowledge, the first to apply observationally-constrained estimates of this parameter variability describing mass-size and fall velocity-size in a modeling framework. Our results showed efficacy of the approach, evaluated using ARM observations. Similarly, to our knowledge, work in this project was the first to propose and evaluate in detail a stochastic approach for unresolved turbulent mixing in high-resolution model simulations against detailed, benchmark large eddy simulations and ARM observations. Results showed some promising behavior, particularly with increased mixing and dilution of air in thunderstorm cores with surrounding environmental air, bringing the stochastic simulations closer to the benchmark large eddy simulations; however, results were somewhat degraded using stochastic mixing compared to observations from the AMIE/DYNAMO field campaign. This project also further refined and applied a modeling methodology called “piggybacking” that can robustly separate dynamical and thermodynamic impacts of model changes, and comparison studies of different models based on cases developed from ARM observations. Finally, this project directly supported three graduate students who completed their PhDs as well as a postdoctoral research fellow.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2019

Carbon Storage and Enhanced Oil Recovery in Pennsylvanian Morrow Formation Clastic Reservoirs: Controls on Oil–Brine and Oil–CO2 Relative Permeability from Diagenetic Heterogeneity and Evolving Wettability

The efficiency of carbon utilization and storage within the Pennsylvanian Morrow B sandstone, Farnsworth Unit, Texas, is dependent on three-phase oil, brine, and CO2 flow behavior, as well as spatial distributions of reservoir properties and wettability. We show that end member two-phase flow properties, with binary pairs of oil–brine and oil–CO2, are directly dependent on heterogeneity derived from diagenetic processes, and evolve progressively with exposure to CO2 and changing wettability. Morrow B sandstone lithofacies exhibit a range of diagenetic processes, which produce variations in pore types and structures, quantified at the core plug scale using X-ray micro computed tomography imaging and optical petrography. Permeability and porosity relationships in the reservoir permit the classification of sedimentologic and diagenetic heterogeneity into five distinct hydraulic flow units, with characteristic pore types including: macroporosity with little to no clay filling intergranular pores; microporous authigenic clay-dominated regions in which intergranular porosity is filled with clay; and carbonate–cement dominated regions with little intergranular porosity. Steady-state oil–brine and oil–CO2 co-injection experiments using reservoir-extracted oil and brine show that differences in relative permeability persist between flow unit core plugs with near-constant porosity, attributable to contrasts in and the spatial arrangement of diagenetic pore types. Core plugs “aged” by exposure to reservoir oil over time exhibit wettability closer to suspected in situ reservoir conditions, compared to “cleaned” core plugs. Together with contact angle measurements, these results suggest that reservoir wettability is transient and modified quickly by oil recovery and carbon storage operations. Reservoir simulation results for enhanced oil recovery, using a five-spot pattern and water-alternating-with-gas injection history at Farnsworth, compare models for cumulative oil and water production using both a single relative permeability determined from history matching, and flow unit-dependent relative permeability determined from experiments herein. Both match cumulative oil production of the field to a satisfactory degree but underestimate historical cumulative water production. Differences in modeled versus observed water production are interpreted in terms of evolving wettability, which we argue is due to the increasing presence of fast paths (flow pathways with connected higher permeability) as the reservoir becomes increasingly water-wet. The control of such fast-paths is thus critical for efficient carbon storage and sweep efficiency for CO2-enhanced oil recovery in heterogeneous reservoirs.

Rasmussen, Lindsey↗
NASA NTRS1974

Convergence properties of simple genetic algorithms

The essential parameters determining the behaviour of genetic algorithms were investigated. Computer runs were made while systematically varying the parameter values. Results based on the progress curves obtained from these runs are presented along with results based on the variability of the population as the run progresses.

Bethke, A. D.↗
NASA NTRS1984

Fuel system research and technology: An overview of the NASA program

The interactions between the design and operation of aircraft fuel systems and the properties of alternative aircraft fuels are discussed. An overview of fuels system research and technology in terms of its rationale, its progress, and future plans is given. The measurement of ambient air temperatures for a wide range of seasonal and geographic variations, design studies on the use of fuels with increased as well as conventional freezing temperatures, the evaluation of fuel heating systems, and the low temperature behavior of fuels are among the topics discussed.

Phillips, B. R.↗
NASA NTRS1984

Vertical and horizontal characteristics of Arctic haze during AFASP - Alaskan Arctic

Vertical and horizontal distributions of ozone, extinction due to aerosol light scattering, condensation nucleus concentrations, aerosol spectra, and meteorological parameters were measured with a NOAA WP-3D research aircraft over the Alaskan Arctic in March 1983. Multiple layers of haze, varying in thickness from a few 10's to 100's of meters, were observed throughout the troposphere. A maximum concentration of aerosols was located between 600 and 800 mb. Distribution of the haze layers was associated with distinct meteorological boundaries. The characteristics of the haze changed in response to stages in the progression of a major Arctic haze episode. On March 17, 1983, the Arctic anticyclone was penetrated and its meteorological and aerosol properties determined.

Schnell, R. C.↗
NASA NTRS1994

Formation and evolution of luminous supersoft X-ray sources

Luminous supersoft X-ray sources, with characteristic luminosities of approximately 10(exp 38) ergs/s and temperatures, kT, of approximately 35 eV, have been established as a new and distinct class of X-ray source through recent Roentgen Satellite (ROSAT) observations. Several possible physical models have been proposed for these sources. One promising scenario (van den Heuvel et al. 1992) involves mass transfer, which is unstable on a thermal timescale, from a main-sequence or subgiant donor star onto the surface of a white dwarf. For a narrow range of accretion rates, steady nuclear burning of the accreted matter can take place. This process can provide the high luminosities and the correct range of temperatures observed in the supersoft sources. However, given the limited range of mass transfer rates that are consistent with this phenomenon, it is far from obvious that a sufficient population of such systems exists in galaxies such as our own, M31, and the Magellanic Clouds, in order to account for the large number of supersoft sources which can be inferred from present observations. This work addresses the population question in detail, through a Monte Carlo simulation of the formation and evolution of such systems, which starts with zero-age primordial binaries. In order to evolve into close binary systems which contain a white dwarf component and a companion transferring mass at a rate within the requisite narrow range, a binary system must undergo a specific progression of evolutionary steps. We find that a sufficient subset of our initial binaries evolve to become systems with the requisite properties, so that they can account for the population of supersoft sources that is inferred from observations. In particular, we find that there should be more than 1000 systems in the Galaxy today with properties that very closely match those of the observed supersoft sources. From our models, we find expected luminosities, white dwarf effective temperatures, and orbital periods in the ranges of 10(exp 37) - 10(exp 38) ergs/s, (1-5) x 10(exp 5) K, and 8 hr-1.4 days, respectively. The masses of the white dwarf and donor star are expected to lie in the range of 0.7-1.05 solar mass and 1.3-2.7 solar mass. Finally, we discuss the role that supersoft X-ray sources may play as the progenitors of Type Ia supernovae, and estimate the rate of production via this channel.

Rappaport, S.↗
NASA NTRS1996

Experiments with Lasers and Frequency Doublers

Solid state laser sources, such as diode-pumped Nd:YAG lasers, have given us CW laser light of high power with unprecedented stability and low noise performance. In these lasers most of the technical sources of noise can be eliminated allowing them to be operated close to the theoretical noise limit set by the quantum properties of light. The next step of reducing the noise below the standard limit is known as squeezing. We present experimental progress in generating reliably squeezed light using the process of frequency doubling. We emphasize the long term stability that makes this a truly practical source of squeezed light. Our experimental results match noise spectra calculated with our recently developed models of coupled systems which include the noise generated inside the laser and its interaction with the frequency doubler. We conclude with some observations on evaluating quadrature squeezed states of light.

Bachor, H.-A.↗
NASA NTRS2008

User-defined Material Model for Thermo-mechanical Progressive Failure Analysis

Previously a user-defined material model for orthotropic bimodulus materials was developed for linear and nonlinear stress analysis of composite structures using either shell or solid finite elements within a nonlinear finite element analysis tool. Extensions of this user-defined material model to thermo-mechanical progressive failure analysis are described, and the required input data are documented. The extensions include providing for temperature-dependent material properties, archival of the elastic strains, and a thermal strain calculation for materials exhibiting a stress-free temperature.

Knight, Norman F., Jr.↗
NASA NTRSDate not supplied

Cavitation Effects on the Structural Dynamics of Turbomachinery Components

The structural integrity of inducer and impeller blades in rocket engine turbomachinery must be evaluated in the face of complex excitation mechanisms including fluctuating pressures due to cavitation. Cavitation occurs when the local fluid pressure drops below the vapor pressure, causing the formation of vapor-filled bubbles. Cavitation can exist to various extents within the typical operating range of rocket engine turbopumps. Despite recent progress towards reducing uncertainties in structural dynamic models of turbomachinery components, the extent to which pump cavitation affects the structural dynamic properties (i.e., natural frequencies, damping, and mode shapes) of inducer and impeller blades remains largely unknown. To study the structural dynamic effects of cavitating flows, experiments are conducted in a high-speed water tunnel. The test articles mimic a single inducer blade that is unwrapped from the hub, thus resembling a low aspect ratio cantilevered plate. To induce cavitation, the plates are oriented at a non-zero angle of attack and have rough strips near their leading edges. To control the extent of cavitation, the static pressure of the water tunnel is controlled between roughly 0.5 and 1.5 atm. A high-speed camera is used to quantify the coverage of the cavitations heet. The sheet coverage is then correlated to changes in fluid-added mass and hydroelstic damping. In addition, a corresponding two-way coupled CFD/FE model is under development for test/analysis correlation.

Ben Davis↗
NASA NTRSDate not supplied

Cavitation Effects on the Structural Dynamics of Turbomachinery Components

The structural integrity of inducer and impeller blades in rocket engine turbomachinery must be evaluated in the face of complex excitation mechanisms including fluctuating pressures due to cavitation. Cavitation occurs when the local fluid pressure drops below the vapor pressure, causing the formation of vapor-filled bubbles. Cavitation can exist to various extents within the typical operating range of rocket engine turbopumps. Despite recent progress towards reducing uncertainties in structural dynamic models of turbomachinery components, the extent to which pump cavitation affects the structural dynamic properties (i.e., natural frequencies, damping, and mode shapes) of inducer and impeller blades remains largely unknown. To study the structural dynamic effects of cavitating flows, experiments are conducted in a high-speed water tunnel. The test article is a low aspect ratio cantilevered plate, thus mimicing a single inducer blade that is unwrapped from its hub. The test article is oriented at zero angle of attack and has a triangular trip at its leading edge to induce cavitation. To change the extent of cavitation, the static pressure of the water tunnel is controlled. A high-speed camera is used to quantify the coverage of the cavitation sheet.

Fluid-Structure Interaction↗
DOE OSTI2016

Battery Thermal Characterization

This poster shows the progress in battery thermal characterization over the previous year. NREL collaborated with U.S. DRIVE and USABC battery developers to obtain thermal properties of their batteries, obtained heat capacity and heat generation of cells under various power profiles, obtained thermal images of the cells under various drive cycles, and used the measured results to validate thermal models. Thermal properties are used for the thermal analysis and design of improved battery thermal management systems to support achieve life and performance targets.

25 ENERGY STORAGE↗
DOE OSTI2018

Feasibility of a Deep Direct-Use Geothermal System at the University of Illinois Urbana-Champaign

This study assesses the feasibility of using deep direct-use (DDU) geothermal energy in agricultural research facilities on the University of Illinois at Urbana-Champaign campus to exploit low-temperature sedimentary basins, such as the Illinois Basin. Subsurface components of the system include extraction and injection wells and downhole pumps. Surface equipment includes heat pumps/exchangers, and fluid transport and monitoring systems. Two geologic formations in the region exhibit a potential as sources for geothermal energy, based on pre initial temperatures and flow rates of fluids. The St. Peter and Mt. Simon Sandstones lie at depths of 634 and 1,280 m, respectively. Geocellular modeling is used to characterize the reservoirs. A St. Peter Sandstone model was made for an area south of the campus. Petrophysical and geothermal properties used are based on data from the closest wells penetrating the formations. Characterization of the Mt. Simon Sandstone is in progress and is not discussed here. Extraction and injection flows simulated with different wellbore configurations provide estimates of fluid flow out of and into the reservoir. The models are used to optimize flow rates, bottomhole pressure, and temperature of the produced fluid. Individual wellbore models simulate subsurface heat loss and gain, providing guidance on the optimal type and amount of insulation in the wellbore. Design of the surface facilities will address aspects of fluid delivery, heat exchange, capital operating costs, heat loss, and corrosion. Heat capacity and flow rates are assessed to estimate life-cycle costs and benefits, including the environmental benefits of reducing greenhouse gases and water use and increased energy efficiency. A preliminary analysis of surface configurations for the DDU system (including cascading applications) based on building heat loads is being conducted to identify multiple system designs that will maximize performance, energy efficiency, and cost recovery.

15 GEOTHERMAL ENERGY↗
DOE OSTI2017

Weld Development of FeCrAl Thin-Wall Cladding for LWR Accident Tolerant Fuel

The development of new cladding materials to replace Zr-based cladding for light water reactors (LWRs) has been actively pursued with improved high-temperature oxidation resistance to significantly suppress hydrogen production from an accident such as a loss of coolant event. FeCrAl alloy with a typical composition of approximately Fe-15Cr-5Al has been selected as a candidate material because of its improved high-temperature oxidation resistance over the present LWR zircaloy cladding. As a result of higher thermal neutron absorption for FeCrAl alloy, the cladding wall thickness needs to be reduced by approximately half compared to that of Zircaloy cladding to be comparable to the current LWR fuel performance under the normal operating condition. New weld techniques for joining the endplug to thin-walled cladding need to be developed. Both laser beam weld and pressure resistance weld were employed. This paper summarizes the recent progress on the laser weld development for FeCrAl cladding with 350 µm wall thickness. The results of microstructural characterization and mechanical property testing of the weld for the cladding-endplug set are discussed.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2020

Advancement of Commercial Intumescent Expanding Foams for Deactivation and Decommissioning in the Nuclear Sector - 20198

Florida International University (FIU), in collaboration with The Department of Energy's Office of Environmental Management (DOE-EM), Savannah River National Laboratory (SRNL), and sites across the Savannah River complex, have identified an operational requirement for a fixative technology that is intended to immobilize and/or isolate residual contamination within a 3-dimensional space. Fixation of radiological contamination can reduce worker risk and mitigate potentially hazardous conditions, however nearly every marketed contamination fixative has been found to be flammable; a significant concern in radiological facilities. Coupled with this, industry fixatives are normally used as a thin coating which can present problems when attempting to stabilize irregular geometry or areas that are difficult to access whilst ensuring full coverage. The technical evaluation and advancement of commercial-off-the-shelf (COTS) polyurethane foams has yielded a down-selected candidate that shows potential in meeting the requirements to support deactivation and decommissioning activities. Several performance criteria have been established and tested to progress the technology readiness level towards an active field demonstration (TRL-7). Such criteria include: mechanical failure limits, adhesive and cohesive properties, thermal/fire resilience, determining thermal behavior, ability to immobilize contamination, and a means of non-destructive evaluation of applications. The test scenario examined was targeted towards an application for decommissioning nuclear pipework, in which the down-selected polyurethane foam would act as a barrier to segregate pipework and mitigate the potential for release during cutting, packaging, and storage operations. Testing carried out at SRNL included: mechanical evaluation of tensile, compressive, and adhesion strength by dynamic mechanical analysis (DMA), as well as thermogravimetric analysis (TGA). FIU examined the foam's fixative properties by utilizing phosphorescent europium-dysprosium doped strontium aluminate powder to investigating the extent to which contamination can be immobilized. FIU has also exploited previous successes in the field of intumescent technologies to assess the down-selected foam's tolerance to an extreme fire scenario, while maintaining the ability to effectively mitigate a contamination release. Parallel to this, extensive thermal investigations were carried out to determine the upper boundary of anticipated heat generation during the curing process as heat generation has the potential to compromise rubber parts of contaminated enclosures. These investigations subsequently yielded a promising method for a non-destructive application evaluation by means of infrared thermography. Utilizing the high sensitivity of modern IR cameras, coupled with the heat generated during the curing process of the polyurethane foam, FIU has been exploring the concept of monitoring the external pipe surface for indications of an irregular or abnormal application, thus informing operational decision making. The testing carried out utilized several current 'best fit' ASTM standards, which serve as helpful guidelines for testing, however, a precise definition of the operational parameters and requirements is still necessary. With continued collaboration with SRNL, FIU aims refine said definitions and develop new standards by which this, and other decommissioning technologies, can be accredited by relevant standards based testing. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
DOE OSTI2021

Recent progress and future prospects of atomic layer deposition to prepare/modify solid-state electrolytes and interfaces between electrodes for next-generation lithium batteries

Lithium ion batteries (LIBs) are encouraging electrochemical devices with remarkable properties including a high energy/power density, fast charging capability, and low self-discharge rate. Further increase in energy density as well as safe usage is needed for next-generation LIBs in electric transportation vehicles. Solid-state electrolytes (SSEs) are very promising for high-performance LIBs since they enable improved safety along with increased energy density compared to flammable liquid organic electrolytes. However, utilizing SSEs with a Li metal anode is very challenging due to the possibility of undesired side reactions and the formation of an unstable solid-electrolyte interphase. Therefore, it is critical to enhance the stability of SSEs against the Li anode. One feasible approach is to form a thin and conductive interlayer between the Li anode and solid-state electrolyte. Atomic layer deposition (ALD) is a unique technique for conformal coating of complex 3D structures with finely controlled film thickness (at the atomic scale). ALD coating on the surface of SSEs can be adopted for engineering solid-electrolyte interfaces with desired attributes and improved stability. In this review paper, we have discussed recent progress in implementing the ALD technique for depositing thin layers on various SSE configurations including lithium phosphorus oxynitride (LiPON), garnets, oxides, perovskites, sulphides, Li 3 BO 3 –Li 2 CO 3 (LBCO), and sodium super ionic conductors (NASICON). We have also highlighted the major areas for future research and development in the field. We believe that this review will be very helpful for directing future research on implementing ALD for synthesizing stable and high-performance SSEs with an engineered solid-electrolyte interface for next-generation electrochemical devices (e.g., Li-ion batteries, supercapacitors, and flow batteries).

36 MATERIALS SCIENCE↗
DOE OSTI2017

PIE of nuclear grade SiC/SiC flexural coupons irradiated to 10 dpa at LWR temperature

Silicon carbide fiber-reinforced SiC matrix (SiC/SiC) composites are being actively investigated for accident-tolerant core structures of light water reactors (LWRs). Owing to the limited number of irradiation studies previously conducted at LWR-coolant temperature, this study examined SiC/SiC composites following neutron irradiation at 230–340°C to 2.0 and 11.8 dpa in the High Flux Isotope Reactor. The investigated materials are chemical vapor infiltrated (CVI) SiC/SiC composites with three different reinforcement fibers. The fiber materials were monolayer pyrolytic carbon (PyC)-coated Hi-NicalonTM Type-S (HNS), TyrannoTM SA3 (SA3), and SCS-Ultra TM (SCS) SiC fibers. The irradiation resistance of these composites was investigated based on flexural behavior, dynamic Young’s modulus, swelling, and microstructures. There was no notable mechanical properties degradation of the irradiated HNS and SA3 SiC/SiC composites except for reduction of the Young’s moduli by up to 18%. The microstructural stability of these composites supported the absence of degradation. In addition, no progressive swelling from 2.0 to 11.8 dpa was confirmed for these composites. On the other hand, the SCS composite showed significant mechanical degradation associated with cracking within the fiber. This study determined that SiC/SiC composites with HNS or SA3 SiC/SiC fibers, a PyC interphase, and a CVI SiC matrix retain their properties beyond the lifetime dose for LWR fuel cladding at the relevant temperature.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗